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Understanding Neutron Radiography Post Exam Reading VIII-Part 2a of 2A

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<strong>Understanding</strong> <strong>Neutron</strong> <strong>Radiography</strong><br />

<strong>Reading</strong> <strong>VIII</strong> <strong>Part</strong> 2(a) <strong>of</strong> 2<br />

16 th August 2016<br />

<strong>Post</strong> <strong>Exam</strong> <strong>Reading</strong><br />

Charlie Chong/ Fion Zhang


Spallation Source<br />

Charlie Chong/ Fion Zhang


Spallation Source<br />

Charlie Chong/ Fion Zhang


Spallation Source<br />

Charlie Chong/ Fion Zhang<br />

http://www.gizmodo.com.au/2014/01/27-amazing-images-from-the-depths-<strong>of</strong>-scientific-labs/


Spallation Source<br />

Charlie Chong/ Fion Zhang<br />

http://www.gizmodo.com.au/2014/01/27-amazing-images-from-the-depths-<strong>of</strong>-scientific-labs/


The Magical Book <strong>of</strong> <strong>Neutron</strong> <strong>Radiography</strong><br />

Charlie Chong/ Fion Zhang


Charlie Chong/ Fion Zhang


ASNT Certification Guide<br />

NDT Level III / PdM Level III<br />

NR - <strong>Neutron</strong> Radiographic Testing<br />

Length: 4 hours Questions: 135<br />

1. Principles/Theory<br />

• Nature <strong>of</strong> penetrating radiation<br />

• Interaction between penetrating radiation and matter<br />

• <strong>Neutron</strong> radiography imaging<br />

• Radiometry<br />

2. Equipment/Materials<br />

• Sources <strong>of</strong> neutrons<br />

• Radiation detectors<br />

• Non-imaging devices<br />

Charlie Chong/ Fion Zhang


3. Techniques/Calibrations<br />

• Blocking and filtering<br />

• Multifilm technique<br />

• Enlargement and projection<br />

• Stereoradiography<br />

• Triangulation methods<br />

• Autoradiography<br />

• Flash <strong>Radiography</strong><br />

• In-motion radiography<br />

• Fluoroscopy<br />

• Electron emission radiography<br />

• Micro-radiography<br />

• Laminography (tomography)<br />

• Control <strong>of</strong> diffraction effects<br />

• Panoramic exposures<br />

•Gaging<br />

• Real time imaging<br />

• Image analysis techniques<br />

Charlie Chong/ Fion Zhang


4. Interpretation/Evaluation<br />

• Image-object relationships<br />

• Material considerations<br />

• Codes, standards, and specifications<br />

5. Procedures<br />

• Imaging considerations<br />

• Film processing<br />

• Viewing <strong>of</strong> radiographs<br />

• Judging radiographic quality<br />

6. Safety and Health<br />

• Exposure hazards<br />

• Methods <strong>of</strong> controlling radiation exposure<br />

• Operation and emergency procedures<br />

Reference Catalog Number<br />

NDT Handbook, Third Edition: Volume 4,<br />

Radiographic Testing 144<br />

ASM Handbook Vol. 17, NDE and QC 105<br />

Charlie Chong/ Fion Zhang


Charlie Chong/ Fion Zhang<br />

Fion Zhang at Copenhagen Harbor<br />

16 th August 2016


Charlie Chong/ Fion Zhang<br />

SME- Subject Matter Expert<br />

http://cn.bing.com/videos/search?q=Walter+Lewin&FORM=HDRSC3<br />

https://www.youtube.com/channel/UCiEHVhv0SBMpP75JbzJShqw


Gamma- <strong>Radiography</strong><br />

TABLE 1. Characteristics <strong>of</strong> three isotope sources commonly used for<br />

