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Evaluating the Impacts of Aviation on Climate Change - Pa.op.dlr.de

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Eos, Vol. 88, No. 14, 3 April 2007<br />

EOS, TRANSACTIONS, AMERICAN GEOPHYSICAL UNION<br />

<str<strong>on</strong>g>Evaluating</str<strong>on</strong>g> <str<strong>on</strong>g>the</str<strong>on</strong>g> <str<strong>on</strong>g>Impacts</str<strong>on</strong>g> <str<strong>on</strong>g>of</str<strong>on</strong>g> <str<strong>on</strong>g>Aviati<strong>on</strong></str<strong>on</strong>g><br />

<strong>on</strong> <strong>Climate</strong> <strong>Change</strong><br />

PAGES 157–160<br />

<str<strong>on</strong>g>Aviati<strong>on</strong></str<strong>on</strong>g> is an integral part <str<strong>on</strong>g>of</str<strong>on</strong>g> <str<strong>on</strong>g>the</str<strong>on</strong>g> global<br />

ec<strong>on</strong>omic and transportati<strong>on</strong> systems. In<br />

fact, aviati<strong>on</strong> expansi<strong>on</strong> outpaces <str<strong>on</strong>g>the</str<strong>on</strong>g> ec<strong>on</strong>omic<br />

growth. Projecti<strong>on</strong>s indicate that over<br />

<str<strong>on</strong>g>the</str<strong>on</strong>g> next 2 <strong>de</strong>ca<strong>de</strong>s, <str<strong>on</strong>g>the</str<strong>on</strong>g> <strong>de</strong>mand for aviati<strong>on</strong><br />

could grow to about 3 times its present level.<br />

This projected growth will likely result in<br />

higher aviati<strong>on</strong> emissi<strong>on</strong>s and associated<br />

impacts <strong>on</strong> <str<strong>on</strong>g>the</str<strong>on</strong>g> envir<strong>on</strong>ment and <strong>on</strong> human<br />

health and welfare, <strong>de</strong>pending up<strong>on</strong> a variety<br />

<str<strong>on</strong>g>of</str<strong>on</strong>g> factors (such as <str<strong>on</strong>g>the</str<strong>on</strong>g> size and mix <str<strong>on</strong>g>of</str<strong>on</strong>g><br />

<str<strong>on</strong>g>the</str<strong>on</strong>g> <strong>op</strong>erati<strong>on</strong>al fleet necessary to meet <str<strong>on</strong>g>the</str<strong>on</strong>g><br />

stated <strong>de</strong>mand, as well as mitigati<strong>on</strong> steps<br />

that could inclu<strong>de</strong> new technological<br />

advances, more efficient <strong>op</strong>erati<strong>on</strong>al procedures,<br />

market-based <strong>op</strong>ti<strong>on</strong>s, or regulatory<br />

interventi<strong>on</strong>). N<strong>on</strong>e<str<strong>on</strong>g>the</str<strong>on</strong>g>less, it is critical to<br />

balance <str<strong>on</strong>g>the</str<strong>on</strong>g> ec<strong>on</strong>omic benefits <str<strong>on</strong>g>of</str<strong>on</strong>g> air travel<br />

with envir<strong>on</strong>mental c<strong>on</strong>cerns associated<br />

with this projected aviati<strong>on</strong> growth.<br />

Presently, <str<strong>on</strong>g>the</str<strong>on</strong>g>re are gaps and uncertainties<br />

in our un<strong>de</strong>rstanding <str<strong>on</strong>g>of</str<strong>on</strong>g> highly inter<strong>de</strong>pen<strong>de</strong>nt<br />

envir<strong>on</strong>mental impacts <str<strong>on</strong>g>of</str<strong>on</strong>g> aviati<strong>on</strong>, which<br />

inclu<strong>de</strong> air quality, climate, and noise. Without<br />

realizing all dimensi<strong>on</strong>s <str<strong>on</strong>g>of</str<strong>on</strong>g> benefits and<br />

related tra<strong>de</strong>-<str<strong>on</strong>g>of</str<strong>on</strong>g>fs, acti<strong>on</strong>s to address envir<strong>on</strong>mental<br />

c<strong>on</strong>cerns in <strong>on</strong>e domain may have<br />

uninten<strong>de</strong>d c<strong>on</strong>sequences in ano<str<strong>on</strong>g>the</str<strong>on</strong>g>r. To<br />

study this, <str<strong>on</strong>g>the</str<strong>on</strong>g> U.S. government’s Joint Planning<br />

and Devel<strong>op</strong>ment Office [2004] <strong>de</strong>vel<strong>op</strong>ed<br />

<str<strong>on</strong>g>the</str<strong>on</strong>g> Next Generati<strong>on</strong> Air Transportati<strong>on</strong><br />

System: Integrated plan. The NextGen visi<strong>on</strong><br />

calls for <strong>de</strong>vel<strong>op</strong>ment by 2025 <str<strong>on</strong>g>of</str<strong>on</strong>g> envir<strong>on</strong>mental<br />

protecti<strong>on</strong> that allows sustained aviati<strong>on</strong><br />

growth. In particular, <str<strong>on</strong>g>the</str<strong>on</strong>g> NextGen<br />

objective is to reduce uncertainties for climate<br />

impacts to a level that enables appr<strong>op</strong>riate<br />

acti<strong>on</strong>s to address <str<strong>on</strong>g>the</str<strong>on</strong>g>m.<br />

In or<strong>de</strong>r to provi<strong>de</strong> scientific input to Next-<br />

Gen within its stated time frame, acti<strong>on</strong> is<br />

now nee<strong>de</strong>d to un<strong>de</strong>rstand and quantify <str<strong>on</strong>g>the</str<strong>on</strong>g><br />

potential climate impacts <str<strong>on</strong>g>of</str<strong>on</strong>g> aviati<strong>on</strong> and<br />

<strong>de</strong>vel<strong>op</strong> emissi<strong>on</strong>-based metrics that can<br />

suitably capture <str<strong>on</strong>g>the</str<strong>on</strong>g>se impacts. This article<br />

<strong>de</strong>scribes <str<strong>on</strong>g>the</str<strong>on</strong>g> key science issues, <str<strong>on</strong>g>the</str<strong>on</strong>g> state <str<strong>on</strong>g>of</str<strong>on</strong>g><br />

un<strong>de</strong>rstanding, and <str<strong>on</strong>g>the</str<strong>on</strong>g> associated gaps and<br />

recommen<strong>de</strong>d research related to aviati<strong>on</strong>induced<br />

emissi<strong>on</strong>s and <str<strong>on</strong>g>the</str<strong>on</strong>g>ir effects <strong>on</strong> climate.<br />

