Understanding Neutron Radiography Post Exam Reading VIII-Part 1 of 2A
Understanding Neutron Radiography Post Exam Reading VIII-Part 1 of 2A
Understanding Neutron Radiography Post Exam Reading VIII-Part 1 of 2A
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<strong>Understanding</strong> <strong>Neutron</strong> <strong>Radiography</strong><br />
<strong>Reading</strong> <strong>VIII</strong> <strong>Part</strong> 1 <strong>of</strong> 2<br />
13 th 2016 August<br />
<strong>Post</strong> <strong>Exam</strong> <strong>Reading</strong><br />
Charlie Chong/ Fion Zhang
Reactor<br />
Charlie Chong/ Fion Zhang
Reactor<br />
Charlie Chong/ Fion Zhang
The Magical Book <strong>of</strong> <strong>Neutron</strong> <strong>Radiography</strong><br />
Charlie Chong/ Fion Zhang
Charlie Chong/ Fion Zhang
ASNT Certification Guide<br />
NDT Level III / PdM Level III<br />
NR - <strong>Neutron</strong> Radiographic Testing<br />
Length: 4 hours Questions: 135<br />
1. Principles/Theory<br />
• Nature <strong>of</strong> penetrating radiation<br />
• Interaction between penetrating radiation and matter<br />
• <strong>Neutron</strong> radiography imaging<br />
• Radiometry<br />
2. Equipment/Materials<br />
• Sources <strong>of</strong> neutrons<br />
• Radiation detectors<br />
• Non-imaging devices<br />
Charlie Chong/ Fion Zhang
3. Techniques/Calibrations<br />
• Blocking and filtering<br />
• Multifilm technique<br />
• Enlargement and projection<br />
• Stereoradiography<br />
• Triangulation methods<br />
• Autoradiography<br />
• Flash <strong>Radiography</strong><br />
• In-motion radiography<br />
• Fluoroscopy<br />
• Electron emission radiography<br />
• Micro-radiography<br />
• Laminography (tomography)<br />
• Control <strong>of</strong> diffraction effects<br />
• Panoramic exposures<br />
•Gaging<br />
• Real time imaging<br />
• Image analysis techniques<br />
Charlie Chong/ Fion Zhang
4. Interpretation/Evaluation<br />
• Image-object relationships<br />
• Material considerations<br />
• Codes, standards, and specifications<br />
5. Procedures<br />
• Imaging considerations<br />
• Film processing<br />
• Viewing <strong>of</strong> radiographs<br />
• Judging radiographic quality<br />
6. Safety and Health<br />
• Exposure hazards<br />
• Methods <strong>of</strong> controlling radiation exposure<br />
• Operation and emergency procedures<br />
Reference Catalog Number<br />
NDT Handbook, Third Edition: Volume 4,<br />
Radiographic Testing 144<br />
ASM Handbook Vol. 17, NDE and QC 105<br />
Charlie Chong/ Fion Zhang
Charlie Chong/ Fion Zhang<br />
Fion Zhang at Copenhagen Harbor<br />
4 th August 2016
Charlie Chong/ Fion Zhang<br />
SME- Subject Matter Expert<br />
http://cn.bing.com/videos/search?q=Walter+Lewin&FORM=HDRSC3<br />
https://www.youtube.com/channel/UCiEHVhv0SBMpP75JbzJShqw
Gamma- <strong>Radiography</strong><br />
TABLE 1. Characteristics <strong>of</strong> three isotope sources commonly used for<br />
radiography.<br />
Source<br />
T½<br />
Energy<br />
HVL<br />
HVL<br />
Specific<br />
Dose rate*<br />
Pb<br />
Fe<br />
Activity<br />
Co60<br />
5.3 year<br />
1.17, 1.33 MeV<br />
12.5mm<br />
22.1mm<br />
50 Cig -1<br />
1.37011<br />
Cs137<br />
30 years<br />
0.66 MeV<br />
6.4mm<br />
17.2mm<br />
25 Cig -1<br />
0.38184<br />
Ir192<br />
75 days<br />
0.14 ~ 1.2 MeV<br />
4.8mm<br />
?<br />
350 Cig -1<br />
0.59163<br />
(Aver. 0.34 MeV)<br />
Th232<br />
0.068376<br />
Dose rate* Rem/hr at one meter per curie<br />
Charlie Chong/ Fion Zhang
八 千 里 路 云 和 月<br />
Charlie Chong/ Fion Zhang
Charlie Chong/ Fion Zhang
闭 门 练 功<br />
Charlie Chong/ Fion Zhang
Charlie Chong/ Fion Zhang<br />
http://greekhouse<strong>of</strong>fonts.com/
Charlie Chong/ Fion Zhang
COLLIMATED NEUTRON BEAM FOR<br />
NEUTRON RADIOGRAPHY<br />
M. DINCA1, M. PAVELESCU2, C. IORGULIS1<br />
1 Institute for Nuclear Research, P.O. Box 078, Pitesti, Romania, dinca@scn.ro<br />
2 Romanian Scientist Academy, Bucharest, Romania, mpavelescu@pcnet.ro<br />
Received October 21, 2005<br />
Charlie Chong/ Fion Zhang
Pitești<br />
Charlie Chong/ Fion Zhang
The obtaining <strong>of</strong> a collimated neutron beam on the tangential channel <strong>of</strong> the<br />
ACPR reactor from INR Pitesti that to satisfy the requests <strong>of</strong> a neutron<br />
radiography facility it is presented. The collimation <strong>of</strong> neutrons means the<br />
elimination from the neutron beam <strong>of</strong> those neutrons that have trajectories<br />
that are not inside the space defined by walls or successive apertures that are<br />
made <strong>of</strong> neutron absorbent materials. The assembly that assures the<br />
collimation <strong>of</strong> neutrons, named collimator, is optimized using MCNP 4B code<br />
based on Monte Carlo method for neutrons and gamma radiation.<br />
Key words: neutron radiography, collimator for neutrons, collimation ratio,<br />
MCNP 4B code.<br />
Charlie Chong/ Fion Zhang
1. INTRODUCTION<br />
A tangential channel <strong>of</strong> a nuclear reactor has some peculiarities regarding<br />
intensity and energetic spectrum <strong>of</strong> neutrons in comparison with a radial<br />
channel <strong>of</strong> a nuclear reactor or tubes used to extract neutrons from other<br />
neutron sources.<br />
On a tangential channel the neutron beam has a bigger cadmium ratio and a<br />
lower gamma contamination than on a radial channel and is more suited to be<br />
used for thermal neutron radiography. For neutron radiography, different <strong>of</strong><br />
other nuclear physics applications that use neutron beams, are necessary<br />
large neutron beams to obtain images <strong>of</strong> a large area <strong>of</strong> the investigated<br />
objects. An ideal neutron beam should be parallel, monoenergetic, with big<br />
intensity, free <strong>of</strong> other contaminant radiation and uniform on its cross section.<br />
In practice it is intended to have experimental arrangements that to<br />
accomplish neutron beam parameters as closely as possible to ideal ones.<br />
Charlie Chong/ Fion Zhang
For this purpose it is used a collimator. The neutrons pass through a<br />
collimator from the entrance aperture placed nearby neutron source to the<br />
exit window where are used for neutron radiography investigations. The inner<br />
space <strong>of</strong> a collimator is evacuated or filled with air, or better filled with helium.<br />
A characteristic parameter <strong>of</strong> a collimator that defines the degree <strong>of</strong><br />
divergence <strong>of</strong> the neutron beam is the L/D ratio, where L is the length <strong>of</strong> the<br />
collimator and D is the diameter (or generally the opening) <strong>of</strong> the entrance<br />
aperture.<br />
Charlie Chong/ Fion Zhang
The place from where thermal neutrons start (the source <strong>of</strong> neutrons) is a<br />
moderator that contains neutrons moving in all directions. In order to have a<br />
neutron beam on a direction, nearby the moderator it is placed a collimator.<br />
The neutrons entering in the collimator must have the direction <strong>of</strong> the exit<br />
window to be useful otherwise they are captured by walls or apertures to<br />
avoid the scattering. The entrance aperture must be big enough to permit a<br />
larger number <strong>of</strong> neutrons to go inside the collimator but small enough to<br />
have a bigger L/D ratio. The L/D ratio depends also by the length <strong>of</strong> the<br />
collimator (or otherwise by the distance from entrance aperture to object<br />
plane if the object is put far away from collimator), a bigger L means a better<br />
resolution.<br />
Charlie Chong/ Fion Zhang
Because the moderator emits neutrons in all directions, their intensity is<br />
proportionally with 1/r 2 . To have a bigger intensity the object must be placed<br />
closer to neutron source but for a better geometrical resolution it must be<br />
placed farther. Bigger neutron intensity determines a better statistics,<br />
therefore a bigger contrast <strong>of</strong> the image that is able to differentiate between<br />
different materials. But for dimensional measurements it is necessary to have<br />
precise separation lines, therefore a big geometrical resolution.<br />
A compromise must be made between the two parameters, L and D. A<br />
transmission method for neutron radiography it is involved because are<br />
detected the neutrons that pass through investigated object. If the neutrons<br />
come to investigated object more scattered, then the projection <strong>of</strong> a detail is<br />
larger in the plane <strong>of</strong> the detector and the geometrical resolution <strong>of</strong> the image<br />
is poorer.<br />
Charlie Chong/ Fion Zhang
There are known different types <strong>of</strong> collimators, more important are:<br />
■ pin-hole,<br />
■ Soller and<br />
■ divergent collimators.<br />
Charlie Chong/ Fion Zhang
Soller Collimator<br />
Charlie Chong/ Fion Zhang
Sóller Collimator<br />
Charlie Chong/ Fion Zhang<br />
http://pd.chem.ucl.ac.uk/pdnn/inst3/soller.htm
The photograph shows the front opening <strong>of</strong> the 10′ Soller collimators <strong>of</strong> the<br />
detector bank <strong>of</strong> D1A taken before its rebuild in the late 1990's. The<br />
protective shielding has been removed so that thin vertical mylar sheets<br />
covered in a white gadolinium oxide paint are visible. The ones shown here<br />
were designed to collimate neutrons to 10 arc minutes (0.17°). (The little hole<br />
seen on the detector bank was a large "pin-hole" collimator, positioned in<br />
front <strong>of</strong> the normally unused 11th detector.)<br />
The Soller collimators designed for use on neutron diffractometers have large<br />
dimensions as illustrated by the figure below for 5′ collimation. The figure<br />
shows just two foils, but in practice many parallel foils are required since the<br />
diameter <strong>of</strong> the detectors is 2 to 5 cm.<br />
Charlie Chong/ Fion Zhang<br />
http://pd.chem.ucl.ac.uk/pdnn/inst3/soller.htm
The town <strong>of</strong> Sóller in the northwest <strong>of</strong> Mallorca became wealthy because <strong>of</strong><br />
the valley’s abundant citrus groves. In the 19th century, when the area was<br />
isolated from the rest <strong>of</strong> Mallorca by mountains, the oranges were shipped to<br />
France from the nearby west coast Port de Sóller (or Puerto de Sóller). Many<br />
locals went to work in France and returned – their fortunes duly made – to<br />
build some <strong>of</strong> the handsome Modernista properties that grace this town today.<br />
Charlie Chong/ Fion Zhang
The pin-hole collimator<br />
The pin-hole collimator has a simple construction. An aperture is placed at a<br />
distance from neutron source in order to establish a L/D ratio <strong>of</strong> the collimator.<br />
For a pin-hole collimator it is necessary a large neutron source that to have<br />
an equal neutron flux on its surface in order to expose uniformly the object to<br />
neutrons.<br />
The Soller collimators<br />
At Soller collimators appear on image the network <strong>of</strong> absorber walls that<br />
delimits inner minicollimators. This type <strong>of</strong> collimator requires a large uniform<br />
neutron source.<br />
The divergent collimator<br />
The most used is the divergent collimator because it permits the investigation<br />
<strong>of</strong> large objects, every point <strong>of</strong> the object being exposed to a neutron beam<br />
with approximately the same L/D (this means an intrinsic geometrical<br />
resolution uniform in the exit window <strong>of</strong> the collimator). A divergence<br />
collimator has the neutron source in its entrance aperture.<br />
Charlie Chong/ Fion Zhang
Based on dimensional constrains <strong>of</strong> the tangential channel <strong>of</strong> ACPR, previous<br />
experimental determinations <strong>of</strong> the thermal neutron flux and intensity<br />
(8 ⋅ 10 11 n/cm 2 /s near core and 1.12 x 10 6 n/cm2/s at the exit <strong>of</strong> tangential<br />
beam tube, at 100 kW operating power <strong>of</strong> ACPR) and working methods<br />
involved, were established the parameters <strong>of</strong> the divergent thermal neutron<br />
beam. Some <strong>of</strong> them are:<br />
Charlie Chong/ Fion Zhang
• the thermal neutron beam intensity at least 5 ⋅105 n/cm2/s;<br />
• the collimation ratio, L/D, at least 90;<br />
• the exit window, 250 mm in diameter;<br />
• the n/γ ratio at least 1⋅10 6 n/cm 2 /mrem (that determines used<br />
investigation methods);<br />
• the divergent angle under 40°;<br />
• the cadmium ratio above 17.<br />
Note: Cadmium Ratio<br />
The ratio <strong>of</strong> the response <strong>of</strong> an uncovered neutron detector to that <strong>of</strong> the<br />
same detector under identical conditions when it is covered with cadmium <strong>of</strong><br />
a specified thickness.<br />
Hint: the larger the cadmium ratio, the more the thermal neutron with energy<br />
less than 0.5Mev?<br />
Charlie Chong/ Fion Zhang
To obtain a thermal neutron beam with such parameters were used:<br />
1. a graphite illuminator placed on channel nearby reactor core to scatter<br />
neutrons towards exit <strong>of</strong> the channel;<br />
2. a mobile monocrystaline bismuth filter for the attenuation <strong>of</strong> the gamma<br />
radiationand scattering <strong>of</strong> fast neutrons that will allow performing direct<br />
neutron radiography investigations and also γ radiography investigations;<br />
3. a set <strong>of</strong> successive apertures from boron, indium and lead for the<br />
formation <strong>of</strong> the divergent collimator.<br />
Charlie Chong/ Fion Zhang
The position and dimensions <strong>of</strong> these components were optimized by<br />
calculus made with MCNP 4B code based on Monte Carlo method both for<br />
thermal neutrons and both for gamma radiation.<br />
Charlie Chong/ Fion Zhang
ACPR- Annular Core Pulse Reactor<br />
Charlie Chong/ Fion Zhang
Charlie Chong/ Fion Zhang
2. CALCULUS WITH WIMS 4D AND MCNP 4B CODES<br />
The tangential beam port has an overall length <strong>of</strong> 5644 mm (Figure 1) and<br />
has two sections. First with the length <strong>of</strong> about 2984 mm and the diameter <strong>of</strong><br />
219 x 6.5 mm, and second with the length <strong>of</strong> about 2660 mm and the<br />
diameter <strong>of</strong> 273 x 6.5 mm.<br />
2660 mm<br />
Charlie Chong/ Fion Zhang
The distance between the center <strong>of</strong> the reactor and the beam port axis is 575<br />
mm. The beam port exceeds with 508 mm, to the axis <strong>of</strong> the pool, the<br />
perpendicular right line on its own axis that passes through the center <strong>of</strong> the<br />
core. The beam port contains a mobile lead shutter with the thickness <strong>of</strong> 381<br />
mm and 406 mm in diameter placed at 1015 mm from beam port exit.<br />
Between the edge <strong>of</strong> the core and the tangential beam port is a distance <strong>of</strong><br />
157.8 mm. The space between core and beam port is filled with regular<br />
demineralised water. A better transmission <strong>of</strong> the neutrons from core to<br />
channel will be assured placing aluminum in free locations <strong>of</strong> the reactor grid.<br />
In this way the reduction <strong>of</strong> the initial thermal neutron flux <strong>of</strong> the channel<br />
through divergent collimator construction is compensated. (?)<br />
mobile lead shutter<br />
Charlie Chong/ Fion Zhang
Fig. 1. Sketch <strong>of</strong> the collimator <strong>of</strong> the neutron radiography facility at the<br />
tangential beam port <strong>of</strong> the ACPR.<br />
Charlie Chong/ Fion Zhang
The optimization <strong>of</strong> the transmission <strong>of</strong> neutrons to channel and the<br />
optimization <strong>of</strong> the dimensions and positions <strong>of</strong> the collimator components is<br />
done using WIMS D4 and MCNP 4B codes. To establish the spectrum <strong>of</strong> the<br />
neutron flux at the edge <strong>of</strong> the ACPR reactor, the transport program WIMS D4<br />
was involved. Because <strong>of</strong> cylindrical shape <strong>of</strong> the reactor, it is suitable to be<br />
modeled by WIMS program. The model consists <strong>of</strong> cylindrical rings that cover<br />
the central hole, ACPR fuel, water etc. The neutron flux calculated for 69<br />
broad groups in a thin volume at the edge <strong>of</strong> the core has been collapsed in 3<br />
or 23 groups. Their weights, after the renormalization to unit and upper<br />
boundaries for energy groups were used in the inputs <strong>of</strong> the MCNPprogram.<br />
The WIMS D4 code was used to study the effect <strong>of</strong> the replacement <strong>of</strong> the<br />
water between core and beam port with an aluminum block, aluminum pins<br />
placed in grid’s holes or air in aluminum box. The replacement <strong>of</strong> the water<br />
leads to an improvement <strong>of</strong> the transfer <strong>of</strong> the neutrons towards beam port.<br />
The results <strong>of</strong> the calculations are shown in Table 1. It can be seen that the<br />
increase <strong>of</strong> the thermal neutron flux is maximum using a box filled with air. To<br />
disturb not other experiments for irradiation tests, a bell box is put in place<br />
from where the water is pushed out and replaced by air.<br />
Charlie Chong/ Fion Zhang
Table 1: Relative units <strong>of</strong> the thermal flux in the graphite illuminator for some<br />
materials between core and tangential beam port<br />
Water Aluminum pins Aluminum block<br />
Air<br />
4.92 14.3 16 19.5<br />
Charlie Chong/ Fion Zhang
In order to assure a maximum thermal neutron beam at the exit <strong>of</strong> the<br />
collimator and a suitable established collimation ratio were performed Monte<br />
Carlo calculation based on MCNP code. Two models were prepared for<br />
Monte Carlo calculations. The first model aimed to establish the thickness<br />
and position <strong>of</strong> the graphite illuminator for the maximum increase <strong>of</strong> the<br />
thermal neutron beam at the exit <strong>of</strong> the collimator. This model contains the<br />
source <strong>of</strong> neutrons <strong>of</strong>fered by WIMS code for 3 and 23 groups, the box with<br />
air and the illuminator placed on beam port. The relative values obtained in a<br />
plane at 100 cm from illuminator, for different thicknesses <strong>of</strong> the illuminator<br />
are shown in Figure 2. The illuminator is placed near centerline. If the<br />
illuminator is placed in a centered position the thermal neutron flux is a little<br />
improved, but epithermal and fast neutrons increase more and it is not<br />
desirable. The maximum neutron beam is obtained for 6.5 cm and 7 cm<br />
illuminator thicknesses.<br />
Charlie Chong/ Fion Zhang
Fig. 2. <strong>Neutron</strong> beam intensity.<br />
Charlie Chong/ Fion Zhang
The second model targeted to establish the position and thickness <strong>of</strong> the<br />
single-crystal Bi filter, to obtain the maximum thermal neutron beam at the<br />
exit <strong>of</strong> the collimator. This model is based on the geometry <strong>of</strong> the collimator<br />
shown in Figure 1 and the source <strong>of</strong> neutrons is placed on the face <strong>of</strong> the<br />
illuminator. We consider the maximization <strong>of</strong> neutron flux below 1.E-06 MeV.<br />