radiography.<br />

Source<br />

T½<br />

Energy<br />

HVL<br />

HVL<br />

Specific<br />

Dose rate*<br />

Pb<br />

Fe<br />

Activity<br />

Co60<br />

5.3 year<br />

1.17, 1.33 MeV<br />

12.5mm<br />

22.1mm<br />

50 Cig -1<br />

1.37011<br />

Cs137<br />

30 years<br />

0.66 MeV<br />

6.4mm<br />

17.2mm<br />

25 Cig -1<br />

0.38184<br />

Ir192<br />

75 days<br />

0.14 ~ 1.2 MeV<br />

4.8mm<br />

?<br />

350 Cig -1<br />

0.59163<br />

(Aver. 0.34 MeV)<br />

Th232<br />

0.068376<br />

Dose rate* Rem/hr at one meter per curie<br />

Charlie Chong/ Fion Zhang


八 千 里 路 云 和 月<br />

Charlie Chong/ Fion Zhang


Charlie Chong/ Fion Zhang


闭 门 练 功<br />

Charlie Chong/ Fion Zhang


Charlie Chong/ Fion Zhang<br />

http://greekhouse<strong>of</strong>fonts.com/


Charlie Chong/ Fion Zhang


Whole Chapter 5<br />

Radiation Measurement<br />

Charlie Chong/ Fion Zhang


PART 1. Principles <strong>of</strong> Radiation Measurement<br />

Emissions from radioactive nuclei and radiation from that portion <strong>of</strong> the<br />

electromagnetic spectrum beyond the ultraviolet energies can cause the<br />

ionization <strong>of</strong> atoms and molecules. Ionizing radiation occurs as three forms:<br />

(1) charged particles such as alpha particles, beta particles and protons,<br />

(2) uncharged particles such as neutrons and<br />

(3) electromagnetic radiation in the form <strong>of</strong> X-rays and gamma rays.<br />

Charlie Chong/ Fion Zhang


Radiation Detection Systems<br />

Some forms <strong>of</strong> radiation, such as light and heat, can be detected by human<br />

sense organs; ionizing radiation, however, can be detected only by the after<br />

effect <strong>of</strong> itsionizing properties. If ionizing radiation does not interact with<br />

matter, its detection and measurement is impossible. For this reason, the<br />

detection process uses substances that respond to radiation, as part <strong>of</strong> a<br />

system for measuring the extent <strong>of</strong> that response. The ionization process<br />

isused by a large class <strong>of</strong> detection systems, including:<br />

■ ion chambers,<br />

■ proportional chambers,<br />

■ geiger-müller counters and<br />

■ semiconductor devices (Table 1).<br />

■ Some systems depend on the excitation and molecular dissociation<br />

( 分 子 离 解 ) that occur with ionization. These processes are useful in (1)<br />

scintillation counters and (2) chemical dosimeters. Although other types <strong>of</strong><br />

detection systems exist, they are not generally used in radiation survey<br />

instruments.<br />

Charlie Chong/ Fion Zhang


TABLE 1. Effect <strong>of</strong> detected and measured ionization.<br />

Charlie Chong/ Fion Zhang


PART 2. Ion Chambers and Proportional<br />

Counters<br />

Principles <strong>of</strong> Ionization<br />

The mechanism most widely used in radiation survey applications is the<br />

ionization principle: charged particles producing ion pairs by direct interaction.<br />

These charged particles may (1) collide with electrons and remove them from<br />

their atoms or (2) transfer energy to an electron by the interaction <strong>of</strong> their<br />

electric fields (Fig. 1). If the energy transfer is not sufficient to completely<br />

remove an electron, the atom is left in a disturbed or excited state.<br />

Gamma and X-ray photons interact with matter mainly by:<br />

■ photoelectric absorption,<br />

■ compton scattering and<br />

■ pair production,<br />

each <strong>of</strong> which produces electrons and ions that may be collected and<br />

measured.<br />

Charlie Chong/ Fion Zhang


The average energy expended in the creation <strong>of</strong> an ion pair, in air and most<br />

gases, is about 34 eV) .<br />

The number <strong>of</strong> ion pairs produced per unit <strong>of</strong> path length is called specific<br />

ionization. Specific ionization is affected by the energy <strong>of</strong> the particle or<br />

photon by its change and by the nature <strong>of</strong> the ionized substance.<br />

