Natural-Product Humic Acid - Laub BioChem
Natural-Product Humic Acid - Laub BioChem
Natural-Product Humic Acid - Laub BioChem
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HUMIC ACIDNATURAL AND SYNTHETIC:BIBLIOGRAPHY AND REFERENCES<strong>Laub</strong> <strong>BioChem</strong>icals Corporation1401 Quail St., Suite 121Newport Beach, CA 92660Supplement V2005 – 2007
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TABLE OF CONTENTSReviews and Monographs ............................................. 1<strong>Natural</strong>-<strong>Product</strong> <strong>Humic</strong> <strong>Acid</strong> .................................... 6Isolation and Preparation Procedures ................................................. 42Synthetic <strong>Humic</strong> <strong>Acid</strong> ....................................................... 76Chemical Synthesis .............................................................................. 76Enzymatic Synthesis ............................................................................ 77Physicochemical Properties andCharacterization .................................................................... 78<strong>Acid</strong>-Base Properties ............................................................................ 79Adsorption ..................................................................................... 81Aliphatic Content .................................................................................. 82Aromaticity ........................................................................................... 82Ash Content ..................................................................................... 82Atomic Absorption Spectroscopy (AAS) ............................................... 83Atomic Force Microscopy ...................................................................... 83Bleaching ..................................................................................... 83Bromate Reduction ............................................................................... 84Bromination ..................................................................................... 84Capillary Electrophoresis (CE) ............................................................ 84Capillary Electrophoresis-Gel Permeation Chromatography(CE-GPC) ..................................................................................... 85Capillary Electrophoresis-Inductively Coupled Plasma Spectroscopy-MassSpectrometry (CE-ICP-MS) ................................. 85Carbon Content ..................................................................................... 86Carboxyl Content .................................................................................. 87Chemiluminescence .............................................................................. 87Chronostratigraphy .............................................................................. 87Color ..................................................................................................... 88Complexation ........................................................................................ 88with Metals ...................................................................................... 99Critical Micelle Concentration (CMC) ................................................. 134Crosslinking .......................................................................................... 134Decolorization ....................................................................................... 134Degradation .......................................................................................... 134Density .................................................................................................. 135-iii-
Derivatization ....................................................................................... 135Dialysis .................................................................................................. 137Differential Scanning Calorimetry (DSC) ........................................... 137Differential Thermal Analysis (DTA) .................................................. 138Differential Thermogravimetric Analysis (DTG) ................................ 139Diffusion Coefficients ........................................................................... 139Electron Paramagnetic Resonance Spectroscopy (EPR) ..................... 139Electron Spectroscopy for Chemical Analysis (ESCA) ........................ 140Electron Spin Resonance Spectroscopy (ESR) ..................................... 141Elemental Composition ........................................................................ 141Field-Flow Fractionation (FFF) ........................................................... 147Field-Flow Fractionation–Mass Spectrometry (FFF-MS) ................... 148Flocculation ..................................................................................... 148Flow Injection Analysis (FIA) .............................................................. 148Fluorescence Spectroscopy ................................................................... 148Fractionation ......................................................................................... 156Fulvic Content ..................................................................................... 166Functional Group Analysis ................................................................... 167Gas Chromatography (GC) ................................................................... 168Gas Chromatography-Mass Spectrometry (GC-MS) ........................... 169Gel-Permeation Chromatography (GPC) ............................................. 171Gel-Permeation Chromatography–Inductively Coupled PlasmaSpectroscopy-Mass Spectrometry (GPC-ICP-MS) ....................... 177Gel-Permeation Chromatography-Mass Spectrometry (GPC-MS) ..... 177Gel-Permeation Chromatography–Polyacrylamide Gel Electrophoresis(GPC-PAGE) .................................................................. 177High-Performance Liquid Chromatography (HPLC) .......................... 177High-Performance Liquid Chromatography–Mass Spectrometry(HPLC-MS) .................................................................................. 179Hydrophobicity ..................................................................................... 180Hygroscopicity ..................................................................................... 180Immobilization ..................................................................................... 180Inductively-Coupled Plasma Spectroscopy-Mass Spectrometry(ICP-MS) ..................................................................................... 182Infrared Spectroscopy (IR) ................................................................... 183Iodination ..................................................................................... 193Iodine Content ..................................................................................... 193Ion Exchange Chromatography ........................................................... 193Isotopic Composition ............................................................................. 194Light Scattering .................................................................................... 194Lipid Content ........................................................................................ 195-iv-
Luminescence Spectroscopy ................................................................. 195Luminescence Microscopy .................................................................... 195Luminescence Spectroscopy ................................................................. 196Lyophilization ....................................................................................... 196Mass Spectrometry (MS) ...................................................................... 196Molecular Weight .................................................................................. 199Monosaccharide Content ...................................................................... 204Neutron Activation Analysis (NAA) ..................................................... 204Neutron Scattering ............................................................................... 205Nitration ................................................................................................ 205Nitrogen Content .................................................................................. 205Nuclear Magnetic Resonance Spectroscopy (NMR) ............................ 206Optical Properties ................................................................................. 215Oxidation ............................................................................................... 215Ozonation .............................................................................................. 216Phenol Content ..................................................................................... 217Phosphorus Content ............................................................................. 