<str<strong>on</strong>g>Aviati<strong>on</strong></str<strong>on</strong>g>-Induced <strong>Climate</strong> C<strong>on</strong>cerns<br />

The chemical species released during <str<strong>on</strong>g>the</str<strong>on</strong>g><br />

fuel combusti<strong>on</strong> process in aircraft engines<br />

inclu<strong>de</strong> carb<strong>on</strong> dioxi<strong>de</strong> (CO 2<br />

), water (H 2<br />

O),<br />

nitrogen oxi<strong>de</strong>s (NO x<br />

), and sulfur oxi<strong>de</strong>s<br />

(SO x<br />

) al<strong>on</strong>g with small amounts <str<strong>on</strong>g>of</str<strong>on</strong>g> soot<br />

carb<strong>on</strong> (C soot<br />

), hydrocarb<strong>on</strong>s (HC), and<br />

carb<strong>on</strong> m<strong>on</strong>oxi<strong>de</strong> (CO), as shown in Figure 1.<br />

Once released at cruise altitu<strong>de</strong>s within <str<strong>on</strong>g>the</str<strong>on</strong>g><br />

upper tr<strong>op</strong>osphere and lower stratosphere<br />

VOLUME 88 NUMBER 14<br />

3 APRIL 2007<br />

PAGES 157–168<br />

(UT/LS), <str<strong>on</strong>g>the</str<strong>on</strong>g>se species interact with <str<strong>on</strong>g>the</str<strong>on</strong>g><br />

background atmosphere and un<strong>de</strong>rgo complex<br />

processes, resulting in potential climate<br />

impacts and related welfare loss as <strong>de</strong>picted<br />

in Figure 1.<br />

Although each comp<strong>on</strong>ent <str<strong>on</strong>g>of</str<strong>on</strong>g> this causeeffect<br />

chain is c<strong>on</strong>ceptually simple, <str<strong>on</strong>g>the</str<strong>on</strong>g><br />

quantificati<strong>on</strong> <str<strong>on</strong>g>of</str<strong>on</strong>g> <str<strong>on</strong>g>the</str<strong>on</strong>g> overall magnitu<strong>de</strong> <str<strong>on</strong>g>of</str<strong>on</strong>g><br />

aviati<strong>on</strong>-induced climate impacts is highly<br />

uncertain. In 1999, a major internati<strong>on</strong>al<br />

coordinated effort to assess <str<strong>on</strong>g>the</str<strong>on</strong>g> impacts <str<strong>on</strong>g>of</str<strong>on</strong>g><br />

aviati<strong>on</strong> <strong>on</strong> <str<strong>on</strong>g>the</str<strong>on</strong>g> global atmosphere was sp<strong>on</strong>sored<br />

by <str<strong>on</strong>g>the</str<strong>on</strong>g> United Nati<strong>on</strong>s Intergovernmental<br />

<strong>Pa</strong>nel <strong>on</strong> <strong>Climate</strong> <strong>Change</strong> (IPCC) [IPCC,<br />

1999]. Figure 2 displays <str<strong>on</strong>g>the</str<strong>on</strong>g> IPCC estimates <str<strong>on</strong>g>of</str<strong>on</strong>g><br />

climate forcing <str<strong>on</strong>g>of</str<strong>on</strong>g> aviati<strong>on</strong> emissi<strong>on</strong>s in<br />

terms <str<strong>on</strong>g>of</str<strong>on</strong>g> radiative forcing (RF) for <str<strong>on</strong>g>the</str<strong>on</strong>g> years<br />

1992 and 2050 (based <strong>on</strong> <str<strong>on</strong>g>the</str<strong>on</strong>g> IPCC Fa1 emissi<strong>on</strong>s<br />

scenario that c<strong>on</strong>si<strong>de</strong>red midrange<br />

ec<strong>on</strong>omic growth and technology advances<br />

BY D. WUEBBLES, M. GUPTA, AND M. KO<br />

Fig. 1. Schematic <str<strong>on</strong>g>of</str<strong>on</strong>g> emissi<strong>on</strong>s released during aircraft fuel combusti<strong>on</strong> and <str<strong>on</strong>g>the</str<strong>on</strong>g>ir resulting potential<br />

impacts <strong>on</strong> climate change and welfare loss.


Eos, Vol. 88, No. 14, 3 April 2007<br />

for both improved fuel efficiency and NO x<br />

reducti<strong>on</strong>).<br />

In 1992, aviati<strong>on</strong> c<strong>on</strong>tributed about 2% <str<strong>on</strong>g>of</str<strong>on</strong>g><br />

<str<strong>on</strong>g>the</str<strong>on</strong>g> total anthr<strong>op</strong>ogenic CO 2<br />

emissi<strong>on</strong>s and<br />

accounted for globally and annually averaged<br />

RF (GAARF) <str<strong>on</strong>g>of</str<strong>on</strong>g> about 0.02 watts per<br />

square meter. In c<strong>on</strong>trast, <str<strong>on</strong>g>the</str<strong>on</strong>g> GAARF for all<br />

n<strong>on</strong>-CO 2<br />

aviati<strong>on</strong> emissi<strong>on</strong>s combined<br />

(excluding cirrus clouds) is as large as that<br />

<str<strong>on</strong>g>of</str<strong>on</strong>g> CO 2<br />

al<strong>on</strong>e, though characterized by relatively<br />

large uncertainties. Figure 2 clearly<br />

indicates that <str<strong>on</strong>g>the</str<strong>on</strong>g> level <str<strong>on</strong>g>of</str<strong>on</strong>g> scientific un<strong>de</strong>rstanding<br />

to estimate climate resp<strong>on</strong>se due to<br />

n<strong>on</strong>-CO 2<br />

emissi<strong>on</strong>s for both cases ranges<br />

from fair to very poor.<br />

GAARF has wi<strong>de</strong>ly been used as a metric <str<strong>on</strong>g>of</str<strong>on</strong>g><br />

climate change for l<strong>on</strong>g-lived greenhouse<br />

gases. However, <str<strong>on</strong>g>the</str<strong>on</strong>g>re are c<strong>on</strong>tinued questi<strong>on</strong>s<br />

about its viability and usefulness for<br />

o<str<strong>on</strong>g>the</str<strong>on</strong>g>r greenhouse gases [Nati<strong>on</strong>al Aca<strong>de</strong>my<br />