On the geometry <strong>of</strong> the second model calculations were done for gamma<br />
radiation also. Based on previous flux measurements and the results<br />
estimated from first MCNP model, it was established a value <strong>of</strong> 4.5 cm for the<br />
diameter <strong>of</strong> the collimator main aperture. Preliminary results obtained with the<br />
second model established a value <strong>of</strong> 3 cm for the thickness <strong>of</strong> the Bi singlerystal.<br />
The main aperture will be built by 13 mm <strong>of</strong> boral, 1 mm indium and<br />
200 mm lead.<br />
Charlie Chong/ Fion Zhang
To optimize the position <strong>of</strong> the aperture and Bi filter, MCNP calculation were<br />
done for different positions <strong>of</strong> the filter. The results are shown in Figure 3.<br />
Supplementary, it was used the condition to have a uniform intensity <strong>of</strong> the<br />
neutron beam in the exit window <strong>of</strong> the collimator. This was precisely<br />
established with AutoCAD program that drawn the extreme lines <strong>of</strong> the<br />
neutron beam. In this way every point in the exit window is seen by the same<br />
area from the surface <strong>of</strong> the illuminator. In these conditions it was established<br />
the maximum distance between illuminator and aperture to be 152.5 cm,<br />
although the maximum <strong>of</strong> the neutron beam is obtained for the distance <strong>of</strong><br />
190-200 mm. The calculations for the distance <strong>of</strong> 152.5 cm, the main aperture<br />
<strong>of</strong> 4.5 cm and 3 cm <strong>of</strong> Bi indicates a decrease <strong>of</strong> the gamma radiation <strong>of</strong><br />
65.19 times, and for neutrons <strong>of</strong> 16.15 times (the Bi filter itself decreases the<br />
beam intensities 8.22 and 2.22 times, respectively). The calculations with<br />
MCNP code were done with polycrystalline Bi. In the real case, for<br />
singlecrystal Bi with cross-section 3 times smaller at room temperature [1], it<br />
is expected a reduction <strong>of</strong> the beam intensity with 41% instead <strong>of</strong> 2.22 times<br />
reduction.<br />
Charlie Chong/ Fion Zhang
Fig. 3. Intensity <strong>of</strong> the thermal neutron beam at the exit <strong>of</strong> the collimator.<br />
Charlie Chong/ Fion Zhang
The minimum distance between illuminator and main aperture is considered<br />
to be 125 cm. For this distance the intensity <strong>of</strong> neutron beam decreases with<br />
17%, but the resolution increases. The lead ring (20 cm) should be positioned<br />
at less 125 cm were is the edge <strong>of</strong> the concrete wall <strong>of</strong> the pool, otherwise the<br />
direct gamma radiation from reactor core cannot be properly stopped. The<br />
secondary apertures are positioned to avoid any trajectory <strong>of</strong> the neutron<br />
directly from illuminator to reach the wall <strong>of</strong> the beam tube. The secondary<br />
apertures are boral plates and lead rings. To increase the neutron beam for<br />
the direct method and to perform gamma radiographs it is designed to<br />
remove vertically the Bi filter with the help <strong>of</strong> a steel cable. The Bi filter is<br />
inside <strong>of</strong> a box, which contains lead ballast to fall back on position when cable<br />
is released.<br />
Charlie Chong/ Fion Zhang
3. CONCLUSIONS<br />
The collimation <strong>of</strong> the neutrons on the tangential beam port <strong>of</strong> the ACPR<br />
reactor is done, in fact, with a pin-hole collimator with an aperture <strong>of</strong> 45 mm<br />
placed at the distance <strong>of</strong> 125-152.5 cm from the surface <strong>of</strong> the illuminator that<br />
has a thickness <strong>of</strong> 6.5 cm and the diameter <strong>of</strong> 18 cm. The estimated beam<br />
intensity for thermal neutrons with bismuth filter is 3.96⋅105 – 4.65⋅10 5 n/cm 2 /s<br />
and 4.85⋅105 – 5.70⋅10 5 n/cm 2 /s without Bi filter. The estimated values for<br />
gamma debit doses (for 152.5 cm illuminator-main aperture distance) are<br />
1.75 rem/h without bismuth and 213 mrem/h with bismuth. The estimated<br />
n/gamma ratio is 1.03⋅10 6 n/cm2/mrem and 8.44⋅10 6 n/cm 2 /mrem,<br />
respectively. The divergent angle <strong>of</strong> the collimator is 3 o -3.3 o and the<br />
collimation ratio 100-92.8 for the domain <strong>of</strong> distances 125-152.5 cm<br />
betweenilluminator and main aperture. These values <strong>of</strong> beam intensity,<br />
n/gamma ratio and collimation ratio are in concordance with that from other<br />
facilities built at TRIGA reactors and <strong>of</strong>fer the base to use with good results<br />
the direct and the transfer methods for neutron radiography.<br />
Charlie Chong/ Fion Zhang
Sandia’s Annular Core Research Reactor<br />
conducts 10,000th operation<br />
Charlie Chong/ Fion Zhang<br />
https://share.sandia.gov/news/resources/news_releases/acrr/#.V65mc-Qkpdg
ACPR- Annular Core Pulse Reactor<br />
Charlie Chong/ Fion Zhang
ACRR- Annular Core (Pulse) Research Reactor<br />
Charlie Chong/ Fion Zhang<br />
https://share.sandia.gov/news/resources/news_releases/acrr/
ACRR- Annular Core (Pulse) Research Reactor<br />
Charlie Chong/ Fion Zhang<br />
https://share.sandia.gov/news/resources/news_releases/acrr/
ALBUQUERQUE, N.M. – With a muffled “pop,” a flash <strong>of</strong> blue light and a few<br />
ripples through 14,000 gallons <strong>of</strong> deionized water, Sandia National<br />
Laboratories’ Annular Core Research Reactor (ACRR) recently conducted its<br />
10,000th operation.<br />
“The ACRR has been a real workhorse for Sandia, and labs leadership and<br />
the nation rely on these experiments and other weapons component testing<br />
done at Sandia to support certification <strong>of</strong> the nuclear weapon stockpile,” said<br />
Lonnie Martin, an ACRR operator.<br />
In its 32-year history, the ACRR time and again has proved itself a valuable<br />
resource for a wide variety <strong>of</strong> experiments in nearly every branch <strong>of</strong> nuclear<br />
science, especially the testing <strong>of</strong> radiation-hardened electronic components.<br />
With a dry, 9-inch diameter cavity in the core’s center, and a 20-inch diameter<br />
external cavity, the ACRR subjects electronics to high-intensity neutron<br />
irradiation and conducts reactor safety research. The ACRR also has done<br />
testing for semiconductor manufacturers, NASA, the Large Hadron Collider in<br />
Switzerland and dozens <strong>of</strong> other users.<br />
Charlie Chong/ Fion Zhang
Sandia’s ACRR is a water-moderated, pool-type research reactor capable <strong>of</strong><br />
steady-state, pulsed and tailored transient operations and, in the past, has<br />
been configured for medical isotope production. Other duties for ACRR<br />
include: reactor-driven laser experiments; space reactor fuels development;<br />
pulse reactor kinetics; reactor heat transfer and fluid flow; electronic<br />
component hardening; and explosive component testing. It is also routinely<br />
used for education and training programs.<br />
Charlie Chong/ Fion Zhang
At peak power in its steady state mode, the ACRR produces up to four<br />
megawatts <strong>of</strong> power. But during a maximum pulse, it generates a whopping<br />
35,000 megawatts <strong>of</strong> power for seven milliseconds. Nuclear engineer and<br />
former University <strong>of</strong> New Mexico pr<strong>of</strong>essor Ron Knief compares its power<br />
output to that <strong>of</strong> the Palo Verde Nuclear Generating Station, outside <strong>of</strong><br />
Phoenix. “For that very short time, we produce three times more power than<br />
the nation’s largest nuclear power station. They have three big reactors, and<br />
yet, for a fraction <strong>of</strong> a second, we produce three times more power than they<br />
do,” Knief said.<br />
Charlie Chong/ Fion Zhang
The ACRR is a descendent <strong>of</strong> the Sandia Annular Core Pulse Reactor<br />
(ACPR), which was replaced in 1978 and is part <strong>of</strong> a large family <strong>of</strong> Training,<br />
Research Isotope Production, General Atomics (TRIGA) reactors. The TRIGA<br />
concept is credited to Manhattan Project physicist Edward Teller and a group<br />
<strong>of</strong> distinguished scientists who assembled the first model in a “Little Red<br />
Schoolhouse” in San Diego in 1956. Teller’s mandate to the team was to<br />
“design a reactor so safe … that if it was started from its shut-down condition<br />
and all its control rods instantaneously removed, it would settle down to a<br />
steady level <strong>of</strong> operation without melting any <strong>of</strong> its fuel,” according to<br />
Freeman Dyson’s, “Disturbing the Universe.” Essentially, even if all the<br />
engineered safety mechanisms failed, the reactor would operate safely,<br />
based on the laws <strong>of</strong> physics.<br />
In 1978, the original ACPR TRIGA fuel was replaced with a new ACRR<br />
ceramic-metal, uranium dioxide/beryllium oxide (UO2/BeO) fuel, which is<br />
designed to allow steady state and pulsed operation at fuel temperatures up<br />
to 2,552 degrees (1,400 degrees C). The reactor underwent extensive<br />
upgrades in 2002, including upgrades to reactivity control circuitry.<br />
Charlie Chong/ Fion Zhang
Key!<br />
Charlie Chong/ Fion Zhang
Charlie Chong/ Fion Zhang
Reactor<br />
Charlie Chong/ Fion Zhang
Reactor<br />
Charlie Chong/ Fion Zhang
<strong>Radiography</strong> may be considered the most effective nondestructive testing<br />
method merely because <strong>of</strong> its universal use and acceptance in industry.<br />
<strong>Radiography</strong> can be used to test most types <strong>of</strong> solid material. Exceptions<br />
include materials <strong>of</strong> very high or very low density. <strong>Neutron</strong> radiography,<br />
however, can <strong>of</strong>ten be used in such cases. There is wide latitude both <strong>of</strong><br />
material thickness that can be tested and in the techniques that can be used.<br />
Usually conditions that result in a two percent or greater difference in<br />
through- section thickness can usually be detected. (≥2% subject sensitivity)<br />
Charlie Chong/ Fion Zhang
Read The following article:<br />
• E 748-95, Standard Practices for Thermal <strong>Neutron</strong> <strong>Radiography</strong> <strong>of</strong><br />
Materials<br />
• E 803, Standard Test Method for Determining the L/D Ratio <strong>of</strong> <strong>Neutron</strong><br />
<strong>Radiography</strong> Beams<br />
• E 1496-97, Standard Test Method for <strong>Neutron</strong> Radiographic Dimensional<br />
Measurements<br />
Charlie Chong/ Fion Zhang
Chapter 5 Radiation Measurement<br />
PART 6. <strong>Neutron</strong> Detection<br />
1.0 Characteristics<br />
The neutron is a part <strong>of</strong> the nucleus, has no charge and is somewhat larger in<br />
mass than the proton. It is similar to the photon in that it has no charge and<br />
produces ionization indirectly; it is different from the photon because it is a<br />
nuclear particle and not a unit <strong>of</strong> electromagnetic energy. (for photon, E=hʋ)<br />
Because the neutron is an uncharged particle, its interactions with matter are<br />
different from those <strong>of</strong> charged particles or photons. Ionization by neutrons is<br />
indirect: as a result <strong>of</strong> neutron interactions with matter, recoil (1) nuclei, (2)<br />
photons or (3) charged particles are produced and then interact with matter<br />
by various mechanisms that cause ionization.<br />
Charlie Chong/ Fion Zhang
Recoil - Measurement <strong>of</strong> Hydrogen Depth Pr<strong>of</strong>ile Using Fast <strong>Neutron</strong>s-<br />
Materials Analysis with Deuterium and Tritium Fusion <strong>Neutron</strong>s<br />
Charlie Chong/ Fion Zhang<br />
http://jolisfukyu.tokai-sc.jaea.go.jp/fukyu/mirai-en/2006/3_13.html
2.0 <strong>Neutron</strong> Sources<br />
<strong>Neutron</strong>s are classified according to their energies as shown in Table 4.<br />
Some radionuclides (such as californium-252) may decay by spontaneous<br />
fission and emit neutrons with fission fragments, photons and electrons.<br />
Induced fission reactions, such as those occurring in a nuclear reactor with<br />
uranium, emit about 2.5 neutrons per fission.<br />
Fission neutrons range in energy from 0.025 eV to about 16 MeV. Other<br />
neutron sources are the result <strong>of</strong> various nuclear reactions and produce either<br />
a spectrum <strong>of</strong> neutron energies or monoenergetic neutrons. Common neutron<br />
producing nuclear reactions are the (γ, n), (α, n), (p, n), (d, n) and (α, 2n)<br />
reactions and may use radionuclide emissions or accelerated particles to<br />
initiate the reaction.<br />
<strong>Neutron</strong> radiography usually uses radionuclides that emit alpha or gamma<br />
photons and produce neutrons by (α, n) and (γ, n) reactions with various<br />
target materials.<br />
Charlie Chong/ Fion Zhang
TABLE 4. <strong>Neutron</strong> classification.<br />
Class<br />
Thermal<br />
Epithermal<br />
Slow<br />
Intermediate<br />
Fast<br />
Relativistic<br />
Energy<br />
< 0.3 meV<br />
>1 eV<br />
30 meV to 100 eV<br />
100 eV to 10 keV<br />
10 keV to 10 MeV<br />
greater than 10 MeV<br />
Charlie Chong/ Fion Zhang
3.0 <strong>Neutron</strong> Detectors<br />
There are several mechanisms and devices used to detect neutrons <strong>of</strong><br />
various energies. Ionization chambers, proportional counters, scintillators,<br />
activation foils, track etch detectors, film emulsions, nuclear emulsions and<br />
thermoluminescent phosphors are some <strong>of</strong> the many devices used to detect<br />
neutrons. The main mechanisms used to detect neutrons in these devices are<br />
the (n, α), (n, p), (n, d), (n, f ) and (n, γ) nuclear reactions.<br />
Charlie Chong/ Fion Zhang
3.1 Proportional <strong>Neutron</strong> Detectors<br />
Many fast and slow neutron counters use proportional counting chambers<br />
filled with boron trifluoride (BF3) gas, <strong>of</strong>ten enriched in boron-10.<br />
The interaction <strong>of</strong> thermal (slow) neutrons with boron gas releases an alpha<br />
particle <strong>of</strong> several megaelectronvolts that is easily detected in the proportional<br />
mode. 10 5 B(n,α)7 3 Li<br />
Fast neutrons are detected by a similar counter, in which thermal neutrons<br />
are absorbed in an external cadmium shield ( 113 Cd(n,γ) 114 Cd ; the fast<br />
neutrons that pass through the shield are thermalized in hydrogen rich<br />
material and counted in the proportional chambers.<br />
γ<br />
hydrogen<br />
rich material<br />
boron trifluoride (BF3) gas<br />
external<br />
Pb Shield?<br />
Charlie Chong/ Fion Zhang
■<br />
http://minerals.usgs.gov/minerals/pubs/commodity/<br />
Charlie Chong/ Fion Zhang
The Cross Section (barns) <strong>of</strong><br />
commonly used conversion<br />
screen<br />
Careful on differential cross<br />
section for isotopes <strong>of</strong> same<br />
element.<br />
Charlie Chong/ Fion Zhang
TABLE 6. Properties <strong>of</strong> Some Thermal <strong>Neutron</strong> <strong>Radiography</strong> Conversion Materials<br />
Material<br />
Useful Reactions<br />
Cross Section for<br />
Life<br />
Thermal <strong>Neutron</strong>s (barns)<br />
Lithium<br />
6 Li(n,α) 3 H<br />
910<br />
prompt<br />
Boron<br />
10 B(n,α) 7 Li<br />
3,830<br />
prompt<br />
Rhodium<br />
103 Rh(n) 104m Rh<br />
11<br />
45 min<br />
103<br />
Rh(n) 104 Rh<br />
139<br />
42 s<br />
Silver<br />
107 Ag(n) 108 Ag<br />
35<br />
2.3 min<br />
109 Ag (n) 110 Ag<br />
91<br />
24 s<br />
Cadmium<br />
113 Cd((n,γ) 114 Cd<br />
20,000<br />
prompt<br />
Indium<br />
115 In(n) 116 n<br />
157<br />
54 min<br />
115<br />
In(n) 116m ln<br />
42<br />
14 s<br />
Samarium<br />
149 Sm(n,γ) 150 Sm<br />
41,000<br />
prompt<br />
I52<br />
Sm(n) 153 Sm<br />
210<br />
47 h<br />
Europium<br />
151 Eu(n) 152 Eu<br />
3,000<br />
9.2 h<br />
Gadolinium<br />
155<br />
Gd(n,γ) I56 Gd<br />
61,000<br />
prompt<br />
157<br />
Gd(n,γ) 158 Gd<br />
254,000<br />
prompt<br />
Dyprosium<br />
164<br />
Dy(n) 165m Dy<br />
2,200<br />
1.25 min<br />
164<br />
Dy(n) 165 Dy<br />
800<br />
140 min<br />
Gold<br />
197 Au(n) 198 Au<br />
99<br />
2.7 days<br />
Charlie Chong/ Fion Zhang
<strong>Neutron</strong> Cross Section <strong>of</strong> the elements<br />
Charlie Chong/ Fion Zhang<br />
http://periodictable.com/Properties/A/<strong>Neutron</strong>CrossSection.html
<strong>Neutron</strong> Cross Section σtotal for Gd =50000 barn<br />
Charlie Chong/ Fion Zhang<br />
http://periodictable.com/Properties/A/<strong>Neutron</strong>CrossSection.html
<strong>Neutron</strong> Cross Section σtotal for Dy =1010 barn<br />
Charlie Chong/ Fion Zhang<br />
http://periodictable.com/Properties/A/<strong>Neutron</strong>CrossSection.html
TABLE X1.1 Thermal <strong>Neutron</strong> Linear Attenuation Coefficients Using<br />
Average Scattering and Thermal Absorption Cross Sections for the<br />
Naturally Occurring Elements<br />
Charlie Chong/ Fion Zhang<br />
E748-02 Standard Practices for Thermal <strong>Neutron</strong> <strong>Radiography</strong> <strong>of</strong> Materials
Material<br />
Useful Reactions<br />
Cross Section for<br />
Life<br />
Thermal <strong>Neutron</strong>s (barns)<br />
Lithium<br />
6 Li(n,α) 3 H<br />
910<br />
prompt<br />
Boron<br />
10<br />
B(n,α) 7 Li<br />
3,830<br />
prompt<br />
Rhodium<br />
103 Rh(n) 104m Rh<br />
11<br />
45 min<br />
103 Rh(n) 104 Rh<br />
139<br />
42 s<br />
Silver<br />
107 Ag(n) 108 Ag<br />
35<br />
2.3 min<br />
109 Ag (n) 110 Ag<br />
91<br />
24 s<br />
Cadmium<br />
113 Cd((n,γ) 114 Cd<br />
20,000<br />
prompt<br />
Indium<br />
115<br />
In(n) 116 n<br />
157<br />
54 min<br />
115<br />
In(n) 116m ln<br />
42<br />
14 s<br />
Samarium<br />
149 Sm(n,γ) 150 Sm<br />
41,000<br />
prompt<br />
I52<br />
Sm(n) 153 Sm<br />
210<br />
47 h<br />
Europium<br />
151 Eu(n) 152 Eu<br />
3,000<br />
9.2 h<br />
Gadolinium<br />
155<br />
Gd(n,γ) I56 Gd<br />
61,000<br />
prompt<br />
157<br />
Gd(n.γ) 158 Gd<br />
254,000<br />
prompt<br />
Avg 64 Gd(n.γ) ? Gd<br />
49,000<br />
prompt<br />
Dyprosium<br />
164<br />
Dy(n) 165 mDy<br />
2,200<br />
1.25 min<br />
164<br />
Dy(n) 165 Dy<br />
800<br />
140 min<br />
Gold<br />
197<br />
Au(n) 198 Au<br />
99<br />
2.7 days<br />
Charlie Chong/ Fion Zhang
Charlie Chong/ Fion Zhang<br />
FIG. X1.1 Approximate Mass Attenuation Coefficients as a Function <strong>of</strong><br />
Atomic Number
TABLE 6. Properties <strong>of</strong> Some Thermal <strong>Neutron</strong> <strong>Radiography</strong> Conversion<br />
Materials<br />
Material<br />
Useful Reactions<br />
Cross Section for<br />
Life<br />
Thermal <strong>Neutron</strong>s (barns)<br />
Lithium<br />
6<br />
Li(n,α) 3 H<br />
910<br />
prompt<br />
Boron<br />
10 B(n,α) 7 Li<br />
3,830<br />
prompt<br />
Rhodium<br />
103 Rh(n) 104m Rh<br />
11<br />
45 min<br />
103<br />
Rh(n) 104 Rh<br />
139<br />
42 s<br />
Silver<br />
107<br />
Ag(n) 108 Ag<br />
35<br />
2.3 min<br />
109 Ag (n) 110 Ag<br />
91<br />
24 s<br />
Cadmium<br />
113<br />
Cd((n,γ) 114 Cd<br />
20,000<br />
prompt<br />
Indium<br />
115 In(n) 116 n<br />
157<br />
54 min<br />
115<br />
In(n) 116m ln<br />
42<br />
14 s<br />
Samarium<br />
149 Sm(n,γ) 150 Sm<br />
41,000<br />
prompt<br />
I52<br />
Sm(n) 153 Sm<br />
210<br />
47 h<br />
Europium<br />
