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Understanding Neutron Radiography Post Exam Reading VIII-Part 1 of 2A

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<strong>Understanding</strong> <strong>Neutron</strong> <strong>Radiography</strong><br />

<strong>Reading</strong> <strong>VIII</strong> <strong>Part</strong> 1 <strong>of</strong> 2<br />

13 th 2016 August<br />

<strong>Post</strong> <strong>Exam</strong> <strong>Reading</strong><br />

Charlie Chong/ Fion Zhang


Reactor<br />

Charlie Chong/ Fion Zhang


Reactor<br />

Charlie Chong/ Fion Zhang


The Magical Book <strong>of</strong> <strong>Neutron</strong> <strong>Radiography</strong><br />

Charlie Chong/ Fion Zhang


Charlie Chong/ Fion Zhang


ASNT Certification Guide<br />

NDT Level III / PdM Level III<br />

NR - <strong>Neutron</strong> Radiographic Testing<br />

Length: 4 hours Questions: 135<br />

1. Principles/Theory<br />

• Nature <strong>of</strong> penetrating radiation<br />

• Interaction between penetrating radiation and matter<br />

• <strong>Neutron</strong> radiography imaging<br />

• Radiometry<br />

2. Equipment/Materials<br />

• Sources <strong>of</strong> neutrons<br />

• Radiation detectors<br />

• Non-imaging devices<br />

Charlie Chong/ Fion Zhang


3. Techniques/Calibrations<br />

• Blocking and filtering<br />

• Multifilm technique<br />

• Enlargement and projection<br />

• Stereoradiography<br />

• Triangulation methods<br />

• Autoradiography<br />

• Flash <strong>Radiography</strong><br />

• In-motion radiography<br />

• Fluoroscopy<br />

• Electron emission radiography<br />

• Micro-radiography<br />

• Laminography (tomography)<br />

• Control <strong>of</strong> diffraction effects<br />

• Panoramic exposures<br />

•Gaging<br />

• Real time imaging<br />

• Image analysis techniques<br />

Charlie Chong/ Fion Zhang


4. Interpretation/Evaluation<br />

• Image-object relationships<br />

• Material considerations<br />

• Codes, standards, and specifications<br />

5. Procedures<br />

• Imaging considerations<br />

• Film processing<br />

• Viewing <strong>of</strong> radiographs<br />

• Judging radiographic quality<br />

6. Safety and Health<br />

• Exposure hazards<br />

• Methods <strong>of</strong> controlling radiation exposure<br />

• Operation and emergency procedures<br />

Reference Catalog Number<br />

NDT Handbook, Third Edition: Volume 4,<br />

Radiographic Testing 144<br />

ASM Handbook Vol. 17, NDE and QC 105<br />

Charlie Chong/ Fion Zhang


Charlie Chong/ Fion Zhang<br />

Fion Zhang at Copenhagen Harbor<br />

4 th August 2016


Charlie Chong/ Fion Zhang<br />

SME- Subject Matter Expert<br />

http://cn.bing.com/videos/search?q=Walter+Lewin&FORM=HDRSC3<br />

https://www.youtube.com/channel/UCiEHVhv0SBMpP75JbzJShqw


Gamma- <strong>Radiography</strong><br />

TABLE 1. Characteristics <strong>of</strong> three isotope sources commonly used for<br />

radiography.<br />

Source<br />

T½<br />

Energy<br />

HVL<br />

HVL<br />

Specific<br />

Dose rate*<br />

Pb<br />

Fe<br />

Activity<br />

Co60<br />

5.3 year<br />

1.17, 1.33 MeV<br />

12.5mm<br />

22.1mm<br />

50 Cig -1<br />

1.37011<br />

Cs137<br />

30 years<br />

0.66 MeV<br />

6.4mm<br />

17.2mm<br />

25 Cig -1<br />

0.38184<br />

Ir192<br />

75 days<br />

0.14 ~ 1.2 MeV<br />

4.8mm<br />

?<br />

350 Cig -1<br />

0.59163<br />

(Aver. 0.34 MeV)<br />

Th232<br />

0.068376<br />

Dose rate* Rem/hr at one meter per curie<br />

Charlie Chong/ Fion Zhang


八 千 里 路 云 和 月<br />

Charlie Chong/ Fion Zhang


Charlie Chong/ Fion Zhang


闭 门 练 功<br />

Charlie Chong/ Fion Zhang


Charlie Chong/ Fion Zhang<br />

http://greekhouse<strong>of</strong>fonts.com/


Charlie Chong/ Fion Zhang


COLLIMATED NEUTRON BEAM FOR<br />

NEUTRON RADIOGRAPHY<br />

M. DINCA1, M. PAVELESCU2, C. IORGULIS1<br />

1 Institute for Nuclear Research, P.O. Box 078, Pitesti, Romania, dinca@scn.ro<br />

2 Romanian Scientist Academy, Bucharest, Romania, mpavelescu@pcnet.ro<br />

Received October 21, 2005<br />

Charlie Chong/ Fion Zhang


Pitești<br />

Charlie Chong/ Fion Zhang


The obtaining <strong>of</strong> a collimated neutron beam on the tangential channel <strong>of</strong> the<br />

ACPR reactor from INR Pitesti that to satisfy the requests <strong>of</strong> a neutron<br />

radiography facility it is presented. The collimation <strong>of</strong> neutrons means the<br />

elimination from the neutron beam <strong>of</strong> those neutrons that have trajectories<br />

that are not inside the space defined by walls or successive apertures that are<br />

made <strong>of</strong> neutron absorbent materials. The assembly that assures the<br />

collimation <strong>of</strong> neutrons, named collimator, is optimized using MCNP 4B code<br />

based on Monte Carlo method for neutrons and gamma radiation.<br />

Key words: neutron radiography, collimator for neutrons, collimation ratio,<br />

MCNP 4B code.<br />

Charlie Chong/ Fion Zhang


1. INTRODUCTION<br />

A tangential channel <strong>of</strong> a nuclear reactor has some peculiarities regarding<br />

intensity and energetic spectrum <strong>of</strong> neutrons in comparison with a radial<br />

channel <strong>of</strong> a nuclear reactor or tubes used to extract neutrons from other<br />

neutron sources.<br />

On a tangential channel the neutron beam has a bigger cadmium ratio and a<br />

lower gamma contamination than on a radial channel and is more suited to be<br />

used for thermal neutron radiography. For neutron radiography, different <strong>of</strong><br />

other nuclear physics applications that use neutron beams, are necessary<br />

large neutron beams to obtain images <strong>of</strong> a large area <strong>of</strong> the investigated<br />

objects. An ideal neutron beam should be parallel, monoenergetic, with big<br />

intensity, free <strong>of</strong> other contaminant radiation and uniform on its cross section.<br />

In practice it is intended to have experimental arrangements that to<br />

accomplish neutron beam parameters as closely as possible to ideal ones.<br />

Charlie Chong/ Fion Zhang


For this purpose it is used a collimator. The neutrons pass through a<br />

collimator from the entrance aperture placed nearby neutron source to the<br />

exit window where are used for neutron radiography investigations. The inner<br />

space <strong>of</strong> a collimator is evacuated or filled with air, or better filled with helium.<br />

A characteristic parameter <strong>of</strong> a collimator that defines the degree <strong>of</strong><br />

divergence <strong>of</strong> the neutron beam is the L/D ratio, where L is the length <strong>of</strong> the<br />

collimator and D is the diameter (or generally the opening) <strong>of</strong> the entrance<br />

aperture.<br />

Charlie Chong/ Fion Zhang


The place from where thermal neutrons start (the source <strong>of</strong> neutrons) is a<br />

moderator that contains neutrons moving in all directions. In order to have a<br />

neutron beam on a direction, nearby the moderator it is placed a collimator.<br />

The neutrons entering in the collimator must have the direction <strong>of</strong> the exit<br />

window to be useful otherwise they are captured by walls or apertures to<br />

avoid the scattering. The entrance aperture must be big enough to permit a<br />

larger number <strong>of</strong> neutrons to go inside the collimator but small enough to<br />

have a bigger L/D ratio. The L/D ratio depends also by the length <strong>of</strong> the<br />

collimator (or otherwise by the distance from entrance aperture to object<br />

plane if the object is put far away from collimator), a bigger L means a better<br />

resolution.<br />

Charlie Chong/ Fion Zhang


Because the moderator emits neutrons in all directions, their intensity is<br />

proportionally with 1/r 2 . To have a bigger intensity the object must be placed<br />

closer to neutron source but for a better geometrical resolution it must be<br />

placed farther. Bigger neutron intensity determines a better statistics,<br />

therefore a bigger contrast <strong>of</strong> the image that is able to differentiate between<br />

different materials. But for dimensional measurements it is necessary to have<br />

precise separation lines, therefore a big geometrical resolution.<br />

A compromise must be made between the two parameters, L and D. A<br />

transmission method for neutron radiography it is involved because are<br />

detected the neutrons that pass through investigated object. If the neutrons<br />

come to investigated object more scattered, then the projection <strong>of</strong> a detail is<br />

larger in the plane <strong>of</strong> the detector and the geometrical resolution <strong>of</strong> the image<br />

is poorer.<br />

Charlie Chong/ Fion Zhang


There are known different types <strong>of</strong> collimators, more important are:<br />

■ pin-hole,<br />

■ Soller and<br />

■ divergent collimators.<br />

Charlie Chong/ Fion Zhang


Soller Collimator<br />

Charlie Chong/ Fion Zhang


Sóller Collimator<br />

Charlie Chong/ Fion Zhang<br />

http://pd.chem.ucl.ac.uk/pdnn/inst3/soller.htm


The photograph shows the front opening <strong>of</strong> the 10′ Soller collimators <strong>of</strong> the<br />

detector bank <strong>of</strong> D1A taken before its rebuild in the late 1990's. The<br />

protective shielding has been removed so that thin vertical mylar sheets<br />

covered in a white gadolinium oxide paint are visible. The ones shown here<br />

were designed to collimate neutrons to 10 arc minutes (0.17°). (The little hole<br />

seen on the detector bank was a large "pin-hole" collimator, positioned in<br />

front <strong>of</strong> the normally unused 11th detector.)<br />

The Soller collimators designed for use on neutron diffractometers have large<br />

dimensions as illustrated by the figure below for 5′ collimation. The figure<br />

shows just two foils, but in practice many parallel foils are required since the<br />

diameter <strong>of</strong> the detectors is 2 to 5 cm.<br />

Charlie Chong/ Fion Zhang<br />

http://pd.chem.ucl.ac.uk/pdnn/inst3/soller.htm


The town <strong>of</strong> Sóller in the northwest <strong>of</strong> Mallorca became wealthy because <strong>of</strong><br />

the valley’s abundant citrus groves. In the 19th century, when the area was<br />

isolated from the rest <strong>of</strong> Mallorca by mountains, the oranges were shipped to<br />

France from the nearby west coast Port de Sóller (or Puerto de Sóller). Many<br />

locals went to work in France and returned – their fortunes duly made – to<br />

build some <strong>of</strong> the handsome Modernista properties that grace this town today.<br />

Charlie Chong/ Fion Zhang


The pin-hole collimator<br />

The pin-hole collimator has a simple construction. An aperture is placed at a<br />

distance from neutron source in order to establish a L/D ratio <strong>of</strong> the collimator.<br />

For a pin-hole collimator it is necessary a large neutron source that to have<br />

an equal neutron flux on its surface in order to expose uniformly the object to<br />

neutrons.<br />

The Soller collimators<br />

At Soller collimators appear on image the network <strong>of</strong> absorber walls that<br />

delimits inner minicollimators. This type <strong>of</strong> collimator requires a large uniform<br />

neutron source.<br />

The divergent collimator<br />

The most used is the divergent collimator because it permits the investigation<br />

<strong>of</strong> large objects, every point <strong>of</strong> the object being exposed to a neutron beam<br />

with approximately the same L/D (this means an intrinsic geometrical<br />

resolution uniform in the exit window <strong>of</strong> the collimator). A divergence<br />

collimator has the neutron source in its entrance aperture.<br />

Charlie Chong/ Fion Zhang


Based on dimensional constrains <strong>of</strong> the tangential channel <strong>of</strong> ACPR, previous<br />

experimental determinations <strong>of</strong> the thermal neutron flux and intensity<br />

(8 ⋅ 10 11 n/cm 2 /s near core and 1.12 x 10 6 n/cm2/s at the exit <strong>of</strong> tangential<br />

beam tube, at 100 kW operating power <strong>of</strong> ACPR) and working methods<br />

involved, were established the parameters <strong>of</strong> the divergent thermal neutron<br />

beam. Some <strong>of</strong> them are:<br />

Charlie Chong/ Fion Zhang


• the thermal neutron beam intensity at least 5 ⋅105 n/cm2/s;<br />

• the collimation ratio, L/D, at least 90;<br />

• the exit window, 250 mm in diameter;<br />

• the n/γ ratio at least 1⋅10 6 n/cm 2 /mrem (that determines used<br />

investigation methods);<br />

• the divergent angle under 40°;<br />

• the cadmium ratio above 17.<br />

Note: Cadmium Ratio<br />

The ratio <strong>of</strong> the response <strong>of</strong> an uncovered neutron detector to that <strong>of</strong> the<br />

same detector under identical conditions when it is covered with cadmium <strong>of</strong><br />

a specified thickness.<br />

Hint: the larger the cadmium ratio, the more the thermal neutron with energy<br />

less than 0.5Mev?<br />

Charlie Chong/ Fion Zhang


To obtain a thermal neutron beam with such parameters were used:<br />

1. a graphite illuminator placed on channel nearby reactor core to scatter<br />

neutrons towards exit <strong>of</strong> the channel;<br />

2. a mobile monocrystaline bismuth filter for the attenuation <strong>of</strong> the gamma<br />

radiationand scattering <strong>of</strong> fast neutrons that will allow performing direct<br />

neutron radiography investigations and also γ radiography investigations;<br />

3. a set <strong>of</strong> successive apertures from boron, indium and lead for the<br />

formation <strong>of</strong> the divergent collimator.<br />

Charlie Chong/ Fion Zhang


The position and dimensions <strong>of</strong> these components were optimized by<br />

calculus made with MCNP 4B code based on Monte Carlo method both for<br />

thermal neutrons and both for gamma radiation.<br />

Charlie Chong/ Fion Zhang


ACPR- Annular Core Pulse Reactor<br />

Charlie Chong/ Fion Zhang


Charlie Chong/ Fion Zhang


2. CALCULUS WITH WIMS 4D AND MCNP 4B CODES<br />

The tangential beam port has an overall length <strong>of</strong> 5644 mm (Figure 1) and<br />

has two sections. First with the length <strong>of</strong> about 2984 mm and the diameter <strong>of</strong><br />

219 x 6.5 mm, and second with the length <strong>of</strong> about 2660 mm and the<br />

diameter <strong>of</strong> 273 x 6.5 mm.<br />

2660 mm<br />

Charlie Chong/ Fion Zhang


The distance between the center <strong>of</strong> the reactor and the beam port axis is 575<br />

mm. The beam port exceeds with 508 mm, to the axis <strong>of</strong> the pool, the<br />

perpendicular right line on its own axis that passes through the center <strong>of</strong> the<br />

core. The beam port contains a mobile lead shutter with the thickness <strong>of</strong> 381<br />

mm and 406 mm in diameter placed at 1015 mm from beam port exit.<br />

Between the edge <strong>of</strong> the core and the tangential beam port is a distance <strong>of</strong><br />

157.8 mm. The space between core and beam port is filled with regular<br />

demineralised water. A better transmission <strong>of</strong> the neutrons from core to<br />

channel will be assured placing aluminum in free locations <strong>of</strong> the reactor grid.<br />

In this way the reduction <strong>of</strong> the initial thermal neutron flux <strong>of</strong> the channel<br />

through divergent collimator construction is compensated. (?)<br />

mobile lead shutter<br />

Charlie Chong/ Fion Zhang


Fig. 1. Sketch <strong>of</strong> the collimator <strong>of</strong> the neutron radiography facility at the<br />

tangential beam port <strong>of</strong> the ACPR.<br />

Charlie Chong/ Fion Zhang


The optimization <strong>of</strong> the transmission <strong>of</strong> neutrons to channel and the<br />

optimization <strong>of</strong> the dimensions and positions <strong>of</strong> the collimator components is<br />

done using WIMS D4 and MCNP 4B codes. To establish the spectrum <strong>of</strong> the<br />

neutron flux at the edge <strong>of</strong> the ACPR reactor, the transport program WIMS D4<br />

was involved. Because <strong>of</strong> cylindrical shape <strong>of</strong> the reactor, it is suitable to be<br />

modeled by WIMS program. The model consists <strong>of</strong> cylindrical rings that cover<br />

the central hole, ACPR fuel, water etc. The neutron flux calculated for 69<br />

broad groups in a thin volume at the edge <strong>of</strong> the core has been collapsed in 3<br />

or 23 groups. Their weights, after the renormalization to unit and upper<br />

boundaries for energy groups were used in the inputs <strong>of</strong> the MCNPprogram.<br />

The WIMS D4 code was used to study the effect <strong>of</strong> the replacement <strong>of</strong> the<br />

water between core and beam port with an aluminum block, aluminum pins<br />

placed in grid’s holes or air in aluminum box. The replacement <strong>of</strong> the water<br />

leads to an improvement <strong>of</strong> the transfer <strong>of</strong> the neutrons towards beam port.<br />

The results <strong>of</strong> the calculations are shown in Table 1. It can be seen that the<br />

increase <strong>of</strong> the thermal neutron flux is maximum using a box filled with air. To<br />

disturb not other experiments for irradiation tests, a bell box is put in place<br />

from where the water is pushed out and replaced by air.<br />

Charlie Chong/ Fion Zhang


Table 1: Relative units <strong>of</strong> the thermal flux in the graphite illuminator for some<br />

materials between core and tangential beam port<br />

Water Aluminum pins Aluminum block<br />

Air<br />

4.92 14.3 16 19.5<br />

Charlie Chong/ Fion Zhang


In order to assure a maximum thermal neutron beam at the exit <strong>of</strong> the<br />

collimator and a suitable established collimation ratio were performed Monte<br />

