1 Prof. Dr. George Kaptay List of publications ... - Miskolci Egyetem

J.145. G. Kaptay: On the atomic masses (weights?) of the elements, J. Min. Metall. B, 2012,vol.48, pp. 153-159 (2011-IF = 1.317).J144. G.Kaptay: Interfacial Forces in Dispersion Science and Technology - Journal ofDispersion Science and Technology, 2012, vol.33, pp.130-140 (2011-IF = 0.560).J143. G.Kaptay: On the optimum contact angle of stability of foams by particles – Advancesin Colloid and Interface Science, 2012, vol.170, pp. 87-88 (2011-IF = 8.120).J.142. G.Kaptay: The conversion of phase diagrams of solid solution type intoelectrochemical synthesis diagrams for binary metallic systems on inert cathodes -Electrochimica Acta, 2012, vol.60, pp.401-409. (2011-IF = 3.832)J.141. Y. Tang, Y. Du, L. Zhang, X. Yuan, G.Kaptay: Thermodynamic description of the Al–Mg–Si system using a new formulation for the excess Gibbs energy – Thermochimica Acta,2012, vol.527, pp.131-142. (2011-IF = 1.805).J.140. G.Kaptay: On the tendency of solutions to tend toward ideal solutions at hightemperatures – Metall Mater Trans A, 2012, vol.43, pp. 531-543. (2011-IF = 1.545).J.139. G.Kaptay: Interfacial phenomena in producing metallic materials. Part 5: Theinterfacial spreading force (in Hungarian). – BKL Kohászat, 2011., vol.144., No.5., pp. 9-13.(IF = 0)J.138. G.Kaptay: On the five base quantities of nature and SI (The International system ofUnits) – JMM B, 2011, vol47, No.2, pp.241-246. (IF = 1.317).J138-c1. KW Craig: No child left behind: teaching the metric system in US schools – Int J Appl Sci Technol,2012, vol.2, No.4, pp.40-48. – „Although there are seven base units in SI, “it is claimed that five is thesmallest number of base quantities that is sufficient to define all derived quantities and allows thedescription of all natural phenomena … length, mass, time, temperature and electric charge … The firstfour … coincide with the current list of base quantities in SI” (Kaptay, 2011, p. 242). There is a proposalto replace electric current with electric charge and to eliminate both the amount of substance andluminous intensity.” – p.41.J.137. D.Madarasz, I.Budai, G.Kaptay: Fabrication of SiC-particles shielded Al-spheres uponrecycling Al/SiC composites – Metal Mater Trans A, 2011, Volume 42, Number 6, 1439-1443 (IF = 1.545).J137-c1. Baumli P.: Fémmátrixú kompozitok előállítása öntészeti módszerekkel – CD-Proc. of 26. Int. Sci. Conf.microCAD, 29-30 March, 2012. – „A NaCl-KCl-KF típusú sókeverékkel az alumínium olvadékban lévőSiC szemcsék is eltávolíthatóak [J137].” – 4.o.J136. I.Budai, O.Z.Nagy, G.Kaptay: Inversion of a liquid Bi/Al metallic emulsion stabilizedby solid SiC particles, Coll Surf A, 2011, vol.377, pp.325-329 (IF = 2.236)J.135. O.Verezub, Z.Kálazi, A.Sytcheva, L.Kuzsella, G.Buza, N.V.Verezub, A.Fedorov,G.Kaptay: Performance of a cutting tool made of steel matrix surface nano-compositeproduced by in-situ laser melt injection technology – J Mater Process Technol., 2011, vol.211,pp.750-758 (IF = 1.783)3

J135-c1. Baumli P.: Fémmátrixú kompozitok előállítása öntészeti módszerekkel – CD-Proc. of 26. Int Sci ConfmicroCAD, 29-30 March, 2012. – „Lézer segítségével felületi kompozitok állíthatóak elő. Ebben azesetben a mátrix anyagául szolgáló fém felületét lézerrel megolvasztják, és az így kialakult fémtócsábamegfelelő sebességgel lövik az erősítő fázisnak szánt szemcséket [J135].” – 4.o.J135-c2. C.W.Rejil, I.Dinaharan, S.J.Vijay, N.Murugan: Microstructure and sliding wear behavior ofAA6360/(TiC+B4C) hybrid surface composite layer synthesized by friction stir processing on aluminumsubstrate. Mater Sci Eng A, 2012, vol.552, pp.336-344. „SCLs (surface composite layers) are fabricatedusing conventional liquid phase processing methods such as high energy laser melt injection [J135], etc…„ – p.336.J134. I.Budai, G.Kaptay: Monotectic Al/Cd alloys with homogeneously dispersed Cd-dropletsstabilized by strontium aluminide precipitates – Intermetallics, 2011, vol.19. pp.423-425 (IF =1.649).J.133. Kaptay Gy.: Határfelületi jelenségek a fémesanyaggyártásban. 4.rész. A határfelületigradiens erő – BKL Kohászat, 2010., 143. évf., 5. szám, 45-54.o. (IF = 0)J.132. G.Kaptay: The Extension of the Phase Rule to Nano-Systems and on the QuaternaryPoint in One-Component Nano Phase Diagrams - J. Nanosci. Nanotechnol., 2010, vol.10,pp.8164–8170. (IF = 1.352).J.131. M.Reger, B.Vero, I.Kardos, E.R.Fabian, G.Kaptay: Diffusion of carbon in thecenterline region of continuous cast slabs – Mater Sci Forum, 2010, vol.659, pp.441-446 (IF =0)J.130. Kaptay Gy.: Határfelületi jelenségek a fémesanyaggyártásban. 3.rész. A görbületindukálta határfelületi erő – BKL Kohászat, 2010., 143. évf., 3. szám, 33-38. (IF = 0)J.129. P.Baumli, J.Sytchev, G.Kaptay: Perfect wettability of carbon by liquid aluminumachieved by a multifunctional flux. J Mater Sci, 2010, vol.45, pp.5177-5190. (IF = 1.859).J129-c1. I.N.Orbulov: Infiltration of ceramic microballons by liquid metals – research plan for SCIEX-NMS,February, 2011, 12 pp. – „There are many papers in the professional literature which are dealing withthe phenomenon of infiltartion [J129]” – p.9.J129-c2. Lévai Gábor (tud. vez.: dr. Török Tamás): Acéllemezek színes tűzi horganyzása, 6. doktoriszeminárium, 2011, június 14., 28 oldal. – “Kaptay és mtsai több alkalommal publikáltak pozitíveredményeket alumíniumnak K 2 TiF 6 sóval történő ötvözéséről [129]”. – p.19.J129-c3. W.Xi, R.L. Peng, W. Wu, N. Li, S. Wang, S. Johansson: Al2O3 nanoparticle reinforced Fe-based alloyssynthesized by thermite reaction – J Mater Sci, 2012, vol.47, pp.3585-3591 – „Many studiesdemonstrate that a low interfacial energy between ceramic particles and metal matrix is the mostimportant condition for obtaining homogeneous distribution of ceramic particles in the metal matrixwhen a metal matrix components is produced by solidification process [J129]” – p.3588.J.128. Á.E. Horváth, F. Járai-Szabó, G.Kaptay, R.Vajtai, Z.Néda: Pattern formation andselection in nanotube arrays - Univ Polit Bucharest Sci Bull – Ser A - Appl Math Phys, 2010,vol.72, Iss.1, pp.27-32. (IF = 0.253).J.127. I.Budai, G.Kaptay: Wettability of SiC and alumina particles by liquid Bi under liquidAl – J. Mater Sci, 2010, vol.45, pp.2090-2098. (IF = 1.859)J127-c1. I.Kaban, M.Köhler, W.Hoyer, L.Ratke: Catalytic efficiency of oxide particles on heterogeneousnucleation in aluminium alloy with miscibility gap – Hig Temperatures – High Pressures, 2010, vol.39,pp.347-355. – „In this case, the advancing contact angle is around 10 degrees and the receeding contactangle is around zero, which correlates with the results of work [J127] were the perfect wetting of aluminaby Bi- and Pb-rich phase has been reported” – p.352.4

J127-c2. I.Kaban, M.Köhler, L.Ratke, W.Hoyer, N.Mattern, J.Eckert, A.L.Geer: Interfacial tension, wetting andnucleation in Al-Bi and Al-Pb monotectic alloys – Acta mater, 2011, vol.59, pp. 6880-6889 – „Budai andKaptay [J127] found that Al 2 O 3 particles were perfectly wetted by the Bi-rich phase in a solidified Al-Bialloy.” – p.6881.J.126. Kaptay Gy.: Határfelületi jelenségek a fémesanyaggyártásban. 2.rész. A határfelületiösszehúzó erő – BKL Kohászat, 2009., 142. évf., 6. szám, 37-46. (IF = 0)J.125. J.Sytchev, G.Kaptay: Influence of alkali metal on the erosion of a graphite cathode andmorphology of carbon nanotubes – Electrochim Acta, 2009, vol.54, pp. 6725-6731. (IF =3.325)J125-c1. C.Schwandt, A.T.Dimitrov, D.J.Fray: The preparation of nano-structured carbon materials byelectrolysis of molten lithium chloride at graphite electrodes – J Electroanal Chem, 2010, vol.647, pp.150-158 – „Kaptay and co-workers also investigated the electrolytic preparation method. Carbonaceousproducts were prepared by using various molten salt electrolytes and fundamental studies likewisesuggested alkali metal intercalation into graphite as an essntial step of the process [J125]” – p.151J125-c2. A.R.Kamali, D.J.Fray, C.Schwandt: Thermokinetic characterisation of lithium chloride – J Therm AnalCalorim, 2011, vol.104, pp.619-626. “More recent investigations have shown that intercalation of lithiuminto graphite may also proceed at elevated temperatures as high as 625 to 900 C [J125]” – p.619.J125-c3. AR Kamali, C Schwandt, DJ Fray: Effect of graphite electrode material on the characteristics of moltensalt electrolitically produced carbon nanomaterials – Mater Charact, 2011, vol.62, pp. 987-994. –„Fundamental investigations have reveasled that the molten salt electrolytic formation of carbonnanomaterials commences with the intercalation of alkali metal from the molten salt electrolyte into thegraphitic cathode [J125]” – p.987.J125-c4. C.Schwandt, AT Dimitrov, DJ Fray: High yield synthesis of multi-walled carbon nanotubes fromgraphite by molten salt electrolysis – Carbon, 2012, vol.50, pp. 1311-1315 – „It is generally accepted thatthe first step of the cathodic reduction is the intercalation of the alkali metal into the spacings between thegraphitic layers and the formation of intercalation compounds, MeC x [J125]” – p.1311.J125-c5. A. Juhasz-Szalai, E. Kiss-Toth-Dojcsak, P. Koska, J. Szebeni, B. Fodor: Characteristic features ofcarbon nanotubes and their application in living systems – Egészségtudományi Közlemények, 2012,vol.2, No.1, pp.105-111 – “Several techniques have been developed for the synthesis of CNTs,including …. molten chloride electrolysis [J125]…” – p.106.J125-c6. Hui Huang, Yang Xia, Xinyong Tao, Jun Du, Junwu Fang, Yongping Gan and Wenkui Zhang:Highly efficient electrolytic exfoliation of graphite into graphene sheets based on Li ions intercalation–expansion–microexplosion mechanism - J. Mater. Chem., 2012, vol.22, pp. 10452-10456.J125-c7. A.R. Kamali, G. Divitini, C. Schwandt, D.J. Fray, Correlation between microstructure andthermokinetic characteristics of electrolytic carbon nanomaterials, Corrosion Science (2012), doi:http://dx.doi.org/ - „…the reaction commences with the diffusion-controlled intercalation of Li into thebulk of the graphite cathode, and it has also been considered that Li is simply deposited onto the surfaceof the graphite cathode in case the rate of Li generation is faster than that of Li inward diffusion[J125].”J.124. O. Verezub, Z. Kálazi, G. Buza, N. V. Verezub, G. Kaptay: Classification of laserbeam induced surface engineering technologies and in situ synthesis of steel matrix surfacenanocomposites - Surface Engineering, 2011, vol.27, No.6, pp. 428-435 (2010-IF = 0.633)J.123. Kaptay György: Határfelületi jelenségek a fémesanyaggyártásban. 1. rész. Ahatárfelületi erők osztályozása. BKL Kohászat, 2009., 142. évf., 3. szám, 39-46.o.Helyreigazítás: 2009., 142. évf., 5. szám, 43. o.J.122. O. Verezub, Z. Kálazi, G. Buza, N.V. Verezub, G. Kaptay: In-situ synthesis of acarbide reinforced steel matrix surface nanocomposite by laser melt injection technology andsubsequent heat treatment, Surface & Coatings Technology, 2009, vol. 203, pp.3049-3057.(IF = 1.793)5

J122-c1. E.Laszlo, A.Sytcheva, J.Szucs: Drilling of aluminium alloys and composites – Diáktudomány, AMiskolci Egyetem tudományos diákköri munkáiból, 2010, Miskolc, pp.87-98, ISBN 978-963-661-932-9 –“A kompozitok és nano-kompozitok fejlesztése az egyik fontos mérnöki feladat anyagtudomány ésgépgyártástechnológia határterületén [J122]”.J122-c2. M.J.Hamedi, M.J.Torkamany, J.Sabbaghzadeh: Effect of pulsed laser parameters on in-situ TiCsynthesis in laser surface treatment – Opt Lasers Eng, 2011, vol.49, pp.557-563. – “Recently, theapplications of the titanium carbide (TiC) composites have been increased … [J122]..” – p.557.J122-c3. B.S. Yilbas, S.S. Akhtar, A. Matthews, C. Karatas: Laser treatment of carbon film coated steel surface,Surface Eng, 2012, vol.28, No.1, pp.57-67.J122-c4. Baumli P.: Fémmátrixú kompozitok előállítása öntészeti módszerekkel – CD-Proc. of 26. Int Sci ConfmicroCAD, 29-30 March, 2012. – „Lézer segítségével felületi kompozitok állíthatóak elő. Ebben azesetben a mátrix anyagául szolgáló fém felületét lézerrel megolvasztják, és az így kialakult fémtócsábamegfelelő sebességgel lövik az erősítő fázisnak szánt szemcséket [J122].” – 4.o.J122-c5. A.P.I. Popoola, B.A. Obadele, O.M. Popoola: Effects of TiC-particulate distribution in AISI 304Lstainless steel matrix - Digest Journal of Nanomaterials and Biostructures, 2012, vol. 7, No. 3, pp. 1245 –1252. „In the present investigations, TiC particulate reinforced austenitic stainless steel has beenfabricated using laser processing. Lately, the applications of carbides especially titanium carbide (TiC)composites have increased. This is as a result of the new and promising materials for wearresistant partsand high temperature engineering structural components [J122], high specific strength, low density andhigh elastic modulus.” – p.1246.J.121. I.Budai, G.Kaptay: A new class of engineering materials: particles stabilized metallicemulsions and monotectic alloys, Metall. Mater Trans A, 2009, vol.40A, pp.1524-1528. (IF =1.564)J121-c1. S.E.Friberg: Foams from Non-aqueous systems – Curr Opinion Coll Interface Sci, 2010, vol.15,pp.359-364 – “The analysis of stability and general properties of solid foams, on the other hand, hasgained a separate place in the scientific literature against the fact that their properties are as muchdependent on details of their preparation and manufacturing as on basic collid phenomena and the latterhave first been adequately examined [J121].” – p.359, “In the area of metallic foams truly significantprogress was made by Kaptay and collaborators [121]….” – p. 362.J121-c2. I.Kaban, M.Köhler, W.Hoyer, L.Ratke: Catalytic efficiency of oxide particles on heterogeneousnucleation in aluminium alloy with miscibility gap – Hig Temperatures – High Pressures, 2010, vol.39,pp.347-355. – “Unfortunately, there are practically no data on the wetting of solids at the liquid-liquidinterfaces in metallic monotectic alloys (a short view of the state of the art can be found in the recent workof Budai and Kaptay [J121])” – p.348. „In this case, the advancing contact angle is around 10 degrees andthe receeding contact angle is around zero, which correlates with the results of work [J121] were theperfect wetting of alumina by Bi- and Pb-rich phase has been reported” – p.352.J121-c3. I.Kaban, M.Köhler, L.Ratke, W.Hoyer, N.Mattern, J.Eckert, A.L.Geer: Interfacial tension, wetting andnucleation in Al-Bi and Al-Pb monotectic alloys – Acta mater, 2011, vol.59, pp.6880-6889 – „Budai andKaptay [J121] found that Al 2 O 3 particles were perfectly wetted by the Bi-rich phase in a solidified Al-Bialloy. On the other hand, the contact angle with SiC particles at the interface between two solid phases inan Al-Bi-Si alloy was about 90 o [J121]” – p.6881.J121-c4. T.Frolov, KA Darling, LJ Kecskes, Y.Mishin: Stabilization and strengthening of nanocrystalline copperby alloying with tantalum – Acta Mater, 2010, vol.60, pp. 2158-2168 – “Alloying with immiscibleelemenets is a promising approach to the design of materials with extraordinary structural stability andmechanical strength at high temperatures [J121]” – p.2158.J.120. T.Gábor, F.H.Kármán, J.Sytchev, E.Kálmán, G.Kaptay: The separation of carbonnanotubes from chlorides – Carbon, 2009, vol.47, pp.1195-1198. (IF = 4.504)J120-c1. C.Schwandt, A.T.Dimitrov, D.J.Fray: The preparation of nano-structured carbon materials byelectrolysis of molten lithium chloride at graphite electrodes – J Electroanal Chem, 2010, vol.647, pp.150-158 – „The separation of the nano-structured components from residual salt and unreacted graphite needsto be optimized. In this context, the suitability of a recently developed extraction technique using ethilacetate [J120] will be ascertained” – p.158J120-c2. Graham KA, Kulawiec M, Owens KM, Li XR, Desouki MM, Chandra D, Singh KK: NADPH oxidase4 is an oncoprotein localized to mitochondria, CANCER BIOLOGY & THERAPY 10: (3) Paper 12207.(2010)J120-c3. A. Juhasz-Szalai, E. Kiss-Toth-Dojcsak, P. Koska, J. Szebeni, B. Fodor: Characteristic features ofcarbon nanotubes and their application in living systems – Egészségtudományi Közlemények, 2012,6

vol.2, No.1, pp.105-111 – “Several techniques have been developed for the synthesis of CNTs,including …. molten chloride electrolysis [J120]…” – p.106.J.119. O.N.Verezub, G.Kaptay, G.Buza, N.V.Verezub: The modification of surface layers ofmaterials by laser alloying method. Part II. Laser melt injection technology of instrumentalcarbon steels - Journal of Functional Materials, 2008, vol.2, No.4, pp.137-143. (in Russian).(IF = 0)J.118. O.N.Verezub, G.Kaptay, G.Buza, N.V.Verezub: The modification of surface layers ofmaterials by laser alloying method. Part I. Journal of Functional Materials, 2008, vol.2, No.3,pp.82-91. (in Russian). (IF = 0)J.117. P.Baumli, G.Kaptay: Wettability of carbon surfaces by pure molten alkali chlorides andtheir penetration into a porous graphite substrate – Mater Sci Eng A, 2008, vol.495, pp.192-196. (IF = 1.860)J117-c1. J.F.Cooper J.R.Selman: Electrochemical Oxidation of Carbon for Electric Power Generation: A Review– Abstract Book of the 214th Meeting of the Electrochemical Society, October 2008http://ecsmeet7.peerxpress.org/ms_files/ecsmeet7/2008/12/15/00001942/00/1942_0_art_0_kbxyy3.pdf -„A recent study of graphite wetting in molten chlorides indicates strong dependence on cationiccomposition and temperature [J117]”J117-c2. N.Esutathopoulos, B.Drevet, S.Brandon, A.Virozub: Basic principles of capillarity in relation to crystalgrowth – Chapter 1 in: Crystal Growth Processes Based on Capillarity: Czochralski, Floating Zone,Shaping and Crucible Techniques, ed. by T.Duffar, 2010, John Wiley and Sons Ltd. – „Thethermodynamic adhesion of molten halides on carbon is weak, as ensured solely by physical interactions[J117]. From modeling molten halide / graphite interactions, it was shown that for the same type ofhalides (for instance chlorides), when the surface tension decreases, the work of adhesion increasesrapidly. According to the Young-Dupré equation, this implies a strong decrease in the contact angle(Table 1.8). Table 1.8 Reprinted with permission from [J117], copyright 2008 Elsevier Ltd.” – p.27.J117-c3. X. Liu, Z. Wang, S. Zhang: Molten Salt Synthesis and Characterization of Titanium Carbide-CoatedGraphite Flakes for Refractory Castable Applications – Int J Appl Ceram Technol, 2011, vol. 8, pp.911-919 – „Among the three molten salts, NaCl has the highest viscosity and wets graphite poorly [J117];therefore, the transport of Ti to the surface of graphite will be hindered considerably. Although LiCl hasthe lowest viscosity it does not wet graphite [J117] and consequently the delivery of Ti to the reactionsites on the graphite surface becomes difficult. Differently from these two molten salts, KCl wets graphitewell [J117] and has a low viscosity which facilitates the diffusion of Ti species in it and thus the rapid TiCcoating formation. Thanks to the useful properties of KCl salt mentioned above, the KCl–LiCl eutecticsalt was also effective in the MSS of TiC coatings”. p.914.J117-c4. I.N.Orbulov, I.Kientzl, J.T.Blücher, Á.Németh, J.Dobránszky, J.Ginsztler: Production and investigationof a metal matrix composite pipe – in: Proc of 14th European Conf on Composite Materials, Paper ID:262-ECCM14, 8 pp. – „Efforst have been done to reduce the contact angle either by coating of the fibersor by using three component reinforcement – salt – matrix systems [J117]” – p.2.J117-c5. Kientzl I.: Alumíniummátrixú kompozithuzalok és kettős kompozit-szerkezetek – PhD értekezés, BME(tud. vez.: dr.Dobránszky János), 2010, 112.o. – „.. ha a porózus test egyforma, szorosan pakoltgömbökből van kirakva, akkor a kritikus peremszög 50,7 o [], amire az első kísérleti bizonyítékBaumlitől származik [J117]” – 20.o.J117-c6. I.N.Orbulov, Á.Németh: Infiltration characteristics of carbon fiber reinforced MMCs – Mater SciForum, 2010, vol.659, pp.229-234. – „Effort have been done to reduce the contact angle either by coatingfibers or by using three component reinforcement – salt – matrix system [J117]” – p. 230.J117-c7. Youliang Cheng, Tiehu Liy, Xianliang Hou, Deqi Jing, Qiang Zhuang, Tingkai Zhao: Effects of AlCl 3 -NaCl Content on the Formation of Mesocarbon Microbeads – Int J Chem Reactor Eng, 2010, vol.8, NoteS7, pp. 1-12 – „Moreover, due to the low wettability of carbon and molten salt [J117], the morphology ofobtained mesophase spheres gets more regular.” – p.5.J117-c8. Korenko M, Simko F: Measurement of Interfacial Tension in Liquid-Liquid High-Temperature Systems– J Chem Eng Data, 2010, vol.55, issue 11, pp. 4561-4573. „Baumli and Kaptay [J117] used contact anglemeasurements for the evaluation of surface tension and wettability of several chlorides (KCl, NaCl, RbCl,CsCl) on graphite and glassy carbon substrates” – p.4570.7

J117-c9. I.N.Orbulov: Infiltration of ceramic microballons by liquid metals – research plan for SCIEX-NMS,February, 2011, 12 pp. – „There are many papers int he professional literature which are dealing withthe phenomenon of infiltartion [J117]” – p.9.J117-c10. Z.Tao, Q.Guo, X.Gao, L.Liu: The wettability and interface thermal resitance of copper/graphitesystem with addition of chromium – Mater Chem, 2011, vol.128, pp.228-232 – „.. there exists a criticalcontact angle for spontaneous filling the surface pores of graphite material. This value is around 50 degwhich has been demonstrated both by theory and experiment [J117]”J.116. C.Mekler, G.Kaptay: Calculation of surface tension and surface phase transition line inbinary Ga-Tl system – Mater Sci Eng A, 2008, vol.495, pp.65-69. (IF = 1.860)J116-c1. Zoltai László (+Dúl Jenő): Grafitcsírák keletkezési lehetőségének elméleti vizsglata – 3.kutatószemináriumi dolgozat, Miskolci Egyetem, 2009. február, 48 oldal – „A paraméter a felületirétegben meglévő kötések hányada, ami 1-nél ksiebb pozitív szám, értéke 0,83 [J116]” – 31.o.J116-c2. S.H.Sheng, R.F.Zhang, S.Veprek: Phase stabilities and decomposition mechanism in the Zr-Si-Nsystem studied by combined ab initio DFT and thermodynamic calculation – Acta Mater, 2011, vol.59,pp.297-307 – “The so-called surface phase transition, which has been theoretically predicted by Cahn andrecently elaborated in more detail by Kaptay et al [J116], essentially states that the system will decreasethe high surface energy of the ionic transition metal nitride by wetting it with covalent Si3N4” – p.305.J116-c3. A.Aqra, A.Ayyad, F.Takrori: Model calculation of the surface tension of liquid Ga-Bi alloy – Appl SurfSci, 2011, vol.257, pp.3577-3580 – “It should be noted that the surface tension of liquid solders may becalculated by means of various methods such as Butler method [J116] – p.3578.J116-c4. F.Aqra, A.Ayyad: Theoretical calculations of the surface tension of Ag-Cu liquid alloys – J AlloysCompounds, 2011, vol.509, pp.5736-5739 – “Many attempts have been made to predict the surfacetension of liquid metals and alloys, such as computer simulation with Monte Carlo or molecular dynamicsmethods and models based on Butler's concept [J116]” – p.5736.J116-c5. L.E.Gonzalez, D.J.Gonzalez: Orbital free ab initio simulation of surface freezing in a dilute Ga-Tl alloy– Eur. Phys. J. Special Topics, 2011, vol. 196, pp.15-26. – “A theoretical thermodynamic calculation ofthe surface phase transition line, separating the regions where the segregation of a Tl-rich nanolayer takesplace or does not take place, has been pursued by Mekler and Kaptay [J116]. They obtained goodagreement with the adsorpőtion measurements of Shim et al.” - pp.17-18.J.115. G.Kaptay: A unified model for the cohesive enthalpy, critical temperature, surfacetension and volume thermal expansion coefficient of liquid metals of bcc, fcc and hcp crystals– Mater Sci Eng A, 2008, vol.495, pp.19-26. (corrigendum: see Mater Sci Eng A, 2009,vol.501, p.255.) (IF = 1.860)J115-c1. Zoltai László (+Dúl Jenő): Grafitcsírák keletkezési lehetőségének elméleti vizsglata – 3.kutatószemináriumi dolgozat, Miskolci Egyetem, 2009. február, 48 oldal – „Az irodalmi érték: Fe-g = 2470– 0.32T mJ/, 2 [J115]” – 30.o.J115-c2. A.G.Cherevko: Nukleacionno-fluktuacionnii podhod k opredeleniiu temperaturnoi zavisimostipoverhnostnogo natiazheniia metallov – Kolloidnii zhurnal, 2009, vol.71, No.6, pp.852-859 (Nucleationfluctuationapproach to determining the temperature dependence of the surface tension of metals – ColloidJournal, 2009, vol.71, No. 6, pp. 869-876) – V rabotach [J115] bili naideni korreliacii poverhnostnogonatiazheniia vblizi temperaturi plavleniia s teplotoi plavleniia i moliarnim obiomom” – p.852.J115-c3. V.Morel, A.Bultel, B.G.Cheron: The critical temperature of aluminum – Int J Thermophys, 2009,vol.30, pp.1853-1863 – „Recently, Kaptay [J115] has given a unified model linking the cohesive enthalpy ofa liquid with the melting point of alkali metals. This model also yields fairly good results for other metals.The cohesive enthalpy is defined as the energy existing in the liquid resulting from the mutual atomicattractions, which vanishes when the critical temperature is reached… (2 equations)”- p.1858. “Table 4.New estimates of the critical temperature for aluminium. Method: cohesive enthalpy, Tc = 6548 K.” –p.1861. “Finally, the recommended critical temperature of aluminium, obtained as the average of our ownresults and the latter, is 6700 800 K” – p.1862.J115-c4. F.Aqra, A.Ayyad: Theoretical calculations of the surface tension of liquid transition metals – MetalMater Trans B, 2011, vol.42B, pp.5-8 – “Few published models [J115]… ” – p.7.J115-c5. F.Aqra, A.Ayyad: Surface tension of pure liquid bismuth and its temperature dependence: Theoreticalcalculations, Mater Letters, 2011, vol.65, pp.760-762 – “few established models [J115]…” – p.760.J115-c6. F.Aqra, A.Ayyad: Surface energies of metals in both liquid and solid states – Appl Surf Sci, 2011,vol.257, pp.6372-6379. – “The surface tension of liquids is defined as the ratio of the excess surface Gibbs8

energy (expressed through excess surface enthalpy and excess surface entropy) divided by the molar surfacearea: Eq.(17-18) where f is a geometrical constant (approximately = 1.0) [J115]” – p.6375.J115-c7. F.Aqra, A.Ayyad: Surface tension of liquid alkali, alkaline, and main group metals: theoreticaltreatment and relationship investigations – Metall Mater Trans A, 2011, vol.42A, pp.2680-2684 –„Establishing an accurate, successful, and universal theoretical model for calculating the surface tension ofliquid metals is necessary [J115]” – p.2680J115-c8. F.Aqra, A.Ayyad: Theoretical estimation of temperature-dependent surface tension of liquid antimony,boron and sulfur – Metall Mater Trans A, 2011, vol.42, pp.437-440 – „Few established models are universal[J115], but the agreement with experiment is not satisfactory” – p. 437.J115-c9. F.Aqra, A.Ayyad: Theoretical temperature-dependence surface tension of pure liquid gold - MaterLetters, 2011, vol.65, pp.2124-2126 – „… it is still difficult to identify successfull model for which bothaccuracy and universality apply. Although few established models are universal [J115], but the agreementwith experiment is not very satisfactory” – p. 2124.J115-c10. F.Aqra, A.Ayyad: Surface tension, surface energy and crystal-melt interfacial energy of metals –Current Applied Phys, 2012, vol.12, pp.31-35 – „… it is still difficult to identify successfull model forwhich both accuracy and universality apply. Although few established models are universal [J115], but theagreement with experiment is not very satisfactory” – p. 34.J115-c11. F.Aqra, A.Ayyad: Surface tension of pure liquid lanthanide and early actinide metals – Phys ChemLiquids, 2012, vol.50, pp. 336-345.J.114. P.Baumli, G.Kaptay: Wettability of carbon surfaces by molten alkali chloride mixtures– Mater Sci Forum, 2008, vol.589, pp.355-359. (IF = 0)J.113. G. Buza, V. Janó, M. Svéda, O. Verezub, Z. Kálazi, G. Kaptay, A. Roósz: On thepossible mechanisms of porosity formation during laser melt injection (LMI) technology –Mater Sci Forum, 2008, vol.589, pp.79-84. (IF = 0)J.112. G.Kaptay: A CALPHAD-compatible method to calculate liquid/liquid interfacialenergies in immiscible metallic systems – Calphad, 2008, vol.32, pp.338-352. (IF = 1.530)J112-c1. J.Lee, S.Min, J.Park: Effect of Ce and La on surface property of Bi-Cu-Sn alloys – PPT file of TOFA2008, June 22-27, Krakow, Poland, 23 slides – „new equation and 2 graphs are taken from paper [J112]” –slide 18.J112-c2. J.Park, S.Min, J.Lee: Effect of REM addition on the surface tension and the critical temperature of theimmiscible liquid phase separation of the 60%Bi-24%Cu-16%Sn alloy – Korean J Mater Res, 2009, vol.19,pp. 111-114. – “Recently, Kaptay [J112] suggested a semiempirical equation to predict the interfacialtension between two immiscible liquids based on the models of Chatain et al. and Hoyer et al. Simply, theinterfacial tension can be expressed as Eq.(2) … This equation successfully described the interfcial tensionof the Ga-Pb and Al-Bi systems [J112]” – p.113. “Fig. Cacilated by Eq.(2)” – p.114.J112-c3. J.Li, B.Ma, S.Min, J.Lee, Z.Yuan, L.Zang: Effect of Ce addition on macroscopic core-shell structure ofCu-Sn-Bi immiscible alloy – Mater Letteres, 2010, vol.64, pp.814-816 – “Kaptay [J112] suggested that theinterfacial tension between two immiscible liquids could be expressed by the equation: …{Eq.2}… “ – p.2.Fig.4. Temperature dependence of interfacial tension of the 24Cu – 16Sn – 60 Bi alloy with 0.05 wt % Ceaddition, calculated using Eq.(2)” – p.815.J112-c4. Mende T.: Az ESTPHAD módszer fejlesztése és alkalmazása kettő-, három- és négyalkotós rendszereklikvidusz hőmérsékletének közelítésére, PhD értekezés, (tud. vez.: Roósz A.), 2010, Miskolc, 129 o. – “A4.33 ábrán a szakirodalomból származó [J112] és a 31. egyenlettel számított szétválási görbe látható. 4.18.táblázat [J112]” – 65.o, „A reguláris elegymodellből levezethetően a szétválási hőmértésklet koncentrációfüggésérea következő egyenlet írható fel [J112]: (34) egyenlet.” – 67.o.J112-c5. Mende T., Roósz A.: Egyensúlyi fázisdiagramok nonvariáns pontjainak nagy pontossággú számításaEstphad módszerrel – BKL Kohászat, 2011, vol.144, No.3, pp.47-50.J112-c6. L.Zhao, J. Zhao: Microstructure formation in a gas-atomized drop of Al-Pb Immiscible alloy – MetallMater Trans A, 2012, doi: 10.1007/s11660-012-1313-3. – “”The critical temperature for a ternaryimmiscible alloy is determined by the alloy composition [J112]” -9

J111. G.Kaptay: Link between the semi-empirical Andrade and Shytil equations and thestatictical-mechanical Born-Green equation for viscosity and surface tension of pure liquidmetals – Metall Mater Trans B, 2008, vol.39B, pp.387-389. (IF = 0.798)J110. G.Kaptay: A new theoretical equation for temperature dependent self-diffusioncoefficient of pure liquid metals – Int J. Mater Res. (formerly Z. Metallkunde), 2008, vol.99,pp.14-17. (IF = 0.819)J110-c1. S.Yang, X.Su, J.Wang, F.Yin, Z.Li, S.Chen, C.Liu: Temperature-evolution of structure and diffusionproperties of liquid transition metals – J Non-Crystalline Solids, 2010, vol.356, pp.1061-1069 – „… arecently derived predictive equation for temperature dependence of self-diffusion coefficients of liquidmetals [J110] has been applied to give theoretical prediction. The new equation was derived combining aunified equation on the viscosity of pure liquid metals with the well known Sutherland-Einstein equationwithout any adjustable parameters. The perfect agreement of the prediction of this new equation with theexperimental values measured under micro-gravity conditions confirms its applicability. The equation hasbeen derived as: {Eq.4}… + 10 lines. The performance of the present MD study was evaluated bydetermining relative difference between the calculated and theoretical prediction values. .... The values arelisted in Table 1. Table 1. Simulated self-diffusion coefficients of liquid transition metal – 1 coloumn iscalculated by Eq.(4) [J110]”.J110-c2. DL Beke: On the composition and pressure dependence of the self-diffusion coefficient in liquid metals– Int J Mater Res, 2010, vol.101, 353-355. - „In a very recent paper Kaptay [J110] presented a unifiedequation for the temperature dependence of the self-diffusioin coefficient, D, in liquid metals. It ismentioned in [J110] that the result is also a prepequisite for modeling of the composition and pressuredependence of D.” – p.353. “.. fortunately this data collection and trial to get a relation expressing at leastthe non-reduced values of D as the function of T was already done in [J110]. Thus it is worth to comparerelation (5) with the results of [J110]: {2 equations, 9 lines copied from [J110]}. – p.354. “The use of the socalled“corrected” melting point for semi metals is a good trial in [J110]: indeed for these elements themelting point is not a good measure of the bonding strength because during melting there are changes in theelectronic structure” – p.354.J110-c3. Beke DL.: Composition and Pressure Dependence of the Diffusion Coefficients in Binary LiquidAlloys – Defect and Diffusion Forum, 2010, vol.297-301, pp.1371-1376. – „Data collection and trial to get arelation expressing at least the non-reduced values of D as the function of T* has already been done [J110].… Furthermore it was shown in [J110] that in fact the logarithm of F2*(T*) is a good linear function ofTm/T (see Figs 1-2 in [J110].” – p.1373.J110-c4. AA Simonova: Obespechenie neobhodimogo kachestva poverhnostnogo sloia obiomnichnanokristallicheskich metallov posle mechanicheskoi obrabotki – Naukovi Notatki (Inzhenerna mechanika),No.24, 2009, Luck, pp.500-506 – „Nabliudeniia, predstavlennie v rabote [J110] pokazali, shto….” – p.503.J109. G.Kaptay: The threshold pressure of infiltration into fibrous preforms normal to thefiber’s axes – Composites Science and Technology, 2008, vol.68, pp.228-237. (IF = 2.533)J109-c1. I.Kientzl, J.Dobránszky: Production and behaviuour of aluminium matrix double composite structures –Mater Sci Forum, 2008, vol.589, pp.105-110 – “Kaptay’s equation describes the threshold pressure asfunction of the contact angle and smallest separation of the fibers divided by the fibre diameter. Thethreshold pressure of non-wetting liquids is found to be inversely proportional to the smallest distancebetween the fibers although it is commonly beleived to be inversely proportional to the diameter of thefibres. Four different cases were distuinguished based on the wettability of fibres and the sapce between thefibres and the equations of thrshold pressures were worked out for all these cases [J109]” – p.105-106.„Based on Kaptay’s method the threshold pressure was calculated and plotted as function of the contactangle and relative distance between the fibers (Fig.2).” – p.107.J109-c2. Orbulov I, Németh Á, Dobránszky J: Manufacturing of Composites by Pressure infiltration, Structureand Mechanical Properties. In: Penninger A, Váradi K, Vörös G (eds.), Gépészet 2008, Proceedings of SixthConference on Mechanical Engineering, BUTE Faculty of Mechanical Engineering – “This thresholdpressure can be calculated by theoretical approaches for various systems [J109]” – p.1/9.J109-c3. Orbulov IN, Németh Á, Dobránszky J: XRD and EDS Investigations of Metal Matrix Composites andSyntactic Foams. 13th European Conference on X-Ray Spectrometry, Cavtat, Croatia, 16-20 June 2008, In:EXRS 2008 Proceedings – “The main parameter in this case is the infiltration pressure, which can beapproximated numerical calculations and is influenced by wetting” – p. 2/10.J109-c4. Kientzl I.: Alumínium mátrixú kompozithuzalok és kettőskompozit szerkezetek – PhD értekezés, 2010.,BME (tud. vezető: Dobránszky János). – „G. Kaptay azonban pontosan egy ilyen számítási módszertmutatott be cikkében határfelületi megfontolásokra alapozva munkáját [J109]. Az ebben a cikkben10

emutatott számítási eljárást ismertetem a következőkben (+ 1 oldal, 2 ábra és 16 egyenlet a cikkből)” – 21-22. o., „… a szálak olvális keresztmetszetűek, hosszirányban 12 μm, keresztirányban 7 μm, így a Kaptayáltal adott módszer, ami kör keresztmetszetű szálakra lett kidolgozva, csak közelítő számításokra alkalmasebben az esetben – 42. ábra” – 44.o.J109-c5. I.N.Orbulov, I.Kientzl, J.T.Blücher, Á.Németh, J.Dobránszky, J.Ginsztler: Production and investigationof a metal matrix composite pipe – in: Proc of 14th European Conf on Composite Materials, Paper ID:262-ECCM14, 8 pp. – „This threshold pressure can be estimated by theoretical approaches for variouswetting or non-wetting systems [J109]” – p.2.J109-c6. Qi LH, Xu R, Su LZ, Zhou JM, Guan JT: Dynamic measurement on infiltration process and formationmechanism of infiltration front – Trans. Nonferr Metals Soc China, 2010, vol.20, pp.980-986 – „As anindispensable step int he fabrication technologies of metal matrix composites (MMC), the liquid metalinfitration process in porous preform, such as squeeze casting, vacuum infiltration, variable pressureinfiltration and liquid infiltration-extrusion, have attracted research interest due to the significantlyeffective improvement int he properties of composite products [J109]” – p.980.J109-c7. Kientzl I.: Alumíniummátrixú kompozithuzalok és kettős kompozit-szerkezetek – PhD értekezés, BME(tud. vez.: dr.Dobránszky János), 2010, 112.o. – „.. Kaptay a hengeres szálak közé való infiltrálástvizsgálta [J109]. Az eredmények szerint a szálakkal párhuzamosan a kritikus peremszög 90 o , míg azokramerőlegesen sokkal kisebb 90 o -nál. A konkrét peremszög értéke függ a szálak térkitöltésétől…” – 20.o.„Kaptay egy új számítási módszert mutatott be határfelületi megfontolásokra alapozva munkáját [J109] +2 oldal + 14 egyenlet + 2 ábra idézet” – 21-23. o. „A Kaptay modell. 1,5 oldal elemzés… A Kaptaymodell a folyamatos infiltrációhoz szükséges küszöbnyomást 0,20 – 0,77 MPa értékre becsüli. Ez atartomány a kísérleti eredményekből származó 0,62-0,83 MPa intervallummal átfedésben van, tehát ez amodell magyarázatot ad a folyamatos infiltráció nyomás-szükségletére… Összefoglalva megállapítható,hogy a White-Mortensen és a Kaptay modellek közül csak a Kaptay-modell mutatott átfedést a mérésieredményeimmel” – 60-64. oldalak. „A Kaptay-model által adott küszöbnyomásfüggvény alapján a szálakritkább elrendeződése esetén, még nagy peremszögek mellett sem nő jelentős mértékben a folyamatosinfiltrációhoz szükséges küszöbnyomások értéke” – 83.o. „2.tézis. A küszöbnyomás 0,62-0,83 MPa-osintervallumát összevetettem két elméleti modellel… .. tehát a kísérleti eredményeim matematikaiközelítésére a Kaptay modell alkalmas” – 84.o.J109-c8. I.N.Orbulov, Á.Németh: Infiltration characteristics of carbon fiber reinforced MMCs – Mater SciForum, 2010, vol.659, pp.229-234. – The threshold pressure can be estimated by theoretical approachesfor various wetting or non-wetting systems [J109]” – p. 230.J109-c9. I Kientzl, J Dobránszky, Á Németh: Effect of the Infiltration Pressure on the Properties of CompositeWires- Materials Science Forum, 2010, vol. 659, pp.177-182. – „Kaptay's equations describe the thresholdpressure as a function of the contact angle and smallest separation of the fibres divided by the fibre diameter[J109]. The threshold pressure of non-wetting liquids is found to be inversely proportional to the smallestdistance between the fibers … „ p.177J109-c10. L.H.Qi, L.Z.Su, J.M.Zhou, J.T.Guan, X.H.Hou, H.J.Li: Infiltration characteristics of liquid AZ91Dalloy into short carbon fiber preform – J Alloys Compds, 2012, vol.527, pp.10-15. – „… much researchwork had also been conducted on the calculation of the threshold pressure for initiation of infiltration[J109]” – p.10.J109-c11. Seung-Wook Han, Nak-Sam Choi and Min-Soo Lee: Analysis of glass fabric impregnation using aresin drop method - J Mechan Sci Technol, 2012, vol. 26, pp. 1477-1482 – “The interplay between thesurface tension of the infiltrating liquid, the wettability of the fibers by the surrounding liquid and themorphological details of the preform fabric directly affects the integrity of the manufactured composites[J109]” – p.1477.J109-c12. MA You-ping, LI Xiu-lan, WANG Cheng-hui, LU Lu: Microstructure and Impact Wear Resistance ofTiN Reinforced High Manganese Steel Matrix – J Iron Steel Res Int. 2012, vol. 19, No. 7, pp. 60-65 – „Themost common surface treatment route is the liquid metal infiltration …. Infiltration technique has beensuccessfully applied in wear parts [J109]” – p.60.J108. K.Wasai, G.Kaptay, K.Mukai, N.Shinozaki: Modified classical homogeneous nucleation theroyand a new minimum in free energy change 2. Behavior of free energy change with a minimumcalculated for various systems - Fluid Phase Equilibria, 2007, vol.255, pp.55-61. (IF = 1.506)11

J108-c1. S.Min, J.Park, J.Lee: Surface tension of the 60%Bi-24%Cu-16%Sn alloy and the critical temperature ofthe immiscible liquid phase separation – Mater Lett, 2008, vol.62, pp.4464-4466 – „In order to control thestructure of the core-shell lead-free solder ball, the surface tension and the interfacial tension between twoimmiscible liquid alloys are required [J108]” – p.4464.J108-c2. Verezub O.: Lézeresen felületkezelt szerszámacél köszörülése – Gyártóeszközök, szerszámok,szerszámgépek, 2008, No.1, pp.65-68. – „A nanométer tartományba tartozó szemcsék kiválásánakfelételeiről lásd [J108]” – p.66.J108-c3. Zoltai László (+Dúl Jenő): Grafitcsírák keletkezési lehetőségének elméleti vizsglata – 3.kutatószemináriumi dolgozat, Miskolci Egyetem, 2009. február, 48 oldal – „Mivel a SiC képződése során azolvadék Si- és C-tartalma csökken, a nano méretű SiC csírák stabiliázlása elméletileg lehetséges [J108]” –2.o. „Wasai, Kaptay, Mukai és Shinozaki ismerték fel először [J108], hogy csíraképződés során azolvadékfázis Gibbs energiája változásának figyelmen kívül hagyása oda vezet, hogy a csíraképződési görbeegyébként létező minimum pontja nem jelenik meg… A levezetés [J108] a nemrég publikált cikkekegyszerűsített változata – 2 oldal egyenletek” – 40. o.J.107. Gábor T., Kármánné H.F., J.Sytchev, Kaptay Gy., Kálmán E.: Sóolvadékok elektrolízise soránkialakult szén nanocsövek kinyerése és minősítése – BKL Kohászat, 2007, vol.140., No.2, pp. 43-50.(IF = 0)J106. K.Wasai, G.Kaptay, K.Mukai, N.Shinozaki: Modified classical homogeneousnucleation theroy and a new minimum in free energy change 1. A new minimum and Kelvinequation – Fluid Phase Equilibria, 2007, vol.254, pp.67-74. (IF = 1.506)J106-c1. Verezub O.: Lézeresen felületkezelt szerszámacél köszörülése – Gyártóeszközök, szerszámok,szerszámgépek, 2008, No.1, pp.65-68. – „A nanométer tartományba tartozó szemcsék kiválásánakfelételeiről lásd [J106]” – p.66.J106-c2. Zoltai László (+Dúl Jenő): Grafitcsírák keletkezési lehetőségének elméleti vizsglata – 3.kutatószemináriumi dolgozat, Miskolci Egyetem, 2009. február, 48 oldal – „Mivel a SiC képződése során azolvadék Si- és C-tartalma csökken, a nano méretű SiC csírák stabiliázlása elméletileg lehetséges [J106]” –2.o. „Wasai, Kaptay, Mukai és Shinozaki ismerték fel először [J106], hogy csíraképződés során azolvadékfázis Gibbs energiája változásának figyelmen kívül hagyása oda vezet, hogy a csíraképződési görbeegyébként létező minimum pontja nem jelenik meg… A levezetés [J106] a nemrég publikált cikkekegyszerűsített változata – 2 oldal egyenletek” – 40. o.J106-c3. Carreon-Calderon B., Soria A., Romero-Martinez A.: Driving Force in First-Order Phase Transitionsand Its Application to Gas Hydrate Nucleation from a Single Phase - AICHE Journal, 2009, vol.55, pp.2433-2447. – „.. authors consider the nucleation work as a maximum of the free energy surface” – p.2434.J106-c4. Teychene S., Biscans B.: Microfluidic Device for the Crystallization of Organic Molecules in OrganicSolvents – Crystal growth & Design, 2011, vol.11, pp.4810-4818. -J105. G.Kaptay: On the wettability, encapsulation and surface phase transition in monotecticliquid metallic systems – Materials Science Forum, 2007, vol.537-538, pp.527-532 (IF = 0)J105-c1. Svéda Mária: Monotektikus felületi rétegek létrehozása lézersugaras felületkezeléssel c. PhDértekezéséhez (tudományos vezető: dr. Roósz András) – 2007. – „A nagyobb sűrűségű Pb olvadéknak azötvözett zóna felszínén való elhelyezkedése a határfelületi jelenségekkel magyarázható [J105]” – p.87.J104. I.Budai, M.Z.Benkő, G.Kaptay: Comparison of different theoretical models toexperimental data on viscosity of binary liquid alloys – Materials Science Forum, 2007,vols.537-538, pp.489-496. (IF = 0)J104-c1. D.Zivkovic: Application of the Kaptay model in calculation of ternary liquid alloys viscosities – Int JMat Res, 2008, vol.99, pp.748-750 – „Kaptay’s approach to estimate the viscosity of liquid metallic alloysfrom viscosities of pure liquid metals and thermodynamic properties of the liquid alloy has been tested fordifferent types of binary systems [J104], including those with considerable deviations from ideality” –pp.748-749.J104-c2. D.Zivkovic: A new approach to estimate the viscosity of the ternary liquid alloys using the Budai-Benko-Kaptay equation – Metall Mater Trans B, 2008, vol.39, pp.395-398 – „The new Budai-benko-Kaptay (BBK) equation has been recently derived for estimation of the viscisity of liquid alloys and testedon numerous binary systems, showing a good agreement with experimentally obtained data. Equations….… The presented new BBK equation for estimation of the viscosity of liquid metallic alloys has been12

already tested for different types of binary systems [J104], showing good compliance with experimentaldata in most cases. IN this article, the applicability of a new equation to ternary systems will be tested inexamples of Au-Ag-Cu alloys. „ – p.395, „There is an agreement between the results of the BBK equationapplication, presented in this work and the experimental literature data… the ability to predict theviscosity, even if the viscosities of the pure componnets are not known, should be underlined int heapplication of the new BBK equation and taken as an advantage among other models int he case whenthese data are not known” – p.396. „The greatest advantage of the presented BBK equation is to beaccetuated – such estimation of the viscosities of multicomponent liquid alloys demands just a fewstarting data for the calculation compared to the other known models, which makes it simple and easy toapply in different cases” – p.397.J104-c3. V.Skliarchuk, A.Iakimovich, M.Dufanec: Rozrahunok viazkosti rozplaviv sistemi Al-Cu –Vseukrainska konferencia molodich vchonich “Suchasne materialoznavstvo: materiali ta technologiiSMMT-2008. (PPT file of a conference talk) – “Modifikovane rivnannia Budai-Benko-Kaptay [J104] ….“ – p. 4, “Rozrahovani znacheniia viazkosti zgidno modeli Chabra i modifikovanogo rivnannia Budai-Benko-Kaptay dobre uzgodzhuiutsia z literaturnimi dannimi“ – p.9.J104-c4. Sklyarchuk VM, Yakimovich AS, Dufanets' MV: Calculation on Viscosity of Al-Cu Liquid Alloys –Metallofizika i noveishie technologii, 2008, vol.30, pp., 315-321.J104-c5. P.Terzieff: The viscosity of liquid alloys of polyvalent metals with Cu, Ag and Au: Theoreticaltreatments based on the enthalpy of mixing – Physica B, 2009, vol.404, pp. 2039-2044 – „The majority ofthe currently used viscosity models are of semi-empirical nature focused on thermodynamic quantitiessuch as enthalpy of mixing [J104]” – 2039, “The extension toi the case of multi-component systemsinvolves the volume of mixing and the enthalpy of mixing as additional input parameters [J104]: Eq.(3)” –p.2040, “Fig-s 1-10: “unified model”” – pp.2041-2033, “The least strenuous way to calculate viscosities isgiven by the unified equation of Kaptay and coworkers [J104]. Except for the Ag-Sb and some extent toCu-Sb, the excess viscosities are in reasonable numerical agreement with the experimental values (Table1). Apart from the model’s obvious overestimation of the viscosity of pure liquid Cu in Cu-BI, Cu-Pb andCu-Sn (Figs 2, 3 and 5) or the disagreement in the values of undercooled Au in Au-Sn (Fig.10) the shapesof the viscosity isotherms are found to be adequately reproduced (curves b). However, it has to be alsonoted that the experimental values reported for liquid Cu differ from one author to the other by more than1 mPaseven at the same temperature (Figs 3. and 4.). The additional isotherms (curves b’) shown for Cu-Bi, Cu-Sb, Ag-Ge and Ag-Sb were obtained by using the corrected melting temperatures for Ge (450 K),Sb (650 K) and Bi (450 K) as recommended by Kaptay [J104]. As compared to the isotherms obtainedwith the uncorrected melting temperatures (curves b) the improvemenets are extremely large for Ag-Ge(Fig.6), less pronounced for Cu-Sb and Ag-Sb (Figs 4, 8) and small for Cu-Bi (Fig.2).” – p.2043.J104-c6. P.Terzieff: Some physico-chemical properties of liquid Ag-Sn-Zn – Physica B, Condensed Matter,2010, vol.405, pp.2668-2672 – From a previous analysis it has been concluded that the semi-empiricalapprach based on Kaptay’s unified equation [J104] is one of the most convenient methods to gain a firstidea of the viscosity of muticomponent systems, even if the viscosities of the pure liquids are unknown.The application requires the melting temperatures of the components, their molar masses, and their molarvolumes. The only requirements for alloy is the knowledge of the excess volume and the enthalpy ofmixing : (Eq.10)” – p.2674.J104-c7. Gasior W, Moser Z, Debski A: New data to the SURDAT-database of modeled and experimentalphysical properties of lead-free solder alloys – Arch Metall Mater, 2009, vol.54, pp. 1253-1259 –„..SURDAT database … experimental … and the viscosity calculated from the dependences proposed by… Kaptay [J104] : Eq.(6)” – p.1256. “Fig.4. Experimental (symbols) and calculated (lines) viscosity (Eq-s(1, 2, 5, 6, 7) of Ag-Sn (Fig.4a) and Sn-Zn (Fig.4b) alloys” – p.1257.J104-c8. Knott S., Terzieff P.: Calculation of the viscosity of the liquid ternary Ag-Au-Sn system – Int. J. Mater.Res., 2010, vol.101, pp.834-838. – „Several viscosity models based on thermodynamic data exist, some ofthem apply adjustable parameters, while others make use of universal parameters [J104] which a reconsidered to be applicable to a large class of alloy systems” – p.834, “The expression for the viscosity,given by Budai et al. [J104] is based on Kaptay-s unified equation for pure liquid metals: Eq.(3)” – p.835.Fig-s 2, 4 and Table 2 are calculated by the model [J104] – pp.836-837. “…the unified equation yields amuch better agreement for Ag-Au system” – p.836. “Conclusions: .. in case of missing experimentalevidence the unified equation might give a first reasonable estimate of the viscosity in liquidmulticomponent systems” – p.838.J104-c9. Wunderlich RK; Fecht H-J: Surface tension and viscosity of NiAl catalytic precursor alloys frommicrogravity experiments – Int J Mater Res, 2011, vol.102, pp.1164-1173. „The Kaptay model was shownto provide better agreement with observed viscosities of binary alloys [J104] than the Moelwyn-Hughesmodel. In the Kaptay model the viscosity is given by: Eq-s.(15-16), Fig.11, Table 2.” – p.1170-1171.13

J104-c10. R.N.Singh, F.Sommer: Viscosity of liquid alloys: generalization of the Andrade’s equation – MonatshChem, 2012, vol.143, pp.1235-1242. – „Results obtained from these relations have been compared withnew or given [J104] experimental viscosity data as a function of composition and temperature.” – p.1235.“A comparison of available semi-empirical models with experimental data of the viscosity of liquid alloyshas been given recently [J104]” – p.1241.J103. Baumli P., Sytchev J., Kaptay Gy.: SiC és Al 2 O 3 kerámia szemcsék felületkezelése sóolvadékban, kompozitok fejlesztése céljából – BKL Kohászat, 2006., 139. évf., 3.szám, 47-50. (IF = 0)J103-c1. Orbulov I., Kientzl I., Németh Á.: Fémhabok és kompozitok előállítása infiltrálásos eljárással – BKLKohászat, 2007, vol.140, No.5, pp.41-46. – „Nagyon fontos, hogy a fémmátrixú kompozitanyagokesetében is csak akkor kapunk megfelelő műszaki tulajdonságokat, ha megfelelő a kapcsolat azerősítőanyag és a mátrixanyag határfelületén [J103]” – p.41.J103-c2. Orbulov I.: Szintaktikus fémhabok keménységmérése – Anyagvizsgálók lapja, 2009, No.1, pp.9-15. –„… vizsgálatok tárgyát képezték az erősítőanyagra felvihető különböző bevonatok is [J103].” – p.9.J102. G.Kaptay: On the equation of the maximum capillary pressure induced by solidparticles to stabilize emulsions and foams and on the emulsion stability diagram - Colloidsand Surfaces A: Physicochem. Eng. Aspects, 2006, vol.282-283, pp.387-401. (IF = 1.611)J102-c1. Gonzenbach UT, Studart AR, Tervoort E, Gauckler LJ: Tailoring the microstructure of particlestabilizedwet foams - LANGMUIR 23 (3): 1025-1032 JAN 30 2007 - „These results suggest that thepreparation of wet foams that are stable against bubble coarsening and drainage requires particle sizesnot larger than a few micrometers in diameter. Theoretical calculations based ont he adsoroption energyof particles at gas – liquid interface and the maximum capillary pressure developed at the interfaceshowed that particles larger than about 3 microns are not able to stabilize foams for long period of time[J102]. These results are in the same order of magnitude as our experimental findings” – p.1029.J102-c2. C.Körner: Integral Foam Molding of Light Metals – Physical and Technological Principles –Habilitation Thesis, Erlangen, 2007 (Ref. No.132) – “Kaptay was the first who realized that stabilizationfor these kind of particles is based on the development of 3D network structures which transfer forcesfrom one interface to the other [J102].” – p.108.J102-c3. Torres LG, Iturbe R, Snowden MJ, Chowdhry BZ, Leharne SA: Preparation of o/w emulsions stabilizedby solid particles and their characterization by oscillatory rheology - COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS 302 (1-3): 439-448 JUL 20 2007 – “Themagnitude of the free energy required to remove a particle from the interface between two immisciblefluids does not provide an insight into the stability of the emulsions [J102]…. It is reported that the waterfil between two drops of the discontinuous oil phase resists rupture if the contact angle of the stabilisingparticle is in the range of 15 – 90 degrees [J102]” – p.440.J102-c4. Studart AR, Gonzenbach UT, Akartuna I, Tervoort E, Gauckler LJ: Materials from foams andemulsions stabilized by colloidal particles - JOURNAL OF MATERIALS CHEMISTRY 17 (31): 3283-3289 2007 – “… stabilization is achieved for intermediate contact angles ranging from 20 to 86 deg foroil-in-water emulsions and foams, and from 94 to 160 deg for water-in-oil emulsions and mists [J102]” –p.3285, “Besides the high energy of adsorption of particles at the interface, the remarkable resistance ofparticle-stabilized foams and emulsions against coalescence has also been attributed to the development ofcapillary forces that impede thinning down the liquid film between bubbles/droplets, as well as to theformation of an attractive network of particles throghout the continouos liquid phase [J102]” – p.3286.J102-c5. SE Friberg, AA Bawab, AA Abdoh: Surface active inverse micelles – Colloid Polym Sci, 2007,vol.285, pp.1625-1630 (Ref. No.17) – “Finally Professor Kaptay [J102] has published a completetreatment on the influence of solid particles on the capillary pressure in their stabilization of emulsionsand foams” – p.1628.J102-c6. Orbulov I., Kientzl I., Németh Á.: Fémhabok és kompozitok előállítása infiltrálásos eljárással – BKLKohászat, 2007, vol.140, No.5, pp.41-46. – „A másik csoportba sorolhatjuk azokat az anyagokat, amelyeklétrehozásánál vagy csak a tömegcsökkentés, vagy valamilyen más különleges követelmény dominál.Ezek a porózus szerkezeti anyagok [J102]” – p.41.J102-c7. L.Torres, R.Iturbe, MJ Snowden, B. Chowdhry, S.Lehrane: Can Pickering emulsion formation aid theremoval of creosote DNAPL from porous media? – Cemosphere, 2008, vol.71, pp.123-132 – “There are,however, problems with the model that undepints the development of Eq.(1) (of Binks). For example themodel does not explain experimental observation that particle stabilised emulsions are maximallystabilised when the particles display a contact angle less than 90 o [J102]…. The role of the particles in14

film stabilisation can be incorporated into a model which then predicts that the film between two drops ofthe discontinuous oil phase resists rupture if the contact angle of the stabilising particlesis in the rangebetween 15 and 90 deg [J102]” – p.125.J.102-c8. TN Hunter, RJ Pugh, GV Franks, GJ Jameson: The role of particles in stabilizing foams and emulsions– Adv. Colloid Interface Sci., 2008, vol.137. pp.57-81 – “A recent review by Kaptay [J102] has broughtthis mechanism back into focus, and it will be briefly surmised here. Kaptay [J102] derived …. 61 lines +Figures 4-5 + Equation (2) ” – pp.62-63.J102-c9. T.S. Horozov: Foams and foam films stabilised by solid particles - Curr Opinion in Colloid InterfaceSci, 2008, vol.13, pp.134-140. – „Several recent works [J102, etc.] treat the problem of liquid filmstability by solid particles theoretically, assuming either a bridging monolayer or a bilayer of hexagonallyclose-packed particles.” – p.137. „A recent review on this subject by Kaptay [J102] is worth to consider.There, previous and more recent theoretical results are analysed and semi-empirical equations for thedependence ofmaxP on the particle contact angle are obtained with the toroidal pore model. Resultsccalculated by these equations are compared in Fig.3….. description of Fig.3 (19 lines + 7 lines of figurecaption [J102])…” – p.138, „Another mechanism of foam film stabilisation by a network of particleaggregates (gel) inside the film has also been discussed in [J102] (Fig.2.c). … description (7 lines)…” –p.138, „Link between the stability of particle stabilised aqueous films and that of particle-stabilised foamsor oil-in-water (o/w) emulsions has also been discussed [J102] … description (15 lines)… .Semiquantitative arguments have been used to estimate the optimum contact angles for the highest foam(o/w emulsion) stability [J102]…decription (3 lines)…” – pp.138-139, „Smaller particles should stabilisethe film better but their attachment to the liquid surface is weaker and vica versa [J102].” – p.139. „Agood review of theoretical studies on liquid films stabilised by solid particles. Useful approximatedequations for the dependence of critical capillary pressure for film rupture on the particle contact angle areobtained. Mechanism of liquid film stabilisation by solid particles are discussed” – p.140.J102-c10. S Ata: Coalescence of bubbles covered by particles – Langmuir, 2008, vol.24, pp.6085-6091. – „Themechanism of film stabilisation has been explained by the capillary pressure between bubbles, given by{equation}. The theory was first proposed by Ivanov and co-workers and developed further by others[J102]” – p.6086-6087.J102-c11. I.Akartuna, AR Studart, E.Tervoort, UT Gozenbach, LJ Gauckler: Stabilization of oil-in-wateremulsions by colloid particles modified with short amphiphiles – Langmuir, 2008, vol.24, pp.7161-7168.– „The adsoroption energy increases monotonically with increasing contact angle reachin a maximum at90 degrees. Besides a strong adsorption at the interafce, the stabilization of emulsions also requires thatthe adsorbed particles impede thinning of the liquid film between droplets. In contract to the adsorptionenergy, earlier studies have shown that the highest resistance against film thinning is achieved forparticles forming contact angles approaching 0 and 180 degrees [J102]. COnsidering these oppositetrends, optimum contact angles between 70 and 86 degrees and between 94 and 110 degrees have beensuggested for the stabilization of oil-in-water and water-in-oil emuslions, respectively, using interfacialadsorbed particles [J102]. Under such conditions, particles should be able to sterically hinder thecoalescence of droplets over long periods of time, which has been experimentally confirmed in a numberof recent studies” – p.7161.J102-c12. H.A.Wege, S.Kim, V.N.Paunov, Q.X.Zhong, O.D.Velev: Long-term stabilization of foams andemulsions with in-situ formed microparticles from hydrophobic cellulose – Langmuir, 2008, vol.24,pp.9245-9253. „Removing such particles from interface requires the expense of a significant transfereneregz, whose magnitude can be estimated by [J102]: (Eq.1).” – p.9245.J102-c13. C.Körner: Foam formation mechanism in particle suspensions applied to metallic foams – Mater SciEng A, 2008, vol.495, pp.227-235 – “Further progress to explain foam stability was made by Kaptay[J102] who uses a model of a three-dimensional network of solid, spherical particles to explain forcetransfer between two interfaces and in this way stability” – p.228.J102-c14. A.J.Klinter, G. Mendoza-Suarez, R.A.L.Drew: Wetting of pure aluminum and selected alloys onpolycrystalline alumina and sapphire – Mater Sci Eng A, 2008, vol.495, pp.147-152. – “Recently it hasbeen derived that the most favorable ciontact angle range for a liquid foam to be stabilized by particlesis between 70 and 86 degrees [J102]. An experimental simulation conducted by Sun et al employingethanol/water mixture and polymeric particles supports this finding showing that the most stable foamswere obtained when the liquid wetted the particles in a range of 70-85 degrees. Therefore, it is assumedthat in order to produce stable aluminum foams, the aluminum alloy melt needs to wet the addedceramic particles in this optimum contact angle range of 70-86 degrees over the temperature spanbetween that of the melt bath in the direct foaming method (typically around 750 – 800 Centigrades)and the solidification of the alloy” – p.148.J102-c15. A.J.Klinter, R.A.L.Drew: Evaluation of the wetting behaviour of Al-7Cu and Al-11.5Si on SiC andsapphire in terms of Al-foam stability. In: METFOAM-2007, ed. by L.P.Lefebre, J.Banhart, D.C.Dunand,15

