Photorefractive Solitons (Chapter in Springer book ... - Tripod
Photorefractive Solitons (Chapter in Springer book ... - Tripod
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<strong>Photorefractive</strong> <strong>Solitons</strong><br />
E. DelRe 1 , M. Segev 2 , D. Christodoulides 3 , B. Crosignani 1 , and G. Salamo 5<br />
1<br />
Dipartimento di Fisica, Università dell’Aquila, 67010 L’Aquila, Italy and<br />
Istituto Nazionale Fisica della Materia - UdR Roma ”La Sapienza”, 00185<br />
Roma, Italy eugenio.delre@aquila.<strong>in</strong>fn.it<br />
2<br />
Physics Department, Technion, Haifa, Israel msegev@tx.technion.ac.il<br />
3<br />
School of Optics-CREOL, University of Central Florida, Orlando, 32816-2700<br />
United States demetri@creol.ucf.edu<br />
4<br />
Physics Department, University of Arkansas, Fayetteville, 72703-0000 United<br />
States salamo@uark.edu<br />
1 Introduction<br />
<strong>Solitons</strong> are a universal phenomenon that appears <strong>in</strong> a wealth of systems <strong>in</strong><br />
nature. The past few decades have witnessed their identification and observation<br />
<strong>in</strong> the more diverse physical systems: <strong>in</strong> shallow and deep water waves,<br />
charge density waves <strong>in</strong> plasma, sound waves <strong>in</strong> liquid helium, matter waves<br />
<strong>in</strong> Bose-E<strong>in</strong>ste<strong>in</strong> condensates, excitations on DNA cha<strong>in</strong>s, ”branes” at the<br />
end of open str<strong>in</strong>gs <strong>in</strong> superstr<strong>in</strong>g theory, doma<strong>in</strong> walls <strong>in</strong> supergravity, and<br />
many more. <strong>Solitons</strong> can even appear for electromagnetic waves <strong>in</strong> vacuum,<br />
where they are supported by QED nonl<strong>in</strong>earities. And, of course, <strong>in</strong> Optics:<br />
here solitons truly manifest themselves <strong>in</strong> a large variety of sett<strong>in</strong>gs (for a review<br />
on optical solitons see Refs.[1, 2, 3, 4]). In all these diverse systems, that<br />
vary <strong>in</strong> almost everyth<strong>in</strong>g from size to dimensionality, from underly<strong>in</strong>g forces<br />
to physical mechanisms, propagation leads to a family of nonl<strong>in</strong>ear waves -<br />
solitons - that have the same, universal, features: they are all self-trapped<br />
entities possess<strong>in</strong>g particle-like behavior.<br />
In this <strong>Chapter</strong> we outl<strong>in</strong>e the mechanisms through which photorefraction<br />
can support optical spatial solitons (for a specific review, see pages 61-125<br />
<strong>in</strong> [4]), give an account of the development of the ma<strong>in</strong> underly<strong>in</strong>g ideas,<br />
and describe the associated phenomenology. S<strong>in</strong>ce the discovery of photorefractive<br />
solitons <strong>in</strong> 1992 [5], they have become one of the most important<br />
experimental means to study universal soliton features. The rich diversity of<br />
photorefractive effects has allowed experimental <strong>in</strong>vestigations <strong>in</strong>to a large<br />
variety of soliton phenomena, many of which have here found their very<br />
first observation, <strong>in</strong> any soliton-support<strong>in</strong>g system <strong>in</strong> nature. For example, it<br />
was with photorefractive solitons that fasc<strong>in</strong>at<strong>in</strong>g soliton <strong>in</strong>teraction effects,<br />
such as 3D soliton spiral<strong>in</strong>g, fission and annihilation, were first demonstrated.<br />
Likewise, random-phase (or <strong>in</strong>coherent) solitons were first observed <strong>in</strong> photorefractives,<br />
and so multi-mode solitons, both <strong>in</strong> 1D and <strong>in</strong> 2D. And, very<br />
recently, solitons <strong>in</strong> two-dimensional nonl<strong>in</strong>ear photonic lattices were demonstrated,<br />
once aga<strong>in</strong>, <strong>in</strong> photorefractives, us<strong>in</strong>g a real-time optically-<strong>in</strong>duced<br />
photonic lattice. Today, almost 12 years after their discovery, photorefrac-
2 E. DelRe, M. Segev, D. Christodoulides, B. Crosignani, and G. Salamo<br />
tive solitons have evolved <strong>in</strong>to a major subject contribut<strong>in</strong>g to research at<br />
the cutt<strong>in</strong>g edge of nonl<strong>in</strong>ear science. The <strong>in</strong>tr<strong>in</strong>sic complexity of the photorefractive<br />
light-<strong>in</strong>duced <strong>in</strong>dex-change, driven by several charge transport<br />
mechanisms, utiliz<strong>in</strong>g l<strong>in</strong>ear and quadratic electro-optic effects, and hav<strong>in</strong>g<br />
a polarization-dependent tensorial behavior, contributes <strong>in</strong> giv<strong>in</strong>g rise to a<br />
rich phenomenology. Much is understood now about the formation processes<br />
of the various types of photorefractive solitons, and many of the parameters<br />
can be controlled <strong>in</strong>dividually: at the same time numerous questions<br />
are still open. Also important, research on solitons <strong>in</strong> photorefractives has<br />
benefited not only the soliton community, but has also <strong>in</strong>troduced a number<br />
of new <strong>in</strong>gredients to photorefractive studies at large. For example, understand<strong>in</strong>g<br />
the propagation dynamics of beams <strong>in</strong> photorefractives (rather than<br />
two- and four-wave-mix<strong>in</strong>g), <strong>in</strong>clud<strong>in</strong>g the formation of self-oscillators (e.g.,<br />
the so-called ”double phase conjugator”) has considerably benefited from the<br />
understand<strong>in</strong>g ga<strong>in</strong>ed <strong>in</strong> photorefrative soliton research. Likewise, explor<strong>in</strong>g<br />
spatially-localized effects that emerge and f<strong>in</strong>d their full realization directly<br />
with<strong>in</strong> the sample, such as <strong>in</strong>stabilities and spontaneous pattern formation,<br />
with and without a cavity, is now nicely understood through the <strong>in</strong>timate<br />
connection between solitons and modulation <strong>in</strong>stability [4]. These dist<strong>in</strong>guish<br />
soliton phenomenology from holographic and wave-mix<strong>in</strong>g schemes, which, by<br />
nature, deal pr<strong>in</strong>cipally with the manipulation of light as a device to an effect<br />
which occurs outside the crystal. In this <strong>Chapter</strong>, we attempt to provide an<br />
updated overview on the fasc<strong>in</strong>at<strong>in</strong>g phenomenon of photorefractive solitons,<br />
which cont<strong>in</strong>uously br<strong>in</strong>gs <strong>in</strong> new surprises, new effects, new excitement, to<br />
the photorefractives community, to the much broader nonl<strong>in</strong>ear optics community,<br />
and to soliton science at large.<br />
2 The discovery of solitons <strong>in</strong> photorefractives<br />
In the wake of renewed <strong>in</strong>terest <strong>in</strong> soliton propagation, triggered by studies<br />
on temporal solitons <strong>in</strong> an ever more competitive fiber optic network, the beg<strong>in</strong>n<strong>in</strong>g<br />
of the 1990s see an <strong>in</strong>tense effort aimed at f<strong>in</strong>d<strong>in</strong>g accessible physical<br />
systems <strong>in</strong> which to experimentally <strong>in</strong>vestigate spatial solitons. Conventional<br />
Kerr-type nonl<strong>in</strong>ear schemes presented crippl<strong>in</strong>g limitations connected to the<br />
extremely high optical <strong>in</strong>tensities <strong>in</strong>volved, and suffer<strong>in</strong>g from the fundamental<br />
constra<strong>in</strong>ts associated with the <strong>in</strong>stabilities and catastrophic collapse of<br />
Kerr solitons <strong>in</strong> bulk media. Motivated by the strong nonl<strong>in</strong>ear response of<br />
photorefractive crystals, even at low optical <strong>in</strong>tensities, M. Segev, B. Crosignani,<br />
and A. Yariv, were able to formulate <strong>in</strong> 1992 the first photorefractionbased<br />
self-trapp<strong>in</strong>g mechanism. This embryonic idea sets the beg<strong>in</strong>n<strong>in</strong>g of the<br />
field, and, <strong>in</strong>deed, of our description [5].<br />
A spatial soliton is a beam which, by virtue of a robust balance between<br />
diffraction and nonl<strong>in</strong>earity, does not change its shape dur<strong>in</strong>g propagation. A<br />
direct observation of a spatial soliton <strong>in</strong> photorefractives is shown <strong>in</strong> Fig.(1).
<strong>Photorefractive</strong> <strong>Solitons</strong> 3<br />
Fig. 1. Top view of spurious scattered light produced by transient centrosymmetric<br />
solitons <strong>in</strong> a biased sample of potassium-lithium-tantalate-niobate (KLTN). (a)<br />
L<strong>in</strong>ear diffraction from an <strong>in</strong>put Full-Width-Half-Maximum (FWHM) of 6 µm to<br />
150 µm. (b-c) <strong>Solitons</strong> formed with opposite values of external field. Taken from<br />
[11]<br />
Before the discovery of photorefractive solitons, nonl<strong>in</strong>ear optics <strong>in</strong> photorefractives<br />
was centered on diffusion-driven wave-mix<strong>in</strong>g schemes, typically result<strong>in</strong>g<br />
<strong>in</strong> high energy exchange between the <strong>in</strong>teract<strong>in</strong>g waves, a mechanism<br />
at the heart of photorefractive self-oscillation and ”passive” phase conjugators.<br />
Dur<strong>in</strong>g that phase, other sett<strong>in</strong>gs, which exhibited elevated phasecoupl<strong>in</strong>g<br />
(and much lower energy-exchange) attracted only remote <strong>in</strong>terest.<br />
Furthermore, dur<strong>in</strong>g diffusion-driven photorefractive wave-mix<strong>in</strong>g, beam energy<br />
is spontaneously driven <strong>in</strong>to modes not present <strong>in</strong> the launch, lead<strong>in</strong>g to<br />
the highly deteriorat<strong>in</strong>g phenomenon called beam fann<strong>in</strong>g: the exact opposite<br />
of a precursor to the orderly events which accompany a solitary wave. Evidently,<br />
at the time there was no <strong>in</strong>dication of any k<strong>in</strong>d that photorefractives<br />
could support solitons. Segev et al., however, argued that s<strong>in</strong>ce wave-mix<strong>in</strong>g<br />
was <strong>in</strong>tr<strong>in</strong>sically accompanied by a mutual phase-modulation, one could f<strong>in</strong>d<br />
a condition <strong>in</strong> which the plane-wave components of a diffract<strong>in</strong>g beam could<br />
mix so as to lead to a trapp<strong>in</strong>g self-phase modulation: their mutual exchange<br />
could compensate for the l<strong>in</strong>ear dephas<strong>in</strong>g between the plane-wave components<br />
of a beam, and thus counteract diffraction altogether. They observed<br />
that, <strong>in</strong> contrast to schemes where the ma<strong>in</strong> mix<strong>in</strong>g agent is diffusion, lead<strong>in</strong>g<br />
to the highly asymmetric fann<strong>in</strong>g process, a symmetric mutual phasemodulation<br />
could be achieved through the application of an external bias<br />
field. They concluded that, when the diffusion space-charge field could be neglected<br />
with respect the external bias field, a symmetric self-focus<strong>in</strong>g occurs<br />
and self-trapp<strong>in</strong>g effects should emerge. Under such conditions, fann<strong>in</strong>g itself,<br />
be<strong>in</strong>g mediated by diffusion, would have a secondary effect [6].<br />
In order to achieve a set-up symmetric with respect to the propagat<strong>in</strong>g<br />
axis, the beam should be launched <strong>in</strong> a zero-cut uniaxial sample along the<br />
ord<strong>in</strong>ary axis a, with the external bias<strong>in</strong>g field E0 applied along the pol<strong>in</strong>g<br />
optical axis c, through two electrodes brought to a relative potential V .