Carlo calculation based on MCNP code. Two models were prepared for<br />

Monte Carlo calculations. The first model aimed to establish the thickness<br />

and position <strong>of</strong> the graphite illuminator for the maximum increase <strong>of</strong> the<br />

thermal neutron beam at the exit <strong>of</strong> the collimator. This model contains the<br />

source <strong>of</strong> neutrons <strong>of</strong>fered by WIMS code for 3 and 23 groups, the box with<br />

air and the illuminator placed on beam port. The relative values obtained in a<br />

plane at 100 cm from illuminator, for different thicknesses <strong>of</strong> the illuminator<br />

are shown in Figure 2. The illuminator is placed near centerline. If the<br />

illuminator is placed in a centered position the thermal neutron flux is a little<br />

improved, but epithermal and fast neutrons increase more and it is not<br />

desirable. The maximum neutron beam is obtained for 6.5 cm and 7 cm<br />

illuminator thicknesses.<br />

Charlie Chong/ Fion Zhang


Fig. 2. <strong>Neutron</strong> beam intensity.<br />

Charlie Chong/ Fion Zhang


The second model targeted to establish the position and thickness <strong>of</strong> the<br />

single-crystal Bi filter, to obtain the maximum thermal neutron beam at the<br />

exit <strong>of</strong> the collimator. This model is based on the geometry <strong>of</strong> the collimator<br />

shown in Figure 1 and the source <strong>of</strong> neutrons is placed on the face <strong>of</strong> the<br />

illuminator. We consider the maximization <strong>of</strong> neutron flux below 1.E-06 MeV.<br />

On the geometry <strong>of</strong> the second model calculations were done for gamma<br />

radiation also. Based on previous flux measurements and the results<br />

estimated from first MCNP model, it was established a value <strong>of</strong> 4.5 cm for the<br />

diameter <strong>of</strong> the collimator main aperture. Preliminary results obtained with the<br />

second model established a value <strong>of</strong> 3 cm for the thickness <strong>of</strong> the Bi singlerystal.<br />

The main aperture will be built by 13 mm <strong>of</strong> boral, 1 mm indium and<br />

200 mm lead.<br />

Charlie Chong/ Fion Zhang


To optimize the position <strong>of</strong> the aperture and Bi filter, MCNP calculation were<br />

done for different positions <strong>of</strong> the filter. The results are shown in Figure 3.<br />

Supplementary, it was used the condition to have a uniform intensity <strong>of</strong> the<br />

neutron beam in the exit window <strong>of</strong> the collimator. This was precisely<br />

established with AutoCAD program that drawn the extreme lines <strong>of</strong> the<br />

neutron beam. In this way every point in the exit window is seen by the same<br />

area from the surface <strong>of</strong> the illuminator. In these conditions it was established<br />

the maximum distance between illuminator and aperture to be 152.5 cm,<br />

although the maximum <strong>of</strong> the neutron beam is obtained for the distance <strong>of</strong><br />

190-200 mm. The calculations for the distance <strong>of</strong> 152.5 cm, the main aperture<br />

<strong>of</strong> 4.5 cm and 3 cm <strong>of</strong> Bi indicates a decrease <strong>of</strong> the gamma radiation <strong>of</strong><br />

65.19 times, and for neutrons <strong>of</strong> 16.15 times (the Bi filter itself decreases the<br />

beam intensities 8.22 and 2.22 times, respectively). The calculations with<br />

MCNP code were done with polycrystalline Bi. In the real case, for<br />

singlecrystal Bi with cross-section 3 times smaller at room temperature [1], it<br />

is expected a reduction <strong>of</strong> the beam intensity with 41% instead <strong>of</strong> 2.22 times<br />

reduction.<br />

Charlie Chong/ Fion Zhang


Fig. 3. Intensity <strong>of</strong> the thermal neutron beam at the exit <strong>of</strong> the collimator.<br />

Charlie Chong/ Fion Zhang


The minimum distance between illuminator and main aperture is considered<br />

to be 125 cm. For this distance the intensity <strong>of</strong> neutron beam decreases with<br />

17%, but the resolution increases. The lead ring (20 cm) should be positioned<br />

at less 125 cm were is the edge <strong>of</strong> the concrete wall <strong>of</strong> the pool, otherwise the<br />

direct gamma radiation from reactor core cannot be properly stopped. The<br />

secondary apertures are positioned to avoid any trajectory <strong>of</strong> the neutron<br />

directly from illuminator to reach the wall <strong>of</strong> the beam tube. The secondary<br />

apertures are boral plates and lead rings. To increase the neutron beam for<br />

the direct method and to perform gamma radiographs it is designed to<br />

remove vertically the Bi filter with the help <strong>of</strong> a steel cable. The Bi filter is<br />

inside <strong>of</strong> a box, which contains lead ballast to fall back on position when cable<br />

is released.<br />

Charlie Chong/ Fion Zhang


3. CONCLUSIONS<br />

The collimation <strong>of</strong> the neutrons on the tangential beam port <strong>of</strong> the ACPR<br />

reactor is done, in fact, with a pin-hole collimator with an aperture <strong>of</strong> 45 mm<br />

placed at the distance <strong>of</strong> 125-152.5 cm from the surface <strong>of</strong> the illuminator that<br />

has a thickness <strong>of</strong> 6.5 cm and the diameter <strong>of</strong> 18 cm. The estimated beam<br />

intensity for thermal neutrons with bismuth filter is 3.96⋅105 – 4.65⋅10 5 n/cm 2 /s<br />

and 4.85⋅105 – 5.70⋅10 5 n/cm 2 /s without Bi filter. The estimated values for<br />

gamma debit doses (for 152.5 cm illuminator-main aperture distance) are<br />

1.75 rem/h without bismuth and 213 mrem/h with bismuth. The estimated<br />

n/gamma ratio is 1.03⋅10 6 n/cm2/mrem and 8.44⋅10 6 n/cm 2 /mrem,<br />

respectively. The divergent angle <strong>of</strong> the collimator is 3 o -3.3 o and the<br />

collimation ratio 100-92.8 for the domain <strong>of</strong> distances 125-152.5 cm<br />

betweenilluminator and main aperture. These values <strong>of</strong> beam intensity,<br />

n/gamma ratio and collimation ratio are in concordance with that from other<br />

facilities built at TRIGA reactors and <strong>of</strong>fer the base to use with good results<br />

the direct and the transfer methods for neutron radiography.<br />

Charlie Chong/ Fion Zhang


Sandia’s Annular Core Research Reactor<br />

conducts 10,000th operation<br />

Charlie Chong/ Fion Zhang<br />

https://share.sandia.gov/news/resources/news_releases/acrr/#.V65mc-Qkpdg


ACPR- Annular Core Pulse Reactor<br />

Charlie Chong/ Fion Zhang


ACRR- Annular Core (Pulse) Research Reactor<br />

Charlie Chong/ Fion Zhang<br />

https://share.sandia.gov/news/resources/news_releases/acrr/


ACRR- Annular Core (Pulse) Research Reactor<br />

Charlie Chong/ Fion Zhang<br />

https://share.sandia.gov/news/resources/news_releases/acrr/


ALBUQUERQUE, N.M. – With a muffled “pop,” a flash <strong>of</strong> blue light and a few<br />

ripples through 14,000 gallons <strong>of</strong> deionized water, Sandia National<br />

Laboratories’ Annular Core Research Reactor (ACRR) recently conducted its<br />

10,000th operation.<br />

“The ACRR has been a real workhorse for Sandia, and labs leadership and<br />

the nation rely on these experiments and other weapons component testing<br />

done at Sandia to support certification <strong>of</strong> the nuclear weapon stockpile,” said<br />

Lonnie Martin, an ACRR operator.<br />

In its 32-year history, the ACRR time and again has proved itself a valuable<br />

resource for a wide variety <strong>of</strong> experiments in nearly every branch <strong>of</strong> nuclear<br />

science, especially the testing <strong>of</strong> radiation-hardened electronic components.<br />

With a dry, 9-inch diameter cavity in the core’s center, and a 20-inch diameter<br />

external cavity, the ACRR subjects electronics to high-intensity neutron<br />

irradiation and conducts reactor safety research. The ACRR also has done<br />

testing for semiconductor manufacturers, NASA, the Large Hadron Collider in<br />

Switzerland and dozens <strong>of</strong> other users.<br />

Charlie Chong/ Fion Zhang


Sandia’s ACRR is a water-moderated, pool-type research reactor capable <strong>of</strong><br />

steady-state, pulsed and tailored transient operations and, in the past, has<br />

been configured for medical isotope production. Other duties for ACRR<br />

include: reactor-driven laser experiments; space reactor fuels development;<br />

pulse reactor kinetics; reactor heat transfer and fluid flow; electronic<br />

component hardening; and explosive component testing. It is also routinely<br />

used for education and training programs.<br />

Charlie Chong/ Fion Zhang


At peak power in its steady state mode, the ACRR produces up to four<br />

megawatts <strong>of</strong> power. But during a maximum pulse, it generates a whopping<br />

35,000 megawatts <strong>of</strong> power for seven milliseconds. Nuclear engineer and<br />

former University <strong>of</strong> New Mexico pr<strong>of</strong>essor Ron Knief compares its power<br />

output to that <strong>of</strong> the Palo Verde Nuclear Generating Station, outside <strong>of</strong><br />

Phoenix. “For that very short time, we produce three times more power than<br />

the nation’s largest nuclear power station. They have three big reactors, and<br />

yet, for a fraction <strong>of</strong> a second, we produce three times more power than they<br />

do,” Knief said.<br />

Charlie Chong/ Fion Zhang


The ACRR is a descendent <strong>of</strong> the Sandia Annular Core Pulse Reactor<br />

(ACPR), which was replaced in 1978 and is part <strong>of</strong> a large family <strong>of</strong> Training,<br />

Research Isotope Production, General Atomics (TRIGA) reactors. The TRIGA<br />

concept is credited to Manhattan Project physicist Edward Teller and a group<br />

<strong>of</strong> distinguished scientists who assembled the first model in a “Little Red<br />

Schoolhouse” in San Diego in 1956. Teller’s mandate to the team was to<br />

“design a reactor so safe … that if it was started from its shut-down condition<br />

and all its control rods instantaneously removed, it would settle down to a<br />

steady level <strong>of</strong> operation without melting any <strong>of</strong> its fuel,” according to<br />

Freeman Dyson’s, “Disturbing the Universe.” Essentially, even if all the<br />

engineered safety mechanisms failed, the reactor would operate safely,<br />

based on the laws <strong>of</strong> physics.<br />

In 1978, the original ACPR TRIGA fuel was replaced with a new ACRR<br />

ceramic-metal, uranium dioxide/beryllium oxide (UO2/BeO) fuel, which is<br />

designed to allow steady state and pulsed operation at fuel temperatures up<br />

to 2,552 degrees (1,400 degrees C). The reactor underwent extensive<br />

upgrades in 2002, including upgrades to reactivity control circuitry.<br />

Charlie Chong/ Fion Zhang


Key!<br />

Charlie Chong/ Fion Zhang


Charlie Chong/ Fion Zhang


Reactor<br />

Charlie Chong/ Fion Zhang


Reactor<br />

Charlie Chong/ Fion Zhang


<strong>Radiography</strong> may be considered the most effective nondestructive testing<br />

method merely because <strong>of</strong> its universal use and acceptance in industry.<br />

<strong>Radiography</strong> can be used to test most types <strong>of</strong> solid material. Exceptions<br />

include materials <strong>of</strong> very high or very low density. <strong>Neutron</strong> radiography,<br />

however, can <strong>of</strong>ten be used in such cases. There is wide latitude both <strong>of</strong><br />

material thickness that can be tested and in the techniques that can be used.<br />

Usually conditions that result in a two percent or greater difference in<br />

through- section thickness can usually be detected. (≥2% subject sensitivity)<br />

Charlie Chong/ Fion Zhang


Read The following article:<br />

• E 748-95, Standard Practices for Thermal <strong>Neutron</strong> <strong>Radiography</strong> <strong>of</strong><br />

Materials<br />

• E 803, Standard Test Method for Determining the L/D Ratio <strong>of</strong> <strong>Neutron</strong><br />

<strong>Radiography</strong> Beams<br />

• E 1496-97, Standard Test Method for <strong>Neutron</strong> Radiographic Dimensional<br />

Measurements<br />

Charlie Chong/ Fion Zhang


Chapter 5 Radiation Measurement<br />

PART 6. <strong>Neutron</strong> Detection<br />

1.0 Characteristics<br />

The neutron is a part <strong>of</strong> the nucleus, has no charge and is somewhat larger in<br />

mass than the proton. It is similar to the photon in that it has no charge and<br />

produces ionization indirectly; it is different from the photon because it is a<br />

nuclear particle and not a unit <strong>of</strong> electromagnetic energy. (for photon, E=hʋ)<br />

Because the neutron is an uncharged particle, its interactions with matter are<br />

different from those <strong>of</strong> charged particles or photons. Ionization by neutrons is<br />

indirect: as a result <strong>of</strong> neutron interactions with matter, recoil (1) nuclei, (2)<br />

photons or (3) charged particles are produced and then interact with matter<br />

by various mechanisms that cause ionization.<br />

Charlie Chong/ Fion Zhang


Recoil - Measurement <strong>of</strong> Hydrogen Depth Pr<strong>of</strong>ile Using Fast <strong>Neutron</strong>s-<br />

Materials Analysis with Deuterium and Tritium Fusion <strong>Neutron</strong>s<br />

Charlie Chong/ Fion Zhang<br />

http://jolisfukyu.tokai-sc.jaea.go.jp/fukyu/mirai-en/2006/3_13.html


2.0 <strong>Neutron</strong> Sources<br />

<strong>Neutron</strong>s are classified according to their energies as shown in Table 4.<br />

Some radionuclides (such as californium-252) may decay by spontaneous<br />

fission and emit neutrons with fission fragments, photons and electrons.<br />

Induced fission reactions, such as those occurring in a nuclear reactor with<br />

uranium, emit about 2.5 neutrons per fission.<br />

Fission neutrons range in energy from 0.025 eV to about 16 MeV. Other<br />

neutron sources are the result <strong>of</strong> various nuclear reactions and produce either<br />

a spectrum <strong>of</strong> neutron energies or monoenergetic neutrons. Common neutron<br />

producing nuclear reactions are the (γ, n), (α, n), (p, n), (d, n) and (α, 2n)<br />

reactions and may use radionuclide emissions or accelerated particles to<br />

initiate the reaction.<br />

<strong>Neutron</strong> radiography usually uses radionuclides that emit alpha or gamma<br />

photons and produce neutrons by (α, n) and (γ, n) reactions with various<br />

target materials.<br />

Charlie Chong/ Fion Zhang


TABLE 4. <strong>Neutron</strong> classification.<br />

Class<br />

Thermal<br />

Epithermal<br />

Slow<br />

Intermediate<br />

Fast<br />

Relativistic<br />

Energy<br />

< 0.3 meV<br />

>1 eV<br />

30 meV to 100 eV<br />

100 eV to 10 keV<br />

10 keV to 10 MeV<br />

greater than 10 MeV<br />

Charlie Chong/ Fion Zhang


3.0 <strong>Neutron</strong> Detectors<br />

There are several mechanisms and devices used to detect neutrons <strong>of</strong><br />

various energies. Ionization chambers, proportional counters, scintillators,<br />

activation foils, track etch detectors, film emulsions, nuclear emulsions and<br />

thermoluminescent phosphors are some <strong>of</strong> the many devices used to detect<br />

neutrons. The main mechanisms used to detect neutrons in these devices are<br />

the (n, α), (n, p), (n, d), (n, f ) and (n, γ) nuclear reactions.<br />

Charlie Chong/ Fion Zhang


3.1 Proportional <strong>Neutron</strong> Detectors<br />

Many fast and slow neutron counters use proportional counting chambers<br />

filled with boron trifluoride (BF3) gas, <strong>of</strong>ten enriched in boron-10.<br />

The interaction <strong>of</strong> thermal (slow) neutrons with boron gas releases an alpha<br />

particle <strong>of</strong> several megaelectronvolts that is easily detected in the proportional<br />

mode. 10 5 B(n,α)7 3 Li<br />

Fast neutrons are detected by a similar counter, in which thermal neutrons<br />

are absorbed in an external cadmium shield ( 113 Cd(n,γ) 114 Cd ; the fast<br />

neutrons that pass through the shield are thermalized in hydrogen rich<br />

material and counted in the proportional chambers.<br />

γ<br />

hydrogen<br />

rich material<br />

boron trifluoride (BF3) gas<br />

external<br />

Pb Shield?<br />

Charlie Chong/ Fion Zhang


■<br />

http://minerals.usgs.gov/minerals/pubs/commodity/<br />

Charlie Chong/ Fion Zhang


The Cross Section (barns) <strong>of</strong><br />

commonly used conversion<br />

screen<br />

Careful on differential cross<br />

section for isotopes <strong>of</strong> same<br />

element.<br />

Charlie Chong/ Fion Zhang


TABLE 6. Properties <strong>of</strong> Some Thermal <strong>Neutron</strong> <strong>Radiography</strong> Conversion Materials<br />