DEStech Publ. Inc, 2008, pp.23-26. – „During the early stages of Al-foam rersearch, it was found thatalumina or SiC particles are essential in order to obtain stable aluminium foams. Originally it wasbelieved that the stabilizing effect of these ceramic particles have on Al-foams was caused by an increasein bulk viscosity of the Al melt due to ceramic particles additions. In a very theoreticla approach,KAPTAY [P41, J84] later developed models suggesting that the improved foam stability was due tocapillary effects between the melt and the particles, preventing the two liquid gas interfaces of a foam cellwall from touching, and the two adjacent cells from coalescencing….. KAPTAY concluded recently in acomplex and theoretical study [J102] that the optimum contact angle for foam stabilization by a single ora closely packed double layer of particles is between 70 and 86 degrees” – p.23. „Fig-s 5 show that Al-11.5Si wets the substrate better than Al-Cu, however neither alloy reaches the optimum contact anglerange for foam stabilization [J102]” – p.25. „Conclusions. … A number of researchers have shown thatmetal foams can be produced using a verity of aluminum alloy – ceramic particle combinations (includingAl2O3, SiC and TiB2). Nevertheless, it is believed that foams with narrower pore size distribution andmore homogeneous properties can be produced if alloy-particle combinations are chosen with wettingproperties int he optimum contact angle range for foam stabilization by particles of 70 to 86 degreesderived by KAPTAY [J102]” – p.26.J102-c16. C.Koerner: Integral Foam Molding of Light Metals – Springer, 2008, 224 pp. – „ Kaptay [J102] wasthe first who realized, that stabilization for this kind of particles is based on the development of 3Dnetwork structures which transfer forces from one interface to the other” – p. 100.J102-c17. Hunter, T.N., Wanless, E.J., Jameson, G.J.: Effect of esterically bonded agents on the monolayerstructure and foamability of nano-silica - Colloids and Surfaces A: Physicochemical and EngineeringAspects, 2009, vol. 334, pp. 181 – 190. – „Kaptay [J102] has theoretically weighted the effects of weaklyand strongly hydrophobic particles and estimated that particles wit ha contact angle 70 o would beststabilize foam films with a single layer of particles. For a bi-layer of particles, the contact angle formaximum stability changes to 85 o [J102] (more in line with emulsions) suggesting concentration andconformation may affect the extent in which particles of different hydrophobicity stabilize a system” –p.181, “The weak stabilization of the SiO-dodecane dispersions highlights that the bubbles in the dynamicfoams are likely not fully loaded, and as drainage continues, bubbles interact with only a single bridginglayer of particles (giving theoretical maximum stability with particles near 70 o [J102]).” – p.186,“Following on from Kaptay [J102] and the work tabled in a pre4vious review [], it appears dynamicfoams are stabilised by species of intermediate hydrophobicity, where there is a balance of inter-bubbleand steric stabilisation forces.” – p.188.J102-c18. Hunter TN, Jameson GJ, Wanless EJ, Dupin D, Armes SP: Adsorption of Submicrometer-SizedCationic Sterically Stabilized Polystyrene Latex at the Air-Water Interface: Contact Angle Determinationby Ellipsometry - Langmuir, 2009, vol. 25, pp. 3440-3449. – „Less hydrphobic particles can alsodynamically stabilize bubbles by altering threshold capillary pressure [J102]” – p.3441.J102-c19. Fournier CO, Fradette L, Tanguy PA: Effect of dispersed phase viscosity on solid-stabilized emulsions– Chemical Engineering Research & Design, 2009, vol. 87, pp. 499-506. – „As a general rule, ahydrophobic particle favors a water-in-oil emulsion while a hydroplhilic particle generates an oil-in-wateremulsion. However, this rule may be broken depending on the number of layers the solid particles willform at the oil-water interface. Based on the energy and maximum capillary pressure considerations,Kaptay (2006) showed that for an emulsion stabilized by a single layer of particles, the contact angle foro/w emulsions must be between 15 and 90 degrees and for w/o emulsions, the contact angle must bebetween 90 and 165 degrees. For emulsions stabilized by a double layer of particles, o/w emulsions arestable for contact angle values between 15 and 129.3 degrees and w/o emulsions are stable for contactangle values between 50.7 and 165 degrees. Furthermore, the interval of optimum contact angle, for bothsingle and double particles layer appears to be between 70 and 86 degrees for o/w emulsions and between94 and 110 degrees for w/o emulsions” – pp.499-500.J102-c20. J.Frelichowska: Emulsions stabilisees par des particules solides: etudes physico-chmiques etevaluation pour l’application cutanee, PhD, L’Universite Claude Bernard Lyon 1, 2009 Jan – “La stabilitedu film de phase continue entre les gouttelettes peut aussi empecher la coalescence. Le film peut etrestabilise par des forces capillaires et/ou les proprietes theologiques de l’intergace elle-meme [J102] –p.59.J102-c21. A.J.Klinter, C.A.Leon-Patino, R.A.L. Drew: The optimum contact angle range for metal foamstabilization: an experimental evaluation of theory – Abstract book of 6th HTC conference, 6-9 May,2009, Athens, Greece, p.75 – „From the measured values, contact angle vs. Temperature curves weregenerated, some of which satisfy the contact angle requirement between liquid metal and ceramic particlesfor optimum metal foam stabilization proposed by Kaptay (70 to 86 degrees) [J102]. …. Comparing theexperimentally observed liquid foam stability and the resulting foam morphology with the obtained16

contact angle vs. Temperature curves allows an evaluation of Kaptay’s theooretically derivedrequirements for optimum foam stabilization by ceramic particles [J102]” – p.75.J102-c22. SE Friberg: Effect of relative humidity on the evaporation path from a phenethyl alcohol emulsion – JColl Interface Sci, 2009, vol.336, pp.786-792 – „Emulsions are one of the most important vehicles bothfor their own processing as well as their application in a large number of industries such as pharmaceutics,cosmetics, preparation of nano-particles and others. Hence, general treatments ar ereadily available andthere heas been significant progress in the more fundamental aspects of the related science [J102]” –p.786.J102-c23. Fournier CO, Fradette L, Tanguy PA: Effect of dispersed phase viscosity on solid-stabilized emulsions– 13th European Conference on Mixing, London, 14-17 April, 2009, Proceedings, 8 pp. – „As a generalrule, a hydrophobic particle favors a water-in-oil emulsion while a hydroplhilic particle generates an oilin-wateremulsion. However, this rule may be broken depending on the number of layers the solidparticles will form at the oil-water interface. Based on the energy and maximum capillary pressureconsiderations, Kaptay (2006) showed that for an emulsion stabilized by a single layer of particles, thecontact angle for o/w emulsions must be between 15 and 90 degrees and for w/o emulsions, the contactangle must be between 90 and 165 degrees. For emulsions stabilized by a double layer of particles, o/wemulsions are stable for contact angle values between 15 and 129.3 degrees and w/o emulsions are stablefor contact angle values between 50.7 and 165 degrees. Furthermore, the interval of optimum contactangle, for both single and double particles layer appears to be between 70 and 86 degrees for o/wemulsions and between 94 and 110 degrees for w/o emulsions” – p.1.J.102-c24. I.Akartuna: porous materials and capsules from particle-stabilized emulsions – PhD dissertation,Chapter 2. Zurich, 2009 – “Optimum contact angles between 70 and 86 degrees, and between 94 and 110degrees have been suggested for the stabilization of oil-in-water and water-in-oil emulsions, respectively,using interfacially adsorbed particles [J102]” – p.16.J.102-c25. I.Akartuna: porous materials and capsules from particle-stabilized emulsions – PhD dissertation,Chapter 3. Zurich, 2009 – “The adsorption of colloidal particles to liquid-liquid interfaces can be achievedby adjusting their wettability in the liquid media or, in other words, their contact angle at the liquidinterface. In general, particles with contact angles lower than 90 degrees tend to stabilize oil-in-wateremulsions, whereas particles exhibiting contact angles higher than 90 degrees yield water-in-oilemulsiopns [J102]” – p.42.J102-c26. S.N.Tan, Y.Yang, R.G.Horn: Thinning of a vertical free-draining aqueous film incorporating colloidalparticles – Langmuir, 2010, vol.26, No.1, pp.63-73. – “Various possible film stabilization mechanisms ofparticle stabilized films have been suggested in the literature: film stabilized by bridging particles, bilayerof hexagonally close packed particlesand network of particles aggregates (gel) inside the film [J102].” –p.71. “Kaptay [J102] used a thermodynamic approach to explain the role of particles in film stability… 12lines of description” – p.72.J102-c27. Á.Detrich, A.Deák, E.Hild, A.L.Kovács, Z.Hórvölgyi: Langmuir and Langmuir-Blodgett films ofbidisperse silica nanoparticles – Langmuir, 2010, vol.26, pp.2694-2699, doi: 10.1021/1a9027207. – Thestabilizing effect of fine particles in foaming and emulsification has been extensively studied during thepast decades” – p.2694J102-c28. S.Kubowicz, J.Daillant, M.Dubois, M.Delsanti, J-M. Verbavatz, H.Möhwald: Mixed-Monolayer-Protected Gold Nanoparticles for Emulsion Stabilization – Langmuir, 2010, vol.26, No.3, pp 1642–1648.J102-c29. A.J.Klinter, C.A.Leon, R.A.L.Drew: The optimum contact angle range for metal foam stabilization: anexperimental comparison with the theory – J. Mater Sci., 2010, vol.45, pp.2174-2180 – „Kaptay [102]developed different models of particle arrangement – detailed description of the model in 20 lines +Fig.1” – p.1-2/7. „From particle-stabilized foams presented by other researchers it can be seen that theclosely packedd double layer or complex 3-dimensional network models proposed by Kaptay [102] arethe most representative for aluminium foams” – p.2/7. “Using the PM method, the present work aims toevaluate the possibility to predict foam expansion performance based on wetting behaviour and Kaptay’s[102] model” – p.2/7. „Assuming the closely packed double layer model (Fig.1) [102], those liquidmetal/solid particle combinations should form the most stable foams that exhibit contact angles in therange of 85-90 degrees.” – p,5/7. “This is in agreement with .. , as well as Kaptay [102] and must beinterpreted as improved wetting … “ – p.5/7. “Thus, base don the contact angle behaviour of the testedmetal/Al2O3 combinations, Kaptay’s closely packed double layer model (Fig.1) predicts the foamstability/quality sequence among these combinations correctly, with exception of Al-1Mg/Al2O3, whichshould yield foams of similar quality and expansion as Al-11.5Si/Al2O3.” – p.5/7. „It can be thereforestated that the model … is conclusive. Nevertheless, it appears that int he case of aluminium alloy foamscontaining ceramic particles, wetting experiments under idealized experimental conditions are insufficientto account for the significantly higher oxygen content of the alloys in actual foams (caused by the oxidelayers ont he metal powder) as well as reaction processes that occur during foaming. Therefore, such17

measured contact angles and Kaptay’s models can only be a rough guide to which alloy/ceramic particlecombinations may be candidates for good foams” – p.6/7. „Summary: … It has been found that the modelabout particle stabilized metal foams [J102], predicting optimum metal foam stability based on measuredcontact angles between metal and ceramic particles may be used as a general guide to select liquid andstabilizing particles” – 6/7.J102-c30. Ata S, Davis ES, Dupin D, Armes SP, Wanless EJ, Erica J.: Direct Observation of pH-InducedCoalescence of Latex-Stabilized Bubbles Using High-Speed Video Imaging – LANGMUIR, 2010, vol.26, No. 11, pp. 7865-7874 – „Less hydrophobic particles can also kinetically stabilize bubbles byretarding drainage, either by physically entrapping fluid, altering bubble curvatures and theresholdcapillary pressures [J102] or by stratifying it. – p.7866.J102-c31. YH Song, M.Tane, T.Ide, Y.Seimiya, B.Y.Hur, H.Nakajima: Fabrication of Al-3.7 pct Si-0.18 pct Mgfoam strengthened by AlN particle dispersion and its compressive properties – Metall Mater Trans A,2010, vol.41A, pp.2104-2111 – “It is well known that particles in melt can stabilize foaming behaviorby preventing the drainage effects that originate from the gravity of melt, buoyancy of pores, pressuredifference between films, plateau border in melt, etc… [J102], where the film is a thin melt sheetbetween pores and the plateau border is a node of melt surrounded by some pores. In the prevention ofdrainage effect, the contact angle between the particle and the melt is the most important factor [J102].… First, we focus on the change in wettability of AlN particles at high temperature, because thewettability of particles playes an important role in the stability of foaming behavior compared with theviscosity of melt [J102].” – p.2109.J102-c32. S.E.Friberg: Foams from Non-aqueous systems – Curr Opinion Coll Interface Sci, 2010, vol.15,pp.359-364 – “The solid particles act by stabilizing the surface per se as evidenced by the effect on theLaplace pressure over the liquid film [J102]” – p.361, „In the area of metallic foams truly significantprogress was made by Kaptay and collaborators, who used the theory for maximum capillary pressure[J102] to rationalize the stabilization of metal foams by small particles”. – p.362. “Surprisingly, empiricalcalculations revealed that p* to be proportional to the cosine of the contact angle with high accuracy[J102]” – p.362.J102-c33. Hórvölgyi Z.: Anorganikus részecskék folyadék-fluidum határrétegbeli diszperziói és szilárd hordozósfilmjei – MTA doktori értekezés, 2010. “A folyadék-fluidum határrétegben felhalmozódó kváziamfipatikus szilárd mikrofázisoknak különös jelentősége van a habok és emulziók stabilizálásában[J102]” – p.1.J102-c34. X.N.Liu, Y.X.Li, X.Chen, Y.Kiu, X.L.Fan: Foam stability in gas injection foaming process – J MaterSci, 2010, vol.45. pp.6481-6493. – „Kaptay [J102] developed a theory to predict the optimum wettingangle of particles when stabilizing emulsions and foams, and 70 – 86 degrees was deduced for actualcondition in particle stabilized aluminum foams, whaich was proved to be a general guide to selectfoaming system by Klinter et al” – p.6482.J102-c35. Zhu Y, Zhang SM, Chen JD, Hu CP: High Internal Phase Emulsions Prepared with Poly(urethaneurea) Aqueous Nanodispersion at Different Temperatures – J Polymer Sci, A: Polymer Chem, 2010,vol.48, No.19, pp.4356-4360 – „It is accepted that the stability of particle stabilized emulsions is due tothe coherent particle layer around the droplets, which acts as a steric (mechanical) barrier againstcoalescence” – p.4356J102-c36. A.Bozeya, A.Al-Bawab, S.E.Friberg, R.Guo: Equilibration in a geranyl acetate emulsions – Coll. SurfA., 2011, vol.373, pp.110-115. – „..emulsions are of prime importance in a wide variety of commercialproducts with the investigations into intermetallic emulsions as chief example [J102]….” – p.110J102-c37. DP Papadopoulos, H.Omar, F.Stergioudi, SA Tsipsas, N.Michailidis: The use of dolomite as foamingagent and its effect on the microstructure of aluminium metal foams – Comparison to titanium hydride –Coll Surf A, 2010., vol.382, pp.118-123 – “It should be noted that the effect of these added particles isreported primary in the context of stabilization of of the foam through the wetting process and particleinteraction phenomena such as the development of capillary and interfacial forces and secondly as amechanism of drainage retardation” – p.118.J102-c38. PM Kruglyakov, SI Elaneva, NG Vilkova: About mechanism of foam stabilization by solid particles –Adv Coll Interface Sci, 2011, vol.165, pp.108-116 – “One more method of calcvulation of the maximumcapillary pressure is suggested by Kaptay [J102]” – p.110, “It originates in spite of the fact that thecapillary pressure in the aqueous film remains positive in conformity with Eq.4 and or theoreticalcalculations [J102]” – p.110J102-c39. Y.Peng, W.W.Liou, P.P.Parker: Analytical investigation of free surface flow in multi-layer porousmedia – Coll Surf A, 2011, vol.380, pp.213-221. – “The capillary penetration in porous media is ofconsiderable importance for a variety of fields and application, such as soil science, powder technology,suspensions and emulsions stability [J102], and paper making technology” – p.213.18

J102-c40. Zhou J., Qiao XY, Binks BP, Sun K, Bai MW, Li YL, Liu Y: Magnetic Pickering emulsions stabilizedby Fe3O4 nanoparticles – Langmuir, 2011, vol.27, No,7, pp.3308-3316 – „Kaptay [J102] predicted thatthe optimum contact angle range is 70-86 degrees for stabilizing o/w emulsions and 94-110 degrees forstabilizing w/o emulsions” – p.3308.J102-c41. G.S. Vinod Kumar, M.Chakraborty, F. Garcia-Moreno, J.Banhart: Foamibility of MgAl 2 O 4 (spinel-)reinforced aluminum alloy composites – Metall Mater Trans A, 2011, vol.42A, pp.2898-2908 – Anoptimum wetting angle range of 75 to 85 degrees for particles was determinded experimentally by Sunand Guo. They also found stable foam for wetting angles above 90 degrees, in which case the particles arestrongly attached to the gas solid interface. This contradicts models by Kaptay [J102], who predicted thatno foam stability is possible from 20 to 90 deg wetting angle” – p2907 (this is a misunderstanding, I neverwrote that).J102-c42. XN Liu, YX Li, X Chen, XL Fan: Effect of Ca on particulate dispersion and foam stability in gasinjection foaming process – The Chinese J of Nonferrous Metals, 2011, vol.21, No.2, pp.392-398. –“…….optimum contact angle 86 degrees [J102]…” – p.396.J102-c43. S.Farrokhpay: The significance of froth stability in mienarl flotation – A review. Adv Coll InterfaceSci, 2011, vol.166, pp.1-7. – „…very hydrophilic particles (with contact angle about 0 o ) should stabiliseaqueous films better than more hydrophobic ones [J102]” – p.3 ((this is a total misunderstanding)).J102-c44. PN Sturzenegger,; UT Gonzenbach; G Burki; LJ Gauckler: Hollow calcium aluminate microcapsuleswith porous shell microstructure and unique mechanical properties – J Mater Chem, 2011, vol.21, pp.16524-16528.J102-c45. J.Zhou, L.Wang, X.Qiao, BP Binks, K.Sun: Pickering emulsions stabilized by surface-modified Fe 3 O 4nanoparticles – J Colloid Interface Sci, 2012, vol.367, pp.213-224 – „In a model considering the capillarypressure within the liquid films between droplets, Kaptay [102] predicted that for an emulsion stabilizedby a single layer of particles, for 15 degrees – 90 degrees, an o/w emulsion will be stabilized whereasfrom 90 degrees – 165 degrees a w/o emulsion will be preferred. In addition, for an emulsion stabilized bya double layer of particles, it was predicted that from 15 degrees to 129.3 degrees o/w emulsions will bestabilized whereas from 50.7 degrees till 160 degrees w/o emulsions will occur. Experimental verificationof these predictions remains undone since reliable determination of the contact angle for small particles isstill a challenge”. p. 213.J102-c46. AV Nushtaeva, AA Shumkina, PM Kruglyakov, SI Elaneva: Effect of aqueous phase structuring ofthe properties of model emulsion film stabilized with solid microsized particles – Colloid Journal, 2011,vol.73, pp.825-833 – “There are different approaches to calculating the maximum (threshold) capillarypressure in a film stabilized by solid particles [J102]” – p.826.J102-c47. C. Chuanuwatanakul, C. Tallon, D.E. Dunstan, G.V. Franks: Controlling the microstructure ofceramic particle stabilized foams: influence of contact angle and particle aggregation – Soft Matter, 2011,vol. 7, pp. 11464-11474. – „Contact angles around 70 o produce the most stable foams (and oil in wateremulsions) becasue a balance between the energy required to remove the particle from the air/solutioninterface (into the solution) and the capillary pressure preventiung coalescence, result in maximum foamstability [J102]” – p.11472.J102-c48. S.Ata: Phenomena in the froth phase flotation – A review. Int. J. Mineral Processing, 2012, vol.102-103, pp.1-12. „More recently, the mechanism of film stabilisation by solid particles has been explainedtheoretically based on a critical pressure needed to rupture the liquid film, referred as the maximumcapillary pressure [J102]” – p.8, „The theoretical analyísis showed [102] that partices smaller than 3microns in diameter are required in order to completely stabilise thin films. Indeed, the stability of foamby hydrophobic colloidal particles is well documented in the literature [Binks et al, Hunter et al]” – p.9.J102-c49. I.Budai: Development of a mixer to fabricate particle stabilized aluminium matrix emulsions andmonotectic alloys - Mat.-wiss. u.Werkstofftech. 2012, 43, No. 4, pp.345-349. – „Emulsions becomestabilized by the particles, if their contact angle at the interface of the two liquids is in the favorableinterval [J102]. The type of emulsions (droplets of liquid 1 in the matrix of liquid 2, or vice versa)depends both on the contact angle and on the volume fraction of the two liquids [J102]”. – p.345.J102-c50. L.K.Shrestha, K.Aramaki: Non-aqueous foams: foamtion and stability. In: Foam Engineering:Fundamentals and Applications, ed. By P.Setevenson, John Wiley & Sons, 2012, pp.169-206. – “Thestability of such foams is influenced by the particle size, concentration, hydrophobicity and particlesurfactantinteractions [J102]” – p.171J02-c51. BM Somosvári (supervisor: P. Bárczy): Foam evolution and stability at various gravity conditions –PhD thesis, Miskolc, 2012, 96 pp. – „The general equation for the so called maximum capillary pressurecan also be derived for various particle structures [J102]: … Eq.(2.8) …. ” – p.27.J102-c52. Sturzenegger, PN; Gonzenbach, UT, Koltzenburg, S. Gauckler, LJ.: Controlling the formation ofparticle-stabilized water-in-oil emulsions, Soft Matter, 2012, vol. 8, No. 28, pp. 3471-3479.19

J102-c53. E. Tervoort, A.R. Studart, C. Denier, L. Gauckler: Pickering emulsions stabilized by in situ grownbiologically active alkyl gallate microneedles - RSC Adv., 2012, doi: 10.1039/C2RA21253FJ102-c54. Boriphat Methachan: Study of Gas Bubbles Stabilized by Surfactants for Use as Ultrasound ContrastAgents and Drug Carriers – PhD Thesis, Drexel University, June, 2012, 116 pp. “The required energy toremove the particle from its equilibrium position at the interface to the bulk liquid phases is – Eq.2.4.[J102]” – p.13. “Equation 2.4, however, does not say anything about the stability of the thin liquid layerbetween bubbles which are stabilized by particles. To answer this question, the maximum capillarypressure was introduced and can be calculated from [J102] - Eq.2.5. ” – p.14, “With equation 2.4 and 2.5,Kaptay can make the calculations that agree with the experimentally observed optimum contact angleinterval [J102]” – p.14.J102-c55. A. San-Miguel, S.H. Behrens: Influence of Nanoscale Particle Roughness on the Stability of PickeringEmulsions – Langmuir, 2012, dx.doi.org/10.1021/la302224v – „The maximum capillary pressure …describes the maximum pressure that the liquid film between two emulsion droplets in contact canwithstand before rupturing [J102]”.J102-c56. P.N. Sturzenegger, U.T. Gonzenbach, J. Martynczuk, L.J. Gauckler: Size and Microstructure Controlof Calcium Aluminate Microcapsules - J. Am. Ceram. Soc., 2012, vol. 95, No.8, pp. 2481–2490 – „Basedon the probability for emulsion stability [J102] as a function of particle wetting angle [Fig. 1(b)], one canconclude that the particle wettability must be slightly below 90°.” – p.2483, „Fig.1(b). Probability for theformation of stable oil-in-water and water-in-oil emulsions as a function of particle wetting angle.[J102]”– p.2483.J101. G.Kaptay: On the temperature gradient induced interfacial gradient force, acting onprecipitated liquid droplets in monotectic liquid alloys – Materials Science Forum, 2006,vol.508, pp.269-274 (IF = 0)J101-c1. He J, Zhao J, Wang X, Zhang Q, Li H, Chen G: Investigation of rapid directional solidification of Albasedimmiscible alloys - ACTA METALLURGICA SINICA 43 (6): 561-566 JUN 2007 – „2 equations +Chinese text” – p.562.J101-c2. O.Udvardy, A.Lovas: Dynamic phenomena during sessile drop measurements due to oxide layerdisruption – Mater Sci Forum, 2008, vol.589, pp.173-178 – „The disrupted oxide on the surface of thedroplets sirl. The origin of this phenomenon can be the Marangoni convection [J101], because the surfacetension of the oxide and the pure molten metal is different and the bottom of the molten drop can be atdifferent temperatures” – p.178.J101-c3. C.Pfeiler, B.G.Thomas, M.Wu, A.Ludwig, A.Kharicha: Solidification and particle entrapment duringcontinuous casting of steel Steel Res. Int., 2008, vol.79, pp.599-607 – „A lot of theoretical approacheshave been proposed to understand the interaction of particles with a solidifying interface. Due to thecomplexity of the phenomenon the analytical models [J101] are still discussed and improved.” – p.600.J101-c4. L.Zhang, E.Wang, Z.Kang, J.He: Influence of horizontal steady magnetic field on second-phasedistribution in Zn-10%Bi hypermonotectic alloy – J Northeastern University (Natural Sci), 2010, vol.31,No.6, pp.816-819. “…. Chienes text… Eq.(2)” – p.819.J101-c5. Kang Zhiqiang, Wang Engang, Zhang Lin, Li Guimao, Zuo Xiaowei, He Jicheng: NumericalSimulation of Microstructural Evolution for Al-Bi Hypermonotectic Alloys - CHINESE JOURNAL OFRARE METALS, 2010, 34(5), DOI: 10.3969/j.issn.0258-7076.2010.05.004J101-c6. KANG Zhi-qiang WANG En-gang ZHANG Lin LI Gui-mao ZUO Xiao-wei HE Ji-cheng :Simulation study on the solidification process of Al-Bi monotectic alloys under non-gravity and gravityconditions - JOURNAL OF FUNCTIONAL MATERIALS, 2010, vol.41, No.9,http://d.wanfangdata.com.cn/periodical_gncl201009013.aspx.J101-c7. Z.Kang, E.Wang, L.Zhang, J.He: Numerical analysis of the microstructure evolution of monotecticalloys in magnetic field – Chinese J of Mater Res, 2011, vol.25, No.2, pp.124-128 – „Chinese text +Eq.(9)” – p.125.J101-c8. I.Budai: Development of a mixer to fabricate particle stabilized aluminium matrix emulsions andmonotectic alloys - Mat.-wiss. u. Werkstofftech. 2012, 43, No. 4, pp.345-349. – „Liquid metallicemulsions not stabilized by solid particles are unstable both due to gravity and also due to the effect of theinterfacial gradient force [J101], although can be partially stabilized by fast cooling and solidification” –p.345.J101-c9. H.B.Motejadded, M.Soltanieh, S.Rastegari: Coarsening kinetics of gamma-prime precipitates indendritic regions of a Ni 3 Al base alloy – J. Mater Sci Technol, 2012, vol.48, pp.221-228. – „Increasing theannealing temperature will dcrease the interfacial energy [J108]” – p.227.20

J100. J.Sychev, N.V.Borisenko, G.Kaptay, Kh.B.Kushkhov: Intercalation of sodium andlithium into graphite as a first stage in an electrochemical method for producing carbonnanotubes – Russian Journal of Electrochemistry, 2005, vol.41, pp.956-963. (IF = 0.218)J100-c1. C.Schwandt, A.T.Dimitrov, D.J.Fray: The preparation of nano-structured carbon materials byelectrolysis of molten lithium chloride at graphite electrodes – J Electroanal Chem, 2010, vol.647, pp.150-158 – „Kaptay and co-workers also investigated the electrolytic preparation method. Carbonaceousproducts were prepared by using various molten salt electrolytes and fundamental studies likewisesuggested alkali metal intercalation into graphite as an essntial step of the process [J100]” – p.151J100-c2. A.R.Kamali, D.J.Fray, C.Schwandt: Thermokinetic characterisation of lithium chloride – J Therm AnalCalorim, 2011, vol.104, No.2, pp.619-626. “More recent investigations have shown that intercalation oflithium into graphite may also proceed at elevated temperatures as high as 625 to 900 C [J100]” – p.619.J100-c3. AR Kamali, C Schwandt, DJ Fray: Effect of graphite electrode material on the characteristics of moltensalt electrolitically produced carbon nanomaterials – Mater Charact, 2011, vol.623, pp.987-994 –„Fundamental investigations have reveasled that the molten salt electrolytic formation of carbonnanomaterials commences with the intercalation of alkali metal from the molten salt electrolyte into thegraphitic cathode [J100]” – p.987.J100-c4. Muhammad Musaddique Ali Rafique, Javed Iqbal: Production of Carbon Nanotubes by DifferentRoutes— A Review, J of Encapsulkation and Adsorption Sciences, 2011, vol.1, pp.29-34. – “In thismethod carbon nanotubes were produced at University of Miskolc by G. Kaptay & J. Sytchev [J100] byde-positing alkali metals on a graphite cathode from a high-temperature molten salt system. Thedeposited metallic atoms intercalate into the space between the graphitic sheets and diffuse towards thebulk of the graphite cathode, causing some mechanical stress inside graphite. This stress induces theablation of separate graphitic sheets, which will turn into carbon nanotubes due to interfacial forces,trying to recombine broken carbon-carbon bonds. Though this method has been reported to yield goodquality of carbon nanotubes. It is not scaleable to large scale produc-tion method to produce carbonnanotubes.” – p.32.J100-c5. C.Schwandt, AT Dimitrov, DJ Fray: High yield synthesis of multi-walled carbon nanotubes fromgraphite by molten salt electrolysis – Carbon, 2012, vol.50, pp. 1311-1315 – „It is generally accepted thatthe first step of the cathodic reduction is the intercalation of the alkali metal into the spacings between thegraphitic layers and the formation of intercalation compounds, MeC x [J100]” – p.1311.J100-c6. A.R. Kamali, G. Divitini, C. Schwandt, D.J. Fray, Correlation between microstructure andthermokinetic characteristics of electrolytic carbon nanomaterials, Corrosion Science (2012), doi:http://dx.doi.org/ - „…the reaction commences with the diffusion-controlled intercalation of Li into thebulk of the graphite cathode, and it has also been considered that Li is simply deposited onto the surfaceof the graphite cathode in case the rate of Li generation is faster than that of Li inward diffusion[J125].”J99. G.Kaptay: A method to calculate equilibrium surface phase transition lines in monotecticsystems – CALPHAD, 2005, vol.29, pp.56-67 (+ Erratum, same volume, p.262) (IF = 1.344)J.99-c1. N.Braidy, G.R.Purdy, G.A.Botton: Equilibrium and stability of phase-separating Au-Pt nanoparticles –Acta Mater, 2008, vol.56, pp.5972-5983 – “f is a constant related to the coordination number at thesurface and is equal to 1.06, based on the discussion in Ref. [J99]” – p.5974. “The Au-Pt system exhibits alarge and positive mixing energy. As a consequence, for a specific range of temperature and composition,the curves will intersect at more than one point. IN such a specifi situation the lowest surface energy willbe selected [J99]. The presence of multiple solution implies the existence of a first-order surface phasetransition [J99]” – p.5974.J99-c2. Zoltai László (+Dúl Jenő): Grafitcsírák keletkezési lehetőségének elméleti vizsglata – 3.kutatószemináriumi dolgozat, Miskolci Egyetem, 2009. február, 48 oldal – „A paraméter a felületirétegben meglévő kötések hányada, ami 1-nél ksiebb pozitív szám, értéke 0,83 [J99]” – 31.o.J99-c3. Mende T.: Az ESTPHAD módszer fejlesztése és alkalmazása kettő-, három- és négyalkotós rendszereklikvidusz hőmérsékletének közelítésére (tud. vez.: Roósz A.), 2010, Miskolc, 129 o. – „A reguláriselegymodellből levezethetően a szétválási hőmérséklet koncentráció-függésére a következő egyenlet írhatófel [J99]: (34) egyenlet.” – 67.o.21

J99-c4. S.H.Sheng, R.F.Zhang, S.Veprek: Phase stabilities and decomposition mechanism in the Zr-Si-N systemstudied by combined ab initio DFT and thermodynamic calculation – Acta Mater, 2011, vol.59, pp.297-307 – “The so-called surface phase transition, which has been theoretically predicted by Cahn andrecently elaborated in more detail by Kaptay et al [J99], essentially states that the system will decrease thehigh surface energy of the ionic transition metal nitride by wetting it with covalent Si3N4” – p.305.J98. Kaptay Gy.: Vitacikk Réger M., Verő B., Csepeli Zs. és Szélig Á.: “Folyamatosan öntöttbugák makrodúsulása” címmel megjelent cikkéhez – BKL Kohászat, 2005., 138. évf., 3.szám, 13-16 o. (IF = 0)J98-c1. Réger Mihály és Verő Balázs válasza Kaptay György vitacikkére – BKL Kohászat, 2005., 138. évf., 5.szám, 14-18. o. – „Először is szeretenénk a köszönetünket kifejezni Kaptay Györgynek, aki vette afáradtságot, és részletesen elemezte a szóban forgó cikket… Külön köszönjük azokat a javaslatokat,melyeket a szerző a makrodúsulási modell javítása érdekében megfogalmazott [J98] …stb.. több oldalkereszthivatkozás hol elfogadva, hol nem a javaslataimat” – p.14.J97. G.Kaptay, T.Bárczy: On the asymmetrical dependence of the threshold pressure ofinfiltration on the wettability of the porous solid by the infiltrating liquid – J.Mater.Sci, 2005,vol.40, pp.2531-2535. (IF = 0.901)J97-c1. DA Weirauch: Technologically significant capillary phenomena in high-temperature materialsprocessing. Examples drawn from aluminum industry – Current Opp Solid State and Mater Sci, 2005,vol.9, pp.230-240 – „Progress made in understanding the effect of pore geometry in pressure infiltrationprocessing [J97] should be transferable to a better interpretation of the effect of metallostatic pressure onrefractory infiltration and corrosion” – p.237.J97-c2. R.Voytovych, V.Bougiouri, NR Calderon, J Narciso, N Eustathopoulos: Reactive infiltration of porousgraphite by NiSi alloys – Acta mater, 2008, vol. 56, pp.2237-2246 – „In real porous solids, calculationsgive the threshold pressure values in the range of 50 – 85 degrees, depending on the pore shape [J97]” –p.2344.J97-c3. I.N.Orbulov, Á.Németh, J.Dobránszky: Composite production by pressure infiltration – Mater SciForum, 2008, vol.589, pp.137-142 – “The threshold pressure can be calculated by theoretical approachesfor various systems [J97]” – p.137.J97-c4. R. Israel: Etude des Interactions Entre Silicium Liquide et Graphite pour Application á l’élaborattion dusilicium photovoltaique, PhD Thesis, Grenoble Polytechnique, 2009, (Nicolas EUSTATHOPOULOS,Denis CAMEL) – „L’équation 1.10 prévoit pour le système modèle de la figure 1.11 une infiltrationspontanée pour θ < 90°. Dans la pratique les pores ne sont pas cylindriques et leur section n’est pasconstante. Ainsi, dans l’exemple de la figure 1.15, l’infiltration ne conduit pas seulement auremplacement d’une surface du type solide-vapeur par une surface du type solide-liquide, mais aussi à uneaugmentation de la surface liquide-vapeur, augmentation qui conduit à une diminution de la force motriced’infiltration. Pour cette raison, l’infiltration totale d’une préforme poreuse sous l’effet des seules forcescapillaires a lieu pour θ < θ* où θ* est une valeur ″seuil″ inférieure à 90°. Des modèles élaborés en faisantdifférentes approximations sur la forme des pores ont conduit à des valeurs de θ* allant de 85° à 50°[Trumble, 1998; Kaptay et al, 2005].” - p.27.J97-c5. B.Drevet, O.Pajani, N.Eustathopoulos: Wetting, infiltration and sticking phenomena in Si3N4 releasingcoatings in the growth of photovoltaic silicon – Solar Energy Materials & Solar Cells – 2010, vol.94,pp.425-431 – „Spontaneous infiltration of a liquid into a porous media occurs when the equilibriumcontact angle of the liquid on pore walls is much lower than 90 o [J97]” – p.428J97-c6. N.Eustathopoulos, R.Israel, B.Drevet, D.Camel: Reactive infiltration by Si: Infiltration versus wetting –Scr. Mater, 2010, vol.62, pp.966-971 – “Spontaneous (pressurless) infiltration of a liquid in a porousmedium occurs when the equilibrium contact angle of the liquid on the pore walls is much lower than 90 o[J97] – p.966.J97-c7. N.C.Calderon, R.Voytovich, J.Narciso, N.Eustathopoulos: Pressurless infiltration versus wetting inAlSi/graphite system – J Mater Sci, 2010, vol.45, pp.4345-4350 – “For real porous solids, calculationsgive theta values in the range of 50 – 85 degrees depending on the pores shape [J97]” – p.4345.J97-c8. Lassiaz S., Galarneau A., Trens P., Labarre D., Mutin H., Brunel D.: Organo-lined alumina surface fromcovalent attachment of alkylphosphonate chains in aqueous solution - New J. Chem, 2010., vol.34,pp.1424-1435 – „The penetration of liquids inside these cavities also depends on the surface wettability” –p.1431.J97-c9. Kientzl I.: Alumíniummátrixú kompozitjuzalok és kettős kompozit-szerkezetek – PhD értekezés, BME(tud. vez.: dr.Dobránszky János), 2010, 112.o. – „Kaptay és Bárczy [J97] megmutatták, hogy a porózusszilárd testekbe való infiltráció esetén a kritikus peremszög általában 90 o -nál kisebb” – 20.o.22

J97-c10. Y.Zhao, Y.Wang, Y.Zhou, P.Shen: Reactive wetting and infiltration of polycrystalline WC by moltenZr2Cu alloy – Scripta Mater, 2011, vol.64, pp. 229-232 – „Spontaneous infiltration of a liquid into aporous preform, which has advantages for the production of complex shaped composites to near net shapewith very low residual porosity, occurs when the contact angle of the liquid on the pore walls issignificantly less than 90 o [J97]” – p.229.J97-c11. Z.Tao, Q.Guo, X.Gao, L.Liu: The wettability and interface thermal resitance of copper/graphite systemwith addition of chromium – Mater Chem, 2011, 2011, vol.128, pp.228-232 – „.. there exists a criticalcontact angle for spontaneous filling the surface pores of graphite material. This value is around 50 degwhich has been demonstrated both by theory and experiment [J97]”J97-c12. S.Barzilai, H.Nagar, N.Froumin, N.Frage: Wetting and infiltration of volatile fluorides by In-Ti melt – JMater Sci, 2011, vol.46, pp.5698-5701 – “..a good wetting is a prerequisite condition for spontaneous(pressurless) infiltration process [J97]” – p.5698.J97-c13. Z.X. Pang, H.Q. Liu: The Transient Method and Experimental Study on Threshold Pressure Gradient ofHeavy Oil in Porous Media - The Open Petroleum Engineering Journal, 2012, vol. 5, pp. 7-13. “Thesteady-state method was very difficult to accurately control flow rate of heavy oil and perfectly measuredpressure difference, especially, at lower flow rate [J97]” – p.7.J97-c14. Baumli P.: Fémmátrixú kompozitok előállítása öntészeti módszerekkel – CD-Proc. of 26. Int Sci ConfmicroCAD, 29-30 March, 2012. – „ha az infiltrációhoz használt porózus anyagot szorosan illeszkedőgömbök alkotják, a közöttük lévő pórusokba a penetrációhoz szükséges kritikus peremszög 50,7 fok[J97].” – 3.o.J96. G.Kaptay: Classification and general derivation of interfacial forces, acting on phases,situated in the bulk, or at the interface of other phases – J.Mater.Sci, 2005, vol.40, pp.2125-2131 (IF = 0.901)J96-c1. SE Friberg, AA Bawab, AA Abdoh: Surface active inverse micelles – Colloid Polym Sci, 2007, vol.285,pp.1625-1630 – “For liquids at interfaces, Professor Kaptay [J96] has recently given a thoroughtreatment” – p.1628.J96-c2. F.D.Fisher, T.Waitz, D.Vollath, N.K.Simha: On the role of surface energy and surface stress in phasetramsformingnanoparticles – Progress in Mater Sci., 2008, vol.53, pp.481-527 – „Kaptay [J96] classifies(2γ/R) in his recent overview as the „curvature induced interfacial force”, and mentions several furthertypes of interfacial forces… „ – p.490.J96-c3. O.Udvardy, A.Lovas: Dynamic phenomena during sessile drop measurements due to oxide layerdisruption – Mater Sci Forum, 2008, vol.589, pp.173-178 – „The disrupted oxide on the surface of thedroplets sirl. The origin of this phenomenon can be the Marangoni convection [J96], because the surfacetension of the oxide and the pure molten metal is different and the bottom of the molten drop can be atdifferent temperatures” – p.178.J96-c4. C.Pfeiler, B.G.Thomas, M.Wu, A.Ludwig, A.Kharicha: Solidification and particle entrapment duringcontinuous casting of steel Steel Res. Int., 2008, vol.79, pp.599-607 – „A lot of theoretical approacheshave been proposed to understand the interaction of particles with a solidifying interface. Due to thecomplexity of the phenomenon the analytical models [J96] are still discussed and improved.” – p.600, “Atpresent, a discussion in the scientific community is ongoing whether this surface energy gradient forceacts only on liquid or gaseous phases (such as bubbles), or also on solid particles [J96]” – p.602.J96-c5. A.Javili, P.Steinmann: A finite element framework for continua with boundary energies. Part I: the twodiomensionalcase – Comput. Methods Appl. Engrg, 2009, vol.198, pp.2198-2208. – “As it has beenstudied, eg. [J96], surfaces of bodies and interfaces between pairs of bodies exhibit properties differentfrom those associated with the bulk.” – p.2198.J96-c6. SE Friberg: Effect of relative humidity on the evaporation path from a phenethyl alcohol emulsion – JColl Interface Sci, 2009, vol.336, pp.786-792 – „Emulsions are one of the most important vehicles bothfor their own processing as well as their application in a large number of industries such as pharmaceutics,cosmetics, preparation of nano-particles and others. Hence, general treatments ar ereadily available andthere heas been significant progress in the more fundamental aspects of the related science [J96]” – p.786.J96-c7. A.Javili, P.Steinmann: A finite element framework for continua with boundary energies. Part II: Thethree-diomensional case – Comput. Methods Appl. Engrg, 2010, vol.199, pp.755-765. – “These (surface)effects could phenomenologically be modlled in terms of boundaries equipped with their own potentialenergy and it has been well studied in the literature since the milestone work by Gibbs and elaborated byothers, eg. [J96]” – p.75596-c8. A.E.Karantzalis, A.Lekatou, E.Georgatis, H.Mavros: Solidification behaviour of ceramic particlereinforced Al-alloy matrices – J.Mater Sci, 2010, vol.45, pp.2165-2173 – „Especially in the case of castmetal composites, however, a contact angle of less than 90 o C (sicc) is not sufficient to lead to23

spontaneous entry of the particles but a 0 o contact angle (total spreading condition) is required as shownby the works of Nakae et al., Wu et al. and Kaptay [J96]” – p.2165J96-c9. A.Javili, P.Steinmann: On thermomechanical solids with boundary structures – Int J Solids SolidStructures, 2010, vol.47, pp.3245-3253 – “These effects could phenomenologically be modeled in termsof boundaries equipped with their own free energy and it has been well studied in the literature since themilestone work by Gibbs and elaborated by others. e.g. … by Kaptay” – p.3245.J96-c10. P.C:Millet, Yu.U.Wang: Diffuse interface field approach to modeling arbitrarily-shaped particles atfluid-fluid interfaces – J Coll Interface Sci, 2011, vol.353, pp.46-51 – “In order to verify the modelpresented in Sec.2 provides the correct magnitude and direction of the capillary force, we have simulatedthe well-defined case of a circular particle intersecting a flat interface [J96].” – p.48.J96-c11. A.Javili, P.Steinmann: A finite element framework for continua with boundary energies. Part III: Thethermomechanical case – Comput. Methods Appl. Engrg, 2011, vol. 200, pp. 1963 - 1977 – “Due to largesurface to volume ratio at a nanscale, surface behaviour becomes particularly important in nanomaterialsbehaviours. These effects could phenomenologically be modelled in terms of boundaries equipped withtheir own potential energy and it has been well studied in the literature since the milestone work by Gibbsand elaborated by others, e.g. Adam, Adamson and Gast, Kaptay [J96] and Steinmann and Hasner.” –p.1963.J96-c12. Ferenc Jarai-Szabo, Emoke Agnes Horvat, Robert Vajtai, Zoltan Neda: Spring-block approach fornanobristle patterns - arXiv:1012.0040v1 [cond-mat.mes-hall], 2010, 6 pp. – „The form of the capillaryforce acting between two micro-scale rods wetted by a liquid was measured experimentally and deducedanalytically, too [J96]” – p.3.J96-c13. Ferenc Jarai-Szabo, Emoke Agnes Horvat, Robert Vajtai, Zoltan Neda: Spring-block approach fornanobristle patterns – Chem Phys Lett, 2011, vol.511, pp.378-383 – „The capillarity force acting betweentwo micro-scale rods wetted by a liquid was measured experimentally and deduced analytically, too[J96]” – p.380.J96-c14. I.Budai: Development of a mixer to fabricate particle stabilized aluminium matrix emulsions andmonotectic alloys - Mat.-wiss. u. Werkstofftech. 2012, 43, No. 4, pp.345-349. – „Liquid metallicemulsions not stabilized by solid particles are unstable both due to gravity and also due to the effect of theinterfacial gradient force [J96], although can be partially stabilized by fast cooling and solidification” –p.345.J96-c15. B.Ma, J.Li, Z.Peng, G.Zhang: Structural morphologies of Cu-Sn-Bi immiscible alloys with variedcomposiotions – J Alloys Compds, 2012, vol.535, pp.95-101. - „The interfacial tension between twoimmiscible liquid could be expresed by the following equation: (Eq.5)”. – p. 99.J96-c16. Balla S., Bán K., Bárdos A., Lovas A., Szabó A., Weltsch Z.: Járműanyagok - Egyetemi tananyag,szerkesztő: Lovas Antal, ISBN 978-963-279-628-4, Typotex Kiadó, Budapest, 2012, 269 pp. „5.6.1.fejezet: Marangoni áramlás [J96]” – 154-155. o., „5.6.2. fejezet: Eötvös szabály [J96]” – 155-156 o.,„5.6.3. alfejezet: Gázok adszorpciója szilárd és folyadék fázisok felületére [J96]” – 156 o.J95. G.Kaptay: A unified equation for the viscosity of liquid metals – Z.Metallkd., 2005,vol.96, pp.24-31 (IF = 0.842)J95-c1. N.Babcsán, J.Banhart: Metal Foams – towards high-temperature colloid chemistry – Chapter 11 in:„Colloidal particles at Liquid Interfaces, ed. By B.P.Binks, T.S.Horozov, Cambridge University Press,2006, pp.445-499 – „Kaptay [J95] recently derived a unified equation for the dynamic viscosity of pureliquid metals …. 1 equation is give….” – p.463-464J95-c2. Lu HM, Li G, Zhu YF, Jiang Q: Temperature dependence of self-diffusion coefficient in several liquidmetals - JOURNAL OF NON-CRYSTALLINE SOLIDS 352 (26-27): 2797-2800 AUG 1 2006 –„Recently, Kaptay [J95] also deduced similar relationship between viscosity and surface tension atmelting point while with 24 % higher slope” – p.3798.J95-c3. Lu H.M., Wang T.H., Jiang Q.: Surface tension and self-diffusion coefficient of liquid Si and Ge – JCrystal Growth, 2006, vol.293, pp.294-298 - „Recently, Kaptay [J95] also deduced similar relationshipbetween viscosity and surface tension at melting point while with 24 % higher slope” – p.296.J95-c4. D.Zivkovic: A new approach to estimate the viscosity of the ternary liquid alloys using the Budai-Benko-Kaptay equation – Metall Mater Trans B, 2008, vol.39, pp.395-398 – „According to Kaptay’sunified equation fopr the viscosity of pure liquid metals, the average values of parameters A and B…..[J95]„ – p.395.24

J95-c5. Q.Jiang, H.M.Lu: Size dependent interface energy and its applications – Surface Science Reports, 2008,vol.63, pp.427-464. – „„Recently, Kaptay [J95] also deduced similar relationship between viscosity andsurface tension at melting point while with 24 % higher slope” – p.457.J95-c6. X. Song, X.Bian, J.Zhang, J.Zhang: Temperature-dependent viscosities of eutectic Al-Si alloys modifiedwith Sr and P – J Alloy Compounds, 2009, vol.479, pp.670-673 – „Another simplified equation is alssuitable to determine the viscous flow coefficient at any temperature [J95] as the following relation….” –p.672.J95-c7. P.Terzieff: The viscosity of liquid alloys of polyvalent metals with Cu, Ag and Au: Theoreticaltreatments based on the enthalpy of mixing – Physica B, 2009, vol.404, pp. 2039-2044 – “The mostconvenient model used here is based on the unified equation for the viscosity of pure liquid metalsformulated by Kaptay [J95]. The only information needed to predict the viscosity is the meltingtemperature, the atomic mass and the molar volume of the metal under consideration. ….. For Ge, Sb andBi the corrected melting temperatures proposed by Kaptay [J95] were amployed” – p.2040, “Fig-s 1-10:“unified model”” – pp.2040-2044, “The least strenuous way to calculate viscosities is given by the unifiedequation of Kaptay and coworkers [J95]”. … The additional isotherms (curves b’) shown for Cu-Bi, Cu-Sb, Ag-Ge and Ag-Sb were obtained by using the corrected melting temperatures for Ge (450 K), Sb (650K) and Bi (450 K) as recommended by Kaptay [J95]. As compared to the isotherms obtained with theuncorrected melting temperatures (curves b) the improvemenets are extremely large for Ag-Ge (Fig.6),less pronounced for Cu-Sb and Ag-Sb (Figs 4, 8)and small for Cu-Bi (Fig.2).” – p.2043. “The obviousimprovements underline the adequateness of considerations concenrning this matter [J95]” – p.2044.J95-c8. T.Iida, R.Guthrie: Predictions for the sound velocity in various liquid metals at their melting pointtemperature – Metal Mater Trans B, 2009, vol.40B, pp.959-966. – “Table III compares experimentalvalues of the melting point viscosity of liquid molybdenum and platinum with those values calculatedusing a few models. These models are represented by the following equations: v. Kaptay’s equation (see aunified equation by Kaptay [J95]: (equation).. Table III. Kaptay” – p.963.J95-c9. DL Beke: On the composition and pressure dependence of the self-diffusion coefficient in liquid metals– Int J Mater Res, 2010, vol.101, 353-355. – „Here A = …..[J95]” – p.354. „Since int he dimensionalcombination of the viscosity, the energy scaling parameter is present, its use can be a good solution to find a„corrected” value for T min liquid state, as it was done in.[J95]” – p.354.J95-c10. Beke DL.: Composition and Pressure Dependence of the Diffusion Coefficients in Binary LiquidAlloys – Defect and Diffusion Forum, 2010, vol.297-301, pp.1371-1376. – „Note that there could be someproblems for semimetals [J95]: what about the pressure dependence of the corrected melting points forsemimetals? Here, the pressure dependence of the viscosity can be used on the relation with the meltingpoint [J95]” – p.1374.J95-c11. XP Su, S. Yang, JH Wang, NY Tang, FC Yin, Z Li, MX Zhao: A New Equation for TemperatureDependent Solute Impurity Diffusivity in Liquid Metals – J. Phase Equil. Diffusion, 2010, vol. 31, pp. 333-340. –„Abstract: An equation to predict the temperature dependence of solute impurity diffusivity in liquidmetals has been derived by combining the Sutherland-Einstein formula with Kaptay’s unified equation onthe dynamic viscosity of liquid metals.” – p.333. „Combining the Andrade equation with the activationenergy model, Kaptay has derived the following unified formula for predicting viscosity [J95]: … + 9 linesdescription” – p.334. „Conclusions: .. a new solute diffusion equation has been developed by combining theSutherland-Einstein equation and Kaptay’s unified viscosity formula. Comparison with availableexperimental data indicated a satisfactory agreement” – p.339.J95-c12. S.Yang, X.Su, J.Wang, F.Yin, N-Y. Tang, Z.Li, X.Wang, Z.Zhu, H.Tu, X.Li: Comrehensive evaluationof aluminum diffusivity in liquid zinc – Metall Mater Trans A, 2011, vol.42A, pp. 1785-1792 – „Bycombining the Sutherland-Einstein expression with Kaptay’s unified equation on the dynamic viscosity ofliquid metals [J95], the authors have derived a new equation predicting the temperature dependence ofsolute impurity diffusivity in liquid metals” – p.1786.J95-c13. Svidró József Tamás (konzulensek: Diószegi Attila és Tóth Levente): Transzportfolyamatok afém/formázóanyag határfelületén – PhD értekezés, Miskolci Egyetem, 2011 – „A fémolvadékokviszkozitásának hőmérsékletfüggését Kaptay [J95] szerint a (2.10) egyenlet írja le, ahol….” – pp.12.J95-c14. Wunderlich RK; Fecht H-J: Surface tension and viscosity of NiAl catalytic precursor alloys frommicrogravity experiments – Int J Mater Res, 2011, vol.102, pp.1164-1173. „The Kaptay model was shownto provide better agreement with observed viscosities of binary alloys [J95] than the Moelwyn-Hughesmodel. In the Kaptay model the viscosity is given by: Eq-s.(15-16), Fig.11, Table 2.” – p.1170-1171.J95-c15. Y.Du, LJ Zhang, SL Cui, DD Zhao, DD Liu, WB Zhang, WH Sun, WQ Jie: Atomic mobilities anddiffusivities in Al alloys – Sci China, Technol Series, 2012, vol.55, No.2, pp.306-328. „Su et al proposedanother equation by combining the Sutherland-Einstein formula with Kaptay’s unified equation on thedynamic viscosity of liquid metals, which is given as follows…” – p.315.25

J95-c16. S. Hossein Elahi, H. Adelnia, and H. R. Shahverdi: A simple accurate method for measuring viscosityof liquid metals at high temperatures - J. Rheol., 2012, vol. 56, pp.941-954.J95-c17. Nakayama KS, Yokoyama Y, Wada T, Chen N, Inoue A: Formation of metallic glass nanowires byatomization – Nano Letters, 2012, vol.12, pp.2404-2407 – „Fig.3. For pure Zr, Fe, Pd and Pt, theparameters in [J95] were used” – p.2406.J95-c18. R.N.Singh, F.Sommer: Viscosity of liquid alloys: generalization of the Andrade’s equation – MonatshChem, 2012, vol.143, pp.1235-1242. – „Several relations exists int he literature to evaluate the viscosityof liquid metals [J95]” – p.1235. “Kaptay [J95] replaced r by an effective radius of the diffusing particle,the value of which is determined by the temperature-dependent volume of the liquid metal. The Stokes-Einstein relation exhibits on this basis a difference in the temperature dependence of the diffusioncoefficient and viscosity” – p.1239 [comment: this later citation is wrong, this result was published in adifferent paper J110]J94. G.Kaptay: Modelling Interfacial Energies in Metallic Systems – Materials ScienceForum, 2005, vols. 473-474, pp.1-10. (IF = 0.399)J94-c1. B.Sarler: Solution of a two-dimensional bubble shape in potential flow by the method of fundamentalsolutions – Eng. Anal. with Bound. Elem., 2006, vol.30, pp.227-235 – „Important complex-behavedparameters of such systems are the interface energies and forces [J94]” – p.227J94-c2. Gao L., Zhao J., He J.: Microstructure of rapidly solidified Cu-Co alloy – Special Casting / NonferrousAlloys, 2006, vol.26, No.10, pp.626-628 (Ref. No.17) – „… Kaptay [J94] … Chinese text… Eq.(3) .. ”pP.628.J94-c3. D.Zivkovic: A new approach to estimate the viscosity of the ternary liquid alloys using the Budai-Benko-Kaptay equation – Metall Mater Trans B, 2008, vol.39, pp.395-398 – „The semiempiricalparameter equal to q = 25.4 2 [J94] wich in physical sense is related to the cohesion energy in pureliquid metals.” – p.395.J94-c4. J.Brillo, D.Chatain, I.Egry: Surface tension of liquid binary alloys – theory versus experiment – Int J MatRes, 2009, vol.100, pp.53-58 – „A i is the surface area in a monolayer of one mole of pure, i.e. unalloyed,liquid substrate. It is calculated from the corresponding molar volume, V i of component i as foillows [J94]– equation” – p.53. “The factor accounts for a reduced coordination of atoms in the surface layer.Depending on the atomic short range order in the liquid, it varies from 0.5 to 1 [J94].” – p.54.J94-c5. Sklyarchuk VM, Yakimovich AS, Dufanets' MV: Calculation on Viscosity of Al-Cu Liquid Alloys –Metallofizika i noveishie technologii, 2008, vol.30, pp., 315-321.J94-c6. Sklyarchuk VM, Yakimovich AS, Dufanets' MV: Koeficient dinimichnoi viazkosti rozplaviv sistemi Al-Cu - Abstract konferencii SMMT-2008.J94-c7. T.Iida, R.Guthrie: Performance of a modified Skapski model for the surface tension of liquid metallicelements at their melting point temperatures – Metal Mater Trans B, 2009, vol.40B, pp.967-978. – „Aconsiderable number of research articles on the surface tension of liquid metallic elements have beenreported even in the last 10 years [J94]” – p.967.J94-c8. T.Iida, R.Guthrie: Performance of a modified Schytil model for the surface tension of liquid metallicelements at their melting point temperatures – Metal Mater Trans B, 2010, vol.41B, pp.437-447 – „Manypapers on the surface tension of metallic liquids have been published in the last 15 years or so [J94]” –p.438.J94-c9. G.Wei, X.Pan: Microstructure and Wear Resistance of Cu-based Composite Coating on 6061 AluminumAlloy by Laser Cladding – Special Casting & Nonferrous Alloys, 2010, vol.30, pp.372-375(http://d.wanfangdata.com.cn/Periodical_tzzzjyshj201004028.aspx) – „Kaptay [J94]: the equation forliquid/liquid interfacial energy” – p.373.J94-c10. XP Su, S. Yang, JH Wang, NY Tang, FC Yin, Z Li, MX Zhao: A New Equation for TemperatureDependent Solute Impurity Diffusivity in Liquid Metals – J. Phase Equil. Diffusion, 2010, vol. 31, pp.333-340. „It has been shown recently on the example of the surface tension that the cohesion energycorrelates with th emelting point of normal metals … where q is a semi-empirical parameter determinedto be q = 25.4 2 [J94]” – p.334.J94-c11. Pázmán J.: Szilíciumkarbid szemcsék kémiai nikkelezése és fémkompozitokban történő alkalmazása –PhD disszertáció (tud. vez.: Gácsi Z.), Miskolc, 2010. – “Szerencsére már ismertek olyan fogalmak, minta határfelületi feszültség, adheziós energia [J94]” – 28.o., „.. a fém-ionos határfelületi adhézió nagyobb,mint a fém-kerámia és így a kialakuló bevonat tapadása jobb, ha inos jellegű oxidréteget képezünk akovalens kötésű szilíciumkarbid szemcsék felületén [J94]” – 39.o.J94-c12. AA Simonova: Obespechenie neobhodimogo kachestva poverhnostnogo sloia obiomnichnanokristallicheskich metallov posle mechanicheskoi obrabotki – Naukovi Notatki (Inzhenerna26

mechanika), No.24, 2009, Luck, pp.500-506 – „sigma: energia stikovoi mezhzerennoi granici [J94]….” –p.502.J94-c13. Gácsi Z., Simon A., Pázmán J.: Fémkompozitok, Miskolci Egyetem, 2011. „A felületi feszültség, azadhéziós energia és a peremszög (2-6 ábra) segítséget nyújtanak a fémkompozit gyártástechnológiamegtervezésében [J94].” – 39 o.J94-c14. I.Budai: Development of a mixer to fabricate particle stabilized aluminium matrix emulsions andmonotectic alloys - Mat.-wiss. u. Werkstofftech. 2012, 43, No. 4, pp.345-349. - „Thus, the design ofparticle stabilized metallic emulsions and monotectic alloys should be based on the existing databank onthe contact angle of particles at the interface of immiscible liquid metals / alloys [J94].” – p.345.J94-c15. Pázmán, J., Mádai, V., Gácsi, Z. and Kovács, Á. (2012) ‘Arrangement of the Al-Ni phases inAl/SiC(Ni)p composites’, Int. J. Microstructure and Materials Properties, 2012, vol. 7, No. 1, pp.49–63. –„… it is well known tha tthe interfacial metallic ion adhesion is stronger than metallic ceramics [J94]” –p.51.J94-c16. Balla S., Bán K., Bárdos A., Lovas A., Szabó A., Weltsch Z.: Járműanyagok - Egyetemi tananyag,szerkesztő: Lovas Antal, ISBN 978-963-279-628-4, Typotex Kiadó, Budapest, 2012, 269 pp. – „5.6.4fejezet: Felületi szegregáció [J94]” – 156-157 o., „5.6.5. fejezet: Adszorpció [J94]” – 157.o.J93. O.Verezub, G.Kaptay, T.Matsushita, K.Mukai: Penetration dynamics of solid particlesinto liquids. High-speed experimental results and modeling - Materials Science Forum, 2005,vols. 473-474, pp.429-434. (IF = 0.399)J93-c1. E.Bitay: Ceramic particle dispersion analysis in laser surface alloying – Materials Science Forum, 2006,vol.508, pp.295-300 – „Other factors, such as wettability of the particle by the liquid, drag force andgravity/buoyancy force was taken into account by some other authors [J93]” – p.298.J93-c2. Kálazi Z. (Buza G.): Alumínium lézersugaras felületötvözése – PhD szemináriumi beszámoló, 2008.december 9., Miskolci Egyetem, 22 oldal.J93-c3. Hórvölgyi Z.: Anorganikus részecskék folyadék-fluidum határrétegbeli diszperziói és szilárd hordozósfilmjei – MTA doktori értekezés, 2010. “A folyadék-fluidum határrétegben felhalmozódó kváziamfipatikus szilárd mikrofázisoknak különös jelentősége van a habok és emulziók stabilizálásában [J93]”– p.1.J93-c4. Baumli P.: Fémmátrixú kompozitok előállítása öntészeti módszerekkel – CD-Proc. of 26. Int Sci ConfmicroCAD, 29-30 March, 2012. – „Lézer segítségével felületi kompozitok állíthatóak elő. Ebben azesetben a mátrix anyagául szolgáló fém felületét lézerrel megolvasztják, és az így kialakult fémtócsábamegfelelő sebességgel lövik az erősítő fázisnak szánt szemcséket. Ezen technológiánál fontos, hogy aszemcséket milyen sebességgel lövik a fémtócsába. Ennek modellezését mutatja be a [J93] irodalom.” –4.o.J92. M.S.Yaghmaee, G.Kaptay: Stability of SiC in Al-rich corner of liquid Al-Si-Mg system -Materials Science Forum, 2005, vols. 473-474, pp.415-420. (IF = 0.399)J92-c1. E.Mostaed, A.Mostaed, H.Saghafian, A.Shokuhfar, H.R.Rezaie: Effect of SiC Particles VolumeFraction on the Mutual Diffusion of Al and Cu during Fabrication of Al-4.5wt%Cu/SiC via MechanicalAlloying – Defect and Diffusion Forum, 2009, vol.283-286, pp.499-503. – „In Eq. (1) and Eq. (2) showthe chemical reactions which take place at the temperature 923-1272 K [J92].” – p.499. „Fig.1. Thestandard Gibbs energy change and equilibrium constant as function of temperature for Eq.(2) [J92]” –p.500.J92-c2. X.Q.Luo, H.M.Guo, X.J.Yang: Heterogeneous nucleation for AZ91 with in situ synthesis Al 4 C 3 – Adv.Mater Res, 2010, vol.97-101, pp.1069-1072. „The surface of SiC particles were coated by Al 4 C 3 [J92]” –p.1071.J92-c3. E.Candan, H.V.Atkinson, Y.Turen, I.Salaoru, S.Candan: Wettability of aluminium-magnesium alloys onsilicon carbide substrates – J Amer Ceram Soc, 2011, vol.94, No.3, pp.867-874. “Yaghmaee and Kaptay[J92] have examined the stability range of SiC in ternary liquid Al-Si-Mg alloy and shown that a certainminimum critical Si content is needed in the melt to avoi the formation of Al4C3 at the interface. Thecritical Si-content has been found to increase both with temperature and with the Mg-content of the melt”– p. 868.J92-c4. Pázmán J.: Szilíciumkarbid szemcsék kémiai nikkelezése és fémkompozitokban történő alkalmazása –PhD disszertáció (tud. vez.: Gácsi Z.), Miskolc, 2010. – “Az Al4C3 vegyület kedvezőtlen tulajdonságai(rideg fázis, mely csökkenti a kompozit törési szívósságát és a hőállóságát, valamint vízzel reagálva akompozit korrózióval szembeni érzékenységét növeli meg [J92]” – 10.o.27

J92-c5. Pázmán, J., Mádai, V., Gácsi, Z. and Kovács, Á.: Arrangement of the Al-Ni phases in Al/SiC(Ni) pcomposites, Int. J. Microstructure and Materials Properties, 2012, vol. 7, No. 1, pp.49–63. – „The surfaceoxidation takes place at a temperature of 1,000°C to 1,100°C and the purpose of this procedure is toprevent the aluminium carbide formation (Al 4 C 3 ) [J92] by developing a silicon oxide layer between thesilicon carbide particles and the metallic aluminium matrix” – p.51.J92-c6. Pázmán, J., Gácsi, Z.: Studying of the microstructure int he AlCuSiMg/SiC(Nt)p composites, CD-Procof 26. Int. Sci Conf microCAD, 29-30 March, 2012, Miskolc, Hungary. – „Surface oxidation is performedat a temperature of 1,000- 1,100°C and the purpose of this procedure is to prevent the carbide formation[J92] by developing a silicon oxide layer between the silicon carbide particles and the metallic aluminiummatrix” – p.1.J91. I.Budai, M.Z.Benkő, G.Kaptay: Analysis of literature models on viscosity of binaryliquid metallic alloys on the example of the Cu-Ag system - Materials Science Forum, 2005,vols. 473-474, pp.309-314. (IF = 0.399)J91-c1. D.Zivkovic: Estimation of the viscosity for Ag-In and In-Sb liquid alloys using different models –Z.Metallkunde, 2006, vol.97, pp.89-93 – „some models can be in conflict with experimental points, aswas already shown [J91]” – p.90, „Eq.(6) works particularly well for system in which the purecomponents have similar properties (i.e. the Ag-Cu system [J91])” – p.91.J91-c2. Brillo J, Brooks R, Egry I, Quested P: Viscosity measurement of liquid ternary Cu-Ni-Fe alloys by anoscillating cup viscometer and comparison with models - INTERNATIONAL JOURNAL OFMATERIALS RESEARCH 98 (6): 457-462 JUN 2007 – „An overview of selected models that will bediscussed in the present work is given in [J91].” – p.457.J91-c3. YH Liu: Viscosity of molten Zn-Al, Zn-Cu and Zn-Al-Cu alloys – Galvantech07 (Proceedings), 2007,pp.171-176 – „Recently it was noticed by the author that prior to Liu’s work, Budai et al [J91] had alreadymodified Seetharaman’s model based on the same argument, but used the excess enthlapy of mixing toreplace the excess Gibbs energy of mixing” – p.172. „Budai et al [J91] pointed out that a positive deltaHwould reduce rather than increase deltaG*, thus changed Eq.(7) to: {Equation 8}” – p.174. „ Summary:The thermodynamic model by Budai, Banko and Kaptay [J91] for predicting the viscosity of binary alloyshas been successfully extended and used in prediction of the viscosity of ternary Al-Cu-Zn alloys” –p.175.J91-c4. S.Gruner, W.Hoyer: The dynamic viscosity of liquid Cu-Si alloys – J Alloys Compds, 2008, vol.460,pp.496-499 – „… both linear and semi-logarithmic mixing rules are used in literature, see [J91]. ….Reviews are to be found in [J91]” – p.498.J91-c5. D.Zivkovic: Application of the Kaptay model in calculation of ternary liquid alloys viscosities – Int JMat Res, 2008, vol.99, pp.748-750 – „Kaptay’s approach to estimate the viscosity of liquid metallic alloysfrom viscosities of pure liquid metals and thermodynamic properties of the liquid alloy has been tested fordifferent types of binary systems [J91], including those with considerable deviations from ideality” –pp.748-749.J91-c6. M.Kehr, M.Schick, W.Hoyer, I.Egry: Viscosity of the binary system Al-Ni – High Temperatures – HighPressures, 2008, vol.37, pp.361-368. – “An overview of the common models is given in [J91]. Afterhaving tested a variety of models it turned out that the two models provide reasonable results in the caseof Al-Ni alloys. One is the model of Kozlov [J91]:.. {Eq.2}. The second model has been developed byKaptay [J91] {Eq-s.3-4}. “ – p.364, “The calculated data are compared to the measured data in Fig.3. TheKozlov model produces values significantly higher than the measured ones. On the other hand theKaptay-model fits the measured values reasonably well. While the Kozlov model is taking into accountonly the viscosity of the pure liquid elements and the enthalpy of mixing, the Kaptay-model also considersthe interaction between the atoms of the liquid. Structural ordering is not taken into account in bothmodels. The partial deviations of the measured values from the smooth function of the Kaptay-model cantherefore be interpreted as a sign of structural ordering in the liquid. - pp.365-367, “Fig.3. Viscosityvalues calculated using the Kozlov-model [J91] (solid line) and the Kaptay-model [J91] (dashed line) andmeasured values of this work” – p.366.J91-c7. S. Gruner, W. Hoyer: A statistical approach to estimate the experimental uncertainty of viscosity dataobtained by the oscillating cup technique – J. Alloys Compounds, 2009, pp. 629-633 – „A variety ofmodel equations for the viscosity of multi-component liquids have been developed – for recent reviewssee [J91]” – p.629J91-c8. S.Gruner, J.Marczinke, W.Hoyer: Short-range order and dynamic viscosity of liquid Cu-Ge alloys – JNon-Cryst. Solids, 2009, vol.355, pp.880-884 – “Reviews of possible approaches (for concentration28

dependence of viscosity) are given in [J91]. From the models presented in [J91] the Kozlov equation isselected for the present study” – p.882.J91-c9. Wunderlich RK; Fecht H-J: Surface tension and viscosity of NiAl catalytic precursor alloys frommicrogravity experiments – Int J Mater Res, 2011, vol.102, pp.1164-1173. „The Kaptay model was shownto provide better agreement with observed viscosities of binary alloys [J95] than the Moelwyn-Hughesmodel. In the Kaptay model the viscosity is given by: Eq-s.(15-16), Fig.11, Table 2.” – p.1170-1171.J91-c10. Wunderlich R.K., Fecht H.J., Egry I., Etay J., Battezzati L., Ricci E., Matsushita T., Seetharaman S.:Thermophysical Properties of a Fe-Cr-Mo Alloy in the Solid and Liquid Phase – Steel Res Int, 2012,vol.83, pp.43-54. „From more recent semi-empirical thermodynamic models [J91] an increase to 8.84mPas for an alloy with more than 94 at % Fe is not to be expected from an alloying effect”. – p.52.J91-c11. M.Schick, J.Brillo, I.Egry, B.Hallstedt: Viscosity of Al-Cu liquid alloys: measurement andthermodynamic description – J Mater Sci, 2012, doi: 10.1007/s10853-012-6710-x – “It has been argued[J91] that, in the simplest way, the pre-exponential factor of the alloy is expressed as a function of theconcentration in the following way: Eq.(10)” – p.J91-c12. R.N.Singh, F.Sommer: Viscosity of liquid alloys: generalization of the Andrade’s equation – MonatshChem, 2012, vol.143, pp.1235-1242. – „Results obtained from these relations have been compared withnew or given [J91] experimental viscosity data as a function of composition and temperature.” – p.1235.J90. T.Bárczy, G.Kaptay: Modelling the infiltration of liquid metals into porous ceramics -Materials Science Forum, 2005, vols. 473-474, pp.297-302. (IF = 0.399)J90-c1. Orbulov IN, Németh Á, Dobránszky J: XRD and EDS Investigations of Metal Matrix Composites andSyntactic Foams. 13th European Conference on X-Ray Spectrometry, Cavtat, Croatia, 16-20 June 2008,In: EXRS 2008 Proceedings. “The required pressure can be estimated by numerical methods and dependson the wetting similarly as in the case of fibre-reinforced MMCs [J90]” – p.2/10J90-c2. Orbulov I, Németh Á, Dobránszky J: Manufacturing of Composites by Pressure infiltration, Structureand Mechanical Properties. In: Penninger A, Váradi K, Vörös G (eds.), Gépészet 2008, Proceedings ofSixth Conference on Mechanical Engineering, BUTE Faculty of Mechanical Engineering – “Thisthreshold pressure can be calculated by theoretical approaches for various systems [J90]” – p.1/9.J90-c3. I.N.Orbulov, J.Dobránszky: Producing metal matrix syntactic foams by pressure infiltration – PeriodicaPolytechnica Mechanical Engineering, 2008, vol.52, No.1, pp.35-42. – „Bárczy and Kaptay (2005)developed a fully theoretical model for closely packed spheres based on the equilibrium of gravitational,capillary and outer forces. The model considered the effect of wetting angle, surface tension and volumefraction [J90] – p.35. “Eq.(1), Table 3, calculated values are given” – p.38J90-c4. I.N.Orbulov, J.Dobranszky, A.Nemeth: Microstructural characterization of syntactic foams – J MaterSci, 2009, vol.44, pp.4013-4019 – “Barczy and Kaptay [J90] developed a theoretical method byconsidering the wetting angle, surface tension and based on the equilibrium of gravitational, capillary andouter forces.” – p.4014.J90-c5. Orbulov I.N.: Szintaktikus fémhabok, PhD értekezés (Dobránszky János és Németh Árpád, BME, 2009.június) – „A küszöbnyomás elméleti becslésére Bárczy és Kaptay analitikus modellt dolgozott ki [J90]. Eza munka tartalmazza…. 1 oldal, 5 egyenlet, 2 ábra a cikkből” – 17-18. oldalak, „8. táblázat: Bárczy-Kaptay modell [J90] (számolt értékek)” – 36. oldal. „Az infiltrálási küszöbnyomás 0,5 és 0 bar között van.Ezt az értéktartományt Rohatgi és Trumble modelljei nagymértékben alulbecslik. A Bárczy-Kaptaymodell helyesebb eredményt ad, bár a küszöbnyomás értéktartományát kismértékben felülbecsüli.” – 38.o.J90-c6. I.N.Orbulov, Á.Németh, J.Dobránszky: Hardness Testing of metal matrix syntactic foams – Proc. Of 7thInt Conf on Mechanical Testing, BME, Hungary, 2010, pp.16-22. – „Bárczy, Kaptay and other authorsdeveloped theoretical and semi-experimental methods to determine the threshold pressure [J90]” – p.16.J90-c7. Kientzl I.: Alumíniummátrixú kompozithuzalok és kettős kompozit-szerkezetek – PhD értekezés, BME(tud. vez.: dr.Dobránszky János), 2010, 112.o. – „.. ha a porózus test egyforma, szorosan pakoltgömbökből van kirakva, akkor a kritikus peremszög 50,7 o [J90]” – 20.o.J90-c8. Orbulov I.N.: Szintaktikus fémhabok mikroszerkezeti vizsgálata – Gép, 2010, No.11, pp.4-8 – „Bárczyés Kaptay [J90] elméleti modellt fejlesztett ki, amely figyelembe veszi a nedvesítési szöget, a felületifeszültséget és a gravitációs, kapilláris és külső erők (infiltráló nyomás) egyensúlyán alapszik”. – p.4.J90-c9. Orbulov I.N., Á.Németh: Global, depth sensing and dynamic hardness of metal matrix syntactic foams –Periodica Polytechnica, 2009, vol. 53, No.-2, pp.93-99. – „Bárczy and Kaptay developed a theoreticalmethod considering wetting angle, surface tension and based ont he equilibrium of gravitational,capillary and outer forces [J90]” – p.93.J90-c10. I.Orbulov, K.Májlinger: On the microstructure of ceramic hollow microspheres – PeriodicaPolytechnica, 2010, vol.54, No.2, pp.89-94. – „… the contact angle between the microspheres and the29

metal matrix has a detrimental effect on the infiltration characteristics and ont he threshold pressure (inthe case of pressure infiltration) [J90]” – p.90.J90-c11. I.N.Orbulov: Infiltration of ceramic microballons by liquid metals – research plan for SCIEX-NMS,February, 2011, 12 pp. – „Other articles are interested especially in the infiltration of microspheres andmicroballons and this is the case of MMSFs [J90]” – p.9.J90-c12. Svidró József Tamás (konzulensek: Diószegi Attila és Tóth Levente): Transzportfolyamatok afém/formázóanyag határfelületén – PhD értekezés, Miskolci Egyetem, 2011 – „2.3.3 alfejezet: A CPESmodell [J90]” – pp.16-17.J90-c13. Rácz A., Tóth L.F.: Eszközfejlesztés mikrogömbhéjak infiltrálásához – TDK dolgozat, 2011, BME(konzulens: Orbulov IN) – “2.9. Fémolvadék infiltrációjának modellezése porózus kerámiába [J90]” – 29-31. o.J90-c14. Orbulov I.N., Kun P., Németh Á., Dobránszky J.: Investigation of Light Weight Metal Foams. In:Borbás Lajos (ed.): 28th Danubia-Adria-Symposium on Advances in Experimental Mechanics.Siófok: GTE, 2011, pp. 267-268. „For successful pressure infiltration a threshold pressure must beensured, which can be estimated by theoretical and experimental methods [J90]” p. 267.J90-c15. E. de Lorgeril, F. Wyss, I.N. Orbulov: Modelling of metal matrix syntactic foams – description of thecompressive stress-strain curves - Periodica polytechnica Mechanical Engineering, 2011, vol.55/1, pp.29-37. – „papers on the problems of MMSF producing were also published [J90]” – p.29.J90-c16. I.N. Orbulov: Syntactic foams produced by pressure infiltration – the effect of pressure and time oninfiltration length- Periodica polytechnica Mechanical Engineering, 2011, vol.55/1, pp.21-27. – „Kaptayet al. developed a fully theoretical model for closely packed spheres (CPES) to predict the thresholdpressure for infiltration. The model based on the equilibrium of gravitational, capillary and outer forcesand considered the e_ect of wetting angle, surface tension and volume fraction [J90] + 2 equations …. ” –p.22.J90-c17. Orbulov IN: Mikrogömbhéjak nyomásos infiltrációjának vizsgálati módszere – OGÉT 2011, XIX.Nemzetközi Gépész Találkozó konferencia kiadványa, Csíksonlyó, Románia, 2011. 04.28-05.01.Szerkesztő: Csibi V-J. Kiadó: Erdélyi Magyar Műszaki Tudományos Társaság, Kolozsvár, Románia,2011, pp.296-299, ISBN: 2068-1267 – „Amennyiben a nyomás kezdeti értéke meghaladta agömbhéjak infiltrálásához szükséges, oxidos nedvesítési viszo-nyokkal számított infiltrálásiküszöbnyomást (Bárczy és Kaptay modellje szerint ~110 kPa [J90]), az ömledékfront behatolt agömbhéjak közé, amelyek – mintegy alaki ellenállást kifejtve – az infiltrálást hajtónyomáskülönbséget folyamatosan csökkentették. ” p. 2092.J90-c18. I.N.Orbulov, J.Ginsztler: Compressive characteristics of metal matrix syntactic foams – Composites A,2012, vol.43, pp.553-561. „Bárczy and Kaptay developed a new infiltration model for closely packedequal spheres CPES structire. In their study the threshold pressure, the threshold contact angle and theequilibrium height of penetration has been determined. The experiments demonstrated the reliability ofthe theoreetical results [J90]” – p.554.J90-c19. Baumli P.: Fémmátrixú kompozitok előállítása öntészeti módszerekkel – CD-Proc. of 26. Int Sci ConfmicroCAD, 29-30 March, 2012. – „ha az infiltrációhoz használt porózus anyagot szorosan illeszkedőgömbök alkotják, a közöttük lévő pórusokba a penetrációhoz szükséges kritikus peremszög 50,7 fok[J90].” – 3.o.J90-c20. I.N.Orbulov: Infiltration and mechanical characteristics of hollow spheres reinforced metal matrixcomposites – Proc. 8th International Conference on Mechanical Engineering, 2012, pp. 403-411. – „Inorder to successful infiltration a threshold pressure must be assured by the infiltrating system. Thispressure can be determined by theoretically and experimentally. Kaptay et al developed a theoreticalmodel for closely packed spheres to predict the threshold pressure [J90].” – p.403.J90-c21. K.Májlinger, I.N.Orbulov: Elemental distribution and orientation analysis on metal matrix syntacticfoams - Proc. 8th International Conference on Mechanical Engineering, 2012, pp. 301-308. – „In all casesthe contact angle between the ceramic microspheres and the metal matrix has a detrimental effect on theinfiltration characteristics and on the threshold pressure (in the case of pressure infiltration) [J90].” –p.302J90-c22. IN Orbulov: Compressive properties of aluminium matrix syntactic foams – Mater Sci Eng A, 2012,vol.555, pp.52-56. – „In all cases poor wetting or large contact angle between the ceramic hollow spheresand the metal has a detrimental effect on the infiltration characteristics and on the threshold pressure (inthe case of pressure infiltration) [J90].” – p.53.J90-c23. IN Orbulov, K.Májlinger: Microstructure of metal-matrix composites reinforced by ceramicmicroballons – Materiali in Tehnologije, 2012, vol.46, No.4, pp.375-382. – „..the contact angle betweenthe ceramic microspheres and the metal matrix has a detrimental effect ont he infiltration characteristics..[J90]” – p.376.30