217Photoelectron Spectroscopy (PES) ....................................................... 218Photolysis ............................................................................................... 218Polyacrylamide Gel Electrophoresis (PAGE) ...................................... 219Potentiometry ....................................................................................... 219Proton Affinity ...................................................................................... 222Pyrolysis ................................................................................................ 222Radiolabeling ........................................................................................ 223Radiolysis .............................................................................................. 223Raman Spectroscopy ............................................................................. 223Reactivity .............................................................................................. 224Redox Properties ................................................................................... 224Refractive Index .................................................................................... 224Scanning Electron Microscopy (SEM) .................................................. 225Silication ............................................................................................... 225Singlet Oxygen Quenching ................................................................... 226Solid Phase Extraction (SPE) ............................................................... 226Spectral Characteristics ....................................................................... 226Structure and Morphology .................................................................... 226Models ........................................................................................... 235of Solutions ...................................................................................... 235Sulfate Content ..................................................................................... 237Sulfur Content ...................................................................................... 237Surface Tension, of Solutions ............................................................... 237-v-
Surfactant ........................................................................................... 237Thermal Stability .................................................................................. 238Thermogravimetric Analysis (TGA) ..................................................... 238Thermolysis ........................................................................................... 240Thermomechanical Analysis (TMA) ..................................................... 241Thin-Layer Chromatography (TLC) ..................................................... 242Transmission Electron Microscopy (TEM) .......................................... 242Transmission X-Ray Microscopy (TXM) .............................................. 242Ultrafiltration ....................................................................................... 243Ultrasonication ..................................................................................... 244Ultraviolet-Visible Spectroscopy (UV-Vis) ........................................... 244Viscometry ............................................................................................ 250Voltammetry ......................................................................................... 251Water Uptake ........................................................................................ 252X-ray Diffraction ................................................................................... 253X-ray Photoelectron Spectroscopy (XPES) ........................................... 254X-ray Scattering .................................................................................... 254X-ray Spectroscopy ............................................................................... 255Zeta Potential ........................................................................................ 257Physiology and Physiological Effects .............. 258Toxicology .............................................................................................. 263Commercial Applications .............................................. 264Activated Carbon Manufacture ............................................................ 265Adhesive Manufacture .......................................................................... 265Adobe Glaze Manufacture .................................................................... 265Agriculture ........................................................................................... 265Bactericide ..................................................................................... 266Fertilizer ..................................................................................... 267Fungicide ..................................................................................... 294Herbicide ..................................................................................... 294Insecticide ..................................................................................... 295Pesticide ..................................................................................... 295Plant Growth Stimulant ................................................................. 296Plant Protectant .............................................................................. 301Panting Mat ..................................................................................... 303Seed Coating/Treatment ................................................................. 304Soil Amendment .............................................................................. 306Air Purification ..................................................................................... 314Algicide ................................................................................................ 314-vi-
Alumina Processing .............................................................................. 315Ammonium Phosphate Processing ....................................................... 315Animal Feed Additive ........................................................................... 315Antiscaling/Corrosion Inhibition .......................................................... 318Aquaculture ..................................................................................... 319Ash/Water Slurries ............................................................................... 320Bactericide ............................................................................................ 321Battery Manufacture ............................................................................ 321Beverage Additive ................................................................................. 323Binder ................................................................................................ 323Coal Briquettes ................................................................................ 324Iron Ore Pellets ............................................................................... 324Wood Pellets .................................................................................... 325Biocide ................................................................................................... 325Bone China Manufacture ..................................................................... 325Brick Manufacture ................................................................................ 325Brick Glaze Additive ............................................................................. 325Calcium Carbonate Processing ............................................................ 326Capacitor Manufacture ......................................................................... 326Catalyst Component ............................................................................. 326Cement/Concrete Manufacture ............................................................ 327Coloring Agent ................................................................................. 327Ceramics Manufacture ......................................................................... 327Clay Processing ..................................................................................... 328Clay/Water Slurries .............................................................................. 329Coal Processing ..................................................................................... 329Coal/Water Slurries .............................................................................. 329Coke Manufacture ................................................................................ 330Construction/Building Materials ......................................................... 330Copy Toner ............................................................................................ 331Cosmetics Additive ............................................................................... 331Culture Medium Additive ..................................................................... 332Deodorizing Agent ................................................................................ 332Gases ................................................................................................ 332Desulfurization ..................................................................................... 332Diaper Manufacture ............................................................................. 332Drilling Mud Additive .......................................................................... 333Dye Applications ................................................................................... 334Electrode Fabrication ........................................................................... 335Fabrics Manufacture ............................................................................ 335-vii-