Charlie Chong/ Fion Zhang


FIGURE 1. Ion pair (showing ejected electron and vacancy in electron orbit <strong>of</strong><br />

atom).<br />

pair<br />

34 eV for Air<br />

Charlie Chong/ Fion Zhang


Ionization Chambers<br />

In an ionization chamber, an electric field is applied across a volume <strong>of</strong> gas,<br />

between two electrodes. Often the chamber’s geometry is cylindrical, a<br />

cylindrical cathode enclosing the gas and an axial, insulated rod anode<br />

(Fig. 2). Charged particles, photons or both pass through the chamber and<br />

ionize the enclosed gas. When an electric field is applied to the gas, ions drift<br />

along the electrical lines <strong>of</strong> force to produce an ionization current. Under<br />

normal conditions, electrons drift at speeds <strong>of</strong> about 104 m·s –1 (22 000 mi·h –1).<br />

The drift velocity <strong>of</strong> positive ions is many orders <strong>of</strong> magnitude less. When the<br />

electric field is increased slightly from zero and a detector is placed in the<br />

constant radiation field the collected ions still will be few in number because<br />

many recombine. As the voltage is further increased, recombination yields to<br />

ionization, where all ions are collected (Fig. 3).<br />

Charlie Chong/ Fion Zhang


FIGURE 2. Basic ionization chamber with high value resistance R and<br />

voltage V.<br />

Charlie Chong/ Fion Zhang


Electromagnetic Energy Interactions<br />

Photons interact with subatomic structures in one <strong>of</strong> the following three ways:<br />

•Photoelectric absorption<br />

•Compton Scatter<br />

•Pair production<br />

The particular type <strong>of</strong> interaction reflects probability statistics based on both<br />

the energy <strong>of</strong> the photon and the atomic number <strong>of</strong> the traversed atom. For<br />

most tissues <strong>of</strong> the body, average atomic number does not vary greatly –<br />

though cortical bone has the highest effective atomic number.<br />

Charlie Chong/ Fion Zhang<br />

https://www.med-ed.virginia.edu/courses/rad/radbiol/01physics/phys-03-02.html


Photoelectric Absorption<br />

An atom completely absorbs a photon, which then disappears; this excess<br />

energy provided to the atom ultimately results in ejection <strong>of</strong> an orbital electron.<br />

The ejected electron is known as a photo electron.<br />

Electrons have binding energies <strong>of</strong> orbit, with outer shells having less energy<br />

than those closer to the positive nucleus. When the initial orbital vacated is<br />

not that <strong>of</strong> an outer valance electron, the atom remains in a high-energy state<br />

until an outer orbital electron shifts to fill its incomplete inner shell. This shift is<br />

accompanied by emission <strong>of</strong> a characteristic X-ray.<br />

Photoelectric Absorption is an important interaction for low energy photons<br />

(


True or False?<br />

The "photo electron" and free radical can interact with other molecules --<br />

ultimately leading to ionizations and bond breakage, which are the<br />

biologically-important molecular manifestations <strong>of</strong> radiation damage.<br />

Charlie Chong/ Fion Zhang<br />

https://www.med-ed.virginia.edu/courses/rad/radbiol/01physics/phys-03-03.html


Compton Scatter<br />

Collision <strong>of</strong> a photon with an electron increases the kinetic energy <strong>of</strong> the<br />

electron. Thus set in motion, the electron is known as a recoil electron. The<br />

incident photon’s energy is not necessarily depleted, but it will diverge from its<br />

path and have lower energy -- i.e., it has a longer wavelength after collision.<br />