<str<strong>on</strong>g>of</str<strong>on</strong>g> Sciences, 2005]. A fundamental issue is<br />

that some RFs (e.g., those from c<strong>on</strong>trails,<br />

induced cirrus clouds, and oz<strong>on</strong>e from NO x<br />

emissi<strong>on</strong>s) are spatially inhomogeneous and<br />

seas<strong>on</strong>ally varying. Therefore, RF from each<br />

<str<strong>on</strong>g>of</str<strong>on</strong>g> <str<strong>on</strong>g>the</str<strong>on</strong>g>se various sources could produce a different<br />

temperature change at <str<strong>on</strong>g>the</str<strong>on</strong>g> surface <str<strong>on</strong>g>of</str<strong>on</strong>g><br />

<str<strong>on</strong>g>the</str<strong>on</strong>g> Earth per unit change in GAARF. In additi<strong>on</strong>,<br />

values given in Figure 2 represent <str<strong>on</strong>g>the</str<strong>on</strong>g><br />

change in forcing from changes in c<strong>on</strong>centrati<strong>on</strong>s<br />

due to all prior aviati<strong>on</strong> activities.<br />

Since <str<strong>on</strong>g>the</str<strong>on</strong>g> atmospheric effects due to aviati<strong>on</strong><br />

emissi<strong>on</strong>s have very different timescales,<br />

ranging from several hundred years for CO 2<br />

to a few hours for c<strong>on</strong>trails, such RF estimates<br />

do not capture <str<strong>on</strong>g>the</str<strong>on</strong>g> relative importance<br />

<str<strong>on</strong>g>of</str<strong>on</strong>g> <str<strong>on</strong>g>the</str<strong>on</strong>g> short- and l<strong>on</strong>g-lived effects.<br />

While new scientific un<strong>de</strong>rstanding and<br />

data sets have become available since <str<strong>on</strong>g>the</str<strong>on</strong>g><br />

last IPCC report <strong>on</strong> <str<strong>on</strong>g>the</str<strong>on</strong>g> impact <str<strong>on</strong>g>of</str<strong>on</strong>g> aviati<strong>on</strong> <strong>on</strong><br />

climate change [IPCC, 1999], <str<strong>on</strong>g>the</str<strong>on</strong>g>re has been<br />

no comprehensive U.S. or internati<strong>on</strong>al<br />

attempt to update <str<strong>on</strong>g>the</str<strong>on</strong>g> assessment and associated<br />

uncertainties. Over <str<strong>on</strong>g>the</str<strong>on</strong>g> past several<br />

years, <str<strong>on</strong>g>the</str<strong>on</strong>g>re has been a lapse in research<br />

activities in <str<strong>on</strong>g>the</str<strong>on</strong>g> United States <strong>on</strong> <str<strong>on</strong>g>the</str<strong>on</strong>g> climate<br />

impacts <str<strong>on</strong>g>of</str<strong>on</strong>g> aviati<strong>on</strong>. In fact, a report to <str<strong>on</strong>g>the</str<strong>on</strong>g> U.<br />

S. C<strong>on</strong>gress <strong>on</strong> aviati<strong>on</strong> and <str<strong>on</strong>g>the</str<strong>on</strong>g> envir<strong>on</strong>ment<br />

[Waitz et al., 2004] clearly stated that <str<strong>on</strong>g>the</str<strong>on</strong>g> climate<br />

change impact <str<strong>on</strong>g>of</str<strong>on</strong>g> aircraft is a t<strong>op</strong>ic <str<strong>on</strong>g>of</str<strong>on</strong>g><br />

great c<strong>on</strong>tenti<strong>on</strong> and <str<strong>on</strong>g>the</str<strong>on</strong>g>re are no major U.S.<br />

research programs to address this.<br />

Un<strong>de</strong>r <str<strong>on</strong>g>the</str<strong>on</strong>g> Eur<strong>op</strong>ean TRADEOFF program,<br />

Sausen et al. [2005] updated <str<strong>on</strong>g>the</str<strong>on</strong>g> GAARFs for<br />

<str<strong>on</strong>g>the</str<strong>on</strong>g> year 2000 and compared <str<strong>on</strong>g>the</str<strong>on</strong>g>m against <str<strong>on</strong>g>the</str<strong>on</strong>g><br />

corresp<strong>on</strong>ding interpolated GAARFs based <strong>on</strong><br />

IPCC estimates for year 1992 and year 2050.<br />

The overall c<strong>on</strong>clusi<strong>on</strong> from that study<br />

remains unchanged: There are significant<br />

uncertainties in quantifying <str<strong>on</strong>g>the</str<strong>on</strong>g> climate<br />

impacts <str<strong>on</strong>g>of</str<strong>on</strong>g> aviati<strong>on</strong> emissi<strong>on</strong>s. Presently, <str<strong>on</strong>g>the</str<strong>on</strong>g>re<br />

are several Eur<strong>op</strong>ean research programs (e.g.,<br />

QUANTIFY) un<strong>de</strong>r way that have focused <strong>on</strong><br />

un<strong>de</strong>rstanding <str<strong>on</strong>g>the</str<strong>on</strong>g> impacts <str<strong>on</strong>g>of</str<strong>on</strong>g> aviati<strong>on</strong> <strong>on</strong><br />

atmospheric compositi<strong>on</strong> and climate.<br />

In North America, a 2006 worksh<strong>op</strong> <strong>on</strong> <str<strong>on</strong>g>the</str<strong>on</strong>g><br />

impacts <str<strong>on</strong>g>of</str<strong>on</strong>g> aviati<strong>on</strong> <strong>on</strong> climate change,<br />

which was sp<strong>on</strong>sored by <str<strong>on</strong>g>the</str<strong>on</strong>g> U.S. Fe<strong>de</strong>ral<br />

<str<strong>on</strong>g>Aviati<strong>on</strong></str<strong>on</strong>g> Administrati<strong>on</strong> (FAA) and assessed<br />

and documented <str<strong>on</strong>g>the</str<strong>on</strong>g> present state <str<strong>on</strong>g>of</str<strong>on</strong>g> scientific<br />

knowledge, i<strong>de</strong>ntified <str<strong>on</strong>g>the</str<strong>on</strong>g> key un<strong>de</strong>rlying<br />