4 E. DelRe, M. Segev, D. Christodoulides, B. Crosignani, and G. Salamo<br />
An optimal arrangement was identified <strong>in</strong> Stontium-Barium-Niobate (SBN)<br />
doped with rhodium impurities. Characterized by an r33 220pm/V ,for<br />
an extraord<strong>in</strong>ary c polarized beam launch, <strong>in</strong>dex modulations of the order<br />
of |∆n| (1/2)n 3 r33E0 ∼ 2 − 5 · 10 −4 for achievable fields of the order of<br />
E0 ∼ 1-3kV/cm could be reached, a nonl<strong>in</strong>earity sufficient to support the<br />
formation of a 10 µm wide soliton.<br />
Fig. 2. The orig<strong>in</strong>al soliton observation schematic, as reported <strong>in</strong> [7]. The extraord<strong>in</strong>ary<br />
launch beam is focused <strong>in</strong> proximity of the <strong>in</strong>put facet. Transient dynamics<br />
were detected record<strong>in</strong>g the output <strong>in</strong>tensity transmitted through an appropriate<br />
aperture positioned before the output detector.<br />
The first pioneer<strong>in</strong>g experiments, reported <strong>in</strong> [7] were carried out with<br />
the set-up <strong>in</strong>dicated <strong>in</strong> Fig.(2). In relat<strong>in</strong>g the first results, we more often<br />
delve upon details of transient - as opposed to steady-state - effects, and<br />
miss the ma<strong>in</strong> and revolutionary po<strong>in</strong>t: where no previous phenomenology<br />
even h<strong>in</strong>ted at self-focus<strong>in</strong>g, these first experiments <strong>in</strong>dicated, unmistakably,<br />
that a visible cont<strong>in</strong>uous-wave beam propagat<strong>in</strong>g <strong>in</strong> a biased sample would<br />
actually self-trap, the ensu<strong>in</strong>g spatial soliton be<strong>in</strong>g readily accessible to direct<br />
observation (see Fig.(1)). Although the <strong>in</strong>itial conjecture would later<br />
not prove to be greatly adherent with first f<strong>in</strong>d<strong>in</strong>gs, it did express the ma<strong>in</strong><br />
physical idea support<strong>in</strong>g the phenomena. These pioneer<strong>in</strong>g results established<br />
that very narrow beams launched <strong>in</strong> a properly-biased photorefractive crystal<br />
would self-trap, and propagate <strong>in</strong> a robust fashion, undistorted by fann<strong>in</strong>g<br />
and other noise sources <strong>in</strong> the crystal or even fairly large deviations from<br />
optimal launch conditions [8]. For example, it was established that a 15 µm<br />
sized cont<strong>in</strong>uous-wave 457nm µW beam would not suffer fann<strong>in</strong>g and selftrap<br />
for external fields from 400-500 V/cm. This observation led to a rapid<br />
series of predictions and experiments, which now form the phenomenological<br />
basis of photorefractive spatial solitons [8, 9, 10].<br />
As commonly occurs when scientific progress is <strong>in</strong> action, those first experiments<br />
posed more questions than answers. First, the results <strong>in</strong>dicated a transient<br />
self-trapp<strong>in</strong>g process (see <strong>in</strong>sert <strong>in</strong> Fig.(2)), dur<strong>in</strong>g a time w<strong>in</strong>dow of<br />
several hundreds of milliseconds, not characterized by str<strong>in</strong>gent existence con-
<strong>Photorefractive</strong> <strong>Solitons</strong> 5<br />
ditions, as would have been expected for normal self-trapp<strong>in</strong>g, where diffraction<br />
is exactly balanced by a specific value of nonl<strong>in</strong>earity. On the contrary,<br />
beam <strong>in</strong>tensity and applied bias field, two parameters assuredly implicated<br />
<strong>in</strong> the nonl<strong>in</strong>ear response, could be considerably varied without significant<br />
changes <strong>in</strong> self-trapp<strong>in</strong>g. But even more astonish<strong>in</strong>gly, the tentative launch<br />
of two-dimensional (circular) beam led to its stable self-trapp<strong>in</strong>g. This at<br />
once <strong>in</strong>dicated that the underly<strong>in</strong>g nonl<strong>in</strong>ear mechanism was not Kerr-like,<br />
s<strong>in</strong>ce the catastrophic collapse associated with self-focus<strong>in</strong>g <strong>in</strong> Kerr media<br />
did not occur. For some reason, the <strong>in</strong>tr<strong>in</strong>sic anisotropy of the light-<strong>in</strong>duced<br />
space-charge-field, result<strong>in</strong>g both from the application of an external bias<br />
along one transverse direction only, and the directionally resolved electrooptic<br />
response, allowed for a two-dimensional soliton [7, 8, 9]. Interest<strong>in</strong>gly,<br />
both aspects, the transient/non-parametric and quasi-circularly-symmetric<br />
nature of these first manifestations, which are reproducible <strong>in</strong> all photorefractive<br />
materials that can support solitons, are still not fully understood<br />
even today (see sections 4 and 5). The observation of a two-dimensional soliton<br />
<strong>in</strong> a bulk medium has attracted <strong>in</strong>terest and sometimes fomented outright<br />
debate. At the same time, the transient nature was generally looked upon as<br />
an undesired and limit<strong>in</strong>g effect. It cast a shadow both as to the nature of<br />
the <strong>in</strong>teraction, but more importantly, as to its stability. Transient effects of<br />
the sort had a history <strong>in</strong> photorefraction, and they were attributed to charge<br />
accumulation <strong>in</strong> dark regions of the sample of the photo-excited charge, deplet<strong>in</strong>g<br />
illum<strong>in</strong>ated portions and possibly screen<strong>in</strong>g external bias.<br />
This triggered the idea that the transient nature of the self-trapp<strong>in</strong>g was<br />
an effect of charge accumulation screen<strong>in</strong>g E0: free-charges would be photoexcited<br />
across the beam profile, and, drift<strong>in</strong>g <strong>in</strong> the external field, would reach<br />
the border<strong>in</strong>g dark regions, and get trapped there. These trapped charges<br />
would give rise to an <strong>in</strong>ternal (space-charge) field with a polarization opposite<br />
to E0. In SBN, this lower<strong>in</strong>g (screen<strong>in</strong>g) of the applied field at the illum<strong>in</strong>ated<br />
regions would locally lead to electro-optic lens<strong>in</strong>g. The decay of this<br />
(<strong>in</strong>duced) lens with time would then be a consequence of the fact that charge<br />
would cont<strong>in</strong>ue to separate until E0 was totally screened, thereby saturat<strong>in</strong>g<br />
and flatten<strong>in</strong>g the <strong>in</strong>duced ”lens”. In this, <strong>in</strong>vestigators found the solution:<br />
they would foresee a compensat<strong>in</strong>g mechanism through which accumulated<br />
charge could be elim<strong>in</strong>ated by homogeneously illum<strong>in</strong>at<strong>in</strong>g the sample, which<br />
amounts to <strong>in</strong>creas<strong>in</strong>g the dark sample conductivity (see Fig.(3)). On the basis<br />
of the relative <strong>in</strong>tensity of the beam to the background, there would exist<br />
a dynamic equilibrium lead<strong>in</strong>g to a steady-state lens<strong>in</strong>g effect [12, 13, 14, 15].<br />
As the model was reformulated on this new, an to some extent, simpler<br />
screen<strong>in</strong>g idea, foresee<strong>in</strong>g the artificial enhancement of crystal dark conductivity,<br />
Castillo et al. [16] reported steady-state self-focus<strong>in</strong>g, us<strong>in</strong>g a homogeneous<br />
illum<strong>in</strong>ation to free accumulated charge. F<strong>in</strong>ally, Shih et al. [17, 18] and<br />
Kos et al. [19] were able to not only observe this non-transient soliton phenomenology,<br />
but also relate it to the new model. This type of self-trapp<strong>in</strong>g is
6 E. DelRe, M. Segev, D. Christodoulides, B. Crosignani, and G. Salamo<br />
Imag<strong>in</strong>g<br />
Lens<br />
CCD<br />
CCD<br />
<strong>Photorefractive</strong><br />
Sample<br />
Spherical<br />
Lens<br />
Polarizer BS<br />
V<br />
c<br />
Beam<br />
Expander<br />
Fig. 3. Scheme used to stabilize screen<strong>in</strong>g solitons, as described <strong>in</strong> [17] and [19].<br />
Now the diffract<strong>in</strong>g launch beam is accompanied by an ord<strong>in</strong>ary unfocused wave<br />
appropriately extracted from the s<strong>in</strong>gle laser.<br />
s<strong>in</strong>ce termed a screen<strong>in</strong>g soliton, and constitutes the most commonly studied<br />
type of photorefractive soliton. Its explanation requires a treatment which<br />
goes beyond the small modulation depth treatment, and for which s<strong>in</strong>gle<br />
mode description, such as the <strong>in</strong>volved <strong>in</strong> two-wave mix<strong>in</strong>g, is unsatisfactory.<br />
<strong>Photorefractive</strong> solitons have s<strong>in</strong>ce been observed <strong>in</strong> SBN, BSO, BGO,<br />
BTO, BaTiO3, LiNbO3, InP, CdZnTe, KLTN, KNbO3, polymers and organic<br />
glass.<br />
3 A saturable nonl<strong>in</strong>earity<br />
The formulation of a descriptive and predictive theory for photorefractive<br />
solitons <strong>in</strong>volves some profoundly different aspects and theoretical tools than<br />
those employed <strong>in</strong> traditional wave-mix<strong>in</strong>g theories. First, no periodic structure<br />
is present, and second, <strong>in</strong> most configurations, all the physical variables<br />
vary across the beam profile by a large fraction (e.g., from peak to zero <strong>in</strong>tensity)<br />
such that the modulation cannot be treated as a small perturbation.<br />
However, steady-state photorefractive solitons have two <strong>in</strong>tr<strong>in</strong>sic symmetries<br />
which reduce the problem: they are evidently time-<strong>in</strong>dependent, and their<br />
<strong>in</strong>tensity I is <strong>in</strong>dependent of the propagation coord<strong>in</strong>ate z. Yet the heart of<br />
complexity is nonl<strong>in</strong>earity, and even for a z-<strong>in</strong>variant photoioniz<strong>in</strong>g <strong>in</strong>tensity I<br />
there is still a wide range of parameters, of which only a small subset can support<br />
solitons. In order to formulate a semi-analytic theory, a one-dimensional<br />
reduction must be implemented: the beam should be such that no y-dynamics<br />
emerge, the soliton <strong>in</strong>tensity be<strong>in</strong>g solely x-dependent [I(x)]. Experimentally,<br />
this was achieved by launch<strong>in</strong>g a beam focused down through a cyl<strong>in</strong>drical<br />
lens, and quite similarly this has led to quasi-steady-state self-trapp<strong>in</strong>g <strong>in</strong> the<br />
absence of background [9], and to steady-state screen<strong>in</strong>g solitons for appropriate<br />
values of E0 (see Fig.(4)) [19].<br />
In fact, <strong>in</strong> many aspects these one-dimensional (stripe) waves, generally<br />
termed one-plus-one dimensional screen<strong>in</strong>g solitons [(1+1D)], share with<br />
z<br />
y<br />
PBS<br />
x<br />
Laser
<strong>Photorefractive</strong> <strong>Solitons</strong> 7<br />
Fig. 4. A one-dimensional soliton observed <strong>in</strong> biased SBN. Top: <strong>in</strong>put <strong>in</strong>tensity distribution,<br />
output l<strong>in</strong>ear diffraction (no bias), and output self-trapped beam. Center<br />
and bottom: profiles. As reported <strong>in</strong> [19]<br />
their needle-like counterparts, which are therefore two-plus-one-dimensional<br />
screen<strong>in</strong>g solitons [(2+1D)], the same behavior. Although (2+1)D self-trapp<strong>in</strong>g<br />
<strong>in</strong> photorefractive media is still not fully theoretically understood (see section<br />
4), the theory of (1+1)D photorefractive solitons [12, 13, 14, 15] constitutes<br />
the basic confirmation that photorefraction supports self-trapp<strong>in</strong>g.<br />
In most conditions of <strong>in</strong>terest, the optical <strong>in</strong>tensity distribution I(x) is<br />
such that, for an electron-dom<strong>in</strong>ated photorefraction, the result<strong>in</strong>g concentration<br />
of photo-excited electrons N, the concentration of acceptor impurities<br />
Na, and the concentration of donor impurities Nd follow the hierarchy<br />
N
8 E. DelRe, M. Segev, D. Christodoulides, B. Crosignani, and G. Salamo<br />
be identified with a saturation scale, i.e., that spatial scale under which the<br />
maximum atta<strong>in</strong>able charge (when the concentration of ionized donors N +<br />
d ≈<br />
Na) cannot screen E0 (which becomes comparable with the saturation field<br />
Eq). From Eq.(1) Y and Q are now related through<br />
′<br />
YQ Q Q<br />
+ a −<br />
1+Y ′ 1+Y ′ (1 + Y ′ <br />
′′<br />
Y = G, (2)<br />
) 2<br />
with a = NakbT/ɛE2 0 and G = gE0/Ib. The prime stands for (d/dξ). Equation<br />
(2) can be formally solved, without approximations, for Y to give<br />
Y = −a Q′<br />
Q<br />
′<br />
′′<br />
G GY Y<br />
+ + + a . (3)<br />
Q Q 1+Y ′<br />
We can now identify the various terms with precise physical processes, as we<br />
shall see. Equation (3) is rendered tractable by the fact that the greater part<br />
of spatial soliton studies <strong>in</strong>volve the trapp<strong>in</strong>g of beams with an <strong>in</strong>tensity Full-<br />
Width-Half-Maximum (FWHM) ∆x ∼10µm. For most configurations, xq ∼<br />
0.1 µm, andη = xq/∆x ∼0.01 represents a smallness parameter. In other<br />
words, screen<strong>in</strong>g solitons do not deplete photorefractive charge. A dimensional<br />
evaluation of the various terms for the appropriate high-modulation<br />
regime <strong>in</strong>dicates that<br />
Y (0) = G<br />
+ o(η), (4)<br />
Q<br />
s<strong>in</strong>ce a ∼2.5 , and G -1 [15]. A first correction is obta<strong>in</strong>ed by iterat<strong>in</strong>g this<br />
solution <strong>in</strong>to Eq.(3), and the result<strong>in</strong>g expression for Y is<br />
Y (1) = G Q′<br />
− aQ′ −<br />
Q Q Q<br />
2 G<br />
+ o(η<br />
Q<br />
2 ). (5)<br />
The first dom<strong>in</strong>ant term is generally referred as the screen<strong>in</strong>g term. It represents,<br />
<strong>in</strong> our discussion, the ma<strong>in</strong> agent lead<strong>in</strong>g to solitons. It is local, <strong>in</strong> that<br />
it does not <strong>in</strong>volve spatial derivatives or <strong>in</strong>tegration, has the same symmetry<br />
of the optical <strong>in</strong>tensity Q, and represents a decrease <strong>in</strong> E with respect to<br />
E0 on consequence of charge rearrangement (G -1). So perhaps the most<br />
astonish<strong>in</strong>g fact of our discussion is that, <strong>in</strong> truth, for a large variety of conditions,<br />
this form of self-focus<strong>in</strong>g (<strong>in</strong>clud<strong>in</strong>g self-defocus<strong>in</strong>g) is the dom<strong>in</strong>ant<br />
effect, as the plentiful family of reported observations that have followed the<br />
1992-1993 discovery imply. The second term, of first order <strong>in</strong> η, is simply<br />
the high-modulation version of what is generally called the diffusion field<br />
(Ed). The third, aga<strong>in</strong> of first order <strong>in</strong> η, is the coupl<strong>in</strong>g of the diffusion field<br />
with the screen<strong>in</strong>g field, a component sometimes referred to as deriv<strong>in</strong>g from<br />
charge-displacement [21]. Both these two last terms are nonlocal, <strong>in</strong> that they<br />
<strong>in</strong>volve a spatial derivative, and thus provide an anti-symmetric contribution<br />
to the space charge field (Y ) for a symmetric beam I(x) =I(−x). That is,<br />
these last two terms lead to a beam self-action of opposite symmetry of that
<strong>Photorefractive</strong> <strong>Solitons</strong> 9<br />
required to support solitons: whereas for conventional mix<strong>in</strong>g studies they<br />
play the central role, here they lead to beam self-bend<strong>in</strong>g (or self-deflection),<br />
which, for most configurations, amounts to a slight parabolic distortion of the<br />
preferentially z-oriented trajectory. The subject has attracted <strong>in</strong>terest over<br />
the years and has helped build an understand<strong>in</strong>g <strong>in</strong>to the limits of the local<br />
saturable nonl<strong>in</strong>earity model [10, 18, 21, 22, 23, 24, 25, 26, 27, 28, 29].<br />
In order to identify the nonl<strong>in</strong>earity, we must now translate the spacecharge<br />
field E <strong>in</strong>to an <strong>in</strong>dex modulation. The standard soliton set-up is such<br />
that a negative uniaxial zero-cut sample is positioned so that the x-axis is<br />
the direction along which E0 is applied, the soliton beam of <strong>in</strong>tensity I is<br />
extraord<strong>in</strong>arily-polarized and is propagat<strong>in</strong>g along z, while Ib is obta<strong>in</strong>ed<br />
through a co-propagat<strong>in</strong>g ord<strong>in</strong>arily-polarized plane-wave [17]. For a noncentrosymmetric<br />
photorefractive, like SBN, ∆n = − 1<br />
2n3r33E, n be<strong>in</strong>g the<br />
unperturbed crystal <strong>in</strong>dex of refraction, and rij the l<strong>in</strong>ear electro-optic tensor<br />
of the sample. On tak<strong>in</strong>g, consistently with our iterative scheme, the<br />
expression of Eq.(4), we obta<strong>in</strong> the nonl<strong>in</strong>earity<br />
∆n(I) =− 1<br />
2 n3 V 1<br />
1<br />
r33<br />
= −∆n0 , (6)<br />
Lx 1+I/Ib 1+I/Ib<br />
which constitutes a saturable nonl<strong>in</strong>earity, identical (with<strong>in</strong> a constant term)<br />
to the nonl<strong>in</strong>ear <strong>in</strong>dex change <strong>in</strong> a homogeneously-broadened two-levelsystem.<br />
3.2 The soliton-support<strong>in</strong>g nonl<strong>in</strong>ear equation<br />
A soliton is loosely def<strong>in</strong>ed as a wave that preserves its shape and velocity<br />
throughout propagation, while, very importantly, display<strong>in</strong>g a particle-like<br />
behavior when made to <strong>in</strong>teract (”collide”) with other solitons. As such, solitons<br />
possess a number of conserved quantities, such as power, momentum,<br />
Hamiltonian, etc. [4]. Optical spatial solitons, <strong>in</strong> their scalar manifestation,<br />
are generally governed by the nonl<strong>in</strong>ear equation for a monochromatic paraxial<br />
beam<br />
<br />
∂ i<br />
−<br />
∂z 2k<br />
d2 dx2 <br />
A(x, z) =− ik<br />
∆nA(x, z) (7)<br />
n<br />
where k =2πn/λ is the wave-vector, A is the extraord<strong>in</strong>ary component of<br />
the slowly vary<strong>in</strong>g optical field, i.e. Eopt(x, z, t) = A(x, z)exp(ikz − iωt),<br />
ω =2πc/nλ, andI = |A(x, z)| 2 . We seek stationary (non-diffract<strong>in</strong>g) solutions<br />
of the form A(x, z) = u(x)eiΓ z√Ib, normalize the transverse spatial<br />
scale to the so-called nonl<strong>in</strong>ear length scale d = (±2kb) −1/2 , i.e.,<br />