Firebrick Manufacture ......................................................................... 335Food <strong>Product</strong>s Additive ........................................................................ 336Fungicide................................................................................................ 336Gypsum Manufacture............................................................................ 336Hair Growth Stimulation ...................................................................... 336Heat Transfer Medium ......................................................................... 336HPLC Substrate..................................................................................... 336Ink Manufacture ................................................................................... 336Ion Exchange Manufacture .................................................................. 337Iron Alloy Manufacture ........................................................................ 337Iron Ore Processing .............................................................................. 337Lip Balm ................................................................................................ 337Microbicide ............................................................................................ 337Oil Absorption ....................................................................................... 337Oil <strong>Product</strong>ion/Processing .................................................................... 338Ointment Manufacture ......................................................................... 338Oral Hygiene <strong>Product</strong>s ......................................................................... 338Oxygen Scavenging ............................................................................... 338Paint Manufacture ................................................................................ 338Polymer Manufacture ........................................................................... 338Porcelain Manufacture ......................................................................... 339Radiation Protection ............................................................................. 339Semiconductor Manufacture ................................................................ 339Skin Care .............................................................................................. 339Sludge Stabilization .............................................................................. 339Soap Manufacture ................................................................................. 340Soil Remediation ................................................................................... 340Surfactant Manufacture ....................................................................... 343Textile Manufacture ............................................................................. 343Printing ............................................................................................ 344Tile Manufacture .................................................................................. 344Tin Ore Processing ................................................................................ 344Veterinary Medicine ............................................................................. 345Waste Gas Treatment ........................................................................... 345Wastewater Treatment ......................................................................... 345Water Purification ................................................................................ 349Water Sealant ....................................................................................... 350Therapeutic Applications ............................................. 351Anaphylactic Shock .............................................................................. 353Anti-Bacterial Agent ............................................................................. 353-viii-
Anti-Cancer Agent ................................................................................ 353Anti-Infective Agent ............................................................................. 354Anti-Inflammatory Properties .............................................................. 354Anti-Microbial Properties ..................................................................... 355Anti-Pyretic Agent ................................................................................ 355Anti-Viral Efficacy ................................................................................ 355AIDS ................................................................................................. 356Cowpox Virus ................................................................................... 356Herpes Viruses ................................................................................ 356Vaccinia Virus ................................................................................. 356Bleeding Disorders ................................................................................ 356Drug Delivery ........................................................................................ 357Drug Synergy ........................................................................................ 357Folk Medicine ........................................................................................ 357Gout ....................................................................................................... 357Heart Disease ........................................................................................ 358Immunostimulation .............................................................................. 358Irritable Bowel Syndrome .................................................................... 358Osteoporosis .......................................................................................... 358Rheumatoid Disease ............................................................................. 359Mud Baths ..................................................................................... 359Therapeutic Textile Manufacture ........................................................ 359Wound Healing ..................................................................................... 359Author Index ............................................................................... 360-ix-
HUMATE MATERIALS<strong>Natural</strong> and Synthetic:Bibliography and ReferencesSupplement V
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(5918) Y. Chen. High-energy maintenance-free sealed lead-acid storagebattery for submarines. CN 1,652,384 (August 10, 2005).(5919) Y. Chen. High-energy maintenance-free sealed lead-acid electricbattery for submarines. CN 1,652,385 (August 10, 2005).(5920) Y. Chen. High-energy maintenance-free sealed lead-acid electricbattery for submarines. CN 1,652,386 (August 10, 2005).(5921) Y. Chen. High-energy maintenance-free sealed lead-acidelectric battery for miner lamp. CN 1,652,388 (August 10,2005).(5922) Y. Chen. Cathode plate structure of high-energy sealed leadacidstorage battery for submarine. CN 1,677,727 (October 5,2005).(5923) P.-a. Zhang, Y.-b. Sui, P. Wang, and J.-p. Ma. Study oncadmium-free alloy for electric bike batteries. Xudianchi 2006,160, 116-117, 121.(5924) M. Zhou and X. Liu. Process for fabricating colloid electrode oflead-acid storage battery. CN 1,758,464 (April 12, 2006).(5925) K. Nishimura. Polyether-type polymer composition, cathodefilm, their manufacture, and lithium secondary batteries. JP2006/156,255 (June 15, 2006).(5926) K. Nishimura. Polyether-type polymer composition, cathodefilm, and lithium battery. JP 2006/156,256 (June 15, 2006).(5927) J. Li, G. Cao, and L. Wang. Lead plaster as negative pole ofvalve-controlled sealed lead-acid storage battery for startingautomobile. CN 1,747,205 (March 15, 2006).(5928) C. Dai, D. Wang. X. Hu, Z. Jiang, L. Gao, and T. Yi. Method forfabricating spirally wound lead-acid battery with foamed-leadnegative plate grid. CN 1,790,796 (June 21, 2006).(5929) X.-f. Zhang, D.-f. Xing, and J.-s. Wu. Discussion onimplementation of some revised technical requirements of drycharged-startingability and cold-starting capacity of lead-acidstorage battery in new standard GB/T 5008.1.2.3-2005.Xudiachi 2006, 159, 82-86.(5930) Y. Chen. High-energy maintenance-free secondary lead-acidbattery for light on miner’s helmet. CN 1,933,231 (March 21,2007).(5931) Y. Chen. High-energy hermetically-sealed lead-acid electricbattery used in naval ships. CN 1,933,220 (March 21, 2007).(5932) Y. Chen. Anode active mass composite for high-energy sealedmaintenance-free secondary lead-acid battery of rail engine. CN1,933,217 (March 21, 2007).-322-