Fig. 2. Estimates <str<strong>on</strong>g>of</str<strong>on</strong>g> globally and annually averaged radiative forcing (GAARF), measured in watts<br />

per square meter, from subs<strong>on</strong>ic aircraft fleet for (a) 1992 and (b) 2050. In both cases, <str<strong>on</strong>g>the</str<strong>on</strong>g> forcing<br />

represents <str<strong>on</strong>g>the</str<strong>on</strong>g> difference caused by historical <strong>op</strong>erati<strong>on</strong> <str<strong>on</strong>g>of</str<strong>on</strong>g> <str<strong>on</strong>g>the</str<strong>on</strong>g> fleet from its first introducti<strong>on</strong> to<br />

1992 or 2050. The forcing for CO 2<br />

is calculated using changes in CO 2<br />

c<strong>on</strong>centrati<strong>on</strong> relative to<br />

<str<strong>on</strong>g>the</str<strong>on</strong>g> historical <strong>op</strong>erati<strong>on</strong>. Values for o<str<strong>on</strong>g>the</str<strong>on</strong>g>r forcings are approximated by <str<strong>on</strong>g>the</str<strong>on</strong>g> steady state resp<strong>on</strong>ses<br />

to a fleet with repeated annual emissi<strong>on</strong>s at <str<strong>on</strong>g>the</str<strong>on</strong>g> 1992 and 2050 levels, respectively. See <str<strong>on</strong>g>the</str<strong>on</strong>g> text<br />

<strong>on</strong> why GAARF may not be a suitable metric for climate impacts <str<strong>on</strong>g>of</str<strong>on</strong>g> aviati<strong>on</strong> emissi<strong>on</strong>s. Adapted<br />

from IPCC [1999].<br />

uncertainties and gaps as well as <strong>on</strong>going<br />

and fur<str<strong>on</strong>g>the</str<strong>on</strong>g>r research nee<strong>de</strong>d, and explored<br />

<str<strong>on</strong>g>the</str<strong>on</strong>g> <strong>de</strong>vel<strong>op</strong>ment <str<strong>on</strong>g>of</str<strong>on</strong>g> climate impact metrics.<br />

The worksh<strong>op</strong> also sought to focus <str<strong>on</strong>g>the</str<strong>on</strong>g> scientific<br />

community <strong>on</strong> aviati<strong>on</strong>–climate change<br />

research needs.<br />

The data shown in Figure 2 clearly indicate<br />

that <str<strong>on</strong>g>the</str<strong>on</strong>g> largest uncertainties are associated<br />

with <str<strong>on</strong>g>the</str<strong>on</strong>g> indirect forcing resulting from<br />

changes in <str<strong>on</strong>g>the</str<strong>on</strong>g> distributi<strong>on</strong>s and c<strong>on</strong>centrati<strong>on</strong>s<br />

<str<strong>on</strong>g>of</str<strong>on</strong>g> oz<strong>on</strong>e (O 3<br />

) and methane (CH 4<br />

) as a<br />

c<strong>on</strong>sequence <str<strong>on</strong>g>of</str<strong>on</strong>g> aircraft NO x<br />

emissi<strong>on</strong>s, and<br />

<str<strong>on</strong>g>the</str<strong>on</strong>g> direct effects (and indirect effects <strong>on</strong><br />

clouds) from emitted aerosols and aerosol<br />

precursors, and effects associated with c<strong>on</strong>trails<br />

and cirrus cloud formati<strong>on</strong>. Because <str<strong>on</strong>g>of</str<strong>on</strong>g><br />

<str<strong>on</strong>g>the</str<strong>on</strong>g> issues with <str<strong>on</strong>g>the</str<strong>on</strong>g> RF metric noted above,<br />

worksh<strong>op</strong> participants were asked to<br />

examine those issues as well as alternatives<br />

for metrics. A brief summary <str<strong>on</strong>g>of</str<strong>on</strong>g> <str<strong>on</strong>g>the</str<strong>on</strong>g> major<br />

t<strong>op</strong>ics covered at <str<strong>on</strong>g>the</str<strong>on</strong>g> worksh<strong>op</strong> is found<br />

below; <str<strong>on</strong>g>the</str<strong>on</strong>g> full report is available at http://<br />

web.mit.edu/aeroastro/partner/reports/<br />

climatewrksp-rpt-0806.pdf.<br />

Emissi<strong>on</strong>s in <str<strong>on</strong>g>the</str<strong>on</strong>g> UT/LS<br />

and Resulting Chemistry Effects<br />

The potential importance <str<strong>on</strong>g>of</str<strong>on</strong>g> aircraft NO x<br />

emissi<strong>on</strong>s <strong>on</strong> tr<strong>op</strong>ospheric and stratospheric<br />

O 3<br />

is well recognized. <str<strong>on</strong>g>Aviati<strong>on</strong></str<strong>on</strong>g>-perturbed<br />

O 3<br />

can also affect <str<strong>on</strong>g>the</str<strong>on</strong>g> tr<strong>op</strong>ospheric<br />

oxidizing capacity, and thus levels <str<strong>on</strong>g>of</str<strong>on</strong>g> CH 4<br />

,<br />

an important greenhouse gas. The database<br />

<str<strong>on</strong>g>of</str<strong>on</strong>g> observati<strong>on</strong>s pertaining to <str<strong>on</strong>g>the</str<strong>on</strong>g> UT/<br />

LS has been greatly expan<strong>de</strong>d since <str<strong>on</strong>g>the</str<strong>on</strong>g><br />

IPCC assessment, and <str<strong>on</strong>g>the</str<strong>on</strong>g> new data are<br />

being used to evaluate global mo<strong>de</strong>ls. In<br />

additi<strong>on</strong>, improvements to <str<strong>on</strong>g>the</str<strong>on</strong>g> representati<strong>on</strong><br />

