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MO P1-27.pdf - University of Maryland

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Controlled Porosity Reservoir Cathodes and Photocathodes<br />

R. Lawrence Ives a , Eric Montgomery b , Blake Riddick b , Zhigang Pan b ,<br />

Lou Falce a David Marsden a , George Collins a<br />

a Calabazas Creek Research, San Mateo, CA 94404 USA<br />

b <strong>University</strong> <strong>of</strong> <strong>Maryland</strong>, College Park, 20742 MD USA<br />

Abstract—Research is continuing to develop controlled<br />

porosity reservoir cathodes and photocathodes. Advances in<br />

design tools and fabrication techniques will be presented as well<br />

as available test results for thermionic cathodes and<br />

photocathodes.<br />

I. INTRODUCTION AND BACKGROUND<br />

HE development <strong>of</strong> material with a uniform array <strong>of</strong><br />

Tmicron scale pores is providing new opportunities for<br />

improved cathodes and photocathodes. Reservoir cathodes<br />

provide significantly greater lifetime than can be achieved<br />

with traditional impregnated cathodes. The tungsten material<br />

with uniform, user-defined porosity provides the reservoir cap<br />

whose structure controls the rate at which work function<br />

reducing material diffuses to the emission surface. The<br />

uniformity <strong>of</strong> the pore array ensures unprecedented uniformity<br />

<strong>of</strong> electron emission.<br />

The significance <strong>of</strong> this development for thermionic<br />

cathodes was recognized with a 2011 R&D 100 award [1].<br />

Research clearly demonstrated the potential for dramatically<br />

improved thermionic cathodes [2]. Research is continuing to<br />

extend the applicability <strong>of</strong> controlled porosity reservoir (CPR)<br />

technology using segmented cathodes and improved design<br />

and fabrication processes.<br />

The potential for photocathodes was demonstrated by recent<br />

experiments at the <strong>University</strong> <strong>of</strong> <strong>Maryland</strong>, where the lifetime<br />

<strong>of</strong> cesiated tungsten photocathodes was increased by more<br />

than two orders <strong>of</strong> magnitude [3]. Photocathode lifetime is a<br />

major issue for electron guns using laser initiated electron<br />

emission. This presentation will describe recent research on<br />

CPR cathodes and photocathodes.<br />

demonstrating the concept and confirming emission<br />

performance and lifetime. More recent research focused on<br />

improving both the design tools and the fabrication<br />

procedures.<br />

CPRCd is a free computer design tool that calculates emitter<br />

and reservoir specifications to achieve a desired emission<br />

current density and lifetime. It calculates Knudsen Flow<br />

through the emitter material at the temperature required for the<br />

specified emission current density.<br />

Figure 1. Sintered wire material for cathode emitters<br />

Research also focused on improving the fabrication and<br />

brazing <strong>of</strong> the emitter material and new assembly processed<br />

for very small cathodes as well as larger cathodes for<br />

magnetron injection guns (MIGs) and high power klystrons.<br />

Current research is focused on developing new electron guns<br />

for advanced electron beam devices.<br />

II. FABRICATION<br />

CPR cathodes utilize a uniform porosity tungsten emitter<br />

over a reservoir <strong>of</strong> work function reducing material [4]. For<br />

thermionic cathodes, this is usually barium calcium aluminate.<br />

For photocathodes, this is typically cesium chromate -<br />

titanium. The emitter material is created by winding 20 micron<br />

diameter tungsten wire around a molybdenum form and<br />

sintering to bond the wires. The material is then sliced<br />

perpendicular to the grain to form the cathode emitters. Figure<br />

1 shows a microphotograph <strong>of</strong> an emission surface.<br />

The cathodes are formed by sealing a reservoir <strong>of</strong> barium or<br />

