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Long term total ozone trend analysis

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Institut für Umweltphysik<br />

Fachbereich 1<br />

Physik<br />

<strong>Long</strong> <strong>term</strong> <strong>total</strong> <strong>ozone</strong> <strong>trend</strong> <strong>analysis</strong> of the years<br />

1979-2011 from merged data sets of various<br />

satellites.<br />

Wissam Chehade, Mark Weber, John P. Burrows<br />

June 19, 2012<br />

ATMOS 2012, Bruges Belgium


Institut für Umweltphysik<br />

� Motivation.<br />

� Ozone datasets.<br />

Contents<br />

� Multiple linear regression.<br />

The main contributions to the <strong>ozone</strong> variability.<br />

� Results.<br />

� Summary and Conclusions.<br />

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Total <strong>ozone</strong> data sets:<br />

� WOUDC („ground“)<br />

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� SBUV/TOMS/OMI Mod V8 („US satellites“)<br />

� GSG data set („European satellites“)<br />

Montreal protocol:<br />

Ozone has leveled off after 2000 after a<br />

long <strong>term</strong> decline until the 1990s.<br />

large variability from year-to-year can still<br />

lead to substantial <strong>ozone</strong> losses at high<br />

latitudes in individual years in coming decades<br />

Weber et al., 2011b<br />

Motivation


Institut für Umweltphysik<br />

The „US“ <strong>total</strong> <strong>ozone</strong> record<br />

Ozone datasets<br />

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Physik<br />

0<br />

TOMS, SBUV(/2) and OMI MOD V8 merged data set.<br />

http://acd-ext.gsfc.nasa.gov/Data_services/merged/instruments.html


The „European“ <strong>total</strong> <strong>ozone</strong> record (GSG)<br />

0<br />

Institut für Umweltphysik<br />

� GOME/ERS2: 1995-2011 (lost global coverage after 2003)<br />

o global coverage: ~3 days, large ground pixel: 320 x 40 km 2<br />

� SCIAMACHY/ENVISAT: 2002-2012<br />

o limb and nadir alternating, global coverage ~6 days<br />

� GOME-2/METOP-A: 2007-present<br />

o wide swath, daily coverage ~1 day, small ground pixel: 80 x 40 km 2<br />

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ERS2, ENVISAT, and METOP-A platforms<br />

WFDOAS <strong>ozone</strong> and overpass data: www.iup.uni-bremen.de/gome/wfdoas<br />

� GOME very stable over 16 year.<br />

� SCIAMACHY data corrected for <strong>trend</strong> (4%/decade), and bais of 1%.<br />

� GOME-2 corrected for bais of 1%.<br />

Ozone datasets


The main contributions to the <strong>ozone</strong> variability<br />

0<br />

Institut für Umweltphysik<br />

Fachbereich 1<br />

Physik<br />

Ozone depleting substances (ODS).<br />

o The various halogen compounds have different potentials to deplete stratospheric <strong>ozone</strong>.<br />

o EESC Equivalent Effective Stratospheric Chlorine<br />

http://acdb‐ext.gsfc.nasa.gov/Data_services/automailer/index.html<br />

� Solar cycle.<br />

o Decadal scale variation of <strong>total</strong> <strong>ozone</strong> correlates with the solar cycle.<br />

[Jackman et al., 1996; Miller et al.,1996]<br />

o The solar activity-<strong>ozone</strong> relationship considered in all international <strong>ozone</strong> <strong>trend</strong><br />

assessments (WMO,1999, 2003).<br />

o solar radio flux at 10.7 cm wavelength.<br />

ftp://ftp.ngdc.noaa.gov/STP/SOLAR_DATA/SOLAR_RADIO/FLUX/Penticton_Observed/monthly/<br />

� Major volcanic eruptions (aerosols).<br />

o Volcanic eruptions El Chichon in 1982 and Mt. Pinatubo in 1991, very low <strong>ozone</strong> in NH<br />