<str<strong>on</strong>g>of</str<strong>on</strong>g> atmospheric transport processes<br />

have resulted in better mo<strong>de</strong>ls for <str<strong>on</strong>g>the</str<strong>on</strong>g> compositi<strong>on</strong><br />

and fluxes <str<strong>on</strong>g>of</str<strong>on</strong>g> O 3<br />

and o<str<strong>on</strong>g>the</str<strong>on</strong>g>r species<br />

in this regi<strong>on</strong>.<br />

However, uncertainties in mo<strong>de</strong>l predicti<strong>on</strong>s<br />

and gaps in un<strong>de</strong>rstanding remain. The<br />

large disagreements between <str<strong>on</strong>g>the</str<strong>on</strong>g> mo<strong>de</strong>led<br />

and measured abundances <str<strong>on</strong>g>of</str<strong>on</strong>g> hydrogen<br />

oxi<strong>de</strong>s (HO x<br />

) and NO x<br />

gases in <str<strong>on</strong>g>the</str<strong>on</strong>g> upper tr<strong>op</strong>osphere<br />

point to ei<str<strong>on</strong>g>the</str<strong>on</strong>g>r measurement errors<br />

or errors in tr<strong>op</strong>ospheric chemical mechanisms<br />

and rates. There remain uncertainties<br />

related to <str<strong>on</strong>g>the</str<strong>on</strong>g> removal <str<strong>on</strong>g>of</str<strong>on</strong>g> atmospheric NO x<br />

through <str<strong>on</strong>g>the</str<strong>on</strong>g> coupling <str<strong>on</strong>g>of</str<strong>on</strong>g> large-scale transport,<br />

c<strong>on</strong>vecti<strong>on</strong>, cloud, and precipitati<strong>on</strong> processes.<br />

A <strong>de</strong>tailed intercomparis<strong>on</strong> <str<strong>on</strong>g>of</str<strong>on</strong>g> current<br />

mo<strong>de</strong>ls and measurements, emphasizing<br />

<str<strong>on</strong>g>the</str<strong>on</strong>g> UT/LS and free tr<strong>op</strong>osphere, is nee<strong>de</strong>d.<br />

This process should lead to mo<strong>de</strong>l<br />

improvements and <str<strong>on</strong>g>the</str<strong>on</strong>g> reducti<strong>on</strong> <str<strong>on</strong>g>of</str<strong>on</strong>g> uncertainty<br />

in mo<strong>de</strong>l predicti<strong>on</strong>s. Also nee<strong>de</strong>d is<br />

an expan<strong>de</strong>d analysis <str<strong>on</strong>g>of</str<strong>on</strong>g> <str<strong>on</strong>g>the</str<strong>on</strong>g> wealth <str<strong>on</strong>g>of</str<strong>on</strong>g> data<br />

currently obtained in <str<strong>on</strong>g>the</str<strong>on</strong>g> UT/LS by aircraft<br />

and satellite platforms with a focus <strong>on</strong><br />

regi<strong>on</strong>s perturbed by impacts <str<strong>on</strong>g>of</str<strong>on</strong>g> aviati<strong>on</strong><br />

emissi<strong>on</strong>s. Presently, most analyses <str<strong>on</strong>g>of</str<strong>on</strong>g> aviati<strong>on</strong><br />

impacts are evaluated relative to current<br />

atmospheric c<strong>on</strong>diti<strong>on</strong>s. Estimates <str<strong>on</strong>g>of</str<strong>on</strong>g><br />

projected climate resp<strong>on</strong>se should c<strong>on</strong>si<strong>de</strong>r<br />

<str<strong>on</strong>g>the</str<strong>on</strong>g> atmospheric c<strong>on</strong>diti<strong>on</strong>s expected<br />

at <str<strong>on</strong>g>the</str<strong>on</strong>g> time <str<strong>on</strong>g>of</str<strong>on</strong>g> future fleet. In <str<strong>on</strong>g>the</str<strong>on</strong>g> l<strong>on</strong>ger<br />

term, field campaigns are required to<br />

address issues with HO x<br />

-NO x<br />

chemistry in<br />

<str<strong>on</strong>g>the</str<strong>on</strong>g> UT and to better un<strong>de</strong>rstand background<br />

processes.<br />

C<strong>on</strong>trails and Cirrus Clouds<br />

C<strong>on</strong>trails form if ambient air al<strong>on</strong>g <str<strong>on</strong>g>the</str<strong>on</strong>g><br />

flight track is col<strong>de</strong>r and moister than a<br />

threshold based <strong>on</strong> known <str<strong>on</strong>g>the</str<strong>on</strong>g>rmodynamic<br />

parameters. Early c<strong>on</strong>trail evoluti<strong>on</strong> <strong>de</strong>pends,<br />

in poorly un<strong>de</strong>rstood ways, <strong>on</strong> aircraft and<br />

engine emissi<strong>on</strong> parameters. In ice-supersaturated<br />

air masses, c<strong>on</strong>trails can organize<br />

<str<strong>on</strong>g>the</str<strong>on</strong>g>mselves in regi<strong>on</strong>al-scale clusters that<br />

add significantly to <str<strong>on</strong>g>the</str<strong>on</strong>g> natural high cloud<br />

cover and have <str<strong>on</strong>g>the</str<strong>on</strong>g> potential, albeit with<br />

large uncertainties, for a relatively large positive<br />

radiative forcing. Factors c<strong>on</strong>trolling <str<strong>on</strong>g>the</str<strong>on</strong>g><br />

radiative pr<strong>op</strong>erties <str<strong>on</strong>g>of</str<strong>on</strong>g> cirrus clouds and


c<strong>on</strong>trail-cirrus (e.g., ice crystal habit, vertical<br />

pr<str<strong>on</strong>g>of</str<strong>on</strong>g>iles <str<strong>on</strong>g>of</str<strong>on</strong>g> ice water c<strong>on</strong>tent, effective radius)<br />

also are poorly c<strong>on</strong>strained by observati<strong>on</strong>s.<br />

The extent <str<strong>on</strong>g>of</str<strong>on</strong>g> global distributi<strong>on</strong> <str<strong>on</strong>g>of</str<strong>on</strong>g> supersaturati<strong>on</strong><br />

in <str<strong>on</strong>g>the</str<strong>on</strong>g> upper tr<strong>op</strong>osphere has not<br />

been a<strong>de</strong>quately verified to enable its reliable<br />

predicti<strong>on</strong>.<br />

Many uncertainties and knowledge gaps<br />

related to aircraft emissi<strong>on</strong> <str<strong>on</strong>g>of</str<strong>on</strong>g> aerosols persist,<br />

including <str<strong>on</strong>g>the</str<strong>on</strong>g>ir role in plume evoluti<strong>on</strong><br />

and <str<strong>on</strong>g>the</str<strong>on</strong>g>ir interacti<strong>on</strong> with <str<strong>on</strong>g>the</str<strong>on</strong>g> background<br />

atmosphere and <str<strong>on</strong>g>the</str<strong>on</strong>g> formati<strong>on</strong> <str<strong>on</strong>g>of</str<strong>on</strong>g> cirrus<br />

clouds. The magnitu<strong>de</strong> <str<strong>on</strong>g>of</str<strong>on</strong>g> <str<strong>on</strong>g>the</str<strong>on</strong>g> atmospheric<br />

impact <strong>de</strong>pends <strong>on</strong> <strong>de</strong>tails <str<strong>on</strong>g>of</str<strong>on</strong>g> plume processing<br />

and <strong>on</strong> <str<strong>on</strong>g>the</str<strong>on</strong>g> relative ability <str<strong>on</strong>g>of</str<strong>on</strong>g> background<br />

aerosol particles to act as ice-forming nuclei.<br />

In additi<strong>on</strong>, mo<strong>de</strong>ls do not a<strong>de</strong>quately treat<br />