In diagnostic radiology, such scattered photons may lower contrast and thus<br />

degrade quality <strong>of</strong> the radiographic image.<br />

Important interaction for intermediate-energy photons (100 KeV to 10 MeV)<br />

Note:<br />

0.34 ~ 1.2 MeV (<strong>Exam</strong> Q)<br />

Charlie Chong/ Fion Zhang<br />

https://www.med-ed.virginia.edu/courses/rad/radbiol/01physics/phys-03-03.html


Compton Scatter<br />

Charlie Chong/ Fion Zhang<br />

https://www.med-ed.virginia.edu/courses/rad/radbiol/01physics/phys-03-03.html


Pair Production<br />

Note pair production requires relatively high photon energies that are<br />

generally not produced in diagnostic imaging.<br />

Photons with quantum energy in excess <strong>of</strong> 1.02 MeV (usually >10 MeV) may<br />

interact with matter to produce a negative electron and its anti-particle<br />

(positron). The value <strong>of</strong> 1.02 MeV equals the combination rest mass energy <strong>of</strong><br />

an electron and a positron.<br />

Charlie Chong/ Fion Zhang<br />

https://www.med-ed.virginia.edu/courses/rad/radbiol/01physics/phys-03-03.html


Pair Production<br />

0.51MeV<br />

0.51MeV<br />

Charlie Chong/ Fion Zhang<br />

https://www.med-ed.virginia.edu/courses/rad/radbiol/01physics/phys-03-03.html


Linear Energy Transfer [LET]<br />

LET is the amount <strong>of</strong> energy transferred to the local environment in the form<br />

<strong>of</strong> ionizations and excitations. Thus, LET indicates the potential for<br />

biologically important damage from radiation.<br />

Linear Energy Transfer can be thought <strong>of</strong> in two ways:<br />

• an average energy for a given path length traveled or<br />

• an average path length for a given deposited energy.<br />

The standard unit <strong>of</strong> measure is keV/um.<br />

Charlie Chong/ Fion Zhang<br />

https://www.med-ed.virginia.edu/courses/rad/radbiol/01physics/phys-03-03.html


Ionization tracts. When particulate or electromagnetic energy penetrates a<br />

cell, one or more ionizations will likely take place. While the precise site <strong>of</strong><br />

interaction is somewhat random, ionizations will distribute along distinct paths.<br />

The density <strong>of</strong> ionizations along a given path relates inversely to kinetic<br />

energy <strong>of</strong> the particle or photon.<br />

Thus a decelerating particle produces the greatest number <strong>of</strong> ionizations just<br />

before coming to rest. Comparing particles or photons, it follows also that LET<br />

for a gamma ray may be smaller than LET for an x-ray.<br />

Charlie Chong/ Fion Zhang<br />

https://www.med-ed.virginia.edu/courses/rad/radbiol/01physics/phys-03-03.html


Simulation <strong>of</strong> various radiation energies passing through a medium – each<br />

hatch mark represents an ionization. The heavy ion is a very high-LET<br />

particle; the delta ray represents secondary electrons with sufficient energy to<br />

make a separate ionization tract. The 5 keV electron is the typical energy <strong>of</strong> a<br />

secondary electron produced by X-ray photons used in diagnostic imaging.<br />

Note that absorption (and attenuation) <strong>of</strong> a photon beam is related to the<br />

atomic number <strong>of</strong> the impinged mass and inversely related to the energy <strong>of</strong><br />

the incident photon beam.<br />

The medium shown is approximately 200 nm in width – a DNA double helix<br />

width is about 2 nm.<br />

(Developed after Cox J.D. and Ang K.K., eds. Radiation Oncology Rationale,<br />

Technique, Results. 8th edition. St Louis, MO: Mosby, 2003. p44.)<br />

Charlie Chong/ Fion Zhang<br />

https://www.med-ed.virginia.edu/courses/rad/radbiol/01physics/phys-03-03.html


Simulation <strong>of</strong> various radiation energies passing through a medium<br />