J90-c24. IN Orbulov, J.Ginsztler: Compressive Behaviour of Metal Matrix Syntactic Foams – Acta Polyt Hung,2012, vol.9, No.2, pp.43-56. – „Bárczy and Kaptay developed a new infiltration model for closely packedequal spheres structure. In their study, the threshold pressure, the threshold contact angle and theequilibrium height of penetration were determined. All these parameters are significantly different fromthose obtained from the traditional capillary penetration model, but similar to the Carman model. Theexperiments demonstrated the reliability of the theoretical results [J90]” – p.45.J89. J.Sytchev, N.Borisenko, G.Kaptay: Intercalation of lithium into graphite as the first stepto produce carbon nanotubes in an electrochemical way – Materials Science Forum, 2005,vols. 473-474, pp.147-152 (IF = 0.399)J89-c1. Adamokova M.N.: Elektrovidelenie metallicheskogo volframa, molibdena i ich karbidovi znizkotemperaturnich galogenidno-oksidnich rasplavov – Diss. na kand. him. nauk, Ekaterinburg, 2005,142 pp. – „V 2000 g. nachala publikovat rezultati issledovanii po polucheniiu nanotrubokelektroliticheskim metodom tretia gruppa – Kaptay G i Sychev J.Iv Vengrii [J89] vosproizveli rezultatirabot Fray-a, takzhe pokazali, shto elektroosozhdenie litiia, natriia, kaliia, magniia, kalciia izsootvetstvuiushich rasplavlennich hloridov privodit k polucheniu uglerodnich nanotrubok. Produktielektroliza bili issledovani metodom atomno-silovoi mikroskopii”….. „G.Kaptay i J.Sichev ssotrudnikami (Vengriia) zanimaiutsia issledovaniem mechanizma obrazovaniia uglerodnich nanotrubokpri osazhedenii shelochnich metallov (litiia i natriia) i shelochnozemelnich metallov (magniia i kalciia) izrasplavlennich solei na grafitovii katod [J89]” – p.25.J88. P.Baumli, J.Sytchev, Zs.H.Göndör, G.Kaptay: Interaction between a titanium-containingmolten salt and an alumina plate - Materials Science Forum, 2005, vols. 473-474, pp.39-44.(IF = 0.399)J88-c1. Zhai XJ, Zhang Z, Li JD, Zhang MJ: Deoxidization mechanism of in-situ electro-deoxidization of TiO2to titanium – in: TMS 2008 ANNUAL MEETING SUPPLEMENTAL PROCEEDINGS, VOL 1:MATERIALS PROCESSING AND PROPERTIES 2008, TMS, pp. 385-390.J87. G.Kaptay: A new equation for the temperature dependence of the excess Gibbs energy ofsolution phases – CALPHAD, 2004, vol.28, pp.115-124. (in „Top 25 articles within thejournal” – „No.13.” in 2nd quarter of 2005, „No.12” in the 4th quarter of 2005 and „No.12” in the 1stquarter of 2006) (IF = 2.119)J87-c1: Schmid-Fetzer R, Janz A, Grobner J, Ohno M: Aspects of quality assurance in a thermodynamic Mgalloy database – Adv Eng Mater, 2005, vol. 7 (12), pp. 1142-1149 - „There is no simple solution togenerally avoid the artifact of the inverted gap within the freamework of the most popular lineartemperature dependency of liquid interaction parameters. Kaptay [J87] has clearly pointed out that thelinearity results in an unrealistic exaggeration of excess mixing quantities at high temperature.However, the suggested solution of exponential temperature dependence [J87] may result in an artificialre-stabilization of the liquid phase at low temperature as detailed recently for the example of Mg-Sialloys” – p.1144.J87-c2. Arroyave R, Liu ZK: Thermodynamic modelling of the Zn-Zr system – Calphad, 2006, vol. 30, pp.1-13.– „The interaction parameters of the liquid phase are modelled with an exponential temperaturedependence, as recommended by Kaptay [J87]. In the latter case, the description of the hcp and bccphases are modified accordingly” – p.1, .. „For the long time, it has been recognized that the (linear)expression may be problematic… To alleviate this problem, Kaptay [J87] has proposed a differenttemperature dependence for the interaction parameters: (Eq.8)…. This feature essentially eliminatesinverted miscibility gaps” – p.3, .. “Model 3. The liquid and solid solution are modeled with interactionparameters that decay exponentially with temperature” – p.4, … “ ..the three models yield essentiallythe same phase diagram… Model 2 is the best… Model 3 is not satisfactory and perhaps a morecomplicated temperature dependence needs to be employed” – p.12.J87-c3. Malakhov DV, Balakumar T: Re-optimization of the Mg-Sb system under topological constraints – Int JMater Res, 2006, vol.97, pp. 517-525 – „If a better model is difficult to find, then various empirical orheurestic approaches can be tried. An interesting and very elegant semi-empirical method for getting ridof an inverted miscibility gap was recently proposed by Kaptay [J87]. The method, however, is notcapable of handling the situations when a phase becomes stable in a region within which it should notexist. Besides, a utilization of Kaptay’s fomalism in practice is hampered by the necessity to rewrite31

source codes upon which Gibbs energy minimizers and procedures for optimization are based.” – p.518.J87-c4. R.Schmid-Fetzer, D.Amdersson, P.Y.Chevalier, L.Eleno, O.Fabrichnaya, U.R.Kattner, B.Sundman,C.Wang, A.Watson, L.Zabdyr, M.Zinkevich: Assessment techniques, database design and softwarefacilities for thermodynamics and diffusion – Calphad, 2007, vol.31, pp.38-52. – „generally, theenthalpy and the excess entropy of mixing should have the same sign [J87]…. The –a/b ratio should bein the order of 3000 K for most systems [J87]…. Another possibility is to try to avoid the artificialmiscibility gap completely, by bringing the liquid excess parameters to zero at high temperatures.Kaptay [J87] suggested an exponential function of the form ..Eq.(5).. (my equation is given)… Thereasoning proposed by Kaptay is convincing since Eq.(5) satisfies all the necessary boundary conditionsat high (and low) temperatures that are demanded. It is also true that over a limited temperature range,where actual experimental data may be provided, the exponential function does not visibly deviate froma straight line, as shown by Kaptay in a graph for the range 0.3 < T/tau < 0.4. However, no Calphadtype analysis was performed in that paper [J87].” – p.43. „We have attempted to re-model the Mg-Sisystem using (Kaptay) Eq. This is a good test system since it contains just one stoichiometricintermediate phase, Mg2Si, having a well defined Gibbs energy and so only the Gibbs energy of theliquid remains to be adjusted. In fact, the inverted gap is avoided, as expected. However, for all themodel parameter settings that came close to a proper description of at least the invariant phaseequilibria in Fig.2, another artifact at low temperature is observed.” – p.43. „Fig 3 shows an attempt toreproduce the stable phase diagram by just refitting the liquid description with two Redlich-Kisterexcess parameters (L0 and L1, with h0, h1, 0, 1) with an exponential T-dependence (Eq-s 6.a-b). Theoptimized values of the 4 coefficients resulting from using only the invariant phase equilibria (but thereare only 3 of them [GK]) as experimental information was: h0 = -95358 J/mol, 0 = 1303.8 K, h1 = 15442 793 J/mol (15 MJ/mol ?? [GK]) and 1 = 120.6146 K (120 K?? [GK]). This attempt removed theinverted miscibility gap but instead the liquid became stable at low temperature, see Fig.3 (the low-Tartifact is caused by not performing full assessment of the system and by finding 4 parameters using 3nonvariant points, meaning one of the parameters is selected freely, thus by doing so it is not proventhat the low-T artifact can happen in reality. However, it indeed proves that the low-T artifact canhappen at least in principle [GK]). This artifact may be avoided by keeping track of the values of h and or by adding extra experimental information to prevent the liquid from becoming stable below somelimit (e.g. 100 K), but it shows that the exponential model cannot be used without care” – p.44.„Therefore, the basic idea of (Kaptay) Eq is good and clearly superior to the popular linear equationand, in fact, solves the problem associated with high temperatures, but unfortunately may induce a newproblem at low temperature” – p.44.J87-c5. Malakhov DV, Balakumar T: Thermodynamic optimization under topological constraints: principles andexamples – Calphad, 2007, vol.31, pp.402-403 (ref. No.4). – „Although the importance of this problemwas understood a while ago, the first method specially tailored to struggle against inverted miscibilitygaps was proposed only two years ago [J87]. Recently, a remarkably elegant Kaptay’s approach wastried for optimizing the Zn-Zr system” – p.403.J87-c6. M.Idbenali, C.Servant, N.Selhaoui, L.Bouirden: A thermodynamic modelling of the Ba-Pb system –Calphad, vol.31, 2007, pp.479-489. – „In order to avoid during the phase diagram calculation theoccurence of an unwanted miscibility gap in the liquid phase up to 6000 K [J87], additional constraintswere imposed, such as the Gibbs energy of the liquid phase with positive curvature d 2 G/dx 2 > 0, on thewhole Pb composition range and every 500 K from 1000 to 6000 K” – p.481.J87-c7. Malakhov DV, Balakumar T: Post-optimization elimination of inverted miscibility gaps -INTERNATIONAL JOURNAL OF MATERIALS RESEARCH 98 (9): 786-796 SEP 2007 – „A veryinteresting and potentially useful refinement proposed by Kaptay [J87] has already been tried foroptimizing the Zn-Zr system…” – p.786.J87-c8. V.Grolier, R.Schmid-Fetzer: Experimental study of Au-Pt-Sn phase equilibria and thermodynamicassessment of the Au-Pt and Au-Pt-Sn systems – J. Electronic Mater, 2008, vol.37, pp.264-278 –’”Kaptay did recently propose for Calphad optimization purposes the constraint simplification: tau0 > 0[J87]” – p.272.J87-c9. M.Idbenali, C.Servant, N.Selhaoui, L.Bouirden: A thermodynamic reassessment of the Ca-Pb system –Calphad, 2008, vol.32, pp.64-73 – „In order to avoid the formation of an unwanted inverted miscibilitygap of the liquid phase during the calculation of the Ca-Pb phase diagram, constraints must be imposedduring the optimization procedure [J87]” – p.66. “Finally, we verified that no miscibility gap wascalculated with our thermodynamic optimized parameters as commended in [J87]” – p.71.J87-c10. C.Guo, Z.Du, C.Li: A thermodynamic description of the Mg-Pr-Y system – Calphad, 2008, vol.32,pp.177-187 – „Kaptay [J87] and Arroyave and Liu [J87-c2] pointed out that this expression of theRedlich-Kister equation may become problematic, especially in cases where the thermodynamic32

description is intended to be valid over a wide temperature range. Usually, the excess enthalpies andentropies of mixing have the same sign. Thus, there is always a temperature at which the L parameterchanges sign. When this change is from negative to positive, and if this effect is more dominant than the… term due to ideal mixing, then spurious miscibility gaps tend to appear.” – pp.185-186.J87-c11. M.Idbenali, N.Selhauni, L.Bouirden, C.Servant: Thermodynamic assessment of Fe-Hf binary system –J Alloys Comp., 2008, vol.456, pp.151-158 – „Two years ago, a method was propsed for avoiding theformation of an artificial inverted miscibility gap above the liquidus line [J87]…. Kaptay [J87] showedthat, when using … 13 lines + eq-s” – p.153., + “5 lines, Eq.” – p.156-157.J87-c12. H.Ran, Z.Du, C.Guo, C.Li: Thermodynamic modeling of the Ru-Zr system – J Alloys Compounds,2008, vol.464, pp.127-132. – “Abstract: The solution phases were modeled with a new semi-empiricalequation, which was recommended by Kaptay.” P.127, “.. To solve this problem, Kaptay [J87] hasproposed a new semi-empirical equation {8 lines}… In order to compare the difference for the liquidphase between the models, two sets of thermodynamic descriptions were considered: the liquid andsolid solutions are modeled with the linear temperature dependence by the Redlich-Kister equation andwith the exponential temperature dependence by the Kaptay equation [J87]” – p.128, “Table 1, Kaptayequation” – p.129, “Fig.1. Calculated Ru-Zr phase diagram by the present thermodynamic descriptionusing (A) Kaptay equation [J87] and (B) Redlich-Kister equation with experimental data” – p.130,“Fig.2, Kaptay equation [J87]”, p.130, “Fig.3, Kaptay equation”, p.130, “Table 2, Kaptay equation[J87]”, p.131, “Fig.4. Calculated Gibbs energies of the bcc solution (A2) and RuZr with CsCl-typestructure (B2) at 1800 K in the Ru-Zr system using Kaptay equation [J87]” – p.131. “Fig.5. CalculatedGibbs energies of the hcp solution (A3) and Ru 2 Zr with MgZn 2 -type structure (C14) at 2000 K in theRu-Zr system using Kaptay equation [J87]” – p.131. “The Ru-Zr phase diagram calculated by means ofthermodynamic parameters using the Kaptay equation [J87] is presented in Fig.1A, and is nearlyidentical to the one represented by experimental data of Eremenko et al.” – p.131. “In view of theestimated experimental errors (about 1-2 at%), all of the 18 experimental invariant reactioncompositions in the Ru-Zr system are well reproduced by the Kaptay equation [J87]” – p.132. “It isshown that the Kaptay equation [J87] is the better one that reproduces the experimental data” – p.132.“Conclusions: A very good agreement is obtained between the calculations and experiments forRedlich-Kister and Kaptay equations, except for the liquid phase using the Redlich-Kister equationbecomes unstable at 4700 K, while it is stable at high temperature using the Kaptay equation” – p.132.J87-c13. D.V.Malakhov: On a shape-preserving thermodynamic optimization – Arch Metall Mater, 2008, vol.53,No.4, p.1097-1106. – „If the choice (of the model) was prompted by a „mathematical convenience”, i.e.if an aphysical formalism was used, then extrpolating may lead to artifacts … Among such artifacts,inverted miscibility gaps in the liquid phase at elevated temperatures are seen most frequently; thereasons behind their appearance are well understood [J87].” – p.1097.J87-c14. Y.Gao, C.Guo, C.Li, S.Cui, Z.Du: Thermodynamic modeling of the Ru-Ti system – J AlloysCompounds, 2009, vol.479, pp.148-151 – “values calculated by means of the thermodynamicparameters using the Redlich-Kister equation and the Kaptay equation are presented in Fig.1a and 1.b,respectively, nearly identical to the one represented by Eremenko.” – p.150. “In view of the estimatedexperimental errors (about 1-2 at %), most of experimental invariant reaction compositions in the Ru-Tisystem are well reproduced for Redlich-Kister and Kaptay equation.” – p.150. “Fig.2. Kaptay equation”– p.151, “Fig.3. Kaptay equation” – p.151, “Fig.3. is the calculated molar Gibbs energies of the bccsolution (A2) and RuTi with CsCl-type structure (B2) at 1600 K in the Ru-Ti system according to theRedlich-Kister equation and Kaptay equation” – p.151. “A very good agreement is obtained betweenthe experiments and two calculations for Redlich-Kister and Kaptay equation” – Conclusion, p.151.J87-c15. X.Yuan, W.Sun, Y.Du: Thermodynamic modeling of the Mg-Si system with Kaptay’s equation forexcess Gibbs energy of liquid phase – Book of Abstracts to the 38 th Calphad conference, 17-22 May,2009, Praha, page 145. – “The Mg-Si system was re-modeled using Kaptay’s equation [J87], in whichthe equation …. was introduced to describe the excess Gibbs energy of the liquid phase. Compared withthe previous assessments, in which the Redlich-Kister polynomial was used for the description of theliquid phase with a linear T-dependence of the interaction energies, the artificial inverted miscibilitygap at high temperature was removed. Moreover, the liquid phase is not restabilized at lowtemperatures. The calculated phase diagram and thermodynamic properties agree well with theexperimental data” – p.145.J87-c16. M.Li, C.Guo, C.Li, Z.Du: A thermodynamic description of the Cr-Ge system – J Alloys Compd, 2009,vol.481, pp.283-290 – “Abstract: The excess Gibbs energies for the solution phases .. were describedusing the polynomial temperature dependence and Kaptay equation” – p.283, “The miscibility gaps donot close and imply that the solution is unstable. To solve this problem Kaptay [J87] proposed a semiempiricalequation (7)…” – p.285. “Kaptay equation” – in Tables 2, 3 + in Figs 1.a, 1.b, 2, 3.a, 3.b, 3.c,6. “As shown in Table, satisfactory agreement is obtained between calculations and experimental33

values”. “Solid lines and dashed lines in Fig.1.a represent the calculated results using the polynomialtemnperature dependence and Kaptay equation [J87], respectively. As shown in Fig.1.a, solid lines areidentical to dashed lines at low temperature range. However, the liquid modeled with the polynomialtemperature dependence has the critical temperature (about 6200 K) for the inverted miscibility gap. Asmentioned in Section 3.2, the interaction parameters with the polynomial temperature dependence areonly valid below the critical temperature and Kaptay equation [J87] is applied to overcome this problemin the present work.”. “Conclusion: A good agreement is obtained between the experiments and twocalculations according to the polynomial temperature dependence and Kaptay equation”. – p.290.J87-c17. S.Arnout: PhD thesis (assessment of phase diagrams in oxide systems with Cr 2 O 3 ), KatholikeUniversitat, Leuven, 2009 – „This is a dangerous situation as it creates inverted miscibility gaps.Instead of the linear terms, Kaptay [J87] proposed to use an exponential term, which goes to zero athigh temperatures. The use of this kind of parameters has, however, not been implemented in thequasichemical model” – p.120.J87-c18. X.Yuan, W.Sun, Y.Du, D.Zhao, H.Yang: Thermodynamic modeling of Mg-Si system with the Kaptayequation for the excess Gibbs energy of the liquid phase – Calphad, 2009, vol.33, pp. 673-678. doi:10.1016/j.calphad.2009.08.004. –„Abstract: The Mg-Si system was remodeled using the Kaptayequation .. Compared with the previous assessments using a linear temperature dependence .. thearitificial inverted miscibility gap at high temperature is removed.” – p.673. „Summary: The Kaptayequation was successfully used to describe the liquid phase int he Mg-Si system.” – p.678.J87-c19. CY Zhan, W.Wang, Z.L.Tang, Z.R.Nie: Thermodynamic Research on Solution Properties of Al-ErAlloys – Mater Sci Forum, 2009, vol.610-613, pp. 674-680 – „Abstract: Mixing enthalpy of Al-Erbinary alloys system has been calculated based on Miedema model, in which a new interactionparameters Li proposed by George Kaptay was considered: Li=h0i.exp(-T/τ0i ), which are used toindirectly calculate the activity of Er in Al-Er alloys and some other thermodynamic properties, such asexcess Gibbs energy and excess entropy at 1073K.”J87-c20. X.Li, C.Li, Z.Du, C.Guo: Thermodynamic analysis on ageing process of Mg-Zn alloys – Chinesejournal at www.paper.edu.cn, 2009, vol.2, No.22, pp.2364-2372 – „… KAPTAY [J87]… Eq.(4) +parameters of Table 6”J87-c21. C.Guo, C.Li, Z.Du: A thermodynamic modeling of the Gd-Tl system – J Alloys Compounds, 2009,vol.492, pp.122-127. – „In the present work, the excess Gibbs energiesof the liquid, bcc and hcpsolution phases were modeled using the polynomial temperature dependence and Kaptay equation” –p.122. „To solve this problem, Kaptay [J87] has proposed a semi-empirical equation: ….” – p.123. „Inaddition, the Kaptay equation [J87] was applied int he solutions liquid, bcc and hcp in order to avoid themetastable miscibility gap at high temperature int he liquid state… Table 3. Thermoduynamicparameters of the liquid, bcc and hcp solution phases using the Kaptay equation in the Gd-Tl system” –p.3. „Table 4. Kaptay equation…” – p.126,, „Fig.1.b Calculated Gd-Tl phase diagram using Kaptayequation [16] with experimental data” – p.126, „Fig.3. Calculated molar Gibbs energies of the bccsolutiion (A2) and GdTl with CsCl-type structure (B2) at 1300 K using polynomial temperaturedeoendence and Kaptay equation [J87] int he Gd-Tl system” – p.126, „The interaction parametersexpressed using Kaptay equation int he excess Gibbs energy for solution phases have certain physicalinterest, and can avoid the artificial miscibility gap in liquid at elevated temperature. Usually, thethermodynamic parameters optimized using Kaptay equation model are recommended to choose.However, in past decades, the interaction parameters int he excess Gibbs energy of the solution phasesfor almost all alloy systems were expressed in polynomial dependence of temperature, which were alsoused in almost all thermodynamic databases. Int he rpesent work, the thermodynamic parameters usingtwo models for solution phases are optimized.” – pp.126-127. „Conclusions. A good agreement isobtained between the experiments and two calculations according to the polynomial temperaturedependence and Kaptay equation.” – p.127.J87-c22. Z.Chunyao, W.Wei, N.Zuoren: Electron Theory Research on Al-4.5Mg-Zr-Er Alloys – MaterialsReview (in Chinese), 2009, vol.18 (http://en.cnki.com.cn/Article_en/CJFDTotal-CLDB200918026.htm)– „Interaction parameter LA-B between components proposed by George Kaptay is introduced,then theinteraction parameters between Al and Er,Zr,Mg are worked out based on Miedema model” – AbstractJ87-c23. Wang XL, Li CR, Guo GP, Du ZM, He W: Precipitation behaviour of GP zones during ageing processof Mg-Zn alloy – Acta Metall Sinica, 2010, vol. 46, No. 5, pp. 575-580 – „Kaptay Eq.(4) [J87]” – p.579J87-c24. C.Niu, M.Liu, C.Li, Z.Du, C.Guo: Thermodynamic description on the miscibility gap of the Mg-basedsolid solution in the Mg-Zn, Mg-Nd and Mg-Zn-Nd systems – Calphad, 2010, vol.34, pp. 428-433 – „Inthe present work a new, semi-empirical equation proposed by Kaptay [J87] is used to describe theinteraction parameter of the hcp-A3 solid solution, in order to prevent the apperance of the artificialmiscibility gap at high temperature” – p.429.34

J87-c25. D.V.Malakhov, M.Hosseinifar: A heuristic method to uncover a possible unsoundness of a physicalchemicalmodel – Calphad, 2010, vol.34, pp.467-477 – „Defect of such models as well as deficienciesof mathematically handy but physically reproachable formalisms usually manifest themselves in the socalledartifacts with inverted miscibility gaps [J87] being most frequent among them” – p. 468.J87-c26. S.H.Sheng, R.F.Zhang, S.Veprek: Phase stabilities and decomposition mechanism in the Zr-Si-Nsystem studied by combined ab initio DFT and thermodynamic calculation – Acta Mater, 2011, vol.59,pp.297-307 – “We consider also the exponential T-dependence which has been recently recommendedby Kaptay [J87] and successfully used for the thermodyanmic modeling of the Zn-Zr system” – p.298,“The exponential dependence of interaction parameter on temperature is given by [J87]: {Eq.(8)} +explanation” – p.303, “Fig-s 4b, 5b, 6c, 7”, - pp. 303-305, “The exponential T-dependence yields crossoverpoints of about x = 0.10-0.15 in better agreement with the experimental results than the linear one”– p.304.J87-c27. Wang W, Guo CP, Li CR, Du ZM: Thermodynamic re-modeling of the Co-Gd system – Int. J. MaterRes., 2010, vol.101, pp.1339-1346.J87-c28. P.Wang, L.Zhou, Y.Du, H.Xu, S.Liu, L.Chen, Y.Ouyang: Thermodynamic optimization of the Cu-Ndsystem – J Alloys Compounds, 2011, vol.509, pp.2679-2683 – „Due to the development of the newthermodynamic software, and the increasingly enhanced awareness of these problems, they can bedetected by powerful sotware [J87]” – p.2679.J87-c29. S.Sheng: Investigations into superhard nitride- and oxide-based nanocomposites by means of combinedab-initio DFT and thermodynamic calculations – Doktors der Naturwissenschaften, TU München, 2010– „Kaptay recently recommended the use of the exponent6ial temperature dependence [J87].”, p.35.“The exponential dependence of interaction parameter on temperature given by Eq. [J87]… “ – p.43.J87-c30. Tang Y, Yuan X, Du Y: Thermodynamic modeling of the Fe-Zn system using exponential temperaturedependence for the excess Gibbs energy – JMM, 2011, vol.37, No.1, pp.1-10. “Abstract: The Fe-Znbinary system was re-modeled using exponential equation to describe the excess Gibbs energy of thesolution hases and intermetallic compounds with large homogenities. A self-consistent set ofthermodyanmic parameters is obtained and the calculated phase diagram and thermodynamic propertiesusing the exponential equation agree well with the experimental data….” – p.1. “… a more generalmethod is to introduce the exponential equation, which is suggested by Kaptay in 2004 [J87], todescribe the excess Gibbs energy for the solution phase. This exponential equation has bee napplied tothe assessment of several (6) binary systems. These results support the practicability of this equation.” –p.2. “In the present work L is expressed by an exponential equation [J87] – Eq.(3)” –p.4. “..thedeviations between the calculation and experiment are very small. Besides, the miscibility gap at hightemperatures, as shown in Fig., was removed in the present work. This is an additional confirmation onthe reliability of the exponential equation” – p.6. “The present work shows that the exponential equationfor the excess Gibbs energy is very efficient to remove the artificial miscibility gap at hightemperatures. Besides, the calculated thermodynamic properties using exponential equation is is morereasonable than those due to the linear equation. It is recommended that the binary systems, which showartificial miscibility gap in the literature, should be checked and reassessed using the exponentialequation” – p.9. “.Conclusion: The exponential equation wa successfully used to describe the excessGibbs energy of both liquid and solid phases in Fe-Zn system …. The aritificial miscibility gap in theliquid phase at high temperatures was removed automatically using the exponential equation withoutapplying any thermodynamic constraints.” – p.9J87-c31. S.H.Sheng, R.F.Zhang, S.Veprek: Study of spinodal decomposition and formation of nc-Al 2 O 3 /ZrO 2nanocomposites by combined ab initio density functional theory and thermodynamic modeling – ActaMater, 2011, vol.59, pp.3498-3509. – „It will be shown that the exponential dependence, which hasbeen recommended by Kaptay [J87], yields the most reliable results” – p.3499, “Conclusions: … It hasbeen shown that using a linear temperasture dependence, or completely ignoring it, as found in manypublished papers, yields physically unsound results, because the calculated maximum spinodialtemperature is far above the melting point of the oxides. Therefore we focused on the thermodynamicmodeling using the exponential temperature dependence of the interaction parameter, as suggested byKaptay [J87].” – p.3508.J87-c32. Weng, LD; Li, WZ; Zuo, JG; Chen, C: Osmolality and Unfrozen Water Content of AqueousSolution of Dimethyl Sulfoxide - J Chem Eng Data, 2011, vol.56, pp. 3175-3182.J87-c33. S. Bajaj, A. Landa, P. Söderlind, P.E.A. Turchi, R. Arróyave: The U–Ti system: Strengths andweaknesses of the CALPHAD method - Journal of Nuclear Materials, 2011, vol.419, pp. 177-185 –„Additionally, the manifestation of such unrealistic phase stabilities could also be prevented byintroducing special phase stability constraints (ensuring positive curvature of the Gibbs energy curvesfor the bcc phase at high temperatures, for example) such as phase stability (QF), or phase driving force35

(DGM) functions in Thermo-Calc, or by employing Kaptay’s function for the excess Gibbs energy[J87]” – p.183.J87-c34. M.Schick, B.Hallstedt, A.Glensk, B.Grabowski, T.Hickel, M.Hampi, J.Göbner, J.Neugebauer, R.Schmid-Fetzer: Combined ab-initio, experimental and Calphad approach for an improvedthermodynamic evaluation of the Mg-Si system – Calphad, 2012, vol.37, pp.77-86. – „There have beennumerous attempts to model this system thermodynamically, but despite some success severe problemsand questions remain to be solved: all evaluations except … show inverted miscibility gaps in the liquidbelow 3000 K, which are physically wrong. To avoid this problem, Yuan et al. Used the Kaptayequation [J87] instead of a standard linear temperature dependence for the liquid interaction.” - p. 77,“In contrast to Yuan et al, who used the Kaptay equation [J87], the temperature dependence of theinteraction parameters is approximated bz standard linear function…. As mentioned in the introduction,the use of the Kaptaz euqation to model the temperature dependnece of the interaction parameteres inthe liquid can help to avoid inverted miscibilitz gaps at elevated temperatures, but maz also lead toartificial phase stabilities at low temperatures, as Schmid-Fetzer et al. have shown” - p.81, “The majorremaining issue concerns the enthalpy of melting of Mg 2 Si and, connected with that, the enthalpy of theeutectic reaction L = Mg 2 Si + Si (diamond). There is a large difference between our experimental data(also supported by independent data) and our optimization (see Table 5). Any attempt to force a betterfit led to large temperature dependences of the parameters for the interaction in the liquid (i.e. a largenegative excess entropy of mixing) causing an inverted liquid miscibility gap” – p.85. ((conclusion ofGK: Authors of this paper do not use my equation due to their mistaken hypothesis, although by the endof their paper they come to the point, when no other choice is left, except that spoiling theiroptimization. They selected spoiling their own paper but resist using my equation – no comment…))J87-c35. T.Abe, K.Ogawa, K.Hashimoto: Analysis of miscibility gaps based on the Redlich-Kister polynomialfor binary solutions – Calphad, 2012, vol.38, pp.161-167 - “Kaptay [J87] introduced the exponentialtemperature dependence into the R-K parameters ….. to suppress the LCP (lower critical point) at hightemperatures. However, it has been rarely used in the thermodynamic assessments.” – p.161J87-c36. Yiwen Lei, Ronglu Sun, Ying Tang, Wei Niu : Experimental and thermodynamic investigations into themicrostructure of laser clad Al-Si coatings on AZ91D alloys – Surf Coating Technol, 2012,http://dx.doi.org/10.1016/j.surfcoat.2012.07.032 - „Interaction parameters of the excess Gibbs energyfor the sublattice model are always presented using RK linear polynomial [X]. The formulation fortemperature dependent excess Gibbs energy of the sublattice model is based on the equation proposedby Kaptay [J87].”J86. G.Kaptay, T.Matsushita, K.Mukai, T.Ohuchi: On Different Modifications of theCapillary Model of Penetration of Inert Liquid Metals into Porous Refractories and theirConnection to the Pore Size Distribution of the Refractories – Metall. Mater. Trans. B, 2004,vol.35B, pp.471-486 (IF = 0.839)J86-c1. Bonadia P, Braulio MAL, Gallo JB, Pandolfelli VC: Refractory selection for long-distance moltenaluminumdelivery - AMERICAN CERAMIC SOCIETY BULLETIN 85 (8): AUG 2006 – “Kaptay etal [A67] propose a model to describe inert liquid metal penetration into porous refractories… (total 33lines + 4 equations + 1 figure describes the paper)” – p. 9303J86-c2. Kocaefe D, Ergin G, Kocaefe Y: Determining the wettability of granular alumina by aluminummagnesiumalloys using the infiltration method – Surf Interface Anal, 2008, vol. 40, pp. 1516-1522.J86-c3. Svidró József Tamás (konzulensek: Diószegi Attila és Tóth Levente): Transzportfolyamatok afém/formázóanyag határfelületén – PhD értekezés, Miskolci Egyetem, 2011 – „Emellett Kaptay [J86]leírta a „pre-penetráció” modelljét is, ami alatt a makroszkópikus penetrációhoz tartozó, küszöbnyomásalatti nyomáson fellépő viszonyleg kismértékű penetráót érti. Ehhez kidolgozta a „periodikusan változósugarú kapilláris” modellt (2.14 ábra), amely esetén ….. stb…” – pp.16-17.J85. G.Kaptay: Discussion of “Thermodynamics of Liquid Al-Na Alloys Determined byUsing CaF 2 Solid Electrolyte” published by S.G.Hansen, J.K.Tuset and G.M.Haarberg inMet.Mat.Trans.B, 2002, vol. 33B, 577-587 - Metall. Mater. Trans., 2004, vol.35B, pp.393-398 (IF = 0.839)36

J85-c1. S.G.Hansen, K.Tang: Thermodynamics of the Al-Na binary alloy – SINTEF report No.STF80MKA05211, 27 th Feb, 2006 – “Kaptay [J85] claimed that the negative deviation from Henry’s law found byHansen et al. was due to the reaction between Al vapour and NaF in the galvanic cell” – p.3. “Thisclearly indicates that the previous results are not reliable ..” – p.5.J85-c2. S.G.Hansen: The solubility of sodium in liquid aluminium – SINTEF Memo of 27 Febr, 2006 - “Kaptay[J85] claimed that the negative deviation from Henry’s law found by Hansen et al. was due to thereaction between Al vapour and NaF in the galvanic cell” – p.3. “None of the results obtained conformthe solubilities previously obtained by Hansen… ” – p.26.J85-c3. X.Yang, A.Jha, S.Ali, R.C.Cochrane: Mass-transport processes at the steel-enamel interface – MetallMater Trans B, 2006, vol.37B, pp.89-98 – “… the Marangoni convection, induced by an interfacialsurface tension gradient [J85] may promote mass transport across the interface and thereby engances therate of reactions” – p.89J85-c4. Zhang SJ, HAN QY, Liu ZK: Thermodynamic modeling of the Al-Mg-Na system – J. Alloys andCompounds, 2006, vol.419, pp.91-97 – “The controversal work of Hansen et al. was criticized byKaptay [J85]. According to thermodynamic calculation of of Kaptay there may be reactions betweenAl(g) and NaF(s). However, Hansen et al. stood by their results. …. Their (Hansen’s) results are notused in this work due to errors as discussed above” – p.92.J85-c5. Zi-Kui Liu, S.Zhang, Q.Han, V.Sikka: The effect of impurities on the processing of aluminum alloys –Penn State, final report, September 2006. – “The controversial work of Hansen et al was criticized byMotzfeldt [] and by Kaptay [J85]. Kaptay considered the reactions between Al(g) and NaF(s) to exist inHansen-s EMF experiments based on his thermodynamic calculations. But Hansen et al stood by theirresults” – p.17.J84. G.Kaptay: Interfacial criteria for stabilization of liquid foams by solid particles –Colloids and Surfaces, A: Physicochemical and Engineering Aspects, 2003 (OR 2004)vol.230, pp.67-80. (IF = 1.513)J84-c1. N.Babcsán, D.Leitlmeier, H.P.Degischer: Foamibility of Particle Reinforced Aluminum Melt – Mat.-wiss. u. Werkstofftech., 2003, vol.34, pp.1-8 – „Kaptay pointed out that wetting angle has to be in acertain range and particles stabilize the gas/liquid bubble interface. In the framework of a model,assuming single layer of particles between in the cell wall it was shown that the foam is stabilized onlyin the interval of’ the contact angles 10 – 90 degrees. However, when a presence of a double, or a’double+’ layer of particles is assumed to be in the cell wall, this interval increases to 10 - 129 degrees,or 10 – 170 degrees, accordingly [J84]”J84-c2. N.Babcsán: Ceramic Particle Stabilized Aluminum Foams – PhD Dissertation, Miskolc, 2003 – “In themiddle 90’s –thanks for H.P.Degischer, J.Banhart and G.Kaptay – science found a partnership with thischallenging material {metallic foam} and some basic question like stability of metal foams {has been}clarified” – p.12, “ “…when a presence of a double, or a double+ layer of particles is assumed to be inthe cell wall, this interval increases to 10-129 degrees, or 10-170 degrees, accordingly. Calculating theprobability function of foam stability optimum values was found for contact angle = 75, 87 and 89degrees in a single, double and double+ layers, respectively. No stabilizing effect can be seen below 30% surface coverage of bubbles by particles [J84]” – p.34. , “Kaptay [J84] predicted that the foamibilityof particle stabilized liquids strongly depends on the surface concentration of particles. This is thecase {for this work} for foams blown by Nitrogen gas, where the foam surface coverage was found tobe a segregated 40 % value (Fig.80 and Fig.81)” – p.81.J84-c3. N.Babcsán, J.Banhart, D.Leitlmeier: Metal foams - manufacture and physics of foaming - in: Proc. ofInt. Conf. „Advanced Metallic Materials”, ed. by J.Jerz, P.Sebo, M.Zemankova, IMMM, SlovakAcademy of Sciences, 2003, pp. 7-15 – „Kaptay pointed out that the wetting angle has to be in a certainrange and particles stabilize the gas/liquid-bubble interface [J84]” – p.9., „It is common believe that thecomposition of the particles determines the stabilizing effect through the contact angle with the melt[J84]”, p.12.J84-c4. T.Wübben: Zur Stabilität flüssiger Metallschaume – Universität Bremen, Germany, 2003, 128 pp. - „Indiesem Zusammenhang wird das schon erwähnte Stabilisierungsmodell von G.Kaptay ausführlicherläutert und kritisch diskutiert” – p.2, „In diesem Kontext hat Kaptay [J84] ein mechanistisches Modellentwickelt, das sowohl den Einfluss der Partikelkonzentration als auch des Kontaktwinkels auf dieStabilität von Metallshaumen beschreibt. Diese Arbeit beschäftigt sich in groSen Teilen mit derUntersuchung der Gültigkeit dieses Modells. Es soll daher folgenden im Detail erläutert werden” –p.30. „Mit Ausnahme von Kaptay in [J84] geben jedoch alle Autoren nur phänomenologischeErklärungen. Die in erstmals angedeutete Hypothese wurde unter Berücksichtigung der im Rahmendieser Arbeit gewonnenen experimentellen Ergebnisse weiterentwickelt, so daS es quantitativeAussagen über die Wirksamkeit von Partikeln in Metallschaumen möglich mach [J84]” – p.31. „Der37

optimale Kontaktwinkel ist gemaS [J84] der, bei dem der Ausdruck ...(3.17) ... sein Maximum erreicht.”– p.34, „Ein weitaus entscheidenderer Kritikpunkt speziell an den quantitativen Berechnungen in [J84]ist jedoch die Annahme, das eine über die gesamte Porenoberflauche gemittelte belegungsdichte f zurberechnungvon p imm,max herangezogen werden kann, selbst dann, wenn f deutlich kleiner als 1 ist” –p.38.J84-c5. N.Babcsán, D.Leitlmeier, H.P.Degischer, H.J.Flankl: Particle stabilised liquid aluminium foams and therole of the oxide skin - in: “Cellular Metals: Manufacture, Properties, Application”, ed. by J.Banhart,N.A.Fleck, A.Mortensen, MIT Verlag, 2003, pp.101-106: “The particles can be characterized by …their wetting [J84]..”, p.101, “in Table 2: Differences and similarities in stabilization mechanism ofliquid foam. Metallic foam: surface active agent (60-90 o contact angle) [J84]” – p.105.RJ84-c6. R.G.Alargova, D.S.Warhadpande, V.N.Paunov, O.D.Velev: Foam superstabilization by polymermicrorods – Langmuir, 2004, vol.20, pp.10371-10374. (Ref. No.8). – “Data and theoretical conclusionsin the literature point out that hydrophobic spherical particles may initiate foam destruction by rupturingthe foam films via a bridging-dewetting mechanism [J84].” – p. 10371.J84-c7. N.Babcsán, D.Leitlmeier, H.P.Degischer, J.Banhart: The role of oxidation in blowing particle-stabilizedaluminium foams – Advanced Engineering Materials, 2004, vol.6, pp.421-428 – „The various factorsinfluencing metallic foam stability ... the effect of particles ... wetting behavior [J84]” – p. 421,“Suitable particles (60-90 o contact angle [J84]) …. are necessary for obtaining a stable liquidaluminium foam” – p.427.J84-c8. V.Gergely, T.W.Clyne: Drainage in standing liquid metal foams: modelling and experimentalobservations - Acta materiala, 2004, vol.52, pp.3047-3058: „Interfacial criteria for stabilization ofmetallic foams by solid particles have recently been derived by Kaptay [J84]” – p.3053J84-c9. B.S.Murray, R.Ettelaie: Foam stabilty: proteins and nanoparticles – Current Opinion in Colloid &Interface Science, 2004, vol.9, pp.314-320 – „Other criteria for stability of particle-stabilized bubbleswere recently derived by Kaptay [J84]. The theoretical arguments presented in this work indicate theexistence of a maximum size (about 3 m for bubbles in water) above which particles are not effectivein prevention of coalescence.” – p.317.J84-c10. Brunke O, Odenbach S, Beckmann F: Structural characterization of aluminium foams by means microcomputed tomography – in: DEVELOPMENTS IN X-RAY TOMOGRAPHY IV Book Series:PROCEEDINGS OF THE SOCIETY OF PHOTO-OPTICAL INSTRUMENTATION ENGINEERS(SPIE), ed. by Bonse U, 2004, vol. 5535, pp. 453-463.J84-c11. Th.Wübben, S.Odenbach: On the stabilization mechanism in liquid metallic foams – PAMM (ProcAppl Math Mech), 2004, vol.4, pp.270-270 – “While some authors attribute the stability to theincreased viscosity due to solid particles that are presdent in the melt, there has also been evidence for astabilizing mechanism based on the wetting properties of solid substances [J84]” – p.270, “…the resultsgive strong evidence for the importance of interface related effects as has been postulated before [J84].According to this assumption, particles act against coalescence of pores in the liquid foam, possibly bythe mechanism described in [J84]” – p.271.J84-c12. N.Babcsán, J.Banhart, D.Leitlmeier: Metal foam – manufacture and physics of foam – Materials World,e-journal, 2005, vol.6, No.1 – “Kaptay pointed out that the wetting angle has to be in a certain range andparticles stabilize the gas/liquid-bubble interface [J84] – p.7,J84-c13. C.Körner, M.Arnold, R.F.Singer: Metal foam stabilization by oxide network particles – Mater. Sci.Eng., 2005, vol.A396, pp.28-40.: “Further progress to explain foam stability was made by Kaptay [J84].He uses a model of a 3D network of solid, spherical particles to explain force transfer between twointerfaces and in this way stability” – p.28.; .J84-c14. N.Babcsán, D.Leitlmeier, J.Banhart: metal foams – high temperature colloids. Part I. Ex situ analysis ofmetal foams – Colloids and Surfaces A, 2005, vol.261, pp.123- 130 – “Kaptay pointed out that thewetting angle has to be in a certain range and particles stabilize the gas/liquid-bubble interface [J84]” –p.125.J84-c15. P.M.Kruglyakov, A.V.Nushtayeva: Investigation of the influence of capillary pressure on stability of athin layer emulsion stabilized by solid particles – Colloids and Surfaces, A: Physicochem. Eng. Aspects,2005, vol.263, pp.330-335 – “Calculation of interfacial pressure separating two bubbles (drops) byparticles was given by Kaptay [J84] also, but this pressure is not equal to the capillary pressure andtherefore the stability criteria of Kaptay displays an inconsistency” – p.330.J84-c16. S-H.Park, Y-S.Um, C-H. Kum, B-Y. Hur: Thermophysical properties of Al and Mg alloys for metalfoam fabrication - Colloids and Surfaces, A: Physicochem. Eng. Aspects, 2005, vol.263, pp.280-283 -“Of-course, in the actual foaming process, the appearance of the rheological characteristics are verymuch influenced from the existing of particles [J84]” – p.280J84-c17. Th.Wübben, S.Odenbach: Stabilization of liquid metallic foams by solid particles – Colloids SurfacesA., 2005, vol.266, pp.207-213: “The stabilization model for liquid foams by solid particles is described38

in details in [J84]. We thus only give a short outline of the basics of this model” – p.207, “1 page ofdescription twice mentioning “Kaptay model”” – p.208. “It should be pointed out that the model ofKaptay does not take into account drainage and flow effects. We therefore carried out experimentsunder reduced gravity conditions” – p.209., “According to the discussion above, we thus have tomeasure the surface of the pores rather than the size of the pores to have a quantitative test of thevalidity of the model proposed by Kaptay” – p.210., “To investigate the validity of the model proposedby Kaptay [J84] we carried out experiments with two different lead powders” – p.210., “According tothe model of Kaptay, the total pore surface of a foam depend on the amount of particles present for filmstabilization” – p.211, “5. Comparison with the stabilization model by Kaptay. To compare the obtainedresults with the model proposed by Kaptay we come back to the assumption that the solid particlesoriginate from the broken oxide skins of the powder grains” – p.212, “The obtained results stronglysupport the validity of the model proposed by Kaptay [J84]” – p.213.J84-c18. A.Irretier, J.Banhart: Lead and lead alloy foams – Acta Mater., 2005, vol.53, pp.4903-4917 – “A certainoxide content is necessary to ensure foam stability… It is well known that metal foams are stabilized bysolid particles floating in the melt… Wübben could recently show [J84-c4] that the ratio between thetotal internal pore surface of a lead foam is proportional to the volume content of the entrained oxideand concluded that the oxides float on the foam films during foaming and create stabilization by a stilldisputed mechanism [J84]” – p. 4914J84-c19. N.Babcsán, F.Garcia-Moreno, D.Leitlmeier, J.Banhart: Liquid-metal foams – feasible in-situexperiments under low gravity – Materials Science Forum, 2006, vol.508, pp.275-280: “Phenomenarelated with aqueous foam stability are detailedly discussed in the literature in large monographs, butonly few publications relate to metal foams [J84]” – p.275J84-c20. Kostakis T, Ettelaie R, Murray BS: Effect of high salt concentrations on the stabilization of bubbles bysilica particles - LANGMUIR 22 (3): 1273-1280 JAN 31 2006 – “In addition, theoretical work fromKaptay [J84] postulated that solid particles can stabilize bubbles only when the bubbles are not largerthan 3 and 30 m” – p.1274J84-21. Asavavisithchai S, Kennedy AR: The effect of Mg addition on the stability of Al-Al 2 O 3 foams made by apowder metallurgy route - SCRIPTA MATERIALIA 54 (7): 1331-1334 APR 2006 – “it is generallyconsidered that particles which show good wetting with the liquid will improve the stabiulity of thefoam [J84]” – p.1331.J84-22. Park SH, Song KH, Um YS, Hur BY: Rheological characterization of Mg-Al alloys with ceramicparticles for metal foam – Mater Sci Forum, 2006, vol.510-511, pp.742-745. “no text given…”J84-c23. Gonzenbach UT, Studart AR, Tervoort E, Gauckler LJ: Ultrastable particle-stabilized foams -ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 45 (21): 3526-3530 2006 - “.. modelinvestigations in the absence of surfactants performed [J84]” – p.3526.J84-c24. Friberg SE: Weight fractions in three-phase emulsions with an L-alpha phase - COLLOIDS ANDSURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS 282: 369-376 JUL 20 2006 –“Emulsions with solid particles as the third phase have been investigated for a long time and have, aftera long period of only intermittent contributions, recently been the object of intense fundamentalresearch [J84]” – p.369.J84-c25. N.Babcsán, J.Banhart: Metal Foams – towards high-temperature colloid chemistry – Chapter 11 in:„Colloidal particles at Liquid Interfaces, ed. By B.P.Binks, T.S.Horozov, Cambridge University Press,2006, pp.445-499 – „Using a static model of a 3-D network of solid spherical particles he (Kaptay)attempted to explain the force transfer between two interfaces of a foam and in this way the stability viaa disjoining pressure [J84]. Various configurations of particles were considered in these models, ofwhich three are shown in Fig.11.7. ((Fig.11.7 copied with permission of Elsevier)). The basic idea isthat a partially wetted particle is pinned to a surface since it has its lowest energy when immersed intothe liquid at a given depth....+ 10 lines description” – pp.461-462. “...It ias not evident from the imageshow mechanical forces can be transmitted from one side of a film to the other via particle networks aspostulated, e.g. by Kaptay [J84], which would be required to create a disjoining force. There are twoexplanations for these difficulties. Firstly, the 2-D character of metallographic analysis could obscurethe structure of the posztulated 3-D betworks. Secondly, it is not guaranteed that the arrangement ofoarticles in solid foams is identical to that in liquid foams…” – p.489. „It is timely to give aninterpretation in terms of models such as the LP2+C model by Kaptay (see Fig.11.7.c). Accordingly, theparticles are pinned to each of the interfaces of a film by means of interfacial forces. This would explainmicrographs such as Fig.11.a. However, it is not clear how the attractive interactions between the twointerfaces are balanced. Kaptay postulates that mechanical forces are responsible for this counterpressure, the disjoining pressure, which in his model are transferred through locally densely packedlayers of particles. Experimental evidence, however, does not support the existence of such bridgesbetween the two surface layers.” – p.492. .. „Körner et al. assume that these meta-particles astabilise the39

cell walls by forming an LP1 layer in Kaptay-s notation. The idea sounds convincing, but is based onvery few and mostly indirect observations” – p.493.J84-c26. Shrestha LK, Acharya DP, Sharma SC, Aramaki K, Asaoka H, Ihara K, Tsunehiro T, Kunieda H:Aqueous foam stabilized by dispersed surfactant solid and lamellar liquid crystalline phase -JOURNAL OF COLLOID AND INTERFACE SCIENCE 301 (1): 274-281 SEP 1 2006 – Manyreports on foam and emulsion stabilized by the small solid particles are available [J84].” – p.275, „Themain factor responsible for the foam stability is the presence of colloidally dispersed particles int hecontinuous medium, which slow down the liquid drainage rate due to increased surface viscosity of thecontinuous phase [J84]…. Kaptay [J84] demonstrated enhanced stability in water based foam by silicaparticles smaller than 3 microns.” – p.280.J84-c27. Shrestha LK, Aramaki K, Kato H, Takase Y, Kunieda H: Foaming properties of monoglycerol fattyacid esters in nonpolar oil systems - LANGMUIR 22 (20): 8337-8345 SEP 26 2006 - – „.. the stabilityof foams is influenced by particle size, concentration, hydrphobicity and nature of the surfactant used[J84].” – p.8338, „Kaptay [J84] demonstrated the enhanced stability in a water based foam by silicaparticles < 3 micron in size” – p.8344.J84-c28. Haibel A, Rack A, Banhart J: Why are metal foams stable? - APPLIED PHYSICS LETTERS 89 (15):Art. No. 154102 OCT 9 2006 – „An idea which has recently become popular in metal foam literatureassumes that opposing partciloe-covered L/G interfaces are mechanically connected by particle bridgesacross films (Fig.1.d [J84]) – p.1, „Our analysis shows that particles do not interact accross liquid metalfilms, e.g., there is no analog to the „disjoining pressure” known to stabilize aqueous foams as claimedby several researchers [J84].” – p.3.J84-c29. J. Banhart: Metal foams: production and stability – Adv. Eng Mater., 2006, vol.8, pp.781-794 –“Kaptay analysed a number of possible particle arrangements in a film and evaluated their capability tostabilise films [J84]. Some are shown in Fig.8.. + ((17 describing lines + Fig.8))” - pp.785-786.J84-c30. J.Banhart: Metal foams: the mystery of stabilisation – in: Porous Metals and Metal FoamingTechnology, eds. H.Nakajima, N.Kanetake, the Japanese Inst. of Metals, 2006, pp.75-86 - “Kaptayanalysed a number of possible particle arrangements in a film and evaluated their capability to stabilisefilms [J84]. Some are shown in Fig.8.. + ((17 describing lines + Fig.8))” - p.79.J84-c31. C.Körner: Integral Foam Molding of Light Metals – Physical and Technological Principles –Habilitation Thesis, Erlangen, 2006 – “Kaptay was the first who realized that stabilization for these kindof particles is based on the development of 3D network structures which transfer forces from oneinterface to the other [J84].” – p.108.J84-c32. E.Dickinson: Interfacial particles in food emulsions and foams – in: Colloidal Particles at LiquidInterfaces, edited by B.P.Binks and T.S.Horozov, Cambridge University Press, 2006, pp.298-327 – Theapplication of underlying principles [J84] to these systems is, however, still somewhat limited” – p.321.J84-c33. Kunieda H, Shrestha LK, Acharya DP, Kato H, Takase Y, Gutierrez JM: Super-stable nonaqueousfoams in diglycerol fatty acid esters - Non polar oil systems - JOURNAL OF DISPERSION SCIENCEAND TECHNOLOGY 28 (1): 133-142 JAN 2007 – „Recently, interest has been focused ont he foamsstabilized by the solid particles whose presence may promote or inhibit foam stability [J84]” – p.134.J84-c34. Shrestha LK, Saito E, Shrestha RG, Kato H, Takase Y, Aramaki K: Foam stabilized by dispersedsurfactant solid and lamellar liquid crystal in aqueous systems of diglycerol fatty acid esters -COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS 293 (1-3):262-271 FEB 1 2007 – “Many reports on foam and emulsion stabilized by the samll solid particles areavailable [J84].” – p.263, “Kaptay [J84] used silica particles smaller than 3 microns and demonstratedthe enhanced stability in water-based foams” – p.270.J84-c35. N.Babcsán, G.S. Vinod Kumar, B.S.Murty, J.Banhart: Grain refiners as liquid foam stabilizers – Trans.Indian Inst. Met., 2007, vol.60, pp.127-132. – „Kaptay derived a stability range of 60-90 o [J84]” –p.127.J84-c36. Yu SR, Liu J, Luo YR, Liu YH: Compressive behavior and damping property of ZA22/SiCp compositefoams - MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALSPROPERTIES MICROSTRUCTURE AND PROCESSING 457 (1-2): 325-328 MAY 25 2007 – “ ..ceramic particles … stabilized the cell walls [J84]” – p.325.J84-c37. Shrestha LK, Shrestha RG, Solans C, Aramaki K: Effect of water on foaming properties of diglycerolfatty acid ester-oil systems - LANGMUIR 23 (13): 6918-6926 JUN 19 2007 – “The stability of suchfoams was influenced by the size of the particle, concentration, hydrophobicity, and nature of thesurfactant used [J84]” – p.6918. “Several reports on the foams stabilized by particles having size of afew microns are reported [J84]” – p.6926J84-c38. Pugh RJ: Foaming in chemical surfactant free aqueous dispersions of anatase (Titanium dioxide)particles - LANGMUIR 23 (15): 7972-7980 JUL 17 2007 – “An alternative mechanism has been40

suggested which is based on a change in capillary pressure caused by the presence of small adsorbedparticles [J84]” – p.7978.J84-c39. Blute I, Pugh RJ, van de Pas J, Callaghan I: Silica nanoparticle sols 1. Surface chemicalcharacterization and evaluation of the foam generation (foamability) - JOURNAL OF COLLOID ANDINTERFACE SCIENCE 313 (2): 645-655 SEP 15 2007 – “It is also important to consider a recentalternative mechanism that has been suggested. It is based on a change in capillary pressure caused bythe presence of adsorbed particles [J84]. – pp.651-652.J84-c40. Somosvari BM, Babcsan N, Barczy P, Berthold A: PVC particles stabilized water-ethanol compoundfoams - COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS309 (1-3): 240-245 NOV 1 2007 – “Kaptay [J84] postulates that the maximum particle size that canstabilize liquid films depends on the liquid properties. For water 3 micron and for liquid metals 30micron were calculated. He also could derive theoretically, the optimum contact angles, measured bythe researchers” – p.240.J84-c41. Kim, HG Seong, BY Hur: Characteristics of Al fopam with high porosity by melt foaming method –Solid State Phenomena, 2007, vol.124-126, pp.1801-1804 – “In the melt formaing process that employsthe addition of TiH 2 in pure aluminium melt, pores generated leave individual hydrides and enter intothe pure molten aluminium due partly to buoyancy forces and due partly to the thermodynamicinstability of systems with enhanced liquid/gas interfaces [J84].” – p.1801.J84-c42. Kadoi K, Nakae H: Effect of particle addition to liquid metal on fabrication of aluminum foam - HIGHTEMPERATURE MATERIALS AND PROCESSES 26 (4): 275-283 2007 – “Some other models,similar to… were proposed… by Kaptay [J84], using an interfacial model” – p. 277.J84-c43. Gokhale AA, Sahu SN, Kulkarni VKWR, Sudhakar B, Rao NR: Effect of titanium hydride powdercharacteristics and aluminium alloy composition on foaming - HIGH TEMPERATURE MATERIALSAND PROCESSES 26 (4): 247-256 2007 – “The above results should be analyzed in light of the foamstability mechanism proposed by Kaptay [J84]. The mechanism …. {21 lines describing my paper + 1equation}” – p.255.J84-c44. Beckmann F, Grupp R, Haibel A, Huppmann M, Noethe M, Pyzalla A, Reimers W, Schreyer A, ZettlerR: In-situ synchrotron X-ray microtomography studies of microstructure and damage evolution inengineering materials - ADVANCED ENGINEERING MATERIALS 9 (11): 939-950 NOV 2007J84-c45. Orbulov I., Kientzl I., Németh Á.: Fémhabok és kompozitok előállítása infiltrálásos eljárással – BKLKohászat, 2007, vol.140, No.5, pp.41-46. – „A másik csoportba sorolhatjuk azokat az anyagokat,amelyek létrehozásánál vagy csak a tömegcsökkentés, vagy valamilyen más különleges követelménydominál. Ezek a porózus szerkezeti anyagok [J84]” – p.41.J84-c46. U.T.Gozenbach, A.R.Studart, E.Tervoort, L.J.Gauckler: Tailoring the microstructure of particlestabilizedwet foams – Langmuir, 2007, vol.23, pp.1025-1032 – „These results suggest that thepreparation of wet foams that are stable against bubble coarsening and drainage requires particle sizesnot larger than a few micrometers in diameter. Theoretical calculations based ont he adsoroption energyof particles at gas – liquid interface and the maximum capillary pressure developed at the interfaceshowed that particles larger than about 3 microns are not able to stabilize foams for long period of time[J84]. These results are in the same order of magnitude as our experimental findings” – p.1029.J84-c47. H Luo, G Yao, YH Liu, XM Zhang: Study on evolution behaviours of bubble in aluminium melt -Aluminium alloys for transport, packaging, aerospace and other applications, 2007, pp.73-80.J84-c48. Z.Cao, G Yao, Y Liu: Fabrication of carbon fibers reinforced aluminium foam – Aluminium alloys fortransport, packaging, aerospace and other applications, 2007, pp.25-32J84-c49. Kostakis T, Ettelaie R, Murray BS: Enhancement of stability of bubbles to disproportionation usinghydrophilic silica particles mixed with surfactants or proteins – in: Food Colloids: Self-Assembly andMaterial Science, ed. by Dickinson E; Leser ME, Book Series: ROYAL SOCIETY OF CHEMISTRYSPECIAL PUBLICATIONS, 2007, vol. 302, pp. 357-368. – „In addition, theoretical work by Kaptay[J84] postulated that solid particles can stabilize bubbles only when the particles are not larger than 3-30 microns” – p.358J84-c50. Unterhaslberger G, Schmitt C, Shojaei-Rami S, Sanchez C: beta-lactoglobulin aggregates from heatingwith charged cosolutes: Formation, characterization and foaming – in: : Food Colloids: Self-Assemblyand Material Science, ed. by Dickinson E; Leser ME, Book Series: ROYAL SOCIETY OFCHEMISTRY SPECIAL PUBLICATIONS, 2007, vol.302, pp. 177-194. – recently, the use of silica orlatex particles with different surface properties and degree of hydrophobicity was demonstrated tostabilize interfacial films against disproportionation [J84]” – p.178.J84-c51. S.Zhang, Q.Lan, Q.Liu, J.Xu, D.Sun: Aqueous foams stabilized by Laponite and CTAB – ColloidsSurfaces A, 2008, vol.317, pp.406-413 – “The hydrphobicity of particles is generally described bycontact angle. It is an important parameter in determining … the foam stability [J84].” – p.408.41

J84-c52. TN Hunter, RJ Pugh, GV Franks, GJ Jameson: The role of particles in stabilizing foams and emulsions– Adv. Colloid Interface Sci., 2008, vol.137. pp.57-81 – “.. it is possible to calculate a theoreticalmaximum capillary pressure sustainable by a given system….Ivanov and co-workers were the first toconsider such a system [ ], and models have been further developed by others including Nushtaeva &Kruglyakov [] and Kaptay [J84].” – p.62, “Kaptay looked at general forces governing stability in foams[J84]…. + 15 lines of description” – p.75, “Another factor in equating the dominating stabilityinteraction from particle addition Is the effects of particle size. First considered in line with volumefraction by Jin et al [], and as revised by Kaptay [J84], there ares osme well grounded conclusions. + 4lines” – p.78.J84-c53. Ho PW, Li QF, Fuh JYH: Evaluation of W-Cu metal matrix composites produced by powder injectionmolding and liquid infiltration – Mater Sci Eng A, 2008, vol. 485, pp. 657-663 – „The interfacial forceacting upwards on spherical particle at a liquid/gas interface has been derived to be [J84]… (Eq.1). –see Fig.12” – p.661.J84-c54. Cao ZK, Li B, Yao GC, Wang Y: Fabrication of aluminum foam stabilized by copper-coated carbonfibers – Mater Sci Eng A, 2008, vol.486, pp.350-356 – „Kaptay evaulated the capability of six differentdefined structures which can in principle stabilize liquid foams, and concluded that loosely packed,clusthered particles, or even their network are mainly responsible for the stabilization of liquid foams[J84]” – p.350.J84-c55. S.Zhang, D.Sun, X.Dong, C.Li, J.Xu: Aqueous foams stabilized with particles and ionic surfactants –Coll Surf A, 2008, vol.324, pp.1-8 – „The stabilization mechanisms are mainly from three aspects: …and changes in capillary pressure caused by the presence of small adsorbed particles [J84]” – p.1, „.. theparticles form a steric layer or coating network that strongly hinders both shrinkage and expansion ofthe bubbles. The three-dimensional network has been suggested in some work [J84]” – p.4J84-c56. T.S. Horozov: Foams and foam films stabilised by solid particles - Curr Opinion in Colloid InterfaceSci, 2008, vol.13, pp.134-140. – „Several recent works [J84, etc.] treat the problem of liquid filmstability by solid particles theoretically, assuming either a bridging monolayer or a bilayer ofhexagonally close-packed particles.” – p.137.J84-c57. M.Vignes-Adler: New foams: fresh challenges and opportunities – Curr Opinion in Colloid InterfaceSci, 2008, vol.13, pp.141-149. – „On the theoretical side, Kaptay derived criteria for stabilization ofaqueous foams by solid particles based on the film pressure and the particle size for several geometricalarrangements of the particles inside of the foam films [J84].” – p.149.J84-c58. S Ata: Coalescence of bubbles covered by particles – Langmuir, 2008, vol.24, pp.6085-6091. - „Themechanism of film stabilisation has been explained by the capillary pressure between bubbles, given by{equation}. The theory was first proposed by Ivanov and co-workers and developed further by others[J84]” – p.6086-6087. “Recently, Kaptay [J84] extended the maximum capillary theory for variousparticle layers at the air-water interface. The optimum value of the contact angle for foam stabilizationwas found to be in the interval between 50 o and 90 o . Interestingly, his calculation showed that, to stabilizethe thin films, the particles should be smaller than 3 microns, which is contradictory to the previousstudies” – p.6086.J84-c59. Y.Luo, S.Yu, W.Li, J.Liu, M.Wei: Compressive behavior of SiC(p)/AlSi9Mg composite foams – J.Alloys Compds, 2008, vol.460, pp.294-298 – To stabilize the preparing process … ceramic particleswere added into metallic foams to form metal matrix composite foams [J84]” – p.294.J84-c60. S.Yu, Y.Luo, J.Liu: Effects of strain rate and SiC particle on the compressive property ofSiC(p)/AlSi9Mg composite foams – Mater Sci Eng A, 2008, vol.487, pp.394-399 – “Recently, there is ahigh interest in using lightweight metallic foams for automotive, railway and aerospace industries forweight reduction and good mechanical and damping capacity [J84]” – p.394.J84-c61. R.J.Davenport, R.L.Pickering, A.K.Goodhead, T.P.Curtis: A universal threshold concept forhydrophobic mycolata in activated sludge foaming – Water Research, 2008, vol.42, p.3446-3454. – It isaccepted that solid particles with hydrophobic properties can lead to stable permanent foams calledthree-phase foams [J84]. – p.3446.42

J84-c62. C.Körner: Foam formation mechanism in particle suspensions applied to metallic foams – Mater SciEng A, 2008, vol.495, pp.227-235 – “Further progress to explain foam stability was made by Kaptay[J84] who uses a model of a three-dimensional network of solid, spherical particles to explain forcetransfer between two interfaces and in this way stability” – p.228.J84-c63. A.J.Klinter, G. Mendoza-Suarez, R.A.L.Drew: Wetting of pure aluminum and selected alloys onpolycrystalline alumina and sapphire – Mater Sci Eng A, 2008, vol.495, pp.147-152. – “Recently, it hasbeen found that the wetting behavior in metal-ceramic systems seems to play an important role in theproduction of aluminum foams [J84].” – p.147. “In theoretical models of Kaptay [J84], the stabilizingeffect of these particles on the liquid aluminum foam is credited to capillary effects between the meltand the particles, preventing the two liquid gas interfaces of a foam cell wall from touching and the twoadjacent cells from coalescence” – p.148.J84-c64. A.J.Klinter, R.A.L.Drew: Evaluation of the wetting behaviour of Al-7Cu and Al-11.5Si on SiC andsapphire in terms of Al-foam stability. In: METFOAM-2007, ed. by L.P.Lefebre, J.Banhart,D.C.Dunand, DEStech Publ. Inc, 2008, pp.23-26. – „During the early stages of Al-foam rersearch, itwas found that alumina or SiC particles are essential in order to obtain stable aluminium foams.Originally it was believed that the stabilizing effect of these ceramic particles have on Al-foams wascaused by an increase in bulk viscosity of the Al melt due to ceramic particles additions. In a verytheoreticla approach, KAPTAY [J84] later developed models suggesting that the improved foamstability was due to capillary effects between the melt and the particles, preventing the two liquid gasinterfaces of a foam cell wall from touching, and the two adjacent cells from coalescencing.” – p.23.J84-c65. K.Kadoi, N.Babcsán, H.Nakae, F.Garcia-Moreno, J.Banhart: Methodology for the in-situ obsrevation ofAlporas foams using X-ray radioscopy. In: METFOAM-2007, ed. by L.P.Lefebre, J.Banhart,D.C.Dunand, DEStech Publ. Inc, 2008, pp.111-114. – „The final structure is influenced by the stabilityof liquid metal and the processing parameters [J84]” – p. 111.J84-c66. A.Dudka, F.Garcia-Moreno, N.Wanderka, J.Banhart: Structure and distribution of oxides in aluminiumfoam – Acta Mater, 2008, vol.56, pp.3990-4001. – „Two theories are mainly considered: i) the increaseof local viscosity to an extent that the flow of liquid is blocked, and ii). stabilization of films throughoxide agglomerations or networks acting as surface active particles and inducing a particle-basedstabilization mechanism similar to the one proposed for other foaming routes [J84]” – p.3990.J84-c67. G.Morris, M.R.Pursell, S.J.Neethling, J.J.Cillers: The effect of particle hydrophobicity, separationdistance and packing patterns ont he stability of a thin film – J Coll Interface Sci, 2008, vol.327,pp.138-144. – „Kaptay [J84] also investigated the effect of attached particles stabilizing a film andshowed that if two layers of particles are attached to opposite sides of the film they can stabilise it atcontact angle above 90 deg” – p. 139, “If there are two or more layers of particles layers of particlesthey can stabilize a film above a contact angle of 90 deg, as demonstrated by Kaptay [J84]” – p.139.J84-c68. L.K.Shrestha, R.G.Shrestha, S.C.Sharma, K.Aramaki: Stabilization of nonaqueous foam with lamellarliquid crystal particles in diglycerol monolaurate/olive oil system – J Colloid Interface Sci, 2008,vol.328, pp.172-179 – “The stability of foams is influnced by the particle size, concentration,hydrophobicity and also by nature of the surfactants [J84].” – p.172, „In the case of particle-stabilizedfoaming systems, foam stability depends ont he tendency of the particles to adsorb at gas-liquidinterface, its shape and size. Silica or polymer latex particles are known to stabilize aqueous foams[J84]” – p.178.J84-c69. C.Koerner: Integral Foam Molding of Light Metals – Springer, 2008, 224 pp. – „ Kaptay [J84] was thefirst who realized, that stabilization for this kind of particles is based on the development of 3D networkstructures which transfer forces from one interface to the other” – p. 100.J84-c70. L.Pilon: Aluminum microfoams for reduced fuel consumption and pollutant emissions of transportationsystems – University of California Energy Institute, Energy Development and Technology 013, ProjectReport, July 2008, Berkeley, 29 pp. – „Some oxide particles are formed and stabilize the bubbles asobserved with other types of the particles (Kaptay, 2003)” – p.21.J84-c71. M.Y.Jung, K.Y.Lee, J.W.Moon: Properties of froth and foam ont he seawater and inorganic saltsolution – Korean journal, 2008, vol.45, No.5, pp.474-483. „…. Kaptay 2003…” – p.476, 480J84-c72. Konno Y., Naito N., Horie W., Aramaki K.: Phase Behavior and Froth Stability in aWater/Lysophospholipid System – J. Oleo Sci, 2009, vol. 58, No.4, pp. 195-201 – „The stability of frothswas influenced by the size of the particle, concentration, hydrophobicity, and nature of surfactant used[J84]” – p.196.J84-c73. A.J.Klinter, C.A.Leon-Patino, R.A.L. Drew: The optimum contact angle range for metal foamstabilization: an experimental evaluation of theory – Abstract book of 6th HTC conference, 6-9 May,2009, Athens, Greece, p.75 – „From the measured values, contact angle vs. Temperature curves weregenerated, some of which satisfy the contact angle requirement between liquid metal and ceramic particlesfor optimum metal foam stabilization proposed by Kaptay (70 to 86 degrees) [J84]. …. Comparing the43

experimentally observed liquid foam stability and the resulting foam morphology with the obtainedcontact angle vs. Temperature curves allows an evaluation of Kaptay’s theooretically derivedrequirements for optimum foam stabilization by ceramic particles [J84]” – p.75.J84-c74. R.Surace, L.A.C.De Filippis, E.Niini, A.D.Ludovico, J.Orkas: Morphological investigation of foamedaluminum parts produced by melt gas injection – Adv Mater Sci Eng, 2009, Article number: 506024 „Theceramic particles trap gas bubbles owing to the favourable interface energy and serve as stabilizer of thecell wals and delay their coalescence [J84]” – p.1.J84-c75. R.Surace, S.Bruno, L.A.C.De Filippis, A.D.Ludovico: Multi-objective optimization of Al-foammanufacturing parameters – Int J Simul Modelling, 2009, vol.8, No.2, pp.81-89.J84-c76. J.C.H. Wong, E.Tervoort, S.Busano, U.T. Gozenbach, A.R. Studart, P. Ermanni, L.J. Gauckler:Macroporous polymers from particle-stabilized foams - J Mater Chem, 2009, vol.19, pp. 5129-5133J84-c77. A. Britan, M. Liverts, G. Ben-Dor: Drainage and attenuation capacity of particulate aqueous foams. In:Shock Waves (book), ed. by K.Hannemann and F. Seiler, Springer Berlin Heidelberg, 2009, pp. 1395-1400, DOI: 10.1007/978-3-540-85181-3.J84-c78. A.V. Byakova, A. I. Sirko, S. V. Gnyloskurenko, T. Nakamura: Aluminium foam formation frompowder compacts with calcium carbonate: In situ experiments – PPT file, presented at Metfoam 2009conference, September 1-4, 2009, Bratislava, Slovakia – „Model originally proposed by Kaptay”J84-c79. A.V.Biakova, V.P.Krasovskii, A.O.Dudnik, S.V.Gniloskurenko, A.I.Sirko: O roli smachivaemosti Iraspredeleniia tviordich chastic v stabilizacii vspenennich aliuminievich rasplavov – Adgeziia rasplavovI paika materialov, 2009, vip.42, pp.5-22. – „Fundamentalnimi teoreticheskimi issleovaniiami bilopokazano [J84]….” – p.7. „razmer tviordich vlkuchenni ne dolzhen previshat 30 mikrometrov [J84]” –p.8. „resultati nastoiashego issledovaniia daiut osnovanie polagat, shto razlichiia v stabilnosti vkarbonatnoi i gidridnoi peni mogut naiti svoio obiasnenie v ramkach modelnich predstavlenii [J84] + 25strok” – p.16. „Fig.5. Schematic presentation of the cell wall structure of carbonate and hydride titanfoams as compared with model configurations [J84]” – p.17.J84-c80. D.Li, J.Li, X.Zhang, T.Sun, G.Yao: Wetting behaviour of Al alloys on a TiH2 substrate – J AlloysComps, 2010, vol.489, pp.L1-L3. – „In theoretical models by Kaptay [J84], the stabilizing effects ofthese particles on the liquid aluminium foam is due to capillary effects between the melt and theparticles and this prevents the two liquid gas interfaces in a foam cell wall from touching and the twoadjacent cells from coalescing” – p.L1.J84-c81. R.G.Screstha, L.K.Shrestha, C.Solans, C.Gonzalez, K.Aramaki: Nonaqueous foam with outstandingstability in diglycerol monomyristate/olive oil system – Coll Surf A, 2010, vol.353, pp.157-165 – “Incase of particle stabilized foams, particle size, concentration, and its ability to adsorb at the interface(contact angle) plays a crucial role in the foam stability [J84]” – p.157.J84-c82. S.Barg, C.Soltmann, A.Schwab, D.Koch, W.Schwieger, G.Grathwohl: Novel open cell aluminumfoams and their use as reactive support for zeolite crystallization – J Porous Mater, 2011, vol.18, pp.89-98 – “Oxide particles withstand forces from one interface to the other in the cell walls, balancing thecapillary effects and providing stability [J84] – p.9544