Material<br />

Useful Reactions<br />

Cross Section for<br />

Life<br />

Thermal <strong>Neutron</strong>s (barns)<br />

Lithium<br />

6 Li(n,α) 3 H<br />

910<br />

prompt<br />

Boron<br />

10 B(n,α) 7 Li<br />

3,830<br />

prompt<br />

Rhodium<br />

103 Rh(n) 104m Rh<br />

11<br />

45 min<br />

103<br />

Rh(n) 104 Rh<br />

139<br />

42 s<br />

Silver<br />

107 Ag(n) 108 Ag<br />

35<br />

2.3 min<br />

109 Ag (n) 110 Ag<br />

91<br />

24 s<br />

Cadmium<br />

113 Cd((n,γ) 114 Cd<br />

20,000<br />

prompt<br />

Indium<br />

115 In(n) 116 n<br />

157<br />

54 min<br />

115<br />

In(n) 116m ln<br />

42<br />

14 s<br />

Samarium<br />

149 Sm(n,γ) 150 Sm<br />

41,000<br />

prompt<br />

I52<br />

Sm(n) 153 Sm<br />

210<br />

47 h<br />

Europium<br />

151 Eu(n) 152 Eu<br />

3,000<br />

9.2 h<br />

Gadolinium<br />

155<br />

Gd(n,γ) I56 Gd<br />

61,000<br />

prompt<br />

157<br />

Gd(n,γ) 158 Gd<br />

254,000<br />

prompt<br />

Dyprosium<br />

164<br />

Dy(n) 165m Dy<br />

2,200<br />

1.25 min<br />

164<br />

Dy(n) 165 Dy<br />

800<br />

140 min<br />

Gold<br />

197 Au(n) 198 Au<br />

99<br />

2.7 days<br />

Charlie Chong/ Fion Zhang


<strong>Neutron</strong> Cross Section <strong>of</strong> the elements<br />

Charlie Chong/ Fion Zhang<br />

http://periodictable.com/Properties/A/<strong>Neutron</strong>CrossSection.html


<strong>Neutron</strong> Cross Section σtotal for Gd =50000 barn<br />

Charlie Chong/ Fion Zhang<br />

http://periodictable.com/Properties/A/<strong>Neutron</strong>CrossSection.html


<strong>Neutron</strong> Cross Section σtotal for Dy =1010 barn<br />

Charlie Chong/ Fion Zhang<br />

http://periodictable.com/Properties/A/<strong>Neutron</strong>CrossSection.html


TABLE X1.1 Thermal <strong>Neutron</strong> Linear Attenuation Coefficients Using<br />

Average Scattering and Thermal Absorption Cross Sections for the<br />

Naturally Occurring Elements<br />

Charlie Chong/ Fion Zhang<br />

E748-02 Standard Practices for Thermal <strong>Neutron</strong> <strong>Radiography</strong> <strong>of</strong> Materials


Material<br />

Useful Reactions<br />

Cross Section for<br />

Life<br />

Thermal <strong>Neutron</strong>s (barns)<br />

Lithium<br />

6 Li(n,α) 3 H<br />

910<br />

prompt<br />

Boron<br />

10<br />

B(n,α) 7 Li<br />

3,830<br />

prompt<br />

Rhodium<br />

103 Rh(n) 104m Rh<br />

11<br />

45 min<br />

103 Rh(n) 104 Rh<br />

139<br />

42 s<br />

Silver<br />

107 Ag(n) 108 Ag<br />

35<br />

2.3 min<br />

109 Ag (n) 110 Ag<br />

91<br />

24 s<br />

Cadmium<br />

113 Cd((n,γ) 114 Cd<br />

20,000<br />

prompt<br />

Indium<br />

115<br />

In(n) 116 n<br />

157<br />

54 min<br />

115<br />

In(n) 116m ln<br />

42<br />

14 s<br />

Samarium<br />

149 Sm(n,γ) 150 Sm<br />

41,000<br />

prompt<br />

I52<br />

Sm(n) 153 Sm<br />

210<br />

47 h<br />

Europium<br />

151 Eu(n) 152 Eu<br />

3,000<br />

9.2 h<br />

Gadolinium<br />

155<br />

Gd(n,γ) I56 Gd<br />

61,000<br />

prompt<br />

157<br />

Gd(n.γ) 158 Gd<br />

254,000<br />

prompt<br />

Avg 64 Gd(n.γ) ? Gd<br />

49,000<br />

prompt<br />

Dyprosium<br />

164<br />

Dy(n) 165 mDy<br />

2,200<br />

1.25 min<br />

164<br />

Dy(n) 165 Dy<br />

800<br />

140 min<br />

Gold<br />

197<br />

Au(n) 198 Au<br />

99<br />

2.7 days<br />

Charlie Chong/ Fion Zhang


Charlie Chong/ Fion Zhang<br />

FIG. X1.1 Approximate Mass Attenuation Coefficients as a Function <strong>of</strong><br />

Atomic Number


TABLE 6. Properties <strong>of</strong> Some Thermal <strong>Neutron</strong> <strong>Radiography</strong> Conversion<br />

Materials<br />

Material<br />

Useful Reactions<br />

Cross Section for<br />

Life<br />

Thermal <strong>Neutron</strong>s (barns)<br />

Lithium<br />

6<br />

Li(n,α) 3 H<br />

910<br />

prompt<br />

Boron<br />

10 B(n,α) 7 Li<br />

3,830<br />

prompt<br />

Rhodium<br />

103 Rh(n) 104m Rh<br />

11<br />

45 min<br />

103<br />

Rh(n) 104 Rh<br />

139<br />

42 s<br />

Silver<br />

107<br />

Ag(n) 108 Ag<br />

35<br />

2.3 min<br />

109 Ag (n) 110 Ag<br />

91<br />

24 s<br />

Cadmium<br />

113<br />

Cd((n,γ) 114 Cd<br />

20,000<br />

prompt<br />

Indium<br />

115 In(n) 116 n<br />

157<br />

54 min<br />

115<br />

In(n) 116m ln<br />

42<br />

14 s<br />

Samarium<br />

149 Sm(n,γ) 150 Sm<br />

41,000<br />

prompt<br />

I52<br />

Sm(n) 153 Sm<br />

210<br />

47 h<br />

Europium<br />

151 Eu(n) 152 Eu<br />

3,000<br />

9.2 h<br />

Gadolinium<br />

155<br />

Gd(n,γ) I56 Gd<br />

61,000<br />

prompt<br />

157<br />

Gd(n.γ) 158 Gd<br />

254,000<br />

prompt<br />

Dyprosium<br />

164<br />

Dy(n) 165 mDy<br />

2,200<br />

1.25 min<br />

164<br />

Dy(n) 165 Dy<br />

800<br />

140 min<br />

Gold<br />

197<br />

Au(n) 198 Au<br />

99<br />

2.7 days<br />

Charlie Chong/ Fion Zhang


TABLE 6. Capture cross sections σ <strong>of</strong> strongly absorbing elements for<br />

neutrons in approximate thermal equilibrium at 300 K (27 °C = 80 °F).<br />

Charlie Chong/ Fion Zhang


TABLE 4. Average Characteristics <strong>of</strong> Thermal-Sources<br />

Type <strong>of</strong> Source<br />

Typical<br />

Resolution**<br />

Exposure<br />

Characteristics<br />

Radiographic<br />

Intensity*<br />

Time<br />

Radioisotope<br />

10 1 to 10 4<br />

Poor to Medium<br />

Long<br />

Stable operation.<br />

medium investment cost.<br />

possibly portable.<br />

Accelerator<br />

10 3 to 10 6<br />

Medium<br />

Average<br />

On-<strong>of</strong>f operation. medium<br />

cost. possibly mobile.<br />

Subcritical<br />

10 4 to 10 6<br />

Good<br />

Average<br />

Stable operation,<br />

Assembly<br />

medium to high investment<br />

cost, mobility difficult<br />

Nuclear reactor<br />

10 5 to 10 8<br />

Excellent<br />

Short<br />

Stable operation,<br />

medium to high investment<br />

cost. mobility difficult<br />

*<strong>Neutron</strong>s per square centimeter per second. n/cm 2 ∙s<br />

**These classifications are relative<br />

Charlie Chong/ Fion Zhang


More <strong>Reading</strong> on Gadolinum<br />

Gadolinium is a silvery-white malleable and ductile rare-earth metal. It<br />

crystallizes in hexagonal, close-packed α-form at room temperature, but,<br />

when heated to temperatures above 1235 °C, it transforms into its β-form,<br />

which has a body-centered cubic structure.<br />

Gadolinium-157 has the highest thermal neutron capture cross-section<br />

among any stable nuclides: 259,000 barns. Only xenon-135 has a higher<br />

cross section, 2 million barns, but that isotope is unstable.<br />

Charlie Chong/ Fion Zhang


Gadolinium is generally believed to be ferromagnetic at temperatures below<br />

20 °C (68 °F) and is strongly paramagnetic above this temperature. There is<br />

some evidence that gadolinium may be a helical antiferromagnet, rather than<br />

a ferromagnet, below 20 °C (68 °F). Gadolinium demonstrates a<br />

magnetocaloric effect whereby its temperature increases when it enters a<br />

magnetic field and decreases when it leaves the magnetic field. The<br />

temperature is lowered to 5 °C (41 °F) for the gadolinium alloy Gd85Er15,<br />

and the effect is considerably stronger for the alloy Gd5(Si2Ge2), but at a<br />

much lower temperature (


Gadolinum<br />

Charlie Chong/ Fion Zhang


Gadolinum<br />

Charlie Chong/ Fion Zhang


isotope NA half-life DM DE (MeV) Decay Product<br />

148Gd syn 75y α 3.271<br />

144<br />

Sm<br />

150Gd syn 1.8×10 6 y α 2.808<br />

146<br />

Sm<br />

152Gd 0.20% 1.08×10 14 y α 2.205<br />

148<br />

Sm<br />

154Gd 2.18% – (α) 0.0812<br />

150<br />

Sm<br />

155Gd 14.80% – (α) 0.0812<br />

151<br />

Sm<br />

156Gd 20.47% – (SF)


σ,Cross Section <strong>of</strong> Gadolinium<br />

Gd Average = 49000 barn prompt<br />

155<br />

Gd(n,γ) 156 Gd = 61,000 barn prompt<br />

157<br />

Gd(n.γ) 158 Gd = 254,000 barn prompt<br />

Charlie Chong/ Fion Zhang


<strong>Neutron</strong><br />

For many years after the proton and electron became comfortable concepts<br />

for building models <strong>of</strong> the atoms <strong>of</strong> the elements but explanations eluded<br />

researchers for the existence <strong>of</strong> isotopes and the extremely penetrating<br />

radiation emitted by the bombardment <strong>of</strong> light elements with alpha particles.<br />

In 1932, Chadwick described a neutral particle with a mass equal to a proton<br />

that he called a neutron. The neutron explained many observations<br />

concerning radiation and particle physics and the concept was rapidly<br />

accepted. <strong>Neutron</strong> characteristics are given in Table 3.<br />

Charlie Chong/ Fion Zhang


TABLE 3. <strong>Neutron</strong> characteristics.<br />

Quantity<br />

Measurement<br />

Charge<br />

neutral<br />

Rest mass<br />

1.675 × 10 –27 kg<br />

Classical radius 1.532 × 10 –18 m<br />

Magnetic moment –9.662 × 10 –27 J·T –1<br />

Compton wavelength 1.320 × 10 –15 m<br />

Charlie Chong/ Fion Zhang


Hydrogen, Deuterium, Tritium<br />

Radioactive materials have existed since the earth was created. All elements<br />

with atomic numbers greater than 83, bismuth, exist only as radioactive<br />

elements and many elements below atomic number 83 have radioactive<br />

isotopes that exist in nature.<br />

The difference between a stable or nonradioactive atom <strong>of</strong> an element and an<br />

unstable or radioactive atom is in the energy content <strong>of</strong> the nucleus. Most<br />

<strong>of</strong>ten an excess or deficiency in the number <strong>of</strong> neutrons in the nucleus<br />

provides the excess energy or instability.<br />

As an example: most hydrogen in nature exists as atoms with only 1 proton<br />

and 1 electron. About 15 <strong>of</strong> every 100 000 atoms <strong>of</strong> hydrogen have a neutron<br />

plus the proton in the nucleus, giving the atom a mass <strong>of</strong> 2 or twice the mass<br />

<strong>of</strong> most hydrogen atoms. Mass 2 hydrogen is called deuterium or heavy<br />

hydrogen and is stable. When a second neutron is added to the nucleus <strong>of</strong><br />

hydrogen, the atom has a mass <strong>of</strong> 3, is called tritium and is radioactive.<br />

The tritium atom is produced in nature by cosmic bombardment to produce a<br />

pre- 1952 concentration in nature <strong>of</strong> between 1 ~ 10 tritium atoms per 10 18<br />

hydrogen atoms.<br />

Charlie Chong/ Fion Zhang


<strong>Neutron</strong>s<br />

<strong>Neutron</strong>s produced by fission, accelerator nuclear reactions or radioisotope<br />

sources have considerable kinetic energy. This kinetic energy is most <strong>of</strong>ten<br />

lost by scattering interactions with or absorption in the nuclei <strong>of</strong> the atoms in<br />

their path. Absorption <strong>of</strong> the neutron is followed by release <strong>of</strong> electromagnetic<br />

radiation or large particles such as protons, multiple neutrons, deuterons or<br />

alpha particles. Interactions with the orbital electrons contribute negligibly to<br />

the absorption <strong>of</strong> neutrons by matter. The nucleus is much smaller than the<br />

electron orbits, so neutron interactions are less frequent than those <strong>of</strong> alpha<br />

or beta particles. And because the neutron has no charge, ionization and<br />

excitation are not major absorption processes.<br />

Charlie Chong/ Fion Zhang


FIGURE 4. Ionization by alpha particle that ejects orbital electron from atom.<br />

Specific ionization is number <strong>of</strong> ion pairs generated by particle per unit path.<br />

Total ionization designates number <strong>of</strong> ion pairs produced by particle along its<br />

entire path.<br />

Charlie Chong/ Fion Zhang


<strong>Neutron</strong>- Elastic Scattering<br />

For elastic scattering, the neutron collides with the nucleus and bounces <strong>of</strong>f,<br />

leaving the nucleus unchanged. This type <strong>of</strong> collision can be treated<br />

straightforwardly as a mechanical billiard ball type <strong>of</strong> collision. In the collision<br />

the energy <strong>of</strong> the neutron is shared by the nucleus, thus each collision<br />

reduces the energy <strong>of</strong> the neutron. After a number <strong>of</strong> collisions with the nuclei,<br />

the energy is reduced to the same average kinetic energy as that <strong>of</strong> the<br />

absorbing medium. This energy is <strong>of</strong>ten referred to as the thermal energy<br />

because it depends primarily on the temperature. <strong>Neutron</strong>s at thermal<br />

equilibrium with their surroundings are thermal neutrons. At 20°C (68°F), a<br />

thermal neutron would have a kinetic energy <strong>of</strong> about 0.025 eV and a velocity<br />

<strong>of</strong> 2200 m·s –1 (4900 mi·h –1 ).<br />

Charlie Chong/ Fion Zhang


The transfer <strong>of</strong> energy from the neutron to the nucleus is greater for light<br />

nuclei. Therefore, low atomic nuclei containing materials such as water,<br />

hydrocarbons, graphite and beryllium are used to reduce neutron energies.<br />

Such materials are called moderators. Hydrogen nuclei have essentially the<br />

same mass as neutrons and can undergo nearly complete kinetic energy<br />

transfer in a single collision. Energy transfer to larger nuclei require many<br />

collisions.<br />

Charlie Chong/ Fion Zhang


<strong>Neutron</strong>- Inelastic Scattering<br />

Here the neutron collides with the nucleus leaving the nucleus in an excited<br />

state. In this process, the nucleus may either stay in the excited state (n,n’) as<br />

a metastable isomer or will immediately emit gamma radiation (n,γn) and<br />

return to the ground or original state.<br />

Keywords:<br />

Excited state - (n,n’)<br />

Emit gamma and return to stable state - (n,n’)<br />

Charlie Chong/ Fion Zhang


Nuclear <strong>Neutron</strong> Absorption<br />

As the neutron has no charge, it can approach the nucleus until the close<br />

range attractive forces <strong>of</strong> the nucleus begin to operate. In this process, the<br />

neutron is captured, forming a compound nucleus. Because there is no<br />

charge barrier, even the slowest neutron can be readily captured.<br />

As the binding energy <strong>of</strong> a neutron into a compound nucleus is nearly 8MeV,<br />

even the capture <strong>of</strong> thermal neutrons can result in a highly excited state for<br />

the nucleus. (the thermal neutron has 0.025~0.1 MeV <strong>of</strong> energy, how this<br />

relate to the 8MeV?)<br />

This excited nucleus can attain relative stability by:<br />

■ ejecting a proton,<br />

■ ejecting an alpha particle, or<br />

■ emitting the excess energy as gamma radiation.<br />

When a particle is ejected, the nucleus becomes a new element; then the<br />

process is also known as nuclear transmutation. The discovery <strong>of</strong><br />

transmutation by slow neutrons led to the realization <strong>of</strong> nuclear fission.<br />

Charlie Chong/ Fion Zhang


As the binding energy <strong>of</strong> a neutron into a compound nucleus is nearly 8MeV,<br />

even the capture <strong>of</strong> thermal neutrons can result in a highly excited state for<br />

the nucleus. (the thermal neutron has 0.025~0.1 MeV <strong>of</strong> energy, how this<br />

relate to the 8MeV?)<br />

Charlie Chong/ Fion Zhang


The simplest capture reaction is that <strong>of</strong> capture <strong>of</strong> slow neutrons with<br />

emission <strong>of</strong> gamma rays (n,γ). Thermal neutron reaction with cobalt is an<br />

example:<br />

59<br />

Co + n → 60 Co + γ → 60 Ni + β - + γ<br />

In heavy nuclei, the capture <strong>of</strong> a slow neutron, followed by the emission <strong>of</strong><br />

gamma radiation, increases the neutron-to-proton ratio — usually making the<br />

nucleus radioactive with decay by electron emission likely. More information<br />

on production <strong>of</strong> radioactive material by neutron capture may be found in the<br />

discussion <strong>of</strong> radioactive materials.<br />

Charlie Chong/ Fion Zhang


As the energy <strong>of</strong> the impinging neutron is made larger, a charged particle can<br />

be ejected. However, a charged particle, because <strong>of</strong> the short range attractive<br />

forces <strong>of</strong> the nuclei, is hindered from leaving the nucleus and processes such<br />

as (n,p), (n,α) and (n,d) can only take place when the incident neutron<br />

supplies sufficient energy to overcome the binding energies <strong>of</strong> the particles in<br />

the nucleus. For heavy nuclei these forces are appreciable and the requisite<br />

neutron energy becomes greater. Thus, for example, a particle ejection is<br />

possible only if the neutron has sufficient energy to overcome the binding<br />

energy <strong>of</strong> the alpha particle; that is, the neutron must be a fast neutron.<br />