151 Eu(n) 152 Eu<br />
3,000<br />
9.2 h<br />
Gadolinium<br />
155<br />
Gd(n,γ) I56 Gd<br />
61,000<br />
prompt<br />
157<br />
Gd(n.γ) 158 Gd<br />
254,000<br />
prompt<br />
Dyprosium<br />
164<br />
Dy(n) 165 mDy<br />
2,200<br />
1.25 min<br />
164<br />
Dy(n) 165 Dy<br />
800<br />
140 min<br />
Gold<br />
197<br />
Au(n) 198 Au<br />
99<br />
2.7 days<br />
Charlie Chong/ Fion Zhang
TABLE 6. Capture cross sections σ <strong>of</strong> strongly absorbing elements for<br />
neutrons in approximate thermal equilibrium at 300 K (27 °C = 80 °F).<br />
Charlie Chong/ Fion Zhang
TABLE 4. Average Characteristics <strong>of</strong> Thermal-Sources<br />
Type <strong>of</strong> Source<br />
Typical<br />
Resolution**<br />
Exposure<br />
Characteristics<br />
Radiographic<br />
Intensity*<br />
Time<br />
Radioisotope<br />
10 1 to 10 4<br />
Poor to Medium<br />
Long<br />
Stable operation.<br />
medium investment cost.<br />
possibly portable.<br />
Accelerator<br />
10 3 to 10 6<br />
Medium<br />
Average<br />
On-<strong>of</strong>f operation. medium<br />
cost. possibly mobile.<br />
Subcritical<br />
10 4 to 10 6<br />
Good<br />
Average<br />
Stable operation,<br />
Assembly<br />
medium to high investment<br />
cost, mobility difficult<br />
Nuclear reactor<br />
10 5 to 10 8<br />
Excellent<br />
Short<br />
Stable operation,<br />
medium to high investment<br />
cost. mobility difficult<br />
*<strong>Neutron</strong>s per square centimeter per second. n/cm 2 ∙s<br />
**These classifications are relative<br />
Charlie Chong/ Fion Zhang
More <strong>Reading</strong> on Gadolinum<br />
Gadolinium is a silvery-white malleable and ductile rare-earth metal. It<br />
crystallizes in hexagonal, close-packed α-form at room temperature, but,<br />
when heated to temperatures above 1235 °C, it transforms into its β-form,<br />
which has a body-centered cubic structure.<br />
Gadolinium-157 has the highest thermal neutron capture cross-section<br />
among any stable nuclides: 259,000 barns. Only xenon-135 has a higher<br />
cross section, 2 million barns, but that isotope is unstable.<br />
Charlie Chong/ Fion Zhang
Gadolinium is generally believed to be ferromagnetic at temperatures below<br />
20 °C (68 °F) and is strongly paramagnetic above this temperature. There is<br />
some evidence that gadolinium may be a helical antiferromagnet, rather than<br />
a ferromagnet, below 20 °C (68 °F). Gadolinium demonstrates a<br />
magnetocaloric effect whereby its temperature increases when it enters a<br />
magnetic field and decreases when it leaves the magnetic field. The<br />
temperature is lowered to 5 °C (41 °F) for the gadolinium alloy Gd85Er15,<br />
and the effect is considerably stronger for the alloy Gd5(Si2Ge2), but at a<br />
much lower temperature (
Gadolinum<br />
Charlie Chong/ Fion Zhang
Gadolinum<br />
Charlie Chong/ Fion Zhang
isotope NA half-life DM DE (MeV) Decay Product<br />
148Gd syn 75y α 3.271<br />
144<br />
Sm<br />
150Gd syn 1.8×10 6 y α 2.808<br />
146<br />
Sm<br />
152Gd 0.20% 1.08×10 14 y α 2.205<br />
148<br />
Sm<br />
154Gd 2.18% – (α) 0.0812<br />
150<br />
Sm<br />
155Gd 14.80% – (α) 0.0812<br />
151<br />
Sm<br />
156Gd 20.47% – (SF)
σ,Cross Section <strong>of</strong> Gadolinium<br />
Gd Average = 49000 barn prompt<br />
155<br />
Gd(n,γ) 156 Gd = 61,000 barn prompt<br />
157<br />
Gd(n.γ) 158 Gd = 254,000 barn prompt<br />
Charlie Chong/ Fion Zhang
<strong>Neutron</strong><br />
For many years after the proton and electron became comfortable concepts<br />
for building models <strong>of</strong> the atoms <strong>of</strong> the elements but explanations eluded<br />
researchers for the existence <strong>of</strong> isotopes and the extremely penetrating<br />
radiation emitted by the bombardment <strong>of</strong> light elements with alpha particles.<br />
In 1932, Chadwick described a neutral particle with a mass equal to a proton<br />
that he called a neutron. The neutron explained many observations<br />
concerning radiation and particle physics and the concept was rapidly<br />
accepted. <strong>Neutron</strong> characteristics are given in Table 3.<br />
Charlie Chong/ Fion Zhang
TABLE 3. <strong>Neutron</strong> characteristics.<br />
Quantity<br />
Measurement<br />
Charge<br />
neutral<br />
Rest mass<br />
1.675 × 10 –27 kg<br />
Classical radius 1.532 × 10 –18 m<br />
Magnetic moment –9.662 × 10 –27 J·T –1<br />
Compton wavelength 1.320 × 10 –15 m<br />
Charlie Chong/ Fion Zhang
Hydrogen, Deuterium, Tritium<br />
Radioactive materials have existed since the earth was created. All elements<br />
with atomic numbers greater than 83, bismuth, exist only as radioactive<br />
elements and many elements below atomic number 83 have radioactive<br />
isotopes that exist in nature.<br />
The difference between a stable or nonradioactive atom <strong>of</strong> an element and an<br />
unstable or radioactive atom is in the energy content <strong>of</strong> the nucleus. Most<br />
<strong>of</strong>ten an excess or deficiency in the number <strong>of</strong> neutrons in the nucleus<br />
provides the excess energy or instability.<br />
As an example: most hydrogen in nature exists as atoms with only 1 proton<br />
and 1 electron. About 15 <strong>of</strong> every 100 000 atoms <strong>of</strong> hydrogen have a neutron<br />
plus the proton in the nucleus, giving the atom a mass <strong>of</strong> 2 or twice the mass<br />
<strong>of</strong> most hydrogen atoms. Mass 2 hydrogen is called deuterium or heavy<br />
hydrogen and is stable. When a second neutron is added to the nucleus <strong>of</strong><br />
hydrogen, the atom has a mass <strong>of</strong> 3, is called tritium and is radioactive.<br />
The tritium atom is produced in nature by cosmic bombardment to produce a<br />
pre- 1952 concentration in nature <strong>of</strong> between 1 ~ 10 tritium atoms per 10 18<br />
hydrogen atoms.<br />
Charlie Chong/ Fion Zhang
<strong>Neutron</strong>s<br />
<strong>Neutron</strong>s produced by fission, accelerator nuclear reactions or radioisotope<br />
sources have considerable kinetic energy. This kinetic energy is most <strong>of</strong>ten<br />
lost by scattering interactions with or absorption in the nuclei <strong>of</strong> the atoms in<br />
their path. Absorption <strong>of</strong> the neutron is followed by release <strong>of</strong> electromagnetic<br />
radiation or large particles such as protons, multiple neutrons, deuterons or<br />
alpha particles. Interactions with the orbital electrons contribute negligibly to<br />
the absorption <strong>of</strong> neutrons by matter. The nucleus is much smaller than the<br />
electron orbits, so neutron interactions are less frequent than those <strong>of</strong> alpha<br />
or beta particles. And because the neutron has no charge, ionization and<br />
excitation are not major absorption processes.<br />
Charlie Chong/ Fion Zhang
FIGURE 4. Ionization by alpha particle that ejects orbital electron from atom.<br />
Specific ionization is number <strong>of</strong> ion pairs generated by particle per unit path.<br />
Total ionization designates number <strong>of</strong> ion pairs produced by particle along its<br />
entire path.<br />
Charlie Chong/ Fion Zhang
<strong>Neutron</strong>- Elastic Scattering<br />
For elastic scattering, the neutron collides with the nucleus and bounces <strong>of</strong>f,<br />
leaving the nucleus unchanged. This type <strong>of</strong> collision can be treated<br />
straightforwardly as a mechanical billiard ball type <strong>of</strong> collision. In the collision<br />
the energy <strong>of</strong> the neutron is shared by the nucleus, thus each collision<br />
reduces the energy <strong>of</strong> the neutron. After a number <strong>of</strong> collisions with the nuclei,<br />
the energy is reduced to the same average kinetic energy as that <strong>of</strong> the<br />
absorbing medium. This energy is <strong>of</strong>ten referred to as the thermal energy<br />
because it depends primarily on the temperature. <strong>Neutron</strong>s at thermal<br />
equilibrium with their surroundings are thermal neutrons. At 20°C (68°F), a<br />
thermal neutron would have a kinetic energy <strong>of</strong> about 0.025 eV and a velocity<br />
<strong>of</strong> 2200 m·s –1 (4900 mi·h –1 ).<br />
Charlie Chong/ Fion Zhang
The transfer <strong>of</strong> energy from the neutron to the nucleus is greater for light<br />
nuclei. Therefore, low atomic nuclei containing materials such as water,<br />
hydrocarbons, graphite and beryllium are used to reduce neutron energies.<br />
Such materials are called moderators. Hydrogen nuclei have essentially the<br />
same mass as neutrons and can undergo nearly complete kinetic energy<br />
transfer in a single collision. Energy transfer to larger nuclei require many<br />
collisions.<br />
Charlie Chong/ Fion Zhang
<strong>Neutron</strong>- Inelastic Scattering<br />
Here the neutron collides with the nucleus leaving the nucleus in an excited<br />
state. In this process, the nucleus may either stay in the excited state (n,n’) as<br />
a metastable isomer or will immediately emit gamma radiation (n,γn) and<br />
return to the ground or original state.<br />
Keywords:<br />
Excited state - (n,n’)<br />
Emit gamma and return to stable state - (n,n’)<br />
Charlie Chong/ Fion Zhang
Nuclear <strong>Neutron</strong> Absorption<br />
As the neutron has no charge, it can approach the nucleus until the close<br />
range attractive forces <strong>of</strong> the nucleus begin to operate. In this process, the<br />
neutron is captured, forming a compound nucleus. Because there is no<br />
charge barrier, even the slowest neutron can be readily captured.<br />
As the binding energy <strong>of</strong> a neutron into a compound nucleus is nearly 8MeV,<br />
even the capture <strong>of</strong> thermal neutrons can result in a highly excited state for<br />
the nucleus. (the thermal neutron has 0.025~0.1 MeV <strong>of</strong> energy, how this<br />
relate to the 8MeV?)<br />
This excited nucleus can attain relative stability by:<br />
■ ejecting a proton,<br />
■ ejecting an alpha particle, or<br />
■ emitting the excess energy as gamma radiation.<br />
When a particle is ejected, the nucleus becomes a new element; then the<br />
process is also known as nuclear transmutation. The discovery <strong>of</strong><br />
transmutation by slow neutrons led to the realization <strong>of</strong> nuclear fission.<br />
Charlie Chong/ Fion Zhang
As the binding energy <strong>of</strong> a neutron into a compound nucleus is nearly 8MeV,<br />
even the capture <strong>of</strong> thermal neutrons can result in a highly excited state for<br />
the nucleus. (the thermal neutron has 0.025~0.1 MeV <strong>of</strong> energy, how this<br />
relate to the 8MeV?)<br />
Charlie Chong/ Fion Zhang
The simplest capture reaction is that <strong>of</strong> capture <strong>of</strong> slow neutrons with<br />
emission <strong>of</strong> gamma rays (n,γ). Thermal neutron reaction with cobalt is an<br />
example:<br />
59<br />
Co + n → 60 Co + γ → 60 Ni + β - + γ<br />
In heavy nuclei, the capture <strong>of</strong> a slow neutron, followed by the emission <strong>of</strong><br />
gamma radiation, increases the neutron-to-proton ratio — usually making the<br />
nucleus radioactive with decay by electron emission likely. More information<br />
on production <strong>of</strong> radioactive material by neutron capture may be found in the<br />
discussion <strong>of</strong> radioactive materials.<br />
Charlie Chong/ Fion Zhang
As the energy <strong>of</strong> the impinging neutron is made larger, a charged particle can<br />
be ejected. However, a charged particle, because <strong>of</strong> the short range attractive<br />
forces <strong>of</strong> the nuclei, is hindered from leaving the nucleus and processes such<br />
as (n,p), (n,α) and (n,d) can only take place when the incident neutron<br />
supplies sufficient energy to overcome the binding energies <strong>of</strong> the particles in<br />
the nucleus. For heavy nuclei these forces are appreciable and the requisite<br />
neutron energy becomes greater. Thus, for example, a particle ejection is<br />
possible only if the neutron has sufficient energy to overcome the binding<br />
energy <strong>of</strong> the alpha particle; that is, the neutron must be a fast neutron.<br />
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In the (n,α) reaction, the product nucleus contains one neutron and two<br />
protons less than the original nucleus. The neutron-to-proton ratio is<br />
increased and the transmutation usually produces a radioactive nucleus that<br />
decays by the emission <strong>of</strong> an electron (beta disintegration).<br />
As the energy <strong>of</strong> the incident neutron approaches 30 MeV, the compound<br />
nucleus can eject three neutrons (n, 3n) or two neutrons and a proton (n, 2np)<br />
as well as other combinations <strong>of</strong> particles. At even higher energies, more<br />
particles may be ejected until the nucleus essentially disappears (spallation).<br />
Finally, nuclear fission (n,f), where the nucleus breaks up with the release <strong>of</strong><br />
several larger particles and several neutrons, can be induced in certain large<br />
nuclides, such as uranium-235, by neutrons <strong>of</strong> almost any energy, whereas in<br />
other nuclides, fast or energetic neutrons are required.<br />
Charlie Chong/ Fion Zhang
Nuclear Cross Sections<br />
Because <strong>of</strong> many reactions possible for absorbing neutrons and their<br />
complicated energy and mass dependencies, there is no simple way to<br />
present the total absorption effect. However, the probability <strong>of</strong> any interaction<br />
between neutrons and matter can be made qualitative by means <strong>of</strong> the<br />
concept <strong>of</strong> cross sections. The cross section σ is the effective target area <strong>of</strong><br />
the nucleus as seen by the impinging neutron <strong>of</strong> a given energy. The number<br />
<strong>of</strong> interactions per unit time will be nvNσ, where n is the number <strong>of</strong> neutrons<br />
per unit volume moving with velocity v towards the target <strong>of</strong> N nuclei. The<br />
quantity nv is the neutron flux density (neutrons per square centimeter<br />
second). The cross section σ is usually expressed in square meters (m 2 ) or<br />
barns (b), where 1 b = 10 –24 cm 2 =10 –28 m 2 .<br />
Charlie Chong/ Fion Zhang
In discussing the variation <strong>of</strong> nuclear cross section with energy <strong>of</strong> the incident<br />
neutrons, certain generalizations <strong>of</strong> a broad character can be made. In<br />
general, there are three regions that can be distinguished.<br />
■ First is the low energy region, which includes the thermal range, where<br />
the cross section decreases steadily with increasing neutron energy. The total<br />
cross section is the sum <strong>of</strong> two terms, one due to neutron scattering is quite<br />
small and almost constant, the other representing absorption by the nucleus<br />
is inversely proportional to the velocity (energy) . This low energy range is<br />
termed the v –1 region, where the time spent by the neutron near the nucleus<br />
is proportional to v–1.<br />
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Second, following the somewhat indefinite v –1 region, many elements exhibit<br />
peaks called resonance peaks, where the neutron cross sections rise sharply<br />
to high values for certain energies, then fall to lower values again. Depending<br />
on the element, the number <strong>of</strong> such peaks may number three or more. These<br />
peaks may be found mostly in the energy range 0.1 to 1 eV, although in a few<br />
elements like uranium-238, they may be found up to energies <strong>of</strong> 10 eV. These<br />
reactions are <strong>of</strong> the (η,γ) (Eta, gamma) type.<br />
And third, with neutrons <strong>of</strong> high energy in the MeV range, the cross sections<br />
are very low, less than 10 –27 m 2 (10 b), compared to the very high cross<br />
sections <strong>of</strong> 4 × 10 –25 m 2 (several thousand barns, ~4000 b) at low energies.<br />
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A simple example <strong>of</strong> the total absorption cross section is that <strong>of</strong> cadmium,<br />
shown in Fig. 5. The v –1 region is shown up to about 0.03 eV, the resonance<br />
at 0.176 eV and the low cross section region for energies greater than about<br />
2 MeV. The dramatic increase in cross sections at the resonance have been<br />
worked out by the theory <strong>of</strong> G. Breit and E.P. Wigner. In its simplicity, if the<br />
energy <strong>of</strong> the neutron is such that a compound nucleus can be formed at or<br />
near one <strong>of</strong> its energy levels, then the probability <strong>of</strong> capture <strong>of</strong> these neutrons<br />
will be exceptionally high.<br />
All elements do not show the resonant absorption effect; for example, boron<br />
has no measurable resonance and the cross section follows the v –1 law from<br />
0.01 eV to over 1000 eV. However, its cross section for (n,α) is so large for<br />
neutrons <strong>of</strong> low energy that this reaction is <strong>of</strong>ten used for neutron detectors.<br />
Table 6 shows the dramatic variation <strong>of</strong> cross section for absorbing thermal<br />
neutrons <strong>of</strong> some <strong>of</strong> the better neutron absorbers.<br />
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FIGURE 5. Absorption <strong>of</strong> neutrons by cadmium, showing resonance peak at<br />
0.176 eV.<br />
0.176 eV<br />
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TABLE 6. Capture cross sections σ <strong>of</strong> strongly absorbing elements for<br />
neutrons in approximate thermal equilibrium at 300 K (27 °C = 80 °F).<br />
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<strong>Neutron</strong> Activation<br />
In the section on neutron interactions with materials, neutron capture was<br />
briefly discussed. This technique, coupled with the large fields <strong>of</strong> neutrons<br />
available in nuclear reactors, produces most <strong>of</strong> the radioisotopes used in<br />
radiography. cobalt-60 and iridium-192 come from thermal neutron<br />
bombardment <strong>of</strong> the stable isotopes (cobalt-59 and iridium-191) <strong>of</strong> these two<br />
elements. Production <strong>of</strong> the radioactivity can be predicted by Eq. 21:<br />
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in which<br />
A is the activity produced in disintegrations per second,<br />
N is number <strong>of</strong> target atoms being bombarded,<br />
f is the neutron flux (in neutrons per centimeter second),<br />
σ is the cross section for neutron capture (in square centimeter),<br />
t i is the irradiation time in the same units as the half life and<br />
T is the half life <strong>of</strong> the radioisotope produced.<br />
The exponential portion <strong>of</strong> the equation corrects the production <strong>of</strong> the<br />
radioactive material for the amount that decays away while more is being<br />
made. This leads to the point <strong>of</strong> diminishing returns for production in that after<br />
about five half lives, almost as much <strong>of</strong> the radioactive material is decaying as<br />
is being produced per each increment <strong>of</strong> neutron bombardment time.<br />
Charlie Chong/ Fion Zhang