ξ = x/d, which for photorefractive solitons is obta<strong>in</strong>ed from the expression<br />
b =(1/2)kn2r33(V/Lx), and obta<strong>in</strong> [12, 15]<br />
d 2 u(ξ)<br />
dξ 2<br />
= ±<br />
Γ<br />
b −<br />
1<br />
1+u(ξ) 2<br />
<br />
u(ξ). (8)
10 E. DelRe, M. Segev, D. Christodoulides, B. Crosignani, and G. Salamo<br />
The plus sign is for b>0, the m<strong>in</strong>us for b0, or a self-defocus<strong>in</strong>g,<br />
for b0, and we observe a self-focus<strong>in</strong>g<br />
nonl<strong>in</strong>earity. It is possible to apply E0 <strong>in</strong> a direction opposite to ferroelectric<br />
axis, thus effectively chang<strong>in</strong>g the sign of b, then E0 must be smaller than the<br />
coercive field, otherwise it may render the ferroelectric crystall<strong>in</strong>e structure<br />
unstable and de-pole the crystal. Both defocus<strong>in</strong>g and focus<strong>in</strong>g nonl<strong>in</strong>earities<br />
support solitons. A self-focus<strong>in</strong>g nonl<strong>in</strong>earity traps a conventional bell-shaped<br />
beam <strong>in</strong>to a bright soliton; a self-defocus<strong>in</strong>g nonl<strong>in</strong>earity traps a wave feature,<br />
such as a notch generated by a π phase jump, whose structure is enlarged by<br />
the diffraction of surround<strong>in</strong>g illum<strong>in</strong>ated regions, the ensu<strong>in</strong>g propagation<br />
<strong>in</strong>variant wave be<strong>in</strong>g termed a dark soliton.<br />
Equation (8) can be <strong>in</strong>tegrated (by quadrature) once, giv<strong>in</strong>g the relationship<br />
Γ/b = log 1+u2 <br />
2<br />
0 /u0 for bright beams, and Γ/b =1/ 1+u2 <br />
∞ for<br />
dark, where u∞ = u(∞) =−u(−∞), and u0 = u(0) (u2 0 = I(0)/Ib be<strong>in</strong>g<br />
referred to as the <strong>in</strong>tensity ratio).<br />
3.3 Soliton waveforms and existence curve<br />
As can be imag<strong>in</strong>ed, the self-trapped waves u, solutions of Eq.(8), form an isolated<br />
subset of all possible dynamical evolutions described by Eq.(7). The imposition<br />
of z-<strong>in</strong>variance implies not only a specific relationship between beam<br />
parameters, but fixes the actual waveform u <strong>in</strong> all its details (see Fig.(5)). In<br />
general, such a prediction can have little if no physical mean<strong>in</strong>g. For solitons,<br />
however, we have two counter<strong>in</strong>g effects, diffraction and self-focus<strong>in</strong>g, which<br />
are coupled by nonl<strong>in</strong>earity to form a feedback mechanism. The result is that<br />
most soliton solutions are stable to perturbations, and represent an attractor<br />
to system dynamics. This, <strong>in</strong> turn, conta<strong>in</strong>s the beauty and physical appeal of<br />
soliton physics: that a propagat<strong>in</strong>g beam, <strong>in</strong>teract<strong>in</strong>g <strong>in</strong> a non-trivial way with<br />
a host<strong>in</strong>g medium, should preferably be attracted to a robust, propagation<strong>in</strong>variant,<br />
and very specific wave-form, <strong>in</strong>stead of produc<strong>in</strong>g an unstable and<br />
unpredictable chaotic system.<br />
Return<strong>in</strong>g to our system, what are the soliton wave-forms, and, more<br />
importantly, what are the beam parameters, ∆ξ (associated to ∆x) and <strong>in</strong>tensity<br />
ratio u 2 0, that characterize the subset of soliton solutions? The issue<br />
is of particular importance, because, although self-trapp<strong>in</strong>g forms an attractor,<br />
launch experiments are designed to determ<strong>in</strong>istically lead to a soliton,<br />
a scheme that requires the launch to be close enough to a self-trapped wave<br />
<strong>in</strong> parameter space (<strong>in</strong>tensity u 2 0 and normalized width ∆ξ). For the family<br />
of <strong>in</strong>tegrable nonl<strong>in</strong>ear equations, such as the S<strong>in</strong>e-Gordon, the Nonl<strong>in</strong>ear<br />
Schroed<strong>in</strong>ger, and the Korteweg and de-Vries equations, an explicit solution
<strong>Photorefractive</strong> <strong>Solitons</strong> 11<br />
can be found, for which the relationship between beam ∆ξ and u 2 0 is unique.<br />
However, for the saturable nonl<strong>in</strong>earity described by Eqs.(6,8) the ∆ξ versus<br />
u 2 0 relation is not unique, but <strong>in</strong>stead yields a cont<strong>in</strong>uous curve commonly<br />
termed the soliton existence curve [15] (see Fig. (6)).<br />
Fig. 5. Soliton waveforms for bright solitons, as reported <strong>in</strong> [19].<br />
The wavefunctions of bright photorefractive screen<strong>in</strong>g solitons are bell-shaped<br />
functions which are neither a Gaussian nor a hyperbolic secant [30]. Experimentally,<br />
such solitons are generated by launch<strong>in</strong>g a focused-down onedimensional<br />
Gaussian beam with a ∆x and peak <strong>in</strong>tensity I0 such that, for<br />
the given configuration of crystal parameters n, r33, andIb, for the given bias<br />
E0, the result<strong>in</strong>g values of ∆ξ and u0 lie on the existence curve. For dark<br />
solitons, <strong>in</strong> turn, the same procedure can be implemented for the relevant<br />
(u∞,∆ξ) parameter space.<br />
3.4 Experiments and theory<br />
The ma<strong>in</strong> advantage of hav<strong>in</strong>g formulated the theory highlight<strong>in</strong>g the saturable<br />
nature of the nonl<strong>in</strong>earity is that, with<strong>in</strong> the limits <strong>in</strong> which the underly<strong>in</strong>g<br />
approximations are valid, it allows the prediction of solitons as a<br />
specific feature <strong>in</strong>dependent on the particular experimental configuration.<br />
Thus a physically identical soliton will emerge for two self-trapped beams<br />
of, say 10 and 20 µm, as long as the applied voltage V , material response,
12 E. DelRe, M. Segev, D. Christodoulides, B. Crosignani, and G. Salamo<br />
Fig. 6. Soliton bright and dark existence curve, as reported <strong>in</strong> [19].<br />
beam <strong>in</strong>tensity and background illum<strong>in</strong>ation are such as to project the two<br />
conditions on the very same po<strong>in</strong>t on the (u0, ∆ξ) parameter space. Note<br />
that this powerful device breaks down as soon as we consider the o(η) terms,<br />
or even simple corrections <strong>in</strong> the actual nonl<strong>in</strong>earity, such as those deriv<strong>in</strong>g<br />
from dielectric nonl<strong>in</strong>earity [31].<br />
In order to test the validity of the treatment, experiments have been carried<br />
out with the aim of detect<strong>in</strong>g for what conditions of launch a 1+1D<br />
steady-state soliton would form [19, 32, 33], and some examples of results are<br />
conta<strong>in</strong>ed <strong>in</strong> Fig.(7) for bright solitons and Fig.(8) for dark.<br />
Indeed other experiments have led to much the same conclusions, for<br />
which the qualitative agreement is full, but for some regions of parameters,<br />
where the quantitative comparison is weaker. At present it is believed that<br />
the discrepancy is due more to the presence of extraneous effects than to<br />
a deficiency <strong>in</strong> the model. For example, it has been observed that some of<br />
the background illum<strong>in</strong>ation, which is made to propagate along an ord<strong>in</strong>ary<br />
mode, <strong>in</strong> order to not undergo substantial evolution, is actually trapped by<br />
the soliton through the f<strong>in</strong>ite r13 coefficient. Another source of uncerta<strong>in</strong>ty<br />
is connected to the difficulty <strong>in</strong> establish<strong>in</strong>g the precise value of rij for the<br />
given sample: this can depend on the level of purity of the pol<strong>in</strong>g, on the<br />
presence of considerable clamp<strong>in</strong>g and on temperature.<br />
Concern<strong>in</strong>g more fundamental aspects of the model, we note that although<br />
the results shown <strong>in</strong> Fig.(7) support the approximation conta<strong>in</strong>ed <strong>in</strong> Eq.(4),<br />
the actual beam evolution shows a clear and reproducible self-bend<strong>in</strong>g effect
<strong>Photorefractive</strong> <strong>Solitons</strong> 13<br />
Fig. 7. Comparison between experiments and theory for (1+1)D bright screen<strong>in</strong>g<br />
solitons, from [32]. Here the low-<strong>in</strong>tensity regime is what we specifically term<br />
screen<strong>in</strong>g solitons.<br />
Fig. 8. Comparison between experiments and theory for (1+1)D dark screen<strong>in</strong>g<br />
solitons, from [?]
14 E. DelRe, M. Segev, D. Christodoulides, B. Crosignani, and G. Salamo<br />
that can only f<strong>in</strong>d its explanation <strong>in</strong> the full expression of Eq.(5). It appears<br />
that, even though these nonlocal terms produce a parabolic trajectory, they<br />
do not greatly <strong>in</strong>fluence the existence curve. From a different perspective,<br />
we note that self-bend<strong>in</strong>g becomes an important issue when experiments are<br />
carried <strong>in</strong> highly solitonic regimes, characterized by a large ratio between selftrapped<br />
propagation distance and l<strong>in</strong>ear diffraction length Lz/Ld: to <strong>in</strong>crease<br />
Lz/Ld we can either use a longer sample, this <strong>in</strong>creas<strong>in</strong>g nonl<strong>in</strong>early the<br />
lateral shift, or use tighter launch beams, this <strong>in</strong>creas<strong>in</strong>g η.<br />
4 Two-dimensional solitons<br />
The (1+1)D screen<strong>in</strong>g solitons represent the firm experimental and theoretical<br />
foothold on which a large part of research rests, especially because of the<br />
appeal<strong>in</strong>g nature of the saturable nonl<strong>in</strong>earity which gives rise to numerous<br />
(fasc<strong>in</strong>at<strong>in</strong>g) soliton <strong>in</strong>teractions not present with Kerr-type solitons. However,<br />
the most ground-break<strong>in</strong>g achievement, both from the physical and from<br />
the applicative po<strong>in</strong>t of view, is the self-trapp<strong>in</strong>g of (2+1)D solitons. As their<br />
lower-dimensional counterparts, needles form both <strong>in</strong> the transient regime<br />
- as quasi-steady-state self-trapp<strong>in</strong>g [7] - and <strong>in</strong> temporal steady state as<br />
(2+1)D screen<strong>in</strong>g solitons [17, 18]. Such needle-like solitons were orig<strong>in</strong>ally<br />
documented <strong>in</strong> SBN, and have been replicated <strong>in</strong> most soliton-support<strong>in</strong>g<br />
photorefractive media, such as other ferroelectrics [34], semiconductors [35],<br />
paraelectrics [36], sillenites [37], and <strong>in</strong>deed for most types of self-trapp<strong>in</strong>g:<br />
bright, photovoltaic [38], multimode [39, 40, 41], and <strong>in</strong>coherent [42, 43], to<br />
name a few. Furthermore, even (2+1)D dark solitons were observed <strong>in</strong> photorefractives,<br />
<strong>in</strong> quasi-steady-state [44] and <strong>in</strong> steady-state [45] under a bias<br />
field, as well as photovoltaic [46] and <strong>in</strong>coherent [47] dark ”vortex” solitons.<br />
An example of a dark vortex screen<strong>in</strong>g soliton is shown <strong>in</strong> Fig.(12). Twoplus-one<br />
dimensional solitons form when a circularly symmetric beam is focused<br />
down onto the <strong>in</strong>put face of the sample, and the <strong>in</strong>itially diffract<strong>in</strong>g<br />
beam collapses <strong>in</strong>to a non-diffract<strong>in</strong>g 2D beam hav<strong>in</strong>g an almost ideally<br />
circularly-symmetric shape (see Fig.(9)). These studies, which constitute<br />
one of the rare possibilities of observ<strong>in</strong>g (2+1)D solitons, have greatly<br />
contributed to the understand<strong>in</strong>g of the physics associated with higher-thanone-dimensional<br />
nonl<strong>in</strong>ear waves. The observation of soliton spiral<strong>in</strong>g <strong>in</strong> full<br />
3D [48], as well as fusion, fission, birth and annihilation of (2+1)D solitons<br />
[49, 50, 51], have extended the very concept of soliton-particle behavior.<br />
The description and understand<strong>in</strong>g of the mechanisms that support<br />
(2+1)D solitons are, to some extent even today, still <strong>in</strong>complete. This is<br />
because the propagation <strong>in</strong>volves a nontrivial three-dimensional, anisotropic,<br />
and spatially nonlocal nonl<strong>in</strong>ear problem [52, 53, 54, 55, 56, 57]. The fact<br />
that photorefractives can support self-trapped needles of (almost ideally)<br />
circularly-symmetric shape seems very surpris<strong>in</strong>g right from the outset. More
<strong>Photorefractive</strong> <strong>Solitons</strong> 15<br />
Fig. 9. The direct and detailed observation of a circularly-symmetric 12 µm needle<br />
phenomenology <strong>in</strong> a non-zero-cut sample of SBN, from [18].<br />
specifically, the external field is applied between two parallel planar electrodes,<br />
and thus breaks the circular symmetry of the problem. The explanation<br />
relates to the fact that the (space charge) field l<strong>in</strong>es bend <strong>in</strong> the regions of<br />
higher illum<strong>in</strong>ation, and, for some range of parameters seem to yield a quasiradial<br />
distribution of the field component giv<strong>in</strong>g rise to a nonl<strong>in</strong>ear <strong>in</strong>dex<br />
change. For example, <strong>in</strong> SBN this means that the c-component of the space<br />
charge field has roughly a circular symmetry. The very fact that such (2+1)D<br />
propagate <strong>in</strong> a stable fashion, not undergo<strong>in</strong>g catastrophic collapse (as such<br />
solitons <strong>in</strong> Kerr media would), is a direct <strong>in</strong>dicative that the photorefractive<br />
nonl<strong>in</strong>earity is saturable also <strong>in</strong> two (transverse) dimensions. However, dur<strong>in</strong>g<br />
the temporal transients, and for various values of applied field, self-trapp<strong>in</strong>g<br />
manifests considerable beam ellipticity [52], exclud<strong>in</strong>g the direct validity of<br />
a circularly-symmetric 2D saturable model. Nevertheless, the large amount<br />
of experimental evidence on 2D solitons <strong>in</strong> almost every photorefractive material<br />
<strong>in</strong> which solitons have been identified, implies that a modified model,<br />
possibly anisotropic and slightly nonlocal, should exist [55]. What clears the<br />
picture are the studies on (2+1)D soliton <strong>in</strong>teraction-collisions. On the one<br />
hand, spiral<strong>in</strong>g and large angle collisions show that whatever anisotropic components<br />
emerge, they do rema<strong>in</strong> localized around the beam [48, 58], whereas<br />
lower angle collisions <strong>in</strong>dicate unmistakably the presence of a saturable yet<br />
anisotropic nonl<strong>in</strong>ear behavior: the repulsion of <strong>in</strong>coherent needles [59].
16 E. DelRe, M. Segev, D. Christodoulides, B. Crosignani, and G. Salamo<br />
From a theoretical perspective, the system has two fundamental anisotropies:<br />
the boundary conditions, which emerge from the application of an external<br />
bias along the x-direction, and the electro-optic response, which implies a<br />
complex tensorial <strong>in</strong>dex modulation depend<strong>in</strong>g on the beam polarization, direction<br />
of the local electric field E, and the relative orientation with respect<br />
to the crystal lattice. The result is that the nonl<strong>in</strong>ear response has a nonlocal<br />
component that is superimposed on the saturable component [54]. In order<br />
for a quasi-circular optical symmetry to appear, the underly<strong>in</strong>g space-charge<br />
field E must be anisotropic, manifest<strong>in</strong>g two characteristic lateral lobes (see<br />
Fig.(10)) [60]. The appearance of these features, that have an <strong>in</strong>creased complexity<br />
with respect to the ioniz<strong>in</strong>g <strong>in</strong>tensity I(x, y), are the basic manifestation<br />
of a nonlocal mechanism. Contrary to what might seem logical, if one<br />
attempts to identify their orig<strong>in</strong> extend<strong>in</strong>g our knowledge of (1+1)D solitons,<br />
these lobes do not emerge because of the nonlocal mechanisms <strong>in</strong>dicated <strong>in</strong><br />
Eq.(5). These lobes emerge due to the match<strong>in</strong>g of boundary conditions <strong>in</strong><br />
the higher dimensional case, i.e., they match the local field structure, <strong>in</strong> the<br />
beam cross-section, to the x-oriented E = E0 far from the beam.<br />
In the 2+1D case we start from the basic relation, valid to zero order <strong>in</strong><br />
η,<br />
and the irrotational condition<br />
∇·(Y Q) = 0 (9)<br />
∇×Y =0. (10)<br />
From these a lobular structure emerges (see Fig.(11)). This anisotropy which<br />
is not at all connected to η, is simply not small <strong>in</strong> any accessible case. In<br />
other words, the nonlocality <strong>in</strong> the (2+1)D case is <strong>in</strong>tr<strong>in</strong>sic to the process,<br />
whereas it is merely a correction for (1+1)D solitons.<br />
The fact that 2+1D solitons are supported by this more complex nonl<strong>in</strong>earity<br />
does not substantially modify our soliton picture. One burden<strong>in</strong>g<br />
consequence, however, is that we do not have a means to formulate <strong>in</strong> a<br />
straightforward manner an existence curve for (2+1)D solitons, nor can we<br />
unequivocally say if such a concise and powerful tool even exists for the<br />
higher dimensional solitons. Nevertheless, if we phenomenologically build the<br />
set of po<strong>in</strong>ts <strong>in</strong> which it is possible to observe circular-symmetric self-trapp<strong>in</strong>g<br />
[18, 36], we f<strong>in</strong>d a s<strong>in</strong>gle valued cont<strong>in</strong>uous curve that behaves and looks just<br />
like the existence curve of (1+1)D solitons (albeit at somewhat higher values<br />
of ∆ξ).<br />
Evidence on both the existence of circularly-symmetric solitons and of<br />
their <strong>in</strong>tr<strong>in</strong>sic difference from (1+1)D solitons <strong>in</strong> photorefractives is highlighted<br />
by the experimental studies on transverse <strong>in</strong>stability of (1+1)D solitons<br />
<strong>in</strong> bulk media. In those experiments, <strong>in</strong>creas<strong>in</strong>g the nonl<strong>in</strong>earity leads<br />
a (1+1)D soliton (at the proper value of nonl<strong>in</strong>earity vs <strong>in</strong>tensity ratio, as
<strong>Photorefractive</strong> <strong>Solitons</strong> 17<br />
Fig. 10. Needle electro-holography from [60]. (a-c) conventional formation of a<br />
centrosymmetric soliton; (d) electroholography show<strong>in</strong>g the lobes.<br />
Fig. 11. Numerically evaluated x-component of E (top) for the soliton beam profile<br />
(bottom), from [55].