Charlie Chong/ Fion Zhang


In the (n,α) reaction, the product nucleus contains one neutron and two<br />

protons less than the original nucleus. The neutron-to-proton ratio is<br />

increased and the transmutation usually produces a radioactive nucleus that<br />

decays by the emission <strong>of</strong> an electron (beta disintegration).<br />

As the energy <strong>of</strong> the incident neutron approaches 30 MeV, the compound<br />

nucleus can eject three neutrons (n, 3n) or two neutrons and a proton (n, 2np)<br />

as well as other combinations <strong>of</strong> particles. At even higher energies, more<br />

particles may be ejected until the nucleus essentially disappears (spallation).<br />

Finally, nuclear fission (n,f), where the nucleus breaks up with the release <strong>of</strong><br />

several larger particles and several neutrons, can be induced in certain large<br />

nuclides, such as uranium-235, by neutrons <strong>of</strong> almost any energy, whereas in<br />

other nuclides, fast or energetic neutrons are required.<br />

Charlie Chong/ Fion Zhang


Nuclear Cross Sections<br />

Because <strong>of</strong> many reactions possible for absorbing neutrons and their<br />

complicated energy and mass dependencies, there is no simple way to<br />

present the total absorption effect. However, the probability <strong>of</strong> any interaction<br />

between neutrons and matter can be made qualitative by means <strong>of</strong> the<br />

concept <strong>of</strong> cross sections. The cross section σ is the effective target area <strong>of</strong><br />

the nucleus as seen by the impinging neutron <strong>of</strong> a given energy. The number<br />

<strong>of</strong> interactions per unit time will be nvNσ, where n is the number <strong>of</strong> neutrons<br />

per unit volume moving with velocity v towards the target <strong>of</strong> N nuclei. The<br />

quantity nv is the neutron flux density (neutrons per square centimeter<br />

second). The cross section σ is usually expressed in square meters (m 2 ) or<br />

barns (b), where 1 b = 10 –24 cm 2 =10 –28 m 2 .<br />

Charlie Chong/ Fion Zhang


In discussing the variation <strong>of</strong> nuclear cross section with energy <strong>of</strong> the incident<br />

neutrons, certain generalizations <strong>of</strong> a broad character can be made. In<br />

general, there are three regions that can be distinguished.<br />

■ First is the low energy region, which includes the thermal range, where<br />

the cross section decreases steadily with increasing neutron energy. The total<br />

cross section is the sum <strong>of</strong> two terms, one due to neutron scattering is quite<br />

small and almost constant, the other representing absorption by the nucleus<br />

is inversely proportional to the velocity (energy) . This low energy range is<br />

termed the v –1 region, where the time spent by the neutron near the nucleus<br />

is proportional to v–1.<br />

Charlie Chong/ Fion Zhang


Second, following the somewhat indefinite v –1 region, many elements exhibit<br />

peaks called resonance peaks, where the neutron cross sections rise sharply<br />

to high values for certain energies, then fall to lower values again. Depending<br />

on the element, the number <strong>of</strong> such peaks may number three or more. These<br />

peaks may be found mostly in the energy range 0.1 to 1 eV, although in a few<br />

elements like uranium-238, they may be found up to energies <strong>of</strong> 10 eV. These<br />

reactions are <strong>of</strong> the (η,γ) (Eta, gamma) type.<br />

And third, with neutrons <strong>of</strong> high energy in the MeV range, the cross sections<br />

are very low, less than 10 –27 m 2 (10 b), compared to the very high cross<br />

sections <strong>of</strong> 4 × 10 –25 m 2 (several thousand barns, ~4000 b) at low energies.<br />

Charlie Chong/ Fion Zhang


A simple example <strong>of</strong> the total absorption cross section is that <strong>of</strong> cadmium,<br />

shown in Fig. 5. The v –1 region is shown up to about 0.03 eV, the resonance<br />

at 0.176 eV and the low cross section region for energies greater than about<br />

2 MeV. The dramatic increase in cross sections at the resonance have been<br />

worked out by the theory <strong>of</strong> G. Breit and E.P. Wigner. In its simplicity, if the<br />

energy <strong>of</strong> the neutron is such that a compound nucleus can be formed at or<br />

near one <strong>of</strong> its energy levels, then the probability <strong>of</strong> capture <strong>of</strong> these neutrons<br />

will be exceptionally high.<br />

All elements do not show the resonant absorption effect; for example, boron<br />

has no measurable resonance and the cross section follows the v –1 law from<br />

0.01 eV to over 1000 eV. However, its cross section for (n,α) is so large for<br />

neutrons <strong>of</strong> low energy that this reaction is <strong>of</strong>ten used for neutron detectors.<br />

Table 6 shows the dramatic variation <strong>of</strong> cross section for absorbing thermal<br />

neutrons <strong>of</strong> some <strong>of</strong> the better neutron absorbers.<br />

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FIGURE 5. Absorption <strong>of</strong> neutrons by cadmium, showing resonance peak at<br />

0.176 eV.<br />

0.176 eV<br />

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TABLE 6. Capture cross sections σ <strong>of</strong> strongly absorbing elements for<br />

neutrons in approximate thermal equilibrium at 300 K (27 °C = 80 °F).<br />

Charlie Chong/ Fion Zhang


<strong>Neutron</strong> Activation<br />

In the section on neutron interactions with materials, neutron capture was<br />

briefly discussed. This technique, coupled with the large fields <strong>of</strong> neutrons<br />

available in nuclear reactors, produces most <strong>of</strong> the radioisotopes used in<br />

radiography. cobalt-60 and iridium-192 come from thermal neutron<br />

bombardment <strong>of</strong> the stable isotopes (cobalt-59 and iridium-191) <strong>of</strong> these two<br />

elements. Production <strong>of</strong> the radioactivity can be predicted by Eq. 21:<br />

Charlie Chong/ Fion Zhang


in which<br />

A is the activity produced in disintegrations per second,<br />

N is number <strong>of</strong> target atoms being bombarded,<br />

f is the neutron flux (in neutrons per centimeter second),<br />

σ is the cross section for neutron capture (in square centimeter),<br />

t i is the irradiation time in the same units as the half life and<br />

T is the half life <strong>of</strong> the radioisotope produced.<br />

The exponential portion <strong>of</strong> the equation corrects the production <strong>of</strong> the<br />

radioactive material for the amount that decays away while more is being<br />

made. This leads to the point <strong>of</strong> diminishing returns for production in that after<br />

about five half lives, almost as much <strong>of</strong> the radioactive material is decaying as<br />

is being produced per each increment <strong>of</strong> neutron bombardment time.<br />

Charlie Chong/ Fion Zhang


Also, the equation is correct only for thin samples <strong>of</strong> the bombarded material.<br />

Absorption <strong>of</strong> neutrons in the outer layers <strong>of</strong> the sample (usually a metal<br />

pellet) reduces the number <strong>of</strong> neutrons incident on the interior atoms. This<br />

self-shielding <strong>of</strong> neutrons coupled with a self-absorption <strong>of</strong> gamma rays<br />

released by radioactive atoms inside <strong>of</strong> the sample gives a gamma output<br />

considerably lower than calculated.<br />

Charlie Chong/ Fion Zhang


Fission Fragments<br />

When uranium-235 or other fissionable atom undergoes fission, multiple<br />

neutrons and two major fragments <strong>of</strong> the nucleus are released. The two<br />

fragments are called fission fragments and are a source <strong>of</strong> radioactive<br />

materials for industrial, medical and research use. The fragments are usually<br />

<strong>of</strong> unequal size and are grouped in two distributions around mass numbers<br />

96 and 138. One <strong>of</strong> the major products is cesium-137, which can be<br />

chemically separated from the other fission fragments for use as a gamma<br />

ray source in radiography, medical therapy and large irradiation facilities for<br />

preservation <strong>of</strong> food and for sterilization <strong>of</strong> medical supplies.<br />

Fission Fragment: cesium-137<br />

Charlie Chong/ Fion Zhang


Accelerator Production<br />

Large particle accelerators such as linatrons, van de graaff generators and<br />

cyclotrons can provide appreciable neutron fluxes or streams <strong>of</strong> high energy<br />

particles including protons, deuterons and helium nuclei. When appropriate<br />

target materials are bombarded by these particles, radioactive nuclei can be<br />

produced. Although radioactive materials for medical use are being produced<br />

in this fashion, generally radiographic sources are not commercially produced<br />

in this fashion.<br />

Charlie Chong/ Fion Zhang


Charlie Chong/ Fion Zhang


The Measurement Units<br />

Charlie Chong/ Fion Zhang<br />

Rolf Maximilian Sievert


Sievert - (Sv) is an unit for health effect <strong>of</strong> ionizing radiation,<br />

numerically it is the energy absorbed by human body (by matters?) <strong>of</strong><br />

1J·Kg -1<br />

The sievert (symbol: Sv is a derived unit <strong>of</strong> ionizing radiation dose in the<br />

International System <strong>of</strong> Units (SI). It is a measure <strong>of</strong> the health effect <strong>of</strong> low<br />

levels <strong>of</strong> ionizing radiation on the human body.<br />

Quantities that are measured in sieverts are intended to represent the<br />

stochastic 随 机 的 health risk, which for radiation dose assessment is defined<br />

as the probability <strong>of</strong> cancer induction and genetic damage.<br />

To enable consideration <strong>of</strong> stochastic health risk, calculations are performed<br />

to convert the physical quantity absorbed dose into equivalent and effective<br />

doses, the details <strong>of</strong> which depend on the radiation type and biological<br />

context. For applications in radiation protection and dosimetry assessment<br />

the International Commission on Radiological Protection (ICRP) and<br />

International Commission on Radiation Units and Measurements (ICRU) have<br />

published recommendations and data which are used to calculate these.<br />

These are under continual review, and changes are advised in the formal<br />

"Reports" <strong>of</strong> those bodies.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Sievert


The sievert is used for radiation dose quantities such as equivalent dose,<br />

effective dose, and committed dose.<br />

It is used to represent both the risk <strong>of</strong> the effect <strong>of</strong> external radiation from<br />

sources outside the body and the effect <strong>of</strong> internal irradiation due to inhaled<br />

or ingested radioactive substances.<br />

Conventionally, the sievert is not used for high dose rates <strong>of</strong> radiation that<br />

produce deterministic effects, which is the severity <strong>of</strong> acute tissue damage<br />

that is certain to happen. Such effects are compared to the physical quantity<br />

absorbed dose measured by the unit gray (Gy).<br />

The sievert is <strong>of</strong> fundamental importance in dosimetry and radiation protection,<br />

and is named after Rolf Maximilian Sievert, a Swedish medical physicist<br />

renowned for work on radiation dosage measurement and research into the<br />

biological effects <strong>of</strong> radiation. One sievert carries with it a 5.5% chance <strong>of</strong><br />

eventually developing cancer.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Sievert


One Sievert equals 100 rem. The rem is an older, non-SI unit <strong>of</strong><br />

measurement.<br />

To enable a comprehensive view <strong>of</strong> the Sievert this article deals with the<br />

definition <strong>of</strong> the Sievert as an SI unit, summarises the recommendations <strong>of</strong><br />

the ICRU and ICRP on how the Sievert is calculated, includes a guide to the<br />

effects <strong>of</strong> ionizing radiation as measured in Sievert, and gives examples <strong>of</strong><br />

approximate figures <strong>of</strong> dose uptake in certain situations.<br />

The gray - quantity "D"<br />

1 Gy = 1 joule/kilogram - a physical quantity. 1 Gy is the deposit <strong>of</strong> a joule <strong>of</strong><br />

radiation energy in a kg <strong>of</strong> matter or tissue.<br />

The sievert - quantity "H"<br />

1 Sv = 1 joule/kilogram - a biological effect. The Sievert represents the<br />

equivalent biological effect <strong>of</strong> the deposit <strong>of</strong> a joule <strong>of</strong> radiation energy in a<br />

kilogram <strong>of</strong> human tissue. The equivalence to absorbed dose is denoted by Q.<br />

H = Q × D<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Sievert


REM - Roentgen equivalent man<br />

The roentgen equivalent in man (abbreviated rem; symbol rem, or <strong>of</strong>ten but<br />

incorrectly R) is an older, CGS unit <strong>of</strong> equivalent dose, effective dose, and<br />

committed dose. Quantities measured in rem are designed to represent the<br />

stochastic biological effects <strong>of</strong> ionizing radiation, primarily radiation-induced<br />

cancer. These quantities are a complex weighted average <strong>of</strong> absorbed dose,<br />

which is a clear physical quantity measured in rads. There is no universally<br />

applicable conversion constant from rad to rem; the conversion depends on<br />

relative biological effectiveness (RBE).<br />

The rem is defined since 1976 as equal to 0.01 sievert, which is the more<br />

commonly used SI unit outside <strong>of</strong> the United States. A number <strong>of</strong> earlier<br />

definitions going back to 1945 were derived from the roentgen unit, which<br />

was named after Wilhelm Röntgen, a German scientist who discovered X-<br />

rays. The acronym is now a misleading historical artifact, since 1 roentgen<br />

actually deposits about 0.96 rem in s<strong>of</strong>t biological tissue, when all weighting<br />

factors equal unity. Older units <strong>of</strong> rem following other definitions are up to<br />

17% smaller than the modern rem.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Roentgen_equivalent_man


One rem carries with it a 0.055% chance <strong>of</strong> eventually developing cancer.<br />

Doses greater than 100 rem received over a short time period are likely to<br />

cause acute radiation syndrome (ARS), possibly leading to death within<br />

weeks if left untreated. Note that the quantities that are measured in rem were<br />

not designed to be correlated to ARS symptoms. The absorbed dose,<br />

measured in rad, is the best indicator <strong>of</strong> ARS.<br />

A rem is a large dose <strong>of</strong> radiation, so the millirem (mrem), which is one<br />

thousandth <strong>of</strong> a rem, is <strong>of</strong>ten used for the dosages commonly encountered,<br />

such as the amount <strong>of</strong> radiation received from medical x-rays and background<br />

sources.<br />

Charlie Chong/ Fion Zhang


Rem Usage<br />

The rem and millirem are CGS units in widest use among the American public,<br />

industry, and government. SI units are the norm outside <strong>of</strong> the United States,<br />

and they are increasingly encountered within the US in academic, scientific,<br />

and engineering environments.<br />

The conventional units for dose rate is mrem/h. Regulatory limits and chronic<br />

doses are <strong>of</strong>ten given in units <strong>of</strong> mrem/yr or rem/yr, where they are<br />

understood to represent the total amount <strong>of</strong> radiation allowed (or received)<br />

over the entire year. In many occupational scenarios, the hourly dose rate<br />

might fluctuate to levels thousands <strong>of</strong> times higher for a brief period <strong>of</strong> time,<br />

without infringing on the annual total exposure limits.<br />

Charlie Chong/ Fion Zhang


There is no exact conversion from hours to years because <strong>of</strong> leap years, but<br />

approximate conversions are:<br />

1 mrem/h = 8766 mrem/yr<br />

0.1141 mrem/h = 1000 mrem/yr<br />

The ICRP once adopted fixed conversion for occupational exposure, although<br />

these have not appeared in recent documents:<br />

8 h = 1 day<br />

40 h = 1 week<br />

50 week = 1 yr<br />

Therefore, for occupation exposures <strong>of</strong> that time period,<br />

1 mrem/h = 2000 mrem/yr<br />

0.5 mrem/h = 1000 mrem/yr<br />

Charlie Chong/ Fion Zhang


The US National Institute <strong>of</strong> Standards and Technology (NIST) strongly<br />

discourages Americans from expressing doses in rem, in favor <strong>of</strong><br />

recommending the SI unit. The NIST recommends defining the rem in relation<br />

to the SI in every document where this unit is used. For US industries and US<br />

firms that do not require the sole use <strong>of</strong> SI, however, the unit rem is <strong>of</strong>ten<br />

preferred.<br />

Charlie Chong/ Fion Zhang


Health Effects<br />

Ionizing radiation has deterministic and stochastic effects on human health.<br />

The deterministic effects that can lead to acute radiation syndrome only occur<br />

in the case <strong>of</strong> high doses (> ~10 rad or > 0.1 Gy) and high dose rates (> ~10<br />

rad/h or > 0.1 Gy/h). A model <strong>of</strong> deterministic risk would require different<br />

weighting factors (not yet established) than are used in the calculation <strong>of</strong><br />

equivalent and effective dose.<br />

To avoid confusion, deterministic effects (either chronic & acute?) are<br />

normally compared to absorbed dose in units <strong>of</strong> rad, not rem.<br />

Stochastic effects are those that occur randomly, such as radiation-induced<br />

cancer. The consensus <strong>of</strong> the nuclear industry, nuclear regulators, and<br />

governments, is that the incidence <strong>of</strong> cancers due to ionizing radiation (not<br />

including excessive high dose rate?) can be modeled as increasing linearly<br />

with effective dose at a rate <strong>of</strong> 0.055% per rem (5.5%/Sv). Individual studies,<br />

alternate models, and earlier versions <strong>of</strong> the industry consensus have<br />

produced other risk estimates scattered around this consensus model.<br />

Charlie Chong/ Fion Zhang


There is general agreement that the risk is much higher for infants and<br />

fetuses than adults, higher for the middle-aged than for seniors, and higher<br />

for women than for men, though there is no quantitative consensus about this.<br />

There is much less data, and much more controversy, regarding the<br />

possibility <strong>of</strong> cardiac and teratogenic 引 起 畸 型 的 effects, and the modelling <strong>of</strong><br />

internal dose<br />

The International Commission on Radiological Protection (ICRP)<br />

recommends limiting artificial irradiation <strong>of</strong> the public to an average <strong>of</strong> 100<br />

mrem (1 mSv) (0.1Rem for public and 5Rem for radiation worker?) <strong>of</strong><br />

effective dose per year, not including medical and occupational exposures.<br />

For comparison, radiation levels inside the US United States Capitol are 85<br />

mrem/yr (0.85 mSv/yr), close to the regulatory limit, because <strong>of</strong> the uranium<br />

content <strong>of</strong> the granite structure. According to the ICRP model, someone who<br />

spent 20 years inside the capitol building would have an extra one in a<br />

thousand chance <strong>of</strong> getting cancer, over and above any other existing risk.<br />