J84-c83. A.J.Klinter, C.A.Leon-Patino, R.A.L.Drew: Wetting phenomena of Al-Cu alloys on sapphire below 800C – Acta Mater, 2010, vol.58, pp.1350-1360 – „As the wetting behaviour of liquid metals on ceramicsstrongly influences various processes like .. the quality of metal foams [J84]” – p.1350.J84-c84. B.M.Somosvári, P.Bárczy, P.Szirovicza, J.Szőke, T.Bárczy: Foam evolution and stability at elevatedgravity levels – Mater Sci Forum, 2010, vol.649, pp.391-397 –“This suspension can be considered as asimple, low-temperature analogue of metallic foams, because particle stabilization works in the case ofthese materials as well [J84]” – p.392.J84-c85. E.Carey, C.Stubenrauch: Foaming properties of mixtures of a non-ionic (C12DMPO) and an ionicsurfactant (C12TAB) – J Coll Interf Sci, 2010, vol.346, pp.414-423 – “Although the majority of studiesdeals with single surfactant systems, polymer-surfactant mixtures, alcohol-surfactant mixtures, solidparticles [J84] and liquid crystals have also been investigated” – p.414J84-c86. G.Morris, S.J.Neethling, J.J.Cillers: The effects of hydrophobicity and orientation of cubic particles onthe stability of thin films – Minerals Engineering, 2010, vol.23, pp.979-984 – “Kaptay [J84] found that,for a given particle spacing, the film stability increased as Theta decreased and that for a given Thetafilm stability decreased as as the particle separation increased” – p.979.J84-c87. K.E.Cole, G.D.M.Morris, J.J.Cilliers: Froth touch samples viewed with scanning electron microscopy –Minerals Engineering, 2010, vol.23, pp.1018-1022 – “Kaptay (2004) derived a model for film stabilitydeterminded by interfacial forces between two neighboring bubbles. It was found that the optimumparticle contact angle for film stability resided in the range 50 – 90 degrees for different monolayer andmultiple layer structures. Multiple layesr of particles and particle clusters had a greater stabilizinginfluence on the film compared to particle monolayers, as the capillary pressure required to rupture thefilm was greater. Loosely packed particle arrangements were considered most likely to occur, with anoptimum contact angle in the range 72 – 88.5 degrees depending on the ratio of the surface energy ofthe solid to the surface tension of the liquid.” – p.1019J84-c88. YH Song, M.Tane, T.Ide, Y.Seimiya, B.Y.Hur, H.Nakajima: Fabrication of Al-3.7 pCt Si-0.18 pct Mgfoam strengthened by AlN particle dispersion and its compressive properties – Metall Mater Trans A,2010, vol.41A, pp.2104-2111 – “It is well known that particles in melt can stabilize foaming behaviorby preventing the drainage effects that originate from the gravity of melt, buoyancy of pores, pressuredifference between films, plateau border in melt, etc… [J84], where the film is a thin melt sheetbetween pores and the plateau border is a node of melt surrounded by some pores. In the prevention ofdrainage effect, the contact angle between the particle and the melt is the most important factor [J84]. Itwas reported that the optimum contact angle for the stabilization of foaming ranges fropm 70 to 86degrees [J84]. … In adduition to Si segregation, the small clusters of AlN particles (Figure 6) possiblycontribute to the stabilization of foaming behavior, because the small clusters consisting of wettingparticles prevent the thinning of film caused by the drainage effect, by decreasing the pressuredifference between films and plateau borders in the melt [J84]. … First, we focus on the change inwettability of AlN particles at high temperature, because the wettability of particles playes an importantrole in the stability of foaming behavior compared with the viscosity of melt [J84].” – p.2109.J84-c89. G.Morris: The Effect of attached hydrophobic particles on the stability of thin films – Book ofAbstracts of 9 th UK Particle Technology Forum, Riccarton, Edinburgh, 25-26 June, 2008, pp.18-19. –“Close packed spherical particles can stabilize a film up to a conrtact angle og 129 degrees [J84]” –p.19.J84-c90. JCH Wong, E Tervoort, S.Busato, UT Gozenbach, AR Studart, P.Emanni, LJ Gauckler: Designingmacroporous polymers from particle-stabilized foams – J Mater Chem, 2010, vol.20, No.27, pp.5628-5640.J84-c91. D.N.H.Tran, C.P.Whitby, D.Fornasiero, J.Ralston: Foamibility of aqueous suspensions of fine graphiteand quartz particles with a trblock copolymer – J Coll Int Sci, 2010, vol.348, pp.460-468 – “Kaptay[J84] inverstigated the general forces governing stability in the froth. He found that particles couldstabilise froths under different conditions in a range of contact angles between 20 o and 90 o .Interestingly, his model predicts that particles above 3 m would probably not be effective stabilisers,which are contradictory to the findings of Dippenaar et al., Johansson and Pugh, Aveyard et al. forexample. This emphasises that foam stability also depends on the particles size, as this governs thedegree of penetration of the liquid films” – p.460.J84-c92. L.Wang, G-C. Yao, H-J. Luo, L-S. Liang, Z-G.Zhang: Effect of addition of Mg powders on foamingbehaviours of Al foams – The Chinese J of Nonferrous Metals, 2010, vol.20, No.7, pp.1339-1345.J84-c93. X.N.Liu, Y.X.Li, X.Chen, Y.Kiu, X.L.Fan: Foam stability in gas injection foaming process – J MaterSci, 2010, vol.45. pp.6481-6493. – „the particles enhance the foam cell wall’s capacity of resistingdisturbance [J102]” – p.6482.J84-c94. Zhu Y, Zhang SM, Chen JD, Hu CP: High Internal Phase Emulsions Prepared with Poly(urethane urea)Aqueous Nanodispersion at Different Temperatures – J Polymer Sci, A: Polymer Chem, 2010, vol.48,45

No.19, pp.4356-4360 – „It is accepted that the stability of particle stabilized emulsions is due to thecoherent particle layer around the droplets, which acts as a steric (mechanical) barrier againstcoalescence” – p.4356J84-с95. G.Morris, S.J.Neethling, J.J.Cilliers: A model for investigating the behaviour of non-spherical particlesat interfaces – J Coll Interface Sci, 2011, vol.354, pp.380-385 – “Ali et al, Denkov et al, Kaptay [J84]and Morris et al agree that, for a given particle spacing, the film stability increases as the contact angledecreases whilst for a given contact angle, the film stability decreases as the particle separationincreases” – p.380.J84-c96. T.Delicato: Drenagem de espumas gas-liquido e influencia da presenca de particluas e anti-espumantes,Dissertacao, Ribeirao Preto, Spain, 2007 – „Estudos realizados por Kaptay [J84] demonstraram queparticulas solidas podem estabiliyar espumas, dependendo do angulo de contato da particula com ainterface do filme e esse angulo deve estar entre 20 deg e 90 deg para ter efeito estabilizante.” p. 41.J84-c97 V.Kevorkijan, S.D.Skapin, I.Paulin, B.Sustarsic, M.Jenko: Synthesis and characterisation of closed cellsaluminium foams containing dolomite powder as foaming agent – Mater Technol, 2010, vol.44, pp.363-371. – „The effect of various processing parameters (temperature, time, melt viscosity, surface tension,wetting behaviour etc..) on the foamility of aluminium alloys and stability of slurry of gas bubbles inmolten metal has been also investigated” – p.363.J84-c98 M.Pliego, C.Fuentes, GJ Guiterez, A.Medina, ME Aguilar: Multiples alturas de equuilibrio en capillaresconicos – Rev Mexicana de Fisica, 2010, vol.56, pp.475-481. – „La penetración capilar de un líquidoque moja, bien o mal, a las paredes de un tubo capilar vertical o, en al caso más general, a las diversasparedes de un espacio capilar, es un fenómeno muy común y de gran interés en áreas de estdio tandiversas como son la micro y nonofluídica, el mojado de medios porosos [J84], la creación desuperficies hidrófilas o hidrófobas, la recuperación de petróleo, el transporte de líquidos en plantas, etc”– p. 475.J84-c99 BM Somosvári, P.Bárczy, J.Szőke, P.Szirovicza, T.Bárczy: FOCUS: Foam evolution and stability inmicrogravity – Coll Surf A, 2011, vol.382, pp.58-63 – „Fundamentals of foam formation and evolutionare well understood, although many interesting questions emerge if we look around int he field ofmicrofluidics, microbubbles, particle stabilization of foams, liquid layers, or the role of gravity [J84]” –p.58J84-c100. Golestanipour, H.A.Mashhadi, M.S.Abravi, M.M.Malekjafarian, M.F.Sadeghian: Manufacturing ofAl/SiC p composite foams using calcium carbonate as foaming agent – Mater Sci Technol, 2011, vol.27,pp.923-927. – “It was thought that ceramic particles changed the curvature of gas/liquid interface,increased the viscosity of melts, and stabilized the cell wall” – p.923.J84-c101 Wong JCH, Tervoort E, Busato S, Gauckler LJ, Ermanni P: Controlling phase distributions inmacroporous composite materials through particles stabilized foams – Langmuir, 2011, vol.27, No.7,pp.3254-3260 – „Particles are reported to best stabilize foams when Theta is between 43 and 90 o , thatis, when the particles are partially wetted by both fluid phases” – p.3255.J84-c102. H.M.Helwig, F.Garcia-Moreno, J.Banhart: A study of Mg and Cu additions ont he foaming behaviourof Al-Si alloys – J Mater Sci, 2011, vol.46, pp.5227-5236. – „Oxide skins or particles at the metal/gasinterface play a crucial role for metal foam stability [J84]” – p.5235.J84-103. S.Beke: Metal foaming controlled by ultrasonic waves – PhD Thesis, TU Wien, 2011, supervisors: HPDegischer and N.Babcsan. – „Several factors influence foam stability, including surface tension, …surface forces, … [J84]” – p.12.J84-c104. G.Morris, S.J.Neethling, J.J.Cilliers: An investigation of the stable orientation of orthorombic particlesin a thin film and their effect on its critical failure pressure – J Coll Interface Sci, 2011, vol.361, pp.370-380 – “Many previous analytical stuidiues, both in 2D and 3D, have analysed the effect of sphericalparticles and their properties on film stability [J84]” – p.370.J84-c105. H.Luo, P.Chen, Y.Liu, Z.Zhao: Preparation process of aluminum foam reinforced by carbon fibers –Suppl. Proc, vol.3, General Paper Selections, TMS, 2011, pp. 139-144.J84-c106. R.Surace, LAC de Filippis: Investigation and comparison of aluminium foams manufactued bydifferent techniques – chapter 6 in „Advanced Knowledge Application in Practice”, 2011, pp.95-118. –„ (particles) … also reduce the velocity of the rising bubbles by increasing the viscosity of the melt[J84]” – p.98 ((I have never said that)).J84-c107. G.D.M. Morris, S.J.Neethling, J.J. Cilliers: A Model for the Stability of Films Stabilized by RandomlyPacked Spherical Particles – Langmuir, 2011, vol.27, No.18, pp.11475-11480.J84-c108. L.J.Gauckler, A.R.Studart, E. Tervoort, U. Gonzenbach, I.Akartuna: Ultrastable particle-stabilizedemulsions – European Patent Application EP 2 361 679 A2, 27-05-2011. „In addition to surface activemolecules, it was recently recongnized that partially hydrophobic particles can als ostabilize air bubblesin surfactant-free diluted suspensions [J84]”.46

J84-c109. C. Chuanuwatanakul, C. Tallon, D.E. Dunstan, G.V. Franks: Controlling the microstructure ofceramic particle stabilized foams: influence of contact angle and particle aggregation – Soft Matter, 2011,vol. 7, pp. 11464-11474. „As a result of the addition of surfactant, and increased contact angle, the energyto detach particles from the air/solution interface increases [J84]” – p.11471. “Kaptay [J84] reported thatthe optimum contact angle value to ensure stabilitz of a foam is also dependant on the arrangement ofparticles and particle aggregates at the liquid-gas interface and in the cell walls. Sepcifically, the balancebetween the energy required to remove a particle from the interface and the capillary pressure which mustbe exceeded in order to coalesce bubbles results in values from about 50 degrees to nearly 90 degrees fromaximum stability foams, consistent with the contact angle values observed in this study” – p.11471.„Contact angles around 70 o produce the most stable foams (and oil in water emulsions) becasue a balancebetween the energy required to remove the particle from the air/solution interface (into the solution) andthe capillary pressure preventiung coalescence, result in maximum foam stability [J84]” – p.11472.“Kaptay [J84] and Hunter et al. stated that the critrical particle siye to promote the stabiliyation of foamsis below 20-30 microns” – p.11464.J84-c110. J.C.H. Wong, E. Tervoort, S. Busato, P. Ermanni, L.J. Gauckler: Engineering Macroporous CompositeMaterials using Competitive Adsorption in Particle-Stabilized Foams - Journal of Colloid and Interface,2012, doi: http://dx.doi.org/10.1016/j.jcis.2012.05.049 - „Particles stabilize foam interfaces mosteffectively when they are partially wetted, that is when θ is in the range of 43 – 90 ○ ” [J84]”J84-c111. BM Somosvári (supervisor: P. Bárczy): Foam evolution and stability at various gravity conditions –PhD thesis, Miskolc, 2012, 96 pp. – „Though the fundamentals of foam formation and evolution are wellunderstood, still many interesting scientific quastions appear if we look around int he field ofmicrofluidics, microbubbles, monodisperse system, particle stabilization of foams, liquid klayers, wetfoam dynamics, or the role of gravity [J84]” – p.2. “Accroding to [J84], six different typical particlearrangements exist that can effectively separate the two liquid-gas interfaces: i…, ii, iii…., iv…, v….,vi…. “ – p.25. “Fig.2.22. Part of the cell wall with different structures build up of the stabilizing particles….. [J84]” – p.26. “To stabilize liquid foams with particles, three subsequent events are needed, and theprobabilities of these events were deduced theoretically by G. KAPTAY in [J84]: 1…., 2….., 3…….” –p.26. “The foam heihts reached as function of contact angle can be compared to the so called product ofprobabilities to stabilize liquid foams [J84]” – p.61. “Table 4.0. Q values gained in the function ofdifferent selected parameter sets, together with standtard deviation and structure data [J84]” – p.62.“Fig.4.5 also clealrly shows that the p curve is in good correlation with our foam height vs contact angledata.” – p.62.J84-c112. Jang-Hoon Ha, Rizwan Ahmad, In-Hyuck Song: A novel method of coating a particle-stabilizedalumina foam on a porous alumina substrate – Mater Letters, 2012,http://dx.doi.org/10.1016/j.matlet.2012.08.007 - „Among the conventional processing methods used forthe preparation of ceramic foams are the replica and sacrificial template methods. These processingmethods use particle]stabilized direct foaming [J84], which has been extensively studied as a promisingroute for the processing of porous materials because of its exceptional stability.”J83. G.Kaptay: Equilibrium electrochemical synthesis diagrams of systems, forminghomogenoeous alloys and compounds – JMM, 2003, vol.39B, No.1-2, pp.383-405 (IF = 0)J83-c1. A.Kostov, B.Friedrich, D.Zivkovic: Predicting thermodynamic properties in Ti-Al binary system byFactSage – Comp.Mater. Sci., 2006, vol.37, pp.355-360 – „Also, there are some works on …equilibrium electrochemical synthesis diagrams of these binaries [J83].” – p.356.J82. N.Borisenko, J.Sytchev, G.Kaptay: Electrochemical study of the electrodeposition andintercalation of sodium into graphite from sodium chloride, as first step of carbon nanotubeformation – JMM, 2003, vol.39B, No.1-2, pp.369-382 (IF = 0)J82-c1. D.Fray: Electrochemical processing using molten salts - Proceedings of EUCHEM 2004 Molten SaltsConference, ed. by J.Kazmierczak and G.Zabinska-Olszak, Wroclaw, 2004, pp.47-57 “Studies haveshown that the alkali atom goes into the structure and forces out the graphite either as tubes or asgraphite sheets that quickly coil to form nanotubes [J82].” – p.56.J82-c2. S.Devyatkin: Electrochemical synthesis of carbon nanotubes in molten carbonates – Proc. of MS7, ed. byP.Taxil, C.Bessada, M.Cassir, M.Gaune-Escard, 2005, vol.1, pp.515-517 – “Molten lithium chlorideelectrolysis at current densities of over 2 A/cm 2 yields carbon nanotubes tens of nanometer in diameteron the consumable graphite cathode [J82]” – p.515.J82-c3. D.Fray: Electrochemical processing using slags, fluxes and salts – Proc. Of 7 th Intern Conf on MoltenSlags, Fluxes and Salts, The South African Institute of Mining and Metallurgy, 2004, pp. 7-12 “Studies47

have shown that it appears that the alkali atom goes into the structure and forces out the graphite, eitheras tubes or as graphite sheets that quickly coil to form nanotubes [J82].” – pp.11-12.J82-c4. DJ Fray: Innovative electrochemical processing using molten salts – Mineral Processing and ExtractiveMetallurgy, 2006, vol.115, No.1, pp.3-7. – „Studies have shown that it appears that the alkali atom goesinto the structure and forces out the graphite either as tubes or as grasphite sheets that quickly coil toform nanotubes [J82]” – p.7.J82-c5. C.Schwandt, A.T.Dimitrov, D.J.Fray: The preparation of nano-structured carbon materials byelectrolysis of molten lithium chloride at graphite electrodes – J Electroanal Chem, 2010, vol.647, pp.150-158 – „Kaptay and co-workers also investigated the electrolytic preparation method. Carbonaceousproducts were prepared by using various molten salt electrolytes and fundamental studies likewisesuggested alkali metal intercalation into graphite as an essntial step of the process [J82]” – p.151J82-c6. C.Schwandt, AT Dimitrov, DJ Fray: High yield synthesis of multi-walled carbon nanotubes fromgraphite by molten salt electrolysis – Carbon, 2012, vol.50, pp. 1311-1315 – „It is generally accepted thatthe first step of the cathodic reduction is the intercalation of the alkali metal into the spacings between thegraphitic layers and the formation of intercalation compounds, MeC x [J82]” – p.1311.J81. M.S.Yaghmaee, Zs.Demeter, J.Sytchev, J.Lakatos, G.Kaptay: Some aspects of theelectrochemical formation of carbon microtubes from molten chlorides – JMM, 2003,vol.39B, No.1-2, pp.343-352 (IF = 0)J81-c1. S.Volkov, I.Novoselova: Modern state of electrolytic synthesis of nanosized carbon materials in moltensalts – EUCHEM 2008 Conference on Molten Salts and Ionic Liquids, Book of Abstracts, p.161 – „Atpresent day four ways and mechanisms of electrolytic synthesis of carbon nanomaterials (CNMs) inmolten salts are known: (1) intercalation of alakali metal (lithium, sodium, potassium) in graphitecathode in chloride melts [J81]” – p.161.J81-c2. C.Schwandt, A.T.Dimitrov, D.J.Fray: The preparation of nano-structured carbon materials byelectrolysis of molten lithium chloride at graphite electrodes – J Electroanal Chem, 2010, vol.647, pp.150-158 – „Kaptay and co-workers also investigated the electrolytic preparation method. Carbonaceousproducts were prepared by using various molten salt electrolytes [J81]” – p.151J80. I.Lukovits, A.Gaovac, E.Kálmán, G.Kaptay, P.Nagy, S.Nikolic, J.Sytchev, N.Trinajstic –Nanotubes: Number of Kekulé Structures and Aromacity – J. Chem. Inf. Comput. Sci., 2003,vol.43, pp.609-614 (IF = 3.078)48

J80-c1. Randic M.: Aromaticity of polycyclic conjugated hydrocarbons – Chemical Reviews, 2003, vol.103,No.9, pp.3449-4605 – „Recently, Lukovits et al. [J80] reported on the number of Kekulé valencestructures for benzenoid belts of different lengths and widths” – p.3594J80-c2. M.V.Diudea: Stability of tubulens – Phys. Chem. Chem. Phys., 2004, vol.6, pp.332-339 – „In thisrespect, Kekule structure count [J80] aimed at measuring the aromacity of polycyclic conjugatedsystems, could help in understanding and predicting the stability and chemical behavior of suchmolecules” – p.336.J80-c3. K.Heberger: Chemometrics in Hungary (the last 10 years) – Chemometrics and Intelligent LaboratorySystems, 2004, vol.72, pp.115-122. (Ref. No. 90). – „Today, he [Lukovits] performs calculations on thenumber of Kekule structures in nanotubes [J80]”- p.118.J80-c4. F.Cai, H.Shao, C.Liu, Y.Jiang: An alternative strategy for count and storage of Kekule and longer rangeresonance valence bond structure – J. Chem. Inf. and Modelling, 2005, vol.45, p.371-378 -„There werealso particular techniques developed to work on this problem [J80] which made it possible to enumerateKekule valence structures for systems with hundreds of atoms, such as nanotubes” – p. 371.J80-c5. B.Mandal: Use of symmetry plane and subsequent substraction for obtaining eigenspectra of somecomplicated graphs in analytical forms – J. Molec. Struct – Teochem – 2005, vol.757, pp.99-111 -„Graph theory has been applied to a wide variety of chemical properties that depend on atomconnectivity in a molecule. Urrently it has been used in various fields of frontier research, such asconstruction of algorithm for computing resistance-distance matrix and its application to study cyclicityof 60 and 70 fullerene isomers, carbon nanostructure analysis [J80], ….” – p.99.J80-c6. M.Randić, X.Guo, D.Plavšić, A.T. Balaban: On the Complexity of Fullerenes and Nanotubes – in:Complexity in Chemistry, Biology, and Ecology (book), Springer US, ed. by D.Bonchev,D.H. Rouvray, 2005, pp. 1-48, DOI: 10.1007/0-387-25871-X_1J80-c7. Mandal B.: Some important formulae using the concept of graphical tree - CHEMICAL PHYSICSLETTERS 417 (4-6): 395-400 JAN 10 2006 – „Graph theory … has been used .. to study the cyclicityof … carbon nanostructure analysis [J80]..” – p.395.J80-c8. M.V.Diudea, C.L.Nagy: Aromacity of Nanostructures – Chapter 6 in: „Periodic Nanostructures”,Springer, 2007, pp.137-166 – „Attempts to predict the aromacity of nanotubes of nanotori have beendone [J80] – p.139.J80-c9. R.Ponec, S.Fias, P.Bultinck, I.Gutman, S.Stankovic: Benzoid szénhidrogének aromás és lokális aromástulajdonságairól – Magyar Kémiai Folyóirat, 2008, 1145. évf., 4. szám, 177-182 – „Lukovits István azelméleti és matematikai kémia számos területén végzett kutatómunkát. Rövid, de igen eredményestudomnényos karrierjének utolsó periódusában főként a policiklikus konjugált molekulák aromástulajdonságaival foglalkozott, elsősorban nanocsövekkel [J80] és benzoid rendszerekkel kapcsolatban”– p.177.J80-c10. R.Kutnar, D.Marusic, D.Vukicevic: On decomposition of leapfrog fullerenes – J Math Chem, 2009,vol.45, pp.406-416 – „One of the many open problems with regards to fullerenes concerns the numberof Kekulé structuresd in a fullerene, the so called Kekulé number [J80]” – p.407.J80-c11. S.M.Azami, R.Pooladi, M.H.Sheiki: Local sigma-pi mixing in C 60 buckminterfullere – J. Molec.Struct., TEOCHEM, 2009, vol. 901, pp.153-156 – “The classical picture of resonance is usually appliedto fullerene and similar nanoscturctures based on Kekule structures [J80]” – p. 153.J80-c12. A. Juhasz-Szalai, E. Kiss-Toth-Dojcsak, P. Koska, J. Szebeni, B. Fodor: Characteristic features ofcarbon nanotubes and their application in living systems – Egészségtudományi Közlemények, 2012,vol.2, No.1, pp.105-111 – “.. the chirality of the tube is characterized by the chiral index [J80]” – p.106.J80-c13. P. Zigert, M. Berlic: Lucas Cubes and Resonance Graphs of Cyclic Polyphenanthrenes - Match-Commun in Mathem and in Comp Chem, 2012, vol.68, No.1, pp. 79-90.J79. G.Kaptay, G.Csicsovszki, M.S.Yaghmaee: An Absolute Scale for the Cohesion Energyof Pure Metals – Materials Science Forum, 2003, Vols. 414-415, pp.235-240 (IF = 0.602)J79-c1. G.L. Hornyak: Introduction to Nanoscience – Lecture 16 Energy at the Nanoscale IV - Copyright: CRCPress 2009 – „Quite an elegant way to provide an absolute (not relative) thermodynamic derivation…”J79-c2. XP Su, S. Yang, JH Wang, NY Tang, FC Yin, Z Li, MX Zhao: A New Equation for TemperatureDependent Solute Impurity Diffusivity in Liquid Metals – J. Phase Equil. Diffusion, 2010, vol. 31, pp.333-340. – „It has been shown recently on the example of the surface tension that the cohesion energycorrelates with the melting point of normal metals [J79]” – p.334.J79-c3. F.Aqra, A.Ayyad: Surface energies of metals in both liquid and solid states – Appl Surf Sci, 2011,vol.257, pp.6372-6379. – “A plot of E b(s) versus E b(L) (the values taken from ref [J79]) for 55 metalsshows a linear relation with a slope equal to 0.8837 (Fig.1)” – p.6374 “Figure 1. Cohesion energy for 55metals at 0 K versus that at melting point (data taken from ref [J79])” – p.6374.49

J78. A.Roósz, J.Farkas, G.Kaptay: Thermodynamics-based semi-empirical description of theliquidus surface and partition coefficients in ternary Al-Mg-Si alloy - Materials ScienceForum, 2003, Vols. 414-415., pp.323-328 (IF = 0.602)J78-c1. R.Zhang, L.Li, Z.Chen, Z.He, W.Jie: Calculation of phase equilibria based on the Levenberg-Marquardtmethod – J. Mater. Sci. Technol., 2005, vol.21, pp.10-12. – “The calculated values agree well with theexperimental results [J78] + Fig.2.” p. 12.J78-c2. He Z., Zhang R.J., Jie W.Q.: Phase equilibria calculation with Levenberg-Marquardt Method –Nonferrous Metals, 2006, vol.58, No.3, pp.51-53 – “Chinese text, reference in p. 52 and Fig.2. Ourmodel data are compared with his model in Fig.2” – p. 52.J78-c3. Raghavan V: Al-Mg-Si (Aluminum-Magnesium-Silicon) - JOURNAL OF PHASE EQUILIBRIA ANDDIFFUSION 28 (2): 189-191 APR 2007 – „Other recent references on the phase equilibria of thissystem include [J78].” – p.190.J77. Á.Borsik, K.K.Kelemen, G.Kaptay: A dynamic model of ceramic particle – solidificationfront interaction - Materials Science Forum, 2003, Vols. 414-415., pp.371-376 (IF = 0.602)J77-c1. Garvin JW, Yang Y, Udaykumar HS: Multiscale modeling of particle-solidification front dynamics, PartI: Methodology – Int. J. Heat Mass Transfer, 2007, vol. 50, pp. 2952-2968 – „Much of the work to dateon particle – solidification front interaction relies on simplified analytical expressions for the drag andthe repulsive intermolecular force [J77]” – p.2952, „Dynamic models that simulate the interaction andsubsequent evolution o fan initially stationary particle being pushed approached by a front have beendeveloped in recent work [J77]” – p.2953, „Previous steady-state as well as dynamic analyses ofparticle-front interactions have employed analytical / empirical models for the forces experienced by theparticle [J77]” – p.2959.J77-c2. Garvin JW, Yang Y, Udaykumar HS: Multiscale modeling of particle-solidification front dynamics. PartII: Pushing-engulfment transition - Int. J. Heat Mass Transfer, vol. 50. pp. 2969-2980 – „The ratio ofthermal conductivity of the particle to that of of the melt plays a major role in determining thesolidification front shape [J77]” – p.2974.J77-c3. J.W.Garwin, Y.Yang, H.S.Udaykumar: Multiscale modeling of particle-solidification front dynamics.Part III: Theoretical aspects and parametric study – Preprint AFRL-MN-EG-TP-2007-7414. – „particlesolidificationfront interactions are abundant in nature and industrial applications. Examples includemicrostuctural development in metal matrix composite manufacturing [J57]” – p.1, „There have been afew dynamic models [J77] of particle-solidification front interactions” – p.5.*J76. Z.Benkő M., G.Kaptay: A Virtual LD-steel-converter - Materials Science Forum, 2003,Vols. 414-415., pp.365-370 (IF = 0.602)J75. M.S.Yaghmaee, G.Kaptay: The Solubility of Nitrogen and Nitrides in Ternary LiquidIron Alloys. The Limits of the ‘Solubility Product’ Concept - Materials Science Forum, 2003,Vols. 414-415., pp.491-496 (IF = 0.602)J75-c1. The Al-Fe-N system - Light Metal Ternary Systems: Phase Diagrams, Crystallographic andThermodynamic Data, Landolt-Borstein – Group IV Physical Chemistry, 2005, vol. 11A2.J74. G.Kaptay: Interfacial Criteria to Produce Metal Matrix Composites and Ceramic ParticleStabilized Metallic Foams - Materials Science Forum, 2003, Vols. 414-415, pp.419-424 (IF =0.602)J74-c1. T.Matsushita, K.Mukai: Penetration behaviour of molten metal into porous oxides - Tetsu-to-Hagane,2004, vol.90, pp.135 – 144 „something in Japanese” – p.138J74-c2. O.N.Verezub: Technologicheskiie osobennosti sozdaniia kompozicionnogo regirovannogo sloia narezhushei poverhnosti nizkolegirovannich stalnich instrumentov metodom lazernoi tviordotelnoiimplantacii – in: „Rezanie i instrument v technologicheskich sistemach”, 2004, vol.66, pp.25-32J74-c3. Janó V.: Study on the production of metal matrix compsites layer by layer melt injection technology –Mater Sci Forum, 2007, vols 537-538, pp.177-184.J74-c4. S.E.Frieberg: Foams from Non-aqueous systems – Curr Opinion Coll Interface Sci, 2010, vol.15,pp.359-364 – “The vital difference from organic plastic foams is the extremely high surface free energy of50

metals resulting in surface and colloidal phenomena playing substantial role: an insight recently broughtto light by the outstanding Hungarian metallurgist Kaptay [J74].” – p.360, “Metallic foams have a sizablesurface free energy and the relation to stability has recently been shown amenable to analysis by Kaptay[J74] – p.360.J74-c5. P.Padhi, S.Kar: A novel route development of bulk Al/SiC metal matrix nano composites – Journal ofNanotechnology, Vol. 2011, Article ID 413512, 5 pages, doi:10.1155/2011/413512 – “In majoprity ofmetal-ceramic combinations [J74] gives the critical velocity for engulfment of particulate in solidifiedmetal … Eq…(1)“ – p.4.J73. Kaptay Gy., Verezub O., Zoltai L., Boross P., Kálazi Z., Verő B.: Fémolvadékokfelületére lőtt mikroszkópikus szilárd szemcsék elmerülésének feltételei (Condition ofPenetration of Microscopic Solid Particles Blown on the Surface of Liquid Metals – AnyagésKohómérnöki Tudományok, Miskolc, 2002, vol. 30., pp.5-22. (IF = 0)J72. H.B.Kushov, G.Kaptay, A.S.Uzdenova, M.K.Vinidzheva: Electrochemical SynthesisDiagrams of the Al-Gd, La-B, Gd-B and Al-La systems – Rasplavi, 2002, No.1, pp.44-48. (IF= 0)51

J71. G.Kaptay: Reduced Critical Solidification Front Velocity of Particle Engulfment due toan Interface Active Solute in the Liquid Metal – Metall. Mater. Trans., 2002, vol.33A,pp.1869-1873 (IF = 1.219)J71-c1. Bassani, B.Previtali, A.Tuissi, S.Arnaboldi, M.Vedani, G.Vimercati, G.Garagnani: Meccanismi disolidificazione e proprieta di getti in compositi a matruice in lega di aluminio – XXXIV ConvegnoNazionale, 14-17 Settembre 2005, Polytecnico Milano (Proceedings, 10 pages, No.8). – „Italiano...” –p.2.J71-c2. Bassani, P; Previtali, B; Tuissi, A; Vedani, M; Vimercati, G; Arnaboldi, S: SOLIDIFICATIONBEHAVIOUR AND MICROSTRUCTURE OF A360-SICp CAST COMPOSITES - MetallurgicalScience and Technology. 2005, Vol. 23, no. 2, pp. 3-10. – „The solidification behaviour of particulatereinforced MMCs is strongly influenced by the interaction of the solid reinforcement phase with thesolidification front… These possibilities significantly affect the degree of reinforcement distribution ofthe cast composite since, when the particles are rejected in the liquid phase, they will concentrate in theinterdendritic regions of the structure, leading to harmful segregation effects [J71]” – p. 4.J71-c3. A.E.Karantzalis, A.Lekatou, E.Georgatis, H.Mavros: Solidification behaviour of ceramic particlereinforced Al-alloy matrices – J.Mater Sci, 2010, vol.45, pp.2165-2173 – „… the importance of otherfactors such as interfacial characteristics and crystallographic compatibility are adressed int he works ofKaptay [J71]…” – p.2165J71-c4. A.E. Karantzalis, A. Lekatou, E. Georgatis, T. Tsiligiannis, H. Mavros: Solidification observations ofdendritic cast Al alloys reinforced with TiC particles – J Mater Eng Perform, 2010, vol.19, No.9,pp.1268-1275. – “The importance of other factors such as interfacial characteristics and crystallographiccompatibility are addressed in the works of Kaptay [J71]” – p.1168.J.70. S.V.Devyatkin, G.Kaptay: Physical, Chemical and Electrochemical Behaviour of BoronOxide in Cryolite-Alumina Melts – Russian Journal of Applied Chemistry, 2002, vol.75,No.4, pp.565-568 (in Russian: Zh. Prikladnoi Khimiii, 2002, vol.75., 579-582) (IF = 0.221)J70-c1. Simakov D, Vassiliev S, Tursunov P, Khasanova N, Ivanov V, Abakumov A, Alekseeva A, Antipov E,Tsirlina G: Electrodeposition of TiB2 from cryolite-alumina melts - LIGHT METALS 2008, ed. byDeYoung DH, 2008, TMS, pp. 1019-1022. - „As it follows from literature [J70], complications can gowith high volatility of boron fluoride compounds and from formation of passive insulating TiO filmwhen titanium compounds in the melt are partly reduced” – p. 1020.J69. A.Magyar, Z.Gácsi, L.Daróczi, G.Kaptay: Morphological investigation of theintermetallic phases in C/Al composite by image analysis – Image Anal. Stereol., 2001,vol.20, Suppl.1, pp.275-280 (IF = 0)J68. S.V.Devyatkin, O.I.Boiko, N.N.Uskova, G.Kaptay: Electrochemical Synthesis ofTitanium Silicides from Molten Salts – Z. Naturforsch. A, 2001, vol. 56 a, pp.739-740 (IF =0.746)J67. G.Kaptay: A Model for the Solid-Liquid Interfacial Energies of Pure Metals – Trans.JWRI (Joining and Welding Research Institute), 2001, vol. 30., Special Issue, pp. 245-250.(IF = 0)J67-c1. Rontó Viktória: A szekunder dendritágak durvulása háromalkotós alumínium ötvözetek kristályosodásaközben – PhD értekezés (tud. vez.: dr. Roósz András), Miskolc, 2001. szeptember – „ értékétG.Kaptay [J67] szerint határoztam meg a szín alumíniumra meghatározott egyenlettel: {idézettegyenlet}” – 72. o.J67-c2. Rontó V., Roósz A.: A dendritág durvulás numerikus szimulációja háromalkotós Al ötvözetek esetén –Anyag- és Kohómérnöki Tudományok, Miskolc, 2001, vol.29, pp.111-121. – „szigma értékét a tisztaAl-ra megadott Kaptay-féle egyenlettel számítottuk [J67]” – p.115.J67-c3. V.Rontó, A.Roósz: Numerical Simulation of Dendrite Arm Coarsening in the Case of Ternary Liquid AlAlloys – Materials Science Forum, 2003, vols. 414-415, pp.483-490 – “The value of is calculated bythe Kaptay equation given for the poor (sic!) Al [J67]: = 73.6 + 0.0862T (mJ/m 2 )” – p.48552

J67-c4. V.M.Samsonov, O.A.Malkov: Thermodynamic model of crystallization and melting of small particles –Central Europ J of Physics, 2004, vol.2, No.1, pp.1895-1902 – „Generally, the available data on solidliquidinterfacial energies are contradictory and not quite reliable. The most accurate treatment of theproblem in question seems to belong to G.Kaptay [J67]” – p.92.J67-c5. Jones H: An evaluation of measurements of solid/liquid interfacial energies in metallic alloy systems bythe groove profile method - METALLURGICAL AND MATERIALS TRANSACTIONS A-PHYSICAL METALLURGY AND MATERIALS SCIENCE 38A (7): 1563-1569 JUL 2007 – “Kaptaycalculated alpha = 0.34, 0.51, 0.58, 0.58, 0.59 and 0.59 for diamond cubic Si, cph Mg, fcc Cu, bcc Naand Fe and cph Zn and fcc Al, respectively, with their melts [J67]” – p,1565.J67-c6. A.Fukuda, T.Yoshikawa, T.Tanaka: A fundamental approach for the measurement of solid-liquidinterfacial energies – J Pys: Conf-ceries, 2009, vol.165, paper 012079, pp.1-4 – “The determinedinterfacial energy between solid copper and liquid Cu-B alloy was in good agreement with reportedvalues between solid and liquid copper of 177 – 232 mN/m [J67]” – p.3.J66. G.Kaptay, E.Báder: Ion-dipole Adhesion Energy Model for Wettability of OxideCeramics by Non-reactive Liquid Metals – Trans. JWRI (Joining and Welding ResearchInstitute), 2001, vol. 30., Special Issue, pp. 55-60. (IF = 0)J66-c1. T.Wübben: Zur Stabilität flüssiger Metallschaume – Universität Bremen, Germany, 2003, 128 pp. (ref.No.72) – “Da die Messung des Benetzungsverhaltens speziell bei Metallen wegen der hohemTemperaturen und erforderlichen hochreinen Umgebungsbedingungen aufwendig ist, beschäftigt sicheine reihe von Arbeiten mit der theoretischen Vorhersage von Kontaktwinkeln verschiedener Metall-Keramik-Materialpare [J66]. Für das System Bleioxid- Blei liegen bislang jedoch keine experimentellenDaten vor. So .. Pb/PbO = 120 o [J66]… . Sie konnte mit freundlicher Unterst-Uzung der Arbeitsgruppevon Prof. Kaptay, Universität Miskolc, Ungarn, mit dem dortigen Great durchgeführt werden. Dabeihandelt es sich um einen Ofen, in dem Metalle auf bis zu 1000 o C aufgeheizt werden können [J66]”– p.50. „Die Messung des Winkels an fünf verschieden Bleitropfen ergab einen Wert von Pb/PbO = 132 2 o ” – p.51.J66-c2. Pázmán J.: „Nanokompozitok” tárgyleírás, PPT diagyűjtemény, 2010, Miskolci Egyetem.J66-c3. A. Karasangabo, C. Bernhard: Investigation of Alumina Wetting by Fe–Ti, Fe–P and Fe–Ti–P Alloys -Journal of Adhesion Science and Technology, 2012, vol 26, Issue 8-9, 2012 pp.1141-1156.J65. E. Báder, L.Zoltai, M.Hördler, P.Arató, R.F.Singer, G.Kaptay: Wettability of SiliconNitride Based Ceramic by Liquid Metals – Trans. JWRI (Joining and Welding ResearchInstitute), 2001, vol. 30., Special Issue, pp. 137-141. (IF = 0)J65-c1. R.Klein, M.Desmaison-Brut, P.Ginet, A.Bellosi, J.Desmaison: Wettability of silicon nitride ceramiccomposites by silver, copper and silver-copper titanium alloys – J.Eur. Ceram. Soc., 2005, vol.25,pp.1757-1763 (No.11). – “The equilibrium value (of the contact angle) between 110 and 130 degprobably corresponded to the Cu-Si 3 N 4 -Y 2 O 3 -Al 2 O 3 system [J65]” – p.1760J65-c2. M.Singh, R.Asthana, F.M.Varela, J.Martinez-Fernandez: Microstructural and mechanical evaluation of aCu-based active braze alloy to join silicon nitride ceramics – J Eur Ceram Soc, 2011, vol.31, pp.1309-1316 – “Contact angle measurements [J65] show that Ti-containing brazes rapidly wet the ceramic, andthe most significant grains are achieved at small (2-10 %) amounts of Ti at which braze ductility is notimpaired but there is sufficiently high Ti activity for reaction with Si 3 N 4 .” – p.1311.J65-c3. M.Singh, J.Martinez-Fernandez, R.Asthana, J.R. Rico: Interfacial characterization of siliconnitride/silicon nitride joints brazed using Cu-base active metal interlayers – Ceramics International,2012, vol. 38, pp.2792-2802. – Contact angle measurements [J65] reveal that Ti-containing Cu and Agbasebrazes rapidly wet silicon nitride ceramics ….” – p.2793.53

J64. G.Kaptay, K.K.Kelemen: An Interfacial Force Acting on a Spherical Particle in theInterfacial Energy Gradient – Trans. JWRI (Joining and Welding Research Institute), 2001,vol. 30., Special Issue, pp. 305-310. (IF = 0)J64-c1. O.Raychenko, A.Byakova, T.Nakamura, S.Gnyloskurenko: Thermocapillary phoresis of inclusions withinterphase surfactant – Mater Sci Eng A, 2008, vol.495, pp.326-329. – Our purpose is to derive thesteady state migration velocity of an inclusion under the above conditions (thermocapillary phoresisvelocity). The onlt driving force exerted on the inclusion in this situation –the thermocapillary force- isexpressed by the equation [J64]: {Equation + explanation is given}.” – pp.326-327.J64-c2. A.I.Raichenko: Phoresis of inclusions in viscous media under the combined action of electromagnetismand thermocapillarity: Theory. Powder Metallurgy and Metal Ceramics, 2011, vol.50, No.1-2., pp.34-42F dE / dh i is the external driving force the medium exerts on the inclusion– “The quantity i z[J64]” – p.36, The calculations similar to those represented in [J64] give: … Eq.(12)” – p.37.J63. G.Kaptay, G.Csicsovszki, M.S.Yaghmaee: Estimation of the absolute values of cohesionenergies of pure metals – Materials’ World (e-journal with ISSN 1586-0140, accessible at:http://materialworld.uni-miskolc.hu), July 2001 (IF =0)J63-c1. DE Smirnova, SV Starikov, VV Stegailov: Interatomic potential for uranium in a wide range ofpressures and temperatures – J.Phys: Condens. Matter, 2012, vol.24, No.1, 015702. – “Cohesion energyof uranium = -4.20 eV (this work), and -4.22 eV [J63]” – Table 3.J63-c2. S.Sanjabi, N. Bayat: Thermodynamic modeling of particle formation and reshaping in metallic catalystnanofilms for carbon nanotube growth – Model Simul Mater Sci Eng, 2012, vol.20, paper No. 035002(10 pp).J63-c3. D.E. Smirnova, S.V. Starikov, V.V. Stegailov: New interatomic potential of mechanical andthermodynamic properties of uranium in a wide range of pressures and temperatures – Phys MetalsMetalography, 2012, vol.113, pp.107-116 (in Russian: Fizika metallov I metallovedenie, 2012, vol.113,No.2, pp.115-124). “Table 3. In addition, the table also shows ther value of the cohesive energy ofin comparison with the known value [J63] in eV = -4.20 eV (this work), and -4.22 eV [J63]”. UJ62. M.S.Yaghmaee, G.Kaptay: On the stability range of SiC in the liquid Al-Si-Mg system –Materials’ World (e-journal with ISSN 1586-0140, accessible at: http://materialworld.unimiskolc.hu),July, 2001. (IF = 0)J62-c1. N.Babcsán: Ceramic Particle Stabilized Aluminum Foams – PhD Dissertation, Miskolc, 2003 – “inTable 9. Calculated thermodynamic stability range of reaction between liquid Al and ceramics – 2 nd row[J62]: Ceramic = SiC, Reaction product = Al 4 C 3 , Reaction stability range: below 7 at% Si content at themelting point, Remarks: increasing the temperature and adding extra Mg the reaction stability rangeincreases by the model, good fit with the experiments” – p.25, “At high temperature the SiC also reactswith the Al melt producing Al 4 C 3 . This is the case by our experimental results (Table 18), which arepredicted exactly by previous theoretical findings [J62]” – p.78.J62-c2. B.Dikici, M.Gavgali, C.Tekmen: Corrosion Behavior of an Artificially Aged (T6) Al–Si–Mg-basedMetal Matrix Composite - Journal of Composite Materials, Vol. 40, No. 14, 1259-1269 (2006) – „.. thereaction products, such as Al 4 C 3 that occured at the matrix-reinforcement interface also affect thecorrosion behaviour of MMCs [J62]. Al 4 C 3 has a detrimental effect on the corrosion resistance of Al-SiC composite because it is water reactive and thus increases the corrosion sensitivity of the composite[J62].J62-c3. E.E.S. Moraes, M.L.A. Graça, C.A.A. Cairo: Study of aluminium alloys wettability on SiC preform –Proc. Of 17º CBECIMat - Congresso Brasileiro de Engenharia e Ciência dos Materiais, 15 a 19 deNovembro de 2006, Foz do Iguaçu, PR, Brasil., pp. 4217-4224. – „An addition of silicon is assigned forthe infiltration, because affects the aluminium alloys fluidity positively, lowers the melting point andavoids the weak phase development. This reaction, if extensive, can be detrimental for the properties ofthe composites, decreases the resistance [J62], because forms a weak phase Al4C3 at the interface[J62]. However, a strong interface can be created to promote a metallurgical bonding between SiC andAl by the chemistry interdifusion and reaction“ – p.4218.J62-c4. WM Khairaldien, AA Khalil, MR Bayoumi: Production of Al-SiC composites using powder metallurgya temperatures above the Al melting point – J. Testing Evaluation, 2007, vol.35, No.6, pp.655-667. –„SiC is thermodynamically unstable at temperatures above the melting point of aluminium and reacts54

with the liquid aluminium to form aluminium carbide and silicon [J62]… This can be understood fromthe Al-Si-C phase diagram [J62]” – p.664.J62-c5. M.Gavgali, B.Dikici, F.Bedir: Corrosion susceptibility of Al-Cu/TiC MMCs fabricated by conventionalhot pressing – Indian J. Eng. Mater Sci, 2007, vol.14, pp.303-308 – In the unaging conditions severalreasons can be stated fro fluctuation in potential values such as the size and volume fraction of TiC,voids at the TiC/Al interface, reactions between the Al alloy matrix and TiC particles, segregation ofalloy elements to TiC/Al interface, high dislocation densities and residual stresses formed in thevicinity of TiC particles, because corrosion resistance of AMMCs may be greatly affected by thesefactors [J62]” – p.306.J62-c6. B.Dikici, C.Tekmen, O.Yigit, M.Gavgali, U.Cocen: Detrimental effect of particle sol-gel coating on thecorrosion behavior of A380-SiC composite – Corrosion Science, 2009, vol.51, pp.469-476 – “The mainproblems in Al/SiC interface during fabrication or remelting are the interfacial chemical reactionproducts, such as Al 4 C 3 , reinforcement degradation and the lack of wettability with the matrix. Al 4 C 3has important detrimental effects, such as reducing reinforcement/matrix interfacial strength andincreasing the corrosive sensitivity of the composite [J62]” – p.469.J62-c7. B.Dikici, F.Bedir, M.Gavgali: Al/TiC in-situ nano kompozitlerin sicak presleme yontemiyle uretilmesi –5. Uluslararasi Ileri Teknolojiler Sempozyumu (IATS 09), 13-15 Mayis 2009, Karabuk, Turkiye, 5 pp,“Al4C3, in-situ kompozitlerin kullanilabilirgli ve mekanik ozellikleri uzerinde olumsuz bir etkiyesahiptir, oldukca gevrek (kirilgan) bir fazdir ve su ile reaktife olarak kompozitin korozyona karsiduyarli hale gelmesime neden olmaktadir [J62] - p.4.J62-c8. M.Akrom, P.Marwoto, Sugianto, J.Fisika: Pembuatan MMC berbasis teknologi metalurgi serbuk denganbahan baku aluminium dari limbah kaleng minumam dan aditif abu sekam padi – J. Pend Fis Ind, 2010,vol.6, No.1, pp.79-87.J62-c9. Burak Dikici, Cagri Tekmen, Mehmet Gavgali, Umit Cocen: The Effect of Electroless Ni Coating of SiCParticles on the Corrosion Behavior of A356 Based Squeeze Cast Composite - Journal of MechanicalEngineering, 2011, vol. 57, pp. 11-20 – „the corrosion susceptibility of the composite increases due tothe presence of Al4C3 phase, which forms at the SiC/Al matrix interface [J62]” – p.11.J62-c10. Z.Yaniv, I.Pavlovsky, N.Jiang, J.P.Novak, R.Fuink, M.Yang, D.Mao, S.Kim: Enhancing thermalproperties of carbon aluminium composites – US patent 2011/0027603 A1, publ. Date: Feb. 3, 2011. –„The phase diagram of Fig.14 may be found in [J62]” – p.7.J62-c11. B. Dikici: Age hardening response of an Al/TiC hot pressed multi-layered composite: Influence oncorrosion – J Comp Mater, 2012, vol. 46, pp. 471-481.J61. G.Kaptay: On the possibility to produce MgB 2 superconductive layer by electrochemicalsynthesis from molten salts – Materials’ World (e-journal with ISSN 1586-0140, accessibleat: http://materialworld.uni-miskolc.hu), July, 2001. (IF = 0)J61-c1. S.Kim, D.S.Stone, J-I.Cho, C-Y.Jeong, C-S. Kang, J-C. Bae: Phase stability determination of the Mg-Bbinary system using the CALPHAD method and ab-initio calculations – J Alloys Compounds, 2009,vol.470, pp.85-89 – “The literature establish upper and lower bounds for the formation enthalpies [J61]”– p.87. “Fig.4. Calculated formation enthalpies of magnesium borides at 298.15 K, compared toexperimental data in the literature [32]” – p.87.J60. J.Miklósi, P.Póczik, I.Sytchev, K.Papp, G.Kaptay, P.Nagy, E.Kálmán: Atomic forcemicroscopy investigation of electrochemically produced carbon nanotubes – Appl.Phys.,2001, vol. A72, pp. S189-S192. (IF = 1,722)J60-c1. G.Z.Chen, D.J.Fray: Recent development in electrolytic formation of carbon nanotubes in molten salts –J. of Mining and Metallurgy, 2003, vol.39B, pp.309-342 “While research in the electrolytic method isgathering forces around the world in the past few years [J60]” – p.311, “Kaptay and coworkers alsoinvestigated the electrolytic product by atomic force microscopy, revealing some interesting nanostructures[J60].” – p.313, “An interesting study of the electrolytic product by atomic force microscopywas jointly reported in 2001 by two Hungarian groups led by George Kaptay [J60]. In addition tofindings similar to that from SEM of the product from the solidified salt, interestingly, tori of about300-400 nanometers in diameter and 10-15 nm in height were observed on samples originated from thesurface of the cathode, see Figure 8.” – pp.327-328.J60-c2. I.A.Kinloch, G.Z.Chen, J.Howes, C.Boothroyd, C.Singh, D.J.Fray, A.H.Windle: Electrolytic, TEM andRaman studies on the production of carbon nanotubes in molten NaCl – Carbon, 2003, vol.41, pp.1127-1141 – “ Kaptay et al agrees with the initial intercalation stage but suggests that the fragmentsresponsible for the nanotube formation are graphite sheets rather than M x C y particles [J60]” – p.1128.55

J60-c3. C.Schwandt, A.T.Dimitrov, D.J.Fray: The preparation of nano-structured carbon materials byelectrolysis of molten lithium chloride at graphite electrodes – J Electroanal Chem, 2010, vol.647, pp.150-158 – „Kaptay and co-workers also investigated the electrolytic preparation method. Carbonaceousproducts were prepared by using various molten salt electrolytes [J60]” – p.151J60-c4. AR Kamali, C Schwandt, DJ Fray: Effect of graphite electrode material on the characteristics of moltensalt electrolitically produced carbon nanomaterials – Mater Charact, 2011, vol.623, pp.987-994 – „Thisfinding was then confirmed further in a number of subsequent studies, in which both lithium chloride andsodium chloride were found suitable molten salt electrolyte [J60]” – p.987J60-c5. A.R. Kamali, C. Schwandt, D.J. Fray, On the oxidation of electrolytic carbon nanomaterials, CorrosionScience, 2012, vol.54, pp.307-313. – „The cathodic reaction leads to the erosion of the graphite and therelease of a variety of carbon nanostructures including multi-walled carbon nanotubes (MWCNTs) andcarbon nanoparticles. The method has been investigated further in a number of studies [J60]” – p. 3.J60-c6. C.Schwandt, AT Dimitrov, DJ Fray: High yield synthesis of multi-walled carbon nanotubes fromgraphite by molten salt electrolysis – Carbon, 2012, vol.50, pp. 1311-1315. „The molten salt electrolysismethod of converting graphite directly into nanoscale carbon materials is a rather unknown approachtoward preparation of CNTs [J60]” – p.1311.J60-c7. A.R. Kamali, G. Divitini, C. Schwandt, D.J. Fray, Correlation between microstructure and thermokineticcharacteristics of electrolytic carbon nanomaterials, Corrosion Science (2012), doi: http://dx.doi.org/ -„bulk graphite sample is cathodically polarised in a molten alkali metal chloride salt, such that the alkalimetal intercalates into the graphite and disintegrates its microstructure whereby the graphite is continuallyeroded into nanometre sized carbon entities. These become detached from the graphite surface andaccumulate in the molten salt bath from where they can be harvested [J60].”J59. G.Kaptay: Discussion of a „Microscale Simulation of Settler Processes in Copper MatteSmelting by K.O.Fagerlund, H.Jalkanen, Metall. Mater. Trans. B, 2000, vol.31B, pp.439-451”– Metall. Mater. Trans. B, 2001, vol.32B, pp.555-557 (IF = 0,754)J59-c1. Xia JL, Ahokainen T, Kankaanpaa T, Jarvi J, Taskinen P: Flow and heat transfer performance of slagand matte in the settler of a copper flash smelting furnace – Steel Res Int, 2007, vol. 78, No.2, pp. 155-159 - “Recently, numerous studies have been carried out on the performance of flash smelting furnaces[J59]” – p.155.J59-c2. H.Hasinovic, SE Friberg: Destabilization mechanisms in a triple emulsion with Janus drops – J ColloidInterface Sci, 2011, vol.361, pp.581-586. – “The fundamentals of the equilibrium between gravitationaland interfacial tension forces for a pendant drop at a liquid interface was given by Kaptay [J59], whodetermined the maximum drop size of a Cu 2 S-FeS matte, floating in liquid low iron wollastonite slag inthe copper matte smelting process. … Fig.5, Eq.3” – p.585.J59-c3. A. Al-Bawab, A. Bozeya, H. Hasinovic, S.E. Friberg: Three- Phase Surfactant-less Emulsions, ArabianJournal of Chemistry (2011), doi: 10.1016/j.arabjc.2011.10.005 – „An exact solution to the problem ofthe passage of a drop through an interface due to gravitational forces was given by Kaptay (Kaptay2001), Figure 11. Kaptay determined the maximum drop size of a Cu2S-FeS, matte, floating on liquidlow iron wollastonite slag in the copper matte smelting process. With the interfacial tensions and thecontact angles in Figure 11 (Kaptay, 2001) known, the critical drop size was given as.. Eq.(13)…. Thenecessary information to apply equation (13) is at present not available; sufficiently accuratemeasurements of the involved factors are in progress” – p.11/33.J58. Á.Borsik, K.K.Kelemen, G.Kaptay: Dynamic simulation of the movement of ceramicparticles in front of growing solidification front – Archives of Mechanical Technology andAutomatization, 2001, vol.21, pp.19-28. (IF = 0)J57. G.Kaptay: Interfacial Criterion of Spontaneous and Forced Engulfment of ReinforcingParticles by an Advancing Solid/Liquid Interface – Metall. Mater. Trans. A., vol.32A, 2001,993-1006. (IF = 1,273)J57-c1. L.Hadji: Thermal force induced by the presence of a particle near a solidifying interface – Phys. Rev. E.,2001, vol.64, 051502/1-6 – “… Other studies have simply considered ad-hoc expressions for the dragforce that also include the thermal conductivities of the particle and the melt. These approaches areincorrect because they yield expressions for the hydrodynamic drag force that depend on the thermalproperties of the particles and thus make no sense physically. For instance, modified formulas for thedrag force have been derived, which show that the force vanishes when the particle is perfectly56

insulating. We refer the reader to the recent papers by Kaptay [J57] and to references therein for athorough discussion of results obtained using this approach. “ – p.5J57-c2.Y.M.Youssef, R.W.Hamilton, R.J.Dashwood, P.D.Lee: Latent heat evolution from TiB 2 particulatereinforced alloys – Materials Science Forum, 2002, vol.369, pp.259-264J57-c3. L.Hadji: Particle engulfment in crystal growth: the thermal puzzle – Current Topics in Crystal Growthresearch, 2002, vol.6, pp.95-104J57-c4. N.Babcsán: Ceramic Particle Stabilized Aluminum Foams – PhD Dissertation, Miskolc, 2003 -“Contrary to aqueous systems solidification is overlapping the distribution of the particles in the liquidmetal. The solid-liquid interface can push or engulf the particles modifying their original distribution inthe liquid [J57]” – p.27J57-c5. Z.Q.Wang, X.F.Liu, Y.H.Liu, Y.H.Zhang, L.N.Yu, X.F.Bian: Structural heredity of TiC and itsinfluences on refinement behaviors of AlTiC master alloys – Trans. of Nonferrous metals Society ofChina, 2003, vol.13, No.4, pp.790-793. „It was reported that solidification parameters could influencethe distribution of particles in Al melt [J57]” – p.792J57-c6. Catalina AV, Stefanescu DM, Sen S: Numerical calculation of the morphology of a solid/liquid interfacenear an insoluble particle, in: MODELING OF CASTING, WELDING AND ADVANCEDSOLIDIFICATION PROCESSES, ed. by: Stefanescu DM; Warren JA; Jolly MR; Krane MJM, 2003,pp.125-132J57-c7. S.Mukherjee, D.M.Stefanescu: Liquid convection effects on the pushing-engulfment transition ofinsoluble particles by a solidifying interface: Part I. Analytical Calculation of the Lift Forces –Metall.Mater.Trans., 2004, vol.35A, pp.613-621 – „The full implication of the surface energy has beenrecently discussed by Kaptay [J57]” – p.614J57-c8. Y.M.Youssef, R.J.Dashwood, P.D.Lee: Effect of clustering on particle pushing and solidificationbehavior in TiB 2 reinforced aluminum PMMCs – Composites A, 2005, vol.36, pp.747-763 – „Thecontact angle value for Al/TiB 2 , the particle/vapor interfacial energy, and the liquid/vapor interfacialenergy were taken from the literature [J57]” – pp760-761.J57-c9. H.Ohta, H.Suito: Dispersion behaviour of MgO, ZrO 2 , Al 2 O 3 , CaO-Al 2 O 3 and MnO-SiO 2 deoxidationparticles during solidification of Fe-10 mass% Ni alloy – ISIJ Int., 2006, vol.46, pp.22-28 – „Footnoteto Table 2: my equation, coloumn 3 of Table 2 is calculated by this equation [ J57]” – p.27.J57-c10. H.Ohta, H.Suito: Effect of sulfur abd oxygen on engulfment and pushing of deoxidation particles ofZrO 2 and Al 2 O 3 during solidification of Fe-10mass%Ni alloy – ISIJ Int., 2006, vol.46, pp.472-479 –„Table 1 and Fig.1 – calculation of solid metal / solid particle interfacial energy [J57]” – pp. 473-474.57

J57-c11. Wang Y., Liu X.: SiC particulate reinforced aluminium matrix composites – the status and developmenttrend – Research Studies on Foundry Equipment, 2003, No.3, pp.18-22 (ref. No.16) – „Chinese text,referring to my equation 2 [J57]” – p.20.csclJ57-c12. Schaffer PL, Miller DN, Dahle AK: Crystallography of engulfed and pushed TiB 2 particles inaluminium - SCRIPTA MATERIALIA 57 (12): 1129-1132 DEC 2007 – “.. many models have beendeveloped to explain the transition between engulfment and pushing [J57]” – p.1129, p. 1132.J57-c13. J.He, J.Zhao, H.Li, X.Zhang, Q.Zhang: Directional solidification and microstructural refinement ofimmiscible alloys – Metall Mater Trans A, 2008, vol.39A, pp.1174-1182 – “There exists threeinteraction modes: repulsion, engulfment and entrapment [J57]” – p.1178.J57-c14. J.W.Garwin, Y.Yang, H.S.Udaykumar: Multiscale modeling of particle-solidification front dynamics.Part III: Theoretical aspects and parametric study – Preprint AFRL-MN-EG-TP-2007-7414. – „particlesolidificationfront interactions are abundant in nature and industrial applications. Examples includemicrostuctural development in metal matrix composite manufacturing [J57]” – p.1J57-c15. A.Ciftja: Solar silicon refining, inclusions, settling, filtration, wetting: PhD Thesis, NTNU, Trondheim,2009 – “The full implications of the surface energy have ben recently discussed by Kaptay [J57]” –p.22.J57-c16. A.E.Karantzalis, A.Lekatou, E.Georgatis, H.Mavros: Solidification behaviour of ceramic particlereinforced Al-alloy matrices – J.Mater Sci, 2010, vol.45, pp.2165-2173. – „… the importance of otherfactors such as interfacial characteristics and crystallographic compatibility are adressed in the works ofKaptay [J57]…” – p.2167J57-c17. D.N.H.Tran, C.P.Whitby, D.Fornasiero, J.Ralston: Foamibility of aqueous suspensions of fine graphiteand quartz particles with a trblock copolymer – J Coll Int Sci, 2010, vol.348, pp.460-468 – “Kaptay[J57] inverstigated the general forces governing stability in the froth. He found that particles couldstabilise froths under different conditions in a range of contact angles between 20 o and 90 o .Interestingly, his model predicts that particles above 3 m would probably not be effective stabilisers,which are contradictory to the findings of Dippenaar et al., Johansson and Pugh, Aveyard et al. forexample. Th8is emphasises that foam stability also depends on the particles size, as this governs thedegree of penetration of the liquid films” – p.460.J57-c18. A.E.Karantzalis, A.Lekatou, E.Georgatis, T.Tsiligiannis, H.Mavros: Solidification observations ofdendritic cast Al alloys reinforced with TiC particles – J Mater Eng Perform, 2010, vol.19, No.9, pp.1268-1275 – “The importance of other factors such as interfacial characteristics and crystallographiccompatibility are addressed in the works of Kaptay [J57]” – p.1268.J57-c19. A.Ciftja: Solar silicon refining, inclusions, settling, filtration, wetting: Lambert Academic Publishing,Saarbrücken, Germany, 2010 – “The full implications of the surface energy have ben recently discussedby Kaptay [J57]” – p.20.J57-c20. H.Kaftelen, N.Ünlü, G.Göller, M.L.Övegcoglu, H.Henein: Comparative processing-structure-propertystudies of Al-Cu matrix composites reinforced with TiC particulates – Composites A, 2011, vol. 42,pp.812-814 – “Due to the strong metallic nature and closely matched crystal structure with Al, TiCparticles are easily wetted by liquid Al during solidification [J57]” – p.3.J56. G.Kaptay, K.K.Kelemen: On the force acting on a sphere moving towards a solidificationfront due to an interfacial energy gradient at the sphere/liquid interface – ISIJ International,2001., vol.41., pp.305-307. (IF = 0,980)J56-c1: K.Mukai, Z.Wang, W.Lin: Reply to the Paper named „The force acting on a sphere moving towards asolidification front due to an interfacial energy gradient at the sphere/liquid interface” – ISIJInternational, 2001, vol.41., pp.308-310 – “We appreciate Kaptay and Kelemen very much for theirsincere concerning to our researches. We believe that this discussion is very helpful for furtherclarifying the mechanism of surface tension gradient influencing the behavior of particles” – p. 310,összesen 3 oldal válaszsl58

J55. Hutkainé Göndör Zs., Gál J, Zambóné Benkő M., Szontagh E., Kaptay Gy.: Alumíniumhegesztőpálcák kémiai fényesítése – Anyag- és Kohómérnöki Tudományok, 2000, vol.28.,pp.5-16. (IF = 0)J54. Báder E., Kaptay Gy.: Határfelületi energiák vizsgálata volfrám-karbid/réz-ónrendszerekben – BKL Kohászat, 2000, 133. évf., 11. szám, 431-435. (IF = 0)J53. S.V.Devyatkin, G.Kaptay: Chemical and Electrochemical Behaviour of TitaniumDiboride in Cryolite-Alumina Melt and in Molten Aluminum – Journal of Solid StateChemistry, 2000, vol.154, pp.107-109. (IF = 1.527)J53-c1. C.Bessada, E.M.Anghel: 11 B, 23 Na, 27 Al and 19 F NMR study of solid and molten Na 3 AlF 6 -Na 2 B 4 O 7 –Inorganic Chemistry, 2003, vol.42., No.12, pp.3884-3890 – „Titanium diboride ... has manyapplications. These includes ... cathodes in Hall-Heroult cells for the electrolytic production ofaluminium [J53]– p.3884.J53-c2. J.Wachsmuth, R.Radhakrishnan, T.S.Sudarshan: Effect of pulsed current on reactively synthesized TiB 2consolidated by plasma pressure compaction – Powder Metallurgy, 2003, vol.46, pp.361-364 –„Although there are reports ont he potential of TiB 2 to fill these application [J53], it is difficult to sinterTiB 2 powders to full density’ – p.361.J53-c3. D.A.Weirauch Jr., W.J.Krafcik, G.Ackart, P.D.Ownby: The wettability of titanium diboride by moltenaluminum drops – J.Mater.Sci., 2005, vol.40, pp.2301-2306 – The results of subsequent studies differedwidely with no convergence of contact angle data above the well known Al wetting onset temperatureof 900-1000 o C [J53].” – p.2301J53-c4. A.Changizi: Production and properties of in-situ aluminum titanium diboride composites formed by slagmetalreaction method – MSc Thesis, 2005, Middle East Technical University, Turkey – „Boron isdeposited from a cryolite-alumina melt in a 3-electron irreversible charge transfer process [J53]” – p.41,„The solubility of Al in TiB 2 is so low that it cannot be measured [J53]” – p.44.J53-c5. Celikkan H, Ozturk MK, Aydin H, Aksu ML: Boriding titanium alloys at lower temperatures usingelectrochemical methods - THIN SOLID FILMS 515 (13): 5348-5352 MAY 7 2007 – „.. the boridingof Ti alloys are generally carried out at 1000 – 1200 o C [J53]” – p.5349.J53-c6. J.Li, X.J. Lü, Y.Q. Lai, Q.Y. Li, Y.X. Liu: Research progress in TiB 2 wettable cathode for aluminumreduction - JOM, August 2008, pp.32-37 – „Coatings were also deposited from the Na 3 AlF 6 – Al 4 B 2 O 9 -TiO 2 and Na 3 AlF 6 – Al 4 B 2 O 9 -CaTiO 3 systems on graphite, glassy carbon, nickel and tungsten cathodes[J53]” – p.34.J53-c7. Simakov D, Vassiliev S, Tursunov P, Khasanova N, Ivanov V, Abakumov A, Alekseeva A, Antipov E,Tsirlina G: Electrodeposition of TiB2 from cryolite-alumina melts - LIGHT METALS 2008, ed. byDeYoung DH, 2008, TMS, pp. 1019-1022. – „Devyatkin et al. [J53] reported a principal possibility oftitanium diboride electrodepostion on various metals from cryolite melt with addition of titanium andboron oxygen-containing compounds. This bath composition is already similar to alumina-cryolite melt,as some oxofluoride complexes surely appear.” – p. 1019. „As it follows from literature [J53],complications can go with high volatility of boron fluoride compounds and from formation of passiveinsulating TiO film when titanium compounds in the melt are partly reduced” – p. 1020.J53-c8. Stojanovic, M.Toplicevic, S.Ristic: Depozicija boridnih slojeva na neke obojene metale – ZastitaMaterijala, 2011, vol.52, pp.295-300. – “Celikkan i saradnici su pokusali da boriraju legure Tielektrohemijskom metodom na sobnoj temperaturi pracenom processom otpustanja na mnogo nizimtemperaturama od onih prijavljenih u literaturi [J53] - p.297.J53-c9. G.V.Arkhipov, Y.S.Gorlanov: Development of technology for producing a wettable coating on a carboncathode by electrodeposition – Light Metals 2012, ed. by C.E. Suarez, TMS, pp.1367-1372. „Since1993, G.Kaptay and S.V.Devyatkin, under laboratory conditions, started to research on synthesis ofborides of high-melting metals from molten salts. They were among the first researchers who set a goalof proving the possibility of electrodeposition of TiB 2 from Na 3 AlF 6 -Al 2 O 3 -TiO 2 -B 2 O 3 melts. Theirattempts to create wettable coatings on carbon and metallic cathodes ended at the laboratory level[J53]” – p. 1367.59