18 E. DelRe, M. Segev, D. Christodoulides, B. Crosignani, and G. Salamo<br />
Fig. 12. A screen<strong>in</strong>g vortex and its guid<strong>in</strong>g features, from [45]. (a) Input <strong>in</strong>tensity<br />
distribution of the vortex; (b) Diffract<strong>in</strong>g vortex after l<strong>in</strong>ear propagation to the<br />
output of the sample; (c) Self-trapped output <strong>in</strong>tensity distribution <strong>in</strong> a biased<br />
sample. (bottom) Probe beam guided propagation.<br />
Fig. 13. Transition from (1+1)D to (2+1)D self-trapp<strong>in</strong>g, from [61].<br />
determ<strong>in</strong>ed by the existence curve); then, a further <strong>in</strong>crease <strong>in</strong> the nonl<strong>in</strong>earity<br />
results <strong>in</strong> beam breakup <strong>in</strong>to an array of circularly-symmetric solitons, as<br />
shown <strong>in</strong> Fig.(13) [61].<br />
5 Temporal effects and quasi-steady-state dynamics<br />
One of the ma<strong>in</strong> characteristics of photorefraction is that it is a cumulative<br />
process. This is the orig<strong>in</strong> of its elevated response even at low optical <strong>in</strong>tensities.<br />
Evolution is dom<strong>in</strong>ated by a charge redistribution process which<br />
leads to a time constant τ ∝ 1/I. For small-modulation depth conditions I is<br />
almost constant, and a s<strong>in</strong>gle-time-constant behavior can be identified. For<br />
spatial solitons the story is quite different: not only are we faced with a high<br />
modulation response, and the time constant changes <strong>in</strong> the transverse plane,<br />
but s<strong>in</strong>ce they form out of a three-dimensionally resolved diffract<strong>in</strong>g beam,<br />
time behavior is also resolved <strong>in</strong> the propagation direction. The result is an<br />
evolution which presents a number of surpris<strong>in</strong>g phenomenologies, which are,
<strong>Photorefractive</strong> <strong>Solitons</strong> 19<br />
however, complicated and difficult to describe (an example that goes beyond<br />
soliton studies can be found <strong>in</strong> [62]).<br />
Possibly the most important, and, <strong>in</strong>deed, surpris<strong>in</strong>gly, effect is observed<br />
when launch<strong>in</strong>g a diffract<strong>in</strong>g beam <strong>in</strong> an appropriately biased sample, without<br />
any appreciable background illum<strong>in</strong>ation. As reported <strong>in</strong> the very first<br />
experiments on solitons by Duree et al. <strong>in</strong> Ref.[7], the beam is observed to<br />
form, after a time <strong>in</strong>terval of the order of 10ms, a spatial soliton, rema<strong>in</strong><br />
almost stationary for an <strong>in</strong>terval of 20ms, and then decay <strong>in</strong>to a once aga<strong>in</strong><br />
diffract<strong>in</strong>g beam. This peculiar sequence, which <strong>in</strong>volves a rare plateau evolution,<br />
is referred to as a quasi-steady-state soliton.<br />
The time dependent version of Eq.(2) truncated at zero order <strong>in</strong> η reads<br />
∂Y<br />
+ QY = G, (11)<br />
∂τ<br />
where τ = t/τd, τd = ɛ0ɛrγNa/(qµs(Nd−Na)Ib) is the characteristic dielectric<br />
time constant, γ is the recomb<strong>in</strong>ation rate, µ the electron mobility, s the donor<br />
impurity photoionization efficiency, and, as occurs for most configurations of<br />
<strong>in</strong>terest to soliton dynamics, the charge recomb<strong>in</strong>ation time τr=1/(Nγ)is<br />
much shorter than charge displacement dynamics, and no time dependence<br />
<strong>in</strong> the boundary conditions are considered (G=-1). For small modulation,<br />
Eq.(11) gives the characteristic exponential dynamics with t = τd/Q, but as<br />
soon as Q is spatially resolved, and furthermore is itself evolv<strong>in</strong>g, a cont<strong>in</strong>uum<br />
of different time constant contribute. Seen <strong>in</strong> a different perspective, soliton<br />
time evolution is highly time-nonlocal, as the formally equivalent <strong>in</strong>tegral<br />
version of Eq.(11)<br />
Y = e −<br />
τ<br />
τ<br />
′<br />
Qdτ<br />
0 1+ dτ<br />
0<br />
′ τ<br />
′ <br />
′′<br />
Qdτ<br />
e 0 , (12)<br />
<strong>in</strong>dicates [54]. The full complexity of this behavior emerges dur<strong>in</strong>g transients,<br />
i.e., when I changes <strong>in</strong> an appreciable manner with time. This occurs most<br />
evidently dur<strong>in</strong>g the very first collaps<strong>in</strong>g stage, for times τ ≤ 1/(1 + u2 0), and<br />
leads to a stretched exponential evolution [63]. A characteristic of multi-scale<br />
processes, this behavior is common to the entire family of soliton support<strong>in</strong>g<br />
cumulative nonl<strong>in</strong>earities. A numerical approach to Eq.(12) coupled to the<br />
parabolic wave equation confirms experimental f<strong>in</strong>d<strong>in</strong>gs, but to date there is<br />
no clear understand<strong>in</strong>g as to why the soliton should pass through a plateau,<br />
and, more importantly, how to evaluate the so-called threshold nonl<strong>in</strong>earity<br />
for which self-trapp<strong>in</strong>g is achieved, the duration of the plateau, and the<br />
nonl<strong>in</strong>ear equation, such as Eq.(8), for which the waves are eigenfunctions.<br />
Furthermore, we do not have a means to predict the actual trapp<strong>in</strong>g ∆x at<br />
the plateau, for a given nonl<strong>in</strong>earity.<br />
In order to highlight the sole role of high modulation depth, we can considerably<br />
simplify our predictions, exclud<strong>in</strong>g nonlocality, by impos<strong>in</strong>g that Q<br />
not have relevant time-dependence [64]. In this case Eq.(12) is simplified to<br />
give
20 E. DelRe, M. Segev, D. Christodoulides, B. Crosignani, and G. Salamo<br />
Y = e −τQ (1 + 1<br />
Q (eτQ − 1)), (13)<br />
where Q is an appropriate time average. Whereas this approach can be<br />
mean<strong>in</strong>gful and useful for conditions <strong>in</strong> which a soliton (i.e., the beam I)<br />
is steady, such as for steady-state <strong>in</strong>coherent solitons which we will describe<br />
below, it can say noth<strong>in</strong>g as to beam transients. It has been speculated that<br />
Eq.(13) could be valid when a negligible amount of diffraction is <strong>in</strong>volved<br />
[65, 66, 67, 68, 69].<br />
Delay<strong>in</strong>g the discussion of <strong>in</strong>coherent self-trapp<strong>in</strong>g, a consequence of cumulative<br />
<strong>in</strong>ertial response, to section 10, we add a mention to the wealth of<br />
transient phenomenologies that occur for higher-dimensional needles [70], and<br />
those associated to a time-dependent external bias E0 [11, 71, 72, 73]. Lastly,<br />
we should mention the study of s<strong>in</strong>gle pulse propagation and space-charge<br />
build-up [74, 75].<br />
6 Various photorefractive mechanisms support<strong>in</strong>g<br />
self-trapp<strong>in</strong>g<br />
One of the nicest features of self-trapp<strong>in</strong>g of optical beams <strong>in</strong> photorefractives<br />
is the diversity of mechanisms that can support solitons. Apart from<br />
the solitons described <strong>in</strong> the previous section, which relied on an externallyapplied<br />
bias field, self-trapp<strong>in</strong>g <strong>in</strong> photorefractives can also arise from photovoltaic<br />
effects [76], or from diffusion-driven effects [77], or from resonantlyenhanced<br />
effects caused by the excitation of both electrons and holes [78]. In<br />
several cases, comb<strong>in</strong>ations of two of these effects can also lead to solitons<br />
[e.g., solitons supported by the photovoltaic and the screen<strong>in</strong>g nonl<strong>in</strong>earities<br />
simultaneously]. Furthermore, <strong>in</strong> some cases, self-trapp<strong>in</strong>g can arise from<br />
semi-permanent changes <strong>in</strong> the crystall<strong>in</strong>e structure, either though cluster<strong>in</strong>g<br />
of ferroelectric doma<strong>in</strong>s [79], or through re-pol<strong>in</strong>g of macroscopic regions<br />
[80, 81], both be<strong>in</strong>g driven by the local space charge field. Such permanent<br />
changes are <strong>in</strong> fact ”fixed” (soliton-<strong>in</strong>duced) waveguides, act<strong>in</strong>g as microstructure<br />
optical circuits ”impressed” <strong>in</strong>to the volume of the bulk nonl<strong>in</strong>ear crystal.<br />
To this date, this is one of the very few techniques to create <strong>in</strong>tricate 3D optical<br />
circuitry. In this section, we briefly review these additional mechanisms<br />
support<strong>in</strong>g self-trapp<strong>in</strong>g of optical beams <strong>in</strong> photorefractive media.<br />
6.1 Photovoltaic solitons<br />
Soliton-support<strong>in</strong>g mechanisms appear <strong>in</strong> photorefractives also <strong>in</strong> the absence<br />
of electric fields, the major example be<strong>in</strong>g photovoltaic solitons [76, 82]. Here,<br />
<strong>in</strong> open-circuit conditions and for the (1+1)D geometry, the non-uniform optical<br />
excitation translates <strong>in</strong>to a non-uniform photo<strong>in</strong>duced current. This, at
<strong>Photorefractive</strong> <strong>Solitons</strong> 21<br />
steady state, must be countered by the drift of photo-excited charge (electrons)<br />
<strong>in</strong> response to E. Under conditions analogous to those lead<strong>in</strong>g to<br />
Eq.(4), for a beam with features ∆x of the order of several microns, we<br />
arrive aga<strong>in</strong> at a saturable nonl<strong>in</strong>earity<br />
∆n(I) =− 1<br />
2 n3 I<br />
I<br />
r33Ep = −∆n0,p , (14)<br />
Id + I Id + I<br />
where Ep = βphNaγ/(qµs), Id the equivalent dark illum<strong>in</strong>ation, the constitutive<br />
relation for the current along x be<strong>in</strong>g J = qµNE + βph(Nd − N +<br />
d ). Much<br />
<strong>in</strong> the same fashion of Eq.(8), this nonl<strong>in</strong>earity leads to a nonl<strong>in</strong>ear soliton<br />
equation that supports bright and dark solitons on the basis of the sign of<br />
∆n0,p, i.e., on the sign of βph [76, 82].<br />
Most of the experiments with photovoltaic solitons have been carried out<br />
<strong>in</strong> LiNbO3, for which βph is negative for an extraord<strong>in</strong>ary beam propagat<strong>in</strong>g<br />
along z, this lead<strong>in</strong>g to the observation of one-dimensional dark photovoltaic<br />
solitons [83].<br />
Fig. 14. Photovoltaic dark soliton setup, from [83]. Note the use of a resolved<br />
transverse phase-structure obta<strong>in</strong>ed by hav<strong>in</strong>g part of the launch beam pass through<br />
an appropriate piece of glass.<br />
As occurs for the screen<strong>in</strong>g type nonl<strong>in</strong>earity, photovoltaic solitons can<br />
also form <strong>in</strong> the higher-dimensional case. For LiNbO3, theseformasdark<br />
vortex solitons which are supported by a ”spiral<strong>in</strong>g” transverse phase modulation<br />
[46] (see Fig.(16) ). In KNSBN, photovoltaic self-action is self-focus<strong>in</strong>g,<br />
and even bright (2+1)D photovoltaic solitons have been detected [38]. Moreover,<br />
it has been predicted and demonstrated that the use of a background<br />
illum<strong>in</strong>ation, not a strict requirement <strong>in</strong> photovoltaics, allows the transitions<br />
from the defocus<strong>in</strong>g to a focus<strong>in</strong>g nonl<strong>in</strong>earity <strong>in</strong> LiNbO3 [84].<br />
6.2 Resonantly-enhanced self-trapp<strong>in</strong>g <strong>in</strong> semiconductors<br />
One of the nicest features of photorefractive solitons is the very low power<br />
level at which they can form, allow<strong>in</strong>g soliton experiments with microwatt
22 E. DelRe, M. Segev, D. Christodoulides, B. Crosignani, and G. Salamo<br />
Fig. 15. Observations of dark photovoltaic solitons, from [83]. (a) l<strong>in</strong>early diffract<strong>in</strong>g<br />
<strong>in</strong>tensity distribution of a dark notch; (b) self-trapped <strong>in</strong>tensity distribution,<br />
for various propagation distances <strong>in</strong> the sample.<br />
Fig. 16. Self-trapp<strong>in</strong>g of a photovoltaic vortex, from [46]. (a) output <strong>in</strong>tensity<br />
distribution before self-focus<strong>in</strong>g beg<strong>in</strong>s, and phase pattern; (b) output <strong>in</strong>tensity<br />
distribution trapped by the photovoltaic field, and phase pattern.<br />
(and lower) power levels. As will be discussed <strong>in</strong> the section on applications,<br />
photorefractive solitons, and the waveguides they <strong>in</strong>duce, comb<strong>in</strong>e properties<br />
that suggest <strong>in</strong>terest<strong>in</strong>g applications rang<strong>in</strong>g from reconfigurable directional<br />
couplers, beam splitters, waveguide switch<strong>in</strong>g devices, tunable waveguides for<br />
second harmonic generation, and highly efficient optical parametric oscillators<br />
<strong>in</strong> soliton-<strong>in</strong>duced waveguides. In general, however, the formation time<br />
of solitons <strong>in</strong> most photorefractive materials is rather long, except when very<br />
high <strong>in</strong>tensities are used [32]. This is because the photorefractive nonl<strong>in</strong>earity<br />
relies on charge separation, for which the response time is the dielectric<br />
relaxation time, i.e., <strong>in</strong>versely proportional to the product of the mobility<br />
and the optical <strong>in</strong>tensity, and the mobility <strong>in</strong> photorefractive oxides is low.<br />
In pr<strong>in</strong>ciple, however, photorefractive semiconductors, (e.g., InP, CdZnTe),<br />
have a high mobility and could offer formation times a thousand fold faster<br />
than <strong>in</strong> the other photorefractives. However, the electrooptic effects <strong>in</strong> these<br />
semiconductors are t<strong>in</strong>y, which implies that solitons that are as narrow as 20<br />
optical wavelengths necessitate very large applied fields, mak<strong>in</strong>g solitons <strong>in</strong>
<strong>Photorefractive</strong> <strong>Solitons</strong> 23<br />
them almost impossible to observe. But, <strong>in</strong> some of these materials (InP and<br />
CdZnTe) that have both holes and electrons as charge carriers, a unique resonance<br />
mechanism can greatly enhance the space charge field by as much as<br />
10 times (and more) over the applied electric field. This enhancement yields<br />
large enough self-focus<strong>in</strong>g effects that can support narrow spatial solitons.<br />
The resonant enhancement of the space charge field has led to the observation<br />
of solitons <strong>in</strong> photorefractive InP [78, 35] and CdZnTe [85].<br />
As mentioned, the resonant enhancement of the space charge field occurs<br />
<strong>in</strong> materials with both types of charge carriers, both be<strong>in</strong>g excited from a<br />
common trap level: one excited optically and the other excited by temperature<br />
(or by a second optical beam of a longer wavelength). These two excitations<br />
work <strong>in</strong> oppos<strong>in</strong>g fashions: one fills (populates) the mid-gap traps whereas<br />
the other empties them. At steady state, when a focused beam illum<strong>in</strong>ates<br />
a biased crystal of this k<strong>in</strong>d, and the beam <strong>in</strong>tensity is such that the photoexcitation<br />
rate of one type of carrier is comparable to the thermal excitation<br />
rate of the other type of carrier, the concentration of both free carriers at<br />
the illum<strong>in</strong>ated region decrease drastically. The <strong>in</strong>tuitive explanation is as<br />
follows [86]. Under proper conditions, the ratio between the concentrations<br />
of electrons and holes is equal to their ratio <strong>in</strong> the absence of light, and thus<br />
has a constant (coord<strong>in</strong>ate-<strong>in</strong>dependent) value (see appendix of [17]). The<br />
net excitation rate of the traps is the difference between the thermal (holes)<br />
and optical (electrons) excitation rates. At resonance, the net excitation rate<br />
goes to zero. At the same time, at steady state the excitation rate must be<br />
equal to the recomb<strong>in</strong>ation rate, which, <strong>in</strong> turn, is proportional to the free<br />
charge concentration. Hence, at resonance (when the excitation rates of holes<br />
and electrons are comparable) the free charge concentration goes to zero.<br />
Consequently, the local electric field is highly enhanced because the current<br />
at steady state must rema<strong>in</strong> constant throughout the crystal. For a given<br />
temperature, this enhancement occurs at a specific <strong>in</strong>tensity (the resonance<br />
<strong>in</strong>tensity), for which the thermal and optical excitation rates are comparable.<br />
It is a resonant enhancement, although it is an <strong>in</strong>tensity-resonance and not an<br />
atomic resonance. The enhanced electric field compensates for the smallness<br />
of the electrooptic coefficient and enables a sufficiently large change <strong>in</strong> the<br />
refractive <strong>in</strong>dex to support narrow solitons.<br />
The observation of solitons <strong>in</strong> photorefractive semiconductors [[78, 35, 85]]<br />
is especially important for several reasons. First, the solitons are generated at<br />
optical telecommunications wavelengths. Second, they facilitate microsecond<br />
soliton formation times even at very low (microwatt) optical power. These<br />
suggest that optical spatial solitons could form from light beams emerg<strong>in</strong>g<br />
from ord<strong>in</strong>ary optical fibers (conventional data-transmission l<strong>in</strong>es) on<br />
nanoseconds time scales, and could be all-optically switched on-off by employ<strong>in</strong>g<br />
the <strong>in</strong>tensity resonance <strong>in</strong> photorefractive semiconductors.