<str<strong>on</strong>g>the</str<strong>on</strong>g> radiative pr<strong>op</strong>erties <str<strong>on</strong>g>of</str<strong>on</strong>g> cirrus, thus limiting<br />

<str<strong>on</strong>g>the</str<strong>on</strong>g>ir abilities to study c<strong>on</strong>trail-cirrus<br />

cloud interacti<strong>on</strong>s. Large uncertainties exist<br />

as to how pr<strong>op</strong>erties <str<strong>on</strong>g>of</str<strong>on</strong>g> ambient aerosols are<br />

perturbed in <str<strong>on</strong>g>the</str<strong>on</strong>g> presence <str<strong>on</strong>g>of</str<strong>on</strong>g> jet engine emissi<strong>on</strong>s<br />

un<strong>de</strong>r various atmospheric c<strong>on</strong>diti<strong>on</strong>s<br />

and aircraft c<strong>on</strong>figurati<strong>on</strong>s.<br />

In or<strong>de</strong>r to improve <str<strong>on</strong>g>the</str<strong>on</strong>g> representati<strong>on</strong> <str<strong>on</strong>g>of</str<strong>on</strong>g><br />

relevant processes in regi<strong>on</strong>al and global<br />

mo<strong>de</strong>ls that are resp<strong>on</strong>sible for formati<strong>on</strong><br />

<str<strong>on</strong>g>of</str<strong>on</strong>g> c<strong>on</strong>trails as well as c<strong>on</strong>trail-induced cirrus<br />

clouds, coordinated regi<strong>on</strong>al-scale<br />

campaigns are nee<strong>de</strong>d to measure variables<br />

to characterize <str<strong>on</strong>g>the</str<strong>on</strong>g> growth, <strong>de</strong>cay, and<br />

trajectories <str<strong>on</strong>g>of</str<strong>on</strong>g> c<strong>on</strong>trail ice particle p<strong>op</strong>ulati<strong>on</strong>s<br />

and to <strong>de</strong>fine <str<strong>on</strong>g>the</str<strong>on</strong>g> abundance and<br />

pr<strong>op</strong>erties <str<strong>on</strong>g>of</str<strong>on</strong>g> ambient aerosols as well as<br />

gaseous aerosol precursor c<strong>on</strong>centrati<strong>on</strong>s.<br />

Process studies that explore <str<strong>on</strong>g>the</str<strong>on</strong>g> role <str<strong>on</strong>g>of</str<strong>on</strong>g><br />

emitted aerosol particles, and how volatile<br />

aerosols interact with each o<str<strong>on</strong>g>the</str<strong>on</strong>g>r and with<br />

background aerosols, are required to<br />

un<strong>de</strong>rstand <str<strong>on</strong>g>the</str<strong>on</strong>g> indirect effect <str<strong>on</strong>g>of</str<strong>on</strong>g> emitted<br />

aerosol particles. Laboratory measurements<br />

are urgently nee<strong>de</strong>d to <strong>de</strong>vel<strong>op</strong> aerosol-related<br />

parameterizati<strong>on</strong>s <str<strong>on</strong>g>of</str<strong>on</strong>g> heterogeneous<br />

ice nucleati<strong>on</strong> for use in mo<strong>de</strong>ls.<br />

L<strong>on</strong>g-term recommen<strong>de</strong>d research<br />

needs inclu<strong>de</strong> enhanced instrumentati<strong>on</strong><br />

to establish background c<strong>on</strong>centrati<strong>on</strong>s<br />

and characteristics <str<strong>on</strong>g>of</str<strong>on</strong>g> heterogeneous ice<br />

nuclei and measure supersaturati<strong>on</strong> accurately.<br />

Also required is <str<strong>on</strong>g>the</str<strong>on</strong>g> <strong>de</strong>vel<strong>op</strong>ment <str<strong>on</strong>g>of</str<strong>on</strong>g><br />

new c<strong>on</strong>cepts relating to ice phase processes<br />

for treatment <str<strong>on</strong>g>of</str<strong>on</strong>g> cirrus and associated<br />

aviati<strong>on</strong> effects in climate mo<strong>de</strong>ls.<br />

<strong>Climate</strong> <str<strong>on</strong>g>Impacts</str<strong>on</strong>g> and <strong>Climate</strong> Metrics<br />

As stated earlier, with <str<strong>on</strong>g>the</str<strong>on</strong>g> excepti<strong>on</strong> <str<strong>on</strong>g>of</str<strong>on</strong>g> CO 2<br />

emissi<strong>on</strong>s, <str<strong>on</strong>g>the</str<strong>on</strong>g>re remain significant uncertainties<br />

in almost all aspects <str<strong>on</strong>g>of</str<strong>on</strong>g> aircraft effects <strong>on</strong><br />

climate. In particular, estimates <str<strong>on</strong>g>of</str<strong>on</strong>g> radiative<br />

impacts due to c<strong>on</strong>trail and c<strong>on</strong>trail-induced<br />

formati<strong>on</strong> <str<strong>on</strong>g>of</str<strong>on</strong>g> cirrus clouds are highly uncertain<br />

[e.g., Minnis et al., 2004; Hansen et al.,<br />

Eos, Vol. 88, No. 14, 3 April 2007<br />

2005]. Projecti<strong>on</strong>s for aviati<strong>on</strong>-induced radiative<br />

impacts are even more unreliable<br />

because <str<strong>on</strong>g>of</str<strong>on</strong>g> uncertainties in predicti<strong>on</strong> <str<strong>on</strong>g>of</str<strong>on</strong>g><br />

future atmospheric c<strong>on</strong>diti<strong>on</strong>s and <str<strong>on</strong>g>the</str<strong>on</strong>g>ir interacti<strong>on</strong>s<br />

with projected aviati<strong>on</strong> emissi<strong>on</strong>s.<br />

Metrics are nee<strong>de</strong>d to measure different<br />

climate forcings and place <str<strong>on</strong>g>the</str<strong>on</strong>g>m <strong>on</strong> a comm<strong>on</strong><br />

scale in or<strong>de</strong>r to assess <str<strong>on</strong>g>the</str<strong>on</strong>g> overall<br />

impact <str<strong>on</strong>g>of</str<strong>on</strong>g> aviati<strong>on</strong> <strong>on</strong> climate and to quantify<br />