Also, the equation is correct only for thin samples <strong>of</strong> the bombarded material.<br />
Absorption <strong>of</strong> neutrons in the outer layers <strong>of</strong> the sample (usually a metal<br />
pellet) reduces the number <strong>of</strong> neutrons incident on the interior atoms. This<br />
self-shielding <strong>of</strong> neutrons coupled with a self-absorption <strong>of</strong> gamma rays<br />
released by radioactive atoms inside <strong>of</strong> the sample gives a gamma output<br />
considerably lower than calculated.<br />
Charlie Chong/ Fion Zhang
Fission Fragments<br />
When uranium-235 or other fissionable atom undergoes fission, multiple<br />
neutrons and two major fragments <strong>of</strong> the nucleus are released. The two<br />
fragments are called fission fragments and are a source <strong>of</strong> radioactive<br />
materials for industrial, medical and research use. The fragments are usually<br />
<strong>of</strong> unequal size and are grouped in two distributions around mass numbers<br />
96 and 138. One <strong>of</strong> the major products is cesium-137, which can be<br />
chemically separated from the other fission fragments for use as a gamma<br />
ray source in radiography, medical therapy and large irradiation facilities for<br />
preservation <strong>of</strong> food and for sterilization <strong>of</strong> medical supplies.<br />
Fission Fragment: cesium-137<br />
Charlie Chong/ Fion Zhang
Accelerator Production<br />
Large particle accelerators such as linatrons, van de graaff generators and<br />
cyclotrons can provide appreciable neutron fluxes or streams <strong>of</strong> high energy<br />
particles including protons, deuterons and helium nuclei. When appropriate<br />
target materials are bombarded by these particles, radioactive nuclei can be<br />
produced. Although radioactive materials for medical use are being produced<br />
in this fashion, generally radiographic sources are not commercially produced<br />
in this fashion.<br />
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The Measurement Units<br />
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Rolf Maximilian Sievert
Sievert - (Sv) is an unit for health effect <strong>of</strong> ionizing radiation,<br />
numerically it is the energy absorbed by human body (by matters?) <strong>of</strong><br />
1J·Kg -1<br />
The sievert (symbol: Sv is a derived unit <strong>of</strong> ionizing radiation dose in the<br />
International System <strong>of</strong> Units (SI). It is a measure <strong>of</strong> the health effect <strong>of</strong> low<br />
levels <strong>of</strong> ionizing radiation on the human body.<br />
Quantities that are measured in sieverts are intended to represent the<br />
stochastic 随 机 的 health risk, which for radiation dose assessment is defined<br />
as the probability <strong>of</strong> cancer induction and genetic damage.<br />
To enable consideration <strong>of</strong> stochastic health risk, calculations are performed<br />
to convert the physical quantity absorbed dose into equivalent and effective<br />
doses, the details <strong>of</strong> which depend on the radiation type and biological<br />
context. For applications in radiation protection and dosimetry assessment<br />
the International Commission on Radiological Protection (ICRP) and<br />
International Commission on Radiation Units and Measurements (ICRU) have<br />
published recommendations and data which are used to calculate these.<br />
These are under continual review, and changes are advised in the formal<br />
"Reports" <strong>of</strong> those bodies.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Sievert
The sievert is used for radiation dose quantities such as equivalent dose,<br />
effective dose, and committed dose.<br />
It is used to represent both the risk <strong>of</strong> the effect <strong>of</strong> external radiation from<br />
sources outside the body and the effect <strong>of</strong> internal irradiation due to inhaled<br />
or ingested radioactive substances.<br />
Conventionally, the sievert is not used for high dose rates <strong>of</strong> radiation that<br />
produce deterministic effects, which is the severity <strong>of</strong> acute tissue damage<br />
that is certain to happen. Such effects are compared to the physical quantity<br />
absorbed dose measured by the unit gray (Gy).<br />
The sievert is <strong>of</strong> fundamental importance in dosimetry and radiation protection,<br />
and is named after Rolf Maximilian Sievert, a Swedish medical physicist<br />
renowned for work on radiation dosage measurement and research into the<br />
biological effects <strong>of</strong> radiation. One sievert carries with it a 5.5% chance <strong>of</strong><br />
eventually developing cancer.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Sievert
One Sievert equals 100 rem. The rem is an older, non-SI unit <strong>of</strong><br />
measurement.<br />
To enable a comprehensive view <strong>of</strong> the Sievert this article deals with the<br />
definition <strong>of</strong> the Sievert as an SI unit, summarises the recommendations <strong>of</strong><br />
the ICRU and ICRP on how the Sievert is calculated, includes a guide to the<br />
effects <strong>of</strong> ionizing radiation as measured in Sievert, and gives examples <strong>of</strong><br />
approximate figures <strong>of</strong> dose uptake in certain situations.<br />
The gray - quantity "D"<br />
1 Gy = 1 joule/kilogram - a physical quantity. 1 Gy is the deposit <strong>of</strong> a joule <strong>of</strong><br />
radiation energy in a kg <strong>of</strong> matter or tissue.<br />
The sievert - quantity "H"<br />
1 Sv = 1 joule/kilogram - a biological effect. The Sievert represents the<br />
equivalent biological effect <strong>of</strong> the deposit <strong>of</strong> a joule <strong>of</strong> radiation energy in a<br />
kilogram <strong>of</strong> human tissue. The equivalence to absorbed dose is denoted by Q.<br />
H = Q × D<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Sievert
REM - Roentgen equivalent man<br />
The roentgen equivalent in man (abbreviated rem; symbol rem, or <strong>of</strong>ten but<br />
incorrectly R) is an older, CGS unit <strong>of</strong> equivalent dose, effective dose, and<br />
committed dose. Quantities measured in rem are designed to represent the<br />
stochastic biological effects <strong>of</strong> ionizing radiation, primarily radiation-induced<br />
cancer. These quantities are a complex weighted average <strong>of</strong> absorbed dose,<br />
which is a clear physical quantity measured in rads. There is no universally<br />
applicable conversion constant from rad to rem; the conversion depends on<br />
relative biological effectiveness (RBE).<br />
The rem is defined since 1976 as equal to 0.01 sievert, which is the more<br />
commonly used SI unit outside <strong>of</strong> the United States. A number <strong>of</strong> earlier<br />
definitions going back to 1945 were derived from the roentgen unit, which<br />
was named after Wilhelm Röntgen, a German scientist who discovered X-<br />
rays. The acronym is now a misleading historical artifact, since 1 roentgen<br />
actually deposits about 0.96 rem in s<strong>of</strong>t biological tissue, when all weighting<br />
factors equal unity. Older units <strong>of</strong> rem following other definitions are up to<br />
17% smaller than the modern rem.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Roentgen_equivalent_man
One rem carries with it a 0.055% chance <strong>of</strong> eventually developing cancer.<br />
Doses greater than 100 rem received over a short time period are likely to<br />
cause acute radiation syndrome (ARS), possibly leading to death within<br />
weeks if left untreated. Note that the quantities that are measured in rem were<br />
not designed to be correlated to ARS symptoms. The absorbed dose,<br />
measured in rad, is the best indicator <strong>of</strong> ARS.<br />
A rem is a large dose <strong>of</strong> radiation, so the millirem (mrem), which is one<br />
thousandth <strong>of</strong> a rem, is <strong>of</strong>ten used for the dosages commonly encountered,<br />
such as the amount <strong>of</strong> radiation received from medical x-rays and background<br />
sources.<br />
Charlie Chong/ Fion Zhang
Rem Usage<br />
The rem and millirem are CGS units in widest use among the American public,<br />
industry, and government. SI units are the norm outside <strong>of</strong> the United States,<br />
and they are increasingly encountered within the US in academic, scientific,<br />
and engineering environments.<br />
The conventional units for dose rate is mrem/h. Regulatory limits and chronic<br />
doses are <strong>of</strong>ten given in units <strong>of</strong> mrem/yr or rem/yr, where they are<br />
understood to represent the total amount <strong>of</strong> radiation allowed (or received)<br />
over the entire year. In many occupational scenarios, the hourly dose rate<br />
might fluctuate to levels thousands <strong>of</strong> times higher for a brief period <strong>of</strong> time,<br />
without infringing on the annual total exposure limits.<br />
Charlie Chong/ Fion Zhang
There is no exact conversion from hours to years because <strong>of</strong> leap years, but<br />
approximate conversions are:<br />
1 mrem/h = 8766 mrem/yr<br />
0.1141 mrem/h = 1000 mrem/yr<br />
The ICRP once adopted fixed conversion for occupational exposure, although<br />
these have not appeared in recent documents:<br />
8 h = 1 day<br />
40 h = 1 week<br />
50 week = 1 yr<br />
Therefore, for occupation exposures <strong>of</strong> that time period,<br />
1 mrem/h = 2000 mrem/yr<br />
0.5 mrem/h = 1000 mrem/yr<br />
Charlie Chong/ Fion Zhang
The US National Institute <strong>of</strong> Standards and Technology (NIST) strongly<br />
discourages Americans from expressing doses in rem, in favor <strong>of</strong><br />
recommending the SI unit. The NIST recommends defining the rem in relation<br />
to the SI in every document where this unit is used. For US industries and US<br />
firms that do not require the sole use <strong>of</strong> SI, however, the unit rem is <strong>of</strong>ten<br />
preferred.<br />
Charlie Chong/ Fion Zhang
Health Effects<br />
Ionizing radiation has deterministic and stochastic effects on human health.<br />
The deterministic effects that can lead to acute radiation syndrome only occur<br />
in the case <strong>of</strong> high doses (> ~10 rad or > 0.1 Gy) and high dose rates (> ~10<br />
rad/h or > 0.1 Gy/h). A model <strong>of</strong> deterministic risk would require different<br />
weighting factors (not yet established) than are used in the calculation <strong>of</strong><br />
equivalent and effective dose.<br />
To avoid confusion, deterministic effects (either chronic & acute?) are<br />
normally compared to absorbed dose in units <strong>of</strong> rad, not rem.<br />
Stochastic effects are those that occur randomly, such as radiation-induced<br />
cancer. The consensus <strong>of</strong> the nuclear industry, nuclear regulators, and<br />
governments, is that the incidence <strong>of</strong> cancers due to ionizing radiation (not<br />
including excessive high dose rate?) can be modeled as increasing linearly<br />
with effective dose at a rate <strong>of</strong> 0.055% per rem (5.5%/Sv). Individual studies,<br />
alternate models, and earlier versions <strong>of</strong> the industry consensus have<br />
produced other risk estimates scattered around this consensus model.<br />
Charlie Chong/ Fion Zhang
There is general agreement that the risk is much higher for infants and<br />
fetuses than adults, higher for the middle-aged than for seniors, and higher<br />
for women than for men, though there is no quantitative consensus about this.<br />
There is much less data, and much more controversy, regarding the<br />
possibility <strong>of</strong> cardiac and teratogenic 引 起 畸 型 的 effects, and the modelling <strong>of</strong><br />
internal dose<br />
The International Commission on Radiological Protection (ICRP)<br />
recommends limiting artificial irradiation <strong>of</strong> the public to an average <strong>of</strong> 100<br />
mrem (1 mSv) (0.1Rem for public and 5Rem for radiation worker?) <strong>of</strong><br />
effective dose per year, not including medical and occupational exposures.<br />
For comparison, radiation levels inside the US United States Capitol are 85<br />
mrem/yr (0.85 mSv/yr), close to the regulatory limit, because <strong>of</strong> the uranium<br />
content <strong>of</strong> the granite structure. According to the ICRP model, someone who<br />
spent 20 years inside the capitol building would have an extra one in a<br />
thousand chance <strong>of</strong> getting cancer, over and above any other existing risk.<br />
(20 yr × 85 mrem/yr × 0.001 rem/mrem × 0.055%/rem = ~0.1%) That<br />
"existing risk" is much higher; an average person would have a one in ten<br />
chance <strong>of</strong> getting cancer during this same 20-year period, even without any<br />
exposure to artificial radiation.<br />
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Radiation-related Quantities<br />
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Radiation-related Quantities<br />
1 gray = 100 rad<br />
J·Kg -1 = 100,000 erg·Kg -1<br />
Joule = 1 x 10 -5 erg<br />
1 Rongent ≠ 1 Rad<br />
Charlie Chong/ Fion Zhang
The Röntgen equivalent physical or rep (symbol rep) is a unit <strong>of</strong><br />
absorbed dose first introduced by Herbert Parker in 1945 to replace an<br />
improper application <strong>of</strong> the roentgen unit to biological tissue. It is the<br />
absorbed energetic dose before the biological efficiency <strong>of</strong> the radiation is<br />
factored in. The rep has variously been defined as 83 or 93 ergs per gram <strong>of</strong><br />
tissue (8.3/9.3 mGy)[2] or per cm 3 <strong>of</strong> tissue. At the time, this was thought to<br />
be the amount <strong>of</strong> energy deposited by 1 roentgen.<br />
Improved measurements have since found that one roentgen <strong>of</strong> air kerma<br />
deposits 8.77 mGy in dry air, or 9.6 mGy in s<strong>of</strong>t tissue, but the rep was<br />
defined as a fixed number <strong>of</strong> ergs per unit gram. A 1952 handbook from the<br />
US National Bureau <strong>of</strong> Standards affirms that "The numerical coefficient <strong>of</strong><br />
the rep has been deliberately changed to 93, instead <strong>of</strong> the earlier 83, to<br />
agree with L. H. Gray's 'energy-unit'." It is unclear what was meant by Gray's<br />
'energy unit', since the gray was not defined until the 1970s; perhaps the<br />
gram-roentgen he introduced in 1940? The rep was commonly used until the<br />
1960s, but was gradually displaced by the rad starting in 1954 and later the<br />
gray starting in 1977.<br />
Charlie Chong/ Fion Zhang
Air Kerma means kerma in a given mass <strong>of</strong> air. The unit used to measure<br />
the quantity <strong>of</strong> air kerma is the Gray (Gy). For X-rays with energies less than<br />
300 kiloelectronvolts (keV), 1 Gy = 100 rad. In air, 1 Gy <strong>of</strong> absorbed dose is<br />
delivered by 114 roentgens (R) <strong>of</strong> exposure.<br />
100 rad = 114 R<br />
Kerma - kinetic energy released in the medium<br />
(Kinetic Energy Released per Unit Mass)<br />
1 abbreviation for kinetic energy released in the medium, a quantity that<br />
describes the transfer <strong>of</strong> energy from a photon to a medium as the ratio <strong>of</strong><br />
energy transferred per unit mass at each point <strong>of</strong> interaction.<br />
2 abbreviation for kinetic energy released in matter, a unit <strong>of</strong> quantity referring<br />
to the kinetic energy transferred from photons to charged particles, such as<br />
electrons in Compton interactions, per unit mass. The SI unit for the KERMA<br />
is the gray, and the special unit is the rad.<br />
Charlie Chong/ Fion Zhang<br />
http://medical-dictionary.thefreedictionary.com/KERMA
Kerma Kinetic Energy Released per Unit Mass.<br />
Kerma is a dose variable. Kerma K is the quotient <strong>of</strong> dEtr and dm; whereby<br />
dEtr is the sum <strong>of</strong> the starting values <strong>of</strong> kinetic energies <strong>of</strong> all charged<br />
particles released by indirectly ionizing radiation from the material in a volume<br />
element dV, and dm is the mass <strong>of</strong> the material in this volume element. All<br />
indications for a Kerma must mention the reference material (i.e. the material<br />
dm). The SI unit <strong>of</strong> the kerma is gray (Gy).<br />
Charlie Chong/ Fion Zhang<br />
http://www.euronuclear.org/info/encyclopedia/k/kerma.htm
Teratogenic 引 起 畸 型 的<br />
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Deterministic Effects<br />
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Chronic Effect<br />
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Deterministic Effects<br />
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ionization chambers<br />
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ionization chambers<br />
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ionization chambers<br />
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ionization<br />
chambers<br />
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ionization chambers<br />
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More <strong>Reading</strong> on ionization chambers<br />
Basically, an ionization chamber consists <strong>of</strong> two electrodes kept at a potential<br />
difference and a gas that fills the space between the electrodes. The<br />
detection process occurs when an X-ray photon interacts with the gas inside<br />
the chamber, forming “N” number <strong>of</strong> electron-ion pairs. The electrons and<br />
ions are separated due to the direction and sense <strong>of</strong> the electric field.<br />
Continuous streams <strong>of</strong> photons originate a continuous production <strong>of</strong> electronhole<br />
pairs and consequently an electric current between two electrodes. This<br />
current, typically in the order <strong>of</strong> a few pico-ampere (pA) (10 -12 ) , is proportional<br />
to the photon flux <strong>of</strong> X-rays.<br />
The electrode measuring the current generated by the camera is called the<br />
collector electrode. This electrode (anode?) is typically maintained at a<br />
potential close to the ground. The other electrode (cathode?) is called the<br />
high-voltage electrode, and must be maintained at a positive (?) voltage (to<br />
collect positive charges) or negative (to collect negative charges). These<br />
electrodes are fixed inside the chamber through electrical insulators.<br />
Charlie Chong/ Fion Zhang<br />
http://lnls.cnpem.br/beamlines/xafs/equipments/ion-chambers/
The chamber can be sealed to use different gases at different pressures. The<br />
figure below represents a parallel plate chamber where radiation passes<br />
between the electrodes. There are two windows, one where the beam<br />
reaches the sensitive volume and the other where the beam exits the<br />
chamber. These windows should be composed <strong>of</strong> a material <strong>of</strong> low atomic<br />
number and should be thin, so not to reduce the intensity <strong>of</strong> radiation. Note<br />
that this type <strong>of</strong> chamber is not stopping the X-ray beam.<br />
Charlie Chong/ Fion Zhang<br />
http://lnls.cnpem.br/beamlines/xafs/equipments/ion-chambers/