(5933) C. Zhao and C. Wu. Lead paste for cathode of lead-acid storagebattery of motorcycle, and its preparation method. CN101,071,855 (November 14, 2007).(5934) G. Feng. Electrode plates and electrolyte of lead storage batteryfor electric bicycle. CN 1,967,912 (May 23, 2007).(5935) Y. Chen. High-energy totally-sealed secondary lead-acid batteryfor starting helicopters. CN 1,960,041 (May 9, 2007).(5936) Y. Dai, C. Ju, K. Sun, and Z. Wang. Anode additive for negativeelectrode of mini-type sealed secondary lead-acid battery. CN1,964,108 (May 16, 2007).(5937) Y. Chen. High-energy hermetically-sealed secondary lead-acidbattery for starting battle planes and bombing planes. CN1,949,566 (April 18, 2007).(5938) Y. Chen. High-energy hermetically-sealed secondary lead-acidbattery for starting tank. CN 1,949,565 (April 18, 2007).(5939) Y. Chen. High-energy sealed lead-acid battery used in electricvehicle. CN 101,060,174 (October 24, 2007).(5940) K.-s. Tai, G.-m. Du, and L.-h. Zhang. Effect of water loss duringoperation on cycle life of lead-acid batteries for electric bicycles.Xudiachi 2007, 163, 71-74.(5941) D.-y. Qian, Z.-h. Deng, Z.-a. Wang, G. Zhu, F.-g. Xu, and H.-t.Liu. Deep-cycling performance of valve regulated lead acidbatteries for electric bicycles. Dianchi Gongye 2007, 12(3), 154-157.(5942) J. Li, G. Lai, H. Huang, X. Xia, J. Xue, and D. Li. Preparation ofhigh density ultrafine composite lithium iron phosphate ascathode material for lithium ion batteries. CN 1,907,844(February 7, 2007).(5943) Y. Song, J. Luo, and X. Huang. Gel storage battery forelectromobile. CN 1,905,264 (January 31, 2007).(5944) K. Xue, X. Lin, M. Zhang, J. Xiao and Y. Yu. Improved pastemixing process for lead-acid battery of electric bicycle. CN1,971,977 (May 30, 2007).Beverage Additive(5945) N. Liu and J. Wang. Health beverage containing humic acidand the application of humic acid in beverage. CN 1,568,827(January 26, 2005).Binder(5950) R. Chen, J. Mou, P. He, and F. Gan. Chrome-free MgO-ZrO 2 -SiO 2 based refractory material for RH vacuum furnace liner.CN 1,715,246 (January 4, 2006).-323-
Coal Briquettes(5946) M. Wang. Manufacture of briquette. CN 1,563,295(January 12, 2005).(5947) G. Chen. Method for preparing multifunctionaladditive for clean gas-production briquette. CN1,710,034 (December 21, 2005).(5948) H. Liu and A. Zhong. Clean modified coal briquetsand their production. CN 1,629,260 (June 22, 2005).(5949) I. F. Savchenko and A. P. Sorokin. <strong>Product</strong>ion of fuelbriquets from low-calorific high-moisture coals. RU2,252,948 (May 27, 2005).(5950) R. Chen, J. Mou, P. He, and F. Gan. Chrome-freeMgO-ZrO 2 -SiO 2 based refractory material for RHvacuum furnace liner. CN 1,715,246 (January 4,2006).(5951) S. Jiang. Method for preparing composite binder ofindustrial briquette. CN 1,772,854 (May 17, 2006).(5952) F. Guo. Method for preparing high-performancebriquette binder for fertilizer gasification. CN1,749,372 (March 22, 2006).(5953) D. Lin and L. Wang. Multi-functional and highperformancebinder for coal briquets for manufactureof ammonia liquor during coking. CN 101,077,986(November 28, 2007).(5954) M. Sato and A. Kobayashi. Method to produce coalbriquet. JP 2007/039,611 (February 15, 2007).(5955) D. Rong. Activated coal-based binder formanufacture of molded coal-based fuel briquets. CN1,923,985 (March 7, 2007).(5956) M. Sun. Method for preparing dry powder binder formolded coal briquets. CN 1,888,033 (January 3,2007).(5957) L. Zhuang, W. Zhuang, and X. Zhang. Compositebinder for fuel briquets. CN 101,077,985 (November28, 2007).Iron Ore Pellets(5958) Y. Zhang, T. Chen, and T. Liu. Manufacture ofadhesive for iron ore pellets. CN 1,814,825 (August9, 2006).-324-
(5959) Y. Zhang, T. Chen, and T. Liu. Method for preparingiron-ore pellets containing boltonite and adhesivewith high thermal stability, high strength and goodreducing property. CN 1,807,662 (July 26, 2006).(5960) F. Xian, D. Yang, and J. Sun. Preparation, directreduction and electric furnace smelting process ofcold bound carbon-containing pellet from vanadiumtitaniummagnetite. CN 1,804,059 (July 19, 2006).(5961) Q. Zhang and Y. Li. Manufacture of iron powderpellets from flue dust for steelmaking. CN 1,733,947(February 15, 2006).(5962) Z. Zhang. Organic adhesives for iron ore pellets andtheir application. CN 1,962,898 (May 16, 2007).Wood Pellets(5963) M. Olsson. Wheat straw and peat for fuel pellets–organic compounds from combustion. BiomassBioenergy 2006, 30(6), 555-564.Biocide(5883) G.-h. Zhou and Y.-n. Lin. Synthesis and application of newcationic water treatment chemicals. Jingxi Yu ZhuanyongHuaxuepin 2007, 15(5), 22-24.Bone China Manufacture(5964) X. Zhu. Introduction on batch formula for bone china castingslurry. Taoci Kexue Yu Yishu 2006, 40(1), 21-22.Brick Manufacture(5965) Z. Li, T. Chen, and Q. Xie. Environment-friendly calcinationfreephosphogypsum bricks produced by pressure molding. CN1,673,154 (September 28, 2005).(5966) J. Song and B. Wu. Improving character and utilization ofquartz sand in brick-making. Feijinshukuang 2005, 28(1), 19-20, 24.(5967) X. Zhong. Manufacture of polished bricks by low-temperaturesintering. CN 1,907,908 (February 7, 2007).(5968) X. Zhong. Manufacture of antique bricks by low-temperaturesintering. CN 1,907,907 (February 7, 2007).Brick Glaze Additive(5969) M. Wang. Application of Zr-based pigment in external wallbrick production. Shandong Taoci 2006, 29(2), 38-40.-325-
Calcium Carbonate Processing(5970) H.-d. Liu, R.-f. Zhao, and Y.-f. Chen. Controlling morphologyand specific surface area of calcium carbonate particles withhumic acid. Guocheng Gongcheng Xuebao 2006, 6(2), 219-222.Capacitor Manufacture(5971) T. Kuwahara. Double-layer capacitors and manufacture ofcapacitors by coating polarized electrode slurry on collectors. JP2005/347,608 (December 15, 2005).Catalyst Component(4706) C. Machado. Catalyst for thermal cracking of vegetable andmineral oils, plastics, rubbers and dehydration of castor oil. WO2001/068,243 (September 20, 2001).(4905) M. Fukushima, Y. Tanabe, K. Morimoto, and K. Tatsumi. Roleof humic acid fraction with higher aromaticity in enhancing theactivity of a biomimetic catalyst, tetra(psulfonatophenyl)porphineiron(III).Biomacromolecules 2007,8(2), 386-391.(5972) Q.-J. Xu, D.-P. Zhou, and Y.-C. Cui. Catalytic performance ofhumic acid supported Pd/Ni bimetallic catalyst for Heckreaction. Youji Huaxue 2007, 27(12), 1520-1524.(5973) J.-P. Aguer, D. Tetegan, and C. Richard. <strong>Humic</strong> substancesmediated phototransformation of 2,4,6-trimethylphenol: acatalytic reaction. Photochem. Photobiol. Sci. 2005, 4(6), 451-453.(5974) K. Stemmler, M. Ammann, C. Donders, J. Kleffmann, and C.George. Photosensitized reduction of nitrogen dioxide on humicacid as a source of nitrous acid. Nature 2006, 440(7081), 195-198.(5975) I. Yu. Vashurina, S. V. Makarov, Yu. A. Kalinnikov, and E. A.Vlasova. <strong>Humic</strong> acids as efficient catalysts fordisproportionation of peroxide in alkaline solutions. Russ. J.Appl. Chem. 2006, 79(2), 275-278.(5976) X. Yin and L. Li. Metal salt-based combustion catalysts for coal.CN 1,718,699 (January 11, 2006).(5977) I. Yu. Vashurina, S. V. Makarov, E. A. Vlasova, and Yu. A.Kalinnikov. <strong>Humic</strong> acids as catalysts of processes for oxidationby hydrogen peroxide. Izv. Vyssh. Ucheb. Zaved. Khim. Khim.Tekhnol. 2006, 49(9), 32-35.(5978) Q.-j. Xu, Y.-c. Cui, and L. Zhang. <strong>Humic</strong> acid supportedpalladium catalyst for Heck reaction. Henan Daxue XuebaoZiran Kexueban 2006, 36(4), 51-54.-326-
(5979) T. A. Hatton and L. E. Bromberg. Catalytic nanoparticles fornerve agent destruction. WO 2007/092,029 (August 16, 2007).(5980) E. A. Aubakirov. Synthesis and catalytic properties ofimmobilized palladium-potassium humate catalysts supportedon mineral supports. Izv. Nats. Akad. Nauk Resp. Kazakh. Ser.Khim. 2007, (4), 30-34.(5981) Q.-j. Xu, Y.-c. Cui, and Z.-h. Ma. Catalytic properties of humicacid supporting metallic complex for Heck reaction. HuaxueYanjiu 2007, 18(4), 37-40.Cement/Concrete Manufacture(4424) J. Wang and Y. Zhao. Method for manufacturing cement waterreducingagent from coal containing humic acid. CN101,054,271 (October 17, 2007).(5982) K. Maeno and R. Morimoto. Manufacture of cement-containingwaterproofing and light weight compositions and waterproofingmethod using same. JP 10,045,454 (February 17, 1998).(5983) Y. Taki, S. Sasaki, and S. Yukiya. Admixture for enhancinghardness of soil containing cement and method of hardening ofsoil using cement. JP 2001/303,053 (October 31, 2001).(5984) J. P. Vijn and B. Dao. Suspending agents for storable watersilicasuspensions for adding to cementitious compositions forwell bores. US 2003/0,181,542 (September 25, 2003).(5985) Z. Yang and S. Gu. Method for manufacturing cement from redmud. CN 1,613,809 (May 11, 2005).(5986) A. Kasai. Cement-based materials and process for solidificationof humic soils. JP 2005/008,826 (January 13, 2005).(5987) Q. Li and H. Li. A method for the production of an agent in thegrinding of cement. CN 1,566,017 (January 19, 2005).(5988) M. Zhang. A method for manufacture of an agent for acceleratedgrinding of cement. CN 1,896,025 (January 17, 2007).Coloring Agent(5989) D. Inoue, H. Sakurai, M. Wake, and T. Ikeshima.Carbon black for coloring cement and method forcoloring molded cement article. WO 2001/046,322(June 28, 2001).Ceramics Manufacture(5167) X.-r. Sun, J.-m. Yu, and Z.-j. Shan. Study on HANa-AANacopolymer as ceramics multi-functional additive. Jingxi YuZhuanyong Huaxuepin 2007, 15(12), 21-23.-327-