(20 yr × 85 mrem/yr × 0.001 rem/mrem × 0.055%/rem = ~0.1%) That<br />

"existing risk" is much higher; an average person would have a one in ten<br />

chance <strong>of</strong> getting cancer during this same 20-year period, even without any<br />

exposure to artificial radiation.<br />

Charlie Chong/ Fion Zhang


Radiation-related Quantities<br />

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Radiation-related Quantities<br />

1 gray = 100 rad<br />

J·Kg -1 = 100,000 erg·Kg -1<br />

Joule = 1 x 10 -5 erg<br />

1 Rongent ≠ 1 Rad<br />

Charlie Chong/ Fion Zhang


The Röntgen equivalent physical or rep (symbol rep) is a unit <strong>of</strong><br />

absorbed dose first introduced by Herbert Parker in 1945 to replace an<br />

improper application <strong>of</strong> the roentgen unit to biological tissue. It is the<br />

absorbed energetic dose before the biological efficiency <strong>of</strong> the radiation is<br />

factored in. The rep has variously been defined as 83 or 93 ergs per gram <strong>of</strong><br />

tissue (8.3/9.3 mGy)[2] or per cm 3 <strong>of</strong> tissue. At the time, this was thought to<br />

be the amount <strong>of</strong> energy deposited by 1 roentgen.<br />

Improved measurements have since found that one roentgen <strong>of</strong> air kerma<br />

deposits 8.77 mGy in dry air, or 9.6 mGy in s<strong>of</strong>t tissue, but the rep was<br />

defined as a fixed number <strong>of</strong> ergs per unit gram. A 1952 handbook from the<br />

US National Bureau <strong>of</strong> Standards affirms that "The numerical coefficient <strong>of</strong><br />

the rep has been deliberately changed to 93, instead <strong>of</strong> the earlier 83, to<br />

agree with L. H. Gray's 'energy-unit'." It is unclear what was meant by Gray's<br />

'energy unit', since the gray was not defined until the 1970s; perhaps the<br />

gram-roentgen he introduced in 1940? The rep was commonly used until the<br />

1960s, but was gradually displaced by the rad starting in 1954 and later the<br />

gray starting in 1977.<br />

Charlie Chong/ Fion Zhang


Air Kerma means kerma in a given mass <strong>of</strong> air. The unit used to measure<br />

the quantity <strong>of</strong> air kerma is the Gray (Gy). For X-rays with energies less than<br />

300 kiloelectronvolts (keV), 1 Gy = 100 rad. In air, 1 Gy <strong>of</strong> absorbed dose is<br />

delivered by 114 roentgens (R) <strong>of</strong> exposure.<br />

100 rad = 114 R<br />

Kerma - kinetic energy released in the medium<br />

(Kinetic Energy Released per Unit Mass)<br />

1 abbreviation for kinetic energy released in the medium, a quantity that<br />

describes the transfer <strong>of</strong> energy from a photon to a medium as the ratio <strong>of</strong><br />

energy transferred per unit mass at each point <strong>of</strong> interaction.<br />

2 abbreviation for kinetic energy released in matter, a unit <strong>of</strong> quantity referring<br />

to the kinetic energy transferred from photons to charged particles, such as<br />

electrons in Compton interactions, per unit mass. The SI unit for the KERMA<br />

is the gray, and the special unit is the rad.<br />

Charlie Chong/ Fion Zhang<br />

http://medical-dictionary.thefreedictionary.com/KERMA


Kerma Kinetic Energy Released per Unit Mass.<br />

Kerma is a dose variable. Kerma K is the quotient <strong>of</strong> dEtr and dm; whereby<br />

dEtr is the sum <strong>of</strong> the starting values <strong>of</strong> kinetic energies <strong>of</strong> all charged<br />

particles released by indirectly ionizing radiation from the material in a volume<br />

element dV, and dm is the mass <strong>of</strong> the material in this volume element. All<br />

indications for a Kerma must mention the reference material (i.e. the material<br />

dm). The SI unit <strong>of</strong> the kerma is gray (Gy).<br />

Charlie Chong/ Fion Zhang<br />

http://www.euronuclear.org/info/encyclopedia/k/kerma.htm


Teratogenic 引 起 畸 型 的<br />

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Deterministic Effects<br />

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Chronic Effect<br />

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Deterministic Effects<br />

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ionization chambers<br />

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ionization chambers<br />

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ionization chambers<br />

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ionization<br />

chambers<br />

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ionization chambers<br />

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More <strong>Reading</strong> on ionization chambers<br />

Basically, an ionization chamber consists <strong>of</strong> two electrodes kept at a potential<br />

difference and a gas that fills the space between the electrodes. The<br />

detection process occurs when an X-ray photon interacts with the gas inside<br />

the chamber, forming “N” number <strong>of</strong> electron-ion pairs. The electrons and<br />

ions are separated due to the direction and sense <strong>of</strong> the electric field.<br />

Continuous streams <strong>of</strong> photons originate a continuous production <strong>of</strong> electronhole<br />

pairs and consequently an electric current between two electrodes. This<br />

current, typically in the order <strong>of</strong> a few pico-ampere (pA) (10 -12 ) , is proportional<br />

to the photon flux <strong>of</strong> X-rays.<br />

The electrode measuring the current generated by the camera is called the<br />

collector electrode. This electrode (anode?) is typically maintained at a<br />

potential close to the ground. The other electrode (cathode?) is called the<br />

high-voltage electrode, and must be maintained at a positive (?) voltage (to<br />

collect positive charges) or negative (to collect negative charges). These<br />

electrodes are fixed inside the chamber through electrical insulators.<br />

Charlie Chong/ Fion Zhang<br />

http://lnls.cnpem.br/beamlines/xafs/equipments/ion-chambers/


The chamber can be sealed to use different gases at different pressures. The<br />

figure below represents a parallel plate chamber where radiation passes<br />

between the electrodes. There are two windows, one where the beam<br />

reaches the sensitive volume and the other where the beam exits the<br />

chamber. These windows should be composed <strong>of</strong> a material <strong>of</strong> low atomic<br />

number and should be thin, so not to reduce the intensity <strong>of</strong> radiation. Note<br />

that this type <strong>of</strong> chamber is not stopping the X-ray beam.<br />

Charlie Chong/ Fion Zhang<br />

http://lnls.cnpem.br/beamlines/xafs/equipments/ion-chambers/


Schematic diagram <strong>of</strong> an ionization chamber with parallel plates.<br />

Charlie Chong/ Fion Zhang<br />

http://lnls.cnpem.br/beamlines/xafs/equipments/ion-chambers/


The Ionization Chamber is the simplest <strong>of</strong> all gas-filled radiation<br />

detectors, and is widely used for the detection and measurement <strong>of</strong> certain<br />

types <strong>of</strong> ionizing radiation; X-rays, gamma rays and beta particles.<br />

Conventionally, the term "ionization chamber" is used exclusively to describe<br />

those detectors which collect all the charges created by direct ionization<br />

within the gas through the application <strong>of</strong> an electric field.<br />

It only uses the discrete charges created by each interaction between the<br />

incident radiation and the gas, and does not involve the gas multiplication<br />

mechanisms used by other radiation instruments, such as the Geiger-Müller<br />

counter or the proportional counter.<br />

Ion chambers have a good uniform response to radiation over a wide range <strong>of</strong><br />

energies and are the preferred means <strong>of</strong> measuring high levels <strong>of</strong> gamma<br />

radiation. They are widely used in the nuclear power industry, research labs,<br />

radiography, radiobiology, and environmental monitoring.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Ionization_chamber


The Ionization Chamber<br />

• Detectors which collect all the charges created by direct ionization within<br />

the gas through the application <strong>of</strong> an electric field.<br />

• It only uses the discrete charges created by each interaction between the<br />

incident radiation and the gas,<br />

• It does not involve the gas multiplication mechanisms used by other<br />

radiation instruments, such as the Geiger-Müller counter or the<br />

proportional counter.<br />

• Ion chambers have a good uniform response to radiation over a wide<br />

range <strong>of</strong> energies<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Ionization_chamber


The Ionization Chamber<br />

• It does not involve the gas multiplication mechanisms used by other<br />

radiation instruments, such as the Geiger-Müller counter or the<br />

proportional counter.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Ionization_chamber


Schematic diagram <strong>of</strong> parallel plate ion chamber, showing drift <strong>of</strong> ions.<br />

Electrons typically drift 1000 times faster than positive ions due to their much<br />

smaller mass.<br />

https://en.wikipedia.org/wiki/Ionization_chamber


Principle <strong>of</strong> operation<br />

An ionization chamber measures the charge from the number <strong>of</strong> ion pairs<br />

created within a gas caused by incident radiation. It consists <strong>of</strong> a gas-filled<br />

chamber with two electrodes; known as anode and cathode. The electrodes<br />

may be in the form <strong>of</strong> parallel plates (Parallel Plate Ionization Chambers:<br />

PPIC), or a cylinder arrangement with a coaxially located internal anode wire.<br />

coaxially located<br />

Parallel Plate<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Ionization_chamber


A voltage potential is applied between the electrodes to create an electric<br />

field in the fill gas. When gas between the electrodes is ionized by incident<br />

ionizing radiation, ion-pairs are created and the resultant positive ions and<br />

dissociated electrons move to the electrodes <strong>of</strong> the opposite polarity under<br />

the influence <strong>of</strong> the electric field. This generates an ionization current which is<br />

measured by an electrometer circuit. The electrometer must be capable <strong>of</strong><br />

measuring the very small output current which is in the region <strong>of</strong> femto<br />

amperes (10 -15 ) to pico amperes (10 -12 ) , depending on the chamber design,<br />

radiation dose and applied voltage.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Ionization_chamber


Each ion pair created deposits or removes a small electric charge to or from<br />

an electrode, such that the accumulated charge is proportional to the number<br />

<strong>of</strong> ion pairs created, and hence the radiation dose. This continual generation<br />

<strong>of</strong> charge produces an ionization current, which is a measure <strong>of</strong> the total<br />

ionizing dose entering the chamber. However, the chamber cannot<br />

discriminate between radiation types (beta or gamma) and cannot produce an<br />

energy spectrum <strong>of</strong> radiation.<br />

The electric field also enables the device to work continuously by mopping up<br />

electrons, which prevents the fill gas from becoming saturated, where no<br />

more ions could be collected, and by preventing the recombination <strong>of</strong> ion<br />

pairs, which would diminish the ion current.<br />

Current Mode<br />

This mode <strong>of</strong> operation is referred to as "current" mode, meaning that the<br />

output signal is a continuous current, and not a pulse output as in the cases<br />

<strong>of</strong> the Geiger-Müller tube or the proportional counter.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Ionization_chamber


Referring to the accompanying ion pair collection graph, it can be seen that in<br />

the "ion chamber" operating region the collection <strong>of</strong> ion pairs is effectively<br />

constant over a range <strong>of</strong> applied voltage, as due to its relatively low electric<br />

field strength the ion chamber does not have any "multiplication effect". This<br />

is in distinction to the Geiger-Müller tube or the proportional counter whereby<br />

secondary electrons, and ultimately multiple avalanches, greatly amplify the<br />

original ion-current charge.<br />

Plot <strong>of</strong> ion current against voltage for a wire cylinder gaseous radiation<br />

detector. The ion chamber uses the lowest usable detection region.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Ionization_chamber


Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Ionization_chamber


Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Ionization_chamber


Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Ionization_chamber


Chamber types and construction<br />

The following chamber types are commonly used.<br />

Free-air chamber<br />

This is a chamber freely open to atmosphere, where the fill gas is ambient air.<br />

The domestic smoke detector is a good example <strong>of</strong> this, where a natural flow<br />

<strong>of</strong> air through the chamber is necessary so that smoke particles can be<br />

detected by the change in ion current. Other examples are applications where<br />

the ions are created outside the chamber but are carried in by a forced flow <strong>of</strong><br />

air or gas.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Ionization_chamber


Chamber pressure<br />

■ Vented chamber<br />

These chambers are normally cylindrical and operate at atmospheric<br />

pressure, but to prevent ingress <strong>of</strong> moisture a filter containing a desiccant is<br />

installed in the vent line. This is to stop moisture building up in the interior <strong>of</strong><br />

the chamber, which would otherwise be introduced by the "pump" effect <strong>of</strong><br />

changing atmospheric air pressure. These chambers have a cylindrical body<br />

made <strong>of</strong> aluminium or plastic a few millimetres thick. The material is selected<br />

to have an atomic number similar to that <strong>of</strong> air so that the wall is said to be<br />

"air equivalent" over a range <strong>of</strong> radiation beam energies. This has the effect<br />

<strong>of</strong> ensuring the gas in the chamber is acting as though it were a portion <strong>of</strong> an<br />

infinitely large gas volume, and increases the accuracy by reducing<br />

interactions <strong>of</strong> gamma with the wall material. The higher the atomic number <strong>of</strong><br />

the wall material, the greater the chance <strong>of</strong> interaction. The wall thickness is a<br />

trade-<strong>of</strong>f between maintaining the air effect with a thicker wall, and increasing<br />

sensitivity by using a thinner wall.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Ionization_chamber


These chambers <strong>of</strong>ten have an end window made <strong>of</strong> material thin enough,<br />

such as mylar, so that beta particles can enter the gas volume. Gamma<br />

radiation enters both through the end window and the side walls. For handheld<br />

instruments the wall thickness is made as uniform as possible to reduce<br />

photon directionality though any beta window response is obviously highly<br />

directional. Vented chambers are susceptible to small changes in efficiency<br />

with air pressure and correction factors can be applied for very accurate<br />

measurement applications.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Ionization_chamber


■ Sealed low pressure chamber<br />

These are similar in construction to the vented chamber but are sealed and<br />

operate at or around atmospheric pressure. They contain a special fill gas to<br />

improve detection efficiency as free electrons are easily captured in air-filled<br />

vented chambers by neutral oxygen which is electronegative, to form negative<br />

ions (?) . These chambers also have the advantage <strong>of</strong> not requiring a vent<br />

and desiccant. The beta end window limits the differential pressure from<br />

atmospheric pressure that can be tolerated, and common materials are<br />

stainless steel or titanium with a typical thickness <strong>of</strong> 25 µm.<br />

■ High pressure chamber<br />

The efficiency <strong>of</strong> the chamber can be further increased by the use <strong>of</strong> a high<br />

pressure gas. Typically a pressure <strong>of</strong> 8-10 atmospheres can be used, and<br />

various noble gases are employed. The higher pressure results in a greater<br />

gas density and thereby a greater chance <strong>of</strong> collision with the fill gas and ion<br />

pair creation by incident radiation. Because <strong>of</strong> the increased wall thickness<br />

required to withstand this high pressure, only gamma radiation can be<br />

detected. These detectors are used in survey meters and for environmental<br />

monitoring.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Ionization_chamber


Instrument types<br />

Ion chambers are widely used in hand held radiation survey meters to<br />

measure beta and gamma radiation. They are particularly preferred for high<br />

dose rate measurements and for gamma radiation they give good accuracy<br />

for energies above 50-100 keV.<br />

There are two basic configurations; the "integral" unit with the chamber and<br />

electronics in the same case, and the "two-piece" instrument which has a<br />

separate ion chamber probe attached to the electronics module by a flexible<br />

cable.<br />

The chamber <strong>of</strong> the integral instrument is generally at the front <strong>of</strong> the case<br />

facing downwards, and for beta/gamma instruments there is a window in the<br />

bottom <strong>of</strong> the casing. This usually has a sliding shield which enables<br />

discrimination between gamma and beta radiation. The operator closes the<br />

shield to exclude beta, and can thereby calculate the rate <strong>of</strong> each radiation<br />

type.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Ionization_chamber


Some hand held instruments generate audible clicks similar to that produced<br />

by a G-M counter to assist operators, who use the audio feedback in radiation<br />

survey and contamination checks. As the ion chamber works in current mode,<br />

not pulse mode, this is synthesised from the radiation rate.<br />

Installed<br />

For industrial process measurements and interlocks with sustained high<br />

radiation levels, the ion chamber is the preferred detector. In these<br />

applications only the chamber is situated in the measurement area, and the<br />

electronics are remotely situated to protect them from radiation and<br />

connected by a cable. Installed instruments can be used for measuring<br />

ambient gamma for personnel protection and normally sound an alarm above<br />

a preset rate, though the Geiger-Müller tube instrument is generally preferred<br />

where high levels <strong>of</strong> accuracy are not required.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Ionization_chamber


Hand-held integral ion chamber survey meter in use<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Ionization_chamber


View <strong>of</strong> sliding beta shield on integral hand held instrument<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Ionization_chamber


General precautions in use<br />

Moisture is the main problem that affects the accuracy <strong>of</strong> ion chambers. The<br />

chamber's internal volume must be kept completely dry, and the vented type<br />

uses a desiccant to help with this.[3] Because <strong>of</strong> the very low currents<br />

generated, any stray leakage current must be kept to a minimum in order to<br />

preserve accuracy. Invisible hygroscopic moisture on the surface <strong>of</strong> cable<br />

dielectrics and connectors can be sufficient to cause a leakage current which<br />

will swamp any radiation-induced ion current. This requires scrupulous<br />

cleaning <strong>of</strong> the chamber, its terminations and cables, and subsequent drying<br />

in an oven. "Guard rings" are generally used as a design feature on higher<br />

voltage tubes to reduce leakage through or along the surface <strong>of</strong> tube<br />

connection insulators which can require a resistance in the order <strong>of</strong> 10 13 Ω.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Ionization_chamber


For industrial applications with remote electronics, the ion chamber is housed<br />

in a separate enclosure which provides mechanical protection and contains a<br />

desiccant to remove moisture which could affect the termination resistance.<br />