Charlie Chong/ Fion Zhang<br />

https://www.med-ed.virginia.edu/courses/rad/radbiol/01physics/phys-03-03.html


Sources <strong>of</strong> Attenuation<br />

The attenuation that results due to the interaction between penetrating<br />

radiation and matter is not a simple process. A single interaction event<br />

between a primary x-ray photon and a particle <strong>of</strong> matter does not usually<br />

result in the photon changing to some other form <strong>of</strong> energy and effectively<br />

disappearing. Several interaction events are usually involved and the total<br />

attenuation is the sum <strong>of</strong> the attenuation due to different types <strong>of</strong> interactions.<br />

These interactions include the photoelectric effect, scattering, and pair<br />

production. The figure below shows an approximation <strong>of</strong> the total absorption<br />

coefficient, (µ), in red, for iron plotted as a function <strong>of</strong> radiation energy.<br />

The four radiation-matter interactions that contribute to the total absorption<br />

are shown in black. The four types <strong>of</strong> interactions are: photoelectric (PE),<br />

Compton scattering (C), pair production (PP), and Thomson or Rayleigh<br />

scattering (R). Since most industrial radiography is done in the 0.1 to 1.5 MeV<br />

range, it can be seen from the plot that photoelectric and Compton scattering<br />

account for the majority <strong>of</strong> attenuation encountered.<br />

Charlie Chong/ Fion Zhang<br />

https://www.nde-ed.org/EducationResources/CommunityCollege/<strong>Radiography</strong>/Physics/attenuation.htm


Total Absorption Coefficient, (µ),<br />

µ<br />

photoelectric (PE),<br />

Compton scattering (C),<br />

pair production (PP), and<br />

Thomson or Rayleigh scattering (R).<br />

Charlie Chong/ Fion Zhang


Charlie Chong/ Fion Zhang


Coherent scattering (also known as unmodified,<br />

classical or elastic scattering) is one <strong>of</strong> three forms <strong>of</strong> photon<br />

interaction which occurs when the energy <strong>of</strong> the X-ray or gamma photon is<br />

small in relation to the ionisation energy <strong>of</strong> the atom. It therefore occurs with<br />

low energy radiation.<br />

Upon interacting with the attenuating medium, the photon does not have<br />

enough energy to liberate the electron from its bound state (i.e. the photon<br />

energy is well below the binding energy <strong>of</strong> the electron) so no energy transfer<br />

occurs. The only change is a change <strong>of</strong> direction (scatter) <strong>of</strong> the photon,<br />

hence 'unmodified' scatter. Coherent scattering is not a major interaction<br />

process encountered in radiography at the energies normally used.<br />

Coherent scattering varies with the atomic number <strong>of</strong> absorber (Z) and<br />

incident photon energy (E) by Z 2 / E.<br />

Charlie Chong/ Fion Zhang<br />

http://radiopaedia.org/articles/coherent-scattering


Charlie Chong/ Fion Zhang<br />

http://radiopaedia.org/articles/coherent-scattering


Photoelectric effect, or photoelectric absorption (PEA)<br />

is a form <strong>of</strong> interaction <strong>of</strong> X-ray or gamma photon with the matter. A low<br />

energy photon interacts with the electron in the atom and removes it from its<br />

shell.<br />

The probability <strong>of</strong> this effect is maximum when:<br />

• the energy <strong>of</strong> the incident photon is equal to or just greater than the<br />

binding energy <strong>of</strong> the electron in its shell ('absorption edge') and<br />

• the electron is tightly bound (as in K shell)<br />

Charlie Chong/ Fion Zhang<br />

http://radiopaedia.org/articles/photoelectric-effect


The electron that is removed is then called a photoelectron. The incident<br />

photon is completely absorbed in the process. Hence it forms one <strong>of</strong> the<br />

reason for attenuation <strong>of</strong> X-ray beam as it passes through the matter.<br />

