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Spin waves and the anomalous Hall effect in ferromagnetic (Ga,Mn)As

Spin waves and the anomalous Hall effect in ferromagnetic (Ga,Mn)As

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to <strong>the</strong>ir sp<strong>in</strong>; it is practically enough to derive such paradigms of physics as<strong>the</strong> Is<strong>in</strong>g, Heisenberg or Hubbard model.Similarly to sp<strong>in</strong>, <strong>the</strong> exchange <strong>in</strong>teraction is a purely quantum phenomenon,which has no analogy <strong>in</strong> <strong>the</strong> classical world. 2 It arises from <strong>the</strong>Coulomb <strong>in</strong>teraction <strong>and</strong> is characterised by an electrostatic potential <strong>in</strong>tegral.It competes with <strong>the</strong> sp<strong>in</strong>-orbit <strong>in</strong>teraction, which couples <strong>the</strong> sp<strong>in</strong> <strong>and</strong>orbital momenta of <strong>the</strong> electron (described <strong>in</strong> Sec. 5.3 <strong>in</strong> more detail). Inthis context, <strong>the</strong> two <strong>in</strong>teractions are often respectively referred to as nonrelativistic<strong>and</strong> relativistic. This seems to be at odds with <strong>the</strong> fact that <strong>the</strong>exchange <strong>in</strong>teraction arises from <strong>the</strong> sp<strong>in</strong> statistics, which results from <strong>the</strong>Lorentz <strong>in</strong>variance of <strong>the</strong> sp<strong>in</strong>or field operators <strong>in</strong> <strong>the</strong> relativistic quantumfield <strong>the</strong>ory. Actually, <strong>the</strong> latter be<strong>in</strong>g <strong>the</strong> epistemically fundamental <strong>the</strong>ory,gives a t<strong>in</strong>t of <strong>the</strong> relativistic character to every physical phenomenon. On<strong>the</strong> o<strong>the</strong>r h<strong>and</strong>, <strong>the</strong> relativistic character of <strong>the</strong> sp<strong>in</strong>-orbit <strong>in</strong>teraction resultsfrom <strong>the</strong> Lorenz <strong>in</strong>variance of <strong>the</strong> electromagnetic field.S<strong>in</strong>ce on <strong>the</strong> atomic scale <strong>the</strong> strength of <strong>the</strong> sp<strong>in</strong>-orbit <strong>in</strong>teraction ismuch lower than that of <strong>the</strong> exchange energy, ca 1Kk B vs. up to 1000Kk B ,one is tempted to th<strong>in</strong>k that <strong>the</strong> former has no chance to make its mark. Infact, compar<strong>in</strong>g <strong>the</strong> Bohr radius, a ⋆ ≈ 0.053nm, represent<strong>in</strong>g <strong>the</strong> nonrelativisticscale, <strong>and</strong> <strong>the</strong> f<strong>in</strong>e structure constant, α = 1/137, represent<strong>in</strong>g <strong>the</strong>relativistic scale, one can see that <strong>the</strong> two types of exchange become comparableat <strong>the</strong> length scales considered <strong>in</strong> solid bodies, a ⋆ /α ≈ 7nm [107].Thus, one can expect to observe <strong>the</strong> veritable cornucopia of physical <strong>effect</strong>sresult<strong>in</strong>g from <strong>the</strong> <strong>in</strong>terplay of <strong>the</strong>se two mechanisms, many of which arediscussed <strong>in</strong> this <strong>the</strong>sis: magnetic anisotropies (Sec. 8.2) <strong>and</strong> formation ofdoma<strong>in</strong> walls, <strong>effect</strong>ive magnetic fields of Bychkov–Rashba <strong>and</strong> Dresselhaus(Sec. 5.4) <strong>and</strong> Dzyalosh<strong>in</strong>skii–Moriya <strong>in</strong>teraction, as well as <strong>the</strong>ir importantconsequences on physics of sp<strong>in</strong> <strong>waves</strong> (Ch. 9) <strong>and</strong> <strong>the</strong> <strong>anomalous</strong> <strong>Hall</strong> <strong>effect</strong>(Ch. 10).Underly<strong>in</strong>g <strong>the</strong> microscopic orig<strong>in</strong> of <strong>the</strong> first Hund rule, <strong>the</strong> exchange<strong>in</strong>teraction maximises <strong>the</strong> total moment with<strong>in</strong> <strong>the</strong> half-filled <strong>Mn</strong> d shell to<strong>the</strong> value of S = 5 2, already mentioned <strong>in</strong> Sec. 3.3. Similarly, it couples <strong>the</strong>s <strong>and</strong> d electrons on <strong>the</strong> same <strong>Mn</strong> site. On <strong>the</strong> o<strong>the</strong>r h<strong>and</strong>, <strong>the</strong> phenomenaof magnetic order require <strong>in</strong>teraction between <strong>Mn</strong> moments, <strong>and</strong> thus<strong>the</strong> exchange coupl<strong>in</strong>g act<strong>in</strong>g between electrons resid<strong>in</strong>g at different sites.Such is <strong>the</strong> coupl<strong>in</strong>g between <strong>the</strong> d electrons of <strong>the</strong> <strong>Mn</strong> substitut<strong>in</strong>g <strong>Ga</strong> sites<strong>and</strong> delocalised p holes which are more heavily weighted on <strong>As</strong> sites of <strong>the</strong>(<strong>Ga</strong>,<strong>Mn</strong>)<strong>As</strong> lattice. The last two <strong>in</strong>teractions result from <strong>the</strong> sp–d hybridisationof atomic orbitals, <strong>and</strong> are called <strong>the</strong> s–d <strong>and</strong> p–d exchange coupl<strong>in</strong>g.an exceptionally beautiful topological explanation (though not a proof) [105].2 <strong>Sp<strong>in</strong></strong> has no classical analogue. The commonly shown picture of a sp<strong>in</strong>n<strong>in</strong>g sphere isjust an underst<strong>and</strong><strong>in</strong>g aid, as <strong>the</strong> electron’s size is so small that it would need to sp<strong>in</strong> wi<strong>the</strong>quatorial speeds faster than <strong>the</strong> speed of light to have <strong>the</strong> required value of <strong>the</strong> angularmomentum, a.k.a. sp<strong>in</strong> [106].34

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