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JAERI 1287 JNDC Nuclear Data Library of Fission Products Fir

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18 <strong>JNDC</strong> <strong>Nuclear</strong> <strong>Data</strong> <strong>Library</strong> <strong>of</strong> <strong>Fission</strong> <strong>Products</strong> <strong>JAERI</strong> <strong>1287</strong><br />

very good.<br />

In a critical reactor, a neutron <strong>of</strong> energy E, is required to perpetuate the chain reaction.<br />

This reduces the average total energy released directly in the fission process to a net value<br />

Q'r = Qf-Ei. (2.5.7)<br />

The effective average total energy Q/(°°) absorbed in the reactor is the value Q'f substracted<br />

by the amount Ea because <strong>of</strong> the low absorption probability <strong>of</strong> antineutrinos in the reactor;<br />

QA°°)=Q'/-Ee. (2.5.8)<br />

Also, the quantities End, Erd, £/?and Ea are time-dependent, and the full magnitude <strong>of</strong> the<br />

latter three quantities is not realized for practicable irradiation and cooling times in a reactor.<br />

This in turn changes the effective average total energy resulting directly from fission so that<br />

where, AEa = AQfi-(AErd+AE^,<br />

Qp - average Q value for beta decay.<br />

Therefore, Qe// can be rewritten as<br />

Qe//=Q'/-Ea+{AQ/3-2(AErd + AEl3)}, (2.5.9)<br />

where the energies AQp, AE0 and AErd depend on the irradiation history <strong>of</strong> the reactor. In<br />

addition to Qe// , energy Qc is liberated by the capture <strong>of</strong> the remaining (v—l) neutrons in<br />

the reactor materials. This latter energy depends on the neutron energy spectrum and the<br />

arrangement, amount, and constituent <strong>of</strong> reactor materials.<br />

Finally the total energy QT released in fission and absorbed in a reactor is given by<br />

Qr=Qeff + Qc (2.5.10)<br />

The quantity Q'f, the net average energy released directly from the fission process, has<br />

been calculated for various fissioning systems with known complete mass-yield distributions<br />

by using: (1) Eqs. 2.5.6 and 2.5.7', (2) the fission product (FP) atomic masses in the Tables <strong>of</strong><br />

Isotopes and (3) fission mass-yield distributions compiled by Rider and Meek 41) . To compare<br />

the energy release Q'f calculated from nuclear masses with that obtained by summation <strong>of</strong> the<br />

Target<br />

Nuclide<br />

235 U<br />

235 U<br />

235 U<br />

238 U<br />

238 U<br />

239pu<br />

239pu<br />

24lpu<br />

233 u<br />

232Th<br />

Neutron<br />

Energy<br />

t a<br />

fb<br />

h c<br />

f<br />

h<br />

t<br />

f<br />

t<br />

t<br />

f<br />

Table 2.5.1 Q'f calculated from nuclear masses<br />

Target<br />

Mass Excess<br />

MeV<br />

40.92<br />

40.92<br />

40.92<br />

47.31<br />

47.31<br />

48.59<br />

48.59<br />

52.95<br />

36.91<br />

35.45<br />

a thermal neutrons.<br />

b fission spectrum neutrons.<br />

c 14-MeV neutrons.<br />

d data from Ref. 52.<br />

FP<br />

Mass Excess<br />

MeV<br />

-173.23<br />

-173.25<br />

-173.97<br />

-173.24<br />

-173.72<br />

-173.68<br />

-173.50<br />

-173.47<br />

-173.20<br />

-173.02<br />

d<br />

V<br />

2.4229 ±0.0066<br />

2.52 ±0.02<br />

4.46 ±0.10<br />

2.81 ±0.05<br />

4.31 ± 0.08<br />

2.8799 ±0.0090<br />

3.01 ±0.05<br />

2.934 ±0.0012<br />

2.4866 ±0.0069<br />

2.36 ±0.07<br />

(v— 1 )«,<br />

MeV<br />

11.48<br />

12.27<br />

27.93<br />

14.61<br />

26.72<br />

15.17<br />

16.22<br />

15.61<br />

12.00<br />

10.98<br />

y /<br />

MeV<br />

202.67<br />

201.90<br />

201.96<br />

205.94<br />

194.31<br />

207.10<br />

205.87<br />

210.81<br />

198.11<br />

196.49

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