Schematic diagram <strong>of</strong> an ionization chamber with parallel plates.<br />
Charlie Chong/ Fion Zhang<br />
http://lnls.cnpem.br/beamlines/xafs/equipments/ion-chambers/
The Ionization Chamber is the simplest <strong>of</strong> all gas-filled radiation<br />
detectors, and is widely used for the detection and measurement <strong>of</strong> certain<br />
types <strong>of</strong> ionizing radiation; X-rays, gamma rays and beta particles.<br />
Conventionally, the term "ionization chamber" is used exclusively to describe<br />
those detectors which collect all the charges created by direct ionization<br />
within the gas through the application <strong>of</strong> an electric field.<br />
It only uses the discrete charges created by each interaction between the<br />
incident radiation and the gas, and does not involve the gas multiplication<br />
mechanisms used by other radiation instruments, such as the Geiger-Müller<br />
counter or the proportional counter.<br />
Ion chambers have a good uniform response to radiation over a wide range <strong>of</strong><br />
energies and are the preferred means <strong>of</strong> measuring high levels <strong>of</strong> gamma<br />
radiation. They are widely used in the nuclear power industry, research labs,<br />
radiography, radiobiology, and environmental monitoring.<br />
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https://en.wikipedia.org/wiki/Ionization_chamber
The Ionization Chamber<br />
• Detectors which collect all the charges created by direct ionization within<br />
the gas through the application <strong>of</strong> an electric field.<br />
• It only uses the discrete charges created by each interaction between the<br />
incident radiation and the gas,<br />
• It does not involve the gas multiplication mechanisms used by other<br />
radiation instruments, such as the Geiger-Müller counter or the<br />
proportional counter.<br />
• Ion chambers have a good uniform response to radiation over a wide<br />
range <strong>of</strong> energies<br />
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The Ionization Chamber<br />
• It does not involve the gas multiplication mechanisms used by other<br />
radiation instruments, such as the Geiger-Müller counter or the<br />
proportional counter.<br />
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Schematic diagram <strong>of</strong> parallel plate ion chamber, showing drift <strong>of</strong> ions.<br />
Electrons typically drift 1000 times faster than positive ions due to their much<br />
smaller mass.<br />
https://en.wikipedia.org/wiki/Ionization_chamber
Principle <strong>of</strong> operation<br />
An ionization chamber measures the charge from the number <strong>of</strong> ion pairs<br />
created within a gas caused by incident radiation. It consists <strong>of</strong> a gas-filled<br />
chamber with two electrodes; known as anode and cathode. The electrodes<br />
may be in the form <strong>of</strong> parallel plates (Parallel Plate Ionization Chambers:<br />
PPIC), or a cylinder arrangement with a coaxially located internal anode wire.<br />
coaxially located<br />
Parallel Plate<br />
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A voltage potential is applied between the electrodes to create an electric<br />
field in the fill gas. When gas between the electrodes is ionized by incident<br />
ionizing radiation, ion-pairs are created and the resultant positive ions and<br />
dissociated electrons move to the electrodes <strong>of</strong> the opposite polarity under<br />
the influence <strong>of</strong> the electric field. This generates an ionization current which is<br />
measured by an electrometer circuit. The electrometer must be capable <strong>of</strong><br />
measuring the very small output current which is in the region <strong>of</strong> femto<br />
amperes (10 -15 ) to pico amperes (10 -12 ) , depending on the chamber design,<br />
radiation dose and applied voltage.<br />
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Each ion pair created deposits or removes a small electric charge to or from<br />
an electrode, such that the accumulated charge is proportional to the number<br />
<strong>of</strong> ion pairs created, and hence the radiation dose. This continual generation<br />
<strong>of</strong> charge produces an ionization current, which is a measure <strong>of</strong> the total<br />
ionizing dose entering the chamber. However, the chamber cannot<br />
discriminate between radiation types (beta or gamma) and cannot produce an<br />
energy spectrum <strong>of</strong> radiation.<br />
The electric field also enables the device to work continuously by mopping up<br />
electrons, which prevents the fill gas from becoming saturated, where no<br />
more ions could be collected, and by preventing the recombination <strong>of</strong> ion<br />
pairs, which would diminish the ion current.<br />
Current Mode<br />
This mode <strong>of</strong> operation is referred to as "current" mode, meaning that the<br />
output signal is a continuous current, and not a pulse output as in the cases<br />
<strong>of</strong> the Geiger-Müller tube or the proportional counter.<br />
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Referring to the accompanying ion pair collection graph, it can be seen that in<br />
the "ion chamber" operating region the collection <strong>of</strong> ion pairs is effectively<br />
constant over a range <strong>of</strong> applied voltage, as due to its relatively low electric<br />
field strength the ion chamber does not have any "multiplication effect". This<br />
is in distinction to the Geiger-Müller tube or the proportional counter whereby<br />
secondary electrons, and ultimately multiple avalanches, greatly amplify the<br />
original ion-current charge.<br />
Plot <strong>of</strong> ion current against voltage for a wire cylinder gaseous radiation<br />
detector. The ion chamber uses the lowest usable detection region.<br />
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Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Ionization_chamber
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Ionization_chamber
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Chamber types and construction<br />
The following chamber types are commonly used.<br />
Free-air chamber<br />
This is a chamber freely open to atmosphere, where the fill gas is ambient air.<br />
The domestic smoke detector is a good example <strong>of</strong> this, where a natural flow<br />
<strong>of</strong> air through the chamber is necessary so that smoke particles can be<br />
detected by the change in ion current. Other examples are applications where<br />
the ions are created outside the chamber but are carried in by a forced flow <strong>of</strong><br />
air or gas.<br />
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Chamber pressure<br />
■ Vented chamber<br />
These chambers are normally cylindrical and operate at atmospheric<br />
pressure, but to prevent ingress <strong>of</strong> moisture a filter containing a desiccant is<br />
installed in the vent line. This is to stop moisture building up in the interior <strong>of</strong><br />
the chamber, which would otherwise be introduced by the "pump" effect <strong>of</strong><br />
changing atmospheric air pressure. These chambers have a cylindrical body<br />
made <strong>of</strong> aluminium or plastic a few millimetres thick. The material is selected<br />
to have an atomic number similar to that <strong>of</strong> air so that the wall is said to be<br />
"air equivalent" over a range <strong>of</strong> radiation beam energies. This has the effect<br />
<strong>of</strong> ensuring the gas in the chamber is acting as though it were a portion <strong>of</strong> an<br />
infinitely large gas volume, and increases the accuracy by reducing<br />
interactions <strong>of</strong> gamma with the wall material. The higher the atomic number <strong>of</strong><br />
the wall material, the greater the chance <strong>of</strong> interaction. The wall thickness is a<br />
trade-<strong>of</strong>f between maintaining the air effect with a thicker wall, and increasing<br />
sensitivity by using a thinner wall.<br />
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These chambers <strong>of</strong>ten have an end window made <strong>of</strong> material thin enough,<br />
such as mylar, so that beta particles can enter the gas volume. Gamma<br />
radiation enters both through the end window and the side walls. For handheld<br />
instruments the wall thickness is made as uniform as possible to reduce<br />
photon directionality though any beta window response is obviously highly<br />
directional. Vented chambers are susceptible to small changes in efficiency<br />
with air pressure and correction factors can be applied for very accurate<br />
measurement applications.<br />
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■ Sealed low pressure chamber<br />
These are similar in construction to the vented chamber but are sealed and<br />
operate at or around atmospheric pressure. They contain a special fill gas to<br />
improve detection efficiency as free electrons are easily captured in air-filled<br />
vented chambers by neutral oxygen which is electronegative, to form negative<br />
ions (?) . These chambers also have the advantage <strong>of</strong> not requiring a vent<br />
and desiccant. The beta end window limits the differential pressure from<br />
atmospheric pressure that can be tolerated, and common materials are<br />
stainless steel or titanium with a typical thickness <strong>of</strong> 25 µm.<br />
■ High pressure chamber<br />
The efficiency <strong>of</strong> the chamber can be further increased by the use <strong>of</strong> a high<br />
pressure gas. Typically a pressure <strong>of</strong> 8-10 atmospheres can be used, and<br />
various noble gases are employed. The higher pressure results in a greater<br />
gas density and thereby a greater chance <strong>of</strong> collision with the fill gas and ion<br />
pair creation by incident radiation. Because <strong>of</strong> the increased wall thickness<br />
required to withstand this high pressure, only gamma radiation can be<br />
detected. These detectors are used in survey meters and for environmental<br />
monitoring.<br />
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Instrument types<br />
Ion chambers are widely used in hand held radiation survey meters to<br />
measure beta and gamma radiation. They are particularly preferred for high<br />
dose rate measurements and for gamma radiation they give good accuracy<br />
for energies above 50-100 keV.<br />
There are two basic configurations; the "integral" unit with the chamber and<br />
electronics in the same case, and the "two-piece" instrument which has a<br />
separate ion chamber probe attached to the electronics module by a flexible<br />
cable.<br />
The chamber <strong>of</strong> the integral instrument is generally at the front <strong>of</strong> the case<br />
facing downwards, and for beta/gamma instruments there is a window in the<br />
bottom <strong>of</strong> the casing. This usually has a sliding shield which enables<br />
discrimination between gamma and beta radiation. The operator closes the<br />
shield to exclude beta, and can thereby calculate the rate <strong>of</strong> each radiation<br />
type.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Ionization_chamber
Some hand held instruments generate audible clicks similar to that produced<br />
by a G-M counter to assist operators, who use the audio feedback in radiation<br />
survey and contamination checks. As the ion chamber works in current mode,<br />
not pulse mode, this is synthesised from the radiation rate.<br />
Installed<br />
For industrial process measurements and interlocks with sustained high<br />
radiation levels, the ion chamber is the preferred detector. In these<br />
applications only the chamber is situated in the measurement area, and the<br />
electronics are remotely situated to protect them from radiation and<br />
connected by a cable. Installed instruments can be used for measuring<br />
ambient gamma for personnel protection and normally sound an alarm above<br />
a preset rate, though the Geiger-Müller tube instrument is generally preferred<br />
where high levels <strong>of</strong> accuracy are not required.<br />
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https://en.wikipedia.org/wiki/Ionization_chamber
Hand-held integral ion chamber survey meter in use<br />
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https://en.wikipedia.org/wiki/Ionization_chamber
View <strong>of</strong> sliding beta shield on integral hand held instrument<br />
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https://en.wikipedia.org/wiki/Ionization_chamber
General precautions in use<br />
Moisture is the main problem that affects the accuracy <strong>of</strong> ion chambers. The<br />
chamber's internal volume must be kept completely dry, and the vented type<br />
uses a desiccant to help with this.[3] Because <strong>of</strong> the very low currents<br />
generated, any stray leakage current must be kept to a minimum in order to<br />
preserve accuracy. Invisible hygroscopic moisture on the surface <strong>of</strong> cable<br />
dielectrics and connectors can be sufficient to cause a leakage current which<br />
will swamp any radiation-induced ion current. This requires scrupulous<br />
cleaning <strong>of</strong> the chamber, its terminations and cables, and subsequent drying<br />
in an oven. "Guard rings" are generally used as a design feature on higher<br />
voltage tubes to reduce leakage through or along the surface <strong>of</strong> tube<br />
connection insulators which can require a resistance in the order <strong>of</strong> 10 13 Ω.<br />
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For industrial applications with remote electronics, the ion chamber is housed<br />
in a separate enclosure which provides mechanical protection and contains a<br />
desiccant to remove moisture which could affect the termination resistance.<br />
In installations where the chamber is a long distance from the measuring<br />
electronics, readings can be affected by external electromagnetic radiation<br />
acting on the cable. To overcome this a local converter module is <strong>of</strong>ten used<br />
to translate the very low ion chamber currents to a pulse train or data signal<br />
related to the incident radiation. These are immune to electromagnetic effects.<br />
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Applications<br />
Nuclear industry<br />
Ionization chambers are widely used in the nuclear industry as they provide<br />
an output that is proportional to radiation dose. They find wide use in<br />
situations where a constant high dose rate is being measured as they have a<br />
greater operating lifetime than standard Geiger-Müller tubes, which suffer<br />
from gas break down and are generally limited to a life <strong>of</strong> about 10 11 count<br />
events. Additionally, the Geiger-Müller tube cannot operate above about 10 4<br />
counts per second, due to dead time effects, whereas there is no similar<br />
limitation on the ion chamber.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Ionization_chamber
Keywords:<br />
• Ionization Chamber provides an output that is proportional to radiation<br />
dose.<br />
• Geiger-Müller tubes, which suffer from gas break down and are generally<br />
limited to a life <strong>of</strong> about 10 11 count events.<br />
• Geiger-Müller tube cannot operate above about 10 4 counts per second<br />
(10 4 N·s -1 ) , due to dead time effects, whereas there is no similar limitation<br />
on the ion chamber.<br />
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Smoke detectors<br />
The ionization chamber has found wide and beneficial use in smoke detectors.<br />
In a smoke detector, ambient air is allowed to freely enter the ionization<br />
chamber. The chamber contains a small amount <strong>of</strong> americium-241, which is<br />
an emitter <strong>of</strong> alpha particles which produce a constant ion current. If smoke<br />
enters the detector, it disrupts this current because ions strike smoke particles<br />
and are neutralized. This drop in current triggers the alarm. The detector also<br />
has a reference chamber which is sealed but is ionized in the same way.<br />
Comparison <strong>of</strong> the ion currents in the two chambers allows compensation for<br />
changes due to air pressure, temperature, or the ageing <strong>of</strong> the source.<br />
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https://en.wikipedia.org/wiki/Ionization_chamber
Medical radiation measurement<br />
In medical physics and radiotherapy, ionization chambers are used to ensure<br />
that the dose delivered from a therapy unit or radiopharmaceutical is what is<br />
intended. The devices used for radiotherapy are called "reference<br />
dosimeters", while those used for radiopharmaceuticals are called<br />
radioisotope dose calibrators. A chamber will have a calibration factor<br />
established by a national standards laboratory such as ARPANSA in Australia<br />
or the NPL in the UK, or will have a factor determined by comparison against<br />
a transfer standard chamber traceable to national standards at the user's site.<br />
Guidance on application use<br />
In the United Kingdom the HSE has issued a user guide on selecting the<br />
correct radiation measurement instrument for the particular application<br />
concerned. This covers all radiation instrument technologies, and is a useful<br />
comparative guide to the use <strong>of</strong> ion chamber instruments.<br />
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The Geiger counter is an instrument used for measuring ionizing<br />
radiation used widely in such applications as radiation dosimetry, radiological<br />
protection, experimental physics and the nuclear industry.<br />
It detects ionizing radiation such as alpha particles, beta particles and gamma<br />
rays using the ionization effect produced in a Geiger–Müller tube; which gives<br />
its name to the instrument. In wide and prominent use as a hand-held<br />
radiation survey instrument, it is perhaps one <strong>of</strong> the world's best-known<br />
radiation detection instruments.<br />
The original detection principle was discovered in 1908, but it was not until<br />
the development <strong>of</strong> the Geiger-Müller tube in 1928 that the Geiger-Müller<br />
counter became a practical instrument. Since then it has been very popular<br />
due to its robust sensing element and relatively low cost.<br />
However, there are limitations in measuring high radiation rates and the<br />
energy <strong>of</strong> incident radiation.<br />
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A "two-piece" bench type Geiger–Müller counter with end-window detector<br />
Charlie Chong/ Fion Zhang
Schematic <strong>of</strong> a Geiger counter using an "end window" tube for low<br />
penetration radiation. A loudspeaker is also used for indication<br />
Charlie Chong/ Fion Zhang
Principle <strong>of</strong> operation<br />
A Geiger counter consists <strong>of</strong> a Geiger-Müller tube, the sensing element which<br />
detects the radiation, and the processing electronics, which displays the<br />
result.<br />
The Geiger-Müller tube is filled with an inert gas such as helium, neon, or<br />
argon at low pressure, to which a high voltage is applied.<br />
The tube briefly conducts electrical charge when a particle or photon <strong>of</strong><br />