J52. Z.Benkő M., Kaptay Gy.: Az LD-konverter anyagmérlege – BKL Kohászat, vol.133(2000) 6-7, pp. 241-248. (IF = 0)J51. G.Kaptay: Further Discussion of „Particle Engulfment and Pushing by SolidifyingInterfaces: Part II. Microgravity Experiments and Theoretical Analysis” – Metall. Mater.Trans. A, vol.31A (2000), 1695 – 1700. (IF = 1,361)J51-c1: D.M.Stefanescu, A.Catalina, S.Sen, F.R.Juretzko, B.K.Dhindaw, P.A.Curreri: Authors’ Reply,Metallurgical and Materials Transactions A, vol.31A (2000), 1700–1705. – „This communication iswritten in response to Kaptay’s criticism [J51]…” 5 oldal válasz.J51-c2. L.Hadji: Thermal force induced by the presence of a particle near a solidifying interface – Phys. Rev. E.,2001, vol.64, 051502/1-6 – “… Other studies have simply considered ad-hoc expressions for the dragforce that also include the thermal conductivities of the particle and the melt. These approaches areincorrect because they yield expressions for the hydrodynamic drag force that depend on the thermalproperties of the particles and thus make no sense physically. For instance, modified formulas for thedrag force have been derived, which show that the force vanishes when the particle is perfectlyinsulating. We refer the reader to the recent papers by Kaptay [J51] and to references therein for athorough discussion of results obtained using this approach. “ – p.5 (Note: this is the first publicrecognition that my discussion papers were written on a matter to be discussed – moreover, this iscoming from the same University where the original paper of Stefanescu was written)J51-c3. L.Hadji: Particle engulfment in crystal growth: the thermal puzzle – Current Topics in Crystal Growthresearch, 2002, vol.6, pp.95-104.J51-c4. J.W.Garvin, H.S.Udaykumar: Drag on a particle being pushed by a solidification front and itsdependence on thermal conductivities - J. of Crystal Growth, 2004, vol.267, pp.724-737 “Still underdebate [J51] is the issue of the proper form of the drag law when the solidification interface is no longerplanar…”- p.727J51-c5. DM Stefanescu: The multidisciplinary facets of particle engulfment and pushing – Trans Ind Inst.Metals, 2007, vol.60, No2-3, pp.79-86J51-c6. D.M.Stefanescu: Science and Engineering of Casting Solidification, 2nd edition, Springer, NY, 2009,395 pp. – „The main problem is the formulation and calculation of delta sigma. In spite of extensiveefforts and sometimes bitter debate [J51], it is clear that because of the uncertainties int he evaulation ofthe various interfacial energies, deltasigma is at best a fitting parameter – p.289.J50. M.S.Yaghmaee, G.Kaptay, G.Jánosfy: Equilibria in the liquid ternary Fe-B-N system –Materials’ World (e-journal with ISSN 1586-0140, accessible at: http://materialworld.unimiskolc.hu),April, 2000. (IF = 0)J49. M.S.Yaghmaee, G.Kaptay, G.Jánosfy: Equilibria in the Ternary Fe-Al-N System –Materials Science Forum, vols 329-330 (2000) 519-524. (IF = 0.597)J49-c1. G.Effenberg (editor): Landolt-Börstein - Numerical Data and Functional Relationships in Scinece andTechnology. New Series, Group IV: Physical Chemistry, Vol. 11A2. Ternary alloy systems. Phasediagrams, crystallographic and thermodynamic data. Subvolume A: Light Metal Systems. Part 2:Selected systems from Al-Cu-Fe to Al-Fe-Ti. Springer, 2005. The Al-Fe-N system: … These resultswere confirmed by the model of ideally associated mixture proposed by [J49]” – p.310J48. G.Kaptay, E.Báder, L.Bolyán: Interfacial Forces and Energies Relevant to Production ofMetal Matrix Composites – Materials Science Forum, vols. 329-330 (2000) 151-156. (IF =0.597)J48-c1. N.Babcsán: Ceramic Particle Stabilized Aluminum Foams – PhD Dissertation, Miskolc, 2003 – “Table 7.Surface tension of pure and alloyed Al and its additives, based on [J11] – {Table on and d/dT ofliquid Al, Mg, Si, Zn, Mn, Cu, Cr, Ni, Fe}” – p.23., “Table 10. Contact angle of pure Al melt / particle /gas interface [J48] {Table for TiB 2 , WC, TiC, BN, SiO 2 , SiC, graphite, Al 2 O 3 , TiN} – p.25, “Surfaceconcentration of alloying elements doesn’t yield significant effects on surface tension in aluminum[J48]” – p.81.J48-c2. T.Wübben: Zur Stabilität flüssiger Metallschaume – Universität Bremen, Germany, 2003, 128 pp. (ref.No.73) – „Aufgrund ihres Kontaktwinkels von SiC/Al = 27 – 400 [J48] ...” – p.3460

J48-c3. Blücher J., Dobránszky J.: Kompozithuzallal erősített alumínium duplakompozitszerkezetek – BKLKohászat, 2003, vol.136, No.5, pp.213-217 – „A méretkorlátokhoz társul egy másik jelentős problémais: az infiltrációs folyamatok nagy nyomásából és nagy hőmérsékletéből adódó hosszú expozíciós idő,amely alatt határfelületi reakciók mehetnek végbe az erősítőszálak és az olvasztott vagy megszilárdult,de még mindig nagy hőmérsékletű mátrix között [J48]” – p.213.J48-c4. O.P.Uteza, E.G.Gamaly, A.V.Rode, M.Samoc, B.Luther-Davies: Gallium transformation underfemtosecond laser excitation: Phase coexistence and incomplete melting - Physical Review, B 70,054108 (2004) – “Transformation into the new phase would be energetically favored at the interfaceprovided the surface tension between the liquid Ga and silica is lower than that between the silica andcrystal-liquid gallium interface [J48]….the surface tension between the crystal and liquid Gallium is720 dyne/cm [J48]” – p.10.J48-c5. J.T.Blucher, J.Dobranszky, U.Narusawa: Aluminium double composite structures reinforced withcomposite wires – Mater. Sci. Eng., 2004, vol.A387-389, pp.867-872 – „..successful infiltration ofcarbon fibers without special surface treatments was sporadic. … Al 2 O 3 , SiO, TiN. TiB as well as Cu anNi coatings all show promising results [J48]” – p.868.J48-c6. N.Babcsán, J.Banhart, D.Leitlmeier: Metal foam – manufacture and physics of foam – Materials World,e-journal, 2005, vol.6, No.1 – “non-oxidized TiB 2 contact angle is 0 o [J48]” – p.12.J48-c7. C.Körner, M.Arnold, R.F.Singer: Metal foam stabilization by oxide network particles – Mater. Sci. Eng.,2005, vol.A396, pp.28-40.: “The equilibrium contact angle between liquid aluminium and Al 2 O 3 wasdetermined as 63 o at 1100 o C in [J48]” – p.34.J48-c8. N.Babcsán, D.Leitlmeier, J.Banhart: Metal foams – high temperature colloids. Part I. Ex situ analysis ofmetal foams – Colloids and Surfaces A, 2005, vol.261, pp.123- 130 – “TiB2 was chosen, as its contactangle is 98 o at 900 o C in pure Al [..], although we are aware that non-oxidized TiB2 contact anglereported to be 0 o as well [J48]” – p.127J48-c9. A.Ender, H.van den Boom, H.Kwast, H-U. Lindenberg – Metallurgical development in steel-plantinternalmulti-injection hot metal desulphurozation – Steel Research Int.,, 2005, vol.76, ppp.562-572 –„The basic principles for calculating or estimating adhesion energies and interfacial tensions aredescribed by Kaptay [J48]” – p.570J48-c10. N.Babcsán, J.Banhart: Metal Foams – towards high-temperature colloid chemistry – Chapter 11 in:„Colloidal particles at Liquid Interfaces, ed. By B.P.Binks, T.S.Horozov, Cambridge University Press,2006, pp.445-499 – „At the melting point, typical surface tensions of oxide-free and oxidised Al meltsare 1184 and 865 mNm -1 respectively [J48]” – p.462. „Some examples for the contact angle of pure Almelt / particle / gas systems at 1100 o C (no oxide layer on liquid Al, purified Ar atmosphere at 10 -8 barresidual pressure) are summarized in Table 11.7. Table 11.7 taken from ref. [J48].” – p.468.J48-c11. Kientzl I, Dobránszky J, Ginsztler J: Effect of Production Parameters on the Properties of CompositeWires - In: Papp É, Mácsay I, Holubetz L, (szerk.) Gépészet 2006 Proceedings of Fifth Conference onMechanical Engineering, Budapest University of Technology and Economics, National TechnicalInformation Centre and Library, Budapest, 2006, CD-ROM – „The looked-at wires were Nextel 440,oval cross-section fibre-reinforced Al 99.99 matrix composites [J48]” – p.3.J48-c12. I.Kientzl, I.Orbulov, J.Dobranszky, A.Németh: Mechanical behaviour Al-matrix composites wires indouble composite structures – in: „Advanced Inorganic Fibrous Composites V”, 2006, ttp, Switzerland,pp. 147-152 – „The effect of insufficient wetting between the carbon fibres and aluminium was anothercause of strength decreasing [J48]” – p. 152.J48-c13. I.Kientzl, J.Dobránszky: Production and examination of double composites – Mater Sci Forum, 2007,vol.537-538, pp.191-197.61

J48-c14. Yaghmaee MS, Shokri B: Effect of size on bulk and surface cohesion energy of metallic nano-particles- Smart Mater & Structures, 2007, vol. 16 (2), pp. 349-354 – „Surface related factors have been takenfrom [J48].” – p.351.J48-c15. N.Babcsán, G.S. Vinod Kumar, B.S.Murty, J.Banhart: Grain refiners as liquid foam stabilizers – Trans.Indian Inst. Met., 2007, vol.60, pp.127-132. – „Kaptay has reported the contact angle of TiB 2 and TiCwith Al in vacuum at 1100 o C as 0 and 10 0 , respectively [J48]. Though the conditions of foaming in thepresent study are different from the above conditions, one can get a rough idea of the wettability of thetwo particles from the above report.” – p.130.J48-c16. M.S. Yaghmaee, B. Shokri: Surface binding stability of metallic nanoparticles – Plasma ProcessPolym, 2007, vol.4, pp.5891-5896 – „The fundamental bulk thermodynamic parameters, surfacerelated factors and other data have been taken from Barin handbook and Kaptay et al [J48]respectively” – p.5894.J48-c17. ZF Xu, H Yu, ZT Wang, YH Zheng, MZ Hu, CC Cai, QS Yan: The properties thermal expansion andprocess of high volume fractions SiCp/Mg composites by vacuum-gas pressure infiltration – J.Functional Mater, 2007, VOL. 38, NO.10, PP.1610-1617 (NO.5) – „CHINESE TEXT…” – P.1610.J48-c18. JH An: Thermal stress induced voids in nanoscale Cu interconnects by in-situ TEM heating – PhDDissertation, University of texas at Austin, December 2007 – „Table 5.1. Energy values forcalculating change in free energy for void formation, SiN x surface energy [J48]” – p.155.J48-c19. N.Babcsán, B.S.Murty, G.S.Vinod Kumar, F.Garcia Moreno, J.Banhart: New foam stabilizingadditive for aluminium. In: METFOAM-2007, ed. by L.P.Lefebre, J.Banhart, D.C.Dunand, DEStechPubl. Inc, 2008, pp.27-30. – „Data on the wettability of TiAl3 by Al is not available, while Kaptay[J48] has reported the contact angle of TiB2 and TiC with Al in vacuum at 1100 oC as 0 and 10degrees, respectively.” – p.29.J48-c20. Zoltai László (+Dúl Jenő): Grafitcsírák keletkezési lehetőségének elméleti vizsglata – 3.kutatószemináriumi dolgozat, Miskolci Egyetem, 2009. február, 48 oldal – „Az irodalmi érték: SiC-g =2040 – 0.1T mJ/, 2 [J48]” – 30.o.J48-c21. A.V.Biakova, V.P.Krasovskii, A.O.Dudnik, S.V.Gniloskurenko, A.I.Sirko: O roli smachivaemosti Iraspredeleniia tviordich chastic v stabilizacii vspenennich aliuminievich rasplavov – Adgeziia rasplavovI paika materialov, 2009, vip.42, pp.5-22. – “Bolshinstvo opublikovannich v literaturedannich popoverhnostnomu natiazheniu binarnich I mnogokomponentnich aliuminievich rasplavov otnositsia koblasti temperature, namnogo previshaiushich temperature vspenivaniia [J48]” – p.8.J48-c22. B.A:Cook, A.M.Russell, J.Peters, J.L.Harringa: Estimation of surface energy and bonding betweenAlMgB14 and TiB2 – J Phys Chem Sol, 2010, vol.71, pp.824-826 – „In order to compare this withavailable publishe values for surface eneryg of TiB2, ZrB2 and HfB2 at 1300 K [J48], the T-dependence must be factored in…. Eq.(3), as derived from Kaptay [J48]…. + 10 lines” – p.3/3. “Fig.3.Estimated temperature dependence of average surface energy in single phase AlMgB14. referencevalues from Kaptay [J48]” – p.826J48-c23. A.Chamaani, E.Marzbanrad, M.R.Rahimipour, M.S. Yaghmaee, A. Aghaei, R.D. Kamachali,Y.Benhamian: Thermodynamics and molecular dynamic investigation of a possible new critical size forsurface and inner cohesive energy of Al nanoparticles – J Nanopart Res, 2011, vol.13, pp.6059-6067 –„For an implicit analysis of the fundamental bulk thermodynamic parameters, surface-related factorsand other data have been taken from the Barin handbook and Kaptay et al. [J48]” – p.6062.J48-c24. S.Asavavisithchai, AR Kennedy: In-situ oxide stabilization development of aluminum foams in powdermetallurgical route - High Temp Mater Process, 2011, vol.30, No.1-2, pp.113-120. – “Contact anglebetween Al2O3 and Al have been reported to be … 63 degrees at 1373 K [J48]” – p.119.J48-c25. Lévai Gábor (tud. vez.: dr. Török Tamás): Acéllemezek színes tűzi horganyzása, 6. doktoriszeminárium, 2011, június 14., 28 oldal. – “Kaptay és mtsai szerint a cink felületi feszültsége 820mJ/m 2 , a titán oxidé ezzel szemben csak 600 mJ/m 2 . Ennek köszönhetően a titán oxid felületifeszültsége kisebb a cinkénél [J48]”. – pp.21-22.J48-c26. Z.G. Zhang a,., Y.J. Wanga, L.J. Xiao a, L.Q. Zhang a, Y. Sub, J.S. Lin: High-temperature oxidation ofhot-dip aluminizing coatings on a Ti3Al–Nb alloy and the effects of element additions – CorrosionScience, 2012, http://dx.doi.org/10.1016/j.corsci.2012.07.009 - „No report about the effect of Mn on thesurface tension of Al can be used to discuss the wettability. The order of the surface tension of puremetal at melting point is Al = Mn > Ag > Si [J48], so the effect of Mn on the surface tension of Almight be complicated.”J47. Kaptay: Interfacial Criteria to Avoid Pushing of Particles during Solidification of MetalMatrix Composites – Materials Science Forum, vols 329-330 (2000) 121-126. (IF = 0.597)J47-c1. J.T.Blucher, J.Dobranszky, U.Narusawa: Aluminium double composite structures reinforced withcomposite wires – Mater. Sci. Eng., 2004, vol.A387-389, pp.867-872 – „..successful infiltration of62

carbon fibers without special surface treatments was sporadic. … Al 2 O 3 , SiO, TiN. TiB as well as Cu anNi coatings all show promising results [J47]” – p.868.J47-c2. W.Xi, R.L. Peng, W. Wu, N. Li, S. Wang, S. Johansson: Al 2 O 3 nanoparticle reinforced Fe-based alloyssynthesized by thermite reaction – J Mater Sci, 2012, vol.47, pp.3585-3591 – „Ahead of thesolidification front, deltasigma was calculated to be 0.85 J/m2 using the following equation [J47]:Eq.(3)” – p.3588.J46. G.Kaptay, S.A.Kuznetsov: Electrochemical synthesis of refractory borides from moltensalts – Review paper – Plasmas & Ions, 2 (1999) 45-56. (IF = 0)J46-c1. H.B.Kushov, A.S.Uzdenova, M.K.Vindizheva, A.V.Zimin: Study of joint electroreduction of complexgadolinium (or lanthanum) ions with tetrafluoroborate-ions in halide melts – Advances in Molten Salts,2000., vol.1., pp. 291-297 …”Borides of rare earth metals have been synthesized in this way in worksof Andrieux […] (see also review [J46])…” - p. 291, „…It should be mentioned that there is noinformation on the electrosynthesis of GdB 6 and GdB 4 phases in the literature [J46].” – p.295.J46-c2. S.V. Devyatkin: Influence of different conditions of electrochemical synthesis on the structure of thedeposited refractory compound coatings, Materials’ World (e-journal, http://materialworld.unimiskolc.hu,July, 2001 – “The results of Baraboshkin [..] obtained mainly for single metallic deposits,were extrapolated to refractory boride phases in [OJ36]” - p.1, “..This is characteristic toelectrochemical synthesis of tantalum diboride. In this case the layered type of coating structure hasbeen obtained (see Fig. 3) […]. The formation of this structure has been theoretically explained [J46]using the Equilibrium Electrochemical Synthesis (EES) Diagrams […]” – p. 3.J46-c3. J. Sytchev, H. Kushkhov: Voltammetric Investigation of the Reduction Processes of Nickel, Cobalt, andIron Ions in Chloride and Chloro-Fluoride Melts, Materials’ World (e-journal, http://materialworld.unimiskolc.hu,July, 2001 – “High-temperature electrochemical synthesis from molten salts is a veryperspective way to produce compounds of high purity, including borides [J46]”, p.1.J46-c4. L.P.Polyakova, E.G.Polyakov, O.V.Makarova, A.A.Shevirev, N.I.Bierrum: Elektrochimicheskii sintezboridov tantala v beskislorodnich i kislorodcoderzhashich ftoridnich rasplavach – Elektrokhimiia, 2001,vol. 37., pp.1451-1457: „V etoi sviazi strannoui vigliadit poziciia avtorov raboti [J46], schitaiushich,shto nabliudaiemaia struktura sostoit iz chereduiushichsia sloiev TaB i TaB 2 …” – 1454J46-c5. Kh.B.Khushkhov, M.K.Vinidzheva, A.S.Uzdenova, Z.A.Zhanikaeva: Joint electroreduction oflanthanum, gadolinium and boron in halide melts – J. of Mining and Metallurgy, 2003, vol.39B,pp.275-280 – “Single borides of rare-earth metals were synthesized in the works of Andrieux [..] (seealso review[J46])” – p.278.J46-c6. P.Taxil, P.Chamelot, L.Massot, C.Hamel: Electrodeposition of alloys or compounds in molten salts andapplications – J. of Mining and Metallurgy, 2003, vol.39B, pp.177-200 – „Kaptay and Kuznetsov usedequations similar to Eq.7 to calculate equilibrium potentials of the boride systems in molten salts [J46].Thermodynamic data allow these authors to elaborate so-called Electrochemical Equilibrium Synthesis(EES) diagrams where the stability of the compounds of the system B/Me is defined as a function oftemperature and the depolarization term which is the second term of Eq.(5); hence these diagramsdisplay the stability of each compound of systems such as Ti/B in areas delimited by boundary linesgiven by Eq.5 computed in the temperature scale adapted to the process of preparing these alloys” –p.183.J46-c7. H.B.Kushkhov, M.K.Vinizheva, A.S.Uzdenova, Z.A.Zhanikaeva: Joint electroreduction of lanthanum,gadolinium and boron in chloride melts – Electrochemical Society Proceedings vol.2002-19, pp.616-621 – “Rare earth metal borides were first synthesized by Andrieux (see also review [J46])” – p.618J46-c8. J.H. von Barner, P.Noye, A.Barhoun, F.Lantelme: Influence of oxide and alloy formation on theelectrochemistry of Ti deposition from the NaCl-KCl-NaF-K 2 TiF 6 melt, reduced by metallic Ti –J.Electrochem.Soc., 2005, vol.152, pp. C20-C26. “Kaptay and Kuznetsov [J46] give references to mostof the work done so far on TiB 2 deposition from molten salts in a recent review.” – p.C20.J46-c9. V.V.Malishev: Visokotemperaturnii elektrochmnicheskii sintez metallo-podobnich tugoplavkichsoedinenii metallov IV – VIA grupp v ionnich rasplavach – Zh. Neorg. Himii, 2004, vol.48, pp.187-194– “V obzore [OJ36] sistematizirovai raboti po elektrochmicheskomu sintezu boridov tugoplavkichmetallov, opisani metodi beztokovogo I elektrochmicheskogo borirovaniia. S pomoshiu ravnovesnichelektrochmicheskich diagram sinteza avtori [J46] ocenivaiut veroiatnost VES boridov 24 perehodnichmetallovi predskazivaiut ich vozmozhnuiu morfologiu” – p.190.J46-c10. V.V.Malyshev: Zashitnie pokritiia tugoplavkimi soedineniiami metallov IV-VIA grupp, nanosimie izionnich rasplavov (obzor) – Zashita metallov, 2004, vol.40, pp.584-600 - „pervie popitki sozdat iobobshit material predpriniati poka lish v statiach V.I.Shapovala i posledovatelei [J46]” – p.58463

J46-11. V.V.Malyshev, Kh.B.Kushkhov: Advances in high-temperature electrochemical synthesis in ionic meltsby the onset of XXI century – Russ J. of General Chem., 2004., vol.74, pp.1139-1146 (Zh. ObsheiHimii, 2004, vol.74, pp.1233-1240) – „Using „equilibrium electrochemical synthesis diagrams”, Kaptayet al [J46] assessed the probability of high-temperature electrochemical synthesis of borides of 24transition metals and predicted their possible morphology” – p.1142.J46-c12. J.Li, B.Li, Z.Dong: Electrodeposition of [001] oriented TiB 2 coatings – Materials Letters, 2005, vol.59,pp.3234-3237 – “As compared with other possible techniques of production of refractory borides,molten salts generally can be considered as a very promising medium for chemical and electrochemicalsynthesis of different refractory borides [J46]” – p.3234J46-c13. Li Jun, Li Bing, Dong Zheng’e: Preparation of the TiB 2 coatings by electroplating in moloten salts –Rare Metals, 2005, vol.24, pp.261-266 - – “Molten salts generally can be considered as a verypromising medium for chemical and electrochemical synthesis of different refractory borides. ascompared with other possible techniques of production of refractory borides, [J46]” – p.261J46-c14. Li B, Jiang LS, Li J: Pulse electrodeposition of titanium diboride in LiF-NaF-KF melts, J Rare Earths,2005, vol. 23, pp. 66-71. - „Electrochemical synthesis has some advantages as compared with otherpossible techniques of production of refractory borides [J46]: i. smooth coatings can be deposited evenat surfaces of complicated geometry, ii. Single crystals, polycrystalline coatings and even ultradispersepowders can be deposited, iii. the composition of the deposit can be precisely controlled throughprocess parameters, iv. relatively low temperatures of synthesis, cheap and simple technologicalbackground and cheap raw materials required make the process attractive from the economic point ofview” – p.66.J46-c15. Gaune-Escard M: Thermodynamics of lanthanide halides and application to high-temperature processes– Scand J Metall, 2005, vol. 34, No. 6, pp. 369-375. - “Electrochemical synthesis in molten salts wasshown to be a promising method for rare earth compounds production. It is very suitable forelectrodeposition of protective coating on massive samples of complex shapes [J46].” – p.373.J46-c16. Kartal G, Timur S, Arslan C: Effects of process current density and temperature on electrochemicalboriding of steel in molten salts - J Electronic Mater, 2005, vol. 34, No. 12, pp. 1538-1542. – “Althoughelectrochemical boriding has been studied since the 1940-s, limited research exists in English languageliterature [J46]. Nevertheless, electrochemical boriding produces thicker coating in shorter times ascompared to the thermochemical birodong techniques” – p.1538.J46-c17. L.Jiang, B.Li, J.Li: Electrodeposition of titanium diboride coating from molten salts containing oxideelectrolyte – Chinese Journal of Rare Metals, 2005, vol.29:22, No.4, pp.162-166 – Chinese text….J46-c18. Li J, Li B, Jiang LS, Dong Z, Ye YF: Preparation of highly preferred orientation TiB2 coatings – RareMetals, 2006, vol. 25, No. 2, pp. 111-117 – … electrochemical synthesis of refractory borides frommolten salts has the following advantages [J46]: …” – p.111.J46-c19. Li J, Li B, Jiang LS, Ye YF, Dong ZE: Preparation of TiB2 coatings by electroplating in KF-KClmolten salt – Rare Metal Mater Eng, 2006, vol. 35, No. 4, pp. 629-633 – “Molten salts generally can beconsidered as a very promising medium for chemical and electrochemical synthesis of differentrefractory borides, as compared with other possible techniques of production of refractory borides[J46]” – p.629.J46-c20. Li J, Li B: Preparation and characterization of highly preferred orientation TiB2 coatings - Rare MetalMater Eng, 2006, vol. 35, No 5, pp. 832-835 – Chinese text??J46-c21. Jun Li, Bing Li: Preparation of the TiB2 coatings by electroplating in molten salts – Mater Letters,2007, vol.61, NO. 6, pp. 1274-1278 – „As compared with other possible techniques of production ofrefractory borides, electrochemical synthesis from molten salts generally can be considered as a verypromising technique for refractory borides [J46]” – p. 1274.J46-c22. Li J, Li B: Electrochemical reduction and electrocrystallization process of B(III) in the LiF-NaF-KF-KBF4 molten salt – Rare Metals, 2007, vol. 26, No. 1, pp. 74-78 – „Molten salts can be generallyconsidered as a promising medium for the chemica land electrochemical synthesis of TiB 2 , as comparedwith other possible techniques for the production of refractory borides [J46]”- p.74.J46-c23. Celikkan H, Ozturk MK, Aydin H, Aksu ML: Boriding titanium alloys at lower temperatures usingelectrochemical methods – Thin Solid Films, 2007, vol. 515, No. 13, pp. 5348-5352 – „Kaptay et al.have explained the electrochemical boriding process in detail [J46].” – p.5348.J46-c24. Devyatkin SV: Electrochemical synthesis of binary and ternary refractory compounds in the system Ti-Si-B from chloride-fluoride melts – Z. Naturforsch A, 2007, vol. 62, No. 9, pp. 524-528 „Kaptay andKuznetsov have reviewed the published papers on electrochemical synthesis of titanium diboride inmolten salts [J46]” – p.524.J46-c25. Y Ban, Z Wang, Z Shi, H Kan, S Yang, X Cao, Z Qiu: Preparation of TiB 2 inert cathode on graphite byelectrodeposition process for aluminum electrolysis – Light Metals, 2007, pp.1055-1060.64

J46-c26. E.Bilgi, H.E.Camurlu, B.Akgün, Y.Topkaya, N.Sevinc: Formation of TiB 2 by volume combustion andmechanichemical process – Mater Res Bull, 2008, vol.43, pp.873-881 – “Fused salt electrolysis [J46] isanother technique for production of titanium diboride” – p.873.J46-c27. V.Malyshev, A.Gab, M.Gaune-Escard: Initial stages of nucleation of molybdenum and tungsten carbidephases in tungstate-molybdate-carbonate melts – J Appl Electrochem, 2008, vol.38, pp.315-320 – „Theresults of related investigations for electrodeposited Mo and W were presented earlier [J46]” – p.315.J46-c28. K.Amalajyothi, L.J.Berchmans, S.Angappan, A.Visuvasam: Electrosynthesis of cerium hexaboride bythe molten salt technique – J Crystal Growth, 2008, vol.310, pp.3376-3379 – “the combined depositionof two electro-active species at the potential more positive than their own deposition potentials at theinert cathode is possible due to their high exchange current density of the cations in the molten salts[J46]” – p.3378.J46-c29. N.Rybakova, M.Souto, H.P.Martinz, Y.Andriyko, W.Artner, J.Godinho, G.E.Nauer: Stability ofelectroplated titanium diboride coatings in high-temperature corrosive media – Corrosion Science,2009, vol.51, pp.1315-1321 – „The electrodeposition of TiB 2 from molten salts is significantly faster,less expensive and permits to obtain well defined and smooth deposits on different substrates withcomplicated surface profiles and homogeneous layer thickness [J46]” – p. 1315.J46-c30. H.Cellikan, A.E.Sanli, H.Aydin, M.L.Aksu: Mechanism of boron tribromide electrodeposition – J ApplElectrochem, 2009, vol.39, pp.1525-1533. – “The boronizing process can be carried out thermally or bythe electrolysis of molten salts [J46]” – p.1525.J46-c31. T.P. Jose, L. Sundar, L.J. Berchmans, A. Visuvasam and S. Angappan: Electrochemical Synthesis andcharacterization of BaB 6 from molten melt - Journal of Mining and Metallurgy, 2009, vol. 45 B, No.1,pp. 101 – 109. – “It is emphasized that coatings with relatively stable stoichiometry can also beobtained, if one should keep the composition of the melt constant and to keep the growing boride phaseideally planar during the process. This would ensure a constant ratio of partial current densities of thetwo components of the boride during the deposition process. Boron and metal atoms both are depositedat more positive potentials than their own equilibrium deposition potentials usually get dissolved in themelt again. But, if such unstable boron and metal atoms appear to be in contact, they will stabilize eachother with the formation of the stable boride phase [J46].J46-c32. A.Güven, B.Fiedrich: Electrochemical titanium diboride (TiB2) synthesis from fluoride melts – ProcEMC, 2009, pp.1-12. „Table 1. Electrochemical production parameters of some metal borides [J46]” –p.3.J46-c33. G. Kartal, S. Timur, M. Urgen, A. Erdemir: Electrochemical Boriding of Titanium for ImprovedMechanical Properties - Surface Coating Technol., 2010, vol.204, pp.3935-3939 – „… there are studiesrelated to the boriding possibilities of of non-ferrous metals and alloys [J46]” – p.3935.J46-c34. G.Kartal, S.Timur, O.L.Erylmaz, A.Erdemir: Influence of process duration on structure and chemistryof borided low carbon steel – Surface Coating Technology, 2010, Volume 205, Issue 5, pp 1578-1583 –“Electrochemical boriding has not attracted much attention and very limited number of publicationappeared in the open literature [J46]” – p.1581.J46-c35. L.J. Berchmans, A. Visuvasam, S. Angappan, C. Subramanian, A.K. Suri: Electrosynthesis ofsamarium hexaboride using tetra borate melt - Ionics, 2010, vol.16, pp.833-838. – “It is explained byKaptay and Kuznetsov that the formation of metal borides occurs by the joint deposition of twocomponents.” – p.837.J46-c36. G.Kartal, O.L.Erylmaz, G.Krumdick, A.Erdemir, S.Timur: Kinetics of electrochemical boriding of lowcarbon steel – Appl. Surf. Sci, 2011, vol.257, pp.6928-6934 – “The majority of researches inelectrochemical boriding have primarily focused on the effects of electrolyte composition, currentdensity, and boriding temperature on the structure and composition of resultrant boride layers [J46]” –p.6928.J46-c37. O.Kahvecioglu, V.Sista, O.L.Eryilmaz, A.Erdemir, S.Timur: Ultra-fast boriding of nickel aluminide –Thin Solid Film, 2011, vol.520, pp.1575-1581 “… the diffusion of boron into the Ni 3 Al substrate beingthe rate limiting step [J46]” – p.1577J46-c38. X.Cao, H.Wang, X.Meng, C.Wang, H.Yang, X.Xue: High temperature electrochemical synthesis oftungsten boride from molten salt – Adv mater Res., 2011, vol.206-307, pp.463-466. – „The synthesiscondition is as follows [J46]: Eq.(2)…” – p. 465.J46-39. Z.Stojanovic, M.Toplicevic, S.Ristic: Depozicija boridnih slojeva na neke obojene metale – ZastitaMaterijala, 2011, vol.52, pp.295-300. – “Celikkan i saradnici su pokusali da boriraju legure Tielektrohemijskom metodom na sobnoj temperaturi pracenom processom otpustanja na mnogo nizimtemperaturama od onih prijavljenih u literaturi [J46]”- p.297.J46-c40. V.Pavlik, M.Boca: Corrosion of titanium diboride in molten FLINAK(eut) – Chemical Papers, 2012,doi: 10.2478/s11696-012-0202-y. – „Titanium diboride … is considered for the use in the process of65

aluminium production in Gereration IV molten salts nuclear reactors probably as coating layer on thetemperature stressed probes [J46]” – p.1.J45. B.Tury, J.I.Sytchev and G.Kaptay: Morphology of titanium diboride obtained byelectrochemical synthesis from molten chloro-fluoride melt - High Temperature MaterialProcesses, 1999, vol.3, p.117-126. (IF = 0.345)J45-c1. S.V. Devyatkin: Influence of different conditions of electrochemical synthesis on the structure of thedeposited refractory compound coatings, Materials’ World (e-journal, http://materialworld.unimiskolc.hu,July, 2001 – “When the pulse technique is used, irregularities can be ‘cut’ and the planarcrystallisation front can be maintained for a coating with larger thickness. This method is well knownfor the electro-crystallisation of metals from water based solutions. The same method wasexperimentally proven to provide a smoother surface of the TiB 2 coating, deposited from a chlorofluoridemelt [J45] – p.6. --J45-c2. U.Fastner, T.Steck, A.Pascual, G.Fafilek, GE Nauer: Electrochemical deposition of TiB 2 in hightemperature molten salts – J Alloys Comp., 2008, vol.452, pp.32-35 – „Among all the electrolytesreported int he literature [J45] our work was focused on….. “ – p.32.J44. Báder E., Bolyán L., Kaptay Gy., Báder I.: Határfelületi energiák vizsgálata kerámiafémolvadékrendszerek korróziója szempontjából – Korróziós Figyelő, 1999, 39. évf., 5.szám, 144-146. (IF = 0)J44-c1. Egész Ádám: Magas porozitású Al 2 O 3 kerámiák fejlesztése kartusokhoz és Al-Al 2 O 3 cermetekhez –Diplomamunka, Miskolci Egyetem, Műszaki Anyagtudományi Kar, Kerámia – és SzilikátmérnökiTanszék, 2010. „(38-as hivatkozás): 17. ábra. A peremszög változása a hőntartás függvényében.Átvéve: [J44]” – 26.o.J44-c2. Egész Ádám: Alumínium-Al 2 O 3 kompozitok fejlesztése - TDK dolgozat (konzulens: dr. Gömze László),Miskolci Egyetem, Műszaki Anyagtudományi Kar, Kerámia – és Szilikátmérnöki Tanszék, 2010. „7.ábra. A peremszög változása a hőntartás függvényében [J44]” – 12.o., „A kemence felfűtésefolyamatos, egyenletes, így a mérés végén megkaphatjuk az alumínium peremszögének folyamatosaváltozását az idő, valamint a hőmérséklet függvényében. Egy ilyen megfigyelést és mérést láthatunk a7. ábrán, amely a hőntartás függvényében szemlélteti a peremszög változását. A felvételeket 1100 Cº-onkészítették 0, 60, 300 és 600 másodperces hőntartási idők után. A képeken jól látszik, hogy azalumínium a hevítési idő növekedésével folyamatosan, egyre nagyobb mértékben terül szét azalumínium-oxid kerámia lapon, tehát nedvesíti azt. Ezen tanulmány eredményként azt állapította meg,hogy ezen a hőmérsékleten, 600 másodperces hőntartási idő után az alumínium nedvesítés peremszöge60º alá csökkent az alumínium-oxid kerámián. [J44]”. – 12-13.o.J43. Kelemen K.K., Kaptay Gy., Borsik Á.: Fémhabok – a géptervezés potenciális szerkezetianyagai (Metallic foams – potential structural materials for machine design) – Gép, 1999., 50.évf, 11. szám, 58-61. (IF = 0)J43-c1. Orbulov I., Kientzl I., Németh Á.: Fémhabok és kompozitok előállítása infiltrálásos eljárással – BKLKohászat, 2007, vol.140, No.5, pp.41-46. – „A másik csoportba sorolhatjuk azokat az anyagokat,amelyek létrehozásánál vagy csak a tömegcsökkentés, vagy valamilyen más különleges követelménydominál. Ezek a porózus szerkezeti anyagok [J43]” – p.41.J42. Jánosfy Gy., Kaptay Gy., Szabó Z., Szélig Á.: A túltelítettség szerepe alumíniummalcsillapított, szilíciumszegény lágyacélok (LCAK) fémesaluímium-tartalmánakoxigénszondával történő beszabályozásában - BKL Kohászat, 1999., 132. évf., 6-7. szám,245-249 o. (IF = 0)66

J41. Báder E., Kaptay Gy.: Az öntőporok szerepe az acél folyamatos öntésekor - BKLKohászat, 1999., 132. évf., 6-7. szám, 250-254 o. (IF = 0)J40. G.Kaptay, J.Sytchev: Thermodynamic Properties of Phases and the ElectrochemicalSynthesis Diagram for the Mo-B System - Ukr. Khim. Zh., 1999, vol.65., No.5., pp.34-41. (IF= 0)J39 Kaptay G.: Discussion of „Particle Engulfment and Pushing by Solidifying Interfaces:Part II. Microgravity Experiments and Theoretical Analysis, by D.M.Stefanescu,F.R.Juretzko, B.K.Dhindaw, A.Catalina, S.Sen, P.A.Curreri, published in Metall. Mater.Trans. A, 1998, vol.29A, pp.1697-1706” - Metall. Mater. Trans. A, 1999, vol. 30A, pp.1887-1890. (IF = 0,993)J39-c1. D.M.Stefanescu, F.R.Juretzko, A.Catalina, B.K.Dhindaw, S.Sen, P.A.Curreri: Authors’ Reply toDiscussion of „Particle Engulfment and Pushing by Solidifying Interfaces: Part II. MicrogravityExperiments and Theoretical Analysis” - Metall. and Materials Trans., A, volume 30A, 1999, pp. 1890 -1894 – lásd a a teljes cikketJ39-c2: D.M.Stefanescu, A.Catalina, S.Sen, F.R.Juretzko, B.K.Dhindaw, P.A.Curreri: Authors’ Reply,Metallurgical and Materials Transactions A, vol.31A (2000), 1700–1705. – „This communication iswritten in response to Kaptay’s comments [J39]…” 5 oldal válasz.J39-c3. J.W.Garvin, H.S.Udaykumar: Drag on a particle being pushed by a solidification front and itsdependence on thermal conductivities - J. of Crystal Growth, 2004, vol.267, pp.724-737 “Still underdebate [J39] is the issue of the proper form of the drag law when the solidification interface is no longerplanar…”- p.727J39-c4. DM Stefanescu: The multidisciplinary facets of particle engulfment and pushing – Trans Ind Inst.Metals, 2007, vol.60, No2-3, pp.79-86J39-5. D.M.Stefanescu: Science and Engineering of Casting Solidification, 2nd edition, Springer, NY, 2009, 395pp. – „The main problem is the formulation and calculation of delta sigma. In spite of extensive effortsand sometimes bitter debate [J39], it is clear that because of the uncertainties int he evaulation of thevarious interfacial energies, deltasigma is at best a fitting parameter – p.289.J38. G.Kaptay, J.Sytchev: Thermodynamic Properties of Phases and the ElectrochemicalSynthesis Diagram for the Mo-B System - Ukr. Khim. Zh., 1999, vol.65., No.5., pp.34-41. (IF= 0)J37. Kaptay Gy., Bolyán L.: Kerámiával erősített fémmátrixú kompozitanyagok gyártásánakhatárfelületi vonatkozásai. II/2. Határfelületi energiák adatbank. Anyagpárválasztás. BKLKohászat, 1998. 131. Évfolyam, 9-10 szám, 305-314. (IF = 0)J37-c1. Magyar Anita: Karbon szállal erősített alumínium mátrixú kompozitok Al/C határfelületének jellemzése– PhD értekezés, Miskolc, 2004. – fél oldal szöveg + 1 ábra átvéve a 26. oldalon, plusz: „..magyarázat agázhólyagok keletkezésére … hogy mihelyt a hőmérséklet a 850 – 900 C-os tartoményba emelkedik(ún. kritikus hőmérséklet [J37]), az Al reakcióba lép az Al 2 O 3 -al Al 2 O gáz keletkezése közben [J37].” –p.57.67

J37-c2. Janó V., Buza G., Kálazi Z.: Diszperz eloszlású, fémmátrixú kerámia kompozitréteg létrehozásalézersugaras felületkezeléssel – BKL Kohászat, 2005., 138. évf., 3. szám, 39-44.J37-c3. Kientzl Imre: Alumínium mátrixú duplakompozit szerkezetek gyártása és vizsgálata – Diplomaterv,BME (konzulens: Dobránszky János), 2005, Bp., 110o. – „16 egyenlet, 6 ábra, 7 táblázat, összesen 11oldal átvéve [J37] „ – 32-42. o.J37-c4. Orbulov I., Kientzl I., Németh Á.: Fémhabok és kompozitok előállítása infiltrálásos eljárással – BKLKohászat, 2007, vol.140, No.5, pp.41-46. – „Nagyon fontos, hogy a fémmátrixú kompozitanyagokesetében is csak akkor kapunk megfelelő műszaki tulajdonságokat, ha megfelelő a kapcsolat azerősítőanyag és a mátrixanyag határfelületén [J37]” – p.41.J37-c5. I.Kientzl, J.Dobránszky: Production and behaviuour of aluminium matrix double composite structures –Mater Sci Forum, 2008, vol.589, pp.105-110 – „The contact angle can be smaller than 140 degdepending on the fact whether there is an oxide layer on the surface of the liquid or not [J37]” – p.107.J37-c6. O.Udvardy, A.Lovas: Dynamic phenomena during sessile drop measurements due to oxide layerdisruption – Mater Sci Forum, 2008, vol.589, pp.173-178 – „The wetting phenomenon between solidsand liquids has an outstanding role in several technological processes [J37]” – p.173.J37-c7. Kientzl I, Dobránszky J: Fabrication Methods of Double Composites. In: Váradi K, Vörös G (eds.),Gépészet 2008, Proceedings of Sixth Conference on Mechanical Engineering, BUTE faculty ofMechanical Engineering, G-2008-J-01. – “The strong bonding has high significance because thecomposite wires covered by alumina skin caused by their aluminium content and there is poor wettingbetween alumina and liquid aluminium [J34]” – p.4/6.J37-c8. Orbulov I.N.: Szintaktikus fémhabok, PhD értekezés (Dobránszky János és Németh Árpád, BME, 2009.június) – „Kaptay és Bolyán összefoglaló műve szerint a peremszöget Al és SiO2, valamint Al2O3között (amelyek a gömbhéjak falanyagát alkotják), a következő, 7. táblázat foglalja össze [J37]. 7.táblázat – 4 számérték a cikkből” – 35.o.J37-c9. Kientzl I.: Alumíniummátrixú kompozithuzalok és kettős kompozit-szerkezetek – PhD értekezés, BME(tud. vez.: dr.Dobránszky János), 2010, 112.o. – Kaptay szerzőtársaival összeállított egy olyanadatbankot, amely nagyszámú fém és kerámiaanyag határfelületi viselkedésére jellemző mérőszámottartalmaz… + 11 sor [J37]” – 28.o.J36. Tury B., Sytchev J., Kaptay Gy.: Elektrokémiai szintézissel előállított TiB 2 morfológiaivizsgálata - Gépgyártástechnológia, 1998., 38. évf., 10. szám, 111-114 o. (IF = 0)J36-c1. R.P.Pawlek: Aluminium Wettable Cathodes: An Update – in: Light Metals 2000, Ed. by R.D.Peterson,TMS 2000, pp. 449-454 – „Tury et al [J36] prepared ceramic TiB 2 by electrolysis at 700 C using amolten salt electrolyte consisting of NaCl, KCl, NaF, KBF 4 and K 2 TiF 6 . The electrolitically preparedTiB 2 has good adherence to the cathode carbon. Compact and homogenous TiB 2 is prepared at currentdensities of 150-300 mA/cm 2 ” á p.449 –J36-c2. Vedernikov G.F.: Inertnie katodi v elektroliziorach dlia proizvodstva aliuminia. Problemi i perspektivi.AO VAMI, Informacionnii listok, No.10, April 2001. – „Tury i dr. [J36] poluchili keramicheskii TiB 2 izrasplava NaCl-KCl-NaF-KBF 4 -K 2 TiF 6 . Poluchennoie elektrochimicheskim putiom pokritie TiB 2kompaktno i odnorodno, horosho prilipaet k ugolnomu katodu” – s.16.J36-c3. Gorlanov ES, Nikiforov SA, Alternative technology to produce a wettable cathode surface layer in Alcells – Proc of the 12 th Int. Conf. “Aluminum of Siberia” (in Russian), Krasnoyarsk, 2006, pp.91-95. –„Naibolee perspektivnii, s popitkoi adaptacii k usloviiam elektroliza v krilito-glinoziomnich rasplavachpredstavlen v rabotach [J36]” – p.92.J35 Kuznetsov S.A., Kuznetsova S.V., Beliaevskii A.T., Devyatkin S.V., Kaptay G.: CathodicProcesses at Electrochemical Synthesis of Niobium Borides from Chloro-Fluoride Melts -Elektrokhimiia (Russian Journal of Electrochemistry), 34 (5) (1998) 520-527. (IF = 0,059)J35-c1. V.V.Malyshev: Zashitnie pokritiia tugoplavkimi soedineniiami metallov IV-VIA grupp, nanosimie izionnich rasplavov (obzor) – Zashita metallov, 2004, vol.40, pp.584-600 - – „az eredmények ismertetése26 + 41 sorban, állásfoglalás nélkül)” – p. 592 and 596J35-c2. O.B.Babushkhina, E.O. Lomako, W. Freyland: Electrochemistry and Raman spectroscopy of niobiumreduction in basic and acidic pyrrolidinium based ionic liquids. Part 1: 1-Butil-1-methylpyrrolidiniumchloride with NbCl 5 – Electrochimica Acta, 2012, vol.62, pp.234-241 – „The following achievementshave been made: …. Alkali fluoride-chloride melts were used as chloride electrolytes with the additiveof K 2 NbF 7 [J35]” – p.234.68

J34. Kaptay Gy., Bolyán L.: Kerámiával erősített fémmátrixú kompozitanyagok gyártásánakhatárfelületi vonatkozásai. II/1. rész. Határfelületi energiák adatbank. Anyagpárválasztás. -BKL Kohászat, 1998, 131. évf., 5-6. szám, 179-185. (IF = 0)J34-c.1. Boross Péter: Karbidkerámia szemcsék viselkedése lézerrel létrehozott olvadéktócsában: TDK dolgozat,2000, tud. vez.: dr. Verő Balázs BAYATI és dr. Hárs György, BME) (ref. No.3, kicsit tévesenmegadva) – „5.táblázat. A vizsgált anyagok felületi feszültsége és hőfoktényezője [J34] (a táblázat 8, acikkemből származó adatot tartalmaz)” – 16.o. „6. táblázat – A megfelelő hőmérsékletre átszámítottfelületi feszültség és adhéziós energia értékek [J34] (a táblázat 18, a cikkemből átvett adatot tartalmaz”– 16.o.J34-c.2. Boross Péter: Lézeres átolvasztással végzett felületmódosítások, Diplomamunka, BME, Bayati, 2001.,tud.vez.: dr. Verő Balázs és dr. Hárs György. “A kerámiákra a [J34] szakirodalom nyomán az egységesközleítő –0,15 J/m 2 K értéket használtam hőfoktényezőként. .. W és cl számítását a [J34] Azirodalomban megadott peremszög - adatokból számoltam… 8.táblázat. A vizsgált anyagok felületifeszültsége és hőfoktényezője [J34].” - p.37.J34-c.3. Boross Péter, Kálazi Zoltán: A lézeres diszpergálás során fellépő jelenségek néhány elméletivonatkozása – BKL Kohászat, 2002, 135. évf., 6-7. szám, 219-223 o. – „A [J34] adatbank alapján azacélolvadékunk és a TiC között nagyjából 70 o -os peremszög van…” 219. o.J34-c4. G.Králik, P.Fülöp, B.Verő, D.Zsámbok: Laser Surface Treatment of Steels – Materials Science Forum,2003, vols.414-415, pp.21-30 – “… based on the work of Gy.Kaptay [J34] we inspected the lawsdetermining the transport of the TiC particles into the molten bath. According to theoreticalconsiderations a particle only submerges into the depth of 2r in the liquid if the wetting is perfectbetween them. Since the wetting only partial between the material and the TiC particle in the presumedthermic and ambiency circumstances the conditions of the particle to travel under the surface of themolten bath are not given.” – p.25J34-c5. Blücher J., Dobránszky J.: Kompozithuzallal erősített alumínium duplakompozitszerkezetek – BKLKohászat, 2003, vol.136, No.5, pp.213-217 – „A méretkorlátokhoz társul egy másik jelentős problémais: az infiltrációs folyamatok nagy nyomásából és nagy hőmérsékletéből adódó hosszú expozíciós idő,amely alatt határfelületi reakciók mehetnek végbe az erősítőszálak és az olvasztott vagy megszilárdult,de még mindig nagy hőmérsékletű mátrix közöt [J34]” – p.213.J34-c6. Magyar Anita: Karbon szállal erősített alumínium mátrixú kompozitok Al/C határfelületének jellemzése– PhD értekezés, Miskolc, 2004. fél oldal bevezető szöveg a cikkem alapján a 23-24 oldalakon,69

J34-c7. Kientzl Imre: Alumínium mátrixú duplakompozit szerkezetek gyártása és vizsgálata – Diplomaterv,BME (konzulens: Dobránszky János), 2005, Bp., 110o. – „16 egyenlet, 6 ábra, 7 táblázat, összesen 11oldal átvéve [J34] „ – 32-42. o.J34-c8. Orbulov I., Kientzl I., Németh Á.: Fémhabok és kompozitok előállítása infiltrálásos eljárással – BKLKohászat, 2007, vol.140, No.5, pp.41-46. – „Nagyon fontos, hogy a fémmátrixú kompozitanyagokesetében is csak akkor kapunk megfelelő műszaki tulajdonságokat, ha megfelelő a kapcsolat azerősítőanyag és a mátrixanyag határfelületén [J34]” – p.41.J34-c9. Verezub O.: Lézeresen felületkezelt szerszámacél köszörülése – Gyártóeszközök, szerszámok,szerszámgépek, 2008, No.1, pp.65-68. – „Az acélolvadékba nem a szerszám felületi rétegébe tervezettTiC-szemcséket vittük be. Ennek bonyolult felületkémiai-hidrodinamikai okait részletesen tartalmazza a[J34] irodalom” – p.66.J34-c10. I.Kientzl, J.Dobránszky: Production and behaviuour of aluminium matrix double composite structures –Mater Sci Forum, 2008, vol.589, pp.105-110 – „The contact angle can be smaller than 140 degdepending on the fact whether there is an oxide layer on the surface of the liquid or not [J34]” – p.107.J34-c11. O.Udvardy, A.Lovas: Dynamic phenomena during sessile drop measurements due to oxide layerdisruption – Mater Sci Forum, 2008, vol.589, pp.173-178 – „The wetting phenomenon between solidsand liquids has an outstanding role in several technological processes [J34]” – p.173.J34-c12. Kientzl I, Dobránszky J: Fabrication Methods of Double Composites. In: Váradi K, Vörös G (eds.),Gépészet 2008, Proceedings of Sixth Conference on Mechanical Engineering, BUTE faculty ofMechanical Engineering, G-2008-J-01 – “The strong bonding has high significance because thecomposite wires covered by alumina skin caused by their aluminium content and there is poor wettingbetween alumina and liquid aluminium [J34]” – p.4/6.J34-c13. Kientzl I.: Alumíniummátrixú kompozithuzalok és kettős kompozit-szerkezetek – PhD értekezés, BME(tud. vez.: dr.Dobránszky János), 2010, 112.o. – „Kaptay szerzőtársaival összeállított egy olyanadatbankot, amely nagyszámú fém és kerámiaanyag határfelületi viselkedésére jellemző mérőszámottartalmaz… + 11 sor [J34]” – 28.o.J33. Kaptay G., Buzinkay E.: Calculation of Equilibrium Electrochemical Synthesis Diagramson an Example of the Titanium - Boron System - Molten Salts Forum 5-6 (1998) 359-362. (IF= 0)J33-c1. N.Ene: Electrosynthesis and electrochemistry of TiB 2 in molten electrolyte, Roumanian ChemicalQuarterly Reviews, 1998, 6(4), 233-245 – „A stochiometric compound could usually be synthesizedfrom salts provided that the following thermodynamic condition is observed [J33]: {egyenlet}. Then theequilibrium synthesis potential can be calculated as: {egyenlet}…+10 sor”, ‘238.o. –J33-c2. N.Ene: Electrosynthesis and electrochemistry of TiB 2 in molten electrolyte – Rev Roum de Chimie,1999, vol.44, pp.643-650. – „The equilibrium potential needed for the synthesis to occur is given by theequation [J33]: {equation cited}” – p.648J33-c3. T.P. Jose, L. Sundar, L.J. Berchmans, A. Visuvasam and S. Angappan: Eectrochemical Synthesis andcharacterization of BaB 6 from molten melt - Journal of Mining and Metallurgy, 2009, vol. 45 B, No.1,pp. 101 – 109. - The joint deposition of boron and barium in molten salts is explained by the so called‘Unstable stoichiometric way’ called ‘kinetic regime’ in the Russian literature [J33].”J33-c4. X.Cao, H.Wang, X.Meng, C.Wang, H.Yang, X.Xue: High temperature electrochemical synthesis oftungsten boride from molten salt – Adv mater Res., 2011, vol.206-307, pp.463-466. – „According toKaptay et al. the synthesis of tungsten boride could be perfomed in “kinetic regime” [J33].” – p.465.J32a. Devyatkin S.V., Kaptay G., Poignet J.-C., Bouteillon J.: Electrochemical Synthesis ofTitanium Diboride Coatings from Cryolite Melts - Molten Salts Forum 5-6 (1998) 331-334.(IF = 0)J32a-c1. S.A.Kuznetsov: Elektrokhimicheskii sintez visokotemperaturnich boridov iz solevich rasplavov –Elektrokhimiia, 1999, t.35., No.11., 1301-1317 – “Sostav elektrolitov i usloviia polucheniiatugoplavkich boridov predstavleni v tabl.2. [J32a]..” pp. 1311-1312J32a-c2. R.P.Pawlek: Aluminium Wettable Cathodes: An Update – in: Light Metals 2000, Ed.by R.D.Peterson,TMS 2000, pp. 449-454 – „Stable titanium diboride cathode coatings have been synthsized on carboncathodes in situ from cryolite alumina melts with additions of some B 2 O 3 , Al 2 O 3 and CaTiO 3. Deviatkinet al [J32a] stated that this technique is very promising to improve service characteristics of existingaluminium electrolysis cells, and that it can be used in development of new generation of aluminiumproduction cells” p.45070

J32a-c3. Vedernikov G.F.: Inertnie katodi v elektroliziorach dlia proizvodstva aliuminia. Problemi i perspektivi.AO VAMI, Informacionnii listok, No.10, April 2001 – „Stabilnie katodnie pokritiia iz diborida titanabili sintetizirovani na ugolnie katodi iz kriolit-glinoziomnich rasplavov s dobavleniem B 2 O 3 , Al 2 O 3 iCaTiO 3 [J32a]. Devyatkin i dr. [J32a] scitaiut etot sposob perspektivnim dlia ispolzovaniia vdeistvuiushich elektroliziorach i ispolzovaniia pri razrabotke elektroliziorov novogo pokoleniia” – c.16.J32a-c4. R.Krendelsberger, M.F.Souto, J.Sytchev, J.O.Besenhard, G.Fafilek, H.Kronberger, G.E.Nauer: Textureeffects in TiB 2 coatings electrodeposited from a NaCl-KCl-K 2 TiF 6 -NaF-NaBF 4 melt at 700 o C – J.Mining and Metallurgy, 2003, vol. 39B, No.1-2, pp.269-274 – „The electrochemical synthesis of TiB 2layers has been widely studied from diverse molten salt systems [J32a]” – p.270.J32a-c5. P.Taxil, P.Chamelot, L.Massot, C.Hamel: Electrodeposition of alloys or compounds in molten salts andapplications – J. of Mining and Metallurgy, 2003, vol.39B, pp.177-200 – „In the industry of aluminiumelectrowinning, titanium or zirconium borides are possibly used to protect the carbon cathodes from theelectrolyte insertion. Numerous works are dedicated to the preparation of these compounds by theelectrodeposition in molten salts, either in molten fluorides or in cryolithe media [J32a]” – p.178.J32a-c6. AL Yurkov: Refractories and carbom cathode materials for the aluminium industry – Refractories andIndustrial Ceramics, 2006, vol.47, pp.11-13 (translated from Novye Ogneupori, 2006, No.1, pp.18-21) –“Electrolytic deposition of TiB2 coatings is carried out either in situ in operating electrolysis cells, orusing specialized baths [J32]. + 14 lines description” – p.12.J32a-c7. Gorlanov ES, Nikiforov SA, Alternative technology to produce a wettable cathode surface layer in Alcells – Proc of the 12 th Int. Conf. “Aluminum of Siberia” (in Russian), Krasnoyarsk, 2006, pp.91-95. –„Naibolee perspektivnii, s popitkoi adaptacii k usloviiam elektroliza v kriolito-glinoziomnichrasplavach predstavlen v rabotach [P4]” – p.92.J32a-c8. T.P. Jose, L. Sundar, L.J. Berchmans, A. Visuvasam and S. Angappan: Eectrochemical Synthesis andcharacterization of BaB 6 from molten melt - Journal of Mining and Metallurgy, 2009, vol. 45 B, No.1,pp. 101 – 109. - The joint deposition of boron and barium in molten salts is explained by the so called‘Unstable stoichiometric way’ [J32] called ‘kinetic regime’ in the Russian literature. This will appear ifthe deposition potentials of boron and the second component of the boride, i.e. the metal component(MC) on inert cathodes are too far from each other. Barium is found to be more electronegative thanboron, so the depolarization of metal deposition should be taken into account. i.e. the condition is asfollows: …… when the above condition is fulfilled, first the macroscopic layer of one of thecomponents will be deposited on the cathode and the formation of boride will take place duringdepositing the second component on this layer with depolarization. In this case the synthesis of boride ispossible only above the limiting current density of the more electropositive component. Hence, thecomposition of the boride phase will strongly depend on the concentration of the ions of the moreelectropositive component in the melt i.e., boron concentration. It also depends on the actual cathodiccurrent density. It has been reported that during the crystal deposition, both the composition of the meltand the effective cathode surface area will continuously change, hence, the final composition of theboride will also be changed. This mechanism has been reported as ‘unstable stoichiometry way’ [J32].J32-a-c9. JRA Godinho: Optimization of TiB 2 coatings electrodepisted from halide melts – Master dissertation inChemistry, April 2008, 70 pp. – “From the 90-s onward some practical aspects of the deposition ofdifferent borides (e.g. TiB 2 ) were clarified, along with the basic electrochemical techniques andthermodynamic calculations [P3]” – p.10.J32ac10. G.V.Arkhipov, Y.S.Gorlanov: Development of technology for producing a wettable coating on acarbon cathode by electrodeposition – Light Metals 2012, ed. by C.E. Suarez, TMS, pp.1367-1372.„Since 1993, G.Kaptay and S.V.Devyatkin, under laboratory conditions, started to research on synthesisof borides of high-melting metals from molten salts. They were among the first researchers who set agoal of proving the possibility of electrodeposition of TiB 2 from Na 3 AlF 6 -Al 2 O 3 -TiO 2 -B 2 O 3 melts. Theirattempts to create wettable coatings on carbon and metallic cathodes ended at the laboratory level[J32a]” – p. 1367.J.32. S.V Devyatkin, G.Kaptay, J.C.Poignet, J.Bouteillon: Chemical and electrochemicalbehaviour of titanium oxide and complexes in cryolite-alumina melts - High TemperatureMaterial Processes, 1998, vol.2, N4, p.497-506. (IF = 0,233)J32-c1. T.E.Jentoftsen: Behaviour of iron and titanium species in cryolite-alumina melts – PhD Thesis,December 2000, Norway. – “the possibility to produce Al-Ti alloys by electrolysis as discussed by71

Devyatkin et al.” – Chapter 4, “devyatkin et al applied cyclic voltammetry to study … (+half page)” –Chapter 6.J32-c2. T.E.Jentofsten, A-A. Lorentsen, E.W.Dewing, G.M.Haarberg, J.Thonstad – Solubility of SomeTransition Metal Oxides in Cryolite Alumina Melts: Part II. Solubility of TiO 2 – Metall. Mater. Trans.,2002, vol. 33B., pp.909-913 – „The possibility of producing aluminum-titanium alloys by electrolysis,as discussed by Qiu et al […] and by Devyatkin et al [J32] is another reason for investigation” – p.909.J32-c3. Simakov D, Vassiliev S, Tursunov P, Khasanova N, Ivanov V, Abakumov A, Alekseeva A, Antipov E,Tsirlina G: Electrodeposition of TiB2 from cryolite-alumina melts - LIGHT METALS 2008, ed. byDeYoung DH, 2008, TMS, pp. 1019-1022. – „These observations agree with the literature data [J32]” –p.1020.J.31. Kuznetsov S.A., Kuznetsova S.V., Devyatkin S.V., Kaptay G.: Electrodeposition ofNiobium Boride Coatings from Chloro-Fluoride Melts - Russ. J. Appl. Chem. (Zh. PrikladnoiKhimii), 71 (1998) 74-80 (IF = 0.169)J31-c1. V.V.Malyshev, High-temperature electrosynthesis of metal-like refractory compounds of group IV-VImetals in ionic melts – Zh. Neorganicheskoi Khimii, 2003, vol.48 (2), pp.142-148 (ref. 32)J31-c2. V.V:Malyshev: High-temperature electrosynthesis of metal-like refractory compounds of group IV-VImetals in ionic melts – Russian J Inorg Chem, 2003, vol.48, pp.142-148 – “Kuznetsov et al. [J31]obtained niobium boride coatings from chloro-fluoride melts…” – p.144.J31-c3. V.V.Malishev: Visokotemperaturnii elektrochmnicheskii sintez metallopodobnich tugoplavkichsoedinenii metallov IV – VIA grupp v ionnich rasplavach – Zh. Neorg. Himii, 2004, vol.48, pp.187-194– “V [J31] pokazana vozmozhnost elektrohimicheskogo sinteza pokritii boridov niobiia sispolzovaniem hloridno-ftoridnich rasplavov. Vibrani sostavi elektrolitov i opredeleni parametriprocessa, pozvoliaiushie poluchat kak kristallicheskie, tak i rentgenoamorfnie sploshnie pokritiiaboridov niobiiia. Avtorami takzhe pokazani, shto elektrochmicheskim poverhnostnim borirovaniemniobievich podlozhek mogut bit polucheni tonkoplionochnie cloi diborida niobiia. Polucheni rezultatigovoriat o tom, shto VES boridov niobiia vozmozhen lish v kineticheskom rezhime. Po mneniuavtorov, pri takom rezhime sinteza reshaiusheezhanchenie imeet koncentraciia elektropolozhitelnogokomponenta (v dannom sluchaie geptaftoroniobata kaliia)” – pp.189-191.J31-c4. V.V.Malyshev: Zashitnie pokritiia tugoplavkimi soedineniiami metallov IV-VIA grupp, nanosimie izionnich rasplavov (obzor) – Zashita metallov, 2004, vol.40, pp.584-600 - – „az eredmények ismertetése41 sorban, állásfoglalás nélkül” – p.596J31-c5. V.V.Malyshev, Kh.B.Kushkhov: Advances in high-temperature electrochemical synthesis in ionic meltsby the onset of XXI century – Russ J. of General Chem., 2004., vol.74, pp.1139-1146 (Zh. ObsheiHimii, 2004, vol.74, pp.1233-1240) – Ref. No. 35. – „see Table 1” – p.1141, „Kuznetsov et al [J31]demonstrated the possibility of electrochemical synthesis of niobium boride coatings using chloridefluoridemelts” – p.1141.J31-c6. M.Noel, N.Suryanarayanan: Electrochemistry of metals and semiconductors in fluoride media –J.Appl.Electrochem., 2005, vol.35, pp.49-60 – “Niobium boride may also be obtained through similarelectrodeposition process using fluoroborate salts [J31]” – p.55.J31-c7. A.I.Hab: Hig-tempearture electrochemcial synthesis of coatings of carbides, borides and silicides ofmetals of the IV-VI B groups from ionic melts (review) – Materials Science, 2007, vol.43, pp.383-397(Fiziko-Himichna Mechanika Materialov, 2007, vol.43, No.3, pp.76-88) – „The cathodic process int hecourse of electrosynthesis of niobium borides were studied in [J31]. +5 lines, describing theexperimental conditions are given” – p.393.J.30. Kuznetsov S.A., Glagolevskaya A.L., Belyaevskii A.T., Devyatkin S.V., G.Kaptay:High temperature electrochemical synthesis of powders of Zirconium Diboride from chlorofluoridemelts - Rus.J.Appl.Chem., (Zh. Prikladnoi Khimii) 70 (1997) 1646-1649 (IF = 0,114)J30-c1. Shumakova NI, Procenko ZM, Gudakova GO, Bugaenko VV: Fazovii, elementnii sklad tamikrostruktura elektrolitichno otrimanich poroshkopodobnich produktiv na osnovi siliciiu, titanu, boruta ich spoluk – Bisnik Sumskogo Derzhavnogo Universiteta, Seriia Fizika, matematika, mechanika,2004, No. 10 (69), 196-205.J30-c2. VV Bugaenko, ZM Procenko, NI Shumakova: Fazovii, elmentnii ta granulometrichnii skladelektrolitichno otrimanich poroshkopodobnich produktiv na osnovi boridiv titanu – Bisnuk SumDU,2006, No.6, pp.114-122 – „Odnim iz bagatoh metodiv oderzhaniia boridiv metalic svisokotemperaturnii elektrohimichnii sintez (VES) b rozplavlenich soliovich elektrolitach, iakii sperspektivnim metodom oderzhaniia poroshkopodobnich boridiv metaliv ta nemetaliv [J30]” – p.115.72

J.29. Kaptay Gy.: Kerámiával erősített fémmátrixú kompozitok gyártásának határfelületivonatkozásai. I/2. Határfelületi kritériumok meghatározása preformába öntött MMC-kgyártásának biztosítására. BKL, Kohászat, 130 (1997) No 8-9, 311-314 (IF = 0)J29-c1. Kientzl Imre: Alumínium mátrixú duplakompozit szerkezetek gyártása és vizsgálata – Diplomaterv,BME (konzulens: Dobránszky János), 2005, Bp., 110o. – „16 egyenlet, 6 ábra, 7 táblázat, összesen 11 oldalátvéve [J29] „ – 32-42. o.J29-c2. Orbulov I., Kientzl I., Németh Á.: Fémhabok és kompozitok előállítása infiltrálásos eljárással – BKLKohászat, 2007, vol.140, No.5, pp.41-46. – „Nagyon fontos, hogy a fémmátrixú kompozitanyagok esetébenis csak akkor kapunk megfelelő műszaki tulajdonságokat, ha megfelelő a kapcsolat az erősítőanyag és amátrixanyag határfelületén [J29]” – p.41.J29-c3. Orbulov I.: Szintaktikus fémhabok keménységmérése – Anyagvizsgálók lapja, 2009, No.1, pp.9-15. – „Aleggyakoribb gyártási módszerek a nyomásos infiltrálás és a keveréses eljárás. Mindkét eljárásban jelentősszerepe van a mátrix és az erősítőanyag közötti határfelületenek, amely kritériumaival Kaptay behatóanfoglalkozott [J29].” – p.9.J29-c4. Pázmán J.: Szilíciumkarbid szemcsék kémiai nikkelezése és fémkompozitokban történő alkalmazása –PhD disszertáció (tud. vez.: Gácsi Z.), Miskolc, 2010. „Ahhoz, hogy stir casting technológiával, vagyinfiltrációval megfelelő minőségű és mechamnikai tulajdonságokkal rendelkező fémkonpozitot lehessengyártani, a részecskék tökéletes nedvesítése szükséges [J29]” – 28.o.J29-c5. Kun P., Orbulov IN: AlCu5 és AlMgSi1 mátrixú szintaktikus fémhabok előállítása és vizsgálata – BKLKohászat, 2011, vol.144, No.3, pp.51-55. – „Mindkét eljárásban jelentős szerepe van a mátrix és azerősítőanyag közötti határfelületi jelenségeknek és a nedvesítésnek, amelyek vizsgálatával Kaptaybehatóan foglalkozott [J29]” – p.51.J29-c6. Gácsi Z., Simon A., Pázmán J.: Fémkompozitok, Miskolci Egyetem, 2011. „Az öntészeti módszerrelgyártott fémkompozitoknál a második fézis homogén eloszlásához biztosítani kell a kerámia szemcsékolvadékba történő bevitelét és benntartását [J29]: Emellett meg kell akadályozni a részecskékkoagulációját, mely gyengítheti a határfelületi kötést.” – 38-39 o.J.28. Kaptay Gy.: Kerámiával erősített fémmátrixú kompozitok gyártásának határfelületivonatkozásai. I. rész. A határfelületi kritériumok levezetése. BKL, Kohászat, 130 (1997) No5-6, 201-208 (IF = 0)J28-c1. Csepeli Zs., Sólyom B., Gácsi Z., Buza G., Teleszky I., Kovács Á.: Részecske- és szálerősítésűfémmátrixú kompozitok előállítási lehetőségei - BKL Kohászat, 131 (1998) 41-47 – „.. a bevonatnakegyszerre kell meggátolnia a szál és a mátrix közötti diffúziót és biztosítani a bevonat és a mátrixközötti tökéletes nedvesítést [J28]… p. 45. --J28-c2. Csepeli Zsolt: Irányítottan kristályosított volfrám szállal erősített alumínium mátrixú kompozitszerkezete - PhD értekezés, Miskolc, 1997 – „A szálerősítésű kompozitok előállításához soklépcsős,nehezen automatizálható eljárásokat használnak. Az alkalmazott módszer egyik legnagyobb problémájaaz optimális nedvesítés biztosítása a szál és a mátrix között [J28].” – p.4. --J28-c3. Boross Péter: Karbidkerámia szemcsék viselkedése lézerrel létrehozott olvadéktócsában: TDK dolgozat,2000, tud. vez.: dr. Verő Balázs BAYATI és dr. Hárs György, BME) – „II.2. fejezet. Kerámiaszemcsékolvadékokban – alapfogalmak [J28]” – fejezetcím, a teljes 3. oldal idézet. “II.3. Kerámiaszemcsékolvadédkokban – elsüllyedési elméletek [J28]” – fejezetcím, a teljes 4-5 oldalakon idézetek, pl.„…amint Kaptay György [J28]-ban megmutatta… „ - 4. oldal. „…Kaptay-féle elmélet…” – 18.o.J28-c4. Boross Péter: Lézeres átolvasztással végzett felületmódosítások, Diplomamunka, ME, Bayati, 2001.,tud.vez.: dr. Verő Balázs és dr. Hárs György. „IV.2. fejezet. Felületfizikai effektusok –kerémiaszmecsék elsüllyedése. IV.2.2. Alapfogalmak [J28] – 17-18. oldalon folyamatos hivatkozés.IV.2.3. Elsüllyedés elméletek összefoglalása [J28] – 18-21 oldalakon az általam alkotott modellismertetése, egyenletekkel és két ábrával.” – 17 – 21.o.J28-c5. Boross Péter, Kálazi Zoltán: A lézeres diszpergálás során fellépő jelenségek néhány elméletivonatkozása – BKL Kohászat, 2002, 135. évf., 6-7. szám, 219-223 o. – 2 oldal szöveg + 7 egyenlet + 2ábra átvéve a 220 – 221 oldalakonJ28-c6. E.R.Fábián, P.Boross, B.Verő, P.Fülöp: Metallographic Aspects of Surface-Treated Steels by usingLaser Technology – Materials Science Forum, 2003, vols. 414-415, pp.201-206 – “The wetting theoremby G.Kaptay [J28] shows that particles with zero contact angle will sink completely in melt pool, butparticles with nonzero contact angle will sink partially, and will float on the surface. … But our systemis not in static state. This means that the static theorem [J28] is unusable, so we need to construct a73

dynamic theorem. The energy equilibrium equations and the method of [J28] are unusable too. We needto solve the problem by dynamic equations. We can determine surface forces from equationsdetermined in [J28] by gradient calculus, and we need to complete it by hydrodynamic drag force…”J28-c7. G.Králik, P.Fülöp, B.Verő, D.Zsámbok: Laser Surface Treatment of Steels – Materials Science Forum,2003, vols.414-415, pp.21-30 – “… based on the work of Gy.Kaptay [J28] we inspected the lawsdetermining the transport of the TiC particles into the molten bath. According to theoreticalconsiderations a particle only submerges into the depth of 2r in the liquid if the wetting is perfectbetween them. Since the wetting only partial between the material and the TiC particle in the presumedthermic and ambiency circumstances the conditions of the particle to travel under the surface of themolten bath are not given.” – p.25J28-c8. Magyar Anita: Karbon szállal erősített alumínium mátrixú kompozitok Al/C határfelületének jellemzése– PhD értekezés, Miskolc, 2004. – 2,5 oldal szöveg és 11 egyenlet átvéve a cikkemből a 24-26oldalakon.J28-c9. Janó V., Búza G., Kálazi Z.: Diszperz eloszlású, fémmátrixú kerámia kompozitréteg létrehozásalézersugaras felületkezeléssel – BKL Kohászat, 2005., 138. évf., 3. szám, 39-44 (No.1).J28-c10. Kientzl Imre: Alumínium mátrixú duplakompozit szerkezetek gyártása és vizsgálata – Diplomaterv,BME (konzulens: Dobránszky János), 2005, Bp., 110o.J28-c11. Orbulov I., Kientzl I., Németh Á.: Fémhabok és kompozitok előállítása infiltrálásos eljárással – BKLKohászat, 2007, vol.140, No.5, pp.41-46. – „Nagyon fontos, hogy a fémmátrixú kompozitanyagokesetében is csak akkor kapunk megfelelő műszaki tulajdonságokat, ha megfelelő a kapcsolat azerősítőanyag és a mátrixanyag határfelületén [J28]” – p.41.J28-c12. Verezub O.: Lézeresen felületkezelt szerszámacél köszörülése – Gyártóeszközök, szerszámok,szerszámgépek, 2008, No.1, pp.65-68. – „Az acélolvadékba nem a szerszám felületi rétegébe tervezettTiC-szemcséket vittük be. Ennek bionyolult felületkémiai-hidrodinamikai okait részletesen tartalmazzaa [J28] irodalom” – p.66.J28-c13. Orbulov I.: Szintaktikus fémhabok keménységmérése – Anyagvizsgálók lapja, 2009, No.1, pp.9-15. –„A leggyakoribb gyártási módszerek a nyomásos infiltrálás és a keveréses eljárás. Mindkét eljárásbanjelentős szerepe van a mátrix és az erősítőanyag közötti határfelületenek, amely kritériumaival Kaptaybehatóan foglalkozott [J28].” – p.9.J28-c14. Pázmán J.: Szilíciumkarbid szemcsék kémiai nikkelezése és fémkompozitokban történő alkalmazása –PhD disszertáció (tud. vez.: Gácsi Z.), Miskolc, 2010. – „.. biztosítani kell a részecskék, sok esetben akerámia szemcsék olvadékba történő bevitalét és benntartását [J28]” – 28.o.J28-c15. Kun P., Orbulov IN: AlCu5 és AlMgSi1 mátrixú szintaktikus fémhabok előállítása és vizsgálata – BKLKohászat, 2011, vol.144, No.3, pp.51-55. – „Mindkét eljárásban jelentős szerepe van a mátrix és azerősítőanyag közötti határfelületi jelenségeknek és a nedvesítésnek, amelyek vizsgálatával Kaptaybehatóan foglalkozott [J28]” – p.51.J28-c16. Gácsi Z., Simon A., Pázmán J.: Fémkompozitok, Miskolci Egyetem, 2011. „Az öntészeti módszerrelgyártott fémkompozitoknál a második fézis homogén eloszlásához biztosítani kell a kerámia szemcsékolvadékba történő bevitelét és benntartását [J28]: Emellett meg kell akadályozni a részecskékkoagulációját, mely gyengítheti a határfelületi kötést.” – 38-39 o.74