<str<strong>on</strong>g>the</str<strong>on</strong>g> potential tra<strong>de</strong>-<str<strong>on</strong>g>of</str<strong>on</strong>g>fs <strong>on</strong> <str<strong>on</strong>g>the</str<strong>on</strong>g> climate<br />

impact due to changes in aircraft technology,<br />

aircraft <strong>op</strong>erati<strong>on</strong>s, and various policy<br />

scenarios. Such tra<strong>de</strong>-<str<strong>on</strong>g>of</str<strong>on</strong>g>fs might c<strong>on</strong>si<strong>de</strong>r,<br />

for example, NO x<br />

reducti<strong>on</strong> technology versus<br />

fuel efficiency, or <str<strong>on</strong>g>the</str<strong>on</strong>g> effects <str<strong>on</strong>g>of</str<strong>on</strong>g> changing<br />

flight altitu<strong>de</strong>s. <strong>Climate</strong> change metrics<br />

play an important role in quantifying <str<strong>on</strong>g>the</str<strong>on</strong>g>se<br />

tra<strong>de</strong>-<str<strong>on</strong>g>of</str<strong>on</strong>g>fs. As stated earlier, RF has l<strong>on</strong>g<br />

been used as a proxy for climate impact for<br />

greenhouse gases, but <str<strong>on</strong>g>the</str<strong>on</strong>g>re are doubts<br />

about its viability and usefulness. The c<strong>on</strong>cept<br />

<str<strong>on</strong>g>of</str<strong>on</strong>g> efficacy, which <strong>de</strong>pends <strong>on</strong> <str<strong>on</strong>g>the</str<strong>on</strong>g> specific<br />

perturbati<strong>on</strong> to <str<strong>on</strong>g>the</str<strong>on</strong>g> climate system, has<br />

been introduced to account for <str<strong>on</strong>g>the</str<strong>on</strong>g> fact that<br />

a unit global mean radiative forcing from<br />

different climate change mechanisms does<br />

not necessarily lead to <str<strong>on</strong>g>the</str<strong>on</strong>g> same climate<br />

impact. In additi<strong>on</strong>, RF is not an emissi<strong>on</strong><br />

metric capable <str<strong>on</strong>g>of</str<strong>on</strong>g> comparing <str<strong>on</strong>g>the</str<strong>on</strong>g> future<br />

impact <str<strong>on</strong>g>of</str<strong>on</strong>g> projected aviati<strong>on</strong> emissi<strong>on</strong> scenarios.<br />

The applicability <str<strong>on</strong>g>of</str<strong>on</strong>g> emissi<strong>on</strong>s metrics,<br />

such as global warming potentials, to<br />

short-lived greenhouse gases has not been<br />

a<strong>de</strong>quately tested and evaluated.<br />

There is no published study that utilizes<br />

<str<strong>on</strong>g>the</str<strong>on</strong>g> current un<strong>de</strong>rstanding <str<strong>on</strong>g>of</str<strong>on</strong>g> <str<strong>on</strong>g>the</str<strong>on</strong>g> impact <str<strong>on</strong>g>of</str<strong>on</strong>g><br />

aviati<strong>on</strong> emissi<strong>on</strong>s <strong>on</strong> atmospheric compositi<strong>on</strong>,<br />

as reflected in state-<str<strong>on</strong>g>of</str<strong>on</strong>g>-<str<strong>on</strong>g>the</str<strong>on</strong>g>-art atmospheric<br />

mo<strong>de</strong>ls, to examine <str<strong>on</strong>g>the</str<strong>on</strong>g> possible<br />

choices, <strong>de</strong>pen<strong>de</strong>ncies, and problems for<br />

metrics suitable for evaluating aviati<strong>on</strong><br />

tra<strong>de</strong>-<str<strong>on</strong>g>of</str<strong>on</strong>g>fs. Such studies would need to<br />

explore <str<strong>on</strong>g>the</str<strong>on</strong>g> utility <str<strong>on</strong>g>of</str<strong>on</strong>g> existing metrics and<br />

<str<strong>on</strong>g>the</str<strong>on</strong>g> possibility <str<strong>on</strong>g>of</str<strong>on</strong>g> <strong>de</strong>signing new metrics.<br />

C<strong>on</strong>clusi<strong>on</strong>s and Next Steps<br />

<str<strong>on</strong>g>Aviati<strong>on</strong></str<strong>on</strong>g>-focused research activities are<br />

required to address <str<strong>on</strong>g>the</str<strong>on</strong>g> uncertainties and<br />

gaps in <str<strong>on</strong>g>the</str<strong>on</strong>g> un<strong>de</strong>rstanding <str<strong>on</strong>g>of</str<strong>on</strong>g> current and<br />

projected impacts <str<strong>on</strong>g>of</str<strong>on</strong>g> aviati<strong>on</strong> <strong>on</strong> climate and<br />

to <strong>de</strong>vel<strong>op</strong> metrics to better characterize<br />

<str<strong>on</strong>g>the</str<strong>on</strong>g>se impacts. This may entail coordinati<strong>on</strong><br />

and/or expansi<strong>on</strong> <str<strong>on</strong>g>of</str<strong>on</strong>g> existing and planned<br />

climate research programs, or new activities.<br />

Such efforts should inclu<strong>de</strong> str<strong>on</strong>g and c<strong>on</strong>tinuing<br />

interacti<strong>on</strong>s am<strong>on</strong>g <str<strong>on</strong>g>the</str<strong>on</strong>g> science and<br />

aviati<strong>on</strong> communities as well as am<strong>on</strong>g policy<br />

makers to <strong>de</strong>vel<strong>op</strong> well-informed <strong>de</strong>cisi<strong>on</strong>s.<br />

More c<strong>on</strong>crete steps would inclu<strong>de</strong><br />

fur<str<strong>on</strong>g>the</str<strong>on</strong>g>r ranking and prioritizing <str<strong>on</strong>g>of</str<strong>on</strong>g> i<strong>de</strong>ntified<br />

research needs; creating a research road<br />

map with associated roles and resp<strong>on</strong>sibilities<br />

<str<strong>on</strong>g>of</str<strong>on</strong>g> various participating agencies and<br />

stakehol<strong>de</strong>rs; and i<strong>de</strong>ntifying resources<br />

nee<strong>de</strong>d to implement <str<strong>on</strong>g>the</str<strong>on</strong>g> road map. In coordinati<strong>on</strong><br />

with participating fe<strong>de</strong>ral research<br />

agencies <str<strong>on</strong>g>of</str<strong>on</strong>g> <str<strong>on</strong>g>the</str<strong>on</strong>g> U.S. <strong>Climate</strong> <strong>Change</strong> Science<br />