In installations where the chamber is a long distance from the measuring<br />

electronics, readings can be affected by external electromagnetic radiation<br />

acting on the cable. To overcome this a local converter module is <strong>of</strong>ten used<br />

to translate the very low ion chamber currents to a pulse train or data signal<br />

related to the incident radiation. These are immune to electromagnetic effects.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Ionization_chamber


Applications<br />

Nuclear industry<br />

Ionization chambers are widely used in the nuclear industry as they provide<br />

an output that is proportional to radiation dose. They find wide use in<br />

situations where a constant high dose rate is being measured as they have a<br />

greater operating lifetime than standard Geiger-Müller tubes, which suffer<br />

from gas break down and are generally limited to a life <strong>of</strong> about 10 11 count<br />

events. Additionally, the Geiger-Müller tube cannot operate above about 10 4<br />

counts per second, due to dead time effects, whereas there is no similar<br />

limitation on the ion chamber.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Ionization_chamber


Keywords:<br />

• Ionization Chamber provides an output that is proportional to radiation<br />

dose.<br />

• Geiger-Müller tubes, which suffer from gas break down and are generally<br />

limited to a life <strong>of</strong> about 10 11 count events.<br />

• Geiger-Müller tube cannot operate above about 10 4 counts per second<br />

(10 4 N·s -1 ) , due to dead time effects, whereas there is no similar limitation<br />

on the ion chamber.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Ionization_chamber


Smoke detectors<br />

The ionization chamber has found wide and beneficial use in smoke detectors.<br />

In a smoke detector, ambient air is allowed to freely enter the ionization<br />

chamber. The chamber contains a small amount <strong>of</strong> americium-241, which is<br />

an emitter <strong>of</strong> alpha particles which produce a constant ion current. If smoke<br />

enters the detector, it disrupts this current because ions strike smoke particles<br />

and are neutralized. This drop in current triggers the alarm. The detector also<br />

has a reference chamber which is sealed but is ionized in the same way.<br />

Comparison <strong>of</strong> the ion currents in the two chambers allows compensation for<br />

changes due to air pressure, temperature, or the ageing <strong>of</strong> the source.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Ionization_chamber


Medical radiation measurement<br />

In medical physics and radiotherapy, ionization chambers are used to ensure<br />

that the dose delivered from a therapy unit or radiopharmaceutical is what is<br />

intended. The devices used for radiotherapy are called "reference<br />

dosimeters", while those used for radiopharmaceuticals are called<br />

radioisotope dose calibrators. A chamber will have a calibration factor<br />

established by a national standards laboratory such as ARPANSA in Australia<br />

or the NPL in the UK, or will have a factor determined by comparison against<br />

a transfer standard chamber traceable to national standards at the user's site.<br />

Guidance on application use<br />

In the United Kingdom the HSE has issued a user guide on selecting the<br />

correct radiation measurement instrument for the particular application<br />

concerned. This covers all radiation instrument technologies, and is a useful<br />

comparative guide to the use <strong>of</strong> ion chamber instruments.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Ionization_chamber


Charlie Chong/ Fion Zhang<br />

http://www.world-nuclear-university.org/imis20/wnu/default.aspx


Charlie Chong/ Fion Zhang<br />

http://www.world-nuclear-university.org/imis20/wnu/default.aspx


The Geiger counter is an instrument used for measuring ionizing<br />

radiation used widely in such applications as radiation dosimetry, radiological<br />

protection, experimental physics and the nuclear industry.<br />

It detects ionizing radiation such as alpha particles, beta particles and gamma<br />

rays using the ionization effect produced in a Geiger–Müller tube; which gives<br />

its name to the instrument. In wide and prominent use as a hand-held<br />

radiation survey instrument, it is perhaps one <strong>of</strong> the world's best-known<br />

radiation detection instruments.<br />

The original detection principle was discovered in 1908, but it was not until<br />

the development <strong>of</strong> the Geiger-Müller tube in 1928 that the Geiger-Müller<br />

counter became a practical instrument. Since then it has been very popular<br />

due to its robust sensing element and relatively low cost.<br />

However, there are limitations in measuring high radiation rates and the<br />

energy <strong>of</strong> incident radiation.<br />

Charlie Chong/ Fion Zhang


A "two-piece" bench type Geiger–Müller counter with end-window detector<br />

Charlie Chong/ Fion Zhang


Schematic <strong>of</strong> a Geiger counter using an "end window" tube for low<br />

penetration radiation. A loudspeaker is also used for indication<br />

Charlie Chong/ Fion Zhang


Principle <strong>of</strong> operation<br />

A Geiger counter consists <strong>of</strong> a Geiger-Müller tube, the sensing element which<br />

detects the radiation, and the processing electronics, which displays the<br />

result.<br />

The Geiger-Müller tube is filled with an inert gas such as helium, neon, or<br />

argon at low pressure, to which a high voltage is applied.<br />

The tube briefly conducts electrical charge when a particle or photon <strong>of</strong><br />

incident radiation makes the gas conductive by ionization. The ionization is<br />

considerably amplified within the tube by the Townsend discharge effect to<br />

produce an easily measured detection pulse, which is fed to the processing<br />

and display electronics. This large pulse from the tube makes the G-M<br />

counter relatively cheap to manufacture, as the subsequent electronics is<br />

greatly simplified. The electronics also generates the high voltage, typically<br />

400–600 volts, that has to be applied to the Geiger-Müller tube to enable its<br />

operation.<br />

Charlie Chong/ Fion Zhang


Readout<br />

There are two types <strong>of</strong> radiation readout; counts or radiation dose.<br />

The counts display is the simplest and is the number <strong>of</strong> ionizing events<br />

displayed either as a count rate, commonly "counts per second", or as a total<br />

over a set time period (an integrated total). The counts readout is normally<br />

used when alpha or beta particles are being detected. More complex to<br />

achieve is a display <strong>of</strong> radiation dose rate, displayed in a unit such as the<br />

sievert which is normally used for measuring gamma or X-ray dose rates. A<br />

G-M tube can detect the presence <strong>of</strong> radiation, but not its energy which<br />

influences the radiation's ionising effect. Consequently, instruments<br />

measuring dose rate require the use <strong>of</strong> an energy compensated G-M tube, so<br />

that the dose displayed relates to the counts detected. The electronics will<br />

apply known factors to make this conversion, which is specific to each<br />

instrument and is determined by design and calibration.<br />

The readout can be analog or digital, and increasingly, modern instruments<br />

are <strong>of</strong>fering serial communications with a host computer or network.<br />

Charlie Chong/ Fion Zhang


There is usually an option to produce audible clicks representing the number<br />

<strong>of</strong> ionization events detected. This is the distinctive sound normally<br />

associated with hand held or portable Geiger counters. The purpose <strong>of</strong> this is<br />

to allow the user to concentrate on manipulation <strong>of</strong> the instrument whilst<br />

retaining auditory feedback on the radiation rate.<br />

Limitations<br />

There are two main limitations <strong>of</strong> the Geiger counter. Because the output<br />

pulse from a Geiger-Müller tube is always the same magnitude regardless <strong>of</strong><br />

the energy <strong>of</strong> the incident radiation, the tube cannot differentiate between<br />

radiation types. A further limitation is the inability to measure high radiation<br />

rates due to the "dead time" <strong>of</strong> the tube. This is an insensitive period after<br />

each ionization <strong>of</strong> the gas during which any further incident radiation will not<br />

result in a count, and the indicated rate is therefore lower than actual.<br />

Typically the dead time will reduce indicated count rates above about 10 4 to<br />

10 5 counts per second depending on the characteristic <strong>of</strong> the tube being used.<br />

Whilst some counters have circuitry which can compensate for this, for<br />

accurate measurements ion chamber instruments are preferred for high<br />

radiation rates.<br />

Charlie Chong/ Fion Zhang


For accurate measurements ion chamber instruments are preferred for<br />

high radiation rates.<br />

Charlie Chong/ Fion Zhang


Ionization Chamber<br />

Charlie Chong/ Fion Zhang


Geiger Muller Counter<br />

Charlie Chong/ Fion Zhang


G-M counter with pancake type probe<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger_counter


Laboratory use <strong>of</strong> a G-M counter with end window probe to measure beta<br />

radiation from a radioactive source<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger_counter


Types and applications<br />

The application and use <strong>of</strong> a Geiger counter is dictated entirely by the design<br />

<strong>of</strong> the tube, <strong>of</strong> which there are a great many, but they can be generally<br />

categorised as "end-window", or windowless "thin-walled" or "thick-walled",<br />

and sometimes hybrids <strong>of</strong> these types.<br />

<strong>Part</strong>icle detection<br />

The first historical uses <strong>of</strong> the Geiger principle were for the detection <strong>of</strong> alpha<br />

and beta particles, and the instrument is still used for this purpose today. For<br />

alpha particles and low energy beta particles the "end-window" type <strong>of</strong> G-M<br />

tube has to be used as these particles have a limited range even in free air,<br />

and are easily stopped by a solid material. Therefore the tube requires a<br />

window which is thin enough to allow as many as possible <strong>of</strong> these particles<br />

through to the fill gas. The window is usually made <strong>of</strong> mica with a density <strong>of</strong><br />

about 1.5 - 2.0 mg/cm 2 .<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger_counter


Alpha particles have the shortest range, and to detect these the window<br />

should ideally be within 10mm <strong>of</strong> the radiation source due to alpha particle<br />

attenuation in free air. However, the G-M tube produces a pulse output which<br />

is the same magnitude for all detected radiation, so a Geiger counter with an<br />

end window tube cannot distinguish between alpha and beta particles. A<br />

skilled operator can use distance to differentiate alpha and high energy beta,<br />

but with the detector in close contact with the radiation source the types are<br />

indistinguishable. The "pancake" Geiger-Muller detector is a variant <strong>of</strong> the<br />

end window probe, but designed with a larger detection area to make<br />

checking quicker. However the pressure <strong>of</strong> the atmosphere against the low<br />

pressure <strong>of</strong> the fill gas limits the window size due to the limited strength <strong>of</strong> the<br />

window membrane.<br />

High energy beta particles can also be detected by a thin-walled<br />

"windowless" G-M tube, which has no end window. Although the tube walls<br />

have a greater stopping power than a thin end window, they still allow these<br />

more energetic particles to reach the fill gas.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger_counter


End-window G-M detectors are still used as a general purpose portable<br />

radioactive contamination measurement and detection instrument, owing to<br />

their relatively low cost, robustness and their relatively high detection<br />

efficiency; particularly with high energy beta particles.<br />

However for discrimination between alpha and beta particles or provision <strong>of</strong><br />

particle energy information, (1) scintillation counters or (2) proportional<br />

counters should be used. Those instrument types are manufactured with<br />

much larger detector areas, which means that checking for surface<br />

contamination is quicker than with a G-M instrument.<br />

Keywords:<br />

However for discrimination between alpha and beta particles or provision <strong>of</strong><br />

particle energy information, (1) scintillation counters or (2) proportional<br />

counters should be used.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger_counter


Gamma and X-ray detection<br />

Geiger counters are widely used to detect gamma radiation, and for this the<br />

windowless tube is used. However, efficiency is generally low due to the poor<br />

interaction <strong>of</strong> gamma rays compared with alpha and beta particles. For<br />

instance, a chrome steel G-M tube is only about 1% efficient over a wide<br />

range <strong>of</strong> energies.<br />

The article on the Geiger-Muller tube carries a more detailed account <strong>of</strong> the<br />

techniques used to detect photon radiation. For high energy gamma it largely<br />

relies on interaction <strong>of</strong> the photon radiation with the tube wall material, usually<br />

1–2 mm <strong>of</strong> chrome steel on a "thick-walled" tube, to produce electrons within<br />

the wall which can enter and ionize the fill gas. This is necessary as the low<br />

pressure gas in the tube has little interaction with high energy gamma<br />

photons. However, for low energy photons there is greater gas interaction and<br />

the direct gas ionisation effect increases. With decreasing energy the wall<br />

effect gives way to a combination <strong>of</strong> wall effect and direct ionisation, until<br />

direct gas ionisation dominates. Due to the variance in response to different<br />

photon energies, windowless tubes employ what is known as "energy<br />

compensation" which attempts to compensate for these variations over a<br />

large energy range.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger_counter


Low energy photon radiation such as low energy X rays or gamma rays<br />

interacts better with the fill gas. Consequently a typical design for low energy<br />

photon detection for these is a long tube with a thin wall or with an end<br />

window. The tube has a larger gas volume than a steel walled tube to give an<br />

increased chance <strong>of</strong> particle interaction.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger_counter


<strong>Neutron</strong> detection<br />

A variation <strong>of</strong> the Geiger tube is used to measure neutrons, where the gas<br />

used is boron trifluoride (BF 3 ) or helium-3 ( 3 He) and a plastic moderator is<br />

used to slow the neutrons. This creates an alpha particle inside the detector<br />

and thus neutrons can be counted.<br />

Geiger tube filled with BF 3 for detection <strong>of</strong> thermal neutrons<br />

10<br />

5 B + n → 7 3 Li + 4 2 α https://www.orau.org/PTP/collection/proportional%20counters/bf3info.htm<br />

3<br />

2 He + n → 3 1 Li + 1 1 P http://large.stanford.edu/courses/2012/ph241/lam1/<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger_counter


Boron trifluoride Detector<br />

This neutron detector was produced by 20th<br />

Century Electronics in England. The company<br />

began manufacturing BF 3 counters in the early<br />

1950s. It is approximately 16 1/2 inches long, 2<br />

inches in diameter, copper walled and filled with<br />

BF3. One end (towards the right in the above<br />

photo) has a threaded cap to protect the fragile<br />

glass insulator.<br />

The model number, marked on the wall <strong>of</strong> the<br />

tube, is 15EB70/50/G/UA0539. The EB refers to<br />

"enriched boron trifluoride." The 50 refers to the<br />

tube diameter, i.e., 50 mm.<br />

Charlie Chong/ Fion Zhang<br />

https://www.orau.org/PTP/collection/proportional%20counters/bf3twentiethlarge.htm


Gamma measurement—personnel protection and<br />

process control<br />

The term "Geiger counter" is commonly used to mean a hand-held survey<br />

type meter, however the Geiger principle is in wide use in installed "area<br />

gamma" alarms for personnel protection, and in process measurement and<br />

interlock applications. A Geiger tube is still the sensing device, but the<br />

processing electronics will have a higher degree <strong>of</strong> sophistication and<br />

reliability than that used in a hand held survey meter.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger_counter


Physical design<br />

For hand-held units there are two fundamental physical configurations: the<br />

"integral" unit with both detector and electronics in the same unit, and the<br />

"two-piece" design which has a separate detector probe and an electronics<br />

module connected by a short cable.<br />

The integral unit allows single-handed operation, so the operator can use the<br />

other hand for personal security in challenging monitoring positions, but the<br />

two piece design allows easier manipulation <strong>of</strong> the detector, and is commonly<br />

used for alpha and beta surface contamination monitoring where careful<br />

manipulation <strong>of</strong> the probe is required or the weight <strong>of</strong> the electronics module<br />

would make operation unwieldy. A number <strong>of</strong> different sized detectors are<br />

available to suit particular situations, such as placing the probe in small<br />

apertures or confined spaces.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger_counter


Gamma and X-Ray detectors generally use an "integral" design so the<br />

Geiger–Müller tube is conveniently within the electronics enclosure. This can<br />

easily be achieved because the casing usually has little attentuation, and is<br />

employed in ambient gamma measurements where distance from the source<br />

<strong>of</strong> radiation is not a significant factor. However, to facilitate more localised<br />

measurements such as "surface dose", the position <strong>of</strong> the tube in the<br />

enclosure is sometimes indicated by targets on the enclosure so an accurate<br />

measurement can be made with the tube at the correct orientation and a<br />

known distance from the surface.<br />

There is a particular type <strong>of</strong> gamma instrument known as a "hot spot" detector<br />

which has the detector tube on the end <strong>of</strong> a long pole or flexible conduit.<br />

These are used to measure high radiation gamma locations whilst protecting<br />

the operator by means <strong>of</strong> distance shielding.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger_counter


<strong>Part</strong>icle detection <strong>of</strong> alpha and beta can used in both integral and two-piece<br />

designs. A pancake probe (for alpha/beta) is generally used to increase the<br />

area <strong>of</strong> detection in two-piece instruments whilst being relatively light weight.<br />

In integral instruments using an end window tube there is a window in the<br />

body <strong>of</strong> the casing to prevent shielding <strong>of</strong> particles. There are also hybrid<br />

instruments which have a separate probe for particle detection and a gamma<br />

detection tube within the electronics module. The detectors are switchable by<br />

the operator, depending the radiation type that is being measured.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger_counter


Pancake G-M tube used for alpha and beta detection; the delicate mica<br />

window is usually protected by a mesh when fitted in an instrument.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger_counter


Guidance on application use[edit]<br />

In the United Kingdom the HSE has issued a user guidance note on selecting<br />

the best portable instrument type for the radiation measurement application<br />

concerned.[4][3] This covers all radiation protection instrument technologies<br />

and is a useful comparative guide to the use <strong>of</strong> G-M detectors. The guide<br />

does not recommend the G-M detector for mixed alpha and beta<br />

contamination detection, and they are only recommended as "satisfactory" for<br />

beta-only contamination. However for gamma and low-voltage X-rays they<br />

are recommended as the best instrument type.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger_counter


Use <strong>of</strong> a "hot spot" detector on a long pole to survey waste casks<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger_counter


G-M pancake detector feeding a microcontroller data-logger sending data to a<br />

PC via bluetooth. A radioactive rock was placed on top the G-M causing the<br />

graph to rise.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger_counter


G-M counters being used as gamma survey monitors, seeking radioactive<br />

satellite debris<br />

Charlie Chong/ Fion Zhang


Geiger–Müller tube<br />

The Geiger–Müller tube or G–M tube is the sensing element <strong>of</strong> the Geiger<br />

counter instrument used for the detection <strong>of</strong> ionizing radiation. It was named<br />

after Hans Geiger, who invented the principle in 1908, and Walther Müller,<br />

who collaborated with Geiger in developing the technique further in 1928 to<br />

produce a practical tube that could detect a number <strong>of</strong> different radiation<br />

types.<br />

It is a gaseous ionization detector and uses the Townsend avalanche<br />

phenomenon to produce an easily detectable electronic pulse from as little as<br />

a single ionising event due to a radiation particle. It is used for the detection <strong>of</strong><br />

gamma radiation, X-rays, and alpha and beta particles. It can also be adapted<br />

to detect neutrons. The tube operates in the "Geiger" region <strong>of</strong> ion pair<br />

generation. This is shown on the accompanying plot for gaseous detectors<br />

showing ion current against applied voltage.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