J27. G.Kaptay, A.Lovas, F.Szigeti, P.Bárczy, L.Bolyán: Correlation between the abrasiveability of ceramic reinforced amorphous metal matrix composites and the adhesion energybetween the amorphous matrix and the ceramic particles - Materials Science and EngineeringA226-228 (1997) 1083-1088 (IF = 0,842)J27-c1. V.V.Maslov, D.Yu.Paderno, A.D.Panasyuk: Effect of Refractory Boride Particles on Crystallization ofthe Amorphous Alloy Fe 85 B 15 – Powder Metallurgy and Metal Ceramics, 2000, vol.39, 474-479 –„According to data in [J27], introduction of refractory particles leads to an increase in Young’smodulus, yield stress, and also wear resistance of amorphous alloy ribbons…” – 474.J27-c2. L.Ma, L.Wang, X.Guo, T.Zhang, A.Inoue: Enhanced glass-forming ability and microhardness ofTi 45 Zr 5 Cu 25 Ni 20 Sn 5 amorphous alloy by addition of TiC particles – J. of Materials Science Letters,2002, vol.21., pp.1435-1437 – „Amorphous MMCs are prepared by mechanical alloying […], meltspinning [J27] and copper mold casting […]”– p.1435.J26. Kaptay G., Bárczy P., Szigeti F., Lovas A., Gácsi Z., Bolyán L.: Interface Phenomena inProcessing of Ceramic Reinforced Amorphous Metal Composites. - J. of Non-crystallineSolids 205-207 (1996) 742-747. (IF = 1,318)RJ26/1. Jiang J.H., Li Z.L., Ye X.M., Zhou R.: Effect of matrices on dissolution of tungsten carbide partiiculates(WC) in WC reinforced iron base composites – Foundry Technology, 2007, vol.28, No.2, pp.199-203 –„G.Kaptay …. WC …. Fe40Ni40Si04B6 …. WC …. . Fe40Ni40Si04B6… WC …… [J26]” – p.199.(…. = Chinese text)RJ26/2. Li Z., Jiang Y., Ye X., ZHou R.: Dissolution of tungsten carbide particulates (WC) int he matrix of WCreinforced gray cast iron matrix composites – Acta Materiae Compositae Sinica – 2007, vol.24, No.2,pp.13-17 – „… Kaptay …. WC …. Fe40Ni40Si14B6 … {Chinese text} [J26]” – p.13.J.25. G. Kaptay: Method for Estimating Solid-Solid Interface Energies in Metal-CeramicSystems. The Aluminium-Silicon Carbide System - Materials Science Forum Vols. 215-216(1996) 475-484. (IF = 0)J25-c1. D.M.Stefanescu, F.R.Juretzko, A.Catalina, B.K.Dhindaw, S.Sen, P.A.Curreri: Authors’ Reply toDiscussion of „Particle Engulfment and Pushing by Solidifying Interfaces: Part II. MicrogravityExperiments and Theoretical Analysis” - Metall. Mater. Trans., A, volume 30A, 1999, pp. 1890 - 1894– “This is further corroborated from data that Kaptay’s generated in a different article [J25], where hehas calculated (in his Table 5) interface energies for the Al-SiC system, assuming both oxidized and notoxidized aluminum surfaces. These values are reproduced in Table II.” p.1893 –J25-c2. J.A.Vreeling, V.Ocelik, Y.T.Pei, D.T.L.van Agterveld, J.T.M. de Hosson: Laser Melt Injection inAluminum Aloys: on the Role of the Oxide Skin – Acta mater. 48 (2000) 4233 – „The values ofinterface energies for both oxidized and unoxidized surfaces of liquid Al are given in Table 1 [J25]. Allof this indicates that the velocity of the particles and the particular state of the melt pool surface playimportant roles in the actual laser melt injection ’ process. …. Table 1. Interface energies of oxidizedand unoxidized Al in the Al(l)/SiC p system [J25] – {táblázat átmásolva [J25]-ből}” – p. 4228.J25-c3. J.A.Vreeling, V.Ocelik, Y.T.Pei, J.Th.M.de Hosson: Laser Melt Injection of SiC Particles in Al – in:„Surface Modification Technologies XIV”, ed. by T.S.Sudarshan and M.Jeandin, ASM International,Materials Park, OH, USA, 2001, pp. 619-623. – „The liquid-vapor and liquid particle interface energiesare different for oxidized and non-oxidized surfaces. The interface energies are listed in Table 1[J25]…. Table.1. Interface energies per unit area of oxidized and not-oxidized Al in the Al(l)/SiC psystem [J25]. – {táblázat átmásolva [J25]-ból}” – p. 622.J25-c4. A.Vreeling: Laser Melt Injection of Ceramic Particles in Metals – PhD Thesis, University of Groningen,Holland, 2001, pp. 136. Chapter 3. „Table 3.1. Interface tensions of oxidized and non-oxidized Al in theAl(l)/SiC p system [J25]” {táblázat átmásolva [J25]-ból}” – p.45, „Important is that lv and lp havedifferent values for oxidized and non-oxidized Al. The values of the interface tensions of the Al(l)-SiCsystem, of both oxidized and un-oxidized Al, are found in the literature and given in Table 3.1 [J25].The data in Table 3.1 are based on calculations that agree with experimental data.” – p.46.75

J25-c5. Y.T.Pei, V.Ocelik, J.Th.De Hosson: SiC p /Ti6Al4V functionally graded materials produced by laser meltinjection – Acta Materiala, 50 (2002) 2035-2051 – „…for the SiC/Ti6Al4V system lp = 1000 mJ/m 2 , pv = 1920 mJ/m 2 [J25]….” – p. 2046.J25-c6. C.Kawai: Fabrication of Al-SiC composites using a hot-forging technique and their thermal conductivity– J. of the Ceramic Society of Japan, 2002, vol.110, pp.1016-1020-„hivatkozás japánul, valószínűlegarról, hogy az Al/SiC rendszerben 1023 o C-on a peremszög 50 o [J25]” – p.1018J25-c7. J.Th.M.de Hosson, B.J.Kooi: Microstructure and properties of interfaces between dissimilar materials –in: „Handbook of Surfaces and Interfaces of Materials, vol.1., Surface and Interface Phenomena”, ed.by H.S.Nalwa, Academic Press, San Diego, 2001, Chapter 1, pp.1-113 – „The values of the interfaceenergies for both oxidized and nonoxidized surfaces of liquid Al are given in Table VII [J25] – TableVII is taken from my paper – „, p.79. „explanation in 17 lines, based on [J25]” – p.81.J25-c8. De Hosson JT, Pei YT: Functionally graded materials produced with high power lasers, in: SURFACEENGINEERING: SCIENCE AND TECHNOLOGY II, ed by Kumar A; Chung YW; Moore JJ; DollGL; Yatsui K; Misra DS, TMS, 2002, pp.163-176J25-c9. J.Th.M.deHosson, V.Ocelik, Y.Pei: Surface Engineering with lasers. Chapter 16 of the book “SurfaceModification and Mechanisms – Friction, Stress and Reaction Engineering”, ed. by G.E.Totten,H.Liang, Marcel Dekker Inc, New York, 2004, pp.603-669.J.24. G. Kaptay: Interfacial Phenomena during Melt Processing of Ceramic Particle-Reinforced Metal Matrix Composites. Part II. Interfacial Force between a Spherical Particleand an Approching Solid/Liquid Interface - Materials Science Forum Vols. 215-216 (1996)467-474. (IF = 0)J24-c1. F.R.Juretzko, D.M.Stefanescu, B.K.Dhindaw, S.Sen: Interfacial energy - Theoretical andexperimental evaluation for metal-ceramic systems – in: „Processing, Properties and Applications ofCast Metal Matrix Composites, ed. by P.K.Rohatgi, TMS, 1996, pp. 21-31 – „Recently, a third way ofcalculation was presented by Kaptay [J24]. According to this derivation the surface energy differenceshould be expressed as {equation is given}…” p.24J24-c2. S.Sen, B.K.Dhindaw, D.M.Stefanescu, A.Catalina, P.A.Curreri: Melt convection effects on the criticalvelocity of particle engulfment - Journal of Crystal Growth, 173 (1997) 574-584 – „According toKaptay [J24] the interface energy difference is: {equation given}…. „ p.583J24-c3. D.M.Stefanescu, F.R.Juretzko, B.K.Dhindaw, A.Catalina, S.Sen and P.A.Curreri: Particle Engulfmentand Pushing by Solidifying Interfaces: Part II. Microgravity Experiments and Theoretical Analysis -Met. and Mat. Trans. A, volume 29A, June 1998, pp. 1697-1706 – „The expression for o and thelocal force during engulfment, as proposed by UCJ and adopted by SAS, can be derived [J24] bywriting the energy balance for the case in Fig1” p.1704 –J24-c4. D.M.Stefanescu, F.R.Juretzko, A.Catalina, B.K.Dhindaw, S.Sen, P.A.Curreri: Authors’ Reply toDiscussion of „Particle Engulfment and Pushing by Solidifying Interfaces: Part II. MicrogravityExperiments and Theoretical Analysis” - Metall. Mater. Trans., A, volume 30A, 1999, pp. 1890 – 1894– „… This derivation followed that proposed by Kaptay [J24]…” p.1890 –J24-c5: D.M.Stefanescu, A.Catalina, S.Sen, F.R.Juretzko, B.K.Dhindaw, P.A.Curreri: Authors’ Reply,Metallurgical and Materials Transactions A, vol.31A (2000), 1700–1705. – „The derivation of thisequation has been attempted earlier by Kaptay [J23] and criticized by us..” 1702-1703 o.J24-c6. Jiang ZW, Ren ZM, Zhong YB: Theoretical model for particle migrating behaviour ahead ofsolidification front in electromagnetic field – Shanghai Nonferrous Metals, 2000, vol.21, No.2, p.49-53(Ref. No.12). – The equation for deltasigma is cited” – p.50.J24-c7. Jiang ZW, Ren ZM, Zhong YB: Theoretical model for particle behaviour at solidifying front inelectromagnetic force field – Journal of Shanghai University, 2000, vol.4, No.3, p.246-249 (Ref.No.12). – “The equation for deltasigma is different in [J24]” – p.247.J24-c8. Á.Borsik: Dynamic Simulation of the Movement of Ceramic Particles in front of an ApproachingSolidification Front, Materials’ World (e-journal, http://material.ini.hu), July, 2001. (ref. No.24)J24-c9. Q.Sun, Y.Zhong, Z.Ren, K.Deng, K.Xu: Advances in Research on Particle-s behaviour in front ofsolidifying interface – Materials Review, 2003, vol.17, No.9, pp.9-12. – “G.Kaptay…. Equation (2)….Chinese text” – p.9.J24-c10. F-H. Li, S-S. Chen, Z-G. Fan: Properties of alumina particles reinforced silver composites – J. ofNortheastern University, Natural Science, 2007, vol.28, pp.696-700 (Ref. No.13). – “Chinese text.” –p.697.J24-c11. W.Xi, R.L. Peng, W. Wu, N. Li, S. Wang, S. Johansson: Al2O3 nanoparticle reinforced Fe-based alloyssynthesized by thermite reaction – J Mater Sci, 2012, vol.47, pp.3585-3591. „Kaptay [J24] reported that76

if the difference in surface free energy, deltasigma is negative, the ceramic particles would be engulfedby the solidification front, leading to homogeneous distribution of the particles in the fuinal product. Incontrast, if deltasigma is positive, the ceramic particles would be pushed away from the solidificationfront. The difference in surface energy can be defined as [J24]: Eq-s (1-2)….” – p.3588.J.23. G. Kaptay: Interfacial Phenomena during Melt Processing of Ceramic Particle-Reinforced Metal Matrix Composites. Part I. Introduction (incorporation) of solid particlesinto melts - Materials Science Forum Vols. 215-216 (1996) 459-466. (IF = 0)J23-c1. J.A.Vreeling, V.Ocelik, Y.T.Pei, D.T.L.van Agterveld, J.T.M. de Hosson: Laser Melt Injection inAluminum Alloys: on the Role of the Oxide Skin – Acta mater. 48 (2000) 4225-4233 – „The totalinterface energy for a particle partially immersed in a melt at depth x, 0x2R (see Fig.5), is given by[J23]: {a cikk (2) egyenlete és 5. ábrája kimásolva [J23]-ból, további magyarázatokkal}..” – p.4228.J23-c2. E.Báder: Wettability of Alumina by Liquid Magnesium and Liquid AZ91 Alloy, Materials’ World (ejournal,http://materialworld.uni-miskolc.hu, July, 2001 – “The wettability of alumina by magnesium isa very important factor in producing metal matrix composites [J23] or metallic foams […] consisting ofthese two phases” – p.1 –J23-c3. J.A.Vreeling, V.Ocelik, Y.T.Pei, J.Th.M.de Hosson: Laser Melt Injection of SiC Particles in Al – in:„Surface Modification Technologies XIV”, ed. by T.S.Sudarshan and M.Jeandin, ASM International,Materials Park, OH, USA, 2001, pp. 619-623. – „If we simplify the problem by assuming that theparticles are spherical, having a radius R, the interface energy of a one-particle system can be calculatedas a function of depth x, defined in Figure 5. The total interface energy is [J23]: {a cikk (2) egyenlete és5. ábrája kimásolva [J23]-ból, további magyarázatokkal}..” – p.622.J23-c4. A.Vreeling: Laser Melt Injection of Ceramic Particles in Metals – PhD Thesis, University of Groningen,Holland, 2001, pp. 136. Chapter 3. „During penetration, the total interface energy changes because theareas of the different interfaces, which have different interface tensions, change. The total interfaceenergy for a particle that is partially immersed in a melt at depth x, where the depth x is defined inFig.3.8., is given by [J23]:… {a disszertáció (3.2) egyenlete kimásolva [J23]-ból, továbbimagyarázatokkal}..” – p.45.J23-c5. J.Th.M.de Hosson, B.J.Kooi: Microstructure and properties of interfaces between dissimilar materials –in: „Handbook of Surfaces and Interfaces of Materials, vol.1., Surface and Interface Phenomena”, ed.by H.S.Nalwa, Academic Press, San Diego, 2001, Chapter 1, pp.1-113 (ref. No.248). – „The totalinterface energy for the particle partially immersed into a melt at depth x is given by [J23].. – (myequation with explanations) –„, p.79J23-c6. HAO Xing Ming, Liu Hongmei, Zhang Feng-lin, Zhao Feng, Su Junyi: Metal matrix compositesinfiltration casting the theory and practice – Research Studies on Foundry Equipment, 2002, No.2, p.50-53 – Chinese text, Ref.No.1.J23-c7. 5 kinai: On the infiltration of metal matrix composites, 2002, No.2, Ref. No.16. (different from J23-c6 –see Google Scolar). 19. cikkJ23-c8. O.N.Verezub: Izuchenie mechanizma proniknoveniia tviordoi chastici v zhidkost, s celiu optimizaciitechnologii lazernoi tviordotelnoi implantacii – in: „Visoki Technologii v Mashinobuduvanni –Kharkiv, 2003, pp.11-16 (ref. No.11)J23-c9. Kínai jelek (Google): Materials Review, 2003, vol.17, No.9 (Ref. No.13)J23-c10. O.N.Verezub, A.I.Grabchenko, T.Matsushita: Eksperimentalno-teoreticheskoie modelirovanie dinamikiproniknoveniia legiruiushich chastic v matricu eksperimentalnogo materiala – in: „Research andEducation”, Nacionalnii Technicheskii Universitet, 2004, Harkov, pp.59-66 – „Uslovie spontannogoproniknoveniia mozhno virazit cherez bezrazmernoie chislo G [J23] – egyenlet…” – p.62, „V tretieigruppe uravnenii [J23] kriticheckii ugol kontakta raven nuliu v tom sluchaie, esli Weber kriticheskiistremitsia k nuliu. Eto polnostiu podtverzhdaiet nashi eksperimentalnie dannie” – p.64.J23-c11. J.Th.M.deHosson, V.Ocelik, Y.Pei: Surface Engineering with lasers. Chapter 16 of the book “SurfaceModification and Mechanisms – Friction, Stress and Reaction Engineering”, ed. by G.E.Totten,H.Liang, Marcel Dekker Inc, New York, 2004, pp.603-669.J23-c12. P.Boross, Z.Kálazi, O.Verezub, B.Verő: Investigation of processes evolving during thin film productionby laser surface modification – Mater. Sci. Forum, 2005, vols. 473-474, pp.303-308 – “Fig.1: Theequilibrium and the penetration depths for different contact angles [J23] + equations + text in pages303-304”J23-c13. DA Weirauch: Technologically significant capillary phenomena in high-temperature materialsprocessing. Examples drawn from aluminum industry – Current Opp Solid State and Mater Sci, 2005,vol.9, pp.230-240 – „There are several good reviews that cover capillarity in composite manufacturing77

[J22]. The general principles of particle incorporation into molten metals have been summarized in[J23].” – p.237.J23-c14. A.E.Karantzalis, A.Lekatou, E.Georgatis, H.Mavros: Solidification behaviour of ceramic particlereinforced Al-alloy matrices – J.Mater Sci, 2010, vol.45, pp.2165-2173 – „Especially in the case of castmetal composites, however, a contact angle of less than 90 o C (sicc) is not sufficient to lead tospontaneous entry of the particles but a 0 o contact angle (total spreading condition) is required as shownby the works of Nakae et al., Wu et al. and Kaptay [J23]” – p. 2165J23-c15. A.Ott: Oberflachen modification von Aluminium legierungen mit Laserstrahlung. Dissertation Uni-Stuttgart (prof. H. Hugel), Herbert Utz Verlag, 2010.J23-c16. B.Balout: Centrifugal casting of ZA8 zinc alloy and composite A356/SiC: study and modeling ofphases and particles segregation – PhD Thesis, University of Quebec, Montreal, 2010. – “Fig.14. Aspherical particle partially immersed ina liquid [J23]” – p.29. “According to Kaptay [J23], the interfaceenergy of the system can be interpreted as … 9 lines and 2 equations” – pp.30-31J.22. Bárczy P., Kaptay Gy., Gácsi Z., Lovas A., Szigeti F. Kerámiarészecskék beépülésegyorsan dermedő fémolvadékba - Publ. Univ. of Miskolc, Series B. Metallurgy vol 39 (1995),pp. 279-290. (IF = 0)J.21. Akhmedov S.N., Kaptay G., Borisoglebskii Yu.V., Gorlanov E.S., Karimov M.I., VetyukovM.M. Chemical and electrochemical behaviour of some 'new materials' in molten salts to be used foraluminium electrolysis - Molten Salt Forum vol. 1-2 (1993/94) pp. 231-232. (IF = 0)J.20. Deviatkin S.V., Kaptay G. Influence of nature of the alkali metal cation on Ti(III) - e =Ti(IV) electrochemical process in chloride melts - Molten Salt Forum vol. 1-2 (1993/94) pp.129-138. (IF = 0)J20–c1. A.Salmi, Y.Berghoute, F.Lantelme: Modelling Multistep Electrochemical Reactions in Molten SaltsElectrowinning of Refractory Metals - Electrochimica Acta, 1995, vol.40., o.4., pp.403-411 – “…However, the solubility of TiCl 4 is low [ ], [J20], and increasing the concentrations Ti(IV) results in arapid evolution of gaseous TiCl 4 .. “ p.410 –J20-c2. F.Lantelme, A.Salmi: Electrochemistry of Titanium in NaCl-KCl Mixtures and Influence of DissolvedFluoride Ions - J.Electrochem. Soc., vol. 142, No.10., 1995, pp.3451-3456 - „Figures 1 and 2 showvoltammograms …. According to previous studies [J20] the reaction corresponds to the Ti(III)/Ti(IV)couple.” p.3452 –J20-c3. F.Lantelme, K.Kuroda, A.Barhoun: Electrochemical and thermodynamic properties of titanium chloridesolutions in various alkali chloride mixtures. Electrochimica Acta, 44 (1998) 421-431 – „Equations inTable 3 show that the dissolution energy is made of two terms [J20]. The values of the enthalpies andentropies of dissolution depend on the solvent salt…” p.427 –J20-c4. F.Lantelme, A.Barhoun, K.Kuroda: Role of the oxoacidity and Ligand Effect in the Electrowinning ofTitanium in Fused Salts - in Refractory Metals in Molten Salts (Their Chemistry, Electrochemistry andTechnology), ed. by D.H.Kerridgeand E.G.Polyakov – Kluwer Academic Publishers, vol.3/53, 1998,pp. 157-172 – „This result is probably due to the low solubility of TiCl 4 [J20] which evaporates andcannot be reduced during the backward sweep.” p.161 –J20-c5. F.Lantelme, A.Barhoun, M.Chemla, J.von Barner – Titanium, Boron and Titanium Diboride Depositionin Alkali Fluorochloride Melts – in Proc. of the 12 th Int. Symp. on Molten Salts, Proceedings volume99-41, ed. by P.S.Trulove, H.C.De Long, G.R.Stafford, S.Deki – The Electrochemical Society,Pennington, NJ, USA, 1999, pp.612-623 – „… When the electrode is maintained at such a positivepotential, evolution of TiCl 4 occurs. According to previous studies [J20] the reaction corresponds to theTi +4 /Ti +3 couple.” – p.614.J.19. Kaptay G., Stefanescu D.M. Theoretical Analysis of the Effect of Oxygen on thePenetration Factor in the Iron/Silica System - AFS Transactions, 1992, v. 100, pp. 707 - 712.(IF = 0)J19-c1. J.Griffin, C.E.Bates: Clean Cast Steel Technology – Final Report, University of Alabama atBirhmingham, 1995 (Ref. No.3). – „As shown in a theoretical discussion by Kaptay and Stefanescu[J19], as the oxygen content in a Fe-C melt increases the contact angle decreases rapidly” – p.6.J19-c2. H.Iwahori, Y.Sugiyama, Y.Awano, K.Yonekura, Y.Ueshima: Metal Penetration defects in cast iron –origins and countermeasures - Japan Foundry Eng. Soc, 1998, vol.33, No.4, pp.33-41. „ Japanese text”– p.34”78

J19-c3. H.Nakae, Y.Matsuda: Influence of Atmospheric Oxygen on Burn-on of Iron Castings J.Japan FoundryEng.Soc., 1999, v.71, 28-33 – „Stefanescu and coworker [J19] have simulated the mechanism ofoccurring burn-on during casting based on the relationship between the amount of oxygen dissolved inliquid iron and the contact angle” – p.28. (japánról angolra fordítva N.Shibata által).J19-c4. H.Nakae, Y.Matsuda: Influence of Chemical Composition of Sands on Burn-on of Iron Castings –J.Japan Foundry Eng. Soc., 2000, vol.72., pp. 102-106 (ref. No. 12) „…Kaptay… [J19]…”, 102.o.,“…Kaptay…[J19]…”, 105.o. japán nyelven előzőhöz hasonló tartalommal.J19-c5. E.Báder: Contact angle and infiltration pressure relevant to fabrication of syntactic magnesium / Al 2 O 3foams, WTM, Germany, Dec. 2000 – Dec. 2001, 26 pp. (Ref. No. 21): “The infiltration process forfabricating ceramic reinforced metal matrix composites has already been studied by the group ofMortensen […], Garcia-Cordovilla […] and Kaptay [J19]..” pp. 11,… “… in order to avoid theinfiltration ‘into the pores the pressure must be lower than the threshold pressure [J19] : {Equation iscited}..” – p. 15.J19-c6. T.Matsushita, K.Mukai: Penetration behaviour of molten metal into porous oxides - Tetsu-to-Hagane,2004, vol.90, pp.135 – 144 „in Japanese” – p.138J19-c7. Kientzl I.: Alumíniummátrixú kompozithuzalok és kettős kompozit-szerkezetek – PhD értekezés, BME(tud. vez.: dr.Dobránszky János), 2010, 112.o. – „.. ha a porózus test egyforma, szorosan pakoltgömbökből van kirakva, akkor a kritikus peremszög 50,7 o [J19]” – 20.o.J18. Gudimenko A.M., Kaptay G., Makogon V.F. Estimation of Thermodynamic Propertiesof Tetrachloroaluminates of Lithium, Rubidium and Caesium - Ukrainian Khim. Zh., 1992,v.58., N.4., pp. 300-305 (IF = 0)J.17. Kaptay Gy., Deviatkin S.V., Berecz E., Sh poval V.I. Átmenetifém borid bevonatokelőállítása fémeken sóolvadékok elektrolízise útján - Gépgyártástechnológia, 1991. XXXI.évf., 10. sz., 445-446 o. (IF = 0)J.16. Kaptay G. : Estimation of excess thermodynamic functions of aluminum monochloridedissolved in alkali chloride melts - Materials Science Forum Vol. 73-75 (1991), pp. 101-108(IF = 0)J.15. Roósz A., Kaptay G., Máté I., Teleszky I., Sólyom J., Regel L.L., Turchaninov A.M.The Ground-based Experiments of Shell Technology - Microgravity sci. technol. 1991., v.IV.,issue 4., pp. 245-253 (IF = 0)J15-c1. T Kraft: Numerische Simulation der Erstarrung mehrkomponentiger Legierungen 1995. Universitat,Darmstadt Disszertáció/PhDJ15-c2. Bárczy P.: Mikrogravitációs kutatások a Miskolci Egyetemen - BKL Kohászat, 1999., 132. évf., 6-7.szám, 269-274 o. – „Intenzív erőfeszítések történtek a gravitációs formatöltés helyettesítése céljából aformafém felület célirányos nedvesítési viszonyainak a kialakítására is [J15].” p.269 --J15-c3. P.Bárczy: Universal Multi-Zone Crystallizator, the ISS Oriented Hungarian Apparatus Materials ScienceForum, 329-330 (2000) 219-228 – no text is given, only the reference No. 4.J15-c4. Bárczy P., Babcsán N., Szőke J., Bárczy T.: A miskolci űrkemence - BKL Kohászat, 2000., 133. évf., 6-7. szám, 263-268.o. – “A CSSZK-1 belsejének hőmérsékletviszonyait a Fémtani Tanszék éveken átvizsgálta, modellezte és publikálta …[J15]” p. 263.J15-c5. P.Bárczy: Universal multizone crystallizator (UMC) – novel challenges and results – Vacuum, 61 (2001)419-425. – “Some years later, the temperature maps inside the capsule travelling in the tube of CSSZK1were measured and also modelled by the Institute [J15]”, p.419.J14. Kaptay G., Berecz E. Determination of the excess thermodynamic functions ofcomponents of binary salt melts in infinitely diluted solution on the basis of the idealassociated solution model. - Chemical Papers (Chemické Zvesti), 1991., v.45., N.2., pp.145-158 (IF = 0,224 (1994-es adat)79

J14-c1. Török B.: Matematikai segéderőként alkalmazható programrendszer használata ’nyersvasmetallurgiaisalakra felállított asszociált oldat-modell számításainál - in: Proc. of microCAD '97 InternationalComputer Science Conference, Section B: Metallurgy, 1997. pp. 89-93. – „Előadásom metallurgiaivonatkozása egy adott összetételű nyersvasmetallurgiai salakra felállított fizikai kémiai modell, ’amelya salakrendszert ideálisan asszociált oldatként kezeli [J14]” p.89 –J14-c2. Török Béla: A TiO 2 hatása nagyolvasztói salakok néhány metallurgiai tulajdonságára, Ph.D. értekezés,1998., 113 o. – „Számításaimhoz a Miskolci Egyetem Fizikai Kémiai Tanszékén egy korábbankidolgozott, ideálisan asszociált oldatokra készült modellt használtam fel segítségül [J14]. A modellmás, kémiai jellegű kutatások alkalmával már bevált, nyersvasmetallurgiai felhasználására ez az elsőalkalom….” p.59. –J14-c3. M.Z.Benkő: On the computer software for the LD converter process at the Dunaferr Works, Materials’World (e-journal, http://materialworld.uni-miskolc.hu, July, 2001 – “The heat due to complex formationwas estimated by the associated model for the slag [J14].” – p. 6.J14-c4. Yaghmaee MS, Shokri B: Modeling the formation of strong couples in high temperature liquid -JOURNAL OF APPLIED PHYSICS 102 (1): Art. No. 014307 JUL 1 2007 – “The basic concept of themodel of an ideally associated mixture is that the major part of interaction between the components isconsumed through the formation of couples (associates) in the liquid phase [J14], while the mixture ofcouples and free atoms is treated as an ideal solution” – p.2, “It can be shown that the thermodynamicactivity of the mmacroscopic components is equal to the mole fraction of monomers in our model [J14]– p.3. “The equilibrium constant of the formation of FeAl can be estimated from the measured activitycoefficient of Al in pure liquid Fe at an infinitely dilute solution as follows [J14] (equation)” – p.3,J.13. Kaptay G. A theory of shapeforming processes by solidification under microgravityconditions. Part I. Basic Principles. Planar liquid/solid interface. - Materials Science ForumVol.77 (1991) pp.125-146 (IF = 0)J.12. Kaptay G., Lámer G. A theory of shapeforming processes by solidification undermicrogravity conditions. Part II. Melts covered by a deformable film. Solidification of Alalloys- Materials Science Forum Vol.77 (1991) pp.147-158 (IF = 0)J.11. Kaptay G. On surface properties of molten aluminum alloys of oxidized surface -Materials Science Forum Vol.77 (1991) pp.315-330 (IF = 0)J11-c1. D.A.Weirauch, W.M.Balaba, A.J.Perrotta: Kinetics of the reactive spreading of molten aluminum onceramic surfaces - J.Mater.Res., vol. 10., No.3., 1995, 640-650 – „Experimental conditions in this studywere chosen to avoid the severe retarding effects of the aluminium oxide film which are generallyknown to affect sessile drop experiments [J11]…” – p.640 –J11-c2. Csepeli Zsolt: Irányítottan kristályosított volfrám szállal erősített alumínium mátrixú kompozitszerkezete - PhD értekezés, Miskolc, 1997 – „A szálerősítésű kompozitok előállításához soklépcsős,nehezen automatizálható eljárásokat használnak. Az alkalmazott módszer egyik legnagyobb problémájaaz optimális nedvesítés biztosítása a szál és a mátrix között [J11].” – p.4.J11-c3. J.L.Sommer: High conductivity, low cost aluminum composite for thermal management – Reportsponsored by Defense Advanced Research Projects Agency, 1997, 57 pp. – „Kaptay suggests thatmolten aluminum will wet all ceramic surfaces if the oxide skin layer could be overcome [J11]…. Manyresearchers have shown that surface properties (surface tension, reactivity, etc…) of molten aluminumare more characteristic of super-cooled liquid Al2O3 than molten aluminum, particularly as the partialpressure of oxygen within the system is increased [J11]. As suggested by Kaptay, the contact angle ofmolten alumium on a wide range of ceramic substrates will fall below 90 degrees above approximately950 C in low vacuum environments [J11]. This transiiton temperature is most likely due to the Al2O3reacting with the liquid aluminum forming gaseous Al2O, according to the following chemicalreaction:… „ – p.23.J11-c4. Csepeli Zs., Sólyom B., Gácsi Z., Buza G., Teleszky I., Kovács Á.: Részecske-és szálerősítésűfémmátrixú kompozitok előállítási lehetőségei - BKL Kohászat, 131 (1998) 41-47 – „.. a bevonatnakegyszerre kell meggátolnia a szál és a mátrix közötti diffúziót és biztosítani a bevonat és a mátrixközötti tökéletes nedvesítést [OJ11]. A két, egymásnak sokszor ellentmondó feltételnek jól megfelel aTiB 2 bevonat [J11]…” p. 45. –80

J11-c5. J.A.Vreeling, V.Ocelik, Y.T.Pei, D.T.L.van Agterveld, J.T.M. de Hosson: Laser Melt Injection inAluminum Aloys: on the Role of the Oxide Skin – Acta mater. 48 (2000) 42-33 – „The oxide layer onmolten Al has a substantial influence on the wetting behavior of ceramic particles with liquid Al[J11]….. For instance, at lower temperatures (640-850 o C), the contact angle between an SiC particleand the Al melt is about 130 o , while at higher temperatures (>1100 o C) the contact angle is decreased toabout 50 o [OJ11].” – p.4225, „…the ex-situ experiments underline the behavior of this oxide skin as afunction of temperature [J11] – {18 sor magyarázat a cikkem alapján}” – p.4230.J11-c6. S.J.Roach, H.Henein, D.C.Owens: A New Techniques to Measure Dynamically the Surface Tension,Viscosity and Density of Molten Metals – Light Metals 2001, ed. by J.L.Aujier, TMS, Warrendale,2001, pp.1285-1291 – “The high surface activity of Al 2 O 3 is firmly established in the literature [J11, ..].The equilibrium constant for the formation of Al 2 O 3 is extremely large (K = 1,3 . 10 71 ). It is very difficultto reach the low oxygen partial pressure necessary to avoid formation of Al 2 O 3 [J11]” – p. 1289.J11-c7. K.I. Ibragimov, B.B.Alchagirov, T.M.Taova, A.M.Chochaeva, K.B.Khokonov: Surface Tension ofAluminium and its Alloys with Indium and Tin -–Trans. JWRI (Joining and Welding ResearchInstitute), 2001, vol. 30., Special Issue, 323-327 – „.. to study the physicochemical properties ofaluminium alloys … is a very difficult problem because of very high affinity for oxygen of liquidaluminium. To study the surface properties of Al alloys the special instruments and devices, andimprovement of researching methods are required [J11].” – p.323.J11-c8. J.A.Vreeling, V.Ocelik, Y.T.Pei, J.Th.M.de Hosson: Laser Melt Injection of SiC Particles in Al – in:„Surface Modification Technologies XIV”, ed. by T.S.Sudarshan and M.Jeandin, ASM International,Materials Park, OH, USA, 2001, pp. 619-623. – It is known from literature [J11] that the oxide layer onmolten Al has a big influence on the wetting behaviour of ceramic particles with liquid Al….” - p.622.„In literature it is reported that at low temperatures (640 – 850 o C) the contact angle between the SiCparticles and Al melt is about 130 o , while at higher temperatures (>1100 o C) the contact angle isdecreased to about 50 o [J11].” – p.623.J11-c9. A.Vreeling: Laser Melt Injection of Ceramic Particles in Metals – PhD Thesis, University of Groningen,Holland, 2001, pp. 136., Chapter 3. – „The oxide layer on molten Al has a substantial influence on thewetting behaviour of ceramic particles with liquid Al [J11]… „ – p.34., „.. the ex-situ experimentsunderline the behaviour described by literature [J11]. Kaptay [J11] studied the behaviour of the oxideskin, as function of temperature. The oxide skin is present on the melt till about 850 o C. Above thistemperature, chemical interactions between Al and it oxide at the interface occur, leading to theformation of gaseous sub-oxides. Consequently, the oxide gradually disappeares and the Al surface, bygrowing Al islands, takes over with increasing temperature. At about 1100 o C the oxide is totallyremoved.” – p.41., „The oxide layer has a strong influence on the wetting behaviour. The contact anglebetween SiC and Al with oxide skin is 130 o , between SiC and Al without oxide layer 50 o , i.e. when thesurface of the Al melt is oxidized there is non-wetting behaviour, while for a clean surface there iswetting behaviour. Actually, the oxide skin prevents direct contact between the particle and Al liquid, atlow temperatures, while when no oxide layer is present there is direct contact between the particle andAl liquid. This results in chemical interactions between the particle and Al melt that lowers the energyof particle/Al interface. The wetting behaviour is therefore improved [J11]. This explains theconnection between temperature of the melt and wetting behavior. At lower temperatures (< 850 o C) ofthe melt, an oxide layer is present and therefore there is non-wetting behavior, while at highertemperatures of the melt (> 1100 o C), the oxide layer is disappeared, which lead to wetting behavior” –p. 50.J11-c10. L. Moraru: Surface tension of molten AlSi 12% in ultrasonic field -Proceedings of Fourteenth International Conference on Surface Modification Technologies; 2001, Paris;France; pp. 572-574. Institute of Materials, (ISSN: 1366-5510), 2001, vol.750,J11-c11. N.Babcsan, D.Leitlmeier, H.P.Degischer: Foamibility of Particle Reinforced Aluminum Melt – Mat.-wiss. u. Werkstofftech., 2003, vol.34, pp.22-29 – „Different authors published data of surface tension ofliquid aluminum and its alloys (good summary can be found in [J11])” – p.3.J11-c12. N.Babcsán: Ceramic Particle Stabilized Aluminum Foams – PhD Dissertation, Miskolc, 2003 - “Above1050 o C the oxide layer of aluminum melt could transform to gaseous aluminum sub-oxides releasingfrom the melt [A9]: 4Al + Al 2 O 3 = 3 Al 2 O” – p.20, “Different authors published data of surface tensionof liquid aluminum and its alloys (good summary can be found in [J11]). ….. Kaptay [J11] extrapolatedand compared the surface tension data of liquid Al 2 O 3 with surface tension of the oxidized moltenaluminum. He states, that oxygen, covering the surface of molten aluminum at relatively lowtemperatures is in a state of supercooled Al 2 O 3 ” – p.23.J11-c13. V.Ocelik, S.Nijman, R.van Ingen, U.Oliviera, J.Th.M. De Hosson: Laser melt injection of hard particlesinto Al and Ti alloys – processing, microstructure and mechanical behaviour – in: Surface TreatmentVI., Computer Methods and Experimental Measurements for Surface Treatment Effects, ed. by81

C.A.Bubbia, J.Th.M.de Hosson, S.I.Nishida, WIT Press, 2003, pp.140-153 – “Kaptay [J11] studied thebehaviour of this oxide skin, as a function of temperature and concluded that the oxide skin is presenton the melt till about 850 o C and above this temperature, chemical reactions between Al and its oxide atthe interface occur, leading to the formation of gaseous sub-oxides. Consequently, the oxide graduallydisappears and the Al melt surface takes over with increasing temperature by growing Al islands. Atabout 1100 o C the oxide is totally removed, according of analysis of indirect observations [J11].” –p.144J11-c14. J.Th.M.de Hosson, B.J.Kooi: Microstructure and properties of interfaces between dissimilar materials –in: „Handbook of Surfaces and Interfaces of Materials, vol.1., Surface and Interface Phenomena”, ed.by H.S.Nalwa, Academic Press, San Diego, 2001, Chapter 1, pp.1-113 (ref. No.246). – „The oxide layeron molten Al has a substantial influence on the wetting behaviour of ceramic particles with liquid Al[J11]. Usually the oxide skin forms an energy barrier for the particles to penetrate...” – p.77,J11-c15. De Hosson JT, Ocelik V, Oliveira U: Coatings with laser melt injection of ceramic particles, Surf Engin Mater Sci II, 2003, pp. 197-207.J11-c16. De Hosson JTM ; Ocelik V: Functionally graded materials produced with high power lasers, Mater SciForum, 2003, vol. 426-4, pp. 123-130.J11-c17. Magyar Anita: Karbon szállal erősített alumínium mátrixú kompozitok Al/C határfelületénekjellemzése – PhD értekezés, Miskolc, 2004. „Kaptay felvet egy kiemelkedő problémát, miszerint azalumínium olvadék felületét vékony oxidhártya fedi, amely valamelyest lecsökkenti a felületi feszültségértékét. Ennél azonban sokkal drasztikusabbnak ítéli az oxidhártya hatását az adhéziós energiára. Azoxidhártyát tehát valahogyan el kell távolítani. Kaptay szerint lehetséges megoldás az előzőekbenkifejtett nagyvákuum + nagy hőmérséklet + kis oxigén parciális nyomás recepten kívül az, ha azalumíniumot pl. 3 t%-nyi Mg-al ötvözzük, amitől a tiszta alumíniumon a tömör oxidhártya szerkezeteátalakul, és rajta keresztül lehetővé válik az alumínium és a kerámia valós kontaktusa [J11]” – p.27.J11-c18. J.Th.M.deHosson, V.Ocelik, Y.Pei: Surface Engineering with lasers. Chapter 16 of the book “SurfaceModification and Mechanisms – Friction, Stress and Reaction Engineering”, ed. by G.E.Totten,H.Liang, Marcel Dekker Inc, New York, 2004, pp.603-669.82

J11-c19. C.Körner, M.Arnold, R.F.Singer: Metal foam stabilization by oxide network particles – Mater. Sci.Eng., 2005, vol.A396, pp.28-40.: “The wetting behaviour of solid materials by molten aluminium isstrongly influenced by an oxide layer covering the surface of the melt [J11]. Generally this oxide layerprevents wetting of molten aluminium with Al 2 O 3 ” – p.34.J11-c20. S.J.Roach, H.Henein: A new method to dynamically measure the surface tension, viscoisty and densityof melts – Metall.Mater.Trans., 2005, vol.36B, pp.667-676 – „Oxide accumulation has been known toaffect the surface tension of these liquids in the presence of very low levels of oxygen [J11]” – p.667,„Kaptay stated that measurements have traditionally been performed in the presence of a layer ofsupercooled Al 2 O 3 on the surface” – p.672.J11-c21. Ricci E, Arato E, Passerone A, Costa P: Oxygen tensioactivity on liquid-metal drops – Adv. Coll.Interface Sci., 2005, vol. 117, pp. 15-32 – “Experimental work has shown clear evidence of a decreasein the contact angle of metals and oxides with a decrease in the oxygen contant of the metal [J11]” –p.16.J11-c22. DA Weirauch: Technologically significant capillary phenomena in gigh-temperature materialsprocessing. Examples drawn from aluminum industry – Current Opp Solid State and Mater Sci, 2005,vol.9, pp.230-240 – „The wetting transition temperature is strongly dependent ont he details of theexperiment [J11]. A consequence of the dominating effect of oxide film behaviour in sessile dropexperiments involving aluminium is that alloying elements that alter the nature of the oxide film areoften mistakenly concluded to alter wetting behaviour” – p.233, „Elements like Mg, that are claimed tobe surface active in molten aluminum through their greater affinity for oxygen than aluminum, also alterthe structure of the oxide film and promote penetration of refractories by aluminum [J11]” – p.234,„One must therefore remain cognizant of the proximity to the 900 – 100 o C wetting transitiontemperature of aluminum alloys [J11]” – p.237J11-c23. Townsend C., Henein H., Corbin S., Apte P.: Static and dynamic wettability of molten Al on Al2O3and ZrO2 substrates – Science and Engineering of Composite Materials, 2006, vol.13, pp.65-77 –„Kaptay discussed the role of alumina on the surface properties of molten aluminium [J11]. He clearlyshowed that the surface tension of molten aluminium covered with alumina decreased with increasingtemperature. In addition, the surface tension of molten alumina increased with decreasin gtemperature.The surface tension of aluminum covered with alumina seemed to coincide with the surface tension ofmolten alumina at the melting point of alumina. This suggests that at temperatures lower than themelting point of alumina, the surface tension of aluminium is influenced by that of alumina.Furthermore it was suggested that the increased thermodynamic stability of Al 2 O gas with increasingtemperature contributes to the reduced surface tension of aluminum.” – p. 71.J11-c24. Giuranno D, Ricci E, Arato E, Costa P.: Dynamic surface tension measurements of an aluminiumoxygensystem - ACTA MATERIALIA 54 (10): 2625-2630 JUN 2006 – “The value of surface tensionof ‘pure aluminium’ is affected by a large scatter. Review papers [.. J11..] indicate values in the rangeof 850 – 1050 N/m at temperatures close to the melting point.” – p.2626.J11-c25. N.Babcsán, J.Banhart: Metal Foams – towards high-temperature colloid chemistry – Chapter 11 in:„Colloidal particles at Liquid Interfaces, ed. By B.P.Binks, T.S.Horozov, Cambridge University Press,2006, pp.445-499 – „Various authors have published surface tension data of liquid aluminium and itsalloys. … A good overview can be found in [J11].” – p.462.J11-c26. L.Bonaccorsi, E.Proverbio, N.Rafaelle: Microstructural investigation of interface phenomena duringPM billets foaming in hollow metal profiles. In: METFOAM-2007, ed. by L.P.Lefebre, J.Banhart,D.C.Dunand, DEStech Publ. Inc, 2008, pp.87-90. – It is known that molten unoxidized aluminium has ahigh surface tension so that it can wet any solid material [J11]. The oxide layer which normally coverthe aluminium reduces a lot the surface energy so the contact angle, a measure of wetting capability of aliquid on a surface, is typically around 160 o , a value that display the non-wetting of solids by moltenoxidized aluminium [J11].” – p. 88.J11-c27. Davis JL, Mendez PF: Wrinkling phenomena to explain vertical fold defects in DC-cast Al-Mg4.5 -LIGHT METALS 2008, ed. by DeYoung DH, TMS, 2008, pp. 733-748. –„This is consistent with theclassic oxidation literature for molten aluminium as described by [J11]” – p.737.J11-c28. A.V.Biakova, V.P.Krasovskii, A.O.Dudnik, S.V.Gniloskurenko, A.I.Sirko: O roli smachivaemosti Iraspredeleniia tviordich chastic v stabilizacii vspenennich aliuminievich rasplavov – Adgeziia rasplavovI paika materialov, 2009, vip.42, pp.5-22. – “Bolshinstvo opublikovannich v literaturedannich (naiboleepolno predstavleno v obzore [J11]) po poverhnostnomu natiazheniu binarnich I mnogokomponentnichaliuminievich rasplavov otnositsia k oblasti temperature, namnogo previshaiushich temperaturevspenivaniia. Na tochnost rezultatov okazivaiut vliianie plionki Al2O3, prisutstvuiushie na poverhnostizhidkogo aliuminia.” – p.8.J11-c29. H.Görner: Removal of dissolved elements in aluminium by infiltration – PhD Thesis, NorwegianUniversity of Science and Technology, Trondheim, 2009 (supervisor: TA Engh). – “Elements like Mg83

alter the structure of the oxide film and promote penetration of refractories by aluminium [J11]”. – p.13.“The wetting transition temperature is stronglz dependent on the details of the experiment (thickness ofoxide film, temperature, local oxzgen partial pressure) [J11]” – p.67.J11-c30. L.Bonaccorsi, E.Proverbio, N.Raffaele: Effect of interface bonding on the mechanical response ofaluminium foam reinforced steel tubes – J Mater Si, 2010, vol.45, pp.1514-1522 – “The chemicalreaction can occur if liquid aluminium wets the metal case, but the pre-existing oxide film covering theprecursors and the enhanced foam oxidation during the heat treatment in air do not allow any sort ofchemical bonding at the foam-tube interface [J11]” – p.1517.J11-c31. A.Ott: Oberflachen modification von Aluminium legierungen mit Laserstrahlung. Dissertation Uni-Stuttgart (prof. H. H-gel), Herbert Utz Verlag, 2010.J11-c32. V. Ocelik, J.Th.M. De Hosson: Laser melt injection of ceramic particles in metals: processing,microstructure and properties – Int J Microstr Mater Process, 2010, vol.5, pp.116-163.J11-c33. Lai-Xin Shi, Ping Shen , Dan Zhang, Qi-Chuan Jiang: Wetting and evaporation behaviors of moltenMg–Al alloy drops on partially oxidized α-SiC substrates – Mater Chem Phys, 2011, vol.130, pp.1125-1133 – “Up to date, the wettability of SiC by pure Al and Al alloys with low concentrations of Mg(usually no more than 5 wt.%) has been investigated by many researchers [J11]” – p.1125.J.10. Borisoglebskii Yu.V., Vetyukov M.M., Karimov M.I., Kaptay G., Shkuryakov N.P.Study of wetting of refractory compounds and composites by cryolite/alumina melt andmolten aluminum (in Russian) - Tsvetn. Met. (Moscow), 199I, (2), 4I-3 (IF = 0)J10-c1: R.P.Pawlek: Recent developments of aluminium wettable cathodes for the Primary aluminium industry,part II. – ALUMINIUM, 72. Jarhgang, 1996 – ½, pp. 35-41 – “Borisoglebskii et al. also examined thepossibility of using aluminium wettable refractories in aluminium smelting….Then they examined [J10]how liquid aluminium wets graphite, titanium nitride, and composites of TiN – TiC - TiB 2 , TiB 2 – TiCcompounds and TiB 2 coatings showed the best resistance….” P.36 –J10-c2. Vedernikov G.F.: Inertnie katodi v elektroliziorach dlia proizvodstva aliuminia. Problemi i perspektivi.AO VAMI, Informacionnii listok, No.10, April 2001. – „Issledovali, kakim obrazom zhidkii aluminiismachivaet grafit, nitrid titana, i kompozicionnie materiali TiN-TiC i TiB 2 – TiC, i ustanovili, stopokritie TiB 2 okazalos naibolee stoikim [J10]” – p. 9.J.9. Borisoglebskii Yu.V., Akhmedov S.N., Kaptay G., Vetyukov M.M., Dzambo P., RatnerA.Kh. Stability of metal-like refractory compounds in chloride melts (in Russian) - Tsvetn.Met. (Moscow), 1990, (6), 60-63 (IF = 0)J.8. Kaptay G. Kémiai reakciók vizsgálata klóraluminát olvadékban - BKL Kohászat, 123.,1990., 2. szám, 88-91. o. (IF = 0)J.7. Kaptay G., Borisoglebskii Yu.V. Evaluation of limiting activity coefficients of aluminumsubchloride in chloro-aluminate melts (in Russian) - Rasplavy, 1990, (1), 42-47 (IF = 0)J.6. Borisoglebskii Yu.V., Kaptay G., Vetyukov M.M., Gorlanov E.S. Solubility of aluminumin chloro-aluminate melts (in Russian) - Tsvetn. Met (Moscow), 1989, (12), 53-6 (IF = 0)J.5. Kaptay G., Akhmedov S.N., Borisoglebskii Yu.V., Zalite I. Thermodynamic properties ofmetal-like refractory compounds and their intermetallides with aluminum (in Russian) - Latv.PSR Zinat. Akad. Vestis, Kim. Ser. 1989, (2), 174-81 (IF = 0)J5-c1. G.Balducci, A.Ciccioli, G.Gigli, D.Gozzi, U.Anselmi-Tamburini: Thermodynamic Study of IntermetallicPhases in the Hf-Al System – J. of Alloys and Compounds, 1995, vol.220., pp.117-121 – „In the eventof any experiental data for the Hf-Al system not being available …. the estimated S 298 o values forHfAl 3 (s) and HfAl 2 (s) [J5] were utilized….. Finally, the entropy values S 298 o for Hf 2 Al 3 (s), Hf 5 Al 4 (s)and HfAl(s) were interpolated from the estimated values for HfAl 3 (s), HfAl 2 (s) and Hf 2 Al(s) [J5]”p.119.J5-c2. Magyar Anita: Karbon szállal erősített alumínium mátrixú kompozitok Al/C határfelületének jellemzése –PhD értekezés, Miskolc, 2004. „Amennyiben az Al 3 Zr képződési szabadentalpia értékét [J5]-ből84

veszem, a szabadentalpia változásra pozitív értéket kapok” – 37.o., „Következésképpen a határfelületennagyobb valószínűséggel képződik TiC” [OJ5] – 39.o.J5-c3. Kálazi Z. (Buza G.): Alumínium lézersugaras felületötvözése – PhD szemináriumi beszámoló, 2008.december 9., Miskolci Egyetem, 22 oldal. – „Az Al 3 Nb képződési entalpiája -118,8 kJ/mol [J5]” – 8. o.J.4. Ratner A.Kh., Kaptay G. Evaluation of thermodynamic properties of molten aluminumtrifluoride (in Russian) - in : Trudi VAMI, "Povysh. Effektiv. i Nadezh. Raboty Alyum.Elektrolizerov", Leningrad, 1988, 103-6 (IF = 0)J.3. Kaptay G., Akhmedov S.N., Borisoglebskii Yu.V. Thermodynamic evaluation of thereactions of metal-like refractory compounds with molten aluminum (in Russian) - Izv.Vyssh. Uchebn. Zaved., Tsvetn. Metall. 1988, (6), 70-7 (IF = 0)J3-c1. Karimov M.I.: Development of refractory composite materials for cathodic materials to be used inAluminum electrolysis cells (in Russian). PhD Thesis, Leningrad, 1989, 274 p. (reference No 171)J3-c2. Duschanek, P.Rogl : The Al-B (aluminum-boron) system – J. Phase Equilibria and Diffusion, 1994,vol15, pp. 543-552 – „Thermodynamic data have been established by various reseacrh gropus [J3]....The coefficients for specific heat are: .... [J3]...” – p. 550, „In table 6 the entropy of αAlB 12 = 88.4J/molK [J3]”.J3-c3. Csepeli Zs., Sólyom B., Gácsi Z., Buza G., Teleszky I., Kovács Á.: Részecske- és szálerősítésűfémmátrixú kompozitok előállítási lehetőségei - BKL Kohászat, 131 (1998) 41-47 – „.. a bevonatnakegyszerre kell meggátolnia a szál és a mátrix közötti diffúziót és biztosítani a bevonat és a mátrixközötti tökéletes nedvesítést. A két, egymásnak sokszor ellentmondó feltételnek jól megfelel a TiB 2bevonat [J3]…” p. 45. –J3-c4. R.P.Pawlek: Recent developments of aluminium wettable cathodes for the primary aluminium industry,part II. – ALUMINIUM, 72. Jarhgang, 1996 – ½, pp. 35-41 – “Borisoglebskii et al. also examined thepossibility of using aluminium wettable refractories in aluminium smelting. First they studied thepublished themodynamic data so as to calculate the equilibrium constants for reactions of transitionmetal borides, nitrides and carbides with molten aluminium [J3].” p.36 –J3-c5. Vedernikov G.F.: Inertnie katodi v elektroliziorach dlia proizvodstva aliuminia. Problemi i perspektivi.AO VAMI, Informacionnii listok, No.10, April 2001.(ref.No.53) – „Borisoglebskii Yu.V. i drugieobobshili opublikovannie dannie po termodinamike dlia raschota konstant ravnovesiia reakcii perehodaboridov, karbidov i nitridov metallov pri reakcii s rasplavlennim aliuminiem [J3]” – s.9.J3-c6. Ratner A.H., Geilikman M.B., Aleksandrovski S.V., Jiang F., Li H-G., Yin Z-M.:Thermodynamiccalculation on metallic thermoreduction during preparation of aluminum-rare master alloys – Trans.Nonferrous Met.Soc.China, 2001, vol.11, 18-21 „The procedures of estimating the standard formationenthalpy of Al 3 Sc is as follows: 1) estimate standard formation enthalpy of Al 3 Sc (-168 kJ/mol) byvariation regularities of standard fromation enthalpies of transition metal trialuminides of subgroup IV –VI reported by Ref.[OJ3]…..the estimated Gibbs energy formation energy of Al 3 Sc at eutectictemperature is –138 kJ/mol, which is very near to the average values in Refs. [J3]. ” – p.19, „inTable 1,the value of standard heat of formation of NbB 2 = -175 kJ/mol [J3]” – p.20.J3-c7. B.Liu, J.H.Edgar, Z.Gu, D.Zhuang, B.Raghothamachar, M.Dudley, A.Sarua, M.Kuball, H.M.Meyer III.:The Durability of Various Crucible Materials for Aluminum Nitride Crystal Growth by Sublimation -MRS Internet J. Nitride Semicond. Res. 9, 6(2004) – „From calculation [J3], the relative tendencies ofthese compounds to react with molten Al were HfC < TaC < NbC < TiC < WC, and TaN< TiN.”J3-c8. B.Predel: Landolt Börstein – Group IV Physical Chemistry, vol. 12A, supplement to subvolume IV/5a –Springer Berlin Heidelberg, 2006.J.2. Borisoglebskii Yu.V., Kaptay G., Vetyukov M.M., Boborin S.V. Durability of compositeelectrodes to be used in electrolythic deposition of aluminum from chloroaluminate melts (inRussian) - Tsvetn. Met. (Moscow), 1988, (10), 72-5 (IF = 0)J.1. Kaptay G., Borisoglebskii Yu.V., Vetyukov M.M. Equilibrium in the system moltenaluminum/chloroaluminate melt (in Russian) - Tsvetn. Met. (Moscow) 1988, (2), 40-1 (IF =0)85

B. Books and books chaptersB12. AI Grabcheko, G.Kaptay, AA Simonova, AP Tarasiuk, VV Dragobeckii, NV Verezub:Cutting of metals with nano- and submicron bulk structure (monograph), Harkov, Ukraine,2012, 218 pp. Tochka, Harkov, Ukraine (in Russian: Rezanie metallov s obiomnoi nano- isubmikrokristallicheskoi strukturoi).B11. G.Kaptay: Equilibrium of metallic nanoparticles – in: Nanoparticles: Productionpathways and appealing applications, ed. by T.Szörényi (ISBN: 978-963-9915-45-9), Collegeof Dunaújváros, Dunaújváros, 2011, pp. 95-113.B10. G.Kaptay, N.Babcsán: Particle Stabilized Foams. Chapter 7 in book: „FoamEngineering: Fundamentals and Applications” ed. by P.Stevenson, John Wiley & Sons, WestSussex, GB, 2012, pp.121-143.B9. Kaptay Gy.: Anyagegyensúlyok (makro-, mikro- és nanoméretű rendszerekben) - RaszterNyomda, 2011, 359 oldal, 500 példány.B9-c1. Roósz A.: Fémtan I. Raszter Nyomda, 2011.B8. Kaptay György: Határfelületi Nanojelenségek, digitális tananyag (48 dia), NemzetiTankönyvkiadó, 2011. - http://ydpteszt.infotec.hu/flipbooks/231/index_blue.htmlB7. Kaptay György: Nanoanyagok egyensúlya, digitális tananyag (24 dia), NemzetiTankönyvkiadó, 2011. - http://ydpteszt.infotec.hu/flipbooks/231/index_blue.htmlB6. G.Kaptay, G.Vermes: Interfacial forces: classification, in: Encyclopedia of Surface andColloid Science (ed by P.Somasundarar, A. Hubbard), Taylor & Francis Group, 2009, ISBN:0-87849-728-5, pp.1-19, DOI: 10.1081/E-ESCS-120044936B5. Kaptay Gy. Fémmátrixú kerámia kompozitok – 3.1. fejezet in: Műszaki felülettudományés orvosbiológiai alkalmazásai, szerk: Bertóti I., Marosi Gy., Tóth A., B+V Lap- ésKönyvkiadó Kft, Budapest, 2003, 47-59 o.B5-c1. Csanády Andrásné, Hargitai Hajnalka, Konczos Géza: Kompozitok – nanokompozitok – 2.1. fejezet in:Bevezetés a nanoszerkezetű anyagok világába (Csanády Andrásné, Kálmán Erika, Konczos Géza,szerk), MTA, ELTE Eötvös Kiadó, 2009, 45.o.B4. Kaptay Gy. Határfelületek energiaviszonyai és alapvető jelenségei – 2.2. fejezet in:Műszaki felülettudomány és orvosbiológiai alkalmazásai, szerk: Bertóti I., Marosi Gy., TóthA., B+V Lap- és Könyvkiadó Kft, Budapest, 2003, 22-46 o.B3. Fizikai-kémiai laboratóriumi gyakorlatok. Szerkesztette dr. Báder Imre. Szerző: dr BáderImre, Báder Enikő, Bolyán László, Dr. Bedő Zsuzsa, Csoma Gáborné, dr. Emmer János, dr.Kaptay György, dr. Lakatos István, dr. Lengyel Attiláné, dr. Raisz Iván, dr. Török Tamás.Miskolci Egyetemi Kiadó, 1998. (saját fejezet: Fémolvadék korróziós hatásának vizsgálatahatárfelületi jellemzők alapján. 2.4. Laboratóriumi gyakorlat, 16-20. o.)B2. G. Kaptay, E.Berecz: Electrochemical Synthesis from Molten Salts: an Application ofChemical Thermodynamics to the Synthesis of Refractory Compounds - published as Chapter11 in: „Chemical Thermodynamics - A ‘Chemistry for the 21 st Century’ monograph”, editedby Trevor Letcher, published by Blackwell Science, 1999, pp. 135-144.86

B2-c1. A.S.Uzdenova: Elektrochimicseskoe vosstanovlenie i sintez soedinenii gadoliniia, bora i aluminiia vgalogenidnich rasplavach – Dissertacia na soiskanie uchionoi stepeni kandidata khimicheskich nauk,Nalchik, 2000, 313 pp.: „..Raschot diagrammi elektrokhimicheskogo sinteza provodili po uravneniiu,privedionnomu v rabote [B2]…”, 104. o.B2-c2. H.B.Kushov, A.S.Uzdenova, M.K.Vindizheva, A.V.Zimin: Study of joint electroreduction of complexgadolinium (or lanthanum) ions with tetrafluoroborate-ions in halide melts – Advances in Molten Salts,2000., vol.1., pp. 291-297 „…calculation of the electrochemical synthesis diagrams were performed byus for the Gd-B system [..]. These calculations are performed based on the principle worked out in[B2]…” – p.295.B2-c3. H.B.Kushov, A.S.Uzdenova, M.K.Vindizheva, M.L.Balkizova: Study of joint electroreduction ofcomplex gadolinium, lanthanum, and fluroaluminate ions in halide melts – Advances in Molten Salts,2000., vol.1., pp. 285-290. „..First, calculation of equilibrium electrochemical synthesis diagrams wereperformed by us for the Gd-Al system [… ]. These calculations are performed based on the principleworked out in [B2]..” – p.288.B2-c4. S.V. Devyatkin: Influence of different conditions of electrochemical synthesis on the structure of thedeposited refractory compound coatings, Materials’ World (e-journal, http://materialworld.unimiskolc.hu,July, 2001 – “.. This is characteristic to electrochemical synthesis of tantalum diboride. Inthis case the layered type of coating structure has been obtained (see Fig. 3) […]. The formation of thisstructure has been theoretically explained […] using the Equilibrium Electrochemical Synthesis (EES)Diagrams [B2]” – p. 3.B2-c5. J. Sytchev, H. Kushkhov: Voltammetric Investigation of the Reduction Processes of Nickel, Cobalt, andIron Ions in Chloride and Chloro-Fluoride Melts, Materials’ World (e-journal, http://materialworld.unimiskolc.hu,July, 2001 – “High-temperature electrochemical synthesis from molten salts is a veryperspective way to produce compounds of high purity, including borides [B2…]”, p.1.B2-c6. H.B.Kushkhov, M.K.Vinizheva, A.S.Uzdenova, Z.A.Zhanikaeva: Joint electroreduction of lanthanum,gadolinium and boron in chloride melts – Electrochemical Society Proceedings vol.2002-19, pp.616-621 – “The calculation of the electrochemical synthesis diagram for the La-B system has been carriedout based on the principle worked out in [B2]” – p.618.B2-c7. V.V.Malyshev, High-temperature electrosynthesis of metal-like refractory compounds of group IV-VImetals in ionic melts – Russian J Inorg Chem, 2003, vol.48, pp.142-148 – “Earlier reviews systematizedinformation concerning electrosynthesis of refractory metal borides and methods of electrochemical andnonelectrochemical boronizing. So-called equilibrium electrochemical synthesis diagrams [B2] wereused to evaulate the possibility of the formation of the borides..” – p.144.B2-c8. Kh.B.Khushkhov, M.K.Vinidzheva, A.S.Uzdenova, Z.A.Zhanikaeva: Joint electroreduction oflanthanum, gadolinium and boron in halide melts – J. of Mining and Metallurgy, 2003, vol.39B,pp.275-280 – “…These calculations are performed based on the principle worked out in [B2]” – p.278B2-c9. V.V.Malishev: Visokotemperaturnii elektrochmnicheskii sintez metallopodobnich tugoplavkichsoedinenii metallov IV – VIA grupp v ionnich rasplavach – Zh. Neorg. Himii, 2004, vol.48, pp.187-194– “V obzorach [..B2] sistematizirovai raboti po elektrochmicheskomu sintezu boridov tugoplavkichmetallov, opisani metodi beztokovogo i elektrochmicheskogo borirovaniia. S pomoshiu ravnovesnichelektrochmicheskich diagram sinteza avtori [B2] ocenivaiut veroiatnost VES boridov 24 perehodnichmetallovi predskazivaiut ich vozmozhnuiu morfologiu” – p.190.B2-c10. V.V.Malyshev, Kh.B.Kushkhov: Advances in high-temperature electrochemical synthesis in ionic meltsby the onset of XXI century – Russ J. of General Chem., 2004., vol.74, pp.1139-1146 (Zh. ObsheiHimii, 2004, vol.74, pp.1233-1240) – „Using „equilibrium electrochemical synthesis diagrams”, Kaptayet al [B2] assessed the probability of high-temperature electrochemical synthesis of borides of 24transition metals and predicted their possible morphology” – p.1142.B2-c11. T.Watanabe, M.Kondo, A.Sagara: Nitriding of 316 stainless steel in molten fluoride salt by anelectrochemical technique – Electrochimica Acta, 2011, vol.58, pp.681-690. “Equilibriumelectrochemical synthesis diagram (EES) will give us a practical prospect about deposition of elementsand compounds on the surface of the specimen at a constant temperature [B2]… 6 equations….” –p.686.B1. Shapoval V.I., Kaptay G., Deviatkin S.V. High-Temperature Electrochemical Synthesisof Intermetallides of Titanium in Molten Salts - published as Chapter 18. of the book:"Electrochemical Technology: Innovation and New Developments", edited by N.Masuko,87

T.Osaka, and Y.Ito; copublished by Kodanscha Ltd and Gordon and Breach SciencePublishers S.A. in 1996 (pp. 361-378).B1-c1. F.Lantelme, A.Barhoun, A.M.Zahidi, J.H.von Barner: Titanium, boron and titanium deposition in alkalifluorochloride melts – Plasmas & Ions, 1999, 2, 133-143 -- “..There is now some interest in thepreparation of intermetallides refractory metals from electrochemical deposition at high temperature[B1]. The purpose of the present paper is to investigate the reaction mechanism of the depositionprocess..” (p.133) –B1-c2. N.Ene: Electrosynthesis and electrochemistry of TiB 2 in molten electrolyte – Rev Roum de Chimie, 1999,vol.44, pp.643-650. – „The equilibrium potential needed for the synthesis to occur is given by theequation [B1]: {equation cited}” – p.648B1-c3. R.Krendelsberger, M.F.Souto, J.Sytchev, J.O.Besenhard, G.Fafilek, H.Kronberger, G.E.Nauer: Textureeffects in TiB 2 coatings electrodeposited from a NaCl-KCl-K 2 TiF 6 -NaF-NaBF 4 melt at 700 o C – J.Mining and Metallurgy, 2003, vol. 39B, No.1-2, pp.269-274 – „The electrodeposition of titanium andboron from high-temperature molten salt electrolytes seems a much more intersting approach, withlower energy consumption, lower level of impurities, and a more precise stoichiometry of the product[B1]” – p.270.B1-c4. T.P. Jose, L. Sundar, L.J. Berchmans, A. Visuvasam and S. Angappan: Electrochemical Synthesis andcharacterization of BaB 6 from molten melt - Journal of Mining and Metallurgy, 2009, vol. 45 B, No.1,pp. 101 – 109. – “The joint deposition of boron and barium in molten salts is explained by the so called‘Unstable stoichiometric way’ [B1] called ‘kinetic regime’ in the Russian literature. This will appear ifthe deposition potentials of boron and the second component of the boride, i.e. the metal component(MC) on inert cathodes are too far from each other. Barium is found to be more electronegative thanboron, so the depolarization of metal deposition should be taken into account. i.e. the condition is asfollows: …… when the above condition is fulfilled, first the macroscopic layer of one of thecomponents will be deposited on the cathode and the formation of boride will take place duringdepositing the second component on this layer with depolarization. In this case the synthesis of boride ispossible only above the limiting current density of the more electropositive component. Hence, thecomposition of the boride phase will strongly depend on the concentration of the ions of the moreelectropositive component in the melt i.e., boron concentration. It also depends on the actual cathodiccurrent density. It has been reported that during the crystal deposition, both the composition of the meltand the effective cathode surface area will continuously change, hence, the final composition of theboride will also be changed. This mechanism has been reported as ‘unstable stoichiometry way’ [B1].B1-c5. JRA Godinho: Optimization of TiB 2 coatings electrodepisted from halide melts – Master dissertation inChemistry, April 2008, 70 pp. – “The model proposed by Kaptay does not assume any specific complexstructure for the active species in solutiuon. It is instead based on adatom-adatom interaction at thesurface [B1]” – p.19.B1-c6. T.Watanabe, M.Kondo, A.Sagara: Nitriding of 316 stainless steel in molten fluoride salt by anelectrochemical technique – Electrochimica Acta, 2011, vol.58, pp.681-690. “Equilibriumelectrochemical synthesis diagram (EES) will give us a practical prospect about deposition of elementsand compounds on the surface of the specimen at a constant temperature [B1]… 6 equations….” –p.686.88

E. Books and-or journal issues, editedE6. N.Eustathopoulos, G.Kaptay, P.Nikolopoulos, A.Paserone: Guest Editors’ Editorial:HTC-2009 – J Mater Sci, 2010, vol.45, pp.1977-1978. Special issue of 6th HTC: 2010,vol.45, No.8, pp. 1977-2245E5. G.Kaptay (guest editor): Journal of Mining and Metallurgy, 2003, vol.39B, No.1-2,special issue „Electrodeposition and Electrochemical Synthesis from Ionic Liquids andMolten Salts”, 405 pp, Editorial (pp.1-2), Available at www.tf.bor.ac.yu/jmm.htm (go toSection B: Metallurgy, and to 39(1)B(2003)1-405)E4. Kaptay Gy. (szerkesztő) - Miskolci Egyetem, Doktoranduszok Fóruma 2002. november 6.- Anyag- és Kohómérnöki Kar szekciókiadványa, Miskolci Egyetem, 2003, 77 oldal.E3. Kaptay Gy. (szerkesztő) - Miskolci Egyetem, Doktoranduszok Fóruma 2001. november 6.- Anyag- és Kohómérnöki Kar szekciókiadványa, Miskolci Egyetem, 2003, 71 oldal.E2. G.Kaptay (guest editor): Materials’ World (e-journal with ISSN 1586-0140, accessible at:http://materialworld.uni-miskolc.hu), July 2001, 110 pp.E1. Kaptay Gy. (szerkesztő) - Miskolci Egyetem, Doktoranduszok Fóruma 2000. október 30.- Anyag- és Kohómérnöki Kar szekciókiadványa, Miskolci Egyetem, 2001, 67 oldal.89