[Randel et al., 1995; Solomon et al., 1996].<br />

o Atmospheric dynamics and radiative forcing Effect [Solomon et al. 1996]<br />

o stratospheric aerosol optical depth at 550 nm.<br />

http://data.giss.nasa.gov/modelforce/strataer/


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� Quasi-Biennial Oscillation (QBO).<br />

0<br />

The main contributions to the <strong>ozone</strong> variability<br />

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QBO<br />

Quasi Biennial Oscillation QBO (zonal winds at 30 and 10 hPa)<br />

http://www.geo.fu‐berlin.de/en/met/ag/strat/produkte/qbo/index.html


0<br />

Institut für Umweltphysik<br />

� Eddy Heat Flux (ehf).<br />

The main contributions to the <strong>ozone</strong> variability<br />

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Physik<br />

transport<br />

polar<br />

<strong>ozone</strong> loss<br />

Weber et al., 2011b


Multiple linear regression<br />

0<br />

Institut für Umweltphysik<br />

Fachbereich 1<br />

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Separate the influence of various dynamical and chemical processes.<br />

Multiple linear regression is a standard tool to quantitatively attribute observed<br />

<strong>total</strong> <strong>ozone</strong> variations to different natural and anthropogenic influences.<br />

[Steinbrecht et al.,2001, 2003; WMO, 2007]<br />

TOZ(n) = TOZ° + α EESC .EESC(n)<br />

+ α qbo10 .qbo10(n) + α qbo30 .qbo30(n)<br />

+ α solar .solar(n)<br />

+ α aerosols .aerosols(n)<br />

+ α ehf .ehf(n)<br />

+ ε(n)<br />

dynamics<br />

chemistry


0<br />

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8.21<br />

DU/decade<br />

QBO 4-5 DU, Solar Cycle ± 5 DU, Eddy Heat Flux ± 10 DU<br />

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Physik<br />

3.71<br />

DU/decade


0<br />

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3.43<br />

DU/decade<br />

QBO 4-7 DU.<br />

Solar Cycle ± 3 DU.<br />

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Physik<br />

1.96<br />

DU/decade


0<br />

Institut für Umweltphysik<br />

The influence of the QBO about 5 DU.<br />

The influence of the Solar Cycle up to 3 DU.<br />

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Physik


0<br />

Institut für Umweltphysik<br />

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� The correlations between observed<br />

annual means and regression results are<br />

high.<br />

�EESC and Eddy heat flux <strong>term</strong>s<br />

contributions increase with latitude.<br />

� Eddy heat flux is dominant at high<br />

latitudes<br />

�QBO contribution from the tropics to<br />

subtropics


0<br />

A senstivity study on the use of the „GSG“ data in the linear regression is performed.<br />

Institut für Umweltphysik<br />

3.21<br />

DU/decade<br />

3.25<br />

DU/decade<br />

Fachbereich 1<br />

Physik<br />

3.43<br />

DU/decade


0<br />

Institut für Umweltphysik<br />

Fachbereich 1<br />

Physik


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Summary and Conclusions.<br />

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�Multiple linear regression <strong>analysis</strong> provides a good near global picture of natural and<br />

anthropogenic contributions to inter-annual variations of <strong>total</strong> <strong>ozone</strong>.<br />

�For the different explanatory variables, <strong>ozone</strong> fluctuations range about 3-10 DU.<br />

�The recent increases (2010) in both hemispheres <strong>total</strong> <strong>ozone</strong> are mainly related to<br />

increases in eddy heat flux (or reduced polar <strong>ozone</strong> loss after a series of cold Arctic<br />

winters in the mid-nineties ).<br />

�For the 2011 decrease, we had the opposite, QBO west phase, little wave activity<br />

and strong chemical <strong>ozone</strong> loss.<br />

� SBUV/TOMS/OMI/GSG shows about the same significance in the overall fitting as<br />

SBUV/TOMS/OMI.<br />

�The fingerprint of recovery is less clear due to the large influence from<br />

atmospheric dynamics.


Institut für Umweltphysik<br />

THANK YOU<br />

Fachbereich 1<br />

Physik

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