24 E. DelRe, M. Segev, D. Christodoulides, B. Crosignani, and G. Salamo<br />
Fig. 17. Observed transverse <strong>in</strong>tensity distribution for (1+1)D self-trapp<strong>in</strong>g <strong>in</strong> InP,<br />
from [78].<br />
6.3 Diffusion-driven self-action<br />
In a conventional noncentrosymmetric crystall<strong>in</strong>e phase, such as that characteriz<strong>in</strong>g<br />
SBN or BaTiO3 at room temperature, charge diffusion leads to an<br />
asymmetric <strong>in</strong>dex profile, which translates <strong>in</strong>to a transverse phase chirp that<br />
produces self-bend<strong>in</strong>g. As discussed <strong>in</strong> section 3.1 <strong>in</strong> conjunction with Eq.(5),<br />
diffusion is typically merely a correction for screen<strong>in</strong>g soliton studies.<br />
Consider now a situation where no external field is applied. On the basis<br />
of Eq.(1) with g = 0 (null current), E = − kbT 1 dI<br />
q I+Ib dx . Higher order corrections<br />
due to saturation <strong>in</strong> this case are even less important, such that for a 10<br />
µm beam, they represent a relative import of the order of ɛr ·10−6 , where ɛr is<br />
the relative dielectric constant. For a sample heated above the ferroelectricparaelectric<br />
phase-transition, manifest<strong>in</strong>g a quadratic electro-optic response,<br />
the result<strong>in</strong>g nonl<strong>in</strong>earity leads to a symmetric lens<strong>in</strong>g effect, of the type<br />
1 dI<br />
∆n(I) ∝ ( I+Id dx )2 . Although <strong>in</strong> most conditions, such self-action is negligi-<br />
ble, <strong>in</strong> the very proximity of the phase-transition, where ɛr atta<strong>in</strong>s values of<br />
the order of 10 4 , self-focus<strong>in</strong>g, the precursor of soliton formation, has been<br />
observed [77, 87]. The result<strong>in</strong>g nonl<strong>in</strong>ear equation, which can be extended<br />
also to the full (2+1)D case, represents the s<strong>in</strong>gular situation <strong>in</strong> which a<br />
nonlocal nonl<strong>in</strong>earity (<strong>in</strong>volv<strong>in</strong>g a spatial derivative) allows for the explicit<br />
analytical prediction of both the observed nonl<strong>in</strong>ear diffraction, along with<br />
such novel effects as ellipticity recovery (see Fig.(18)), and the prediction of<br />
a full family of solitons, which, however, requir<strong>in</strong>g extremely pure samples<br />
and precise thermal conditions, and have not been observed.<br />
6.4 Fix<strong>in</strong>g the photorefractive soliton: Self-trapp<strong>in</strong>g by alter<strong>in</strong>g<br />
the crystall<strong>in</strong>e structure<br />
<strong>Solitons</strong> <strong>in</strong> photorefractives are typically supported by the l<strong>in</strong>ear polarization<br />
response to the local space-charge field, P = ɛE. However, optical beams can<br />
also self-trap <strong>in</strong> photorefractiue media by alter<strong>in</strong>g the crystall<strong>in</strong>e structure
<strong>Photorefractive</strong> <strong>Solitons</strong> 25<br />
Fig. 18. Diffusion-driven ellipticity recovery. The <strong>in</strong>put ellipticity (a) Λ is recovered<br />
at the output (b-e) as the crystal temperature T is brought closer to the Curie<br />
temperature, enhanc<strong>in</strong>g diffusion-driven effects, from [87].<br />
of the nonl<strong>in</strong>ear medium <strong>in</strong> which the beam propagates. This happens when<br />
the local space charge field E becomes comparable with the coercive field<br />
Ec, and is directed <strong>in</strong> a direction different from the pol<strong>in</strong>g direction. For<br />
low-modulation grat<strong>in</strong>gs, such conditions rarely emerge. But photorefractive<br />
solitons, be<strong>in</strong>g entities with an <strong>in</strong>herently high modulation depth, are always<br />
associated with locally high electric fields that can readily depolarize a sample.<br />
Consider a screen<strong>in</strong>g soliton, which exists as a consequence of an external<br />
bias E0 directed along the pol<strong>in</strong>g axis x. Once the soliton has formed, charge<br />
has redistributed so as to screen, at least <strong>in</strong> part, the field. This means that<br />
across the beam profile, charge distribution engenders a field that is approximately<br />
opposite the bias. Remov<strong>in</strong>g the illum<strong>in</strong>ation (and the background)<br />
and switch<strong>in</strong>g the external bias off unravels this field. The result is that<br />
EV =0 −E0 <strong>in</strong> the region that before hosted the soliton. In SBN Klotz et<br />
al. have shown how this field can, not only depolarize the sample, but actually<br />
permanently fix the waveguid<strong>in</strong>g structure that accompanies the soliton,<br />
an achievement that can have considerable impact <strong>in</strong> soliton based devices<br />
[80, 81].<br />
Fig. 19. Doma<strong>in</strong> and cluster structure <strong>in</strong>duced by a spontaneous self-trapped process<br />
<strong>in</strong> metastable KLTN, from [79]. (a-b) Underly<strong>in</strong>g doma<strong>in</strong> structure as seen<br />
with the two pr<strong>in</strong>cipal polarizations; (c-d) melt<strong>in</strong>g away of doma<strong>in</strong>s <strong>in</strong>to clusters,<br />
clusters <strong>in</strong>to a homogeneous structure, as temperature is <strong>in</strong>creased from the Curie<br />
po<strong>in</strong>t.
26 E. DelRe, M. Segev, D. Christodoulides, B. Crosignani, and G. Salamo<br />
Ferroelectric clusters can also play a more dynamic role <strong>in</strong> spatial selftrapp<strong>in</strong>g,<br />
when they <strong>in</strong>terplay with light-generated space-charge dur<strong>in</strong>g soliton<br />
formation. This has been observed <strong>in</strong> a metastable paraelectric, <strong>in</strong> proximity<br />
of the transition temperature, where charge-diffusion fields become<br />
comparable to Ec [79]. The result is a complicated optical-doma<strong>in</strong> dynamic<br />
which also leads, <strong>in</strong> appropriate conditions, to a form of spatial self-action<br />
known as spontaneous self-trapp<strong>in</strong>g (see Fig.(19)). The description of these<br />
processes, which requires the modell<strong>in</strong>g of doma<strong>in</strong> formation, and their lightmatter<br />
<strong>in</strong>teraction throughout propagation, is beyond the l<strong>in</strong>ear polarization<br />
approach. Such a theory has yet to be formulated. Nevertheless, the phenomenology<br />
seems to <strong>in</strong>dicate a more general behavior of propagation <strong>in</strong><br />
metastable hosts.<br />
7 Alternative photorefractive materials<br />
Research <strong>in</strong>to nonl<strong>in</strong>ear beam propagation <strong>in</strong> photorefractives is carried out,<br />
<strong>in</strong> parallel, <strong>in</strong> a series of relatively different materials, each present<strong>in</strong>g a<br />
slightly modified version of the ma<strong>in</strong>stream screen<strong>in</strong>g type nonl<strong>in</strong>earity, with<br />
its advantages and setbacks. Amongst these, we should mention the sillenites,<br />
such as BTO, BSO and BGO, paraelectrics, such as KLTN, and photorefractive<br />
polymers [88, 89] and organic gels [90].<br />
Some of the orig<strong>in</strong>al research <strong>in</strong> photorefractive self-trapp<strong>in</strong>g was carried out<br />
us<strong>in</strong>g nonferroelectric sillenites, <strong>in</strong> a configuration similar to that used for<br />
ferroelectric samples [16, 91, 92, 93]. The ma<strong>in</strong> difference between the physical<br />
processes is that sillenites present a fairly strong natural optical activity,<br />
which leads to polarization rotation (dur<strong>in</strong>g propagation) of both the selffocused<br />
and the background beams. This causes the effective nonl<strong>in</strong>earity to<br />
change <strong>in</strong> z. Strictly speak<strong>in</strong>g, solitons (diffraction-free) beams cannot exists<br />
<strong>in</strong> such optically-active materials [94, 95, 96], at least not <strong>in</strong> the typical<br />
scheme of screen<strong>in</strong>g solitons. However, us<strong>in</strong>g very short samples (a typical<br />
value of optical activity is ρ0 6 ◦ /mm), and employ<strong>in</strong>g pre-compensation<br />
(<strong>in</strong> which the beams are not extraord<strong>in</strong>arily- and ord<strong>in</strong>arily-polarized, but<br />
evolve to these halfway through the sample), does allow the observation of<br />
quasi-solitons. Another setback <strong>in</strong> us<strong>in</strong>g sillenite crystals is <strong>in</strong> the relatively<br />
weak effective electro-optic coefficient reff 0.06pm/V (for BTO), which<br />
implies the use of very high bias fields. Altogether, the sillenite crystals have<br />
served an important role <strong>in</strong> the first explorations of steady-state self-focus<strong>in</strong>g<br />
[16], but have been rarely used for solitons experiments s<strong>in</strong>ce then, simply<br />
because other materials offer more favorable conditions for soliton generation.<br />
Part of screen<strong>in</strong>g soliton studies are carried out <strong>in</strong> paraelectrics, where the<br />
quadratic electro-optic effect supports a screen<strong>in</strong>g nonl<strong>in</strong>earity <strong>in</strong> all similar to<br />
the noncentrosymmetric counterpart, of the form ∆n ∝ (E0) 2 /(1+I/Ib) 2 [97].<br />
In these, almost all the conventional photorefractive soliton phenomenology<br />
can be observed, from (1+1)D [33] to (2+1)D solitons [36]. Dark solitons have
<strong>Photorefractive</strong> <strong>Solitons</strong> 27<br />
yet to f<strong>in</strong>d an appropriate material, because <strong>in</strong> such crystals the nature of the<br />
<strong>in</strong>dex change cannot be reversed upon reversal of the applied field, as is the<br />
case for noncentrosymmetric crystals with the l<strong>in</strong>ear electrooptic effect. Given<br />
the generally weak electro-optic response <strong>in</strong> the high-symmetry phase, most<br />
studies are carried out <strong>in</strong> proximity of the ferroelectric-paraelectric transition:<br />
the crystals must be thermalized to stabilize their dielectric response.<br />
8 Soliton <strong>in</strong>teraction-collisions<br />
Nonl<strong>in</strong>earity generally allows the coupl<strong>in</strong>g and energy exchange among beams<br />
and modes. For solitons, nonl<strong>in</strong>earity not only supports their propagation<strong>in</strong>variant<br />
nature, but leads to a unique coupl<strong>in</strong>g dynamic <strong>in</strong> which the s<strong>in</strong>gle<br />
solitons behave as quasi-rigid particles when they are made to <strong>in</strong>teract with<br />
one another. In fact, this particle-like dynamic is the very reason for the<br />
term ”soliton”. In this spirit, <strong>in</strong>teractions between solitons are commonly<br />
referred to as soliton collisions, and constitute the most fasc<strong>in</strong>at<strong>in</strong>g features<br />
of soliton phenomena. Soliton <strong>in</strong>teractions can be generally classified<br />
<strong>in</strong>to coherent and <strong>in</strong>coherent <strong>in</strong>teractions. Coherent <strong>in</strong>teractions of solitons<br />
occur when the nonl<strong>in</strong>ear medium can respond to <strong>in</strong>terference effects<br />
that take place when the beams are overlapped. They occur for all nonl<strong>in</strong>earities<br />
with an <strong>in</strong>stantaneous (or extremely fast) time response (e.g., the<br />
optical Kerr effect and the quadratic nonl<strong>in</strong>earity). For all other nonl<strong>in</strong>earities<br />
that have a fairly long response time (e.g., photorefractive and thermal),<br />
the relative phase between the <strong>in</strong>teract<strong>in</strong>g beams must be kept stationary<br />
on a time scale much longer than the response time of the medium. When<br />
this occurs, the material responds to <strong>in</strong>terference between the overlapp<strong>in</strong>g<br />
beams and they exert on each other attractive or repulsive forces, depend<strong>in</strong>g<br />
on the relative phase between the beams. Incoherent <strong>in</strong>teractions, on<br />
the other hand, occur when the relative phase between the (soliton) beams<br />
varies much faster than the response time of the medium. In this case the<br />
resultant force between such bright solitons is always attractive. Altogether,<br />
soliton <strong>in</strong>teraction-collisions are universal, exhibit<strong>in</strong>g the same basic features<br />
<strong>in</strong> spite of the widely diverse physical orig<strong>in</strong>s for the self-trapp<strong>in</strong>g. For a<br />
detailed review on soliton <strong>in</strong>teraction forces, see [3].<br />
<strong>Photorefractive</strong> solitons play an especially important role <strong>in</strong> the study of<br />
soliton <strong>in</strong>teractions, and have here greatly contributed to soliton research at<br />
large. This lead<strong>in</strong>g role is a consequence of a series of factors: the relative<br />
ease <strong>in</strong> soliton generation, which lowers the complexity of multiple soliton<br />
support<strong>in</strong>g schemes; the saturable nature of the nonl<strong>in</strong>earity, which offers<br />
many features that are simply non-existent with ideal Kerr-type solitons; the<br />
availability of both (1+1)D and (2+1)D solitons, <strong>in</strong> a 3D bulk environment;<br />
and the relatively slow response of photorefractive materials which facilitates<br />
the possibility of study<strong>in</strong>g both coherent and <strong>in</strong>coherent collisions <strong>in</strong> the<br />
same material system. Over the past eight years, many groups have come
28 E. DelRe, M. Segev, D. Christodoulides, B. Crosignani, and G. Salamo<br />
to realize the wealth of possibilities offered by soliton <strong>in</strong>teraction studies <strong>in</strong><br />
photorefractives, and consequently many of the soliton collision features were<br />
first demonstrated with photorefractive solitons.<br />
The physical <strong>in</strong>tuition beh<strong>in</strong>d soliton collisions relies on the generic idea<br />
that a soliton is a bound state of its own <strong>in</strong>duced potential, or, <strong>in</strong> optics,<br />
a guided mode of its own <strong>in</strong>duced waveguide. Hav<strong>in</strong>g this <strong>in</strong> m<strong>in</strong>d, one can<br />
understand soliton collisions by compar<strong>in</strong>g the collision angle to the (complementary)<br />
critical angle for guidance <strong>in</strong> the s<strong>in</strong>gle soliton-<strong>in</strong>duced waveguides<br />
(that is, to the angle with the propagation axis below which total <strong>in</strong>ternal<br />
reflection occurs). Whether or not energy is coupled from one soliton <strong>in</strong>to the<br />
waveguide <strong>in</strong>duced by the other soliton, depends on the relation between the<br />
collision angle and that critical angle. In terms of a ”potential well”, capture<br />
depends on whether the k<strong>in</strong>etic energy of the collid<strong>in</strong>g wave-packets results<br />
<strong>in</strong> a velocity that is smaller than the escape velocity. If the collision occurs<br />
at an angle larger than the critical angle, the solitons simply go through each<br />
other unaffected - very similar to the behavior of Kerr solitons (the beams<br />
refract twice while go<strong>in</strong>g through each other’s <strong>in</strong>duced waveguide but cannot<br />
couple light <strong>in</strong>to it). If the collision occurs at ”shallow” angles, the beams<br />
can couple light <strong>in</strong>to each other’s <strong>in</strong>duced waveguide. Now if the waveguide<br />
can guide only a s<strong>in</strong>gle-mode (a s<strong>in</strong>gle bound state), the collision outcome<br />
will be elastic, essentially very similar to that of a similar collision <strong>in</strong> Kerr<br />
media (with the exception that now some very small fraction of the energy<br />
is lost to free radiation). However, if the waveguide can guide more than<br />
one mode, and if the collision is attractive, higher modes are excited <strong>in</strong> each<br />
waveguide and, <strong>in</strong> some cases, the waveguides merge and the solitons fuse to<br />
form one s<strong>in</strong>gle soliton beam. Such a fusion process is always followed by a<br />
small energy loss to radiation waves, much like <strong>in</strong>elastic collisions between<br />
real particles. This naive picture of soliton <strong>in</strong>teractions gives qualitative understand<strong>in</strong>g<br />
of the complex behavior of soliton collisions, yet it is <strong>in</strong>complete.<br />
In reality, the <strong>in</strong>teract<strong>in</strong>g solitons affect each other’s <strong>in</strong>duced waveguide, and<br />
the true collision process is much more complicated.<br />
The first experimental papers on collisions between photorefractive solitons<br />
were also the first papers report<strong>in</strong>g fusion of solitons <strong>in</strong> any medium<br />
[49, 98] (<strong>in</strong> parallel to a similar observation with solitons <strong>in</strong> atomic vapor,<br />
for which the nonl<strong>in</strong>earity is also saturable). These experiments reported<br />
on <strong>in</strong>coherent collisions, between (2+1)D [49] and between (1+1)D solitons<br />
[98], dur<strong>in</strong>g which at large collision angles the solitons passed through one<br />
another unaffected, whereas at shallow collision angles they fused to one another.<br />
Follow<strong>in</strong>g these experiments, a team headed by W. Krolikowski studied<br />
coherent collisions and demonstrated fission of solitons (”birth” and annihilation<br />
of solitons [50, 51], which also constitutes the first observation of such<br />
effects <strong>in</strong> any solitonic system. Other groups have followed and mapped out<br />
coherent <strong>in</strong>teractions between (1+1)D and (2+1)D solitons [99, 100]. All of<br />
these were collisions between solitons launched with trajectories <strong>in</strong> the same
