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Nonlinear Optical Probes and Processes in Polymers and Liquid ...

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26<br />

−2ik2∇E20 + k 2 0F ∗ E10 = 0<br />

Express<strong>in</strong>g the wave vectors k1 <strong>and</strong> k2 <strong>in</strong> coord<strong>in</strong>ates as k1 = k(ˆz cos θ + ˆx s<strong>in</strong> θ),<br />

√ √<br />

k2 = k(ˆz cos θ − ˆx s<strong>in</strong> θ) where k = k0 ε0 (= 2π ε0 /λ), we rewrite the Eqs. 2.14 <strong>in</strong><br />

the form<br />

∂E10<br />

∂z<br />

F k0<br />

+ i<br />

2 √ ε0 cos θ E20 = 0 (2.15)<br />

∂E20<br />

∂z + i F ∗ k0<br />

2 √ ε 0 cos θ E10 = 0<br />

Here we recall that F ∼ Esc,max. The amplitude of space charge field Esc,max depends<br />

on the depth of the <strong>in</strong>tensity modulation<br />

as [5]<br />

m =<br />

2E10E ∗ 20<br />

|E10| 2 + |E20| 2<br />

Esc,max = mEw<br />

(2.16)<br />

(2.17)<br />

where Ew is the part of the space charge field that does not depend on the <strong>in</strong>tensity<br />

of the <strong>in</strong>cident beams. Substitution of Eqs. 2.16, 2.17 <strong>and</strong> Eq. 2.10 <strong>in</strong>to Eqs. 2.15<br />

yields<br />

∂E10<br />

∂z − <strong>in</strong>3 reEwk0<br />

2 cos θ<br />

∂E20<br />

∂z − <strong>in</strong>3 reEwk0<br />

2 cos θ<br />

|E20| 2E10 |E10| 2 = 0<br />

+ |E20|<br />

2<br />

|E10| 2E20 |E10| 2 = 0<br />

+ |E20|<br />

2<br />

(2.18)

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