(5989) X. Huo. Study on new ceramic body reinforcing agent. Taoci(Xianyang, China) 2006, (12), 23-25.(5990) S. Li. Manufacture of infrared ceramic electrothermalsubstrate. CN 1,731,897 (February 8, 2006).(5991) Y. Chen and M. Li. Heat resistant ceramic prepared bymoderate temperature sintering, and its preparation method.CN 1,730,430 (February 8, 2006).(5992) W. Zhu, F. Zhao, J. Yao, X. Zhang, H. Wang, C. Xia, and C.-Z. Li.<strong>Humic</strong> acids as a complexible fuel for combustion synthesis ofceramic nanoparticles. J. Amer. Ceram. Soc. 2007, 90(12), 4012-4014.(5993) T. Zhang. Manufacture and application of full-ceramic bibcockvalve. CN 101,067,461 (November 7, 2007).(5994) D. Lu and G. Zhang. Manufacture of ceramic mold with longservice life. CN 101,020,605 (August 22, 2007).(5995) T. Hishiki. Zirconia-based ceramic porous membranes, ceramicfilters, and their manufacture for water purification. JP2007/254,222 (October 4, 2007).(5996) E. V. Gaysler, G. G. Volokitin, N. K. Skripnikova, A. N.Kupryakhin, and P. A. Beznosov. Raw material mix formanufacture of ash-ceramic tiles and brick. RU 2,308,439(October 20, 2007).(5997) P. Bagliono, M. Abrosi, L. Dei, M. Faneschi, L. Mancioli, and S.Santoni. Compositions comprising nanoparticles of zirconiumhydroxide and/or glass frits for coating ceramic products. EP1,845,073 (October 17, 2007).(5998) Y. Jiang, H. Liu, Z. Jiang, Z. Yao, R. Cui, and G. Hao.Preparation and photocatalytic property of platinum-modifiedTiO 2 ceramic film using different compound techniques. KeyEng. Mater. 2007, 336-338(Part 3, High-Performance CeramicsIV), 1939-1942.(5999) E. Saleh. <strong>Product</strong>ion of clay-based ceramics and sanitary warefrom silica, silicate minerals and clay mixtures. US2007/0,149,383 (June 28, 2007).Clay Processing(6000) R. J. Thomas. Low-carbon silica-based clay slurries for slipcasting.US 2005/0,266,978 (December 1, 2005).(6001) V. C. Kelessidis, G. Christidis, P. Makri, V. Hadjistamou, C.Tsamantaki, A. Mihalakis, C. Papanicolaou, and A. Foscolos.Gelation of water-bentonite suspensions at high temperaturesand rheological control with lignite addition. Appl. Clay Sci.2007, 36(4), 221-231.-328-
Clay/Water Slurries(6000) R. J. Thomas. Low-carbon silica-based clay slurries for slipcasting.US 2005/0,266,978 (December 1, 2005).Coal Processing(6002) Q. Zhang and J. Liu. <strong>Product</strong>ion process for industrial moldedcoal. CN 1,597,882 (March 23, 2005).(6003) P. Zhang and J. Li. Manufacture of coal-fuel oil emulsion forindustrial boiler. CN 1,958,754 (May 9, 2007).(6004) W. Yuan, F. Tan, and M. Yuan. Method for producing highefficiencyadditive for coal. CN 1,931,978 (March 21, 2007).(6005) S. Ge. Manufacture and application of environmentally-friendlycoal for gas production. CN 1,931,973 (March 21, 2007).(6006) G. Tang, J. Zhao, K. Wang, L. Dang, X. Cai, and E. Wang.Sodium humate-containing coal spheres prepared from browncoal-derived sodium humate solution. CN 101,070,494(November 14, 2007).Coal/Water Slurries(4341) X. Chen, Y. Ding, Z. Li, and Y. Li. Effect of structuralcharacteristics of anionic additives on zeta potential of coalwater slurry. Meitan Zhuanhua 2006, 29(1), 27-32.(6007) J. Zhang, R. Zhang, and L. Chen. Study on chemicalmodification of humic acid disperser for coal water slurry.Henan Huagong 2005, 22(9), 18-20.(6008) M. Pawlik. Polymer dispersants for coal-water slurries.Colloids Surf. A: Physicochem. Eng. Asp. 2005, 266(1-3), 82-90.(6009) G. Jiang. Sludge-coal aqueous slurry and its production. CN1,594,514 (March 16, 2005).(6010) A. V. Papin, A. N. Zaostrovskii, G. A. Solodov, M. S. Ismagilov,and A. I. Gudkov. Method for utilizing of coal slurries withwaste of humate production. Vest. Kuzbass. Gosud. Tekhnich.Univ. 2006, (2), 86-87.(6011) A. V. Papin, G. A. Solodov, A. N. Zaostrovskii, and A. I. Gudkov.Process of combined use of peat and brown coals with wastesfrom coal beneficiation. Vest. Kuzbass. Gosud. Tekhnich. Univ.2006, (3), 107-110.(6012) V. P. Potapov, G. A. Solodov, A. N. Zaostrovskii, A. V. Papin, S.A. Babenko, and O. K. Semakina. <strong>Product</strong>ion of a water-coalfuel. RU 2,277,120 (May 27, 2006).-329-
(6013) A. V. Papin, A. N. Zaostrovskii, G. A. Solodov, V. I. Murko, andS. I. Zherebtsov. Process for use of sodium humate as aplasticizing reagent for water-coal suspensions. Vest. Kuzbass.Gosud. Tekhnich. Univ. 2005, (4, Part 1), 63-65.(6014) Y.-j. Ding and Y.-x. Li. Effect of the structural characteristics ofanionic additive on the properties of coal water slurry. RanliaoHuaxue Xuebao 2005, 33(6), 661-665.(6015) R. Zhu and Y. Wu. Study on coal/water slurry additive fromalkali extract of lignite. Henan Huagong 2006, 23(10), 20-22.(6016) R. Zhu, X. Liu, and F. Yan. Study on additive for preparation ofcoal water mixture from paper-making waste water and lignin.Henan Huagong 2007, 24(3), 19-21.(6017) H. Chang, Z. Li, J. Ma, X. Li, D. Zhang, and S. Geng. Methodfor manufacturing desulfurized coke aqueous slurry. CN101,029,259 (September 5, 2007).(6018) J. Lu, Y. Zhang, and B. Zhang. Manufacture of fast dissolublecoal slurries with good stability and low viscosity. CN101,029,260 (September 5, 2007).(6019) T. Wei, Y. Li, and C. Li. Method for treating textile-dyeingwastewater by utilizing coal water slurry. CN 101,033,103(September 12, 2007).(6020) A. M. Leonov, M. I. Bychev, and G. I. Petrova. Method fordecreasing dynamic viscosity of water-coal suspensions. RU2,297,024 (April 10, 2007).Coke Manufacture(4797) Y. Xie, Q. Zhang, and G. Chen. Process for producing oxidizedcoke. CN 101,074,401 (November 21, 2007).(6021) J. Wu, Z. Wei, H. Chen, Y. Guo, and J. Li. Method for producingformed coke used for gasification from coke powder. CN1,718,691 (January 11, 2006).(6022) S. Cheng. Preparation of adhesive for coke powder molding. CN1,789,392 (June 21, 2006).(6023) W. Ning, X. Li, and L. Wu. Method for preparing formed cokefrom weakly caking coal. CN 1,850,942 (October 25, 2006).Construction/Building Materials(5983) Y. Taki, S. Sasaki, and S. Yukiya. Admixture for enhancinghardness of soil containing cement and method of hardening ofsoil using cement. JP 2001/303,053 (October 31, 2001).(6024) B. Wu, Y. Zhou, and J. Song. A method for the production ofbuilding materials, based on quartz sand. CN 1,709,818(December 21, 2005).-330-
(6025) G. Deng. A method for manufacturing a curing agent forconstruction materials. CN 1,884,182 (December 27, 2006).Copy Toner(6026) T. Asami, K. Tsubushi, and A. Ishikawa. Electrophotographictoner for textile printing containing phosphor dye coloring agent.JP 2005/256,220 (September 22, 2005).(6027) T. Asami, K. Tsubushi, and A. Ishikawa. Electrophotographicliquid toner containing colorant with functional group and imageformation. JP 2005/084,258 (March 31, 2005).(6028) R. D. Patel, K. A. Moffat, F. M. Mayer, and A. K. Chen. Tonerprocesses. US 2006/0,166,122 (July 27, 2006).(6029) R. D. Patel, G. G. Sacripante, E. G. Zwartz, E. E. Agur, A. K.Chen, T. H. Ng, K. D. Nosella, C. Vong, and K. A. Moffat.Hybrid toner preparation processes. US 2006/0,166,121 (July27, 2006).(6030) D. Vanbesien, D. J. Sanders, R. D. Patel, C. D. Anderson, P. A.Burns, and N.-S. Ro. Economical processes for chemical in situpreparation of electrophotographic toners. US 2007/0,042,286(February 22, 2007).Cosmetics Additive(4586) A. A. Novitskii. <strong>Humic</strong> acids-containing sapropel concentrateand its preparation method. RU 2,264,371 (November 20,2005).(6031) A. K. Sengupta, R. Spindler, and J. W. Darlington, Jr.Multifunctional particulate additive for personal care andcosmetic compositions. WO 2002/062,310 (August 15, 2002).(6032) J. Batzer, W. Berens, T. Blatt, R. Keyhani, I. Kruse, C. Mundt,A. Schepky, M. Schmidt, U. Schoenrock, J. Schulz, C. Smuda, F.Staeb, and R. Wolber. Cosmetic preparations containingantioxidants in combination with cis-9-octadecenedioic acid forthe prevention of skin pigmentation. WO 2003/032,941 (April24, 2003).(6033) N. Liu and J. Wang. <strong>Humic</strong> acids-containing cosmetics andapplication of humic acids in cosmetics. CN 1,568,929 (January26, 2005).(6034) T. Tasawa, K. Shimada, and M. Ando. Cosmetics, watertreatment agents, or deodorants containing chitosan and acids.JP 2005/139,103 (June 2, 2005).(6035) S. Liao, D. Liang, and T. Liang. Stabilized pharmaceutical andcosmetic composition of catechins or derivatives. CA 2,518,844(January 27, 2007).-331-