<strong>Photorefractive</strong> <strong>Solitons</strong> 29<br />
plane. However, because the photorefractive nonl<strong>in</strong>earity is saturable, one<br />
can also look at collisions of (2+1)D solitons with trajectories that also do<br />
not lie <strong>in</strong> the same plane: full 3D <strong>in</strong>teractions. When non-parallel solitons<br />
with trajectories that do not lie <strong>in</strong> the same plane are launched simultaneously,<br />
they <strong>in</strong>teract (attract or repel each other) via the nonl<strong>in</strong>earity and<br />
their trajectories bend. The system possesses <strong>in</strong>itial angular momentum: if<br />
the soliton attraction exactly balances the ”centrifugal force” due to rotation,<br />
the solitons can ”capture” each other <strong>in</strong>to orbit and spiral about each<br />
other, much like two celestial objects or two mov<strong>in</strong>g charged particles. This<br />
idea was suggested <strong>in</strong> the context of coherent collisions. However, because coherent<br />
<strong>in</strong>teractions are critically sensitive to phase, <strong>in</strong> this case solitons can<br />
never atta<strong>in</strong> stable orbits, and spiral about each other. Instead, they always<br />
either fuse to form a s<strong>in</strong>gle beam, or ”escape away” from each other. On the<br />
other hand, the purely attractive nature of the force between <strong>in</strong>coherent solitons<br />
and its <strong>in</strong>dependence of the relative phase of the two <strong>in</strong>teract<strong>in</strong>g solitons<br />
makes these ideal for the orbit<strong>in</strong>g observation. Under proper <strong>in</strong>itial conditions<br />
of separation and beam trajectories, solitons <strong>in</strong>deed capture each other <strong>in</strong>to<br />
an elliptic orbit [48]. If the <strong>in</strong>itial distance between the solitons is <strong>in</strong>creased,<br />
their trajectories slightly bend toward each other, but their ”velocity” is<br />
larger than the escape velocity, and they do not form a ”bound pair”. On<br />
the other hand, if their separation is too small, they spiral on a ”converg<strong>in</strong>g<br />
orbit” and eventually fuse. In reality, the 3D spiral<strong>in</strong>g-<strong>in</strong>teraction mechanism<br />
is much richer and more complicated than <strong>in</strong>itially thought. It turns out that<br />
the two spiral<strong>in</strong>g-<strong>in</strong>teract<strong>in</strong>g solitons exchange energy by coupl<strong>in</strong>g light <strong>in</strong>to<br />
each other’s <strong>in</strong>duced waveguide. This is because the nonl<strong>in</strong>earity is saturable<br />
and the trajectories are at shallow angles. But, because the two <strong>in</strong>teract<strong>in</strong>g<br />
solitons have equal power, the energy exchange is symmetric. The energy exchanged<br />
is, of course, phase-coherent with its ”source” but phase <strong>in</strong>coherent<br />
with the soliton <strong>in</strong>to which it was coupled. Thus, even though the solitons<br />
are <strong>in</strong>itially <strong>in</strong>coherent with each other, the energy exchange <strong>in</strong>duces partial<br />
coherence and thus contributes to the forces <strong>in</strong>volved. The end result is that<br />
the two solitons orbit periodically about each other and at the same time<br />
exchange energy periodically, with the two periods (the spiral<strong>in</strong>g period and<br />
the energy exchange period) be<strong>in</strong>g only <strong>in</strong>directly related [101]. This complicated<br />
motion is stable over a wide range of parameters [101]. To some<br />
extent, whether or not the spiral<strong>in</strong>g can go on <strong>in</strong>def<strong>in</strong>itely is yet an open<br />
question, because it is possible that, after long enough propagation distances<br />
(far beyond the present experimental reach), the solitons eventually merge<br />
[102, 103]. Another <strong>in</strong>terest<strong>in</strong>g feature of spiral<strong>in</strong>g-<strong>in</strong>teract<strong>in</strong>g solitons is the<br />
fact that if one adds a t<strong>in</strong>y seed <strong>in</strong> one of the <strong>in</strong>put solitons that is coherent<br />
with the other soliton, the relative phase between these coherent components<br />
(the seed and the other soliton) controls the outcome of the collision process,<br />
and can turn a spiral<strong>in</strong>g motion <strong>in</strong>to fusion or repulsion [101]. Altogether,<br />
the observation of spiral<strong>in</strong>g-<strong>in</strong>teract<strong>in</strong>g solitons has <strong>in</strong>troduced new concepts
30 E. DelRe, M. Segev, D. Christodoulides, B. Crosignani, and G. Salamo<br />
to soliton physics: not only energy (power) and momentum are conserved,<br />
but also the conservation of angular momentum, which is the fundamental<br />
symmetry that enables spiral<strong>in</strong>g. These pioneer<strong>in</strong>g experiments are a characteristic<br />
example of the contribution of photorefractive solitons to nonl<strong>in</strong>ear<br />
science.<br />
Fig. 20. Collisions, from [49]. Top view of collid<strong>in</strong>g <strong>in</strong>coherent diffract<strong>in</strong>g beams<br />
and solitons for different relative angles.<br />
Fig. 21. Hybrid-soliton collisions, from [104]. (a) <strong>in</strong>put launch of a two-dimensional<br />
and a one-dimensional diffract<strong>in</strong>g beam, output <strong>in</strong>tensity distribution with no applied<br />
field, output <strong>in</strong>tensity distribution with applied self-trapp<strong>in</strong>g field; (b) same<br />
as (a) but for a smaller collision angle; (c-d) s<strong>in</strong>gle beam self-trapp<strong>in</strong>g <strong>in</strong> the same<br />
experimental conditions.<br />
It is <strong>in</strong>terest<strong>in</strong>g to compare soliton and plane-wave <strong>in</strong>teraction phenomenology<br />
<strong>in</strong> a photorefractive. The cross<strong>in</strong>g of two plane waves, even at low<br />
angles of the order of fractions of a degree, leads to energy transfer, which,<br />
even if mediated by space-charge components of the order of η, br<strong>in</strong>gs to<br />
f<strong>in</strong>ite if not total coupl<strong>in</strong>g from one beam to the other. Two solitons, on the<br />
other hand, behave <strong>in</strong> a diametrically opposite manner: they cross each other<br />
without appreciable energy transfer, even when they are mutually coherent.
<strong>Photorefractive</strong> <strong>Solitons</strong> 31<br />
Fig. 22. Soliton fusion, from [50]. Two identical solitons fuse at the output of the<br />
sample when they are <strong>in</strong>-phase (a), whereas they repel when they are out-of-phase<br />
(b).<br />
Fig. 23. Soliton spirall<strong>in</strong>g, from [48].(a) Beams A and B at the <strong>in</strong>put face of the<br />
crystal, (b) the spiral<strong>in</strong>g soliton pair after 6.5 mm of propagation, and (c) after<br />
13 mm of propagation. The centers of diffract<strong>in</strong>g A and B are marked by white<br />
triangles. The white cross <strong>in</strong>dicates the center of mass of the diffract<strong>in</strong>g beams A<br />
and B <strong>in</strong> (b) and (c).<br />
The conundrum has a straightforward geometrical explanation: even though<br />
no soliton mechanism forbids the formation of a resonant coupl<strong>in</strong>g grat<strong>in</strong>g <strong>in</strong><br />
the region where the two beams overlap, this overlap is spatially limited by<br />
the mutual angle θ <strong>in</strong> their propagation direction and their very narrow width<br />
∆x, which is typically no more than 20 wavelengths wide. Thus, <strong>in</strong> two-wavemix<strong>in</strong>g<br />
term<strong>in</strong>ology, even though the coupl<strong>in</strong>g coefficient γ can be reasonably<br />
high (e.g., at angles correspond<strong>in</strong>g to the Debye length), the equivalent energy<br />
transfer γL, where L is the effective <strong>in</strong>teraction distance <strong>in</strong> the sample, is<br />
negligible. Altogether, s<strong>in</strong>ce self-lens<strong>in</strong>g is a purely phase-modulat<strong>in</strong>g mechanism<br />
without energy coupl<strong>in</strong>g to new modes, soliton <strong>in</strong>teractions, even <strong>in</strong><br />
photorefractives (which could give rise to energy transfer driven by the diffusion<br />
field) is well described by means of soliton <strong>in</strong>teraction forces based<br />
on wave-overlap <strong>in</strong>tegrals, and the <strong>in</strong>tr<strong>in</strong>sic energy coupl<strong>in</strong>g mechanism that<br />
acts <strong>in</strong> two-wave-mix<strong>in</strong>g is absent.
32 E. DelRe, M. Segev, D. Christodoulides, B. Crosignani, and G. Salamo<br />
In the spirit of driv<strong>in</strong>g nonl<strong>in</strong>ear soliton studies to their most extreme consequences,<br />
photorefraction forwards a unique possibility of study<strong>in</strong>g hybridodimensional<br />
soliton collisions [104]. Namely, test<strong>in</strong>g to what extent a soliton<br />
undergoes particle-like dynamics even dur<strong>in</strong>g a collision between two solitons<br />
of different dimensionality. The possibility of carry<strong>in</strong>g out these studies arises<br />
from the saturable nature of the nonl<strong>in</strong>earity, which facilitates stable (2+1)D<br />
solitons, as well as the quasi-stable propagation of (1+1)D solitons <strong>in</strong> 3D bulk<br />
media. Strictly speak<strong>in</strong>g, the latter case is not stable <strong>in</strong> the absolute sense,<br />
and would, after a sufficiently large propagation distance, suffer from transverse<br />
<strong>in</strong>stabilities and dis<strong>in</strong>tegrate <strong>in</strong>to an array of 2D filaments. However,<br />
if the (1+1)D soliton is launched with parameters close enough to the soliton<br />
existence curve, and if its parameters are chosen such that the operation<br />
po<strong>in</strong>t is <strong>in</strong> the saturated regime, the ”<strong>in</strong>stability length” is very long, and for<br />
all practical purposes such a (1+1)D soliton propagates <strong>in</strong> a stable fashion<br />
<strong>in</strong> the bulk. These conditions have <strong>in</strong>deed allowed to experimentally observe<br />
the collision between a ”needle soliton” and a ”stripe soliton” [104], result<strong>in</strong>g<br />
<strong>in</strong> a new avenue <strong>in</strong> the <strong>in</strong>vestigation of particle-like behavior of solitons at<br />
large.<br />
A more recent series of studies targeted collisions of solitons propagat<strong>in</strong>g<br />
<strong>in</strong> opposite directions [105, 106, 107, 108]. The concept actually applies to<br />
any soliton-support<strong>in</strong>g system and <strong>in</strong>troduces a profoundly different scenario<br />
for <strong>in</strong>teract<strong>in</strong>g solitons [109]. Experimentally, thus far only <strong>in</strong>coherent collisions<br />
between such solitons have been studied [106, 108], whereas the more<br />
<strong>in</strong>terest<strong>in</strong>g case of coherent collisions [109, 107] is still unexplored [apart for<br />
the very specific case of a vector soliton formed by counter-propagat<strong>in</strong>g fields<br />
which has been recently demonstrated [110]; but this is not really a vector<br />
soliton, and not a soliton collision experiment]. In photorefractives, however,<br />
dur<strong>in</strong>g an almost head-to-head collision, the <strong>in</strong>teraction between the solitons<br />
occurs along a spatially extended region, hence spatially nonlocal effects, such<br />
as self-bend<strong>in</strong>g driven by diffusion fields, have an important impact on the<br />
collision dynamics. The experiments of [106, 108] show that the soliton collision<br />
dramatically modifies the self-bend<strong>in</strong>g of both solitons, <strong>in</strong> a way that<br />
can be directly utilized for all-optical beam deflection, steer<strong>in</strong>g and control.<br />
9 Vector and composite solitons<br />
In their most basic form, solitons are a coherent entity described by a s<strong>in</strong>gle<br />
optical wavefunction. The simplest (so-called scalar) soliton occurs when<br />
the soliton constitutes of a s<strong>in</strong>gle field, which populates the lowest mode of<br />
its own <strong>in</strong>duced-waveguide. A more complex soliton, a vector soliton, occurs<br />
when more than one field populates the lowest mode. These were first suggested<br />
by Manakov <strong>in</strong> Kerr media, when self- and cross-phase modulation<br />
are equal. Vector solitons, however, can be also composite: they can be composed<br />
of optical fields that populate different modes of their jo<strong>in</strong>tly <strong>in</strong>duced-
<strong>Photorefractive</strong> <strong>Solitons</strong> 33<br />
waveguide. In one realization, composite solitons are made of a bell-shaped<br />
(bright) component populat<strong>in</strong>g the lowest mode and a dark component be<strong>in</strong>g<br />
the second mode. A more <strong>in</strong>terest<strong>in</strong>g situation occurs when the field constituents<br />
of the composite-soliton populate different bound-modes of their<br />
jo<strong>in</strong>tly-<strong>in</strong>duced potential. These composite, multi-mode, solitons can have<br />
two or more <strong>in</strong>tensity humps, and can appear <strong>in</strong> (1+1)D and <strong>in</strong> (2+1)D, <strong>in</strong> a<br />
variety of <strong>in</strong>trigu<strong>in</strong>g comb<strong>in</strong>ations, <strong>in</strong>clud<strong>in</strong>g (2+1)D composite solitons carry<strong>in</strong>g<br />
angular momentum with<strong>in</strong> their field constituents. As will be expla<strong>in</strong>ed<br />
below, almost all the experiments with vector solitons, and practically all the<br />
experiments with multi-mode solitons, were carried out <strong>in</strong> photorefractives.<br />
A key issue regard<strong>in</strong>g a vector soliton is that <strong>in</strong>terference terms between<br />
the soliton constituents should not contribute to the nonl<strong>in</strong>ear <strong>in</strong>dex change<br />
(otherwise the <strong>in</strong>duced potential would vary periodically dur<strong>in</strong>g propagation).<br />
Thus, the field constituents mak<strong>in</strong>g up a vector soliton could orig<strong>in</strong>ate from<br />
orthogonal polarizations states, or from fields at widely-spaced frequencies.<br />
In the polarization-based technique, there are no <strong>in</strong>terference terms, whereas<br />
<strong>in</strong> the widely spaced frequencies method, the <strong>in</strong>terference terms are not synchronized<br />
with either of the soliton constituents. <strong>Photorefractive</strong>s, however,<br />
have offered a much more appeal<strong>in</strong>g technique to generate vector solitons:<br />
mak<strong>in</strong>g up a vector soliton from field constituents that are <strong>in</strong>coherent with<br />
one another, that is, their relative phases are randomly fluctuat<strong>in</strong>g. When the<br />
relative phase between the fields mak<strong>in</strong>g up the soliton fluctuates much faster<br />
than the response time of the nonl<strong>in</strong>earity, their contribution to <strong>in</strong>terference<br />
terms averages out to zero. This method, suggested by Christodoulides [111],<br />
has revolutionized the area of vector solitons. With this mutual <strong>in</strong>coherence<br />
method, first a degenerate (Manakov-like) soliton was observed [112], the<br />
same year that the first Manakov-type solitons were observed <strong>in</strong> Kerr media.<br />
This was followed by an observation of a vector soliton made up of a bright<br />
and a dark component [113]. Shortly thereafter, the first multi-mode/multihump<br />
solitons were observed [114]. In this multi-mode soliton experiment,<br />
the two <strong>in</strong>put field distributions resembled the first and/or second and third<br />
modes of a slab waveguide. Interest<strong>in</strong>gly, the experiment has also shown that<br />
it is possible to observe multi-mode solitons made up of solely higher modes<br />
(the second plus the third modes, trapped <strong>in</strong> their jo<strong>in</strong>tly-<strong>in</strong>duced potential<br />
[114]). That is, the experiment has <strong>in</strong>dicated that multi-mode solitons can<br />
exist and propagate <strong>in</strong> a stable fashion for distances much larger than the<br />
diffraction length, <strong>in</strong> spite of the fact they are made up of excited states only.<br />
Several years later, (2+1)D dipole-type composite solitons were also demonstrated<br />
experimentally [39, 41]. These vector solitons consist of a bell-shaped<br />
component jo<strong>in</strong>tly trapped with a 2D dipole mode. The ability to generate<br />
(2+1)D composite solitons opens up a whole new range of possibilities that<br />
has no counterpart <strong>in</strong> a lower dimensionality. One fasc<strong>in</strong>at<strong>in</strong>g example is the<br />
recently observed rotat<strong>in</strong>g ”propeller” soliton [40]. This is a composite soliton<br />
made of a rotat<strong>in</strong>g dipole component jo<strong>in</strong>tly trapped with a bell-shaped
34 E. DelRe, M. Segev, D. Christodoulides, B. Crosignani, and G. Salamo<br />
component. It carries and conserves angular momentum, although its constituents<br />
exchange angular momentum as they propagate. The soliton turns<br />
out to be generically robust, so much that even dur<strong>in</strong>g <strong>in</strong>elastic collisions<br />
with other composite solitons, the collision products are predicted to be also<br />
composite rotat<strong>in</strong>g propeller solitons [115].<br />
The relatively ease with which vector and composite solitons are generated<br />
<strong>in</strong> photorefractives, by employ<strong>in</strong>g the mutual <strong>in</strong>coherence technique,<br />
has also led to a series of experimental efforts demonstrat<strong>in</strong>g <strong>in</strong>teractioncollisions<br />
between vector solitons. It turns out that temporal optical vector<br />