JP. Journal papers on non-scientific issues (politics)JP14. Kaptay Gy., Krállics Gy.: Bemutatkozik a BAY-NANO kutatóintézet. Van-eperspektívája a nanotechnológiának az acélok gyártásában? – ISD Dunaferr MűszakiGazdasági Közlemények, 2007, XLVII. évf, 3. szám, 111-116. o.JP.13. Kaptay Gy.: (megjelent „Anonymus Kohászoktató” szerzői álnéven): Meddig él egycikkünk? - BKL Kohászat, 2006, 139. évf., 3. szám, 13-18 o.JP12. G.Kaptay: Book review for V.L.Cherginets, Oxoacidity: Reactions of Oxo-Compounds in IonicSolvents, vol.41 of the Series Comprehensive Chemical Kinetics, edited by N.J.B.Green, Elsevier,Amsterdam, 2005 - Electrochimica Acta, 2006, vol.51, pp.3181-3182JP11. Kaptay Gy., Z.Benkő M.: A kohászati és anyagmérnöki felsőoktatás jövője a bolognaifolyamatra való áttérés után – BKL Kohászat, 2006., 139. évf., 1. szám, 6-11JP11-c1. Dúl Jenő: A hazai öntészeti oktatás rövid története – kézirat, 2012 július, 36 oldal. „A hallgatók aszakirány-csoportokból választottak 2 szakirányt az érvényes szakirány-választási szabályok szerint. A(fél)szakirányok tantárgyait a hallgatók 22 kredit és kontaktóra keretben az 5-7. félévben tanulták [JP11].”– 5.o. „A Magyar Akkreditációs Bizottság (MAB) 2006-ban elfogadta a Műszaki Anyagtudományi Karáltal előterjesztett MSc anyagmérnök és kohómérnök szak tantervét. A képzési- és képesítésikövetelmények (KKK) és a tanterv elfogadtatásában jelentős szerepet vállalt az MTA MetallurgiaiBizottsága és a MAB szakterületünkhöz tartozó tagjai (Dr. Tardy Pál és Dr. Bakó Károly) [JP11]. „ – 7.o.JP.10. Kaptay Gy., Z.Benkő M.: A történelmi Kohómérnöki Kar szervezeti átalakítása és új képzésistruktúrája – DUNAFERR Műszaki Gazdasági Közlemények, 2004., 4. szám, 281-287.JP.9. Átalakulások az Anyag és Kohómérnöki Karon – dr. Kaptay György dékánnak azOMBKE 93. Küldöttgyűlésén elhangzott tájékoztatója – Bányászati és Kohászati Lapok,2004, 137. évfolyam, 4. szám, 37-38. o.JP9-c1. Dúl Jenő: A hazai öntészeti oktatás rövid története – kézirat, 2012 július, 36 oldal. „2004-ben a karivezetés a tanszékek összevonásáról döntött, ennek következtében a Vaskohászattani, a Fémkohászattaniés az Öntészeti intézeti tanszékeket Metallurgiai és Öntészeti Tanszék néven egyesítették [JP9]. „ – 12.o.JP.8. Kaptay Gy., Z.Benkő M., Tóth L., Károly Gy.: Beszámoló az Anyag- és KohómérnökiKaron történtekről a 2000. július 1. és 2003. október 15. közötti időszakban, avagykonszolidáció és újabb válságmenedzselés – BKL Kohászat, 2003., 136. évf., 3. szám, 113-120. oldalJP8-c1. Dúl Jenő: A hazai öntészeti oktatás rövid története – kézirat, 2012 július, 36 oldal. „A kettősspecializáció bevezetését a klasszikus kohómérnök-képzés iránti felvételi érdeklődés csökkenése és avégzettek elhelyezkedési lehetőségeinek kiterjesztése indokolta [JP8]” – 3.o. , „A fentiek és aDUNAFERR Zrt. privatizációját követő fejlesztések szakember-igénye alapján a Kari Tanács elé 2005tavaszán az a javaslat került, hogy a kohómérnöki szakon 4 szakirány helyett 2 szakirány legyen. A„metallurgus” szakirány és az „öntő” szakirány „metallurgiai és öntő szakirány” néven, a „hő- ésfelületkezelő” szakirány és az „alakítástechnológiai” szakirány „fémtechnológiai szakirány” névenkerüljön összevonásra. Ezt a javaslatot a fémtannal, az alakítástechnológiával és a metallurgiávalfoglalkozó kollégák jónak tartották, de erősen ellenezték az öntészet oktatók [JP8]” – 4.o.90

JP.7. G.Kaptay: On the activity of the LIMOS R&D Group in the field of Materials Science –Materials’ World (e-journal with ISSN 1586-0140, accessible at: http://materialworld.unimiskolc.hu),July, 2001.JP.6. Kaptay G., Z.M.Benkő: The new educational structure of the branch of metallurgicalengineering at the University of Miskolc – Materials’ World (e-journal with ISSN 1586-0140,accessible at: http://materialworld.uni-miskolc.hu), October, 2000.JP.5. Kaptay Gy., Z.Benkő M., Tóth L., Roósz A.: Beszámoló a karon 1999. júliusa és 2000.júniusa között történtekről (A Kohómérnöki Kar utolsó félévének és az Anyag- ésKohómérnöki Kar első félévének fontosabb történéseiről) – BKL Kohászat, 2000., 133.évfolyam, 6-7. szám, 221-229. o.JP.4. Kaptay Gy.: Rövid tájékoztató a TMS (AIME) 129., éves konferenciájáról – BKLKohászat, 2000., 133. évfolyam, 3. szám, 118.o.JP.3. Kaptay Gy.: Anyagfajták csoportosítása, avagy mi van a tetraéder csúcsában? A II.Országos anyagtudományi, anyagvizsgálati és anyaginformatikai konferencia és kiállítás(II.OAAAKK) emblémájának egyik lehetséges értelmezése. BKL Kohászat, 1999., 132. évf.,420.o.JP.2. Kaptay Gy., Z.Benkő M., Tóth L.: A Kohómérnöki Kar oktatási stratégiája - BKLKohászat, 1999., 132. évf., 6-7. szám, 228-235 o.JP.1. Kaptay Gy., Z.Benkő Mária, Tóth L., Roósz A.: A Kohómérnöki Kar átalakítása - az újmenedzsment első nyolc hónapja. BKL Kohászat, 1999., 132. évf., 6-7. szám, 222-227 o.91

P. Proceedings papersP.117. Á.Végh, Cs.Mekler, GKaptay: Optimization of the Ga-Bi monotectic systems andmodelling of surface phase transition line – CD-Proc. 26th microCAD Int Sci Conf, 29-30March, 2012, Miskolc, Hungary.P.116. J.Szabó, O.Nagy, G.Kaptay: Feasibility of in-situ stabilization of liquid metallicemulsions – CD-Proc. 26th microCAD Int Sci Conf, 29-30 March, 2012, Miskolc, Hungary.P.115. AA Simonova, G.Kaptay, NV Verezub: Opredelenie oblasti racionalnich usloviilezviinoi obrabotki submikrokristallicheskich metallov – Vestnik Nac. Tech. Uni HPI,53/2010, pp.114-121.P.114. N.V.Verezub, G.Kaptay, A.A.Simonova: The management of surface quality of metalwith nano and submicron crystalline structure during machining – „Suchasni Technologii vmashinobuduvanii – NTU, Harkiv, 2010, pp.244-249.P.113. N.V.Verezub, G.Kaptay, A.A.Simonova: Metodology of mechanical processes ofmachining bulk nano-crystal materials (in Russian) – „Suchasni Technologii vmashinobuduvanii – NTU, Harkiv, 2008, pp.19-26.P112. J.Sytchev, N.Borisenko, H.B.Kushkhov, G.Kaptay: On the temperature dependence oflithium intercalation into graphite as the first step of carbon nanotubes electrolytic production– Proc. of MS7, ed. by P.Taxil, C.Bessada, M.Cassir, M.Gaune-Escard, vol.1, 2005, pp.237-240.P111. Budai I., Babcsán N., Kaptay Gy.: Alumíniumalapú kompozit-olvadékviszkozitásmérésének problematikája és fejlesztése a Stokes módszer alapján – Tavaszi Szélkonferencia kiadványa, 2005, pp.48-5192

P110. P.Baumli, J.Sytchev, Zs.H.Göndör, G.Kaptay: Interaction of a titanium-containing meltwith SiO 2 and Al 2 O 3 – Proceedings of EUCHEM 2004 Molten Salts Conference, ed. byJ.Kazmierczak and G.Zabinska-Olszak, Wroclaw, 2004, pp.122-127P109. G.Kaptay: Role of Interfacial Phenomena in Processing Metal-Matrix CompositeMaterials – Proceedings of the 2nd International Symposium on Light Metals and CompositeMaterials, published by the Association of Metallurgical Engineers SCG, 2004, pp.81-84P108. I.Budai, M.Z.Benkő, G.Kaptay: Comparison of theoretical models, describing theconcentration dependence of viscosity of liquid alloys on the example of the Ag-Sb system -MICROCAD 2004 Int. Conf., Section: Materials Science, 2004, University of Miskolc,Hungary, pp.27-32.P108-c1. D.Zivkovic: Estimation of the viscosity for Ag-In and In-Sb liquid alloys using different models –Z.Metallkunde, 2006, vol.97, pp.89-93 – „Recently, Budai et al [P108] gave a complete comparativesurvey on theoretical models describing the concentration dependence of viscosity of liquid alloys withthe example of Ag-Sb system.” – p.89, „some of the calculation models could be in conflict withexperimental points, as was already shown in different cases [P108]” – p.90.P107. T.Bárczy, G.Kaptay: Modelling the infitlration of liquid metals into porous ceramics -MICROCAD 2004 Int. Conf., Section: Materials Science, 2004, University of Miskolc,Hungary, pp.13-17.P106. P.Baumli, J.Sytchev, Zs.H.Göndör, G.Kaptay: Study of chemical reactions between analumina plate and titanium-containing molten salt – MICROCAD 2004 Int. Conf., Section:Chemistry, 2004, University of Miskolc, Hungary, pp.15-21.93

P105. G.Kaptay: An improved interfacial model of stabilzation of metallic foams by solidparticles - in: “Cellular Metals: Manufacture, Properties, Application”, ed. by J.Banhart,N.A.Fleck, A.Mortensen, MIT Verlag, 2003, pp.107-112.P105-c1. V.Gergely, T.W.Clyne: Drainage in standing liquid metal foams: modelling and experimentalobservations - Acta materiala, 2004, vol.52, pp.3047-3058: „Interfacial criteria for stabilisation ofmetallic foams by solid particles have recently been derived by Kaptay [P105]” – p.3053P105-c2. C.Körner, M.Hirschmann, V.Brautigam, R.F.Singer: Endogenous particle Stabilization duringmagnesium integral foam production – Advanced Engineering materials, 2004, vol.6, No.6, pp.1-6. “Itis well known, that the development of foam requires some stabilization. For metals, stabilization isrealized by obstacles captured in the cell walls threby preventing further cell wall thinning. Theseobstacles may either be compact particles like SiC or Al 2 O 3 particles [P105] or complex structures, likeoxide fragments, which act as effective particles” – p.4.P105-c3. C.Körner, M.Arnold, R.F.Singer: Metal foam stabilization by oxide network particles – Mater. Sci.Eng., 2005, vol.A396, pp.28-40.: “Further progress to explain foam stability was made by Kaptay[P105]. He uses a model of a 3D network of solid, spherical particles to explain force transfer betweentwo interfaces and in this way stability” – p.28.P105-c4. Bryant JD, Wilhelmy D, Kallivayalil J, Wang W: Development of aluminum foam processes andproducts - ALUMINIUM ALLOYS 2006, PTS 1 AND 2 MATERIALS SCIENCE FORUM 519-521:1193-1200, Part 1-2 2006 – “.. the prior particle boundaries (and in some cases residual solid phases)can be used to provide stabilization [P105]” – p.1194.P105-c5. C.Körner: Integral Foam Molding of Light Metals – Physical and Technological Principles –Habilitation Thesis, Erlangen, 2006 – “Kaptay was the first who realized that stabilization for these kindof particles is based on the development of 3D network structures which transfer forces from oneinterface to the other [P105].” – p.108.P105-c6. C.Körner: Foam formation mechanism in particle suspensions applied to metallic foams – Mater SciEng A, 2008, vol.495, pp.227-235 – “Further progress to explain foam stability was made by Kaptay[P105] who uses a model of a three-dimensional network of solid, spherical particles to explain forcetransfer between two interfaces and in this way stability” – p.228.P105-c7. A.Dudka, F.Garcia-Moreno, N.Wanderka, J.Banhart: Structure and distribution of oxides in aluminiumfoam – Acta Mater, 2008, vol.56, pp.3990-4001. – „Two theories are mainly considered: i) the increaseof local viscosity to an extent that the flow of liquid is blocked, and ii). stabilization of films throughoxide agglomerations or networks acting as surface active particles and inducing a particle-basedstabilization mechanism similar to the one proposed for other foaming routes [P105]” – p.3990.P105-c8. C.Koerner: Integral Foam Molding of Light Metals – Springer, 2008, 224 pp. – „Kaptay [P105] wasthe first who realized, that stabilization for this kind of particles is based on the development of 3Dnetwork structures which transfer forces from one interface to the other” – p. 100.P105-c9. S.Beke: Metal foaming controlled by ultrasonic waves – PhD Thesis, TU Wien, 2011, supervisors: HPDegischer and N Babcsan. – „Several factors influence foam stability, including surface tension, …surface forces, … [P105]” – p.12.P105-c10. Garcia-Moreno F. ; Solorzano E. ; Banhart J.: Kinetics of coalescence in liquid aluminium foams -Soft Matter, 2011, Vol. 7 Issue: 19 pp. 9216-9223 -P104. R.Krendelsberger, A.Pascual, M.F.Souto, J.Sytchev, G.E.Nauer, G.Kaptay: Textures ofTiB 2 coatings from molten salts – Proc. of Int. Symp. On Ionic Liquids in Honour of MarcelleGaune-Escard, France, 26-28 June 2003, pp.95-103P103. G.Kaptay: Classification of interfacial forces, acting on solid particles in technologiesof advanced metallic materials – in: Proc. of Int. Conf. „Advanced Metallic Materials”, ed. byJ.Jerz, P.Sebo, M.Zemankova, IMMM, Slovak Academy of Sciences, 2003, pp. 135-140.94

P103-c1. C.Körner, M.Arnold, R.F.Singer: Metal foam stabilization by oxide network particles – Mater. Sci.Eng., 2005, vol.A396, pp.28-40: “It is generally accepted that foamability is intimately correlated withthe presence of particles [P103]” – p.28.P103-c2. C.Körner: Integral Foam Molding of Light Metals – Physical and Technological Principles –Habilitation Thesis, Erlangen, 2006 – “Kaptay was the first who realized that stabilization for these kindof particles is based on the development of 3D network structures which transfer forces from oneinterface to the other [P103].” – p.108.P103-c3. C.Körner: Foam formation mechanism in particle suspensions applied to metallic foams – Mater SciEng A, 2008, vol.495, pp.227-235 – “Now it is generally accepted that foamibility of metals isintimately correlated with the presence of particles [P103]. – p.227.P103-c4. C.Koerner: Integral Foam Molding of Light Metals – Springer, 2008, 224 pp. – „ Kaptay [P103] wasthe first who realized, that stabilization for this kind of particles is based on the development of 3Dnetwork structures which transfer forces from one interface to the other” – p. 100.P103-c5. G.S. Vinod Kumar, M.Chakraborty, F. Garcia-Moreno, J.Banhart: Foamibility of MgAl 2 O 4 (spinel-)reinforced aluminum alloy composites – Metall Mater Trans A, 2011, vol.42A, pp.2898-2908 –„Ceramic and intermetallic particles are required for foam stabilization [P103], which can be adisadvantage especially when SiC particles are used” – p.2898.P102. O.N.Verezub, Z.Kálazi, G.Buza, P.Boross, B.Verő, G.Kaptay: Surface Metal MatrixComposite Fe-Ti-C/TiC Layers Produced by Laser Melt Injection Technology – in: Proc. ofInt. Conf. „Advanced Metallic Materials”, ed. by J.Jerz, P.Sebo, M.Zemankova, IMMM,Slovak Academy of Sciences, 2003, pp. 297-300.P101. D.Zivkovic, G.Kaptay: A new approach to estimate viscosity of ternary liquid metallicalloys – Proceedings of the 35th International October Conference on Mining and Metallurgy,ed. by R.V.Pantivic, University of Belgrade, Serbia & Montenegro, 2003, pp. 276-282P100. O.N.Verezub, A.I.Grabchenko, P.Boross, Z.Kálazi, B.Verő, G.Kaptay: Ulushsheniepoverhnostnogo sloia nizkolegirovannich instrrumentalnich materialov s pomoshiu lazernoitviordotelnoi implantacii – Vestnik Nacionalnogo technicheskogo Universiteta HPI, 2003,tom 1., No.8, pp.7-16.P99. Bárczy T., Kaptay Gy.: Az infiltráció elméleti alapjai – Fiatal Műszakiak TudományosÜlésszaka VIII., Erdélyi Múzeum Egyesület kiadványa, Kolozsvár, Románia, 2003., pp. 205-210P98 O.Verezub, P.Boross, Z.Kálazi, B.Verő, A.Grabchenko, G.Kaptay: Possibilities to ObtainW-alloyed, TiC-reinforced Composite Surface Layers on Carbon Steels by Laser MeltInjection. A theoretical Analysis. Proc. of microCAD 2003 Conference, Section Metallurgy,University of Miskolc, 2003, pp. 59-64.P97. A.Borsik, Cs.Varga, G.Kaptay: A Software for Determining Surface Tension of LiquidMetals from the Shape of a Sessile Drop - Proc. of microCAD 2003 Conference, SectionMetallurgy, University of Miskolc, 2003, pp. 53-58.P96. G.Kaptay: A New Equation to Estimate the Concentration Dependence of the Viscosityof Liquid Metallic Alloys from the Heat of Mixing Data - Proc. of microCAD 2003Conference, Section Metallurgy, University of Miskolc, 2003, pp. 23-28.P96-c1. D.Zivkovic, D.Manasijevic: An optimal method to calculate the viscosity of simple liquid ternary alloysfrom the measured binary data – Calphad, 2005, vol.29, pp.312-316 – „Different models have beendeveloped to describe the viscosity of multicomponent alloys [P96]”, „The second group of models isderived regarding the activation energy of an alloy, the enthalpy of mixing and a correction associatedwith mixing of unlike atoms not involving an arbitrary parameter [P96]” – p.31295

P96-c2. D.Zivkovic: Estimation of the viscosity for Ag-In and In-Sb liquid alloys using different models –Z.Metallkunde, 2006, vol.97, pp.89-93 - „This paper presents the results of viscoisty estimation for theAg-In and In-Sb liqiud allos, using ….the Kaptay model [P96]…. The Kaptay equation [P96] wasdeveloped ….. ((11 lines + 1 equation))” – pp.90-91. „For the Ag-In alloys … the experimentalliterature data are in excellent agreement with the calculated results according to the Kaptay model atboth investigated temperatures” – p.91. „The model due to Kaptay describe the character of theexperimental data correctly at all investigated temperatures for both explored systems: - p.92.P96-c3. Brillo J, Brooks R, Egry I, Quested P: Viscosity measurement of liquid ternary Cu-Ni-Fe alloys by anoscillating cup viscometer and comparison with models - Int J Mater Res 98 (6): 457-462 JUN 2007 –Abstract: „Close agreement of the experimental results was found with the predictions of two models byKaptay and Hirai” p.457. „For this work we consider the following models:… the Kaptay-equation[P96]…” – p.457. „The Kaptay equation [P96] relates the activation energy to the enthalpy of mixingby introducing a semiempirical parameter, which has been estimated from the properties of pure metals:Eq.(6)” – p.458. As shown in Fig.7 the … Kaptay model, Eq.(6) agree well with the experimentaldata….. The best agreement is found for the Kaptay equation, which fits to the data very closely” –p.461. Conclusions: „…At constant temperature, the experimental results were compared to severalmodels and those of Kaptay and Hirai gave the closest agreement” – p.462.P96-c4. D.Zivkovic: Application of the Kaptay model in calculation of ternary liquid alloys viscosities – Int JMat Res, 2008, vol.99, pp.748-750 – „Conclusions: The equation derived by Kaptay [P96] to extrapolatethe dynamic viscosity of pure liquid metals to the viscosity of liquid metallic alloys has been applied andtested on ternary Au – Ag - Cu system. Calculates values have been compared with literature data andgood agreement was found” – p.750.P96-c5. D.Zivkovic: A new approach to estimate the viscosity of the ternary liquid alloys using the Budai-Benko-Kaptay equation – Metall Mater Trans B, 2008, vol.39, pp.395-398 – „The rarity and controversialcharacter of experimentally determinded viscosity data for the multicomponent alloys has influenceddevelopment of different theoretical models to describe the composition dependence of the viscosity ofliquid alloys [P96]” – p.395.P96-c6. J.Brillo, R.Brooks, I.Egry, P.Quested: Density and viscosity of liquid ternary Al-Cu-Ag alloys - HighTemperatures-High Pressures, 2008, Vol. 37, pp. 371–381 – “We find that the model of Hirai and Kaptay[P96] describe our data best” – p.373.P96-c7. P.Terzieff: The viscosity of liquid alloys of polyvalent metals with Cu, Ag and Au: Theoreticaltreatments based on the enthalpy of mixing – Physica B, 2009, vol.404, pp. 2039-2044 – „The majority ofthe currently used viscosity models are of semi-empirical nature focused on thermodynamic quantitiessuch as free energy of mixing [P96]” – 2039.P96-c8. P.Terzieff: Some physico-chemical properties of liquid Ag-Sn-Zn – Physica B, Condensed Matter, 2010,vol.405, pp.2668-2672 – „From a previous analysis it has been concluded that the semi-empirical apprachbased on Kaptay’s unified equation [P96] is one of the most convenient methods to gain a first idea of theviscosity of muticomponent systems, even if the viscosities of the pure liquids are unknown. Theapplication requires the melting temperatures of the components, their molar masses, and their molarvolumes. The only requirements for alloy is the knowledge of the excess volume and the enthalpy ofmixing : (Eq.10)” – p.2672.P96-c9. Gasior W, Moser Z, Debski A: New data to the SURDAT-database of modeled and experimentalphysical properties of lead-free solder alloys – Arch Metall Mater, 2009, vol.54, pp. 1253-1259 –„..SURDAT database … experimental … and the viscosity calculated from the dependences proposed by… Kaptay [P96] : Eq.(6)” – p.1256. “Fig.4. Experimental (symbols) and calculated (lines) viscosity (Eq-s(1, 2, 5, 6, 7) of Ag-Sn (Fig.4a) and Sn-Zn (Fig.4b) alloys” – p.1257.P96-c10. Knott S., Terzieff P.: Calculation of the viscosity of the liquid ternary Ag-Au-Sn system – Int. J. Mater.Res., 2010, vol.101, pp.834-838. – „Several viscosity models based on thermodynamic data exist, some ofthem apply adjustable parameters, while others make use of universal parameters [P96] which a reconsidered to be applicable to a large class of alloy systems” – p.834, “The expression for the viscosity,given by Budai et al. is based on Kaptay-s unified equation [P96] for pure liquid metals: Eq.(3)” – p.835.P96-c11. OK Echendu, EC Mbamala, BC Anusionwu: Theoretical investigation of the viscosity of some liquidmetals and alloys – Physics and Chemistry of Liquids, 2011, vol.49, pp.247-258 – “The Kaptay model[P96] .. takes into account the theoretical relationship between the cohesive energy of the alloy and theactivation energy of viscous flow” – p.249.P96-c12 T. Gancarz, Z. Moser, W. Gasior, J. Pstrus, H. Henein: A Comparison of Surface Tension, Viscosity,and Density of Sn and Sn–Ag Alloys Using Different Measurement Techniques - Int J Thermophys, 2011,vol.32, pp.1210-1233: „In 2004, Kaptay [P96] proposed a modification of the Seetharaman and Sichenmodel for viscosity calculations; it consists of substituting the excess free energy into the equation ofactivation energy with the enthalpy of mixing multiplied by an α coefficient, which, according to the96

author, amounts to 0.155 to 0.015, resulting in the following equation for the viscosity with the followingform…” – p.1230.P96-c13. Wunderlich RK; Fecht H-J: Surface tension and viscosity of NiAl catalytic precursor alloys frommicrogravity experiments – Int J Mater Res, 2011, vol.102, pp.1164-1173. „Various thermodynamicmodels of the viscosity of binary metallic alloys have been brough forward which include the interactionof the different atomic species in terms of an interaction parameter analogous to a regular solution model”– p. 1170.P96-c14. I.Egry, M.Schick: The viscosity of eutectic Pd-Si alloys - a case study – Int J Mater Res, 2011, vol.102,pp.1468-1472. „…it cannot be explained by semi-empirical models realting the viscosity to ther enthalpyof mixing [P96]” – p.1469.P96-c15. M.Schick, J.Brillo, I.Egry, B.Hallstedt: Viscosity of Al-Cu liquid alloys: measurement andthermodynamic description – J Mater Sci, 2012, doi: 10.1007/s10853-012-6710-x – “A similar expressionis derived by Kaptay [P96], who introduces the enthalpy of mixing multiplied with a semiempirical factor,which has been adjusted to a number of certain binary alloys: Eq.(5)” – p., “The curve calculated from themodel of Kaptay [P96] exhibits a similar shape without a pronounced maximum, predicting even lowerviscosities” – p.P96-c16. R.N.Singh, F.Sommer: Viscosity of liquid alloys: generalization of the Andrade’s equation – MonatshChem, 2012, vol.143, pp.1235-1242. – „Several relations exists in the literature to evaluate the viscosityof liquid metals and of liquid alloys with known and unknown [P96] viscosities of the components.” –p.1235. “The starting point for the new model to evaluate the compositzion and temperature dependenceof the viscosity is the ofet used [P96] expression for pure liquids due to Andrade” – p.1235.P95. T.Bárczy, G.Kaptay: Theory of Penetration/Infiltration of Liquids into a Closely Packed,Equal Spheres (CPES) Structure - Proc. of microCAD 2003 Conference, Section MaterialsTechnology, University of Miskolc, 2003, pp. 1-6.P94. N.Borisenko, J.Sytchev, G.Kaptay: Deposition of Sodium from Molten Sodium Chlorideon Different Cathode Materials - Proc. of microCAD 2003 Conference, Section Chemistry,University of Miskolc, 2003, pp. 15-20.P93. Baumli P., H.Göndör Zs., Sytchev J., Kaptay Gy.: Kerámiaszemcsék fémmel valóbevonása sóolvadékból – Proc. of microCAD 2003 Conference, Section Chemistry,University of Miskolc, 2003, pp. 1-4.P92. M.F.Souto, I.Sytchev, A.Koepf, G.E.Nauer, G.Kaptay: Study of the Morphology of TiB 2Coatings on Molybdenium Substrate Electrodeposited from a NaCl-KCl-K 2 TiF 6 -NaBF 4 Meltat 700 o C – Proc. of the Electrochemical Society, PV 2002-19, ed. by H.C.Delong,R.W.Bradshaw, M.Matsunaga, G.R.Stafford, P.S.Trulove, 2002, pp.857-862.P91. I.Sytchev, Z.H.Göndör, G.Kaptay: Electroless Coating of Non-Conducting Surfaces andParticles with Metallic Titanium from Molten Salts – Proc. of the Electrochemical Society,PV 002-19, ed. by H.C.Delong, R.W.Bradshaw, M.Matsunaga, G.R.Stafford, P.S.Trulove,2002, pp.803-809.P90. G.Kaptay: Construction principle of complex electrochemcal synthesis (ES) diagrams onthe example of the Ti-B system – Proc. of the Electrochemical Society, PV 2002-19, ed. byH.C.Delong, R.W.Bradshaw, M.Matsunaga, G.R.Stafford, P.S.Trulove, 2002, pp.700-712.P89. G.Kaptay: Modeling Penetration of Liquid Metals into Porous Ceramics – in: AnnualReport of SVBL at KIT, Japan, No. 6, August 2002, pp.152-157.97

P88. Cs.Varga, A.Borsik, G.Kaptay: A method to determine density of liquid metals fromphotographs taken by a sessile drop method. Proc. of the microCAD 2002 Int. Sci. Conf.,University of Miskolc, 2002, pp. 87-92.P87. G.Kaptay: On the excess entropy of liquid binary metallic alloys. Proceedings of 34 thInternational October Conference on Mining and Metallurgy, ed. by Z.S.Markovic andD.T.Zivkovic, University of Belgrade, Technical Faculty of Bor, Yugoslavia, 2002, pp. 552-557.P86. G.Kaptay: On the concentration dependence of the surface tension of liquid metallicalloys. Theoretical basis - Proc. of Microcad 2002, Section: Materials Science, University ofMiskolc, 2002, 45-50.P86-c1. J.Brillo, Y.Plevachuk, I.Egry: Surface tension of liquid Al-Cu-Ag ternary alloys – J Mater Sci, 2010,vol.45, pp.5150-5157 – „ A value of f = 1.06, based on a coordination number of z = 11 was suggestedrecently [P86]. Within the experimental error, the difference using the above value of f = 1.09 isnegligible” – p.5151.P85. J.Sytchev, Zs.H.Göndör, P.Baumli, Z.Gácsi, Á.Kovács, J.Sólyom, G.Kaptay: CoatingNon-conducting particles with metallic titanium in molten salts - Proc. of Microcad 2002,Section: Chemistry, University of Miskolc, 2002, 131-136.P84. O.N.Verezub, L.Zoltai, G.Kaptay: Wettability of WC/Co/TiC ceramic substrates byliquid copper – Proc. of Microcad 2002, Section: Materials Science, University of Miskolc,2002, 107-112.P83. M.S.Yaghmaee, G.Kaptay: On the Validity of the „Solubility Product” Concept - Proc.of MICROCAD 2001, Section: Chemistry, 2001, pp. 63-68P82. Hutkainé Göndör Zs., Zambóné Benkő M., Kaptay Gy., Gál J., Szontagh E.: Új kémiaipolírozó technológiai és minősítő rendszer kifejlesztése ötvözött és ötvözetlen alumíniumhegesztőpálcák felületkezelésére - Proc. of MICROCAD 2001, Section: Chemistry, 2001, pp.23-28.P81. J.Miklósi, P.Nagy, E.Kálmán, I.Sytchev, M.S.Yaghmaee, G.Kaptay: Examination ofCarbon Nanotubes Developed by the Electrochemical Synthesis - Proc. of MICROCAD 2001,Section: Chemistry, 2001, pp. 81-86P80. G.Kaptay, L.Zoltai, E.Báder: A Model to Predict Adhesion Energy and Contact Angle inSi 3 N 4 / Nonreactive Liquid Metal Systems – Proc. of MICROCAD 2001, Section:Metallurgical Science, 2001, pp. 17-22P79. G.Kaptay: A Generalized Stability Diagram of Production of Metallic Foams by the MeltRoute – in: „Cellular Metals and Metal Foaming Technology”, ed. by J.Banhart, M.F.Ashby,N.A.Fleck, MIT, Bremen, 2001, pp. 117-122.P79-c1. N.Babcsan, D.Leitlmeier, H.P.Degischer: Foamibility of Particle Reinforced Aluminum Melt – Mat.-wiss. u. Werkstofftech., 2003, vol.34, pp.1-8 – ”The first stability map of metal foams was published byI.Jin [ ]. This map theoretically was revised by Kaptay [P79].” – p.2P79-c2. N.Babcsán: Ceramic Particle Stabilized Aluminum Foams – PhD Dissertation, Miskolc, 2003 – “In themiddle of 90-s – thanks to H.P.Degischer, J.Banhart and G.Kaptay – science found a partnership with thischallenging material {metallic foam} and some basic questions like stability of of metal foams {has98

een} clarified”. – p.12, “The first stability map of metal foams was published by I.Jin [..]. This maptheoretically was revised by Kaptay [P79]” – p.34.P79-c3. Babcsán N., Bárczy P.: Alumíniumhabok – BKL, Kohászat, 2003., vol.136., No.2, pp.97-101 – „A jóminőségű fémhab előállítása és a fémolvadék habosíthatóságának megértése [P79] igen összetett, azirodalomban eddig még alig tárgyalt szakterület” – 98.o.P79-c4. N.Babcsán, J.Banhart, D.Leitlmeier: Metal foams manufacture and physics of foaming - in: Proc. of Int.Conf. „Advanced Metallic Materials”, ed. by J.Jerz, P.Sebo, M.Zemankova, IMMM, Slovak Academy ofSciences, 2003, pp. 7-15 – „The first schematic stability map giving limits for the volume content andparticle size required for metal foam creation was published by I.Jin [..]. This map was interpreted byKaptay [P79] on the basis of theoretical considerations” – p.8.P79-c5. T.Wübben: Zur Stabilitat flüssiger Metallschaume – Universitat Bremen, Germany, 2003, 128 pp. (ref.No.70) - „In diesem Zusammenhang wird das schon erwahnte Stabilisierungsmodell von G.Kaptayausführlich erlautert und kritisch diskutiert” – p.2, „Nach einer kurzen Beschreibung der gegenwartigenDiskussion über die Wirkungsweise von Partikeln in Metallschaumen wird schlieslich ein von Kaptayentwickeltes Modell [P79]. Die im Rahmen dieser Arbeit gefundenen experimentellen Resultate habendeutliche Indizien für die prinzipielle Gültigkeit dieses Modells erbracht” – p.25, „In diesem Kontext hatKaptay [P79] ein mechanistisches Modell entwickelt, das sowohl den Einflus der Partikelkonzentrationals auch des Kontaktwinkels auf die Stabilitat von Metallshaumen beschreibt. Diese Arbeit beschaftigtsich in groSen Teilen mit der Untersuchung der Gültigkeit deises Modells. Es soll daher folgenden imDetail erlautert werden” – p.30. „Mit Ausnahme von Kaptay in [P79] geben jedoch alle Autoren nurphanomenologische Erklarungen” – p.31.P79-c6. M.Arnold, C.Körner, R.F.Singer: PM aluminium foams: stabilizing mechanisms and optimization – in:“Cellular Metals: Manufacture, Properties, Application”, ed. by J.Banhart, N.A.Fleck, A.Mortensen, MITVerlag, 2003, pp.71-76: “Basic investigations of the mechanisms show that besides the increase of theviscosity also interfacial forces between the particles and the melt play an important role [P79]” – p.71.P79-c7. A.R.Kennedy, S.Asavavisihchai: The effect of ceramic particle addition on foam expansion and thestability in compacted Al-TiH 2 powder precursor - in: “Cellular Metals: Manufacture, Properties,Application”, ed. by J.Banhart, N.A.Fleck, A.Mortensen, MIT Verlag, 2003, pp.147-150 – “An additionalmechanism for improving foam stability is that particles can attach to the gas/liquid interface… this canonly be achieved if the particles show good wetting with the liquid metal [P79]” – p.147. “The behaviourobserved correlates well with semi-empirical models of foam stabilization based on an interfacial forcemodel [P79]” – p.149.P79-c8. A.R.Kennedy, S.Asavavisithchai: Effect of ceramic particle additions on foam expansion and stability incompacted Al-TiH2 powder precursors - Advanced Eng. Mater., 2004, vol.6, N.6, pp.1-6: “An additionalmechanism for improving foam stability is that particles can attach to the gas/liquid interface… It hasbeen remarked, however, that this can only be achieved if the particles show good wetting with the liquidmetal [P79]” – p.1P79-c9. N.Babcsán, J.Banhart, D.Leitlmeier: Metal foam – manufacture and physics of foam – Materials World,e-journal, 2005, vol.6, No.1: “The first schematic stability map giving limits for the volume content andparticle size required for metal foam creation was published by I.Jin [..]. This map was interpreted byKaptay [P79] on the basis of theoretical considerations” – p.6.P79-c10. N.Babcsán, D.Leitlmeier, J.Banhart: Metal foams – high temperature colloids. Part I. Ex situ analysisof metal foams – Colloids and Surfaces A, 2005, vol.261, pp.123- 130 - “The first schematic stability mapgiving limits for the volume content and particle size required for metal foam creation was published byI.Jin [..]. This map was interpreted by Kaptay [P79] on the basis of theoretical considerations” – p.125.P79-c11. T.Wübben, S.Odenbach: Stabilisation of liquid metallic foams by solid particles – Colloids SurfacesA., 2005, vol.266, pp.207-213 – “Another, thermophysical, stabilizing mechanism was suggested byKaptay [P79], relying on the adhesion properties of solid particles and liquid metals” – p.207.P79-c12. Esmaeelzadeh S, Simchi A, Lehmhus D: Effect of ceramic particle addition on the foaming behavior,cell structure and mechanical properties of P/M AlSi7 foam – Mater Sci Eng A, 2006, vol. 424, No. 1-2,pp. 290-299 – “The material is melted with conventional foundry equipment and tranferred to a tundish,where gas is introduced as the foaming agent [P79]” – p. 290P79-c13. N.Babcsán, J.Banhart: Metal Foams – towards high-temperature colloid chemistry – Chapter 11 in:„Colloidal particles at Liquid Interfaces, ed. By B.P.Binks, T.S.Horozov, Cambridge University Press,2006, pp.445-499 – „The satbility map of Jin et al was interpreted by Kaptay [P79] ont he basis ofthoretical considerations. He pointed out that a wetting angle between particles and liquid has to be in acertain range for particles to be able to stabilise the gas-liquid bubbles surface.” – p.461.P79-c14. J.Banhart: Metal foams: production and stabilty – Adv. Eng Mater., 2006, vol.8, pp.781-794 – “Someof the inventors at Alcan have described a relationship between particle content and foam stability in a99

qualitative way.. Kaptay has discussed this diagramme theoretically by considering interfacial forcesbetween particles and melt [P79]” – p.787.P79-c15. J.Banhart: Metal foams: the mystery of stabilisation – in: Porous Metals and Metal FoamingTechnology, eds. H.Nakajima, N.Kanetake, the Japanese Inst. of Metals, 2006, pp.75-86 - “Some of theinventors at Alcan have described a relationship between particle content and foam stability in aqualitative way.. Kaptay has discussed this diagramme theoretically by considering interfacial forcesbetween particles and melt [P79]” – p.83.P79-c16. F.Campana, G.Santuzzi: Caratterizzazione meccanica di schiume in alluminio sottoposte a trattamentitermici – Proc. XXXIV Convegno Nazionale, Associazione Italiana per l Analisi Solecitazione,Politechnico Milano, 2005, 10 pp. (Ref. No.13).P79-c17. Babcsan N, Moreno FG, Banhart J: Metal foams - High temperature colloids - Part II: In situ analysisof metal foams – Coll Surf A, 2007, vol. 309 (1-3), pp. 254-263 – “The particles may segregate on thesurface of melts and lose their stabilizing properties or sediment if their size exceeds 50 – 100 μm [P79]”– p. 254.P79-c18. Somosvari BM, Babcsan N, Barczy P, Berthold A: PVC particles stabilized water-ethanol compoundfoams - Coll Surf A, 2007, vol. 309 (1-3), pp. 240-245 – “Kaptay [P79] postulates that the maximumparticle size that can stabilize liquid films depends on the liquid properties. For water 3 micron and forliquid metals 30 micron were calculated. He also could derive theoretically, the optimum contact angles,measured by the researchers” – p.240.P79-c19. S.Esmaeelzadeh, A.Simchi: Foamability and compressive properties of AlSi7- 3 vol% SiC – 0.5 wt %TiH 2 powder compact – Materials Letters, 2008, vol.62, pp.1561-1564 – “Direct foaming of metallicmelts [P79] ….” – p.1561.P79-c20. D.P.He, et al., A Chinese journal, 2009, vol.39, No.2, pp.97-105http://scholar.google.com/scholar?hl=en&lr=&scoring=r&q=kaptay&as_ylo=2009P79-c21. P. Fernández, L. J. Cruz, J. Coleto: Procesos de fabricación de metales celulares. Parte II: Víasólida, deposición de metales, otros procesos - Revista de Metalurgia, Vol 45, No 2, pp.124-142(2009)P79-c22. A.V.Biakova, V.P.Krasovskii, A.O.Dudnik, S.V.Gniloskurenko, A.I.Sirko: O roli smachivaemosti Iraspredeleniia tviordich chastic v stabilizacii vspenennich aliuminievich rasplavov – Adgeziia rasplavovI paika materialov, 2009, vip.42, pp.5-22. – „Provedionnimi k nastoiashemu vremeni issledovaniiamuiubeditelno pokazano, shto vspenivanie metallicheskich rasplavov okazivaietsia nevozmozhnim priotsutstvii v nich tviordich vkliuchenii [P79].P79-c23. S.Beke: Metal foaming controlled by ultrasonic waves – PhD Thesis, TU Wien, 2011, supervisors: HPDegischer and N. Babcsan. – „For liquid metal foams particles seem to be the only way of foamstabilization [P79]” – p.13.P78. Á.Borsik, K.K.Kelemen, G.Kaptay: Dynamic Simulation of the Movement of a CeramicParticle in Front of a Solidifying Interface - in: „Affordable Metal-Matrix Composites forHigh Performance Applications”, ed. by A.B.Pandey, K.L.Kendig and T.J.Watson – TMS,Warrendale, PA, 2001, pp.101-111.P77. G.Kaptay: Interfacial Aspects to Produce Particulate Reinforced Metal MatrixComposites – in: „Affordable Metal-Matrix Composites for High Performance Applications”,ed. by A.B.Pandey, K.L.Kendig and T.J.Watson – TMS, Warrendale, PA, 2001, pp.71-99.P77.-c.1. E.Báder: Contact angle and infiltration pressure relevant to fabrication of syntactic magnesium / Al 2 O 3foams, WTM, Germany, Dec. 2000 – Dec. 2001, 26 pp.: “The infiltration process for fabricatingceramic reinforced metal matrix composites has already been studied by the group of Mortensen […],Garcia- Cordovilla […] and Kaptay [P77]..” pp. 11,… “… If the ceramic particles are closely packed,like in Fig.11, the pressure required for infiltration can be calculated with the following equation [P77]:{Equation is cited}..” – p. 12.P77-c2. 3 kinai név (Google): Summarization on preparation for particle reinforces metal matrix composites –Modern Electric Power, 2002, No.6.P77-c3. E.R.Fábián, P.Boross, B.Verő, P.Fülöp: Metallographic Aspects of Surface-Treated Steels by usingLaser Technology – Materials Science Forum, 2003, vols. 414-415, pp.201-206 - “no text, justreference”P77-c4. N.Babcsán: Ceramic Particle Stabilized Aluminum Foams – PhD Dissertation, Miskolc, 2003 – “Metalmatrix composite melts also behave as colloids, but until now there is no adequate explanation to the100

interactions thereby the driving force of particles distribution [P77]” – p.27. {is it an acknowledgementor a criticism ???}P77-c5. Th.Wuebben, H.Stanzick, J.Banhart. S.Odenbach: Stability of metallic foams studied under microgravity– J.Phys. C: Solid State Phys., 2003, vol.15, pp.427-433 – Ref. No.13, with no text”P77-c6.O.N.Verezub, A.I.Grabchenko, T.Matsushita: Eksperimentalno-teoreticheskoie modelirovanie dinamikiproniknoveniia legiruiushich chastic v matricu eksperimentalnogo materiala – in: „Research andEducation”, Nacionalnii Technicheskii Universitet, 2004, Harkov, pp.59-66 – „V tretiei gruppeuravnenii [P77] kriticheckii ugol kontakta raven nuliu v tom sluchaie, esli Weber kriticheskii stremitsiak nuliu. Eto polnostiu podtverzhdaiet nashi eksperimentalnie dannie” – p.64.P77-c7. J.T.Blucher, J.Dobranszky, U.Narusawa: Aluminium double composite structures reinforced withcomposite wires – Mater. Sci. Eng., 2004, vol.A387-389, pp.867-872 – „..successful infiltration ofcarbon fibers without special surface treatments was sporadic. … Al 2 O 3 , SiO, TiN. TiB as well as Cu anNi coatings all show promising results [P77]” – p.868.P77-c8. Baumli P.: SiO 2 és Al 2 O 3 reakciója titán tartalmú sóolvadékkal – ME Doktorandusz Fóruma, 2005, ME,47-53 – „Kerámiával erősített fémmátrixú kompozitokat csak akkor lehet előállítani megfelelőminőségben, ha a fémolvadék a kerámiát tökéletesen nedvesíti [P77]” – p.47.P77-c9. Kientzl I, Dobránszky J, Ginsztler J: Effect of Production Parameters on the Properties of CompositeWires - In: Papp É, Mácsay I, Holubetz L, (szerk.) Gépészet 2006 Proceedings of Fifth Conference onMechanical Engineering, Budapest University of Technology and Economics, National TechnicalInformation Centre and Library, Budapest, 2006, CD-ROM – „For an examination of reactions at theinterface, it is worth investigating, via an EDS-analysis, the changes in components through the crosssectionof a filament [P77]” – p.3.P77-c10. I.Kientzl, J.Dobránszky: Production and examination of double composites – Mater Sci Forum, 2007,vol.537-538, pp.191-197.P77-c11. Kadoi K, Nakae H: Effect of particle addition to liquid metal on fabrication of aluminum foam - HIGHTEMPERATURE MATERIALS AND PROCESSES 26 (4): 275-283 2007 – “Some other models,similar to… were proposed… by Kaptay [P77], using an interfacial model” – p. 277.P77-c12. M.A.Taha, N.A.El-Mahallawy, A.M.El-Sabbagh: Some experimental data on workability ofaluminium-particulate-reinforced metal matrix composites – J. Mater. Process. Technol., 2008, vol.202,pp.380-385 – “Powder metallurgy method … almost avoids matrix oxidation and reinforcementinterfacial reaction [P77]” – p.381, “Kaptay [P77], who also obtained improvement in the workabilityof PMMC, discussed the results on basis of coupling of both the positive influence of decreasing theparticulate size and the negative effect of particulate’s increased resistance to wettability” – p.382.P77-c13. Csanády Andrásné: Nanoszerkezetek határfelületei és határfelületeken kialakuló nanoszerkezetek – 2.3.fejezet in: Bevezetés a nanoszerkezetű anyagok világába (Csanády Andrásné, Kálmán Erika, KonczosGéza, szerk), MTA, ELTE Eötvös Kiadó, 2009, 60.o. – „A határfelületek szabadenergia felesleggelrendelkeznek, ezt növelik az érintkező felületeken kialakuló feszültésgek… [P77]” – p.60.P77-c14. A.E.Karantzalis, A.Lekatou, E.Georgatis, H.Mavros: Solidification behaviour of ceramic particlereinforced Al-alloy matrices – J.Mater Sci, 2010, vol.45, pp.2165-2173 – „Especially in the case of castmetal composites, however, a contact angle of less than 90 o C (sicc) is not sufficient to lead tospontaneous entry of the particles but a 0 o contact angle (total spreading condition) is required as shownby the works of Nakae et al., Wu et al. And Kaptay [P77]” – p.2165.P77-c15. Kientzl I.: Alumíniummátrixú kompozithuzalok és kettős kompozit-szerkezetek – PhD értekezés, BME(tud. vez.: dr.Dobránszky János), 2010, 112.o. – „Az infiltrált hosszt az idő és a nyomáskülönbségbőlszámolják [P77]”P77-c16. Bian Xinyu, Fan Jianzhong, Ma Zili, Zuo Tao, Wei Shaohua: Influence of Particulate InhomogeneousDistribution on Performance of Particulate-Reinforced Aluminum Matrix Composites - Chinese Journalof Rare Metals, 2010, vol. 34, No.3, pp.357-362. „Chinese text..?”P77-c17. I.N.Orbulov: Infiltration of ceramic microballons by liquid metals – research plan for SCIEX-NMS,February, 2011, 12 pp. – „There are many papers in the professional literature which are dealing withthe phenomenon of infiltartion [P77]” – p.9.P77-c18. S.Beke: Metal foaming controlled by ultrasonic waves – PhD Thesis, TU Wien, 2011, supervisors: HPDegischer and N Babcsan. – „Because ceramic particles are in the melt, the foam is relatively stable[P77]” – p.22.P77-c19. Rácz A., Tóth L.F.: Eszközfejlesztés mikrogömbhéjak infiltrálásához – TDK dolgozat, 2011, BME(konzulens: Orbulov IN) – “2.8. A szemcseméret hatása az infoltrációra [P77]” – 28-29. o.P77-c20. I.N. Orbulov: Syntactic foams produced by pressure infiltration – the effect of pressure and time oninfiltration length- Periodica polytechnica Mechanical Engineering, 2011, vol.55/1, pp.21-27. – „Morerecently Kaptay derived theoretical function for infiltrated length and this one is again parabolic in natureand shows linear dependence on the square root of time [P77]. ” – p.25.101

P77-c21. Orbulov IN: Mikrogömbhéjak nyomásos infiltrációjának vizsgálati módszere – OGÉT 2011, XIX.Nemzetközi Gépész Találkozó konferencia kiadványa, Csíksonlyó, Románia, 2011. 04.28-05.01.Szerkesztő: Csibi V-J. Kiadó: Erdélyi Magyar Műszaki Tudományos Társaság, Kolozsvár, Románia,2011, pp.296-299, ISBN: 2068-1267 – „A legtöbb publikáció egyetért abban, hogy ezek a kapcsolatok afenti feltételezéseket és egyszerűsítéseket felvonultató rendszerekre, a viszonylag hosz-szabb (többperces) időtartományban érvényesek. Ugyanakkor a kis idő- és nyomástartományokban (néhány s és aküszöbnyomáshoz közeli nyomások) az L-p és L-t görbék az elméleti lineáris és gyökös görbéktőlexponenciális jellegű eltérést mutatnak [P77].” p. 2069.P77-c22. I.N.Orbulov: Infiltration and mechanical characteristics of hollow spheres reinforced metal matrixcomposites – Proc. 8th International Conference on Mechanical Engineering, 2012, pp. 403-411. – „Morerecently Kaptay derived theoretical function for infiltrated length and this one is again parabolic in natureand shows linear dependence on the square root of time [P77].” – p.406.P76. Borsik Á., K.Kelemen K., Kaptay Gy.: Fémolvadékban a kristályfront előtt levőkerámiaszemcse mozgásának számítógépes szimulációja – ME Doktoranduszok Fóruma2000, Anyag- és Kohómérnöki Kar szekciókiadványa, ME, 2001, 32-37.P75. G.Kaptay: On the Surface Tension of Pure Molten Alkali Halides – Proc. 6 th Int. Symp.on Molten Salt Chemistry and Technology, ed. by Chen Nianyi and Qiao Zhiyu, ShanghaiUniversity Press, 2001, 182-185.P74. G.Kaptay, I.Sytchev, Zs.H.Göndör: Coating Quartz Samples by Metallic Titanium inMolten Salts – Proc. 6 th Int. Symp. on Molten Salt Chemistry and Technology, ed. by ChenNianyi and Qiao Zhiyu, Shanghai University Press, 2001, 178-181.P73. G.Kaptay: Estimation of Thermodynamic Properties of Pure Liquid Titanium Dichloride– Proc. 6 th Int. Symp. on Molten Salt Chemistry and Technology, ed. by Chen Nianyi andQiao Zhiyu, Shanghai University Press, 2001, 174-177.P72. G.Kaptay, I.Sytchev, M.S.Yaghmaee, A.Kovács, E.Cserta, M.Árk: ElectrochemicalSynthesis of Refractory Borides and Carbon Nano-Micro Tubes from Molten Salts – Proc. 6 thInt. Symp. on Molten Salt Chemistry and Technology, ed. by Chen Nianyi and Qiao Zhiyu,Shanghai University Press, 2001, 168-173.P72-c.1. A.T.Dimitrov, G.Z.Chen, I.A.Kinloch, D.J.Fray: A feasibility study of scaling-up the electrolyticproduction of carbon nanotubes in molten salts – Electrochimica Acta, 2002, vol.48, pp.91-102: “…asit was initially postulated in this laboratory, the intercalation of alkali metal could lead to the extrusionof carbon… Interestingly, this prediction had not been experimentally confirmed in this and otherlaboratories […] until recently when Kaptay et al. reported their observation of carbon micro-tubes onthe surface of a graphite cathode [P72]”, p.92.102

P71. Kaptay Gy.: Határfelületi jelenségek szerepe a fémes anyag-gyártásban – EMTBányászat, Kohászat, Földtan konferencia kiadványa, Csíksomlyó, EMT, 2001., 51-56 o.P71-c1. K.Szocs, M.Vaida: Border surface changes on the edge of the castings with nodular graphite – Mater.Sci. Forum, 2005, vols 473-474, pp.153-158.P70b. S.Yaghmaee Maziar, Csicsovszki G., Kaptay Gy.: Fémek kohéziós energiájánaklehetséges definíciói – Pro Scientia Aranyérmesek Társasága, Budapest, 2000, 227-231.P70a. S.Yaghmaee Maziar, Kaptay Gy., Jánosfy Gy.: A Fe-Al-N, Fe-B-N és Fe-Al-N-Bolvadék rendszerek termodinamikai modellezése – Pro Scientia Aranyérmesek Társasága,Budapest, 2000, 95-100.P70. M.Z.Benkő, G.Kaptay: Thermal Balance of LD converters – Proc. of Microcad ‘2000,Section C.: High Temperature Devices, University of Miskolc, pp.13-18.P69. Magyar Anita, Gácsi Zoltán, Kaptay György, Szalai Ibolya: Hibridszerkezetekfejlesztése - Proc. of Microcad ’2000, Section B: Materials Technology, University ofMiskolc, pp. 121-126.P69-c1. Baumli P.: Fémmátrixú kompozitok előállítása öntészeti módszerekkel – CD-Proc. of 26. Int Sci ConfmicroCAD, 29-30 March, 2012. – „Az oxidhártya csökkentésére K2ZrF6-tal vonták be a grafit felületét,mint ahogy Magyar és munkatársai is [P69]. A kezelés a küszöbnyomást kb. a felére csökkentette” – 3.o.P68. L.Zoltai, E.Bader, G.Kaptay, P.Arato: Wettability of Si 3 N 4 ceramics by liquid metals –Proc. of Microcad ’2000, Section B: Materials Technology, University of Miskolc, pp. 121-126.P67. J.Sytchev, G.Kaptay, H.Kushov: Investigation of the reduction process oftetrafloroborate ions at different electrodes in chloro-fluoride melts – Progress in Molten SaltChemistry, vol.1. (Proc. of EUCHEM 2000), 2000, Elsevier, Paris, pp. 523-528.P66. R. Román, G. Kaptay, J. Lakatos, H. Verelst, F. Rivet, A. Buekens: Development of achemical treatment method by molten salts for removing zinc from fly ash - Progress inMolten Salt Chemistry, vol.1. (Proc. of EUCHEM 2000), 2000, Elsevier, Paris, pp. 455-460.P65. G.Kaptay, I.Sytchev, J.Miklósi, P.Póczik, K.Papp, P.Nagy, E.Kálmán : Electrochemicalsynthesis of carbon nanotubes and microtubes from molten salts – Progress in Molten SaltChemistry, vol.1. (Proc. of EUCHEM 2000), 2000, Elsevier, Paris, pp. 257-262.P65-c1. G.Z.Chen, D.J.Fray: Novel Cathodic Processes in Molten Salts - Proc. 6 th Int. Symp. on Molten SaltChemistry and Technology, ed. by Chen Nianyi and Qiao Zhiyu, Shanghai University Press, 2001, 79-85– “While this research is being extended into more molten molten salt systems as demonstrated by Kaptayet al [P65], understanding of the nanotube formation mechanism has also progressed” – p.84.P65-c2. M. S.Yaghmaee, E. Cserta, A.Kovács, M. Árk: Carbon Micro-Tubes Produced by ElectrochemicalSynthesis from Molten Salts, Materials’ World (e-journal, http://materialworld.uni-miskolc.hu, July, 2001– “The second effort on synthesis of carbon nano-tubes in Hungary is in progress in the framework ofcooperation between the LIMOS R&D Group at the University of Miskolc (lead by G.Kaptay), where thesynthesis was carried out from molten salts, and between the group at KKK (lead by ‘E.Kálmán), wherethe nano-characterization of the samples is being performed [P65]. During this cooperation it has beennoted, that during the electrochemical synthesis of carbon nanotubes from molten salts carbon tubes witha very wide range of diameter are actually formed, scaling from several nanometers to severalmicrometers [P65]”– p.1.P65-c3. A.T.Dimitrov, G.Z.Chen, I.A.Kinloch, D.J.Fray: A feasibility study of scaling-up the electrolyticproduction of carbon nanotubes in molten salts – Electrochimica Acta, 2002, vol.48, pp.91-102 – “In103

2000, Kaptay et al reported that, on graphite cathode, the electro-deposition of Li, Na, K, Mg and Ca fromthe respective molten chlorides all led to the formation of CNTs, but not of Sn and Ni [P65].” – p.91,“Based on the facts that CNTs were collectable from the solidified salt phase and also the CNT yielddepended strongly on electrolysis current and temperature [P65], it was further proposed …… Thecarbon based fragments may then enter the molten salt and, without the protection of the graphite lattice,undergo through an inter- and/or intra-fragment recombination process, leading to the formation ofvarious carbon nanoparticles and nanotubes in the electrolyte [P65].” – p.92.P65-c4. Q.Xu, C.Schwandt, G.Z.Chen, D.J.Fray: Electrochemical investigation of lithium intercalation intographite from molten lithium chloride – J. of Electroanalytical Chemistry, 2002, vol. 530, pp.16-22 – “..The process has been described in several publications [P65]. There is indeed some experimental evidencethat alkali metal intercalation into graphite is an important step in the electrochemical synthesis [P65] –p.16.P65-c5. Zs.Demeter, M.S.Yaghmaee: Some Aspects of Intercalation Phenomena and Growth Mechanism ofCarbon Nano-micro Tubes in Molten Salts – Proc. of microCAD 2003 Conference, Section MechanicalTechnologies and Material Science Engineering, University of Miskolc, 2003, pp. 7-12 – “The secondeffort on synthesis of carbon ano-tubes in Hungary is in progress in the framework of cooperationbetween the LIMOS R&D Group at the University of Miskolc (lead by G.Kaptay), where the synthesiswas carried out from molten salts, and between the group at KKK (lead by E.Kálmán), where the nanocharacterizationof the samples is being performed [P65]. During this cooperation it has been noted thatduring the electrochemical synthesis of carbon nanotubes from molten salts carbon tubes with very widerange of diameter are actually formed, scaling from several nano-meters to several micrometers [P65]” –p.7.P65-c6. G.Z.Chen, D.J.Fray: Recent development in electrolytic formation of carbon nanotubes in molten salts –J. of Mining and Metallurgy, 2003, vol.39B, pp.309-342 “.. research in the electrolytic method isgathering forces around the world in the past few years [P65]..” – p.311, “Kaptay and co-workers inHungary reproduced the results of the authors, and reported that the electrodeposition of Li, Na, K, Mg,Ca from respective chloride salts all led to the formation of CNTs, but not Sn and Ni [P65]” – p.313,“Based on SEM and TEM estimations of different research groups [P65], the electrolytic carbon nanomaterialscontain CNTs in the range of 5 to 50 vol%…” – p.325, “This postulation had not beenexperimentally confirmed in the Cambridge laboratory and other [..], until recently when Kaptay et al.reported their observation of a carbon micro-tube on the surface of a graphite cathode [P65]” – p.331,“The Cambridge team’s CNTs formation mechanism was generally advocated by Kaptay et al [P65]…. Inaddition, they argued that once suspended in the molten salt, tube formation was driven by the attractiveinterfacial forces between the two edges of the suspended graphite planes having broken carbon bonds.” –p.332-33P65-c7. Q.Xu, C.Schwandt, D.J.Fray: Electrochemical investigation of lithium and tin reduction at a graphitecathode in molten chlorides – J. of Electroanal. Chem., 2004, vol.562, pp.15-21: “Most of the studies …focused on the preparation of carbon nanotubes [P65]. Tin reduction, as opposed to lithium reduction,does not lead to the formation of nano-sized carbon materials [P65]”, p.15.P65-c8. I.A.Kinloch, G.Z.Chen, J.Howes, C.Boothroyd, C.Singh, D.J.Fray, A.H.Windle: Electrolytic, TEM andRaman studies on the production of carbon nanotubes in molten NaCl – Carbon, 2003, vol.41, pp.1127-1141 – “Chen et al. have previously reported the formation of tambourines and it is possible that thesetambourines are the same strutcture as the nano-tori viewed by AFM by Miklosi et al [P65]” – p.1138.104

P65-c9. D.Babic, DJ Klein, J von Knop, N.Trinajstic: Combinatorial enumeration in chemistry – in: ChemicalModelling: Applications and Theory, vol.3, The Royal Society of Chemistry, 2004, pp.126-170. –„CNTs possess conducting or semiconducting properties depending ont he tube structure and may beprepared by a laser technique or by electrochemical procedures [P65] or in some other way…– p.137.P65-c10. Adamokova M.N.: Elektrovidelenie metallicheskogo volframa, molibdena i ich karbidovi znizkotemperaturnich galogenidno-oksidnich rasplavov – Diss. na kand. him. nauk, Ekaterinburg, 2005,142 pp. – „V 2000 g. nachala publikovat rezultati issledovanii po polucheniiu nanotrubokelektroliticheskim metodom tretia gruppa – Kaptay G i Sychev J.Iv Vengrii [P65] vosproizveli rezultatirabot Fray-a, takzhe pokazali, shto elektroosozhdenie litiia, natriia, kaliia, magniia, kalciia izsootvetstvuiushich rasplavlennich hloridov privodit k polucheniu uglerodnich nanotrubok. Produktielektroliza bili issledovani metodom atomno-silovoi mikroskopii”….. „G.Kaptay i J.Sichev ssotrudnikami (Vengriia) zanimaiutsia issledovaniem mechanizma obrazovaniia uglerodnich nanotrubokpri osazhedenii shelochnich metallov (litiia i natriia) i shelochnozemelnich metallov (magniia i kalciia) izrasplavlennich solei na grafitovii katod [P65]” – p.25.P65-c11. JH Lee, JB Shim, EH Kim, JH Yoo, SW Park: A feasibility study for the development of alternativemethods to treat a spent TRISO fuel – Nucelar Technol, 2008, vol.162, pp.250-258 – „Carbon also formsintercalation compounds with magnesium” – p.256.P65-c12. C.Schwandt, A.T.Dimitrov, D.J.Fray: The preparation of nano-structured carbon materials byelectrolysis of molten lithium chloride at graphite electrodes – J Electroanal Chem, 2010, vol.647, pp.150-158 – „Kaptay and co-workers also investigated the electrolytic preparation method. Carbonaceousproducts were prepared by using various molten salt electrolytes [P65]” – p.151.P65-c13. AT Dimitrov, A.Tomova, A.Grozdanov, P.Paunovic: Production, purification, characterization andapplication of CNTs - Chapter 13 of book: Nanotechnological Basis for Advanced Sensors, ed. by JPReithmaier, P.Paunovic, W.Kulisch, C.Popov, P.Petkov. Springer, Dordrecht, Netherlands, 2011, pp.121-142. – „Kaptay Mechanism. Kaptay et al. did research on the molten salt electrolysis to produce CNTs.They use the intercalation mechanism of sodium into the cathode to explain the formation of the speciesobserved [P65]. They proposed a mechanism of formation of nanotubes summarized below: … threesteps” – p.133.P65-c14. AR Kamali, C Schwandt, DJ Fray: Effect of graphite electrode material on the characteristics of moltensalt electrolitically produced carbon nanomaterials – Mater Charact, 2011, vol.623, pp.987-994 – „Thisfinding was then confirmed further in a number of subsequent studies, in which both lithium chloride andsodium chloride were found suitable molten salt electrolyte [P65]” – p.987P65-c15. Y.Ito: Formation of a carbon film by the molten salt electrochemical process and its applications –TANSO, 2011, NO.248, pp.144-151 (in Japanese).P65-c16. A.R. Kamali, C. Schwandt, D.J. Fray, On the oxidation of electrolytic carbon nanomaterials, CorrosionScience, 2012, vol.54, pp.307-313 – „The cathodic reaction leads to the erosion of the graphite and therelease of a variety of carbon nanostructures including multi-walled carbon nanotubes (MWCNTs) andcarbon nanoparticles. The method has been investigated further in a number of studies [P65]” – p. 3.P65-c17. C.Schwandt, AT Dimitrov, DJ Fray: High yield synthesis of multi-walled carbon nanotubes fromgraphite by molten salt electrolysis – Carbon, 2012, vol.50, pp. 1311-1315. „The molten salt electrolysismethod of converting graphite directly into nanoscale carbon materials is a rather unknown approachtoward preparation of CNTs [P65]” – p.1311.P65-c18. A.R. Kamali, G. Divitini, C. Schwandt, D.J. Fray, Correlation between microstructure andthermokinetic characteristics of electrolytic carbon nanomaterials, Corrosion Science (2012), doi:http://dx.doi.org/ - „bulk graphite sample is cathodically polarised in a molten alkali metal chloride salt,such that the alkali metal intercalates into the graphite and disintegrates its microstructure whereby thegraphite is continually eroded into nanometre sized carbon entities. These become detached from thegraphite surface and accumulate in the molten salt bath from where they can be harvested [P65].”105

P64. G.Jánosfy, G.Károly, G.Kaptay, M.S.Yaghmaee, V.Beszterczey: Quality AssuranceProblems in the Production of Boron Microalloyed Case-hardening Steel Grades – EOSC ’00,3 rd European Oxygen Steelmaking Conference, 30 October – 1 November 2000, ICC,Birmingham, UK. pp. 493-503.P63. G.Kaptay, K.K.Kelemen: Corrections to the Stokes Equation - Proc. of Microcad 2000,Section D: Applied Chemistry, pp. 23-28.P62. A.Borsik, K.K.Kelemen, G.Kaptay: Simulation of the movement of ceramic particles inliquid metals in front of solidification fronts – Proc. of Microcad, 2000 Section D: AppliedChemistry, pp. 9-14.P61. J.Sytchev, G.Kaptay, H.Kushkov: Voltammetric investigation of the reduction processesof nickel and iron divalent ions in chloro-fluoride melts – Proc. of Microcad 2000, Section D:Applied Chemistry, pp. 69-68.P60. R.Roman, G.Kaptay, A.Mihalik, H.Verelst, F.Rivet, A.Buekens: Removal of HeavyMetals from fly ash with molten chlorides. Part II.: Experimental verification – Proc. ofMicrocad 2000, Section D: Applied Chemistry, pp. 63-68.P59. R.Roman, G.Kaptay, A.Mihalik, H.Verelst, F.Rivet, A.Buekens: Removal of HeavyMetals from fly ash with molten chlorides. Part I.: Theoretical Analysis andThermogravimetry experiments – Proc. of Microcad 2000., Section D: Applied Chemistry,pp. 57-62.P58. G.Kaptay, K.K.Kelemen: On the Drag Force Acting on Ceramic Particles duringProcessing of Cast MMCs – in: „State of the Art in Cast MMCs”, ed. by P.K.Rohatgi, TMS,2000, pp.45-60.P58-c1. D.M.Stefanescu: Science and Engineering of Casting Solidification – Kluwer Academic / PlenumPublishers, NY, 2002, 342 pp. – „The relative viscosity can be calculated with: {equation 4.45}.Numerous expressions were proposed for the correction factor (see review by Kaptay, 2000)” – p.57.“Table 4.1. {Equation} (Kaptay 2000)” – p.57.P58-c2. D.M.Stefanescu: Science and Engineering of Casting Solidification, 2nd edition, Springer, NY, 2009,395 pp. – „The relative viscosity can be calculated with: {equation 4.45}. Numerous expressions wereproposed for the correction factor (see review by Kaptay, 2000)” – p.64.P58-c3. W.Sobieski: Drag coefficient in solid-fluid system modeling with the Eulerian multiphase model –Drying Technology, 2011, vol.29, pp.111-125 – “According to Kaptay and Kelemen [P58], thetheoretically highest possible density of a fluid medium is 0.74, but in real environment, this value usuallyapproximates 0.60-0.63. At this level of packing, the particles are unable to move, and the drag runsinfinity” – p.122.P57. E.Báder, G.Kaptay, L.Zoltai: Wettability studies for the production of Cu-Sn/WCcomposites. – Proc. of International Scientific Conference ‘Competitive Materials,Technologies and Products’ (CMTP), Miskolc, 2000, pp. 39-45.106

P56. B.Tury, G.Kaptay, G.M.Kale: Electrochemical Intercalation of Na from Al to LiMn 2 O 4 –Proc. of International Scientific Conference ‘Competitive Materials, Technologies andProducts’ (CMTP), Miskolc, 2000., pp. 147-152 (paper to be disregarded due to falsificationof Fig1. by B.Tury)P55. J.Sytchev, G.Kaptay, H.Kushov: Study of the electroreduction process oftetrafluoroborate ions at different electrodes in chloro-fluoride melts – Miskolci EgyetemDoktoranduszok Fóruma, Miskolc, 1999. november 4-5. Kohómérnöki Kar szekciókiadványa,Miskolc-Egyetemváros, 2000., pp.106-112.P54. Román R., Kaptay Gy., H.Verelst, F.Rivet, A.Buekens: Szállóhamu nehézfémtartalmánakeltávolítása sóolvadékos kezeléssel - Miskolci Egyetem Doktoranduszok Fóruma,Miskolc, 1999. /november 4-5. Kohómérnöki Kar szekciókiadványa, Miskolc-Egyetemváros,2000., pp. 75-81.P53. Báder E., Kaptay Gy.: Volfrám karbid nedvesíthetősége Cu-Sn olvadt ötvözetek által –Miskolci Egyetem Doktoranduszok Fóruma, Miskolc, 1999. november 4-5. Kohómérnöki Karszekciókiadványa, Miskolc-Egyetemváros, 2000., pp. 7-12.P52. G.Kaptay, H.B.Kushkov, A.S.Uzdenova, M.K.Vindizheva: Electrochemical SynthesisDiagrams of the La-Gd, Gd-Al, La-B, Gd-B systems – Vestnik KBSU, Seriya chem.nauk,vip.3., Nalchik, 1999, pp.56-60.P51. S.V Devyatkin, G.Kaptay, J.C.Poignet, J.Bouteillon: Chemical and electrochemicalbehaviour of titanium oxide and complexes in cryolite-alumina melts - in: „Advances inMolten Salts – From Structural Aspects to Waste Processing”, ed. by M.Gaune-Escard, begellhouse inc., New-York, 1999, pp.178-187.P50. B.Tury, J.I.Sytchev and G.Kaptay: Morphology of titanium diboride obtained byelectrochemical synthesis from molten chloro-fluoride melt - in: „Advances in Molten Salts –From Structural Aspects to Waste Processing”, ed. by M.Gaune-Escard, begell house inc.,New-York, 1999, pp.260-269.P49. G.Kaptay: Control of Phases to be Synthesised by Electrochemical Synthesis fromMolten Salts: the ternary EES diagram for the Ti-Al-B system – in: „Advances in MoltenSalts – From Structural Aspects to Waste Processing”, ed. by M.Gaune-Escard, begell houseinc., New-York, 1999, pp.249-259.P49-c1. P.Taxil, P.Chamelot, L.Massot, C.Hamel: Electrodeposition of alloys or compounds in molten salts andapplications – J. of Mining and Metallurgy, 2003, vol.39B, pp.177-200 „Kaptay elaborated the EESdiagram of the ternary system Ti/Al/B at 1000 K in cryolithe melts containing alumina, and Ti andboron oxides, combining data from the respective binary systems. The goal is to optimize the potentialof the carbon cathode for the electrochemical synthesis of titanium boride, used as a protective layer ofthe carbon as a function of the Ti/B system, the diagram delimits the area of stability in terms ofequilibrium potential of each binary compound [P49]” – p.184.107