(6036) S. Liao, D. Liang, and J. Liang. New formulations of catechin orits derivatives for medical and cosmetic use. CN 1,951,383(April 25, 2007).Culture Medium Additive(6037) G. I. Alekseeva, N. G. Pavlov, and A. A. Perk. Method forobtaining culture medium for Mycobacterium tuberculosis. RU2,295,561 (March 20, 2007).Deodorizing Agent(6034) T. Tasawa, K. Shimada, and M. Ando. Cosmetics, watertreatment agents, or deodorants containing chitosan and acids.JP 2005/139,103 (June 2, 2005).Gases(6038) Z. Wen, S. Wang, and M. Xue. Manufacture andapplication of sodium/potassium humate asbiochemical deodorant for refuse deodorization. CN1,607,009 (April 20, 2005).(6039) T. Sato. Pellet showing deodorizing and catalyticfunction for filtration and its manufacture. JP2005/237,913 (September 8, 2005).(6040) Y. Nishida and H. Shiohara. Preparation ofdeodorants from humic substances-containingvolcanic ash agglomerated granules. JP2006/325,752 (December 7, 2006).(6041) M. Prunty and D. Seaby. Granular deodorant forrefuse and compost composition comprising humicsubstance, such as peat, on structural carrier. GB2,439,047 (December 19, 2007).Desulfurization(6042) W.-s. Sun, Y. Meng, and T.-e. Tan. Effects of additives on masstransfer in wet limestone flue gas desulfurization process.Qingdao Daxue Xuebao Gongcheng Jishuban 2006, 21(3), 33-37.(6043) R. Zhao, H. Liu, S. Ye, Y. Xie, and Y. Chen. Ca-based sorbentsmodified with humic acid for flue gas desulfurization. Ind. Eng.Chem. Res. 2006, 45(21), 7120-7125.Diaper Manufacture(6044) M. C. Barney, A. Navarro, and D. S. Ryder. Antimicrobial hopacids for diapers and wet wipes. WO 2002/051,458 (July 4,2002).-332-
Drilling Mud Additive(5304) M. Lu. Method for preparing organosilicon potassium humate.CN 101,024,698 (August 29, 2007).(5370) H. Ni. Collapse-resistant asphalt emulsions containing cationicasphalt emulsifier. CN 1,715,333 (January 4, 2006).(6045) J. R. Von Krosigk. Nutrient source for marine organisms basedon drilling fluids and cuttings treated with biodegradationenhancingadditives. US 2002/0,169,083 (November 14, 2002).(6046) J. R. Von Krosigk. Composition for oil and gas drilling fluidscontaining organic compound contaminants. WO 2002/092,720(November 21, 2002).(6047) J. Hayes. Dry mix for water based drilling fluid. WO2003/025,086 (March 27, 2003).(6048) Y. Wang. Effect of molecular structure of humic acid onperformance of slurry treating agent in well drilling. HenanHuagong 2005, 22(7), 20-21.(6049) C. Yang, B. Yang, X. Ma, Z. Lin, J. Zhang, H. Wen, and E. Chen.Oil-soluble temporary plugging drilling fluid for protecting lowpermeablesand petroleum-gas reservoirs. CN 1,664,049(September 7, 2005).(6050) Z. Huang and Y. Liu. Composite K-Ca ion inhibitor for welldrilling fluid. CN 1,616,589 (May 18, 2005).(6051) Z. Yin, X. Wang, F. Xu, X. Yu, Y. Mao, G. Liu, and C. Lin.Slurry for horizontal directional drilling of sand layer. CN1,563,262 (January 12, 2005).(6052) Z. Yin, X. Wang, F. Xu, X. Geng, Y. Wang, C. Lin, and X. Li.Slurry for horizontal directional drilling of drift sand layer. CN1,563,261 (January 12, 2005).(6053) J. R. Hayes. High performance water-based mud system. US2005/0,187,113 (August 25, 2005).(6054) K. Lu, Z. Qiu, and J. Xu. Preparation and application ofpolyether polyol drilling fluid. Shiyou Xuebao 2006, 27(1), 101-105.(6055) G. Tan. Preparation of high-temperature-resistant viscosityreducing agent for drilling fluid. CN 1,807,542 (July 26, 2006).(6056) H.-b. Geng, L.-h. Qi, and W.-h. Zhao. Application of compoundpolymer drilling fluid in exploration engineering. Meitan Jishu2006, 25(5), 106-107.(6057) G. Tan. Method for preparing high-temperature resistant fluidloss additive for drilling fluid. CN 1,807,543 (July 26, 2006).(6058) H. Ni. Manufacture of anti-collapse asphalt powder for drillingfluids. CN 1,715,334 (January 4, 2006).-333-
(6059) E. V. Kusturova, O. A. Zhugan, A. A. Vasil’chenko, N. V.Gordiichuk, and V. L. Kushnarev. Biopolymer drilling fluid.RU 2,289,603 (December 20, 2006).(6060) M. A. Myslyuk, A. A. Vasil’chenko, Yu. M. Slyzhin, and E. V.Kusturova. Selection of a formulation for treatment of a drillingmud taking into account thermal stability. Strotel. Neft. Gazov.Skvazh. Sushe More 2006, (8), 47-52.(6061) J. Liu, S. Hu, W. Zhu, and F. Ye. Nontoxic coating compositionsfor inner walls. CN 1,982,379 (June 20, 2007).(6062) A. O. Vasil’chenko, O. V. Kusturova, and M. A. Mislyuk.Synergetic compositions of chemical reagents as a basis ofsystems of drilling fluids. Naft. Gaz. Promisl. 2007, (1), 24-26.(6063) M. G. Tutuianu, I. Ana, and M. Orosz. Polymer-based drillingfluid. RO 121,217 (January 30, 2007).(6064) H. Jiang, N. Zhan, W. Xue, Z. Yu, H. Zou, X. Bai, and W. Wang.New type post pad for well cementation. CN 101,081,975(December 5, 2007).(6065) H. Zou, Z. Qiu, W. Wang, C. Huang, G. Qiao, Z. Zhang, S. Ma, G.Liu, and J. Zhang. Strengthened collapse-resistant aqueousdrilling fluid for selective plugging of reservoir strata. CN1,903,973 (January 31, 2007).Dye Applications(4775) P. Savarino, E. Montoneri, M. Biasizzo, P. Quagliotto, G.Viscardi, and V. Boffa. Upgrading biomass wastes in chemicaltechnology. <strong>Humic</strong> acid-like matter isolated from compost aschemical auxiliary for textile dyeing. J. Chem. Technol.Biotechnol. 2007, 82(10), 939-948.(5844) G. Yang, L. Yang, X. Wang, and Y. Li. Experimental study ofdyeing ammonium phosphate with humic acid. Huafei Gongye2007, 34(6), 19-20, 24.(6066) D. J. Hughes. Colorant for foliage of humic and/or fulvic acidand dye. WO 2004/096,920 (November 11, 2004).(6067) T. Yoshida. Agent for colorization of non-transparent deeplybluewater in storage tank and its preparation. JP2005/263,820 (September 29, 2005).(6068) R. L. Beatty and H. W. Rasmussen. Method for coloring rockswith natural appearance of desert varnish using fulvic acid andhumic acid mixtures. US 1005/0,163,936 (July 28, 2005).(6069) B. Li, R. Chen, and S. Wang. Coagulation-preventing colorationconditioner. CN 1,597,639 (March 23, 2005).-334-
(6070) M. Matsuda, A. Urashima, F. Kining, K. Hayakawa, H. Murata,and I. Furukawa. Dyeing with humic acid. Sen’i Gakkaishi2006, 62(2), 39-45.(6071) H. Murata, I. Mukoyoshi, I. Furukawa, M. Matsuda, A.Urashima, F. Kining, and K. Hayakawa. Dyeing with humicacid. Kogoshima-ken Kogyo Gijutsu Senta Kenkyu Hokoku 2005,19, 25-28.Electrode Fabrication(6072) Y. Fu. Lead-acid accumulator jar containing lead oxide and leadnanoparticles in magnetic plate electrodes. CN 1,700,497(November 23, 2005).(6073) K. Toda. Corrosion-proof system for steel-reinforced concrete.JP 2005/097,931 (April 14, 2005).(6074) L. S. Silva, T. N. Oliveira, M. A. Ballin, and C. R. M. Peixoto.Ascorbic acid determination using a carbon paste electrodemodified with iron(III) ions adsorbed on humic acid. Eclet.Quim. 2006, 31(4), 39-42.(6075) A. Profumo, F. Zavarise, D. Merli, I. Tredici, G. Alberti, S.Protti, and M. Fagnoni. Derivatized humic acids modified goldelectrode: electrochemical characterization and analyticalapplications. Anal. Chim. Acta 2007, 598(1), 58-64.(6076) F. P. S. Airoldi, W. T. L. Da Silva, F. N. Crespilho, and M. O. O.Rezende. Evaluation of the electrochemical behavior ofpentachlorophenol by cyclic voltammetry on carbon pasteelectrode modified by humic acids. Water Environ. Res. 2007,79(1), 63-67.(6077) T. Zhong, Y. Qu, S. Huang, and F. Li. Electrochemical studies ofcytochrome C on gold electrodes with promoter of humic acidand 4-aminothiophenol. Microchim. Acta 2007, 158(3-4), 291-297.Fabrics Manufacture(5386) T. Roess, W. Spyra, G. Sieling, A. Biegel, and M. Noack. Fabricsor fibrous materials consisting of lignite fibers for use inhorticulture, environmental protection, construction, etc. WO2006/100,065 (September 28, 2006).Firebrick Manufacture(6078) T. Teraushi. Effects of humic substances in ball clays on thedispersion and the shaping properties of firebrick bodies.Seramikkusu 2007, 42(8), 582-585.-335-
Food <strong>Product</strong>s Additive(4977) J. Szollosy. Solid food supplementary compositions containinghoney and complexes of iron-, chromium-, selenium-, and zinchumicacid and their production. HU 2003/003,225 (April 28,2006).(6079) M. Yamada. Agents and method for deterioration inhibition ofedible oils, and cooking utensils containing the agents. JP2006/050,959 (February 23, 2006).(6080) X. Qi. Slimming ice cream preparation. CN 101,069,556(November 14, 2007).(6081) K. K. Gusev. Biologically active additive. RU 2,259,147 (August27, 2005).Fungicide(5149) P. Kraft-Klaunzer and N. Klaunzer. Copper compounds andtheir use as fungicides, algicides and bactericides. DE10/2005/061,691 (June 28, 2007).Gypsum Manufacture(6082) H. Chen, Y. Ren, and J. Li. Influence of several additives on theperformances of mold gypsum. Xiandai Jishu Taoci 2007, 28(1),6-10.Hair Growth Stimulation(5356) K. S. Day and G. A. Hansen. Compositions and methods forhuman use containing fulvic acid. US 2007/0,212,434(September 13, 2007).Heat Transfer Medium(6083) S. Ming. Heat-transfer medium and methods of making andusing the same. US 2005/0,179,001 (August 18, 2005).HPLC Substrate(4912) N. Casadei, M. Thomassin, Y.-C. Guillaume, and C. Andre. Ahumic acid stationary phase for the high performance liquidchromatography separation of buckminsterfullerenes:theoretical and practical aspects. Anal. Chim. Acta 2007,588(2), 268-273.Ink Manufacture(6084) T. Uemura, T. Iguchi, and Y. Iida. Light- and weather-resistantwater-thinned ink-jet inks. JP 10,219,165 (August 18, 1998).-336-