incident radiation makes the gas conductive by ionization. The ionization is<br />
considerably amplified within the tube by the Townsend discharge effect to<br />
produce an easily measured detection pulse, which is fed to the processing<br />
and display electronics. This large pulse from the tube makes the G-M<br />
counter relatively cheap to manufacture, as the subsequent electronics is<br />
greatly simplified. The electronics also generates the high voltage, typically<br />
400–600 volts, that has to be applied to the Geiger-Müller tube to enable its<br />
operation.<br />
Charlie Chong/ Fion Zhang
Readout<br />
There are two types <strong>of</strong> radiation readout; counts or radiation dose.<br />
The counts display is the simplest and is the number <strong>of</strong> ionizing events<br />
displayed either as a count rate, commonly "counts per second", or as a total<br />
over a set time period (an integrated total). The counts readout is normally<br />
used when alpha or beta particles are being detected. More complex to<br />
achieve is a display <strong>of</strong> radiation dose rate, displayed in a unit such as the<br />
sievert which is normally used for measuring gamma or X-ray dose rates. A<br />
G-M tube can detect the presence <strong>of</strong> radiation, but not its energy which<br />
influences the radiation's ionising effect. Consequently, instruments<br />
measuring dose rate require the use <strong>of</strong> an energy compensated G-M tube, so<br />
that the dose displayed relates to the counts detected. The electronics will<br />
apply known factors to make this conversion, which is specific to each<br />
instrument and is determined by design and calibration.<br />
The readout can be analog or digital, and increasingly, modern instruments<br />
are <strong>of</strong>fering serial communications with a host computer or network.<br />
Charlie Chong/ Fion Zhang
There is usually an option to produce audible clicks representing the number<br />
<strong>of</strong> ionization events detected. This is the distinctive sound normally<br />
associated with hand held or portable Geiger counters. The purpose <strong>of</strong> this is<br />
to allow the user to concentrate on manipulation <strong>of</strong> the instrument whilst<br />
retaining auditory feedback on the radiation rate.<br />
Limitations<br />
There are two main limitations <strong>of</strong> the Geiger counter. Because the output<br />
pulse from a Geiger-Müller tube is always the same magnitude regardless <strong>of</strong><br />
the energy <strong>of</strong> the incident radiation, the tube cannot differentiate between<br />
radiation types. A further limitation is the inability to measure high radiation<br />
rates due to the "dead time" <strong>of</strong> the tube. This is an insensitive period after<br />
each ionization <strong>of</strong> the gas during which any further incident radiation will not<br />
result in a count, and the indicated rate is therefore lower than actual.<br />
Typically the dead time will reduce indicated count rates above about 10 4 to<br />
10 5 counts per second depending on the characteristic <strong>of</strong> the tube being used.<br />
Whilst some counters have circuitry which can compensate for this, for<br />
accurate measurements ion chamber instruments are preferred for high<br />
radiation rates.<br />
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For accurate measurements ion chamber instruments are preferred for<br />
high radiation rates.<br />
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Ionization Chamber<br />
Charlie Chong/ Fion Zhang
Geiger Muller Counter<br />
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G-M counter with pancake type probe<br />
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Laboratory use <strong>of</strong> a G-M counter with end window probe to measure beta<br />
radiation from a radioactive source<br />
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https://en.wikipedia.org/wiki/Geiger_counter
Types and applications<br />
The application and use <strong>of</strong> a Geiger counter is dictated entirely by the design<br />
<strong>of</strong> the tube, <strong>of</strong> which there are a great many, but they can be generally<br />
categorised as "end-window", or windowless "thin-walled" or "thick-walled",<br />
and sometimes hybrids <strong>of</strong> these types.<br />
<strong>Part</strong>icle detection<br />
The first historical uses <strong>of</strong> the Geiger principle were for the detection <strong>of</strong> alpha<br />
and beta particles, and the instrument is still used for this purpose today. For<br />
alpha particles and low energy beta particles the "end-window" type <strong>of</strong> G-M<br />
tube has to be used as these particles have a limited range even in free air,<br />
and are easily stopped by a solid material. Therefore the tube requires a<br />
window which is thin enough to allow as many as possible <strong>of</strong> these particles<br />
through to the fill gas. The window is usually made <strong>of</strong> mica with a density <strong>of</strong><br />
about 1.5 - 2.0 mg/cm 2 .<br />
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Alpha particles have the shortest range, and to detect these the window<br />
should ideally be within 10mm <strong>of</strong> the radiation source due to alpha particle<br />
attenuation in free air. However, the G-M tube produces a pulse output which<br />
is the same magnitude for all detected radiation, so a Geiger counter with an<br />
end window tube cannot distinguish between alpha and beta particles. A<br />
skilled operator can use distance to differentiate alpha and high energy beta,<br />
but with the detector in close contact with the radiation source the types are<br />
indistinguishable. The "pancake" Geiger-Muller detector is a variant <strong>of</strong> the<br />
end window probe, but designed with a larger detection area to make<br />
checking quicker. However the pressure <strong>of</strong> the atmosphere against the low<br />
pressure <strong>of</strong> the fill gas limits the window size due to the limited strength <strong>of</strong> the<br />
window membrane.<br />
High energy beta particles can also be detected by a thin-walled<br />
"windowless" G-M tube, which has no end window. Although the tube walls<br />
have a greater stopping power than a thin end window, they still allow these<br />
more energetic particles to reach the fill gas.<br />
Charlie Chong/ Fion Zhang<br />
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End-window G-M detectors are still used as a general purpose portable<br />
radioactive contamination measurement and detection instrument, owing to<br />
their relatively low cost, robustness and their relatively high detection<br />
efficiency; particularly with high energy beta particles.<br />
However for discrimination between alpha and beta particles or provision <strong>of</strong><br />
particle energy information, (1) scintillation counters or (2) proportional<br />
counters should be used. Those instrument types are manufactured with<br />
much larger detector areas, which means that checking for surface<br />
contamination is quicker than with a G-M instrument.<br />
Keywords:<br />
However for discrimination between alpha and beta particles or provision <strong>of</strong><br />
particle energy information, (1) scintillation counters or (2) proportional<br />
counters should be used.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger_counter
Gamma and X-ray detection<br />
Geiger counters are widely used to detect gamma radiation, and for this the<br />
windowless tube is used. However, efficiency is generally low due to the poor<br />
interaction <strong>of</strong> gamma rays compared with alpha and beta particles. For<br />
instance, a chrome steel G-M tube is only about 1% efficient over a wide<br />
range <strong>of</strong> energies.<br />
The article on the Geiger-Muller tube carries a more detailed account <strong>of</strong> the<br />
techniques used to detect photon radiation. For high energy gamma it largely<br />
relies on interaction <strong>of</strong> the photon radiation with the tube wall material, usually<br />
1–2 mm <strong>of</strong> chrome steel on a "thick-walled" tube, to produce electrons within<br />
the wall which can enter and ionize the fill gas. This is necessary as the low<br />
pressure gas in the tube has little interaction with high energy gamma<br />
photons. However, for low energy photons there is greater gas interaction and<br />
the direct gas ionisation effect increases. With decreasing energy the wall<br />
effect gives way to a combination <strong>of</strong> wall effect and direct ionisation, until<br />
direct gas ionisation dominates. Due to the variance in response to different<br />
photon energies, windowless tubes employ what is known as "energy<br />
compensation" which attempts to compensate for these variations over a<br />
large energy range.<br />
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Low energy photon radiation such as low energy X rays or gamma rays<br />
interacts better with the fill gas. Consequently a typical design for low energy<br />
photon detection for these is a long tube with a thin wall or with an end<br />
window. The tube has a larger gas volume than a steel walled tube to give an<br />
increased chance <strong>of</strong> particle interaction.<br />
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<strong>Neutron</strong> detection<br />
A variation <strong>of</strong> the Geiger tube is used to measure neutrons, where the gas<br />
used is boron trifluoride (BF 3 ) or helium-3 ( 3 He) and a plastic moderator is<br />
used to slow the neutrons. This creates an alpha particle inside the detector<br />
and thus neutrons can be counted.<br />
Geiger tube filled with BF 3 for detection <strong>of</strong> thermal neutrons<br />
10<br />
5 B + n → 7 3 Li + 4 2 α https://www.orau.org/PTP/collection/proportional%20counters/bf3info.htm<br />
3<br />
2 He + n → 3 1 Li + 1 1 P http://large.stanford.edu/courses/2012/ph241/lam1/<br />
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Boron trifluoride Detector<br />
This neutron detector was produced by 20th<br />
Century Electronics in England. The company<br />
began manufacturing BF 3 counters in the early<br />
1950s. It is approximately 16 1/2 inches long, 2<br />
inches in diameter, copper walled and filled with<br />
BF3. One end (towards the right in the above<br />
photo) has a threaded cap to protect the fragile<br />
glass insulator.<br />
The model number, marked on the wall <strong>of</strong> the<br />
tube, is 15EB70/50/G/UA0539. The EB refers to<br />
"enriched boron trifluoride." The 50 refers to the<br />
tube diameter, i.e., 50 mm.<br />
Charlie Chong/ Fion Zhang<br />
https://www.orau.org/PTP/collection/proportional%20counters/bf3twentiethlarge.htm
Gamma measurement—personnel protection and<br />
process control<br />
The term "Geiger counter" is commonly used to mean a hand-held survey<br />
type meter, however the Geiger principle is in wide use in installed "area<br />
gamma" alarms for personnel protection, and in process measurement and<br />
interlock applications. A Geiger tube is still the sensing device, but the<br />
processing electronics will have a higher degree <strong>of</strong> sophistication and<br />
reliability than that used in a hand held survey meter.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger_counter
Physical design<br />
For hand-held units there are two fundamental physical configurations: the<br />
"integral" unit with both detector and electronics in the same unit, and the<br />
"two-piece" design which has a separate detector probe and an electronics<br />
module connected by a short cable.<br />
The integral unit allows single-handed operation, so the operator can use the<br />
other hand for personal security in challenging monitoring positions, but the<br />
two piece design allows easier manipulation <strong>of</strong> the detector, and is commonly<br />
used for alpha and beta surface contamination monitoring where careful<br />
manipulation <strong>of</strong> the probe is required or the weight <strong>of</strong> the electronics module<br />
would make operation unwieldy. A number <strong>of</strong> different sized detectors are<br />
available to suit particular situations, such as placing the probe in small<br />
apertures or confined spaces.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger_counter
Gamma and X-Ray detectors generally use an "integral" design so the<br />
Geiger–Müller tube is conveniently within the electronics enclosure. This can<br />
easily be achieved because the casing usually has little attentuation, and is<br />
employed in ambient gamma measurements where distance from the source<br />
<strong>of</strong> radiation is not a significant factor. However, to facilitate more localised<br />
measurements such as "surface dose", the position <strong>of</strong> the tube in the<br />
enclosure is sometimes indicated by targets on the enclosure so an accurate<br />
measurement can be made with the tube at the correct orientation and a<br />
known distance from the surface.<br />
There is a particular type <strong>of</strong> gamma instrument known as a "hot spot" detector<br />
which has the detector tube on the end <strong>of</strong> a long pole or flexible conduit.<br />
These are used to measure high radiation gamma locations whilst protecting<br />
the operator by means <strong>of</strong> distance shielding.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger_counter
<strong>Part</strong>icle detection <strong>of</strong> alpha and beta can used in both integral and two-piece<br />
designs. A pancake probe (for alpha/beta) is generally used to increase the<br />
area <strong>of</strong> detection in two-piece instruments whilst being relatively light weight.<br />
In integral instruments using an end window tube there is a window in the<br />
body <strong>of</strong> the casing to prevent shielding <strong>of</strong> particles. There are also hybrid<br />
instruments which have a separate probe for particle detection and a gamma<br />
detection tube within the electronics module. The detectors are switchable by<br />
the operator, depending the radiation type that is being measured.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger_counter
Pancake G-M tube used for alpha and beta detection; the delicate mica<br />
window is usually protected by a mesh when fitted in an instrument.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger_counter
Guidance on application use[edit]<br />
In the United Kingdom the HSE has issued a user guidance note on selecting<br />
the best portable instrument type for the radiation measurement application<br />
concerned.[4][3] This covers all radiation protection instrument technologies<br />
and is a useful comparative guide to the use <strong>of</strong> G-M detectors. The guide<br />
does not recommend the G-M detector for mixed alpha and beta<br />
contamination detection, and they are only recommended as "satisfactory" for<br />
beta-only contamination. However for gamma and low-voltage X-rays they<br />
are recommended as the best instrument type.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger_counter
Use <strong>of</strong> a "hot spot" detector on a long pole to survey waste casks<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger_counter
G-M pancake detector feeding a microcontroller data-logger sending data to a<br />
PC via bluetooth. A radioactive rock was placed on top the G-M causing the<br />
graph to rise.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger_counter
G-M counters being used as gamma survey monitors, seeking radioactive<br />
satellite debris<br />
Charlie Chong/ Fion Zhang
Geiger–Müller tube<br />
The Geiger–Müller tube or G–M tube is the sensing element <strong>of</strong> the Geiger<br />
counter instrument used for the detection <strong>of</strong> ionizing radiation. It was named<br />
after Hans Geiger, who invented the principle in 1908, and Walther Müller,<br />
who collaborated with Geiger in developing the technique further in 1928 to<br />
produce a practical tube that could detect a number <strong>of</strong> different radiation<br />
types.<br />
It is a gaseous ionization detector and uses the Townsend avalanche<br />
phenomenon to produce an easily detectable electronic pulse from as little as<br />
a single ionising event due to a radiation particle. It is used for the detection <strong>of</strong><br />
gamma radiation, X-rays, and alpha and beta particles. It can also be adapted<br />
to detect neutrons. The tube operates in the "Geiger" region <strong>of</strong> ion pair<br />
generation. This is shown on the accompanying plot for gaseous detectors<br />
showing ion current against applied voltage.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube
Whilst it is a robust and inexpensive detector, the G–M is:<br />
• unable to measure high radiation rates efficiently,<br />
• has a finite life in high radiation areas and<br />
• is unable to measure incident radiation energy, so no spectral information<br />
can be generated and there is no discrimination between radiation type.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube
Plot <strong>of</strong> ion pair current against applied voltage for a cylindrical gaseous<br />
radiation detector with a central wire anode.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube
Principle <strong>of</strong> operation<br />
The tube consists <strong>of</strong> a chamber filled with an inert gas at low-pressure (about<br />
0.1 atmosphere). The chamber contains two electrodes, between which there<br />
is a potential difference <strong>of</strong> several hundred volts. The walls <strong>of</strong> the tube are<br />
either metal or have their inside surface coated with a conductor to form the<br />
cathode, while the anode is a wire in the center <strong>of</strong> the chamber.<br />
several hundred volts<br />
0.1 atmosphere<br />
Charlie Chong/ Fion Zhang<br />
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When ionizing radiation strikes the tube, some molecules <strong>of</strong> the gas are<br />
ionized, either directly by the incident radiation or indirectly by means <strong>of</strong><br />
secondary electrons produced in the walls <strong>of</strong> the tube. This creates positively<br />
charged ions and electrons, known as “ion pairs”, in the fill gas.<br />
The strong electric field created by the tube's electrodes accelerates the<br />
positive ions towards the cathode and the electrons towards the anode. Close<br />
to the anode in the "avalanche region" the electrons gain sufficient energy to<br />
ionize additional gas molecules and create a large number <strong>of</strong> electron<br />
avalanches which spread along the anode and effectively throughout the<br />
avalanche region. This is the "gas multiplication" effect which gives the tube<br />
its key characteristic <strong>of</strong> being able to produce a significant output pulse from a<br />
single ionising event<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube
If there were to be only one avalanche per original ionising event, then the<br />
number <strong>of</strong> excited molecules would be in the order <strong>of</strong> 10 6 to 10 8 . However the<br />
production <strong>of</strong> multiple avalanches results in an increased multiplication factor<br />
which can produce 10 9 to 10 10 ion pairs.<br />
Keypoint:<br />