Whilst it is a robust and inexpensive detector, the G–M is:<br />

• unable to measure high radiation rates efficiently,<br />

• has a finite life in high radiation areas and<br />

• is unable to measure incident radiation energy, so no spectral information<br />

can be generated and there is no discrimination between radiation type.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


Plot <strong>of</strong> ion pair current against applied voltage for a cylindrical gaseous<br />

radiation detector with a central wire anode.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


Principle <strong>of</strong> operation<br />

The tube consists <strong>of</strong> a chamber filled with an inert gas at low-pressure (about<br />

0.1 atmosphere). The chamber contains two electrodes, between which there<br />

is a potential difference <strong>of</strong> several hundred volts. The walls <strong>of</strong> the tube are<br />

either metal or have their inside surface coated with a conductor to form the<br />

cathode, while the anode is a wire in the center <strong>of</strong> the chamber.<br />

several hundred volts<br />

0.1 atmosphere<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


When ionizing radiation strikes the tube, some molecules <strong>of</strong> the gas are<br />

ionized, either directly by the incident radiation or indirectly by means <strong>of</strong><br />

secondary electrons produced in the walls <strong>of</strong> the tube. This creates positively<br />

charged ions and electrons, known as “ion pairs”, in the fill gas.<br />

The strong electric field created by the tube's electrodes accelerates the<br />

positive ions towards the cathode and the electrons towards the anode. Close<br />

to the anode in the "avalanche region" the electrons gain sufficient energy to<br />

ionize additional gas molecules and create a large number <strong>of</strong> electron<br />

avalanches which spread along the anode and effectively throughout the<br />

avalanche region. This is the "gas multiplication" effect which gives the tube<br />

its key characteristic <strong>of</strong> being able to produce a significant output pulse from a<br />

single ionising event<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


If there were to be only one avalanche per original ionising event, then the<br />

number <strong>of</strong> excited molecules would be in the order <strong>of</strong> 10 6 to 10 8 . However the<br />

production <strong>of</strong> multiple avalanches results in an increased multiplication factor<br />

which can produce 10 9 to 10 10 ion pairs.<br />

Keypoint:<br />

Single event multiplication factor: 10 6 to 10 8<br />

Multiple event multiplication factor: 10 9 to 10 10<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


The creation <strong>of</strong> multiple avalanches is due to the production <strong>of</strong> UV photons in<br />

the original avalanche, which are not affected by the electric field and move<br />

laterally to the axis <strong>of</strong> the anode to instigate further ionising events by<br />

collision with gas molecules. These collisions produce further avalanches,<br />

which in turn produce more photons, and thereby more avalanches in a chain<br />

reaction which spreads laterally through the fill gas, and envelops the anode<br />

wire.<br />

The accompanying diagram shows this graphically. The speed <strong>of</strong> propagation<br />

<strong>of</strong> the avalanches is typically 2–4 cm per microsecond, so that for common<br />

sizes <strong>of</strong> tubes the complete ionisation <strong>of</strong> the gas around the anode takes just<br />

a few microseconds. This short, intense pulse <strong>of</strong> current can be measured as<br />

a count event in the form <strong>of</strong> a voltage pulse developed across an external<br />

electrical resistor. This can be in the order <strong>of</strong> volts, thus making further<br />

electronic processing simple.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


Visualisation <strong>of</strong> the spread <strong>of</strong> Townsend avalanches by means <strong>of</strong> UV photons.<br />

This mechanism allows a single ionising event to ionise all the gas<br />

surrounding the anode by triggering multiple avalanches.<br />

Spread <strong>of</strong> avalanches<br />

In a GM Tube<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


The discharge is terminated by the collective effect <strong>of</strong> the positive ions<br />

created by the avalanches. These ions have lower mobility than the free<br />

electrons due to their higher mass and remain in the area <strong>of</strong> the anode wire.<br />

This creates a "space charge" which counteracts the electric field which is<br />

necessary for continued avalanche generation.<br />

For a particular tube geometry and operating voltage this termination always<br />

occurs when a certain number <strong>of</strong> avalanches have been created, therefore<br />

the pulses from the tube are always <strong>of</strong> the same magnitude regardless <strong>of</strong> the<br />

energy <strong>of</strong> the initiating particle. Consequently, there is no radiation energy<br />

information in the pulses which means the Geiger–Muller tube cannot be<br />

used to generate spectral information about the incident radiation.<br />

Pressure <strong>of</strong> the fill gas is important in the generation <strong>of</strong> avalanches. Too low a<br />

pressure and the efficiency <strong>of</strong> interaction with incident radiation is reduced.<br />

Too high a pressure, and the “mean free path” for collisions between<br />

accelerated electrons and the fill gas is too small, and the electrons cannot<br />

gather enough energy between each collision to cause ionisation <strong>of</strong> the gas.<br />

The energy gained by electrons is proportional to the ratio “e/p”, where “e” is<br />

the electric field strength at that point in the gas, and “p” is the gas pressure.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


Detection <strong>of</strong> higher energy gamma in a thick-walled tube. Secondary<br />

electrons generated in the wall can reach the fill gas to produce avalanches.<br />

Multiple avalanches omitted for clarity<br />

Interaction <strong>of</strong><br />

gamma radiation<br />

with GM tube wall<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


Types <strong>of</strong> tube<br />

Broadly, there are two main types <strong>of</strong> Geiger tube construction.<br />

End window type<br />

For alpha particles, low energy beta particles, and low energy X-rays, the<br />

usual form is a cylindrical end-window tube. This type has a window at one<br />

end covered in a thin material through which low-penetrating radiation can<br />

easily pass. Mica is a commonly used material due to its low mass per unit<br />

area. The other end houses the electrical connection to the anode.<br />

Pancake tube<br />

Pancake G–M tube, the circular concentric anode can clearly be seen.<br />

The pancake tube is a variant <strong>of</strong> the end window tube, but which is designed<br />

for use for beta and gamma contamination monitoring. It has roughly the<br />

same sensitivity to particles as the end window type, but has a flat annular<br />

shape so the largest window area can be utilised with a minimum <strong>of</strong> gas<br />

space. Like the cylindrical end window tube, mica is a commonly used<br />

window material due to its low mass per unit area. The anode is normally<br />

multi-wired in concentric circles so it extends fully throughout the gas space.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


Windowless type<br />

This general type is distinct from the dedicated end window type, but has two<br />

main sub-types, which use different radiation interaction mechanisms to<br />

obtain a count.<br />

Thick walled<br />

A selection <strong>of</strong> thick walled G–M tubes for gamma detection. The largest has<br />

an energy compensation ring; the others are not energy compensated<br />

Used for high energy gamma detection, this type generally has an overall wall<br />

thickness <strong>of</strong> about 1-2 mm <strong>of</strong> chrome steel. Because most high energy<br />

gamma photons will pass through the low density fill gas without interacting,<br />

the tube uses the interaction <strong>of</strong> photons on the molecules <strong>of</strong> the wall material<br />

to produce high energy secondary electrons within the wall. Some <strong>of</strong> these<br />

electrons are produced close enough to the inner wall <strong>of</strong> the tube to escape<br />

into the fill gas. As soon as this happens the electron drifts to the anode and<br />

an electron avalanche occurs as though the free electron had been created<br />

within the gas. The avalanche is a secondary effect <strong>of</strong> a process that starts<br />

within the tube wall; the avalanche is not the effect <strong>of</strong> radiation directly on the<br />

gas itself.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


Thin walled<br />

Thin walled tubes are used for:<br />

high energy beta detection, where the beta enters via the side <strong>of</strong> the tube and<br />

interacts directly with the gas, but the radiation has to be energetic enough to<br />

penetrate the tube wall. Low energy beta, which would penetrate an end<br />

window, would be stopped by the tube wall.<br />

Low energy gamma and X-ray detection.<br />

The lower energy photons interact better with the fill gas so this design<br />

concentrates on increasing the volume <strong>of</strong> the fill gas by using a long thin<br />

walled tube and does not use the interaction <strong>of</strong> photons in the tube wall. The<br />

transition from thin walled to thick walled design takes place at the 300–400<br />

KeV energy levels. Above these levels thick walled designs are used, and<br />

beneath these levels the direct gas ionisation effect is predominant.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


Schematic <strong>of</strong> a Geiger counter using an "end window" tube for lowpenetrating<br />

radiation. A loudspeaker is also used for indication<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


Pancake G–M tube, the circular concentric anode can clearly be seen.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


A selection <strong>of</strong> thick walled G–M tubes for gamma detection. The largest has<br />

an energy compensation ring; the others are not energy compensated<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


<strong>Neutron</strong><br />

G–M tubes will not detect neutrons since these do not ionise the gas.<br />

However, neutron-sensitive tubes can be produced which either have the (1)<br />

inside <strong>of</strong> the tube coated with boron, or (2) the tube contains boron trifluoride<br />

or (3) helium-3 as the fill gas.<br />

The neutrons interact with the boron nuclei, producing alpha particles, or<br />

directly with the helium-3 nuclei producing hydrogen (proton) and tritium ions<br />

and electrons. These charged particles then trigger the normal avalanche<br />

process.<br />

10<br />

5 B + n → 7 3 Li + 4 2 α + 2e-<br />

3<br />

2 He + n → 1 1 H+ + 3 1 H + e-<br />

3<br />

2 He + n → 1 1 H + 3 1 H+ + e -<br />

Charlie Chong/ Fion Zhang<br />

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Gas mixtures<br />

The main component <strong>of</strong> the gas fill mixture is an inert gas such as helium,<br />

argon or neon, in some cases in a Penning mixture, and a "quench" gas <strong>of</strong> 5–<br />

10% <strong>of</strong> an organic vapor or a halogen gas to prevent multiple pulsing. The<br />

halogen-filled G–M tube was invented by Sidney H. Liebson in 1947 and has<br />

several advantages over the tubes with older organic mixtures. The halogen<br />

tube discharge takes advantage <strong>of</strong> a metastable state <strong>of</strong> the inert gas atom to<br />

more-readily ionize a halogen molecule than an organic vapor, enabling the<br />

tube to operate at much lower voltages, typically 400–600 volts instead <strong>of</strong><br />

900–1200 volts. It also has a longer life than tubes quenched with organic<br />

compounds, because the halogen ions can recombine while the organic<br />

vapor is gradually destroyed by the discharge process (giving the latter a life<br />

<strong>of</strong> around 10 8 events). For these reasons, the halogen-filled tube is now the<br />

most common.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


Geiger plateau<br />

The Geiger plateau is the voltage range in which the GM tube operates in its<br />

correct mode. If a G–M tube is exposed to a steady radiation source and the<br />

applied voltage is increased from zero, it follows the plot <strong>of</strong> ion current shown<br />

in this article. In the "Geiger region" the gradient flattens; this is the Geiger<br />

plateau.<br />

Depending on the characteristics <strong>of</strong> the specific tube (manufacturer, size, gas<br />

type, etc.) the voltage range <strong>of</strong> the plateau will vary. In this region, the<br />

potential difference in the counter is strong enough to allow the creation <strong>of</strong><br />

multiple avalanches.<br />

A lower voltage is not sufficient to cause a complete discharge along the<br />

anode, and individual Townsend avalanches are the result, and the tube tries<br />

to act as a proportional counter. If the applied voltage is higher than the<br />

plateau, a continuous glow discharge is formed and the tube cannot detect<br />

radiation.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


The plateau has a slight slope caused by increasing sensitivity to low energy<br />

radiation as the voltage increases. Normally when a particle ionizes gas<br />

atoms, complete ionization <strong>of</strong> the gas occurs. But for a low energy particle, it<br />

is possible that the kinetic energy in addition to the potential energy <strong>of</strong> the<br />

voltage are insufficient for the avalanche to occur and the ion recombines. As<br />

applied voltage rises, the threshold for the minimum radiation response falls,<br />

thus the counter's sensitivity rises; giving rise to the slope.<br />

The counting rate for a given radiation source varies slightly as the applied<br />

voltage is varied and to prevent this, a regulated voltage is used. However, it<br />

is normal to operate the tube in the middle <strong>of</strong> the plateau to allow for<br />

variations in the tube supply voltage.<br />

Keypoints:<br />

In Geiger Muller counter the ionization is by Multiple Avalanches<br />

Charlie Chong/ Fion Zhang<br />

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Quenching and dead time<br />

The ideal G–M tube should produce a single pulse on entry <strong>of</strong> a single<br />

ionising particle. It must not give any spurious pulses, and must recover<br />

quickly to the passive state.<br />

Unfortunately for these requirements, when positive argon ions reach the<br />

cathode and become neutral argon atoms again by obtaining electrons from it,<br />

the atoms can acquire their electrons in enhanced energy levels. These<br />

atoms then return to their ground state by emitting photons which can in turn<br />

produce further ionisation and hence cause spurious secondary pulse<br />

discharges. If nothing were done to counteract it, ionisation could even<br />

escalate, causing a so-called current "avalanche" which if prolonged could<br />

damage the tube. Some form <strong>of</strong> quenching <strong>of</strong> the ionisation is therefore<br />

essential.<br />

Charlie Chong/ Fion Zhang<br />

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The disadvantage <strong>of</strong> quenching is that for a short time after a discharge pulse<br />

has occurred (the so-called dead time, which is typically 50–100<br />

microseconds), the tube is rendered insensitive and is thus temporarily<br />

unable to detect the arrival <strong>of</strong> any new ionising particle. This effectively<br />

causes a loss <strong>of</strong> counts at sufficiently high count rates and limits the G–M<br />

tube to a count rate <strong>of</strong> between 10 4 to 10 5 counts per second, depending on<br />

its characteristic. A consequence <strong>of</strong> this is that ion chamber instruments were<br />

sometimes preferred for higher count rates, however the modern application<br />

<strong>of</strong> "electronic quenching" (see below) can extend this upper limit considerably.<br />

Charlie Chong/ Fion Zhang<br />

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Chemical quenching<br />

Self-quenching or internal-quenching tubes stop the discharge without<br />

external assistance, by means <strong>of</strong> the addition <strong>of</strong> a small amount <strong>of</strong> a<br />

polyatomic organic vapor such as butane or ethanol, or alternatively a<br />

halogen such as bromine or chlorine.<br />

If a poor diatomic gas quencher is introduced to the tube, the positive argon<br />

ions, during their motion toward the cathode, would have multiple collisions<br />

with the quencher gas molecules and transfer their charge and some energy<br />

to them. Thus, neutral argon atoms would be produced and the quencher gas<br />

ions in their turn would reach the cathode, gain electrons there from, and<br />

move into excited states which would decay by photon emission, producing<br />

tube discharge. However, effective quencher molecules, when excited, lose<br />

their energy not by photon emission, but by dissociation into neutral quencher<br />

molecules. No spurious pulses are thus produced.<br />

Charlie Chong/ Fion Zhang<br />

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External quenching, sometimes also called "active quenching" or "electronic<br />

quenching", uses high speed control electronics to rapidly remove and reapply<br />

the high voltage between the electrodes after each discharge peak.<br />

This results in faster quenching <strong>of</strong> the tube than using the effect <strong>of</strong> gas alone,<br />

and allows for greatly increased tube lifetimes.<br />

A technique known as "time-to-first-count" is sometimes used in conjunction<br />

with this to greatly increase the maximum count rate <strong>of</strong> the tube.<br />

Charlie Chong/ Fion Zhang<br />

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Dead time and recovery time in a Geiger Muller tube.[4] The tube can<br />

produce no further pulses during the dead time, and is able to produce only<br />

pulses <strong>of</strong> limited height until the recovery time elapses.<br />

Charlie Chong/ Fion Zhang<br />

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Fold-back<br />

One consequence <strong>of</strong> the dead time effect is the possibility <strong>of</strong> a high count rate<br />

continually triggering the tube before the recovery time has elapsed. This may<br />

produce pulses too small for the counting electronics to detect and lead to the<br />

very undesirable situation whereby a G–M counter in a very high radiation<br />

field is falsely indicating a low level. This phenomenon is known as "foldback".<br />

An industry rule <strong>of</strong> thumb is that the discriminator circuit receiving the<br />

output from the tube should detect down to 1/10 <strong>of</strong> the magnitude <strong>of</strong> a normal<br />

pulse to guard against this. Additionally the circuit should detect when "pulse<br />

pile-up " has occurred, where the apparent anode voltage has moved to a<br />

new dc level through the combination <strong>of</strong> high pulse count and noise. The<br />

electronic design <strong>of</strong> Geiger–Muller counters must be able to detect this<br />

situation and give an alarm; it is normally done by setting a threshold for<br />

excessive tube current.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


Detection efficiency<br />

The efficiency <strong>of</strong> detection <strong>of</strong> a G–M tube varies with the type <strong>of</strong> incident<br />

radiation. Tubes with thin end windows have very high efficiencies (can be<br />

nearly 100%) for high energy beta, though this drops <strong>of</strong>f as the beta energy<br />

decreases due to attenuation by the window material. Alpha particles are also<br />

attenuated by the window. As alpha particles have a maximum range <strong>of</strong> less<br />

than 50 mm in air, the detection window should be as close as possible to the<br />

source <strong>of</strong> radiation. The attenuation <strong>of</strong> the window adds to the attenuation <strong>of</strong><br />

air, so the window should have a density as low as 1.5 to 2.0 mg/cm 2 to give<br />

an acceptable level <strong>of</strong> detection efficiency. The article on stopping power<br />

explains in more detail the ranges for particles types <strong>of</strong> various energies. The<br />

counting efficiency <strong>of</strong> photon radiation (gamma and X-rays above 25 keV)<br />

depends on the efficiency <strong>of</strong> radiation interaction in the tube wall, which<br />

increases with the atomic number <strong>of</strong> the wall material. Chromium iron is a<br />

commonly used material, which gives an efficiency <strong>of</strong> about 1% over a wide<br />

range <strong>of</strong> energies.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