Ion Exchange Manufacture(6085) A. A. Zaripova. Synthesis of ion-exchange resins on the base ofhumic acids and p-fenilendiamin. Izv. Nats. Akad. Nauk Kyrgyz.Resp. 2007, (3), 43-48.(6086) A. A. Zaripova. Synthesis of ion-exchange resins from humicacids and furfural. Izv. Nats. Akad. Nauk Kyrgyz. Resp. 2007,(4), 46-48.Iron Alloy Manufacture(6087) Z. Ye, W. Chen, and Q. Shen. Moulding of lignite semicoke usedin ferroalloy production. Meitan Zhuanhua 2005, 28(4), 27-29.Iron Ore Processing(5381) Y. Wang, J. Zhang, and S. Li. Method for preparing pelletadhesive from starch and humate. CN 1,818,097 (August 16,2006).(6088) Y. Li and X. Zhang. Method for pre-treating raw materials usedin silicon-iron smelting. CN 101,020,961 (August 22, 2007).(6089) Yaj. Su, Y. Du, N. Yin, and Yad. Su. Manufacture of cold boundcarbon-containing iron ore pellets. CN 1,718,780 (January 11,2006).(6090) Y. Li. Refractory cast material for air inlet pipe of blast furnace,and its preparation method. CN 1,730,441 (February 8, 2006).(6091) F. D. Oeste. Iron containing precipitates in firm and loose rocks.DE 10,2005/045,521 (May 4, 2006).(6092) I. D. Dos Santos and J. F. Oliveira. Utilization of humic acid asa depressant for hematite in the reverse flotation of iron ore.Miner. Eng. 2007, 20(10), 1003-1007.Lip Balm(6093) F. Schiller, P. Wutzler, R. Kloecking, B. Helbig, K. D. Thiel, andA. Moebius. Antiviral UV-protective lip cream. DE 4,229,713(March 10, 1994).Microbicide(6044) M. C. Barney, A. Navarro, and D. S. Ryder. Antimicrobial hopacids for diapers and wet wipes. WO 2002/051,458 (July 4,2002).Oil Absorption(6094) N. E. Sosnovskaya, A. S. Samsonova, A. E. Tomson, and A. A.Terent’ev. Effect of peat composition on its oil and oil productsabsorption ability. Prirodn. Res. 2006, (4), 77-82.-337-
Oil <strong>Product</strong>ion/Processing(5304) M. Lu. Method for preparing organosilicon potassium humate.CN 101,024,698 (August 29, 2007).(6095) Z. Shen. <strong>Acid</strong>ic detergent for oil delivery pipe. CN 1,754,954(April 5, 2006).(6096) G. Zhang, Q. Zhang, M. Sun, J. Ge, and D. Zhang. Preparationof composite oil displacement agent for tertiary oil recovery. CN1,560,181 (January 5, 2005).(6097) N. Castellano. Composition and method to enhance recoveryfrom oil wells. WO 2007/005,944 (January 11, 2007).(6098) C. W. Roddy, J. Chatterji, D. C. Brenneis, and B. J. King.Settable spotting compositions containing cement kiln dust foruse in treatment of petroleum wells. US 7,199,086 (April 3,2007).Ointment Manufacture(6099) R. R. Ismatova, T. V. Romanko, and V. E. Narkevich.Rheological studies of the ointment with sodium humate.Bashk. Khim. Zh. 2007, 14(3), 95-97.(6193) K. Golz-Berner and L. Zastrow. Use of radical capturingsubstances in a topical preparation for antipyretic treatment.WO 2006/117,404 (November 9, 2006).(6203) A. I. Kosolapova and E. I. Smyshlyaev. Anti-inflammatoryointment containing potassium humate and birch tar. RU2,280,458 (July 27, 2006).Oral Hygiene <strong>Product</strong>s(6100) B. Giles. Compositions for oral hygiene containing cesium andrubidium salts. WO 2005/099,658 (October 27, 2005).Oxygen Scavenging(6101) Z. Shen. Oxygen scavenger for boiler with corrosion resistance.CN 1,854,082 (November 1, 2006).Paint Manufacture(6102) G. Gao, G. Yao, H. Sun, and P. Ren. II type Zn-Cr compositecoating for antisepsis. CN 1,962,945 (May 16, 2007).Polymer Manufacture(6103) Z. G. Akkulova. <strong>Natural</strong>-synthetic polymers from coal humicacids. Izv. Nats. Akad. Nauk Resp. Kazakh. Ser. Khim. 2006,(3), 73-76.-338-
Porcelain Manufacture(6104) J. Ouyang. Method and apparatus for manufacturing split tilewith art texture. CN 1,598,214 (March 23, 2005).(6105) K. Dong. Manufacture of colored porcelain for daily use andartworks. CN 1,587,183 (March 2, 2005).(6106) F. Li, H. Yang, and K. Dong. Preparation of decorative porcelainwith colorful glaze. CN 1,583,658 (February 23, 2005).(6107) X. Zhu. Research on the recipe of casting slip of bone porcelain.Taoci (Xianyang, China) 2006, (6), 27-28.Radiation Protection(6108) V. P. Shipov, E. S. Pigarev, E. I. Fedoros, and N. P. Trofimova.Method for producing humus-based radioprotectant. WO2006/088,394 (August 24, 2006).Semiconductor Manufacture(6109) L. L. Ang, T. H. Tan, and T. Masuda. Epoxy resin compositionfor semiconductor sealing and semiconductor device. SG120,855 (April 26, 2006).Skin Care(4724) Y. Ishida and K. Suzuki. Humus, humus extracts, humusderivedskin-moisturizers, and production thereof. JP2006/273,734.(5375) A. K. Sengupta, K. Cureton, I. Lin, and T. W. Beihoffer. Highefficiency sunscreen composition particularly useful for wipesand sprays. US 2007/0,178,057 (August 2, 2007).(6093) F. Schiller, P. Wutzler, R. Kloecking, B. Helbig, K. D. Thiel, andA. Moebius. Antiviral UV-protective lip cream. DE 4,229,713(March 10, 1994).(6110) S. Kuehn. Investigations on the mechanism of UV-B-protectiveeffect of humic acid in vitro. Metadata Internet Doc. (Ger. Diss.)2005, D0712-4.(6111) A. K. Sengupta and I. Lin. Stable sunscreen compositionscontaining zinc oxide. US 2006/0,280,702 (December 14, 2006).Sludge Stabilization(6112) J. Sun. Y. Liu, and L. Liang. Composition of sludge stabilizerand its application. CN 101,081,718 (December 5, 2007).-339-
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(5332) T. F. Krzeminski, J. K. Nozynski, J. Grzyb, M. Proc, S. Zeglen, V.Filas, E. Skopinska-Rozewska, E. Sommer, and M. Filewska.Angiogenesis and cardioprotection after TNF-inducer-Tolpa PeatPreparation treatment in rat’s hearts after experimental myocardialinfarction in vivo. Vasc. Pharmacol. 2005, 43(3), 164-170.(5352) K. Golz-Berner and L. Zastrow. Use of radical capturing substancesin a topical preparation for antipyretic treatment. WO 2006/117,404(November 9, 2006).(5356) K. S. Day and G. A. Hansen. Compositions and methods for humanuse containing fulvic acid. US 2007/0,212,434 (September 13, 2007).(5945) N. Liu and J. Wang. Health beverage containing humic acid and theapplication of humic acid in beverage. CN 1,568,827 (January 26,2005).(6035) S. Liao, D. Liang, and T. Liang. Stabilized pharmaceutical andcosmetic composition of catechins or derivatives. CA 2,518,844(January 27, 2007).(6036) S. Liao, D. Liang, and J. Liang. New formulations of catechin or itsderivatives for medical and cosmetic use. CN 1,951,383 (April 25,2007).(6093) F. Schiller, P. Wutzler, R. Kloecking, B. Helbig, K. D. Thiel, and A.Moebius. Antiviral UV-protective lip cream. DE 4,229,713 (March10, 1994).(6110) S. Kuehn. Investigations on the mechanism of UV-B-protective effectof humic acid in vitro. Metadata Internet Doc. (Ger. Diss.) 2005,D0712-4.(6140) I. Lasenko. Textile articles for treating fungal and bacterialinfections. LV 13,314 (October 20, 2005).(6141) K. Matsuda and Y. Tanaka. Acrylic fibers having washfast, longlastinghygroscopicity and antimicrobial properties and theirmanufacture. JP 2005/336,621 (December 8, 2005).(6142) I. Lyashenko, P. Nousiainen, and I. Pyykko. Textile article fortherapeutic use. WO 2006/088,342 (August 24, 2006).(6189) A. C. Bittner, R. M. Croffut, and M. C. Stranahan. Prescript-assistprobiotic-prebiotic treatment for irritable bowel syndrome: amethodologically oriented, 2-week, randomized, placebo-controlled,double-blind clinical study. Clin. Therap. 2005, 27(6), 755-761.(6190) J. B. Windsor, S. J. Roux, A. M. Lloyd, and C. E. Thomas. Methodsand compositions for increasing the efficacy of biologically-activeingredients such as antitumor agents. WO 2005/014,777 (February17, 2005).(6191) C. F. Van Der Westhuizen. Detoxifying and immunity-boostercomposition comprising microbes and fulvic acid. WO 2006/064,449(June 22, 2006).-352-