P48. G.Jánosfy, G.Kaptay, M.S.Yaghmaee: Computer Aided Determination of the PhaseBoundary of Liquid Iron and Aluminium Nitride in the Fe-Al-N Ternary System –Proceedings of MICROCAD ’99, Section B: Metallurgy, Energetics, 1999, pp.27-32P47. Török B., Tóth L.A., Kaptay Gy.: Asszociált elegymodell alkalmazása nagyolvasztóisalakrendszerre – Proceedings of MICROCAD ’99, Section B: Metallurgy, Energetics, 1999,pp.75-81.P47-c1. M.Z.Benkő: On the computer software for the LD converter process at the Dunaferr Works,Materials’ World (e-journal, http://materialworld.uni-miskolc.hu, July, 2001 – “The heat dueto complex formation was estimated by the associated model for the slag [P47].” – p. 6.P46. R.Gemela, K.Kelemen, G.Kaptay: Dynamics of vapour-to-liquid transfer of SiC particlesinto Fe 40 Ni 40 Si 6 B 14 liquid matrix of amorphous metal matrix composites – Proceedings ofMICROCAD ’99, Section C: Materials Science and Technology, 1999, pp. 187-192P46.-c.1. Boross Péter: Lézeres átolvasztással végzett felületmódosítások, Diplomamunka, BME, Bayati, 2001.,tud.vez.: dr. Verő Balázs és dr. Hárs György. „Ennek [P46] szerint csillapodó oszcilláló megoldásalesz” – p.23.P45. E.Báder, L.Bolyán, G.Kaptay, G.Zs.Hutkai: Measuring and Modelling of AdhesionEnergy between non-reactive Liquid Metals and Oxide Ceramics – Proceedings ofMICROCAD ’99, Section C: Materials Science and Technology, 1999, pp. 175-179P44. G.Kaptay: Interfacial Theory of Producing Particle Stabilised Metallic Foams –Proceedings of MICROCAD ’99, Section C: Materials Science and Technology, 1999, pp.79-84P43. M.S.Yaghmaee, G.Kaptay: Calculation of Tie-Lines between Solid and Liquid Phasesmainly in Al-rich corner of the Ternary Al-Mg-Zn System Based on ThermodynamicProperties of Phases in Equilibrium – Proceedings of MICROCAD ’99, Section C: MaterialsScience and Technology, 1999, pp. 165-168P42. B.Tury, G.Kaptay, J.Sychev: The Calculation of Equilibrium Electrochemical SynthesisDiagrams for Ni-Ti-B system – Proceedings of MICROCAD ’99, Section C: MaterialsScience and Technology, 1999, pp. 159-164P41. G.Kaptay: Interfacial Criteria for ceramic particle stabilised metallic foams – in: MetalFoams and Porous Metal Structures, ed. by J.Banhart, M.F.Ashby, N.A.Fleck, MIT Verlag,Bremen, 1999, pp. 141-145.P41.-c.1. J.Banhart: Manufacturing Routes for Metallic Foams – JOM December 2000, pp. 22-27. “..This castsdoubts on the hypothesis that solid particles floating on the walls of films are responsible for theirstabilization in analogy to the action of surfactants in aqueous foams [P41].” – p.26, “ Metallic foams,therefore, appear to be stabilized by solid particles. The action of foam stabilization is not entirely clearyet, but some current ideas on metal foams have been published [P41]” – p.26., “ The wetting angle hasto in a certain range to ensure that the bubble/particle interfaces are stable when the bubbles risesthrough the melt (i.e., the particles are not stripped off the bubbles), and that the particles on theinterface lower the total interface energy of a pair of bubbles with particles in between (i.e. stabilizebubble / particle / bubble interfaces). There is nostabilization effect for insufficient wetting (highcontact angle) as well as for overwetting (low contact angle). In principle, from the known wettingangles of ceramic particles with given melt, particles can be selected that have an optimum stabilizationeffect [P41]” – p.27.P41-c2. J.Banhart: Metallic foams: Challenges and opportunities – in:”Foams, Emulsions and Applications”, Eds.P.Zitha, J.Banhart, G.Verbist, Verlag MIT Publishing, Bremen, 2000, pp.13-20. – „The action offoam stabilisation is not entirely clear yet. An outline of the current ideas shall be given here using108

some of the sparse information on metal foams available in the literature [P41]” – p.18., „It has beenderived that the wetting angle has to be in a certain range to ensure that i. the bubble/particle interfacesare stable when the bubbles rise through the melt, i.e. the particles are not stripped of the bubbles, ii.that the particles on the interface lower the total energy of a pair of bubbles with particles in between,i.e. stabilise buble/particle/bubble interfcaes. For insufficient wetting (high contact angle) as well as fortoo good wetting (low contact angle) there is no stabilisation effect. In principle, from the knownwetting angle of ceramic particles with a given melt particles can be selected which have an optimumstabilisation effect [P41]” – p.19.P41-c3. E.Báder: Wettability of Alumina by Liquid Magnesium and Liquid AZ91 Alloy, Materials’ World (ejournal,http://materialworld.uni-miskolc.hu, July, 2001 – “The wettability of alumina by magnesium isa very important factor in producing metal matrix composites [ .. .] or metallic foams [P41] consistingof these two phases” – p.1P41-c4. J.Banhart: Manufacture, characterisation and application of cellular metals and metal foams – Progressin Materials Science, 2001, vol.46, pp.559-632 – „The particles help to stabilize the foam bymechanisms which are discussed in the literature [P41]. It is widely accepted that the accumulation ofthe particles on the cell walls plays a key role in this stabilistaion process. Firstly, the particles increasethe surface viscosity, thus retarding drainage in films [..]. Secondly, the particles are partially wetted bythe melt. It has been derived [P41] that the wetting angle has to be in a certain range to ensure that: thebubble/particle interface is stable when the bubble rises through the melt, i.e. the particles are notstripped off the bubbles, that the particles on the interface lower the total energy of a pair of bubbleswith particles in between, i.e. stabilise bubble/particle/bubble interfaces. For insufficient wetting (highcontact angle) as well as for too good wetting (too low contact angle) there is no stabilisation effect. Inprinciple, from the known wetting angles of ceramic particles with a given melt particles can beselected which have an optimum stabilisation effect [P41].” – pp. 565-566.P41-c5. C.Körner, R.F.Singer: Foaming Process for Al – in: “Handbook of Cellular Metals, Production,Processing, Applications”, ed. by H-P.Degischer, B.Kriszt, Wiley-VCH, 2002, pp.8-14 – “Theoreticalwork of Kaptay [P41] and experimental work of Weigand [ ] indicate that a reduction ofparticle sizewill not lead to a higher stabilization and therefore to a smaller critical cell wall thickness” – p.13(Sajnálattal meg kell jegyeznem, hogy Körner és mtsai félreértelmezték az elméletemet…”)P41-c6. C.Körner, M.Arnold, M.Thies, R.F.Singer: The Physics of foaming: structure formation and stability -in: “Handbook of Cellular Metals, Production, Processing, Applications”, ed. by H-P.Degischer,B.Kriszt, Wiley-VCH, 2002, pp.32-43 – “Additives in the fluid like SiC or Al 2 O 3 particles influence themovement of the bubbles and are able to stabilize them [P41]. They have an effect on both theviscosity of the melt and the surface tension.” – p.35.P41-c7. Y.Q.Sun, T.Gao: The optimum wetting angle for the stabilization of liquid metal foams by ceramicparticles: experimental simulations – Metall. Mater. Trans. A., 2002, vol.33A., pp.3285-3292. –„Another explanation ascribes the improved foam stability to the appropriate wetting behaviour of theceramic particles in the liquid metal [P41]. Theoretical analysis incorporating several mechanismspredicted an ambigous wetting-angle range of 20 to 90 deg for foaming Al [P41].” – pp.3285-3286,„..The maximum foaming height occurs in a narrow wetting angular range of 75 to 85 deg. …. We notethat stable foam exist at wetting angles considerably greater than 90 deg. This is contrary to thetheoretical analysis of Kaptay [P41], who predicted no foam stability outside the 20 to 90 deg wettingangle range” – p.3288, „Kaptay [P41] proposed that, to stabilzie the foam, the solid particles mustremain attached to the liquid surface against buoyancy. From this a necessary wetting-angle range of 20to 90 deg is suggested; this is clearly at variance with the present simulation results, which have shownstable foams at much larger wetting angles” – p.3290P41-c8. Gao T, Sun YQ: Role of wetting behavior in the stabilization of liquid metal foams by ceramic particles:An experimental simulation study - PROCESSSING AND PROPERTIES OF LIGHTWEIGHTCELLULAR METALS AND STRUCTURES, 2002, pp.115-123.P41-c9. N.Babcsán, D.Leitlmeier, H.P.Degischer: Foamibility of Particle Reinforced Aluminum Melt – Mat.-wiss. u. Werkstofftech., 2003, vol.34, pp.1-8 – „Kaptay pointed out that wetting angle has to be in acertain range and particles stabilize the gas/liquid-bubble interface. In the framework of a model,assuming single layer of particles between in the cell wall it was shown that the foam is stabilized onlyin the interval of’ the contact angles 10 – 90 degrees [P41]. However, when a presence of a double, or a’double+’ layer of particles is assumed to be in the cell wall, this interval increases to 10-129 degrees,or 10 – 170 degrees, accordingly”P41-c10. N.Babcsán: Ceramic Particle Stabilized Aluminum Foams – PhD Dissertation, Miskolc, 2003 – “In themiddle of 90-s – thanks to H.P.Degischer, J.Banhart and G.Kaptay – science found a partnership withthis challenging material {metallic foam} and some basic questions like stability of of metal foams {hasbeen} clarified”. – p.12,“Kaptay pointed out that wetting angle has to be in a certain range and particles109

stabilize the gas bubble/liquid interface. In the framework of a model, assuming single layer of particlesin the cell wall it was shown that the foam is stabilized only in the interval of the contact angles 10-90degrees [P41]” – p.34.P41-c11. Th.Wuebben, H.Stanzick, J.Banhart. S.Odenbach: Stability of metallic foams studied undermicrogravity – J.Phys. C: Solid State Phys., 2003, vol.15, pp.S427-S433 – „We suggest that, possibly inaddition to the viscosity effect, postulated previously, the main function of stabilizing particles is toprevent coalescence. Presumably the oxide filaments float to the surface of the liquid metal films andcreate layers at the liquid/gas interface (Fig. 4). Figure 4. Non-metallic particles forming a layer at theliquid-gas interface in a metallic foam (after [P41]).” – p. 432P41-c12. T.Wübben: Zur Stabilitat flüssiger Metallschaume – Universitat Bremen, Germany, 2003, 128 pp. – „Indiesem Zusammenhang wird das schon erwahnte Stabilisierungsmodell von G.Kaptay ausführlicherlautert und kritisch diskutiert” – p.2, „Nach einer kurzen Beschreibung der gegenwartigen Diskussionüber die Wirkungsweise von Partikeln in Metallschaumen wird schlieslich ein von Kaptay entwickeltesModell [P41]. Die im Rahmen dieser Arbeit gefundenen experimentellen Resultate haben deutlicheIndizien für die prinzipielle Gültigkeit dieses Modells erbracht” – p.25, „In diesem Kontext hat Kaptay[P41] ein mechanistisches Modell entwickelt, das sowohl den Einflus der Partikelkonzentration als auchdes Kontaktwinkels auf die Stabilitat von Metallshaumen beschreibt. Diese Arbeit beschaftigt sich ingroSen Teilen mit der Untersuchung der Gültigkeit deises Modells. Es soll daher folgenden im Detailerlautert werden” – p.30. „Mit Ausnahme von Kaptay in [P41] geben jedoch alle Autoren nurphanomenologische Erklarungen. Die in [P41] erstmals angedeutete Hypothese wurde unterBerücksichtigung der im Rahmen dieser Arbeit gewonnenen experimentellen Ergebnisseweiterenwickelt, so daS es quantitative Aussagen über die Wirksamkeit von Partikeln inMetallschaumen möglich mach” – p.31. „Das von Kaptay entworfene Modell versucht eine Erklarungfür die beobachtete stabilisierende Wirkung von Partikeln auf flüssige metallische Schaume zu geben.”– p.37.P41-c13. S.V.Gnyloskurenko, T.Nakamura: Wettability effect on bubble formation at nozzles in liquidaluminum – Mater. Trans., 2003, vol.44, pp.2298-2302 – „the contact angle for SiO 2 in liquid Al.Kaptay [P41] indicated = 50 – 60 o .” – p.2299P41-c14. A.Haibel, J.Banhart: Metallschaumcharakterisierung mittels Synchrotron-Tomografie – DACHJahrestagung, 2004, Salzburg, 7 pp (Ref. No. 5). – “Dadurch nimmt die Drainage ab und dieOberflachenspannung im Schaum reduziert, was zu einer Verringerung des Porenplatzens führt [P41]”– p.1P41-c15. E.Baumeister: Hohlkugelkomposit – Charakterizung thermischer und mechanischer Eigenschafteneines neuen Leichtbauwerkstoffes – Dissertation, 2004, Magdeburg (Ref. 79). – „Probleme bereiten diegeringe Duktilitat und die schlechte Bearbeitbarkeit der geschaumten MMC-Werkstoffe [P41]” – p.11.P41-c16. Alex Buetow: Diploma Arbeiten, TU Berlin, 2004 (Ref.No.9). – „Dieses Verfahren wurde gleichzetigund unabhangig von den Firmen Alcan und Norsk Hydro entwickelt [P41]” – p.6.P41-c17. S.V.Gnyloskurenko, A.Byakova, T.Nakamura, O.Raychenko: Influence of wettability on bubbleformation in liquid – J.Mater.Sci., 2005, vol.40, pp.2437-2441 – „the contact angle for SiO 2 in liquidAl.. Kaptay [P41] indicated = 50 – 60 o .” – p.2438P41-c18. Th.Wübben, S.Odenbach: Stabilisation of liquid metallic foams by solid particles – Colloids SurfacesA., 2005, vol.266, pp.207-213 – “Another, thermophysical, stabilizing mechanism was suggested byKaptay [P41], relying on the adhesion properties of solid particles and liquid metals” – p.207.P41-c19. A.J.Klinter, G. Mendoza-Suarez, R.A.L.Drew: Wetting of pure aluminum and selected alloys onpolycrystalline alumina and sapphire – Mater Sci Eng A, 2008, vol.495, pp.147-152. – “Recently, it hasbeen found that the wetting behavior in metal-ceramic systems seems to play an important role in theproduction of aluminum foams [P41].” – p.147. “In theoretical models of Kaptay [P41], the stabiklizingeffect of these particles on the liquid aluminum foam is credited to capillary effects between the meltand the particles, preventing the two liquid gas interfaces of a foam cell wall from touching and the twoadjacent cells from coalescence” – p.148.110

P41-c20. A.J.Klinter, R.A.L.Drew: Evaluation of the wetting behaviour of Al-7Cu and Al-11.5Si on SiC andsapphire in terms of Al-foam stability. In: METFOAM-2007, ed. by L.P.Lefebre, J.Banhart,D.C.Dunand, DEStech Publ. Inc, 2008, pp.23-26. – „During the early stages of Al-foam rersearch, itwas found that alumina or SiC particles are essential in order to obtain stable aluminium foams.Originally it was believed that the stabilizing effect of these ceramic particles have on Al-foams wascaused by an increase in bulk viscosity of the Al melt due to ceramic particles additions. In a verytheoreticla approach, KAPTAY [P41] later developed models suggesting that the improved foamstability was due to capillary effects between the melt and the particles, preventing the two liquid gasinterfaces of a foam cell wall from touching, and the two adjacent cells from coalescencing.” – p.23.P41-c21. P.Fernandez, LJ Cruz, Coleto J: Manufacturing processes of cellular metals. Part I. Liquid routeprocesses – Rev Metall, 2008, vol.44, pp.540-555.P41-c22. D.P.He, et al: www.scichina.com, 2009, vol.39, No.2, pp.97-105 in Chinese.P41-c23. A.V.Biakova, V.P.Krasovskii, A.O.Dudnik, S.V.Gniloskurenko, A.I.Sirko: O roli smachivaemosti Iraspredeleniia tviordich chastic v stabilizacii vspenennich aliuminievich rasplavov – Adgeziia rasplavovI paika materialov, 2009, vip.42, pp.5-22. – „Provedionnimi k nastoiashemu vremeni issledovaniiamuiubeditelno pokazano, shto vspenivanie metallicheskich rasplavov okazivaietsia nevozmozhnim priotsutstvii v nich tviordich vkliuchenii [P41].P41-c24. A.J.Klinter, C.A.Leon, R.A.L.Drew: The optimum contact angle range for metal foam stabilization: anexperimental comparison with the theory – J. Mater Sci., 2010, vol.45, pp.2174-2180 – „Based on theexperimental simulation of Sun et al., as well as a theory by Kaptay [P41], it is belived that thealuminium alloy melt needs to wet the added ceramic particles in a certain contact angle range” –p.2174.P41-c25. A.J.Klinter, C.A.Leon-Patino, R.A.L.Drew: Wetting phenomena of Al-Cu alloys on sapphire below800 C – Acta Mater, 2010, vol.58, pp.1350-1360 – „As the wetting behaviour of liquid metals onceramics strongly influences various processes like .. the quality of metal foams [P41]” – p.1350.P41-c26. S.Beke: Metal foaming controlled by ultrasonic waves – PhD Thesis, TU Wien, 2011, supervisors: HPDegischer and N.Babcsan. – „For liquid metal foams particles seem to be the only way of foamstabilization [P41]” – p.13.P41-c27. R. Montanari: Studio dei principali parametri di schiumatura per schiume di alluminio e supporto allaprogettazione di un impianto pilota di schiumatura, Report RdS/2011/201, Agenzia Nazionale per leNuove Tecnologie, l’Energia e lo Sviluppo Economico Sostenibile, Roma, Septembre, 2011. 94 pp. –„Kaptay [P41] ha sviluppato il seguente criterio per la selezione delle particelle ceramiche con cuistabilizzare schiume di Al con celle di dimensione predefinita (raggio R) separate da pareti di spessorepredefinito t: ….Eq.1….” – p.63.P40. G.Kaptay, S.V.Devyatkin: Titanium Diboride Coating Preparation in situ in the Cell byElectrochemical Synthesis – Proc. of 10 th Slovakian-Norvegian Symposium on AluminiumSmelting Technology, Stara Lesna – Ziar nad Hronom, Slovakia, 21-23 September, 1999, pp.80-84.P40-c1. G.V.Arkhipov, Y.S.Gorlanov: Development of technology for producing a wettable coating on a carboncathode by electrodeposition – Light Metals 2012, ed. by C.E. Suarez, TMS, pp.1367-1372. „Since1993, G.Kaptay and S.V.Devyatkin, under laboratory conditions, started to research on synthesis ofborides of high-melting metals from molten salts. They were among the first researchers who set a goalof proving the possibility of electrodeposition of TiB 2 from Na 3 AlF 6 -Al 2 O 3 -TiO 2 -B 2 O 3 melts. Theirattempts to create wettable coatings on carbon and metallic cathodes ended at the laboratory level[P40]” – p. 1367.P39. Kaptay G., Benkő Z.M., Tóth L.: The New Educational Structure of the Branch ofMetallurgical Engineering at the University of Miskolc - Int. Conf. on Engineering Education1999 (ICEE 99), August 10 - 14, 1999, Ostrava - Prague, Czech Republic. Proceedings issuedon CD-ROM (ISSN 1562-3580), paper No. 157.111

P38. Báder E., Kaptay Gy.: Acél folyamatos öntésekor fellépő határfelületi energiákvizsgálata. Miskolci Egyetem Doktoranduszok Fóruma, Kohómérnöki kar szekció kiadványa,Miskolc, 1999, 1-6.P37. S.V.Devyatkin, G.Kaptay, V.I.Shapoval, I.V.Zarutskii, V.P.Lugovoi, S.A.Kuznetsov:Deposition of Titanium, Zirconium and Hafnium Diboride Coatings by High-TemperatureElectrochemical Synthesis from Chloro-Fluoride Melts - in Refractory Metals in Molten Salts,ed. by D.H.Kerridge and E.G.Polyakov, Kluwer Academic Publishers, Netherlands, 1998, pp.73-80.P37-c1. V.V.Malyshev: High-temperature electrosynthesis of metal-like refractory compounds of IV-VI metalsin ionic melts – Russian J Inorg Chem, 2003, vol.48, pp.142-148 – „.. The electrolysis conditions forthe deposition of Group IVA metal diborides from chloro-fluoride melts are listed in [P37]” – p.144.P37-c2. V.V.Malishev: Visokotemperaturnii elektrochmnicheskii sintez metallopodobnich tugoplavkichsoedinenii metallov IV – VIA grupp v ionnich rasplavach – Zh. Neorg. Himii, 2004, vol.48, pp.187-194– “Usloviia osozhdeniia diboridov metallov IVA gruppi iz hloridno-ftoridnich rasplavov obobsheni v[P37]” – p.189.P37-c3. V.V.Malyshev: Zashitnie pokritiia tugoplavkimi soedineniiami metallov IV-VIA grupp, nanosimie izionnich rasplavov (obzor) – Zashita metallov, 2004, vol.40, pp.584-600 - „opisanie rezultatov [P37] v38 strokach (az eredmények ismertetése 38 sorban, állásfoglalás nélkül)” – p.595P37-c4. V.V.Malyshev, Kh.B.Kushkhov: Advances in high-temperature electrochemical synthesis in ionic meltsby the onset of XXI century – Russ J. of General Chem., 2004., vol.74, pp.1139-1146 (Zh. ObsheiHimii, 2004, vol.74, pp.1233-1240) – „see Table 1” – p.1141, „COnditions for deposition of GroupIVA metal diborides from chloro-fluoride melts are summarized in [P37].” – p.1141.P37-c5. V.V.Malyshev: Electrochemical Sysnthesis of Protective Coatings of Refractory Compounds of GroupIva-Via Metals from Ionic Melts – Russian Journal of Non-Ferrous Metals, 2007, vol.48, pp.177-183(Izv. Vuzov Cvetnaya Metallurgiya, 2007, No.3, pp.20-27) – “The authors of [P37] refined theconditions of electrodeposition of titanium, zirconium and hafnium diborides from chloro-fluoride KCl- NaCl (1:1) - NaF - KBF 4 - K 2 MF 6 (M = Ti, Zr, Hf) melts”. – p.178. Table 1 – a line is taken from[P37]” – p.178.P37-c6. A.I.Hab: Hig-tempearture electrochemcial synthesis of coatings of carbides, borides and silicides ofmetals of the IV-VI B groups from ionic melts (review) – Materials Science, 2007, vol.43, pp.383-397(Fiziko-Himichna Mechanika Materialov, 2007, vol.43, No.3, pp.76-88) – „As noted in [P37], chloridefluoridemelts are more promising as compared with fluoride and oxofluoride melts: the former are lesscorrosive, the separation of products from the electrolyte is simpler, and the current yield is higher. Inthis work, …. 11 lines of description of the results” – p.393.P37-c7. U.Fastner, T.Steck, A.Pascual, G.Fafilek, GE Nauer: Electrochemical deposition of TiB 2 in hightemperature molten salts – J Alloys Comp., 2008, vol.452, pp.32-35 – „Among all the electrolytesreported int he literature [P37] our work was focused on….. “ – p.32. “The mechanism of TiB 2 cathodicdeposition used in the calculations was proposed by Devyatkin and Kaptay [P37] as follows: 6 lines + 2equations follow” – p.33.P37-c8. W. Friedhoff, E. Milke, M. Binnewies: The Unexpected Formation of MB2 Layers (M = RefractoryMetal) on Metal Surfaces - Eur. J. Inorg. Chem., 2011, vol.2011, pp.3398-3402. – „Somewhat thickerlayers can be formed by sputtering (500 nm) and electrodeposition [P37]” – p.3398.P36. Bolyán L., Kaptay Gy.: Nedvesítési viszonyok meghatározása fémolvadék/kerámiarendszerekben a kompozitanyaggyártás optimalizálása céljából - Miskolci EgyetemDoktoranduszi Fórum (1997. nov.16). Kohómérnöki Kar szekciókiadványa, 1998. Miskolc,18 - 26 o.P35. Jánosfy Gy., Kaptay Gy.: Fémesalumínium-tartalom meghatározása aktívoxigén-mérőszondával a végtermék fémesalumínium-tartalmának beszabályozásához - XIII. OrszágosNyersvas- és Acélgyártó konferencia kiadványa, II. kötet, 235-243 o., Dunaferr, 1998.112

P34. R.Román, E.Báder, G.Kaptay: Penetration of Molten Calcium Chloride and MagnesiumChloride into Porous Oxide Ceramics and Pressed Fly-Ash Substrates - Proc. of MICROCAD‘98 Int. Computer Science Conference, Section C: Materials Science and Technologies,Miskolci Egyetem, 1998, pp. 115-116P33. P.Barkóczy, G.Kaptay: On the Interfacial Force Acting during Liquid Phase Sintering -Proc. of MICROCAD ‘98 Int. Computer Science Conference, Section C: Materials Scienceand Technologies, Miskolci Egyetem, 1998, pp. 113-114P32. M.S.Yaghmaee, G.Kaptay: Calculation of Mg-Cu Equilibrium Binary Phase Diagram -Proc. of MICROCAD ‘98 Int. Computer Science Conference, Section C: Materials Scienceand Technologies, Miskolci Egyetem, 1998, pp. 111-112P31. G.Kaptay: Calculation of Equilibrium Electrochemical Synthesis Diagram fopr the Ti +4 -B +3 System on the Reactive Carbon Cathode - Proc. of MICROCAD ‘98 Int. ComputerScience Conference, Section C: Materials Science and Technologies, Miskolci Egyetem,1998, pp. 109-110P30. K.Kelemen, R.Gemela, G.Kaptay: Dinamic Study of Incorporation of MicroscopicParticles into Liquid Metals - Proc. of MICROCAD ‘98 Int. Computer Science Conference,Section C: Materials Science and Technologies, Miskolci Egyetem, 1998, pp. 107-108P29. L.Bolyán, E.Báder, G.Kaptay: Wettability of Aluminium Oxide and Silicon OxideCeramics by Liquid Metals - Proc. of MICROCAD ‘98 Int. Computer Science Conference,Section C: Materials Science and Technologies, Miskolci Egyetem, 1998, pp. 105-106P28. G.Kaptay: Activity of the Working Group on Liquid Metals and Molten Salts (LIMOSGroup) at the Interface of Materials and Computer Sciences in 1997 - Proc. of MICROCAD‘98 Int. Computer Science Conference, Section C: Materials Science and Technologies,Miskolci Egyetem, 1998, pp. 101-104P27. G.Kaptay: Interfacial Criteria for Producing Ceramic Reinforced Metal-MatrixComposites - Proc. of the 2 nd Int. Conf. High Temperature Capillarity HTC 97 held inCracow, 29 June - 2 July 1997, ed. by N.Eustathopoulos and N.Sobczak, published in 1998 byFoundry Research Institute, Cracow, Poland. pp. 388-393P27-c1. E.Báder: Wettability of Alumina by Liquid Magnesium and Liquid AZ91 Alloy, Materials’ World (ejournal,http://materialworld.uni-miskolc.hu, July, 2001 – “The wettability of alumina by magnesium isa very important factor in producing metal matrix composites [P27] or metallic foams […] consisting ofthese two phases” – p.1 --P27-c2. Gao Y.G., Yao X.R., Liu Z.J., Li F.Z., Ren S.Z.: Development and application of ferrous matrixcomposites in foreign countries – Journal of Hefei University of Technology (Natural Science), 2006,vol.29, No.4, pp.431-436 (ref. No. 33).P27-c3. C.Borgonovo: Aluminum Nano-composites for elevated temperature applications – MSc Thesis atWorcester Polytechnic Institute, UK, June 2010 (advisors: D.Apelian, R.D.Sisson). „When injected inthe spray stram, the secondary phase tends to surround the strwam boundaries, causing inhomogeneousdispersion int he final piece [P27]” – p.23.P27-c4. WJ Shaw: Medical devices, US Patent No: US 7,854,756 B2, Dec,21, 2010.P27-c5. C.Borgonovo, D.Apelian: Manufacture of aluminum nanocomposites: a critical review – Mater SciForum, 2011, vol.678, pp.1-22 – „Kaptay [P27] noted that when the partially infiltrated liquid metalreaches the equilibrium depth (the depth at which interfacial forces are zero), further infiltration willoccur by additional pressure. The threshold pressure is given by: …. Eq.(6).” – p.14.113

P26. Maziar S. Yaghmaee és Kaptay György: Ón-ólom egyensúlyi fázisdiagram számításatermodinamikai alapadatokból - Termodinamikai Közlemények 1996. Szerkesztette LámerGéza, ELFT, Budapest, 1997, 100-112.P25. Kaptay Gy.: A Young egyenlet levezetése vektorok nélkül, azaz energiajellegűmennyiségekként értelmezve a határfelületi energiákat - Termodinamikai Közlemények 1996.Szerkesztette Lámer Géza, ELFT, Budapest, 1997, 90-99.P24. Buzinkay Emil, Kaptay György: Anyagtudományi célú kémiai termodinamikai adatbankfejlesztése. Első szint: szervetlen anyagok standard termodinamikai függvényei -Termodinamikai Közlemények 1996. Szerkesztette Lámer Géza, ELFT, Budapest, 1997, 86-89.P23. Bolyán László, Kaptay Gy.: Tiszta fémolvadékok határfelületi jellemzői -Termodinamikai Közlemények 1996. Szerkesztette Lámer Géza, ELFT, Budapest, 1997, 73-85.P22. Maziar Sahba Yaghmaee, G. Kaptay: Calculation of binary phase diagrams based onthermodynamic description of phases being in equilibrium - XX. Kémiai Előadói Napok,Program és előadásvázlatok, Szeged, 1997, pp. 72- 77P21. G.Kaptay: On the Interfacial Force between Ceramic Particles and Moving Solid-LiquidInterface during Solidification of Metal Matrix Composites - Proc. of the EUROMAT 97Conference held in Maastricht, Holland, 21-23 April 1997, published in volume 1. "Metalsand Composites", pp. 435-438.P21-c1. J.Braszczinski, M.Cisowska: Proba oceny krzepniecia kompozytow hybrydovych AlMg/SiC+Gr –Krzepniecie Metali i Stopow, 1999, Nr. 40, pp. 75-87 – „Z dotychczasowych badan wynika ponadto, zenie sa sluszne rozwazania G.Kaptay’s [P21[ w zakresie wplywu frontu krystalizacji na rozklad czastekw osnowie,gdyz roznica grafitu i weglika krzemu nie odegrala widocznej roli w ich rozkladzie wosnowie” – pp.85-86.P21-c2. J.Braszczynski, A.Zyska: Analysis of the influence of ceramic particles on the solidification process ofmetal matrix composites – Materials Science and Engineering A278 (2000) 195-203 – “… It resultsfrom this equation that the rate of the nuclei growth depends on the crystallization kinetics and thenucleation rate, so it is also dependent on the number of particles and their size. It is in good accordancewith the previous theoretical analyses concerning the behaviour of the particles at the solidificationfront and the restriction of the crystallization growth caused by the presence of the particles [P21] “–p.202P21-c3. Á.Borsik: Dynamic Simulation of the Movement of Ceramic Particles in front of an ApproachingSolidification Front, Materials’ World (e-journal, http://materialworld.uni-miskolc.hu, July, 2001 – “the interfacial force [P21] appears due to the interaction of surface atoms/ions/molecules of the ceramicparticle and the solid metal through the thin film of the liquid metal” - p.2. –P21-c4. J.T.Blucher, J.Dobranszky, U.Narusawa: Aluminium double composite structures reinforced withcomposite wires – Mater. Sci. Eng., 2004, vol.A387-389, pp.867-872 – „..successful infiltration ofcarbon fibers without special surface treatments was sporadic. … Al 2 O 3 , SiO, TiN. TiB as well as Cu anNi coatings all show promising results [P21]” – p.868.P20. L.Bolyán, G.Kaptay, S.V.Devyatkin: Wettability of Graphite by Cryolite Melt withDifferent Oxide Additions - Proc. of 8 th Int. Congress of ICSOBA, Milan, Italy, 16-18 1997,published in TRAVAUX, vol. 24., 1997 (No 28) pp. 510-519P19. G.Kaptay, S.V.Devyatkin: On Possibility of Preparation of Titanium Diboride CathodeCoating in situ in the Aluminum Electrolysis Cell by Electrochemical Synthesis - Proc.of 8 th Int. Congress of ICSOBA, Milan, Italy, 16-18 1997, published in TRAVAUX(ICSOBA), vol. 24., 1997 (No 28) pp. 135-144114

P19-c1. R.P.Pawlek: Aluminium Wettable Cathodes: An Update – in: Light Metals 2000, Ed. by R.D.Peterson,TMS 2000, pp. 449-454 – „High temperature electrochemical synthesis of TiB 2 from cryolite aluminamelts containing oxides of boron and titanium was tried by Deviatkin [ ] and Kaptay [P19]… „ + 14lines describing our results – pp. 449-450 –P19-c2. Vedernikov G.F.: Inertnie katodi v elektroliziorach dlia proizvodstva aliuminia. Problemi i perspektivi.AO VAMI, Informacionnii listok, No.10, April 2001. – „Kaptay i Devyatkin ispolzovalivisokotemperaturnii elektrochimicheskii sintez TiB 2 kriolito-glinoziomnich rasplavov [P19]. DOnachala ispitanii po osazhdeniu TiB 2 na grafitovich, molibdenovich i niobievich katodach, bili izuchenitermodinamicheskie svoistva TiB 2 v kriolito-glinoziomnich rasplavach, soderzhashich oksidi titana ibora. V sluchae ispolzovaniia ugolnich katodov adgeziia uluchalas sza chot obrazovaniia tonkogo sloiaTiC meczhdu uglerodom i diboridom titana” – c.16.P19-c3. Gorlanov ES, Nikiforov SA, Alternative technology to produce a wettable cathode surface layer in Alcells – Proc of the 12 th Int. Conf. “Aluminum of Siberia” (in Russian), Krasnoyarsk, 2006, pp.91-95. –„Naibolee perspektivnii, s popitkoi adaptacii k usloviiam elektroliza v krilito-glinoziomnich rasplavachpredstavlen v rabotach [P19]” – p.92.P19-c4. G.V.Arkhipov, Y.S.Gorlanov: Development of technology for producing a wettable coating on a carboncathode by electrodeposition – Light Metals 2012, ed. by C.E. Suarez, TMS, pp.1367-1372. „Since1993, G.Kaptay and S.V.Devyatkin, under laboratory conditions, started to research on synthesis ofborides of high-melting metals from molten salts. They were among the first researchers who set a goalof proving the possibility of electrodeposition of TiB 2 from Na 3 AlF 6 -Al 2 O 3 -TiO 2 -B 2 O 3 melts. Theirattempts to create wettable coatings on carbon and metallic cathodes ended at the laboratory level[P19]” – p. 1367.P18. Gy. Jánosfy, Gy. Kaptay.: Theoretical Method to Determine the Deoxidation Constant ofAl for Fe-Al-O System - in: Proceedings of microCAD '97 International Computer ScienceConference, Section B: Metallurgy, 1997. pp. 107-110.P17. Bolyán L., Buzinkay E., Kaptay Gy.: Fémolvadék/kerámia rendszerek határfelületijellemzői szoftver és adatbank ismertetése - in: Proceedings of microCAD '97 InternationalComputer Science Conference, Section C: Materials Science, Miskolc, 1997. pp. 117-118.P16. M.S.Yaghmaee, Kaptay Gy.: Calculation of Binary Eutectic Phase Diagrams on theExample of the Pb-Sn system - in: Proceedings of microCAD '97 International ComputerScience Conference, Section C: Materials Science, Miskolc, 1997. pp. 97-98.P15. Buzinkay E., Kaptay Gy: Kémiai reakciók számítására alkalmas szoftver és adatbank -in: Proceedings of microCAD '97 International Computer Science Conference, Section C:Materials Science, Miskolc, 1997. pp. 95-96.P14. Kaptay Gy.: Az Olvadék Munkacsoport tevékenysége az Anyagtudomány és aSzámítástechnika határterületén (avagy előszó három poszter bemutatónkhoz) - in:Proceedings of microCAD '97 International Computer Science Conference, Section C:Materials Science, Miskolc, 1997. pp. 39-42.P13. S.V.Deviatkin, K.I.Arsenin, G.Kaptay: High Temperature Interaction of Boron Oxidewith Aluminum Fluoride - in Proc of the 10 th International Symposium on Molten Salts,edited by R.T.Carlin, S.Deki, M.Matsunaga, D.S.Newman, J.R.Selman, G.R.Stafford,Electrochemical Society Proceedings, volume 96-7, 1996, pp. 312-319.P13-c1. A.S.Uzdenova: Elektrochimicseskoe vosstanovlenie i sintez soedinenii gadoliniia, bora i aluminiia vgalogenidnich rasplavach – Dissertacia na soiskanie uchionoi stepeni kandidata khimicheskich nauk,Nalchik, 2000, 313 pp.: „..V rabote [P13] IK-spektroskopiei i derivatografiei izuchenovisokotemperaturnoe vzaimodeistvie B 2 O 3 s AlF 3 . Naideno obrazovanie letuchego BF 3 i nekotorichkompleksnich Al-B-oksidov, kotorie okazivaiut stabiliziruiussee deistvie na bor pri moliarnomsootnoshenii B 2 O 3 :AlF 3 = 1:2 i nizhe.”, 31. o.115

P12. V.P.Lugovoi, S.V.Deviatkin, G.Kaptay, S.A.Kuznetsov: High TemperatureElectrochemical Synthesis of Zirconium Diboride from Chloro-Fluoride Melts - in Proc of the10 th International Symposium on Molten Salts, edited by R.T.Carlin, S.Deki, M.Matsunaga,D.S.Newman, J.R.Selman, G.R.Stafford, Electrochemical Society Proceedings, volume 96-7,1996, pp. 303-311.P12-c1. V.V.Malishev: Visokotemperaturnii elektrochmnicheskii sintez metallopodobnich tugoplavkichsoedinenii metallov IV – VIA grupp v ionnich rasplavach – Zh. Neorg. Himii, 2004, vol.48, pp.187-194– “Dalneishee razvitie VES diborida cirkonia iz hlordnich, ftoridnich i oksidnich rasplavov rassmotrenv [P12]. Termodinamicheskim rasschotom pokazano, shto raznost ravnovesnich potencialov cirkoniia ibora sostavliaet 0.75 V (pri 973 K), 0.53 V (pri 973 K) i 0.45 V (pri 1273 K) cootvetstvenno.Cepcialnie pokritiia ZrB2 na steklouglerode iz rasplava NaCl + KCl + k2ZrF6 + KBF4 + NaFpolucheni lish pri dobavke B2O3 (dlia snizheniia katodnoi passivacii) i plotnosti toka 0.05 – 0.5 A/cm2.Uvelichenie plotnosti toka privodit k obrazovaniu poroshkovich osadkov” – p.189.P12-c2. V.V.Malyshev: High-temperature electrosynthesis of metal-like refractory compounds of group IV-VImetals in ionic melts – Russian J Inorg Chem, 2003, vol.48, pp.142-148 – „Further advances int heelectrosynthesis of zirconium diboride in chloride, fluoride and oxide melts are considered in [P12]” –p.144.P12-c3. V.V.Malyshev, Kh.B.Kushkhov: Advances in high-temperature electrochemical synthesis in ionic meltsby the onset of XXI century – Russ J. of General Chem., 2004., vol.74, pp.1139-1146 (Zh. ObsheiHimii, 2004, vol.74, pp.1233-1240) - – „see Table 1” – p.1141, „Further advances in high-temperatureelectrochemical synthesis of zirconiuum diboride from chloride, fluoride and oxide malts wereconsidered in [P12]” – p.1141.P12-c4. Shumakova NI, Procenko ZM, Gudakova GO, Bugaenko VV: Fazovii, elementnii sklad tamikrostruktura elektrolitichno otrimanich poroshkopodobnich produktiv na osnovi siliciiu, titanu, boruta ich spoluk – Bisnik Sumskogo Derzhavnogo Universiteta, Seriia Fizika, matematika, mechanika,2004, No. 10 (69), 196-205.P12-c5. VV Bugaenko, ZM Procenko, NI Shumakova: Fazovii, elmentnii ta granulometrichnii skladelektrolitichno otrimanich poroshkopodobnich produktiv na osnovi boridiv titanu – Bisnuk SumDU,2006, No.6, pp.114-122 – „Odnim iz bagatoh metodiv oderzhaniia boridiv metalic svisokotemperaturnii elektrohimichnii sintez (VES) b rozplavlenich soliovich elektrolitach, iakii sperspektivnim metodom oderzhaniia poroshkopodobnich boridiv metaliv ta nemetaliv [P12]” – p.115.P11. L. Bolyán, E. Buzinkay, G. Kaptay : Szoftver és adatbank tiszta fémolvadékok fizikaitulajdonságainak számolására a hőmérséklet függvényében. in: Proceedings of microCAD '96International Computer Science Conference, Section C: Materials Science, Miskolc, 1996. pp.53-54.P10. L. Bolyán, G. Kaptay : Tiszta fémolvadékok felületi feszültségének számolásáraalkalmas szakértői rendszer. in: Proceedings of microCAD '95 Int. Computer ScienceConference, Section C: Material Science, Miskolc, 1995., pp.147-152.P9. E. Buzinkay, G. Kaptay: Anyagtudományi célú kémiai-termodinamikai adatbankfejlesztése. in: Proceedings of microCAD '95 Int. Computer Science Conference, Section C:Material Science, Miskolc, 1995., pp.142-146.P8. Kaptay Gy.: Anyagtudományi célú kémiai-termodinamikai adatbank tervezete. in:"Termodinamikai Előadások", szerk. Lámer G., ELFT, Budapest, 1994., pp. 171-173.P7. Deviatkin Sz., Kaptay Gy., Berecz E.: Stabil sztöchiometriájú fémboridok elektrokémiaiszintézisének kémiai-termodinamikai kritériumai. in: "Termodinamikai Előadások", szerk.Lámer G., ELFT, Budapest, 1994., pp.165-170.116

P6. Kaptay Gy., Lámer G.: Alakadás mikrogravitációban. in: "Termodinamikai Előadások",szerk. Lámer G., ELFT, Budapest, 1994., pp.72-75.P5. Kaptay Gy.: Asszociált elegymodellek alkalmazása fém- és sóolvadék elegyektermodinamikai leírásához. in: "Termodinamikai Előadások", szerk. Lámer G., ELFT,Budapest, 1994., pp.48-53.P4. S.V.Deviatkin, G.Kaptay, E.Berecz : High-temperature electrochemical synthesis of TiB 2from cryolite-alumina melts containing oxides of Boron and Titanium. In Proc. of the 9 th Int.Symp. on Molten Salts, edited by C.L.Hussey, D.S.Newman, G.Mamantov, Y.Ito. Proc.volume 94-13 of the Electrochemical Society Inc, pp. 548-557.P4-c1: L.P.Polyakova, E.G.Polyakov, N.J.Bjerrum: The study of electrode processes in LiF-NaF-KF-K 2 TaF 7 -KBF 4 melt – Plasmas and Ions, 1999, 2, 117-125 – „Analysis of the literature shows that the relevantpublications are mostly dedicated to the synthesis of titanium and zirconium borides [P4].” p.117 –P4-c2. S.A.Kuznetsov: Elektrokhimicheskii sintez visokotemperaturnich boridov iz solevich rasplavov –Elektrokhimiia, 1999, t.35., No.11., 1301-1317 – “Sostav elektrolitov i usloviia polucheniiatugoplavkich boridov predstavleni v tabl.2. [P4]..” p. 1311P4-c3. N.Ene: Electrosynthesis and electrochemistry of TiB 2 in molten electrolyte – Rev Roum de Chimie, 1999,vol.44, pp.643-650. – „The equilibrium potential needed for the synthesis to occur is given by theequation [P4]: {equation cited}” – p.648P4-c4. R.P.Pawlek: Aluminium Wettable Cathodes: An Update – in: Light Metals 2000, Ed. by R.D.Peterson,TMS 2000, pp. 449-454 – „High temperature electrochemical synthesis of TiB 2 from cryolite aluminamelts containing oxides of boron and titanium was tried by Deviatkin [P4] and Kaptay [ ]… „ + 14 linesdescribing our results – pp. 449-450 –P4-c5. Vedernikov G.F.: Inertnie katodi v elektroliziorach dlia proizvodstva aliuminia. Problemi i perspektivi.AO VAMI, Informacionnii listok, No.10, April 2001. – Devyatkin i dr. ispolzovali visokotemperaturniielektrochimicheskii sintez TiB 2 kriolito-glinoziomnich rasplavov, soderzhashich oksidi bora i titana[P4]”. – c.16.P4-c6. P.Taxil, P.Chamelot, L.Massot, C.Hamel: Electrodeposition of alloys or compounds in molten salts andapplications – J. of Mining and Metallurgy, 2003, vol.39B, pp.177-200 – „In the industry of aluminiumelectrowinning, titanium or zirconium borides are possibly used to protect the carbon cathodes from theelectrolyte insertion. Numerous works are dedicated to the preparation of these compounds by theelectrodeposition in molten salts, either in molten fluorides or in cryolithe meia [P4]” – p.178.P4-c7. V.V.Malyshev: High-temperature electrosynthesis of metal-like refractory compounds of IV-VI metals inionic melts – Russian J Inorg Chem, 2003, vol.48, pp.142-148 – „.. Devyatkin et al. [P4] carried out athermodynamic plausability analysis of the electrosynthesis of TiB 2 and found the conditions for theformation of this compound. They noted that a TiC film forms on graphite cathode early in the process,favoring a better adherence of TiB 2 layers” – p.144.P4-c8. V.V.Malishev: Visokotemperaturnii elektrochmnicheskii sintez metallopodobnich tugoplavkichsoedinenii metallov IV – VIA grupp v ionnich rasplavach – Zh. Neorg. Himii, 2004, vol.48, pp.187-194– “…VES diboridov metallov IVA gruppi vozmozhen i iz kriolito-glinoziomnich rasplavov. Primenenieetich rasplavov s prakticheskoi tochki zreniia neobhodimo dlia zashiti grafitovich elektrodov ipolucheniia aliuminievich ligatur. Termodinamicheskaia ocenka vozmozhnosti elektrosinteza TiB2 iusloviia ego eksperimentalnogo osushestvleniia pokazani v [P4]. Avtori otmechaiut, shto v nachalniimoment osazhdeniia na grafitovich katodach obrazuetsia sloi karbida titana TiC, sposobstvuiushiiuvelicheniu scepleniia dalneishich sloev TiB2 s materialom katoda” – p.189.P4-c9. V.V.Malyshev, Kh.B.Kushkhov: Advances in high-temperature electrochemical synthesis in ionic meltsby the onset of XXI century – Russ J. of General Chem., 2004., vol.74, pp.1139-1146 (Zh. ObsheiHimii, 2004, vol.74, pp.1233-1240) – – „see Table 1” – p.1141, „The possibility and experimentalconditions of electrochemical synthesis of TiB2 are evaluated thermodynamically in [P4]. It is noted,that initially a TiC layer is formed on the graphite cathode – this layer improves the adhesion of thesubsequently deposited TiB2 layers on the cathode material” – p.1141.P4-c10. Gorlanov ES, Nikiforov SA, Alternative technology to produce a wettable cathode surface layer in Alcells – Proc of the 12 th Int. Conf. “Aluminum of Siberia” (in Russian), Krasnoyarsk, 2006, pp.91-95. –„Naibolee perspektivnii, s popitkoi adaptacii k usloviiam elektroliza v krilito-glinoziomnich rasplavachpredstavlen v rabotach [P4]” – p.92.P4-c11. G.V.Arkhipov, Y.S.Gorlanov: Development of technology for producing a wettable coating on a carboncathode by electrodeposition – Light Metals 2012, ed. by C.E. Suarez, TMS, pp.1367-1372. „Since117

1993, G.Kaptay and S.V.Devyatkin, under laboratory conditions, started to research on synthesis ofborides of high-melting metals from molten salts. They were among the first researchers who set a goalof proving the possibility of electrodeposition of TiB 2 from Na 3 AlF 6 -Al 2 O 3 -TiO 2 -B 2 O 3 melts [P4]” – p.1367.P3. S.V.Deviatkin, G.Kaptay, V.I.Shapoval, E.Berecz Electrochemical synthesis of transitionmetal diborides from molten salts - in : Proceedings of the International Symposium onMolten Salt Chemistry and Technology, 1993, Ed. by M-L. Saboungi and H. Kojima, Proc.vol.93-9 of the Electrochemical Society Inc., pp. 584-599.P3-c1. S.A.Kuznetsov, A.L.Glagolevskaya, A.T.Belyaevskii: Electrodeposition of Tantalum Boride Coatings inSalt Melts - Russian Journal of Applied Chemistry, vol.67, No7., Part1, 1994, pp. 967-973 – “Dannie povisokotemperaturnomu elektrohimicheskomu sintezu boridov tantala prakticheski otsutstvuiut, lish vrabotah [P3], gde izuchalis katodnie processi, imeiutsia otdelnie ukazaniia po ih polucheniiu.” p.1093 --P3-c2. L.P.Polyakova, G.A.Bukatova, E.G.Polyakov, E.Kristensen, I.Barner, N.Bjerrum: Katodnie processi provosstanovlenii bora vo ftoridnom rasplave – Elektrokhimiia, 1995, tom 31, No 12, 1348-1353 –„Bolsinstve avtorov [P3] nahodiat ego (katodnoe videlenie bora) odnostadiinim ….” p. 1348 --P3-c3. L.P.Polyakova, G.A.Bukatova, E.G.Polyakov, E.Christensen, J.H. von Barner, N.J.Bjerrum:Electrochemical Behaviour of Boron in LiF-NaF-KF Melts - J. Electrochem. Soc., vol 143, No 10.,1996, pp. 3178-3186 – „These authors as well as others [P3] suggested that the process of boron(III)reduction in chloride-fluoride and fluoride melts proceeded in one step without the particpation ofintermediates…” p.3179P3-c4. E.Polyakov, O.Makarova, L.Polyakova, A.Shevyryov, E.Christensen, N.J.Bjerrum: Electrodeposition ofTantalum Boride Coatings from Oxo-fluoride Melts - Molten Salt Forum, vols 5-6, 1998, 375-378 – „Inthe 90’s electrochemical synthesis of tantalum borides attracted the attention of scientists [P3].” p.375 --P3-c5. N.Ene: Electrosynthesis and electrochemistry of TiB 2 in molten electrolyte, Roumanian ChemicalQuarterly Reviews, 1998, 6(4), 233-245 – „Thermodynamic estimation of the possibility ofelectrochemical synthesis of TiB 2 from cryolite based electrolytes has been carried out using the generalequation [P3]: {egyenelet}. This equation and the existing electrochemical and thermodynamic data[…] afforded the calculation of the following theoretical equilibrium deposition potential in cryolitebasewd electrolytes containing dissolved B 2 O 3 and TiO 2 at 1273 K (Table 1) (9 soros táblázatszámításokkal az egyenlet segítségével) – 238.o.P3-c6: L.P.Polyakova, E.G.Polyakov, G.A.Bukatova, A.A.Shevyryov, A.V.Makarova. N.J.Bjerrum: Study ofElectrode Processes in FLINAK-K 2 TaF 7 -KBF 4 melt - in Refractory Metals in Molten Salts (TheirChemistry, Electrochemistry and Technology), ed. by D.H.Kerridgeand E.G.Polyakov - KluwerAcademic Publishers, vol.3/53, 1998, pp. 103-108. – „The data on electrochemical synthesis oftantalum borides are contradictory and limited by the area of chloro-fluoride melts [P3]” p. 103 --P3-c7: L.P.Polyakova, E.G.Polyakov, N.J.Bjerrum: The study of electrode processes in LiF-NaF-KF-K 2 TaF 7 -KBF 4 melt – Plasmas and Ions, 1999, 2, 117-125 – „The data on high-temperature electrochemicalsynthesis of tantalum borides are few [P3] and mostly deal with mixed chloro-fluoride electrolytes.”p.117 --P3-c8. S.A.Kuznetsov: Elektrokhimicheskii sintez visokotemperaturnich boridov iz solevich rasplavov –Elektrokhimiia, 1999, t.35., No.11., 1301-1317 – “Sostav elektrolitov i usloviia polucheniiatugoplavkich boridov predstavleni v tabl.2. [P3]..” pp. 1311P3-c9. N.Ene: Electrosynthesis and electrochemistry of TiB 2 in molten electrolyte – Rev. Roum. De Chimie,1999, vol.44, pp.643-650 (ref.No.9)P3-c10. S.A.Kuznetsov: Elektrochimicheskii sintez novich soedineniiu i perspektivnich materialov razlichnogofunkcionalnogo naznacheniia v solevich rasplavach – Otchot gos zakaz, 2004 (Ref. No.5). –„Termodinamicheskomu obosnovaniu processov elektrochimicheskogo sinteza, osnovannomu nasopostovlenii temperaturnich zavisimostei potencialov videleniia metallov i bora iz nich razlichnichsoedinenii posviashena rabota [P3]” – p.1.P3-c11. N.Rybakova, M.Souto, Y.Andriyko, W.Artner, J.Godinho, G.E.Nauer: Morphology and mechanicalproperties of TiB2 coatings deposited from chloride-fluoride melts by pulse electroplating – JElectrochem Soc, 2009, vol.156, pp.D131-D137 – „The method of electrochemical depostion of TiB2from molten salt electrolytes, which was developing over the last decades, is more flexible [P3]” – p.D131.118

P3-c12. N.Rybakova, M.Souto, H.P.Martinz, Y.Andriyko, W.Artner, J.Godinho, G.E.Nauer: Stability ofelectroplated titanium diboride coatings in high-temperature corrosive media – Corrosion Science,2009, vol.51, pp.1315-1321 – The electrodeposition of TiB 2 from molten salts is significantly faster,less expensive and permits to obtain well defined and smooth deposits on different substrates withcomplicated surface profiles and homogeneous layer thickness [P3]” – p. 1315.P3-c13. JRA Godinho: Optimization of TiB 2 coatings electrodepisted from halide melts – Master dissertation inChemistry, April 2008, 70 pp. – “From the 90-s onward some practical aspects of the deposition ofdifferent borides (e.g. TiB 2 ) were clarified, along with the basic electrochemical techniques andthermodynamic calculations [P3]” – p.10.P3-c14. G.V.Arkhipov, Y.S.Gorlanov: Development of technology for producing a wettable coating on a carboncathode by electrodeposition – Light Metals 2012, ed. by C.E. Suarez, TMS, pp.1367-1372. „Since1993, G.Kaptay and S.V.Devyatkin, under laboratory conditions, started to research on synthesis ofborides of high-melting metals from molten salts. They were among the first researchers who set a goalof proving the possibility of electrodeposition of TiB 2 from Na 3 AlF 6 -Al 2 O 3 -TiO 2 -B 2 O 3 melts [P3]” – p.1367.P2. Kaptay Gy., Akhmedov S.N., Borisoglebskii Yu.V., Deviatkin S.V., Berecz E. Újanyagok az alumínium elektrolízisben - In: "A Kohómérnöki Kar kutatási eredményei",Miskolci Egyetem, Miskolc, 1992. június 25. pp. 101 - 109.P1. Borisoglebskiy Yu.V., Akhmedov S.N., Kaptay G., Vetyukov M.M. Corrosion of metallikerefractory materials in chloroaluminate melts and molten aluminum. In : "Proc. ofEUROCORR'91", ed. by I.Karl and M.Bod, vol.I., pp.313-318.119

M. Selected manuscripts (with citations)M507. Kaptay Gy.: Tantárgyi kommunikációs dosszié és tantárgyleírás a Határfelületi nanojelenségekc. BSc tantárgyhoz. Javított és kiegészített verzió, 79 oldal, 2010. május 18.M507-c1. Pázmán J.: Szilíciumkarbid szemcsék kémiai nikkelezése és fémkompozitokban történő alkalmazása –PhD disszertáció (tud. vez.: Gácsi Z.), Miskolc, 2010. – „1.19. ábra. Szilárd/folyadék/gáz határfelületnedvesíthetőség és a peremszög kapcsolata [M507]” – 27.o.M507-c2. Balla S., Bán K., Bárdos A., Lovas A., Szabó A., Weltsch Z.: Járműanyagok - Egyetemi tananyag,szerkesztő: Lovas Antal, ISBN 978-963-279-628-4, Typotex Kiadó, Budapest, 2012, 269 pp. – „5.2.fejezet. Határfelületi energia termodinamikai és mechanikai értelmezése [M507]” – 148-149 o. “5.4.fejezet: Folyadékcsepp egyensúlyi alakjai más fázisokkal kontaktusban [M507]” – 150-153 o., „5.6.1.fejezet: Marangoni áramlás [M507]” – 154-155. o., „5.6.2. fejezet: Eötvös szabály [M507]” – 155-156 o.,„5.6.3. alfejezet: Gázok adszorpciója szilárd és folyadék fázisok felületére [M507]” – 156 o., „5.6.4fejezet: Felületi szegregáció [M507]” – 156-157 o., „5.6.5. fejezet: Adszorpció [M507]” – 157.o.M.343. Az Fe-Mn ausztenitben oldott karbon aktivitása, illetve a karbon diffúzió hajtóereje -Réger Mihály részére, 2008. október 11-12, 7 pp.M343-c1: M.Réger, B.Verő, I.Kardos, P.Varga: The effects of alloying elements on centerline segregation –Defect Diff Forum, 2010, vol.297-301, pp.148-153. – „Fig.4 compares the carbon activity results of threemodels [M343]…” – p.150.M.305. Az Estphad függvények alkalmazhatósága monotektikus diagramok szétválásigörbéjének leírására (Roósz András, Mende Tamás és Farkas János részére, Mende TamásTDK-ja nyomán, 2008. február 15-16., George) – 8 oldal.M.305-c1. T.Mende, A.Roosz: Calculation of the miscibility gap by Estphad method – Mater Sci Forum, 2010,vol.659, pp.423-428. – The function of concentration of separation temperature can be derived from theregular solution model [M305]: … Eq.(2)” – p.424. „The boundary condition can be fulfilled byintroducing the quantity having a character of X* mole fraction as well as by introducing the kdimensionless coefficient and they can be included int he correction factor [M305]” – p.425.M.170. Kaptay Gy.: Fémolvadék széterülésének feltétele fémolvadékon monotektikusrendszerekben - Svéda Marika és munkatársai részére, 2004. február 20., 4 oldalM170-c1. Svéda Mária: Monotektikus felületi rétegek létrehozása lézersugaras felületkezeléssel c. PhD értekezés(tudományos vezető: dr. Roósz András) – 2007 (Ref. No.44).M.163. Kaptay G: Határfelületi energiák, erők és jelenségek fizikai-kémiai modellezése ametallurgia és a fémes anyagmérnökség egyes területein – MTA doktori értekezés, 2003.szeptember, 141 ppM163-c1. N.Babcsan, D.Leitlmeier, H.P.Degischer: Foamibility of Particle Reinforced Aluminum Melt – Mat.-wiss. u. Werkstofftech., 2003, vol.34, pp.1-8 (ref. No.31)M163-c2. N.Babcsán: Ceramic Particle Stabilized Aluminum Foams – PhD Dissertation, Miskolc, 2003 (ref.No.93)M163-c3. A.Ender, H.van den Boom, H.Kwast, H-U. Lindenberg – Metallurgical development in steel-plantinternalmulti-injection hot metal desulphurozation – Steel Research Int., 2005, vol.76, ppp.562-572M142. Kaptay Gy.: Az ESTPHAD algoritmus (történelem lecke + sztandartizálási javaslat) –dr. Roósz A., Farkas J., Kövér Zs. és Mende T. r., 2002. november 24., 11 o.M142-c1. Zs.Kövér, A.Roósz: Calculation of the equilibrium phase diagram of Fe-Ni alloy system bythe ESTPHAD method – Materials Science Forum, 2006, vol.508, pp.609-614 (No.1)M142-c2. J.Farkas, A.Roósz: Calculation of the liquidus and solidus surface of Al-rich corner of Al-Mg-Si alloy system by ESTPHAD method – Materials Science Forum, 2006, vol.508, pp.635-640 (No.1)120

M112. Kaptay Gy.: WC szemcsék kémiai kölcsönhatása Al-4Cu-1Si olvadékkal (egyszerűsítetttermodinamikai analízis) - rövid feljegyzés Roósz András és Sólyom Jenő részére, 2001. augusztus 7.,6 oldal.M112-c1. J.Sólyom, A.Roósz, I.Teleszky, B.Sólyom: Laser Alloying of the Surface Layer of Al4.5Cu1Si Alloywith TiC and WC Particles – Materials Science Forum, 2003, vols. 414-415, pp.37-44 (ref. No.8).M61. Kaptay Gy., M.Z.Yaghmaee, Jánosfy Gy., Károly Gy.: A Fe-Al-N-B olvadékrendszertermodinamikai vizsgálata. Részjelentés, mely készült a „A bórral mikroötvözött acélokgyártásbiztonságának és megfelelőségének további javítása” c., DAM-kutatási témához. Miskolc,1999 május-június. M61.-a: Maziar’s summer work, 1999 September.M61-c1. Besztercey Viktor: A bór mikroötvözés metallurgiai szempontjai. Miskolci Egyetem DoktoranduszokFóruma, Miskolc, 1999. november 4-5. Kohómérnöki Kar szekciókiadványa, Miskolc-Egyetemváros,2000., pp. 28-33 (reference No. 6.).M60. Kaptay Gy., Z.Benkõ Mária: LD konverter fizikai-neurális, vagy neurális-fizikai hibridmodelljének fizikai-kémiai alapjai. Miskolc, 1999. június. 46 oldal.M60-c1. P.Berényi, J.Valyon, G.Horváth: Neural Modelling of Industrial Process with Noisy data - in:„Engineering of Intelligent Systems, IEA/AIE 2001, LNAI 2070“, edited by L.Monostori, J.Váncza,M.Ali, Springer Verlag, Berlin, 2001, pp.269-280.M50. Kaptay Gy.: Határfelületi energiák és jelenségek vizsgálata metallurgiai és anyagmérnökitechnológiákban - Habilitációs tézisfüzet, Miskolci Egyetem, 1998. augusztus 30., 60 oldal.M50-c1. P.Harmat, I.Kotsis, L.Laczkó, L.Bartha: Melting and phase transformation of hardmetal powders –Solid State Ionics, 2001, vol.141-142, pp.157-161 (ref. No.7).M50-c2. G.Králik, P.Fülöp, B.Verő, D.Zsámbok: Laser Surface Treatment of Steels – Materials Science Forum,2003, vols.414-415, pp.21-30 (ref. No.2).M.6. Kaptay G. Study of chemical interaction of high-temperature chloro-aluminate melts with liquidaluminum, some refractory materials and oxygen with the aim of developing a new aluminumelectrolysis process. (in Russian) - Ph.D. Thesis, Leningrad, 1988, 268 p.M6-c1. Akhmedov S.N.: Study of durability of refractory materials in Aluminium containing melts in order totheir usage in Aluminium electrolysis cells. (in Russian). PhD Thesis, Leningrad, 1988, 267 p. (referenceNo 124)121

h-indexIndependent citations / yearStatistics140120100growing phasex38 20Cit 10Fig.1.a80604020incubation phaseCit x 28 20independent citations25 30 35 40 45 50 55Age (years)18161412y = 0,0226x 2 - 1,1531x + 14,721R 2 = 0,9873dh/dt=1Fig.1.b1086dh/dt=1/24dh/dt=02025 30 35 40 45 50 Age 5529 3241Fig.1. The dynamics of publications and independent citations (Fig.1.a) and that of the h-index calculated from independent citations (Fig.1.b)122

Statistics for independent citations of my papers and the calculation of my h-index*Papers with the given number of independent citationsCitationsCode of papers (see the list above) amount Totalamount1 J43, J49, J56, J61, J70, J75, J83, J88, J89, J98, J105, J137, J138, JP8, JP9, JP11, 37 103–139P13, P40, P46, P47, P49, P69, P71, P72, P86, P108, M57, M6, M60, M61,M112, M170, M305, M343, M507, B5, B9,2 J10, J26, J27, J30, J35, J44, J45, J47, J64, J81, J103, J127, J135, M50, M142 15 88 – 1023 J5, J32, J36, J59, J63, J65, J66, J77, J78, J79, J86, J108, J120, J129, P58, M163 16 70 – 874 J14, J33, J71, J93, J99, J106, J110, J121, J122, P19, P21, 11 61 – 715 J15, J20, J39, J74, J85, J116, P12, P27, P103, 9 52 – 606 J29, J51, J67, J82, J92, J100, J112, B1, 8 44 – 517 J19, J31, J60, J125, 4 40 – 438 J3, P37, 2 38 – 399 J25, J37, J53, J101, 4 34 – 3710 J32a, J104, J117, P105, 4 30 – 3311 J24, J62, J115, P4, B2, 5 25 – 2912 J91, J109, 2 23-2413 J34, J80, 2 21 – 2214 J97, P3, 2 19 – 201516 J23, J28, J94, J96, P96, 5 14 – 181718 P65, J95, 2 12-131920 J57 1 112122 P77, 1 1023 P79 1 924 J90, 1 82526 J48 1 727 P41 1 6282930313233 J11 1 5343536 J87 1 437383940 J46 1 3414243444546474849123

12450515253545556 J102 1 257585960616263646566676869707172737475767778798081828384858687888990919293949596979899100101102103104105106107

108109110111112 J84 1 1The h-index is the number of papers, for which at least the same number of independent citations is obtained. Asfollows from the table above, my current h-index is: h = 16 (see papers J84 – J102 – J46 – J87 - J11 – P41 – J48– J90 – P79 – P77 – J57 – P65 – J95 – J23 – J28 – J94 – J96 - P96).125

Papers with impact factors (IF, according to ISI values)No Year Journal IF SUM (IF) Authors(n)IF/n SUM(I/n)SUM(IF/n)/SUM(IF)1 J14 1991 Chemical Papers 0.150 0.150 2 0.075 0.075 0.5002 J26 1996 J. of Non-Cryst. Sol. 1.318 1.468 6 0.220 0.295 0.2013 J27 1997 Mat Sci & Eng A 0.842 2.310 5 0.168 0.463 0.2004 J30 1997 Russ. J.Appl.Chem. 0.114 2.424 5 0.023 0.486 0.2005 J31 1998 Russ. J. Appl. Chem. 0.169 2.593 4 0.042 0.528 0.2046 J35 1998 Elektrokhimiia 0.059 2.652 5 0.012 0.540 0.2047 J32 1998 High Temp.Mat.Proc. 0.233 2.885 4 0.058 0.598 0.2078 J39 1999 Metall. Mater. Trans.A 0.993 3.878 1 1.061 1.659 0.4289 J45 1999 High Temp Mater Proc 0.345 4.223 3 0.115 1.774 0.42010 J47 2000 Mater. Sci. Forum 0.597 4.820 1 0.597 2.371 0.49211 J48 2000 Mater.Sci.Forum 0.597 5.417 3 0.199 2.570 0.47412 J49 2000 Mater.Sci.Forum 0.597 6.014 3 0.199 2.769 0.46013 J51 2000 Metall. Mater. Trans.A 1.361 7.375 1 1.361 4.130 0.56014 J53 2000 J. of Solid State Chem 1.527 8.902 2 0.764 4.894 0.55015 J56 2001 ISIJ International 0.980 9.882 2 0.490 5.384 0.54516 J57 2001 Metall. Mater. Trans. A 1.273 11.155 1 1.273 6.657 0.59717 J59 2001 Metall. Mater. Trans. B 0.754 11.909 1 0.754 7.411 0.62218 J60 2001 Appl. Phys. A 1.722 13.631 7 0.330 7.741 0.56819 J68 2001 Z.Naturforsch. A 0.746 14.377 4 0.187 7.928 0.55120 J70 2002 Russ. J. Applied Chem. 0.221 14.598 2 0.111 8.039 0.55121 J71 2002 Metall.Mater.Trans.A. 1.219 15.817 1 1.219 9.258 0.58522 J74 2003 Mater Science Forum 0.602 16.419 3 0.201 9.459 0.57623 J75 2003 Mater Science Forum 0.602 17.021 1 0.602 10.061 0.59124 J76 2003 Mater Science Forum 0.602 17.623 2 0.301 10.362 0.58825 J77 2003 Mater Science Forum 0.602 18.225 2 0.301 10.663 0.58526 J78 2003 Mater Science Forum 0.602 18.827 3 0.201 10.864 0.57727 J79 2003 Mater Science Forum 0.602 19.429 3 0.301 11.165 0.57528 J80 2003 J Chem Inf Comput Sci 3.078 22.507 8 0.385 11.550 0.51329 J84 2004 Colloids and Surfaces A 1.513 24.02 1 1.513 13.063 0.54430 J85 2004 Metall. Mater. Trans. B 0.839 24.859 1 0.839 13.902 0.55931 J86 2004 Metall.Mater.Trans. B 0.839 25.698 4 0.210 14.112 0.54932 J87 2004 Calphad 2.119 27.817 1 2.119 16.231 0.58333 J88 2005 Mater. Sci. Forum 0.399 28.216 4 0.100 16.331 0.57934 J89 2005 Mater. Sci. Forum 0.399 28.615 3 0.133 16.464 0.57535 J90 2005 Mater. Sci. Forum 0.399 29.014 2 0.200 16.664 0.57436 J91 2005 Mater. Sci. Forum 0.399 29,413 3 0.133 16.797 0.57137 J92 2005 Mater. Sci. Forum 0.399 29.812 2 0.200 16.997 0.57038 J93 2005 Mater. Sci. Forum 0.399 30.211 4 0.100 17.097 0.56639 J94 2005 Mater. Sci. Forum 0.399 30.61 1 0.399 17.496 0.57240 J95 2005 Z. Metallkunde 0.842 31.452 1 0.842 18.338 0.58341 J96 2005 J. Mater. Sci. 0.901 32.353 1 0.901 19.239 0.59542 J97 2005 J. Mater. Sci. 0.901 33.254 2 0.450 19.689 0.59243 J99 2005 Calphad 1.344 34.598 1 1.344 21.033 0.60844 J100 2005 Russian J Electrochem 0.218 34.816 4 0.055 21.088 0.60645 J102 2006 Colloids Surfaces A 1.611 36.427 1 1.611 22.699 0.62346 J106 2007 Fluid Phase Equilibria 1.506 37.933 4 0.377 23.076 0.60747 J108 2007 Fluid Phase Equlibria 1.506 39.439 4 0.377 23.453 0.59248 J109 2008 Composite Sci Technol 2.533 41.972 1 2.533 25.986 0.61949 J110 2008 Int J Mater Res 0.819 42.791 1 0.819 26.805 0.62650 J111 2008 Metall Mater Trans B 0.798 43.589 1 0.798 27.603 0.63351 J112 2008 Calphad 1.530 45.119 1 1.530 29.133 0.64652 J115 2008 Mater Sci Eng A 1.806 46.925 1 1.806 30.939 0.65953 J116 2008 Mater Sci Eng A 1.806 48.731 2 0.903 31.842 0.653126

54 J117 2008 Mater Sci Eng A 1.806 50.537 2 0.903 32.745 0.64855 J120 2009 Carbon 4.504 55.041 5 0.901 33.646 0.61156 J121 2009 Metall Mater Trans A 1.564 56.605 2 0.782 34.428 0.60857 J122 2009 Surf Coat Technol 1.793 58.398 5 0.359 34.787 0.59658 J124 2011 Surface Engineering* 0.633 59.031 5 0.127 34.914 0.59359 J125 2009 Electrochimica Acta 3,325 62.345 2 1,663 36,577 0,58860 J127 2010 J Mater Sci 1,859 64,215 2 0,930 37,507 0,58561 J128 2010 Univ Polit Buchar Sci 0.253 64.468 5 0.051 37.558 0.58362 J129 2010 J Mater Sci 1,859 66.327 3 0,620 38,178 0,57863 J132 2010 J Nanosci Nanotechn 1.352 67,679 1 1,352 39,530 0,58764 J134 2011 Intermetallics 1.649 69,328 2 0,825 40,355 0,58265 J135 2011 J Mater Proc Technol 1,783 71,111 8 0,223 40,578 0,57166 J136 2011 Coll Surf A 2,236 73,347 3 0,745 41,323 0,56367 J137 2011 Metal Mater Trans A 1,545 74,892 3 0,515 41,838 0,55968 J138 2011 JMM B 1,317 76,209 1 1,317 43,155 0,56669 J140 2012 Metal Mater Trans A* 1,545 77,754 1 1,545 44,700 0,57570 J141 2012 Thermochimica Acta* 1,805 79,559 5 0,361 45,061 0,56671 J142 2012 Electrochimica Acta* 3,832 83.391 1 3,832 48,893 0,58672 J143 2012 Adv Coll Interface Sci* 8,120 91,511 1 8,120 57,013 0,62373 J144 2012 J Disp Sci Technol* 0.560 92,071 1 0.560 57,573 0.62774 J145 2012 JMM B* 1.317 93,388 1 1.317 58,890 0.63175 J146 2012 J Nanosci Nanotech* 1.563 94,951 1 1.563 60,453 0.63776 J147 2012 Mat.-wiss. Werkstoff. * 0.543 95,494 3 0.181 60,634 0.63577 J148 2012 Int J Pharma* 3.350 98,844 1 3.350 63.984 0.64778 J149 2012 Intermetallics* 1.649 100,493 3 0.550 64.534 0.64279 J150 2012 J Nanosci Nanotech* 1.563 102.056 8 0.195 64.729 0.63480 J151 2012 J Alloys Compds* 2.289 104.345 4 0.572 65,301 0.62681 J153 2012 J Mater Sci* 2.015 106.360 1 2.015 67.316 0.63382 J154 2012 Metal Mater Trans A* 1.545 107.905 4 0.386 67.702 0.62783 J155 2012 Int J Thermophysics* 0.953 108.858 1 0.953 68.655 0.63184 J156 2012 Composites A* 2.695 111.553 5 0.539 69.194 0.62085 J157 2012 Acta Mater* 3.755 115.308 1 3.755 72.949 0.633* IF of 2011127