solitons, and non-optical vector solitons are very difficult to generate, hence<br />
the collision experiments with optical spatial vector soliton were truly pioneer<strong>in</strong>g.<br />
For example, it has been predicted, more than two decades ago, that<br />
collisions between Manakov-like vector solitons give rise to a symmetric exchange<br />
of energy between the soliton constituents. This elegant phenomenon<br />
was observed only recently, with photorefractive vector (Manakov-like) solitons<br />
[116, 117]. The energy-exchanges between the soliton components (which<br />
have noth<strong>in</strong>g to do with photorefractive two-wave-mix<strong>in</strong>g) have direct implications<br />
<strong>in</strong> a new form of reversible comput<strong>in</strong>g, <strong>in</strong> which a ”state” is coded<br />
as the ratio between the soliton components [118]. In this scheme, computation<br />
is performed through the energy-exchange <strong>in</strong>teractions (<strong>in</strong> which the<br />
”states” change) dur<strong>in</strong>g collisions between vector solitons. The experiments<br />
have shown that <strong>in</strong>deed, not only such symmetric energy exchanges do occur,<br />
but also <strong>in</strong>formation can be transferred through a series of cascaded collisions<br />
between vector solitons [116, 117].<br />
F<strong>in</strong>ally, photorefractives were also the means for experimental studies<br />
of <strong>in</strong>teraction-collisions between multi-mode solitons, <strong>in</strong> which shape transformations<br />
were observed [119]. These were the first ever experiments with<br />
collisions of multi-mode solitons.<br />
The general ideas beh<strong>in</strong>d multi-component vector solitons proved <strong>in</strong>valuable<br />
for later developments and <strong>in</strong> particular to the area of <strong>in</strong>coherent solitons<br />
discussed <strong>in</strong> the next section.<br />
10 Incoherent solitons: self-trapp<strong>in</strong>g of<br />
weakly-correlated wavepackets<br />
Until 1996, the commonly held belief was that all soliton structures should be<br />
<strong>in</strong>herently coherent entities. In that year however, an experiment carried out<br />
at Pr<strong>in</strong>ceton demonstrated beyond doubt that self-trapp<strong>in</strong>g of a partially<br />
spatially-<strong>in</strong>coherent light beam [42] is <strong>in</strong> fact possible, if the nonl<strong>in</strong>earity<br />
has a non-<strong>in</strong>stantaneous temporal response. In that experiment, the optical<br />
beam was quasi-monochromatic, but partially spatially-<strong>in</strong>coherent and the<br />
nonl<strong>in</strong>ear medium was photorefractive, with a response much slower than<br />
the characteristic time of the phase fluctuations <strong>in</strong> the <strong>in</strong>coherent beam. The<br />
resultant self-trapped beam is now commonly referred to as an ”<strong>in</strong>coherent
<strong>Photorefractive</strong> <strong>Solitons</strong> 35<br />
Fig. 24. The observation of a multimode soliton, from [114],with mode 2/mode 1 =<br />
1.0 (a),(b) <strong>in</strong>put (18 µm FWHM) and l<strong>in</strong>ear diffraction (27 µm) of mode 1; (c),(d)<br />
<strong>in</strong>put (28 µm) and l<strong>in</strong>ear diffraction (62 µm) of mode 2; (e),(f) comb<strong>in</strong>ed <strong>in</strong>put<br />
(26 µm) and comb<strong>in</strong>ed l<strong>in</strong>ear diffraction (58 µm); (g) composite soliton formed (26<br />
µm) with application of 800 V/4 mm; (h) first mode obta<strong>in</strong>ed after quickly block<strong>in</strong>g<br />
second mode; (i) steady state of first mode alone with nonl<strong>in</strong>earity on; (j) second<br />
mode obta<strong>in</strong>ed after quickly block<strong>in</strong>g first mode; and (k) steady state of second<br />
mode alone with nonl<strong>in</strong>earity on.<br />
soliton” or a ”random-phase soliton”. One year later, the same group observed<br />
a similar self-trapp<strong>in</strong>g effect with white light from an <strong>in</strong>candescent light bulb<br />
emitt<strong>in</strong>g light with a wide 380-720 nm spectrum of wavelengths. This was the<br />
first observation of a self-trapped beam made of light both temporally and<br />
spatially <strong>in</strong>coherent: a white light soliton [43]. These two experiments have<br />
set the basis for a new field of study <strong>in</strong> nonl<strong>in</strong>ear optics: <strong>in</strong>coherent solitons.<br />
In yet another experiment, self-trapp<strong>in</strong>g of dark <strong>in</strong>coherent ”beams”, i.e., 1D<br />
or 2D ”voids” nested <strong>in</strong> a spatially <strong>in</strong>coherent beam, was also demonstrated<br />
[47].<br />
For self-trapp<strong>in</strong>g of an <strong>in</strong>coherent beam (an <strong>in</strong>coherent soliton) to occur,<br />
several conditions must be satisfied. First, the nonl<strong>in</strong>earity must be non<strong>in</strong>stantaneous<br />
with a response time that is much longer than the phase fluctuation<br />
time across the optical beam. Such a nonl<strong>in</strong>earity responds to the<br />
time-averaged envelope and not to the <strong>in</strong>stantaneous ”speckles” that constitute<br />
the <strong>in</strong>coherent field. Second, the multi-mode (speckled) beam should<br />
be able to <strong>in</strong>duce, via the nonl<strong>in</strong>earity, a multi-mode waveguide. Otherwise,
36 E. DelRe, M. Segev, D. Christodoulides, B. Crosignani, and G. Salamo<br />
if the <strong>in</strong>duced waveguide is able to support only a s<strong>in</strong>gle guided mode, the<br />
<strong>in</strong>coherent beam will simply undergo spatial filter<strong>in</strong>g, thus radiat<strong>in</strong>g all of its<br />
power but the small fraction that co<strong>in</strong>cides with that guided mode. Third, as<br />
with all solitons, self-trapp<strong>in</strong>g requires self-consistency: the multi-mode beam<br />
must be able to guide itself <strong>in</strong> its own <strong>in</strong>duced waveguide (pages 86-125 <strong>in</strong><br />
Ref.[4]).<br />
The understand<strong>in</strong>g of how such an <strong>in</strong>coherent soliton can form also raises<br />
some <strong>in</strong>trigu<strong>in</strong>g aspects <strong>in</strong> comparison to other nonl<strong>in</strong>ear phenomena. Conventional<br />
nonl<strong>in</strong>ear optical effects are a consequence of strong material response<br />
to (<strong>in</strong>tense) optical excitation, but their macroscopic manifestation is<br />
generally the result of distributed enhancement effects, <strong>in</strong> which weak scatter<strong>in</strong>g<br />
is amplified by the cooperative excitation of large portions of material.<br />
This is the basis, for example, for efficient harmonic generation and wavemix<strong>in</strong>g.<br />
The distributed effect is <strong>in</strong>duced by an extended spatial and temporal<br />
coherence, itself transferred by the coherence of the coupl<strong>in</strong>g waves.<br />
The discovery of <strong>in</strong>coherent solitons has made evident the basic fact that<br />
solitons naturally break this scheme. Even though they do result from nonl<strong>in</strong>earity,<br />
their nature has noth<strong>in</strong>g to do with the constructive <strong>in</strong>terference of<br />
distributed effects. On the contrary, it is an <strong>in</strong>tr<strong>in</strong>sically local effect where<br />
no coherence transfer mechanism <strong>in</strong>tervenes. Thus, for the more diverse nonoptical<br />
media that support solitons, the very concept of wave is an abstract<br />
average envelope of <strong>in</strong>tr<strong>in</strong>sically uncorrelated underly<strong>in</strong>g motion, that atta<strong>in</strong>s<br />
physical mean<strong>in</strong>g when the wave-medium <strong>in</strong>teraction does not react to the<br />
erratic fluctuations of the wave constituent.<br />
The experiments demonstrat<strong>in</strong>g <strong>in</strong>coherent solitons have taken the solitons<br />
community by surprise, because typically, <strong>in</strong> most of soliton research<br />
(also beyond Optics), all experiments were preceded by a theory predict<strong>in</strong>g<br />
the ma<strong>in</strong> effects. The experiments demonstrated beyond doubt that <strong>in</strong>coherent<br />
solitons <strong>in</strong>deed exist. Yet, at the time, someth<strong>in</strong>g quite important was<br />
still miss<strong>in</strong>g: a theory! Unlike the case of coherent solitons, where the evolution<br />
equation can be straightforwardly derived by add<strong>in</strong>g the nonl<strong>in</strong>earity<br />
to the paraxial equation of diffraction, the description of <strong>in</strong>coherent solitons<br />
was far from be<strong>in</strong>g clear. The experiments were of course based on <strong>in</strong>sight<br />
and <strong>in</strong>tuition, but then aga<strong>in</strong> they gave only few clues, if any, as to how one<br />
could develop a theory. Only one th<strong>in</strong>g was certa<strong>in</strong> - the theory of <strong>in</strong>coherent<br />
solitons had to be derived from first pr<strong>in</strong>ciples. With<strong>in</strong> a year, two different<br />
theories were developed to describe <strong>in</strong>coherent solitons: the coherent density<br />
theory [120] and the modal theory [121]. The coherent density theory is, by its<br />
very nature, a dynamic approach that is better suited to study the evolution<br />
dynamics of <strong>in</strong>coherent solitons, their <strong>in</strong>teractions, <strong>in</strong>stabilities etc, as they<br />
occur <strong>in</strong> experimental set-ups. In this formalism, the <strong>in</strong>coherent field is described<br />
by means of an auxiliary non-observable function from where one can<br />
deduce the optical <strong>in</strong>tensity as well as the associated correlation statistics.<br />
The modal theory, on the other hand, by virtue of its <strong>in</strong>herent simplicity be-
<strong>Photorefractive</strong> <strong>Solitons</strong> 37<br />
came the method of choice <strong>in</strong> terms of identify<strong>in</strong>g <strong>in</strong>coherent solitons, their<br />
range of existence and correlation properties. One year later, yet another<br />
theory was proposed: the theory describ<strong>in</strong>g the propagation of the mutual<br />
coherence [122]. Interest<strong>in</strong>gly enough, even though at first sight these three<br />
theoretical approaches seem to be dissimilar, they are <strong>in</strong> fact formally equivalent<br />
to one another [123]. All describe quasi-monochromatic yet partially<br />
spatially <strong>in</strong>coherent solitons: they expla<strong>in</strong> the behavior of such entities, provide<br />
their statistical properties, and predict their behavior as they <strong>in</strong>teract<br />
with one another. As such, they became a very powerful analytical and numerical<br />
tool. More recently, these theories were expanded to describe white<br />
light solitons: solitons that are made of temporally and spatially <strong>in</strong>coherent<br />
light [124, 125].<br />
The pioneer<strong>in</strong>g experiments of Refs.[42, 43, 47] that were the first to<br />
show the unexpected fact that random-phase solitons can exist with both<br />
spatial and temporal <strong>in</strong>coherence, opened the way for several other important<br />
results. These <strong>in</strong>clude for example, anti-dark <strong>in</strong>coherent states [126],<br />
elliptic <strong>in</strong>coherent solitons [127, 128], coherence control us<strong>in</strong>g <strong>in</strong>teractions<br />
of <strong>in</strong>coherent solitons [129, 130], and more. Especially noteworthy are the<br />
fundamental studies on modulation <strong>in</strong>stability of <strong>in</strong>coherent waves and spontaneous<br />
pattern formation <strong>in</strong> weakly correlated system. It has been found,<br />
theoretically and experimentally, that such weakly correlated systems <strong>in</strong>deed<br />
exhibit modulation <strong>in</strong>stability, and a uniform (homogeneous) partially <strong>in</strong>coherent<br />
wavefront breaks up <strong>in</strong>to an array of soliton-like filaments. However,<br />
for this to occur the nonl<strong>in</strong>earity needs to exceed a threshold value determ<strong>in</strong>ed<br />
by the coherence properties of the waves [131, 132, 133, 134, 135, 136]. This<br />
fact stands <strong>in</strong> sharp contradist<strong>in</strong>ction with coherent systems, for which there<br />
is no such threshold for modulation <strong>in</strong>stability (<strong>in</strong> a coherent self-focus<strong>in</strong>g<br />
system, a uniform wave always breaks up <strong>in</strong>to an array of soliton-like structures).<br />
Once this threshold is exceeded, the partially <strong>in</strong>coherent uniform wave<br />
breaks up <strong>in</strong>to an array of localized structures, each behav<strong>in</strong>g as an <strong>in</strong>coherent<br />
soliton. These solitonic ”breakup products” <strong>in</strong>teract with one another<br />
<strong>in</strong> an <strong>in</strong>coherent fashion, exert<strong>in</strong>g long-range attraction on each other. After<br />
sufficiently large propagation distance, they aggregate and form clusters<br />
of f<strong>in</strong>e-scale structures, leav<strong>in</strong>g large voids between adjacent soliton clusters<br />
(aggregates of solitons) [137, 138]. More recent work along these ve<strong>in</strong>s is the<br />
prediction of modulation <strong>in</strong>stability of white light [139], along with its very<br />
recent experimental observation [140], and the work on <strong>in</strong>coherent pattern<br />
formation <strong>in</strong> cavities [141, 142, 143, 144].<br />
Studies on <strong>in</strong>coherent solitons and <strong>in</strong>coherent pattern formation have established<br />
that these are not some k<strong>in</strong>d of esoteric creatures, specific to photorefractives,<br />
but are <strong>in</strong> fact a general and rich new class of solitons, whose<br />
existence is relevant to many other diverse fields beyond nonl<strong>in</strong>ear optics. For<br />
example, <strong>in</strong>coherent modulation <strong>in</strong>stability effects, soliton cluster<strong>in</strong>g and <strong>in</strong>coherent<br />
pattern formation, relate to many systems <strong>in</strong> nature: from cluster<strong>in</strong>g
38 E. DelRe, M. Segev, D. Christodoulides, B. Crosignani, and G. Salamo<br />
<strong>in</strong> a cooled atomic gas to self-supported ”stripes” of electrons <strong>in</strong> semiconductors,<br />
as well as to gravitational-like effects. In fact, the underly<strong>in</strong>g physics<br />
relates to any weakly-correlated wave-system hav<strong>in</strong>g a non-<strong>in</strong>stantaneous<br />
nonl<strong>in</strong>earity. Altogether, it is fair to say that <strong>in</strong>coherent solitons are most<br />
probably the s<strong>in</strong>gle most important discovery made with self-trapp<strong>in</strong>g effect<br />
<strong>in</strong> photorefractive systems. It has <strong>in</strong>troduced a new concept <strong>in</strong>to soliton research,<br />
and has many implications beyond optics, <strong>in</strong>to other arenas where<br />
random phase waves and nonl<strong>in</strong>earities coexist.<br />
11 Applications<br />
11.1 Passive devices<br />
The most basic functionality afforded by a soliton <strong>in</strong> any physical system,<br />
is the transfer of a localized energy/<strong>in</strong>formation bear<strong>in</strong>g wave perturbation<br />
along an otherwise dispersive propagation. For an optical spatial soliton,<br />
this translates <strong>in</strong>to the fact that far-field effects are absent, and the spatial<br />
resolution, its phase curvature and coherence properties, and the transverse<br />
distribution of energy, rema<strong>in</strong> unaltered: a guided propagation <strong>in</strong> an otherwise<br />
bulk and homogeneous medium, the guide itself be<strong>in</strong>g <strong>in</strong>duced by the modes<br />
it supports.<br />
For photorefractive solitons, the composite nonl<strong>in</strong>earity that <strong>in</strong>tervenes<br />
allows for a series of useful attributes. For one, a photorefractive soliton<br />
can passively guide a second beam of longer wavelength, on consequence of<br />
the fact that whereas self-trapp<strong>in</strong>g is a product of nonl<strong>in</strong>earity, the <strong>in</strong>dexmodulat<strong>in</strong>g<br />
system is only weakly wavelength dependent, and will act on an<br />
<strong>in</strong>frared beam <strong>in</strong> much the same manner that it acts on the soliton [145, 146,<br />
147, 148, 149, 150, 151]. Not be<strong>in</strong>g of nonl<strong>in</strong>ear orig<strong>in</strong>, this phenomenon does<br />
not depend on the <strong>in</strong>tensity of the guided signal, and, <strong>in</strong> the measure <strong>in</strong> which<br />
the deposited charge displacement which accompanies the soliton does not<br />
redistributed, does not even require the presence of the visible nonl<strong>in</strong>ear wave.<br />
This property can be used to <strong>in</strong>tegrate a material <strong>in</strong>to a fiber or waveguide<br />
device without the development of a crystal-specific technique to grow or<br />
tailor a waveguide, the sample itself serv<strong>in</strong>g either as an electro-optic phasetransducer,<br />
the waveguide not be<strong>in</strong>g greatly modified by the application of<br />
an arbitrary bias for l<strong>in</strong>ear electro-optic response, or simply as redirect<strong>in</strong>g<br />
component.<br />
Passive waveguid<strong>in</strong>g gives us the opportunity of differentiat<strong>in</strong>g between a<br />
nonl<strong>in</strong>ear and a l<strong>in</strong>ear behavior. Consider, for example, a dark soliton, which<br />
consists of a nondiffract<strong>in</strong>g <strong>in</strong>tensity notch engendered by a π phase jump.<br />
In the very same conditions that lead to its formation, it can passively guide<br />
a bright longer wavelength mode, even though such a photoactive mode (at<br />
the shorter wavelength) could never self-trap <strong>in</strong> the same conditions.