(6192) V. P. Shipov, E. S. Pigarev, E. I. Fedoros, and N. P. Trofimova.Method for producing anticancer platinum-humic acids complexes.WO 2006/088,393 (August 24, 2006).(6193) K. Golz-Berner and L. Zastrow. Use of radical capturing substancesin a topical preparation for antipyretic treatment. WO 2006/117,404(November 9, 2006).(6194) V. P. Shipov, E. S. Pigarev, E. I. Fedoros, and N. P. Trofimova.Method for producing anticancer platinum-humic acids complexes.WO 2006/088,393 (August 24, 2006).(6195) W. Jy, J. J. Jimenez, L. L. Horstmann, Y. S. Ahn, and E. Ahn. Cellderivedmicroparticles as hemostatic agents for control ofhemorrhage and treatment of bleeding disorders. WO 2006/062,945(June 15, 2006).(6196) S. D. Patil, F. Papadmitrakopoulos, and D. J. Burgess. Concurrentdelivery of dexamethasone and VEGF for localized inflammationcontrol and angiogenesis. J. Contr. Release 2007, 117(1), 68-79.(6197) A. Dinda, S. C. Si, B. B. Barik, and I. Biswal. Sustained releasedelivery of budesonide from PLGA microspheres embedded withinpoly-acid containing PVA hydrogel. PHARMBIT 2007, 16(2), 130-142.(6198) G. Liu. Preparation of compound medicine with traditional Chinesemedicine and western medicine for treating gout. CN 101,023,962(August 29, 2007).Anaphylactic Shock(4465) R. R. Ismatova, A. U. Ziganshin, and S. E. Dmitruk. Effects ofsodium humate isolated from peat obtained in Tomsk region onallergic reactions. Eksper. Klin. Farmakol. 2007, 70(6), 29-31.Anti-Bacterial Agent(4705) J. Dekker and C. E. Medien. Oxihumic acid and its use in thetreatment of various conditions. WO 2000/016,786 (March 30,2000).(5329) J. Dekker and C. E. Medlen. <strong>Humic</strong> acid and its use in thetreatment of various conditions. WO 2000/016,785 (March 30,2000).(6141) K. Matsuda and Y. Tanaka. Acrylic fibers having washfast,long-lasting hygroscopicity and antimicrobial properties andtheir manufacture. JP 2005/336,621 (December 8, 2005).Anti-Cancer Agent(4705) J. Dekker and C. E. Medien. Oxihumic acid and its use in thetreatment of various conditions. WO 2000/016,786 (March 30,2000).-353-
(5329) J. Dekker and C. E. Medlen. <strong>Humic</strong> acid and its use in thetreatment of various conditions. WO 2000/016,785 (March 30,2000).(6190) J. B. Windsor, S. J. Roux, A. M. Lloyd, and C. E. Thomas.Methods and compositions for increasing the efficacy ofbiologically-active ingredients such as antitumor agents. WO2005/014,777 (February 17, 2005).(6192) V. P. Shipov, E. S. Pigarev, E. I. Fedoros, and N. P. Trofimova.Method for producing anticancer platinum-humic acidscomplexes. WO 2006/088,393 (August 24, 2006).(6194) V. P. Shipov, E. S. Pigarev, E. I. Fedoros, and N. P. Trofimova.Method for producing anticancer platinum-humic acidscomplexes. WO 2006/088,393 (August 24, 2006).(6199) V. A. Trofimov, V. P. Shipov, E. S. Pigarev, A. I. Popov, and V.N. Ivanov. Anticancer agent. WO 2002/066,039 (August 29,2002).(6200) H. Kodama. Antitumor effect of humus extract on murinetransplantable L1210 leukemia. J. Vet. Med. Sci./Jpn. Soc. Vet.Sci. 2007, 69(10), 1069-1071.Anti-Infective Agent(6140) I. Lasenko. Textile articles for treating fungal and bacterialinfections. LV 13,314 (October 20, 2005).Anti-Inflammatory Properties(4705) J. Dekker and C. E. Medien. Oxihumic acid and its use in thetreatment of various conditions. WO 2000/016,786 (March 30,2000).(4779) C. E. J. Resnburg, J. R. Snyman, T. Mokoele, and A. D.Cromarty. Brown coal derived humate inhibits contacthypersensitivity: an efficacy, toxicity and teratogenicity study inrats. Inflammation 2007, 30(5), 148-152.(6196) S. D. Patil, F. Papadmitrakopoulos, and D. J. Burgess.Concurrent delivery of dexamethasone and VEGF for localizedinflammation control and angiogenesis. J. Contr. Release 2007,117(1), 68-79.(6201) J. F. Lown, K. Gill, S. J. Cutler, H. G. Cutler, and S. H. Pollock.Anti-inflammatory humate compositions and methods of usethereof. US 2004/0,131,705 (July 8, 2004).(6202) W. J. Serfontein. Nutritional compositions containing seleniumand lithium and use thereof as anti-HIV and anti-AIDSnutraceuticals and immunostimulants. WO 2004/107,881(December 16, 2004).-354-
(6203) A. I. Kosolapova and E. I. Smyshlyaev. Anti-inflammatoryointment containing potassium humate and birch tar. RU2,280,458 (July 27, 2006).Anti-Microbial Properties(4941) H. M. Bialk, C. Hedman, A. Castillo, and J. A. Pedersen.Laccase-mediated Michael addition of 15 N-sulfapyridine to amodel humic constituent. Environ. Sci. Technol. 2007, 41(10),3593-3600.(5191) H. M. Bialk, A. J. Simpson, and J. A. Pedersen. Cross-couplingof sulfonamide antimicrobial agents with model humicconstituents. Environ. Sci. Technol. 2005, 39(12), 4463-4473.(6204) H. M. Bialk. Covalent cross-coupling of sulfonamideantimicrobials with model humic components and humicsubstances. Diss. Abstr. Int. B 2006, 67(6), 3031.Anti-Pyretic Agent(5352) K. Golz-Berner and L. Zastrow. Use of radical capturingsubstances in a topical preparation for antipyretic treatment.WO 2006/117,404 (November 9, 2006).(6192) V. P. Shipov, E. S. Pigarev, E. I. Fedoros, and N. P. Trofimova.Method for producing anticancer platinum-humic acidscomplexes. WO 2006/088,393 (August 24, 2006).(6193) K. Golz-Berner and L. Zastrow. Use of radical capturingsubstances in a topical preparation for antipyretic treatment.WO 2006/117,404 (November 9, 2006).Anti-Viral Efficacy(4705) J. Dekker and C. E. Medien. Oxihumic acid and its use in thetreatment of various conditions. WO 2000/016,786 (March 30,2000).(4807) A. Sauerbrei, C. Meier, A. Meerbach, M. Schiel, B. Helbig, andP. Wutzler. In vitro activity of cycloSal-nucleosidemonophosphates and polyhydroxycarboxylates againstorthopoxviruses. Antiviral Res. 2005, 67(3), 147-154.(5329) J. Dekker and C. E. Medlen. <strong>Humic</strong> acid and its use in thetreatment of various conditions. WO 2000/016,785 (March 30,2000).(5945) N. Liu and J. Wang. Health beverage containing humic acidand the application of humic acid in beverage. CN 1,568,827(January 26, 2005).(6093) F. Schiller, P. Wutzler, R. Kloecking, B. Helbig, K. D. Thiel, andA. Moebius. Antiviral UV-protective lip cream. DE 4,229,713(March 10, 1994).-355-
AIDS(4705) J. Dekker and C. E. Medien. Oxihumic acid and itsuse in the treatment of various conditions. WO2000/016,786 (March 30, 2000).(5308) B. Halford. Dendrimers branch out. Chem. Eng. News2005, 83(24), 30-33.(5329) J. Dekker and C. E. Medlen. <strong>Humic</strong> acid and its use inthe treatment of various conditions. WO 2000/016,785(March 30, 2000).(6201) J. F. Lown, K. Gill, S. J. Cutler, H. G. Cutler, and S. H.Pollock. Anti-inflammatory humate compositions andmethods of use thereof. US 2004/0,131,705 (July 8,2004).Cowpox Virus(4807) A. Sauerbrei, C. Meier, A. Meerbach, M. Schiel, B.Helbig, and P. Wutzler. In vitro activity of cycloSalnucleosidemonophosphates and polyhydroxycarboxylatesagainst orthopoxviruses. Antiviral Res.2005, 67(3), 147-154.Herpes Viruses(4705) J. Dekker and C. E. Medien. Oxihumic acid and itsuse in the treatment of various conditions. WO2000/016,786 (March 30, 2000).(6093) F. Schiller, P. Wutzler, R. Kloecking, B. Helbig, K. D.Thiel, and A. Moebius. Antiviral UV-protective lipcream. DE 4,229,713 (March 10, 1994).Vaccinia Virus(4807) A. Sauerbrei, C. Meier, A. Meerbach, M. Schiel, B.Helbig, and P. Wutzler. In vitro activity of cycloSalnucleosidemonophosphates and polyhydroxycarboxylatesagainst orthopoxviruses. Antiviral Res.2005, 67(3), 147-154.Bleeding Disorders(6195) W. Jy, J. J. Jimenez, L. L. Horstmann, Y. S. Ahn, and E. Ahn.Cell-derived microparticles as hemostatic agents for control ofhemorrhage and treatment of bleeding disorders. WO2006/062,945 (June 15, 2006).-356-
Drug Delivery(4941) H. M. Bialk, C. Hedman, A. Castillo, and J. A. Pedersen.Laccase-mediated Michael addition of 15 N-sulfapyridine to amodel humic constituent. Environ. Sci. Technol. 2007, 41(10),3593-3600.(5191) H. M. Bialk, A. J. Simpson, and J. A. Pedersen. Cross-couplingof sulfonamide antimicrobial agents with model humicconstituents. Environ. Sci. Technol. 2005, 39(12), 4463-4473.(6197) A. Dinda, S. C. Si, B. B. Barik, and I. Biswal. Sustained releasedelivery of budesonide from PLGA microspheres embeddedwithin poly-acid containing PVA hydrogel. PHARMBIT 2007,16(2), 130-142.(6204) H. M. Bialk. Covalent cross-coupling of sulfonamideantimicrobials with model humic components and humicsubstances. Diss. Abstr. Int. B 2006, 67(6), 3031.Drug Synergy(4448) L. Aristilde and G. Sposito. Reactivity of the antibioticciprofloxacin with humic substances: effects of solutionchemistry. In Book of Abstracts, 234 th ACS National Meeting;Boston, Massachusetts: American Chemical Society, 2007;ENVR-160.(4632) R. Khanna, S. P. Agarwal, and R. K. Khar. A novel complexes.IN 2005/DE00,532 (December 1, 2006).(4892) S. P. Agarwal, M. Aqil, and Md. K. Anwer. Enhancement of thedissolution and diuretic effect of furosemide through a novelcomplexation with humic acid extracted from shilajit. Asian J.Chem. 2007, 19(6), 4711-4718.Folk Medicine(6198) G. Liu. Preparation of compound medicine with traditionalChinese medicine and western medicine for treating gout. CN101,023,962 (August 29, 2007).Gout(6198) G. Liu. Preparation of compound medicine with traditionalChinese medicine and western medicine for treating gout. CN101,023,962 (August 29, 2007).-357-
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Rheumatoid DiseaseMud Baths(5161) E. Odabasi, H. Gul, E. Macit, M. Turan, and O. Yildiz.Lipophilic components of different therapeutic mudspecies. J. Alt. Complem. Med. 2007, 13(10), 1115-1118.Therapeutic Textile Manufacture(6141) K. Matsuda and Y. Tanaka. Acrylic fibers having washfast,long-lasting hygroscopicity and antimicrobial properties andtheir manufacture. JP 2005/336,621 (December 8, 2005).(6142) I. Lyashenko, P. Nousiainen, and I. Pyykko. Textile article fortherapeutic use. WO 2006/088,342 (August 24, 2006).Wound Healing(6207) N. P. Avvakumova, S. V. Pervushkin, V. V. Rossinskaya, M. A.Krivopalova, A. M. Burylina, Yu. V. Karpeeva, and A. A.Avvakumova. Wound-healing agent. RU 2,274,456 (April 20,2006).-359-
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