Energy compensation<br />

If a G–M tube is to be used for gamma or X-ray dosimetry measurements the<br />

energy <strong>of</strong> incident radiation, which affects the ionising effect, must be taken<br />

into account. However individual pulses from a G–M tube do not carry any<br />

energy information. A solution is to assign a radiation dose to each counting<br />

event, so the tube characteristic relates the number <strong>of</strong> counts to the intensity<br />

<strong>of</strong> incident radiation.<br />

At low photon energy levels the response increases as low energy photons<br />

have a greater interaction with the fill gas than high energy photons. The tube<br />

therefore has an increased response for radiation which has a lower dose<br />

rate, and a correction must be applied to prevent an incorrect high reading for<br />

low energy photons. This discrepancy can be 2–3 times greater or more, and<br />

for a thick-walled tube usually peaks at about 60 keV, where radiation<br />

interactions with the gas are still large, but the shielding effect <strong>of</strong> the wall has<br />

not become dominant.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


This correction is achieved by 'energy compensation' <strong>of</strong> the tube, which<br />

modifies the number <strong>of</strong> count events in accordance with the energy <strong>of</strong> the<br />

incident radiation by using an external filter collar <strong>of</strong> energy absorbing<br />

material. The collar has an increased attenuation <strong>of</strong> low energy gamma, and<br />

so compensates for the increased energy response <strong>of</strong> the naked tube at<br />

those levels. The aim is that sensitivity/energy characteristic <strong>of</strong> the tube<br />

should be matched by the absorption/energy characteristic <strong>of</strong> the filter. This<br />

results in a more uniform response over the stated range <strong>of</strong> detection<br />

energies for the tube.<br />

Lead and tin are commonly used materials, and a simple filter effective above<br />

150 keV can be made using a continuous collar along the length <strong>of</strong> the tube.<br />

However, at lower energy levels this attenuation can become too great, so air<br />

gaps are left in the collar to allow low energy radiation to have a greater effect.<br />

In practice, compensation filter design is an empirical compromise to produce<br />

an acceptably uniform response, and a number <strong>of</strong> different materials and<br />

geometries are used to obtain the required correction.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


Comparative response curves for GM tube with and without radiation energy<br />

compensation<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


Thin-walled glass G–M tube showing a spiral wire cathode. The tape bands<br />

are for fixing compensating rings<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


Thin-walled glass G–M tube showing a spiral wire cathode. The tape bands<br />

are for fixing compensating rings<br />

Charlie Chong/ Fion Zhang


Thin-walled glass G–M tube showing a spiral wire cathode. The tape bands<br />

are for fixing compensating rings<br />

Charlie Chong/ Fion Zhang


Thin-walled glass G–M tube with energy compensating rings fitted. The<br />

complete assembly fits into the aluminium housing.<br />

energy compensating rings- Absorb the<br />

low energy photon & enhanced high<br />

energy photon by production <strong>of</strong> secondary<br />

electron at ring internal<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube


Thin-walled glass G–M tube with energy compensating rings fitted. The<br />

complete assembly fits into the aluminium housing.<br />

Charlie Chong/ Fion Zhang


Thin-walled glass G–M tube with energy compensating rings fitted. The<br />

complete assembly fits into the aluminium housing.<br />

Charlie Chong/ Fion Zhang


Proportional counter<br />

The proportional counter is a type <strong>of</strong> gaseous ionization detector device used<br />

to measure particles <strong>of</strong> ionizing radiation.<br />

The key feature is its ability to measure the energy <strong>of</strong> incident radiation, by<br />

producing a detector output that is proportional to the radiation energy; hence<br />

the detector's name. It is widely used where energy levels <strong>of</strong> incident<br />

radiation must be known, such as in the discrimination between alpha and<br />

beta particles, or accurate measurement <strong>of</strong> X-ray radiation dose. A<br />

proportional counter uses a combination <strong>of</strong> the mechanisms <strong>of</strong> a Geiger–<br />

Müller tube and an ionization chamber, and operates in an intermediate<br />

voltage region between these. The accompanying plot shows the proportional<br />

counter operating voltage region for a co-axial cylinder arrangement.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Proportional_counter


Plot <strong>of</strong> variation <strong>of</strong> ion pair current against applied voltage for a wire cylinder<br />

gaseous radiation detector.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Proportional_counter


Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Proportional_counter


Operation<br />

In a proportional counter the fill gas <strong>of</strong> the chamber is an inert gas which is<br />

ionised by incident radiation, and a quench gas to ensure each pulse<br />

discharge terminates; a common mixture is 90% argon, 10% methane, known<br />

as P-10.<br />

What is P10:<br />

Proportional counter with 90% Argon (inert gas) with 10% quenched gas<br />

(10% methane)<br />

An ionising particle entering the gas collides with an atom <strong>of</strong> the inert gas and<br />

ionises it to produce an electron and a positively charged ion, commonly<br />

known as an "ion pair". As the charged particle travels through the chamber it<br />

leaves a trail <strong>of</strong> ion pairs along its trajectory, the number <strong>of</strong> which is<br />

proportional to the energy <strong>of</strong> the particle if it is fully stopped within the gas.<br />

Typically a 1 MeV stopped particle will create about 30,000 ion pairs.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Proportional_counter


What is P10:<br />

Proportional counter with 90% Argon (inert gas) with 10% quenched gas<br />

(10% methane)<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Proportional_counter


The chamber geometry and the applied voltage is such that in most <strong>of</strong> the<br />

chamber the electric field strength is low and the chamber acts as an ion<br />

chamber. However, the field is strong enough to prevent re-combination <strong>of</strong><br />

the ion pairs and causes positive ions to drift towards the cathode and<br />

electrons towards the anode. This is the "ion drift" region. In the immediate<br />

vicinity <strong>of</strong> the anode wire, the field strength becomes large enough to produce<br />

Townsend avalanches. This avalanche region occurs only fractions <strong>of</strong> a<br />

millimeter from the anode wire, which itself is <strong>of</strong> a very small diameter. The<br />

purpose <strong>of</strong> this is to use the multiplication effect <strong>of</strong> the avalanche produced by<br />

each ion pair. This is the "avalanche" region.<br />

A key design goal is that each original ionising event due to incident radiation<br />

produces only one avalanche. This is to ensure proportionality between the<br />

number <strong>of</strong> original events and the total ion current. For this reason the applied<br />

voltage, the geometry <strong>of</strong> the chamber and the diameter <strong>of</strong> the anode wire are<br />

critical to ensure proportional operation. If avalanches start to self-multiply<br />

due to UV photons as they do in a Geiger–Muller tube, then the counter<br />

enters a region <strong>of</strong> "limited proportionality" until at a higher applied voltage the<br />

Geiger discharge mechanism occurs with complete ionisation <strong>of</strong> the gas<br />

enveloping the anode wire and consequent loss <strong>of</strong> particle energy information.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Proportional_counter


Plot <strong>of</strong> variation <strong>of</strong> ion pair current against applied voltage for a wire cylinder<br />

gaseous radiation detector.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Proportional_counter


Therefore, it can be said that the proportional counter has the key design<br />

feature <strong>of</strong> two distinct ionisation regions:<br />

1. Ion drift region: in the outer volume <strong>of</strong> the chamber – creation <strong>of</strong> number<br />

ion pairs proportional to incident radiation energy.<br />

2. Avalanche region: in the immediate vicinity <strong>of</strong> the anode – Charge<br />

amplification <strong>of</strong> ion pair currents, while maintaining localised avalanches.<br />

The process <strong>of</strong> charge amplification greatly improves the signal-to-noise ratio<br />

<strong>of</strong> the detector and reduces the subsequent electronic amplification required.<br />

In summary, the proportional counter is an ingenious combination <strong>of</strong> two<br />

ionisation mechanisms in one chamber which finds wide practical use.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Proportional_counter


The generation <strong>of</strong> discrete Townsend avalanches in a proportional counter.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Proportional_counter


Plot <strong>of</strong> electric field strength at the anode, showing boundary <strong>of</strong> avalanche<br />

region.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Proportional_counter


The gas flow proportional counter for alpha counting was invented in 1943 by John Simpson at the<br />

University <strong>of</strong> Chicago Metallurgical Laboratory. Its purpose was to measure plutonium (an alpha emitter) in the presence <strong>of</strong> beta-emitting fission products.<br />

The key feature <strong>of</strong> this instrument that allowed it to reject beta pulses was its use <strong>of</strong> methane as the counting gas. Simpson would later invent P-10 gas<br />

(10% methane, 90% argon), the most widely employed gas in proportional counters. The instrument also featured a short time constant which reduced pulse<br />

pile up and assisted in rejecting the beta pulses.<br />

Charlie Chong/ Fion Zhang<br />

https://www.orau.org/PTP/collection/proportional%20counters/Proportionalcounters.htm


RCL Mark 2, Model 201 Fast <strong>Neutron</strong> Proportional Counter (1950s)<br />

This is a fast neutron detector produced by Radiation Counter Laboratories (RCL) <strong>of</strong> Skokie, Illinois.<br />

The tube is approximately 8 1/4 inches long and 1 7/8 inches in diameter. A brass evacuation tube can be<br />

seen projecting to the right from the brass chamber. The actual proportional counter chamber is 1.2 inches long,<br />

lined with 1/16 inch <strong>of</strong> polyethylene, and filled with methane at a pressure <strong>of</strong> 150 cm. It operated at 2100 volts.<br />

Fast neutrons knock protons <strong>of</strong>f the polyethylene lining. The protons then ionize the methane fill gas to produce<br />

the signal. The RCL detector designation is the Mark 2, Model 201, Serial 127. The "1" at the end <strong>of</strong> the model<br />

number (201) refers to the number <strong>of</strong> chambers housed in the unit. The Models 202 and 203 used two and<br />

three chambers respectively.<br />

Charlie Chong/ Fion Zhang<br />

https://www.orau.org/PTP/collection/proportional%20counters/bf3rclmk2mod201l.htm


Proportional Counter<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Proportional_counter


Proportional Counter<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Proportional_counter


Applications<br />

Spectroscopy<br />

The proportionality between the energy <strong>of</strong> the charged particle travelling<br />

through the chamber and the total charge created makes proportional<br />

counters useful for charged particle spectroscopy. By measuring the total<br />

charge (time integral <strong>of</strong> the electric current) between the electrodes, we can<br />

determine the particle's kinetic energy because the number <strong>of</strong> ion pairs<br />

created by the incident ionizing charged particle is proportional to its energy.<br />

The energy resolution <strong>of</strong> a proportional counter, however, is limited because<br />

both the initial ionization event and the subsequent 'multiplication' event are<br />

subject to statistical fluctuations characterised by a standard deviation equal<br />

to the square root <strong>of</strong> the average number formed. However, in practice these<br />

are not as great as would be predicted due to the effect <strong>of</strong> the empirical Fano<br />

factor which reduces these fluctuations. In the case <strong>of</strong> argon, this is<br />

experimentally about 0.2.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Proportional_counter


Photon detection<br />

Proportional counters are also useful for detection <strong>of</strong> high energy photons,<br />

such as gamma-rays, provided these can penetrate the entrance window.<br />

They are also used for the detection <strong>of</strong> X-rays to below 1 Kev energy levels,<br />

using thin walled tubes operating at or around atmospheric pressure.<br />

Radioactive contamination detection<br />

Proportional counters in the form <strong>of</strong> large area planar detectors are used<br />

extensively to check for radioactive contamination on personnel, flat surfaces,<br />

tools and items <strong>of</strong> clothing. This is normally in the form <strong>of</strong> installed<br />

instrumentation because <strong>of</strong> the difficulties <strong>of</strong> providing portable gas supplies<br />

for hand-held devices. They are constructed with a large area detection<br />

window made from such as metallised mylar which forms one wall <strong>of</strong> the<br />

detection chamber and is part <strong>of</strong> the cathode. The anode wire is routed in a<br />

convoluted manner within the detector chamber to optimise the detection<br />

efficiency.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Proportional_counter


They are normally used to detect alpha and beta particles, and can enable<br />

discrimination between them by providing a pulse output proportional to the<br />

energy deposited in the chamber by each particle. They have a high<br />

efficiency for beta, but lower for alpha. The efficiency reduction for alpha is<br />

due to the attenuation effect <strong>of</strong> the entry window, though distance from the<br />

surface being checked also has a significant effect, and ideally a source <strong>of</strong><br />

alpha radiation should be less than 10mm from the detector due to<br />

attenuation in air.<br />

These chambers operate at very slight positive pressure above ambient<br />

atmospheric pressure. The gas can be sealed in the chamber, or can be<br />

changed continuously, in which case they are known as "gas-flow<br />

proportional counters". Gas flow types have the advantage that they will<br />

tolerate small holes in the mylar screen which can occur in use, but they do<br />

require a continuous gas supply.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Proportional_counter


Guidance on application use<br />

In the United Kingdom the HSE has issued a user guidance note on selecting<br />

the correct radiation measurement instrument for the application concerned.<br />

This covers all radiation instrument technologies, and is a useful comparative<br />

guide to the use <strong>of</strong> proportional counters.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Proportional_counter


■ ωσμ∙Ωπ∆ ∇ º≠δ≤>ηθφФρ|β≠Ɛ∠ ʋ λαρτ√ ≠≥ѵФε ≠≥ѵФdsssa<br />

Charlie Chong/ Fion Zhang


Biological Half-life<br />

Charlie Chong/ Fion Zhang<br />

http://hyperphysics.phy-astr.gsu.edu/hbase/Nuclear/biohalf.html


Biological Half-life<br />

The radioactive half-life for a given radioisotope is physically determined and<br />

unaffected by the physical or chemical conditions around it. However, if that<br />

radioisotope is in a living organism it may be excreted so that it no longer is a<br />

source <strong>of</strong> radiation exposure to the organism. For a number <strong>of</strong> radioisotopes<br />

<strong>of</strong> particular medical interest, the rate <strong>of</strong> excretion has been cast in the form<br />

<strong>of</strong> an effective biological half-life. The rate <strong>of</strong> decrease <strong>of</strong> radiation exposure<br />

is then affected by both the physical and biological half-life, giving an effective<br />

half-life for the isotope in the body. Though the biological half-life cannot be<br />

expected to be as precise as the physical half-life, it is useful compute an<br />

effective half-life from:<br />

1/T Effective = 1/T Physical + 1/T Biological<br />

Charlie Chong/ Fion Zhang<br />

http://hyperphysics.phy-astr.gsu.edu/hbase/Nuclear/biohalf.html


<strong>Exam</strong>ples <strong>of</strong> the half-lives show that biological clearing is sometimes<br />

dominant and sometimes physical decay is the dominant influence.<br />

Half Life in day<br />

Isotopes<br />

T Physical<br />

T Biological<br />

T Effective<br />

3 H<br />

4.5 x 10 3<br />

12<br />

12<br />

22<br />

P<br />

14.3<br />

1155<br />

14.1<br />

90 Sr<br />

1.1 x 10 4<br />

1.8 x 10 4<br />

6.8 x 10 3<br />

99m<br />

Tc<br />

0.25<br />

1<br />

0.20<br />

Charlie Chong/ Fion Zhang<br />

http://hyperphysics.phy-astr.gsu.edu/hbase/Nuclear/biohalf.html


Tritium, 3 H, has a fairly long physical half life but clears from the body quickly,<br />

lessening the exposure. Phosphorous, 32 P, is used for some kinds <strong>of</strong> bone<br />

scans. The phosphorous tends to be held in the bones, leading to a long<br />

biological half-life, but its physical half-life is short enough to minimize<br />

exposure. Strontium, 90 Sr, is very bad news in the environment. It mimics<br />

calcium and therefore gets trapped in bone. This gives it a long biological<br />

half-life to go with its long physical half-life, making it doubly dangerous.<br />

Technetium, 99m Tc, is one <strong>of</strong> the favorites for diagnostic scans because <strong>of</strong><br />

short physical and biological half-lives. It clears from the body very quickly<br />

after the imaging procedures.<br />

Charlie Chong/ Fion Zhang<br />

http://hyperphysics.phy-astr.gsu.edu/hbase/Nuclear/biohalf.html


The biological half-life or terminal half-life <strong>of</strong> a substance is the time it takes<br />

for a substance (for example a metabolite, drug, signalling molecule,<br />

radioactive nuclide, or other substance) to lose half <strong>of</strong> its pharmacologic,<br />

physiologic, or radiologic activity, according to the Medical Subject Headings<br />

(MeSH) definition. Typically, this refers to the body's cleansing through the<br />

function <strong>of</strong> kidneys and liver in addition to excretion functions to eliminate a<br />

substance from the body. In a medical context, half-life may also describe the<br />

time it takes for the blood plasma concentration <strong>of</strong> a substance to halve<br />

(plasma half-life) its steady-state. The relationship between the biological and<br />

plasma half-lives <strong>of</strong> a substance can be complex depending on the substance<br />

in question, due to factors including accumulation in tissues (protein binding),<br />

active metabolites, and receptor interactions.<br />

Biological half-life is an important pharmacokinetic parameter and is usually<br />

denoted by the abbreviation t ½<br />

While a radioactive isotope decays perfectly according to first order kinetics<br />

where the rate constant is fixed, the elimination <strong>of</strong> a substance from a living<br />

organism follows more complex chemical kinetics.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Biological_half-life


Charlie Chong/ Fion Zhang


More <strong>Reading</strong><br />

http://www.euronuclear.org/info/encyclopedia.htm<br />

Charlie Chong/ Fion Zhang


■ ωσμ∙Ωπ∆ ∇ º≠δ≤>ηθφФρ|β≠Ɛ∠ ʋ λαρτ√ ≠≥ѵФε ≠≥ѵФdsssa<br />

Charlie Chong/ Fion Zhang


Charlie Chong/ Fion Zhang


Charlie Chong/ Fion Zhang


Charlie Chong/ Fion Zhang


Good Luck!<br />

Charlie Chong/ Fion Zhang

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