<strong>Photorefractive</strong> <strong>Solitons</strong> 39<br />
Evidently, more complicated passive devices can be demonstrated, such<br />
as reconfigurable directional couplers based on two bright solitons formed<br />
<strong>in</strong> close proximity, Y-junctions, along with more complex multisoliton structures<br />
and hybrid soliton-fabricated-waveguides systems [152, 153, 154, 155,<br />
156, 157, 158]. Moreover, <strong>in</strong> conditions <strong>in</strong> which charge redistribution cannot<br />
be avoided, a considerable advantage can be obta<strong>in</strong>ed by implement<strong>in</strong>g the<br />
ferroelectric fix<strong>in</strong>g of the rout<strong>in</strong>g device [159].<br />
11.2 Active devices<br />
A second functionality is based on the fact that photorefractives offer alloptical<br />
functionality even at low <strong>in</strong>tensities, even though this is burdened by<br />
slow time response [160, 161, 162, 163, 164, 165]. For example, logic operations<br />
can be carried out simply by hav<strong>in</strong>g two solitons <strong>in</strong>teract, or by modulat<strong>in</strong>g<br />
two different components of a s<strong>in</strong>gle vector soliton. We might note that a<br />
truly all-optical soliton device must imply a partial absorbtion, and this does<br />
not generally spouse implementation. A slightly less ambitious alternative is<br />
to use the all-optical operation to steer non photoactive signals.<br />
A second form of active device is that for which soliton dynamics are<br />
controlled externally by means of a modulation <strong>in</strong> the support<strong>in</strong>g physical<br />
parameters. Thus for example, the output direction of propagation can be<br />
changed by chang<strong>in</strong>g the bias voltage, as a consequence of self-bend<strong>in</strong>g [21].<br />
Once aga<strong>in</strong>, whereas the signal can be delivered <strong>in</strong> a fast capacity-limited<br />
regime, the optical response will be dom<strong>in</strong>ated by the photorefractive time<br />
constants.<br />
11.3 Electro-optic manipulation<br />
Passive electro-optic effects have been <strong>in</strong>vestigated for soliton-deposited<br />
space-charge <strong>in</strong> paraelectric samples [166]. This allows the fast capacitylimited<br />
manipulation of optical circuitry through the sole electro-optic effect,<br />
much <strong>in</strong> the same manner as electro-holographic technology.<br />
In order to grasp the phenomenon, note that <strong>in</strong> a l<strong>in</strong>ear electro-optic<br />
response, once a soliton has been formed through a self-trapp<strong>in</strong>g ∆ns, the<br />
application of an arbitrary control external bias <strong>in</strong> comb<strong>in</strong>ation with E0 leads<br />
to a ∆n(Econ) ∝ (E + Econ), which simply changes the constant pedestal on<br />
which the soliton guid<strong>in</strong>g pattern <strong>in</strong>duced by E is embedded. This means, for<br />
example, that passive guid<strong>in</strong>g can be achieved also for a zero applied external<br />
field. For a paraelectric, which is characterized by a quadratic response,<br />
∆n(Econ) ∝ (E + Econ) 2 = E 2 +2EEcon + E 2 con. The second mixed term allows<br />
for an electro-optic distortion of the pattern, which, not imply<strong>in</strong>g charge<br />
redistribution, is a purely spatially resolved electro-response. This has allowed<br />
the demonstration of a series of beam manipulation devices, culm<strong>in</strong>at<strong>in</strong>g <strong>in</strong><br />
a two-needle switch<strong>in</strong>g device [167] (see Fig.25).
40 E. DelRe, M. Segev, D. Christodoulides, B. Crosignani, and G. Salamo<br />
11.4 Nonl<strong>in</strong>ear frequency conversion <strong>in</strong> waveguides <strong>in</strong>duced by<br />
photorefractive solitons<br />
The most promis<strong>in</strong>g application of waveguides <strong>in</strong>duced by photorefractive<br />
solitons is nonl<strong>in</strong>ear frequency conversion. The conversion efficiency <strong>in</strong> χ 2<br />
processes is proportional to the <strong>in</strong>tensity of the pump beam, so it is desirable<br />
to work with very narrow beams. One easy way to achieve that is to<br />
use a focused pump beam. However, <strong>in</strong> a bulk crystal, the more focused a<br />
beam is, the faster it diffracts, and diffraction limits the frequency conversion<br />
efficiency because as the <strong>in</strong>teract<strong>in</strong>g beams diffract, (1) their <strong>in</strong>tensities<br />
decrease, and (2) the phase-match<strong>in</strong>g condition cannot be satisfied across<br />
their entire cross section. Therefore, us<strong>in</strong>g waveguides for frequency conversion<br />
can greatly improve the conversion efficiency. But thus far it has been<br />
difficult to fabricate waveguides from most materials that allow for phase<br />
match<strong>in</strong>g, and two-dimensional waveguides are especially difficult to make.<br />
Now, (2+1)D photorefractive solitons <strong>in</strong>duce 2D waveguides, and almost all<br />
photorefractives are highly efficient <strong>in</strong> χ 2 frequency conversion. In waveguides,<br />
phase-match<strong>in</strong>g should take place among the propagation constants<br />
of the guided modes, and is typically obta<strong>in</strong>ed through birefr<strong>in</strong>gence or periodic<br />
pol<strong>in</strong>g. In a fabricated waveguide, however, the structure is fixed, so<br />
tun<strong>in</strong>g techniques rely on vary<strong>in</strong>g the temperature, or on lateral translation<br />
<strong>in</strong> structures with several periods of pol<strong>in</strong>g parallel to one other. But waveguides<br />
<strong>in</strong>duced by photorefractive solitons offer much flexibility because their<br />
waveguide structure and propagation axis (with respect to the crystall<strong>in</strong>e<br />
axes) can be modified at will and <strong>in</strong> real time. Work<strong>in</strong>g with photorefractive<br />
solitons, one can achieve wavelength tunability while avoid<strong>in</strong>g diffraction by<br />
simply rotat<strong>in</strong>g the crystal and launch<strong>in</strong>g a soliton <strong>in</strong> the new direction. One<br />
can also f<strong>in</strong>e-tune the frequency conversion process by chang<strong>in</strong>g the propagation<br />
constants of the guided modes through vary<strong>in</strong>g the <strong>in</strong>tensity ratio and<br />
external voltage, allow<strong>in</strong>g tun<strong>in</strong>g with no mechanical movements.<br />
The first step <strong>in</strong> the direction of nonl<strong>in</strong>ear frequency conversion <strong>in</strong> waveguides<br />
<strong>in</strong>duced by photorefractive solitons was the demonstration of efficient<br />
second-harmonic generation [168, 169, 170]. The experiment have shown that<br />
the conversion efficiency can be considerably <strong>in</strong>creased [168], and high tunability<br />
can be obta<strong>in</strong>ed by rotat<strong>in</strong>g the crystal [169]. However, a much more<br />
important scenario occurs <strong>in</strong> a soliton-based optical parametric oscillator<br />
(OPO). In an OPO, the threshold pump power is dependent on the signal<br />
ga<strong>in</strong> per pass through the crystal. To lower the threshold, one has to <strong>in</strong>crease<br />
the signal ga<strong>in</strong> per pass. A waveguide that conf<strong>in</strong>es the pump beam<br />
as well as the signal and idler <strong>in</strong> a small area is one very effective way to<br />
achieve this. Consider a Gaussian beam at the pump frequency launched<br />
<strong>in</strong>to a nonl<strong>in</strong>ear crystal and assume that phase match<strong>in</strong>g is satisfied at the<br />
waist, located at the <strong>in</strong>put surface. The threshold pump power is proportional<br />
to [z0 arctan 2 (L/z0)+ln 2 (1 + L 2 /z 2 0)/4] −1 , where z0 is the Rayleigh<br />
(diffraction) length of the beam and L is the crystal length. For a given L,
<strong>Photorefractive</strong> <strong>Solitons</strong> 41<br />
there exists an optimum beam size for m<strong>in</strong>imum threshold pump power, when<br />
z0 = L/2.84. However, if a waveguide is used to keep all beams at the same<br />
widths throughout propagation <strong>in</strong> the crystal, the threshold is simply proportional<br />
to z0/L 2 , which cont<strong>in</strong>ues to decrease as we focus the beam more.<br />
The m<strong>in</strong>imum threshold is determ<strong>in</strong>ed by the smallest size of the waveguide<br />
that can be made. To estimate the improvement, consider a focused Gaussian<br />
beam with a m<strong>in</strong>imum beam waist of 21 mm and a 15 mm long crystal. An<br />
OPO constructed <strong>in</strong> a waveguide has a threshold pump power 60 percent<br />
lower than that of an OPO with the same beam waist <strong>in</strong> bulk. Therefore,<br />
<strong>in</strong> a waveguide OPO the signal ga<strong>in</strong> per pass can be considerably improved,<br />
and the threshold pump power can be substantially lowered for the same cavity<br />
loss. This generic idea was recently demonstrated with a doubly-resonant<br />
optical parametric oscillator <strong>in</strong> a waveguide <strong>in</strong>duced by a photorefractive soliton<br />
[171]. The OPO threshold was considerably lowered by construct<strong>in</strong>g it<br />
with<strong>in</strong> a soliton-<strong>in</strong>duced waveguide. This technique should work even better<br />
with s<strong>in</strong>gly resonant OPOs and it can substantially reduce the threshold<br />
pump power when very narrow solitons are employed. For example, us<strong>in</strong>g a<br />
soliton beam with a beam waist of 8 mm and a 15 mm long crystal, the OPO<br />
threshold pump could be reduced to only 3.5 percent of that for an OPO <strong>in</strong><br />
the same nonl<strong>in</strong>ear medium, us<strong>in</strong>g the same mirrors but without the soliton.<br />
Fig. 25. Electro-optic switch<strong>in</strong>g, from [167]<br />
12 New frontiers <strong>in</strong> photorefractive solitons and<br />
conclud<strong>in</strong>g remarks<br />
As we hope transpires from the brief review, there is still much to be understood<br />
as to the mechanisms underly<strong>in</strong>g spatial photorefractive self-trapp<strong>in</strong>g,<br />
from the formation of 2+1D solitons to quasi-steady-state solitons, from dark<br />
<strong>in</strong>coherent solitons to spontaneous self-trapp<strong>in</strong>g. The field, however, is <strong>in</strong><br />
constant expansion, and we cannot refra<strong>in</strong> from mention<strong>in</strong>g the important
42 E. DelRe, M. Segev, D. Christodoulides, B. Crosignani, and G. Salamo<br />
Fig. 26. Second harmonic generation <strong>in</strong> photorefractive solitons, from [168].<br />
Fig. 27. Second harmonic conversion efficiency <strong>in</strong>crease mediated by spatial solitons,<br />
from [168]<br />
achievements <strong>in</strong> the field of soliton lattices and discrete soliton observation<br />
obta<strong>in</strong>ed <strong>in</strong> photorefractive SBN [172, 173, 174, 175, 176, 177], and <strong>in</strong> the<br />
trapp<strong>in</strong>g of more exotic excitations such as r<strong>in</strong>gs [178].<br />
Although we have attempted to give a detailed account of all aspects<br />
of photorefractive self-trapp<strong>in</strong>g, the field has undergone such a rapid and<br />
extensive evolution that we can hardly guarantee that all contributions have<br />
been cited and described. Perhaps this is yet another accomplishment of<br />
photorefraction, that is, hav<strong>in</strong>g given to the soliton science community a<br />
powerful and accessible tool with which to further its research and develop<br />
new and possibly useful scientific and practical tools.<br />
13 Dedication<br />
Moti Segev would like to dedicate this <strong>Chapter</strong> to his friend Galit Staier, who<br />
was critically wounded <strong>in</strong> the murderous Palest<strong>in</strong>ian suicide attack on October<br />
4, 2003, <strong>in</strong> the Maxim restaurant <strong>in</strong> Haifa, Israel. In that suicide bomb a<br />
Palest<strong>in</strong>ian woman blew herself up kill<strong>in</strong>g 21 civilians. Galit has has lost her<br />
11-year old son Assaf Staier, her father Ze’ev Almog (71), her mother Ruth
<strong>Photorefractive</strong> <strong>Solitons</strong> 43<br />
Almog (70), her brother Moshe (43), and his son Tomer Almog (9). Moshe’s<br />
other son, Oran Almog (11), was critically wounded, while Moshe’s wife, Orly<br />
Almog, and their daughter Adi Almog (4), were moderately wounded as well.<br />
Galit and the survivors of the Staier-Almog family are now slowly recover<strong>in</strong>g.<br />
We all hope that Galit will fully recover soon, for her husband (Moti’s friend)<br />
Ofer Staier, for their son Omri, and for her family and friends.<br />
The Authors jo<strong>in</strong> <strong>in</strong> express<strong>in</strong>g the hope that the sacrifice of the Staier-<br />
Almog family lighten the way to a real peace, free of horrible actions aga<strong>in</strong>st<br />
humanity, such as suicide bomb<strong>in</strong>gs.<br />
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