Single event multiplication factor: 10 6 to 10 8<br />
Multiple event multiplication factor: 10 9 to 10 10<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube
The creation <strong>of</strong> multiple avalanches is due to the production <strong>of</strong> UV photons in<br />
the original avalanche, which are not affected by the electric field and move<br />
laterally to the axis <strong>of</strong> the anode to instigate further ionising events by<br />
collision with gas molecules. These collisions produce further avalanches,<br />
which in turn produce more photons, and thereby more avalanches in a chain<br />
reaction which spreads laterally through the fill gas, and envelops the anode<br />
wire.<br />
The accompanying diagram shows this graphically. The speed <strong>of</strong> propagation<br />
<strong>of</strong> the avalanches is typically 2–4 cm per microsecond, so that for common<br />
sizes <strong>of</strong> tubes the complete ionisation <strong>of</strong> the gas around the anode takes just<br />
a few microseconds. This short, intense pulse <strong>of</strong> current can be measured as<br />
a count event in the form <strong>of</strong> a voltage pulse developed across an external<br />
electrical resistor. This can be in the order <strong>of</strong> volts, thus making further<br />
electronic processing simple.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube
Visualisation <strong>of</strong> the spread <strong>of</strong> Townsend avalanches by means <strong>of</strong> UV photons.<br />
This mechanism allows a single ionising event to ionise all the gas<br />
surrounding the anode by triggering multiple avalanches.<br />
Spread <strong>of</strong> avalanches<br />
In a GM Tube<br />
Charlie Chong/ Fion Zhang<br />
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The discharge is terminated by the collective effect <strong>of</strong> the positive ions<br />
created by the avalanches. These ions have lower mobility than the free<br />
electrons due to their higher mass and remain in the area <strong>of</strong> the anode wire.<br />
This creates a "space charge" which counteracts the electric field which is<br />
necessary for continued avalanche generation.<br />
For a particular tube geometry and operating voltage this termination always<br />
occurs when a certain number <strong>of</strong> avalanches have been created, therefore<br />
the pulses from the tube are always <strong>of</strong> the same magnitude regardless <strong>of</strong> the<br />
energy <strong>of</strong> the initiating particle. Consequently, there is no radiation energy<br />
information in the pulses which means the Geiger–Muller tube cannot be<br />
used to generate spectral information about the incident radiation.<br />
Pressure <strong>of</strong> the fill gas is important in the generation <strong>of</strong> avalanches. Too low a<br />
pressure and the efficiency <strong>of</strong> interaction with incident radiation is reduced.<br />
Too high a pressure, and the “mean free path” for collisions between<br />
accelerated electrons and the fill gas is too small, and the electrons cannot<br />
gather enough energy between each collision to cause ionisation <strong>of</strong> the gas.<br />
The energy gained by electrons is proportional to the ratio “e/p”, where “e” is<br />
the electric field strength at that point in the gas, and “p” is the gas pressure.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube
Detection <strong>of</strong> higher energy gamma in a thick-walled tube. Secondary<br />
electrons generated in the wall can reach the fill gas to produce avalanches.<br />
Multiple avalanches omitted for clarity<br />
Interaction <strong>of</strong><br />
gamma radiation<br />
with GM tube wall<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube
Types <strong>of</strong> tube<br />
Broadly, there are two main types <strong>of</strong> Geiger tube construction.<br />
End window type<br />
For alpha particles, low energy beta particles, and low energy X-rays, the<br />
usual form is a cylindrical end-window tube. This type has a window at one<br />
end covered in a thin material through which low-penetrating radiation can<br />
easily pass. Mica is a commonly used material due to its low mass per unit<br />
area. The other end houses the electrical connection to the anode.<br />
Pancake tube<br />
Pancake G–M tube, the circular concentric anode can clearly be seen.<br />
The pancake tube is a variant <strong>of</strong> the end window tube, but which is designed<br />
for use for beta and gamma contamination monitoring. It has roughly the<br />
same sensitivity to particles as the end window type, but has a flat annular<br />
shape so the largest window area can be utilised with a minimum <strong>of</strong> gas<br />
space. Like the cylindrical end window tube, mica is a commonly used<br />
window material due to its low mass per unit area. The anode is normally<br />
multi-wired in concentric circles so it extends fully throughout the gas space.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube
Windowless type<br />
This general type is distinct from the dedicated end window type, but has two<br />
main sub-types, which use different radiation interaction mechanisms to<br />
obtain a count.<br />
Thick walled<br />
A selection <strong>of</strong> thick walled G–M tubes for gamma detection. The largest has<br />
an energy compensation ring; the others are not energy compensated<br />
Used for high energy gamma detection, this type generally has an overall wall<br />
thickness <strong>of</strong> about 1-2 mm <strong>of</strong> chrome steel. Because most high energy<br />
gamma photons will pass through the low density fill gas without interacting,<br />
the tube uses the interaction <strong>of</strong> photons on the molecules <strong>of</strong> the wall material<br />
to produce high energy secondary electrons within the wall. Some <strong>of</strong> these<br />
electrons are produced close enough to the inner wall <strong>of</strong> the tube to escape<br />
into the fill gas. As soon as this happens the electron drifts to the anode and<br />
an electron avalanche occurs as though the free electron had been created<br />
within the gas. The avalanche is a secondary effect <strong>of</strong> a process that starts<br />
within the tube wall; the avalanche is not the effect <strong>of</strong> radiation directly on the<br />
gas itself.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube
Thin walled<br />
Thin walled tubes are used for:<br />
high energy beta detection, where the beta enters via the side <strong>of</strong> the tube and<br />
interacts directly with the gas, but the radiation has to be energetic enough to<br />
penetrate the tube wall. Low energy beta, which would penetrate an end<br />
window, would be stopped by the tube wall.<br />
Low energy gamma and X-ray detection.<br />
The lower energy photons interact better with the fill gas so this design<br />
concentrates on increasing the volume <strong>of</strong> the fill gas by using a long thin<br />
walled tube and does not use the interaction <strong>of</strong> photons in the tube wall. The<br />
transition from thin walled to thick walled design takes place at the 300–400<br />
KeV energy levels. Above these levels thick walled designs are used, and<br />
beneath these levels the direct gas ionisation effect is predominant.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube
Schematic <strong>of</strong> a Geiger counter using an "end window" tube for lowpenetrating<br />
radiation. A loudspeaker is also used for indication<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube
Pancake G–M tube, the circular concentric anode can clearly be seen.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube
A selection <strong>of</strong> thick walled G–M tubes for gamma detection. The largest has<br />
an energy compensation ring; the others are not energy compensated<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube
<strong>Neutron</strong><br />
G–M tubes will not detect neutrons since these do not ionise the gas.<br />
However, neutron-sensitive tubes can be produced which either have the (1)<br />
inside <strong>of</strong> the tube coated with boron, or (2) the tube contains boron trifluoride<br />
or (3) helium-3 as the fill gas.<br />
The neutrons interact with the boron nuclei, producing alpha particles, or<br />
directly with the helium-3 nuclei producing hydrogen (proton) and tritium ions<br />
and electrons. These charged particles then trigger the normal avalanche<br />
process.<br />
10<br />
5 B + n → 7 3 Li + 4 2 α + 2e-<br />
3<br />
2 He + n → 1 1 H+ + 3 1 H + e-<br />
3<br />
2 He + n → 1 1 H + 3 1 H+ + e -<br />
Charlie Chong/ Fion Zhang<br />
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Gas mixtures<br />
The main component <strong>of</strong> the gas fill mixture is an inert gas such as helium,<br />
argon or neon, in some cases in a Penning mixture, and a "quench" gas <strong>of</strong> 5–<br />
10% <strong>of</strong> an organic vapor or a halogen gas to prevent multiple pulsing. The<br />
halogen-filled G–M tube was invented by Sidney H. Liebson in 1947 and has<br />
several advantages over the tubes with older organic mixtures. The halogen<br />
tube discharge takes advantage <strong>of</strong> a metastable state <strong>of</strong> the inert gas atom to<br />
more-readily ionize a halogen molecule than an organic vapor, enabling the<br />
tube to operate at much lower voltages, typically 400–600 volts instead <strong>of</strong><br />
900–1200 volts. It also has a longer life than tubes quenched with organic<br />
compounds, because the halogen ions can recombine while the organic<br />
vapor is gradually destroyed by the discharge process (giving the latter a life<br />
<strong>of</strong> around 10 8 events). For these reasons, the halogen-filled tube is now the<br />
most common.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube
Geiger plateau<br />
The Geiger plateau is the voltage range in which the GM tube operates in its<br />
correct mode. If a G–M tube is exposed to a steady radiation source and the<br />
applied voltage is increased from zero, it follows the plot <strong>of</strong> ion current shown<br />
in this article. In the "Geiger region" the gradient flattens; this is the Geiger<br />
plateau.<br />
Depending on the characteristics <strong>of</strong> the specific tube (manufacturer, size, gas<br />
type, etc.) the voltage range <strong>of</strong> the plateau will vary. In this region, the<br />
potential difference in the counter is strong enough to allow the creation <strong>of</strong><br />
multiple avalanches.<br />
A lower voltage is not sufficient to cause a complete discharge along the<br />
anode, and individual Townsend avalanches are the result, and the tube tries<br />
to act as a proportional counter. If the applied voltage is higher than the<br />
plateau, a continuous glow discharge is formed and the tube cannot detect<br />
radiation.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube
The plateau has a slight slope caused by increasing sensitivity to low energy<br />
radiation as the voltage increases. Normally when a particle ionizes gas<br />
atoms, complete ionization <strong>of</strong> the gas occurs. But for a low energy particle, it<br />
is possible that the kinetic energy in addition to the potential energy <strong>of</strong> the<br />
voltage are insufficient for the avalanche to occur and the ion recombines. As<br />
applied voltage rises, the threshold for the minimum radiation response falls,<br />
thus the counter's sensitivity rises; giving rise to the slope.<br />
The counting rate for a given radiation source varies slightly as the applied<br />
voltage is varied and to prevent this, a regulated voltage is used. However, it<br />
is normal to operate the tube in the middle <strong>of</strong> the plateau to allow for<br />
variations in the tube supply voltage.<br />
Keypoints:<br />
In Geiger Muller counter the ionization is by Multiple Avalanches<br />
Charlie Chong/ Fion Zhang<br />
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Quenching and dead time<br />
The ideal G–M tube should produce a single pulse on entry <strong>of</strong> a single<br />
ionising particle. It must not give any spurious pulses, and must recover<br />
quickly to the passive state.<br />
Unfortunately for these requirements, when positive argon ions reach the<br />
cathode and become neutral argon atoms again by obtaining electrons from it,<br />
the atoms can acquire their electrons in enhanced energy levels. These<br />
atoms then return to their ground state by emitting photons which can in turn<br />
produce further ionisation and hence cause spurious secondary pulse<br />
discharges. If nothing were done to counteract it, ionisation could even<br />
escalate, causing a so-called current "avalanche" which if prolonged could<br />
damage the tube. Some form <strong>of</strong> quenching <strong>of</strong> the ionisation is therefore<br />
essential.<br />
Charlie Chong/ Fion Zhang<br />
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The disadvantage <strong>of</strong> quenching is that for a short time after a discharge pulse<br />
has occurred (the so-called dead time, which is typically 50–100<br />
microseconds), the tube is rendered insensitive and is thus temporarily<br />
unable to detect the arrival <strong>of</strong> any new ionising particle. This effectively<br />
causes a loss <strong>of</strong> counts at sufficiently high count rates and limits the G–M<br />
tube to a count rate <strong>of</strong> between 10 4 to 10 5 counts per second, depending on<br />
its characteristic. A consequence <strong>of</strong> this is that ion chamber instruments were<br />
sometimes preferred for higher count rates, however the modern application<br />
<strong>of</strong> "electronic quenching" (see below) can extend this upper limit considerably.<br />
Charlie Chong/ Fion Zhang<br />
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Chemical quenching<br />
Self-quenching or internal-quenching tubes stop the discharge without<br />
external assistance, by means <strong>of</strong> the addition <strong>of</strong> a small amount <strong>of</strong> a<br />
polyatomic organic vapor such as butane or ethanol, or alternatively a<br />
halogen such as bromine or chlorine.<br />
If a poor diatomic gas quencher is introduced to the tube, the positive argon<br />
ions, during their motion toward the cathode, would have multiple collisions<br />
with the quencher gas molecules and transfer their charge and some energy<br />
to them. Thus, neutral argon atoms would be produced and the quencher gas<br />
ions in their turn would reach the cathode, gain electrons there from, and<br />
move into excited states which would decay by photon emission, producing<br />
tube discharge. However, effective quencher molecules, when excited, lose<br />
their energy not by photon emission, but by dissociation into neutral quencher<br />
molecules. No spurious pulses are thus produced.<br />
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External quenching, sometimes also called "active quenching" or "electronic<br />
quenching", uses high speed control electronics to rapidly remove and reapply<br />
the high voltage between the electrodes after each discharge peak.<br />
This results in faster quenching <strong>of</strong> the tube than using the effect <strong>of</strong> gas alone,<br />
and allows for greatly increased tube lifetimes.<br />
A technique known as "time-to-first-count" is sometimes used in conjunction<br />
with this to greatly increase the maximum count rate <strong>of</strong> the tube.<br />
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Dead time and recovery time in a Geiger Muller tube.[4] The tube can<br />
produce no further pulses during the dead time, and is able to produce only<br />
pulses <strong>of</strong> limited height until the recovery time elapses.<br />
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Fold-back<br />
One consequence <strong>of</strong> the dead time effect is the possibility <strong>of</strong> a high count rate<br />
continually triggering the tube before the recovery time has elapsed. This may<br />
produce pulses too small for the counting electronics to detect and lead to the<br />
very undesirable situation whereby a G–M counter in a very high radiation<br />
field is falsely indicating a low level. This phenomenon is known as "foldback".<br />
An industry rule <strong>of</strong> thumb is that the discriminator circuit receiving the<br />
output from the tube should detect down to 1/10 <strong>of</strong> the magnitude <strong>of</strong> a normal<br />
pulse to guard against this. Additionally the circuit should detect when "pulse<br />
pile-up " has occurred, where the apparent anode voltage has moved to a<br />
new dc level through the combination <strong>of</strong> high pulse count and noise. The<br />
electronic design <strong>of</strong> Geiger–Muller counters must be able to detect this<br />
situation and give an alarm; it is normally done by setting a threshold for<br />
excessive tube current.<br />
Charlie Chong/ Fion Zhang<br />
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Detection efficiency<br />
The efficiency <strong>of</strong> detection <strong>of</strong> a G–M tube varies with the type <strong>of</strong> incident<br />
radiation. Tubes with thin end windows have very high efficiencies (can be<br />
nearly 100%) for high energy beta, though this drops <strong>of</strong>f as the beta energy<br />
decreases due to attenuation by the window material. Alpha particles are also<br />
attenuated by the window. As alpha particles have a maximum range <strong>of</strong> less<br />
than 50 mm in air, the detection window should be as close as possible to the<br />
source <strong>of</strong> radiation. The attenuation <strong>of</strong> the window adds to the attenuation <strong>of</strong><br />
air, so the window should have a density as low as 1.5 to 2.0 mg/cm 2 to give<br />
an acceptable level <strong>of</strong> detection efficiency. The article on stopping power<br />
explains in more detail the ranges for particles types <strong>of</strong> various energies. The<br />
counting efficiency <strong>of</strong> photon radiation (gamma and X-rays above 25 keV)<br />
depends on the efficiency <strong>of</strong> radiation interaction in the tube wall, which<br />
increases with the atomic number <strong>of</strong> the wall material. Chromium iron is a<br />
commonly used material, which gives an efficiency <strong>of</strong> about 1% over a wide<br />
range <strong>of</strong> energies.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube
Energy compensation<br />
If a G–M tube is to be used for gamma or X-ray dosimetry measurements the<br />
energy <strong>of</strong> incident radiation, which affects the ionising effect, must be taken<br />
into account. However individual pulses from a G–M tube do not carry any<br />
energy information. A solution is to assign a radiation dose to each counting<br />
event, so the tube characteristic relates the number <strong>of</strong> counts to the intensity<br />
<strong>of</strong> incident radiation.<br />
At low photon energy levels the response increases as low energy photons<br />
have a greater interaction with the fill gas than high energy photons. The tube<br />
therefore has an increased response for radiation which has a lower dose<br />
rate, and a correction must be applied to prevent an incorrect high reading for<br />