Program, <str<strong>on</strong>g>the</str<strong>on</strong>g> FAA is exploring possible<br />

means <str<strong>on</strong>g>of</str<strong>on</strong>g> addressing research needs i<strong>de</strong>ntified<br />

by <str<strong>on</strong>g>the</str<strong>on</strong>g> worksh<strong>op</strong>.<br />

Acknowledgments<br />

The June 2006 Worksh<strong>op</strong> <strong>on</strong> <str<strong>on</strong>g>the</str<strong>on</strong>g> <str<strong>on</strong>g>Impacts</str<strong>on</strong>g> <str<strong>on</strong>g>of</str<strong>on</strong>g><br />

<str<strong>on</strong>g>Aviati<strong>on</strong></str<strong>on</strong>g> <strong>on</strong> <strong>Climate</strong> <strong>Change</strong> was held in Bost<strong>on</strong>,<br />

Mass., un<strong>de</strong>r <str<strong>on</strong>g>the</str<strong>on</strong>g> auspices <str<strong>on</strong>g>of</str<strong>on</strong>g> <str<strong>on</strong>g>the</str<strong>on</strong>g> Envir<strong>on</strong>mental<br />

Integrated Product Team <str<strong>on</strong>g>of</str<strong>on</strong>g> <str<strong>on</strong>g>the</str<strong>on</strong>g> Joint<br />

Planning and Devel<strong>op</strong>ment Office <str<strong>on</strong>g>of</str<strong>on</strong>g> NextGen<br />

and PARTNER (<strong>Pa</strong>rtnership for Air Transportati<strong>on</strong><br />

Noise and Emissi<strong>on</strong>s Reducti<strong>on</strong>; a Center<br />

<str<strong>on</strong>g>of</str<strong>on</strong>g> Excellence supported by <str<strong>on</strong>g>the</str<strong>on</strong>g> FAA,<br />

NASA, and Transport Canada), and jointly<br />

sp<strong>on</strong>sored by <str<strong>on</strong>g>the</str<strong>on</strong>g> FAA and NASA.<br />

References<br />

Hansen, J., et al. (2005), Efficacy <str<strong>on</strong>g>of</str<strong>on</strong>g> climate forcings,<br />

J. Ge<strong>op</strong>hys. Res., 110, D18104, doi:10.1029/<br />

2005JD005776.<br />

Intergovernmental <strong>Pa</strong>nel <strong>on</strong> <strong>Climate</strong> <strong>Change</strong><br />

(1999), <str<strong>on</strong>g>Aviati<strong>on</strong></str<strong>on</strong>g> and <str<strong>on</strong>g>the</str<strong>on</strong>g> Global Atmosphere,<br />

Cambridge Univ. Press, New York. (Available at<br />

http://www.grida.no/climate/ipcc/aviati<strong>on</strong>/in<strong>de</strong>x.<br />

htm)<br />

Joint Planning and Devel<strong>op</strong>ment Office (2004),<br />

Next Generati<strong>on</strong> Air Transportati<strong>on</strong> System: Integrated<br />

plan, Washingt<strong>on</strong>, D. C. (Available at<br />

http://www.jpdo.aero/pdf/NGATS_v1_1204r.pdf)<br />

Minnis, P., J. K. Ayers, R. <strong>Pa</strong>lik<strong>on</strong>da, and D. Phan<br />

(2004), C<strong>on</strong>trails, cirrus, trends, and climate,<br />

J. Clim., 17, 1671–1685.<br />

Nati<strong>on</strong>al Aca<strong>de</strong>my <str<strong>on</strong>g>of</str<strong>on</strong>g> Sciences (2005), Radiative<br />

Forcing <str<strong>on</strong>g>of</str<strong>on</strong>g> <strong>Climate</strong> <strong>Change</strong>: Expanding <str<strong>on</strong>g>the</str<strong>on</strong>g> C<strong>on</strong>cept<br />

and Addressing Uncertainties, Washingt<strong>on</strong>,<br />

D. C.<br />

Sausen, R., et al. (2005), <str<strong>on</strong>g>Aviati<strong>on</strong></str<strong>on</strong>g> radiative forcing<br />

in 2000: An update <strong>on</strong> IPCC (1999), Meteorol. Z.,<br />

14, 555–561.<br />

Waitz, I., J. Townsend, J. Cutcher-Gershenfeld, E.<br />

Greitzer, and J. Kerrebrock (2004), <str<strong>on</strong>g>Aviati<strong>on</strong></str<strong>on</strong>g> and<br />

<str<strong>on</strong>g>the</str<strong>on</strong>g> envir<strong>on</strong>ment: Report to <str<strong>on</strong>g>the</str<strong>on</strong>g> United States C<strong>on</strong>gress,<br />

<strong>Pa</strong>rtnership for Air Transp. Noise and Emissi<strong>on</strong>s<br />

Reduct., Mass. Inst. <str<strong>on</strong>g>of</str<strong>on</strong>g> Technol., Cambridge.<br />

(Available at http://web.mit.edu/aeroastro/partner/<br />

reports/c<strong>on</strong>grept_aviati<strong>on</strong>_envirn.pdf)<br />

Author Informati<strong>on</strong><br />

D<strong>on</strong> Wuebbles, Department <str<strong>on</strong>g>of</str<strong>on</strong>g> Atmospheric Sciences,<br />

University <str<strong>on</strong>g>of</str<strong>on</strong>g> Illinois at Urbana-Champaign;<br />

E-mail: wuebbles@uiuc.edu; Mohan Gupta, Office<br />

<str<strong>on</strong>g>of</str<strong>on</strong>g> Envir<strong>on</strong>ment and Energy, U.S. Fe<strong>de</strong>ral <str<strong>on</strong>g>Aviati<strong>on</strong></str<strong>on</strong>g><br />

Administrati<strong>on</strong>, Washingt<strong>on</strong>, D. C.; and Malcolm Ko,<br />

Science Directorate, NASA Langley Research Center,<br />

Hampt<strong>on</strong>, Va.

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