cesium at one end with the cathode/photocathode emitter and<br />

the other end with a heater. A schematic diagram is shown in<br />

Figure 2.<br />

Initial research utilized thermionic cathodes designed for<br />

traditional Life Test Vehicles. This research focused on<br />

Figure 2. Schematic <strong>of</strong> controller porosity reservoir<br />

cathode<br />

III. CATHODES AND PHOTOCATHODES<br />

Fabrication <strong>of</strong> both a magnetron injection gun (MIG)<br />

cathode and high power gridded cathodes is in progress. The<br />

MIG cathode will be implemented in a 28 GHz gyrotron at<br />

Karlesruhe Institute <strong>of</strong> Technology, and the high power<br />

klystron cathode is targeted for a 5 MW, X-Band klystron.<br />

CCR recently completed a 15-beam electron gun for an X-<br />

Band klystron. The cathodes operate with an emission current


density <strong>of</strong> 31 A/cm 2 and eliminate requirements for beam<br />

compression. This dramatically simplified the gun design and<br />

improved the beam quality. The estimated lifetime exceeds<br />

90,000 hours.<br />

Figure 3. Photograph <strong>of</strong> 15-beam electron gun with CPR<br />

cathodes operating at 30 A/cm 2<br />

Figure 4 shows a solid model <strong>of</strong> the segmented MIG being<br />

built for KIT. The gun will be used to study the effects <strong>of</strong> nonuniform<br />

cathode emission on<br />

gyrotron performance. The<br />

current emitted from each<br />

segment will be externally<br />

controlled.<br />

Photocathode research is<br />

focused on extending the<br />

reservoir concept to<br />

photocathode materials with<br />

higher quantum efficiency.<br />

The Figure 6 shows current Figure 4. Solid model <strong>of</strong><br />

performance <strong>of</strong> photocathodes,<br />

including the recent advance<br />

for cesiated tungsten. CPR<br />

segmented MIG using CPR<br />

cathodes<br />

photocathodes use a modified version <strong>of</strong> the configuration<br />

shown in Figure 2. Because <strong>of</strong> the increased volatility <strong>of</strong><br />

cesium, the reservoir is capped by a section <strong>of</strong> sintered<br />

tungsten powder. This is followed by a mixing section and<br />

controlled porosity material for uniform cesium distribution<br />

over the surface. The unique feature <strong>of</strong> this configuration is<br />

that the cesium diffusion can be precisely controlled to match<br />

the surface evaporation rate.<br />

Current research is investigating evaporative and atomic<br />

layer deposition to deposit higher quantum efficiency<br />

materials onto the CPR tungsten material. Experiments will<br />

measure both the quantum efficiency <strong>of</strong> the photocathodes and<br />

the evaporation rate <strong>of</strong> cesium. This will allow estimation <strong>of</strong><br />

the lifetime. The goal is to increase the lifetime <strong>of</strong> high<br />

quantum efficiency materials by two orders <strong>of</strong> magnitude or<br />

more.<br />

Cathode and photocathode designs will be describes as well<br />

as available experimental results.<br />

Figure 6. Quantum efficiency and lifetime for common<br />

photocathode materials. Some cathodes have longer<br />

reported lifetimes under high vacuum, so the graph is<br />

normalized to a nanoTorr, assuming contaminationlimited<br />

lifetime scales linearly with chamber pressure.<br />

Figure 5. CPR configuration for cesiated photocathodes<br />

IV. SUMMARY<br />

CPR cathodes provide increased performance for both<br />

thermionic and photocathodes. This will lead to improved<br />

electron guns for electron beam devices<br />

V. ACKNOWLEDGEMENTS<br />

This research was supported by U.S. Department <strong>of</strong> Energy<br />

grants Nos. DE-FG02-04ER83918, DE-SC0006208, DE-<br />

SC0004570, and DE-SC0009583, and by the U.S. Army<br />

Research Office under contract W911NF-08C-0051 as part <strong>of</strong><br />

the DARPA HiFIVE program.<br />

REFERENCES<br />

[1] “Controlled porosity elevates performance, lifetime <strong>of</strong> cathodes,” R&D<br />

Magazine, Vol. 53, No. 5, September 2011.<br />

[2] R. Lawrence Ives, Senior Member, IEEE, Louis R. Falce, George<br />

Miram, George Collins, “Controlled Porosity Cathodes for High Current<br />

Density Applications,” IEEE Trans. Plasma Sci., Special Edition on<br />

High Power Microwave Sources, Vol. 38, No. 6, pp. 1345-1353, June<br />

2010.<br />

[3] Eric Montgomery, et al, “Enhanced Lifetime Hybrid-Diffuser Cesium<br />

Reservoir Photocathode,” Advanced Accelerator Concepts Workshop,<br />

Austin, TX June 2012.<br />

[4] R.L. Ives, L.R. Falce, S. Schwartzkopf, and R. Witherspoon, “Controlled<br />

Porosity Cathodes from Sintered Tungsten Wires, IEEE Trans. On<br />

Electron Devices, Vol. 52, No. 12, pp. 2800-2805, December 2005.

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