low energy photons. This discrepancy can be 2–3 times greater or more, and<br />
for a thick-walled tube usually peaks at about 60 keV, where radiation<br />
interactions with the gas are still large, but the shielding effect <strong>of</strong> the wall has<br />
not become dominant.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube
This correction is achieved by 'energy compensation' <strong>of</strong> the tube, which<br />
modifies the number <strong>of</strong> count events in accordance with the energy <strong>of</strong> the<br />
incident radiation by using an external filter collar <strong>of</strong> energy absorbing<br />
material. The collar has an increased attenuation <strong>of</strong> low energy gamma, and<br />
so compensates for the increased energy response <strong>of</strong> the naked tube at<br />
those levels. The aim is that sensitivity/energy characteristic <strong>of</strong> the tube<br />
should be matched by the absorption/energy characteristic <strong>of</strong> the filter. This<br />
results in a more uniform response over the stated range <strong>of</strong> detection<br />
energies for the tube.<br />
Lead and tin are commonly used materials, and a simple filter effective above<br />
150 keV can be made using a continuous collar along the length <strong>of</strong> the tube.<br />
However, at lower energy levels this attenuation can become too great, so air<br />
gaps are left in the collar to allow low energy radiation to have a greater effect.<br />
In practice, compensation filter design is an empirical compromise to produce<br />
an acceptably uniform response, and a number <strong>of</strong> different materials and<br />
geometries are used to obtain the required correction.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube
Comparative response curves for GM tube with and without radiation energy<br />
compensation<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube
Thin-walled glass G–M tube showing a spiral wire cathode. The tape bands<br />
are for fixing compensating rings<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube
Thin-walled glass G–M tube showing a spiral wire cathode. The tape bands<br />
are for fixing compensating rings<br />
Charlie Chong/ Fion Zhang
Thin-walled glass G–M tube showing a spiral wire cathode. The tape bands<br />
are for fixing compensating rings<br />
Charlie Chong/ Fion Zhang
Thin-walled glass G–M tube with energy compensating rings fitted. The<br />
complete assembly fits into the aluminium housing.<br />
energy compensating rings- Absorb the<br />
low energy photon & enhanced high<br />
energy photon by production <strong>of</strong> secondary<br />
electron at ring internal<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Geiger%E2%80%93M%C3%BCller_tube
Thin-walled glass G–M tube with energy compensating rings fitted. The<br />
complete assembly fits into the aluminium housing.<br />
Charlie Chong/ Fion Zhang
Thin-walled glass G–M tube with energy compensating rings fitted. The<br />
complete assembly fits into the aluminium housing.<br />
Charlie Chong/ Fion Zhang
Proportional counter<br />
The proportional counter is a type <strong>of</strong> gaseous ionization detector device used<br />
to measure particles <strong>of</strong> ionizing radiation.<br />
The key feature is its ability to measure the energy <strong>of</strong> incident radiation, by<br />
producing a detector output that is proportional to the radiation energy; hence<br />
the detector's name. It is widely used where energy levels <strong>of</strong> incident<br />
radiation must be known, such as in the discrimination between alpha and<br />
beta particles, or accurate measurement <strong>of</strong> X-ray radiation dose. A<br />
proportional counter uses a combination <strong>of</strong> the mechanisms <strong>of</strong> a Geiger–<br />
Müller tube and an ionization chamber, and operates in an intermediate<br />
voltage region between these. The accompanying plot shows the proportional<br />
counter operating voltage region for a co-axial cylinder arrangement.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Proportional_counter
Plot <strong>of</strong> variation <strong>of</strong> ion pair current against applied voltage for a wire cylinder<br />
gaseous radiation detector.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Proportional_counter
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Proportional_counter
Operation<br />
In a proportional counter the fill gas <strong>of</strong> the chamber is an inert gas which is<br />
ionised by incident radiation, and a quench gas to ensure each pulse<br />
discharge terminates; a common mixture is 90% argon, 10% methane, known<br />
as P-10.<br />
What is P10:<br />
Proportional counter with 90% Argon (inert gas) with 10% quenched gas<br />
(10% methane)<br />
An ionising particle entering the gas collides with an atom <strong>of</strong> the inert gas and<br />
ionises it to produce an electron and a positively charged ion, commonly<br />
known as an "ion pair". As the charged particle travels through the chamber it<br />
leaves a trail <strong>of</strong> ion pairs along its trajectory, the number <strong>of</strong> which is<br />
proportional to the energy <strong>of</strong> the particle if it is fully stopped within the gas.<br />
Typically a 1 MeV stopped particle will create about 30,000 ion pairs.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Proportional_counter
What is P10:<br />
Proportional counter with 90% Argon (inert gas) with 10% quenched gas<br />
(10% methane)<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Proportional_counter
The chamber geometry and the applied voltage is such that in most <strong>of</strong> the<br />
chamber the electric field strength is low and the chamber acts as an ion<br />
chamber. However, the field is strong enough to prevent re-combination <strong>of</strong><br />
the ion pairs and causes positive ions to drift towards the cathode and<br />
electrons towards the anode. This is the "ion drift" region. In the immediate<br />
vicinity <strong>of</strong> the anode wire, the field strength becomes large enough to produce<br />
Townsend avalanches. This avalanche region occurs only fractions <strong>of</strong> a<br />
millimeter from the anode wire, which itself is <strong>of</strong> a very small diameter. The<br />
purpose <strong>of</strong> this is to use the multiplication effect <strong>of</strong> the avalanche produced by<br />
each ion pair. This is the "avalanche" region.<br />
A key design goal is that each original ionising event due to incident radiation<br />
produces only one avalanche. This is to ensure proportionality between the<br />
number <strong>of</strong> original events and the total ion current. For this reason the applied<br />
voltage, the geometry <strong>of</strong> the chamber and the diameter <strong>of</strong> the anode wire are<br />
critical to ensure proportional operation. If avalanches start to self-multiply<br />
due to UV photons as they do in a Geiger–Muller tube, then the counter<br />
enters a region <strong>of</strong> "limited proportionality" until at a higher applied voltage the<br />
Geiger discharge mechanism occurs with complete ionisation <strong>of</strong> the gas<br />
enveloping the anode wire and consequent loss <strong>of</strong> particle energy information.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Proportional_counter
Plot <strong>of</strong> variation <strong>of</strong> ion pair current against applied voltage for a wire cylinder<br />
gaseous radiation detector.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Proportional_counter
Therefore, it can be said that the proportional counter has the key design<br />
feature <strong>of</strong> two distinct ionisation regions:<br />
1. Ion drift region: in the outer volume <strong>of</strong> the chamber – creation <strong>of</strong> number<br />
ion pairs proportional to incident radiation energy.<br />
2. Avalanche region: in the immediate vicinity <strong>of</strong> the anode – Charge<br />
amplification <strong>of</strong> ion pair currents, while maintaining localised avalanches.<br />
The process <strong>of</strong> charge amplification greatly improves the signal-to-noise ratio<br />
<strong>of</strong> the detector and reduces the subsequent electronic amplification required.<br />
In summary, the proportional counter is an ingenious combination <strong>of</strong> two<br />
ionisation mechanisms in one chamber which finds wide practical use.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Proportional_counter
The generation <strong>of</strong> discrete Townsend avalanches in a proportional counter.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Proportional_counter
Plot <strong>of</strong> electric field strength at the anode, showing boundary <strong>of</strong> avalanche<br />
region.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Proportional_counter
The gas flow proportional counter for alpha counting was invented in 1943 by John Simpson at the<br />
University <strong>of</strong> Chicago Metallurgical Laboratory. Its purpose was to measure plutonium (an alpha emitter) in the presence <strong>of</strong> beta-emitting fission products.<br />
The key feature <strong>of</strong> this instrument that allowed it to reject beta pulses was its use <strong>of</strong> methane as the counting gas. Simpson would later invent P-10 gas<br />
(10% methane, 90% argon), the most widely employed gas in proportional counters. The instrument also featured a short time constant which reduced pulse<br />
pile up and assisted in rejecting the beta pulses.<br />
Charlie Chong/ Fion Zhang<br />
https://www.orau.org/PTP/collection/proportional%20counters/Proportionalcounters.htm
RCL Mark 2, Model 201 Fast <strong>Neutron</strong> Proportional Counter (1950s)<br />
This is a fast neutron detector produced by Radiation Counter Laboratories (RCL) <strong>of</strong> Skokie, Illinois.<br />
The tube is approximately 8 1/4 inches long and 1 7/8 inches in diameter. A brass evacuation tube can be<br />
seen projecting to the right from the brass chamber. The actual proportional counter chamber is 1.2 inches long,<br />
lined with 1/16 inch <strong>of</strong> polyethylene, and filled with methane at a pressure <strong>of</strong> 150 cm. It operated at 2100 volts.<br />
Fast neutrons knock protons <strong>of</strong>f the polyethylene lining. The protons then ionize the methane fill gas to produce<br />
the signal. The RCL detector designation is the Mark 2, Model 201, Serial 127. The "1" at the end <strong>of</strong> the model<br />
number (201) refers to the number <strong>of</strong> chambers housed in the unit. The Models 202 and 203 used two and<br />
three chambers respectively.<br />
Charlie Chong/ Fion Zhang<br />
https://www.orau.org/PTP/collection/proportional%20counters/bf3rclmk2mod201l.htm
Proportional Counter<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Proportional_counter
Proportional Counter<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Proportional_counter
Applications<br />
Spectroscopy<br />
The proportionality between the energy <strong>of</strong> the charged particle travelling<br />
through the chamber and the total charge created makes proportional<br />
counters useful for charged particle spectroscopy. By measuring the total<br />
charge (time integral <strong>of</strong> the electric current) between the electrodes, we can<br />
determine the particle's kinetic energy because the number <strong>of</strong> ion pairs<br />
created by the incident ionizing charged particle is proportional to its energy.<br />
The energy resolution <strong>of</strong> a proportional counter, however, is limited because<br />
both the initial ionization event and the subsequent 'multiplication' event are<br />
subject to statistical fluctuations characterised by a standard deviation equal<br />
to the square root <strong>of</strong> the average number formed. However, in practice these<br />
are not as great as would be predicted due to the effect <strong>of</strong> the empirical Fano<br />
factor which reduces these fluctuations. In the case <strong>of</strong> argon, this is<br />
experimentally about 0.2.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Proportional_counter
Photon detection<br />
Proportional counters are also useful for detection <strong>of</strong> high energy photons,<br />
such as gamma-rays, provided these can penetrate the entrance window.<br />
They are also used for the detection <strong>of</strong> X-rays to below 1 Kev energy levels,<br />
using thin walled tubes operating at or around atmospheric pressure.<br />
Radioactive contamination detection<br />
Proportional counters in the form <strong>of</strong> large area planar detectors are used<br />
extensively to check for radioactive contamination on personnel, flat surfaces,<br />
tools and items <strong>of</strong> clothing. This is normally in the form <strong>of</strong> installed<br />
instrumentation because <strong>of</strong> the difficulties <strong>of</strong> providing portable gas supplies<br />
for hand-held devices. They are constructed with a large area detection<br />
window made from such as metallised mylar which forms one wall <strong>of</strong> the<br />
detection chamber and is part <strong>of</strong> the cathode. The anode wire is routed in a<br />
convoluted manner within the detector chamber to optimise the detection<br />
efficiency.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Proportional_counter
They are normally used to detect alpha and beta particles, and can enable<br />
discrimination between them by providing a pulse output proportional to the<br />
energy deposited in the chamber by each particle. They have a high<br />
efficiency for beta, but lower for alpha. The efficiency reduction for alpha is<br />
due to the attenuation effect <strong>of</strong> the entry window, though distance from the<br />
surface being checked also has a significant effect, and ideally a source <strong>of</strong><br />
alpha radiation should be less than 10mm from the detector due to<br />
attenuation in air.<br />
These chambers operate at very slight positive pressure above ambient<br />
atmospheric pressure. The gas can be sealed in the chamber, or can be<br />
changed continuously, in which case they are known as "gas-flow<br />
proportional counters". Gas flow types have the advantage that they will<br />
tolerate small holes in the mylar screen which can occur in use, but they do<br />
require a continuous gas supply.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Proportional_counter
Guidance on application use<br />
In the United Kingdom the HSE has issued a user guidance note on selecting<br />
the correct radiation measurement instrument for the application concerned.<br />
This covers all radiation instrument technologies, and is a useful comparative<br />
guide to the use <strong>of</strong> proportional counters.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Proportional_counter
■ ωσμ∙Ωπ∆ ∇ º≠δ≤>ηθφФρ|β≠Ɛ∠ ʋ λαρτ√ ≠≥ѵФε ≠≥ѵФdsssa<br />
Charlie Chong/ Fion Zhang
Biological Half-life<br />
Charlie Chong/ Fion Zhang<br />
http://hyperphysics.phy-astr.gsu.edu/hbase/Nuclear/biohalf.html
Biological Half-life<br />
The radioactive half-life for a given radioisotope is physically determined and<br />
unaffected by the physical or chemical conditions around it. However, if that<br />
radioisotope is in a living organism it may be excreted so that it no longer is a<br />
source <strong>of</strong> radiation exposure to the organism. For a number <strong>of</strong> radioisotopes<br />
<strong>of</strong> particular medical interest, the rate <strong>of</strong> excretion has been cast in the form<br />
<strong>of</strong> an effective biological half-life. The rate <strong>of</strong> decrease <strong>of</strong> radiation exposure<br />
is then affected by both the physical and biological half-life, giving an effective<br />
half-life for the isotope in the body. Though the biological half-life cannot be<br />
expected to be as precise as the physical half-life, it is useful compute an<br />
effective half-life from:<br />
1/T Effective = 1/T Physical + 1/T Biological<br />
Charlie Chong/ Fion Zhang<br />
http://hyperphysics.phy-astr.gsu.edu/hbase/Nuclear/biohalf.html
<strong>Exam</strong>ples <strong>of</strong> the half-lives show that biological clearing is sometimes<br />
dominant and sometimes physical decay is the dominant influence.<br />
Half Life in day<br />
Isotopes<br />
T Physical<br />
T Biological<br />
T Effective<br />
3 H<br />
4.5 x 10 3<br />
12<br />
12<br />
22<br />
P<br />
14.3<br />
1155<br />
14.1<br />
90 Sr<br />
1.1 x 10 4<br />
1.8 x 10 4<br />
6.8 x 10 3<br />
99m<br />
Tc<br />
0.25<br />
1<br />
0.20<br />
Charlie Chong/ Fion Zhang<br />
http://hyperphysics.phy-astr.gsu.edu/hbase/Nuclear/biohalf.html
Tritium, 3 H, has a fairly long physical half life but clears from the body quickly,<br />
lessening the exposure. Phosphorous, 32 P, is used for some kinds <strong>of</strong> bone<br />
scans. The phosphorous tends to be held in the bones, leading to a long<br />
biological half-life, but its physical half-life is short enough to minimize<br />
exposure. Strontium, 90 Sr, is very bad news in the environment. It mimics<br />
calcium and therefore gets trapped in bone. This gives it a long biological<br />
half-life to go with its long physical half-life, making it doubly dangerous.<br />
Technetium, 99m Tc, is one <strong>of</strong> the favorites for diagnostic scans because <strong>of</strong><br />
short physical and biological half-lives. It clears from the body very quickly<br />
after the imaging procedures.<br />
Charlie Chong/ Fion Zhang<br />
http://hyperphysics.phy-astr.gsu.edu/hbase/Nuclear/biohalf.html
The biological half-life or terminal half-life <strong>of</strong> a substance is the time it takes<br />
for a substance (for example a metabolite, drug, signalling molecule,<br />
radioactive nuclide, or other substance) to lose half <strong>of</strong> its pharmacologic,<br />
physiologic, or radiologic activity, according to the Medical Subject Headings<br />
(MeSH) definition. Typically, this refers to the body's cleansing through the<br />
function <strong>of</strong> kidneys and liver in addition to excretion functions to eliminate a<br />
substance from the body. In a medical context, half-life may also describe the<br />
time it takes for the blood plasma concentration <strong>of</strong> a substance to halve<br />
(plasma half-life) its steady-state. The relationship between the biological and<br />
plasma half-lives <strong>of</strong> a substance can be complex depending on the substance<br />
in question, due to factors including accumulation in tissues (protein binding),<br />
active metabolites, and receptor interactions.<br />
Biological half-life is an important pharmacokinetic parameter and is usually<br />
denoted by the abbreviation t ½<br />
While a radioactive isotope decays perfectly according to first order kinetics<br />
where the rate constant is fixed, the elimination <strong>of</strong> a substance from a living<br />
organism follows more complex chemical kinetics.<br />
Charlie Chong/ Fion Zhang<br />
https://en.wikipedia.org/wiki/Biological_half-life
Charlie Chong/ Fion Zhang
More <strong>Reading</strong><br />
http://www.euronuclear.org/info/encyclopedia.htm<br />
Charlie Chong/ Fion Zhang
■ ωσμ∙Ωπ∆ ∇ º≠δ≤>ηθφФρ|β≠Ɛ∠ ʋ λαρτ√ ≠≥ѵФε ≠≥ѵФdsssa<br />
Charlie Chong/ Fion Zhang
Charlie Chong/ Fion Zhang
Charlie Chong/ Fion Zhang
Charlie Chong/ Fion Zhang
Good Luck!<br />
Charlie Chong/ Fion Zhang