PEA is related to the atomic number <strong>of</strong> the attenuating medium (Z), the<br />

energy <strong>of</strong> the incident photon (E) and the physical density <strong>of</strong> the attenuating<br />

medium (p) by: Z³ p / E³.<br />

Therefore, if Z doubles, PEA will increase by a factor <strong>of</strong> 8 (because 2³ is 8)<br />

and if E doubles, PEA will reduce by 8. As small changes in Z can have quite<br />

pr<strong>of</strong>ound changes in PEA this has practical implications in the field <strong>of</strong><br />

radiation protection and is why materials with a high Z such as lead (Z = 82)<br />

are useful shielding materials.<br />

Charlie Chong/ Fion Zhang<br />

http://radiopaedia.org/articles/photoelectric-effect


The incident photon is<br />

completely absorbed<br />

in the process.<br />

Charlie Chong/ Fion Zhang


Photoelectric effect<br />

ABSORBED<br />

Charlie Chong/ Fion Zhang


Completely Heroes<br />

Charlie Chong/ Fion Zhang


Compton effect or Compton scatter is one <strong>of</strong> three principle<br />

forms <strong>of</strong> photon interaction. It is the main cause <strong>of</strong> scattered radiation in a<br />

material. It occurs due to the interaction <strong>of</strong> the X-ray or gamma photon with<br />

the outermost (and hence loosely bound) valence electron at the atomic level.<br />

The resultant incident photon gets scattered (changes direction) as well as<br />

ejects the electron (recoil electron), which further ionizes other atoms.<br />

Therefore the Compton effect is a partial absorption process and as the<br />

original photon has lost energy, this is known as Compton shift (the shift<br />

being a shift <strong>of</strong> wavelength/frequency).<br />

Probability <strong>of</strong> Compton effect:<br />

• directly proportional to<br />

• number <strong>of</strong> outer shell electrons, i.e. the electron density<br />

• physical density <strong>of</strong> material<br />

• inversely proportional to<br />

• photon energy<br />

• does not depend on<br />

• atomic number (unlike photoelectric effect and pair production)<br />

Charlie Chong/ Fion Zhang<br />

http://radiopaedia.org/articles/compton-effect


History and etymology<br />

Named after Pr<strong>of</strong>essor Arthur Holly Compton (1892-<br />

1962), US physicist, who was awarded the Nobel Prize<br />

in Physics in 1927 for his discovery <strong>of</strong> Compton effect.<br />

Charlie Chong/ Fion Zhang


Charlie Chong/ Fion Zhang


Pair production (PP), like the photoelectric effect, results in the<br />

complete attenuation <strong>of</strong> the incident photon. Pair production can only occur if<br />

the incident photon energy is at least 1.022 MeV. As the photon interacts with<br />

the strong electric field around the nucleus it undergoes a change <strong>of</strong> state and<br />

is transformed into two particles (essentially creating matter from energy):<br />

■ one electron<br />

■ one positron (antimatter equivalent <strong>of</strong> the electron)<br />

These two particles form the pair referred to in the name <strong>of</strong> the process. It is<br />

noteworthy that other 'pairs' <strong>of</strong> leptons (<strong>of</strong> which the electron is a type) can be<br />

created such as muon - antimuon and tau - antitau pairs, however the type <strong>of</strong><br />

lepton pair would dictate the energy <strong>of</strong> the incident photon necessary to<br />

create them as both have far higher resting energy masses (1776 MeV for the<br />

tau and 105 MeV for the muon) than the electron and positron.<br />

Charlie Chong/ Fion Zhang<br />

http://radiopaedia.org/articles/pair-production


The reason at least 1.022 MeV <strong>of</strong> photon energy is necessary is because the<br />

resting mass (using E=MC² ) <strong>of</strong> the electron and positron expressed in units<br />

<strong>of</strong> energy is 0.511 MeV (or 9.1 x 10 -31 kg) each, therefore unless there is at<br />

least 0.511 MeV *2 (i.e., 1.022 MeV) it is not possible for the electron-positron<br />

pair to be created. If the energy <strong>of</strong> the incident photon is greater than 1.022<br />

MeV, the excess is shared (although not always equally) between the<br />

electron and positron as kinetic energy.<br />

PP is related to the atomic number (Z) <strong>of</strong> attenuator, incident photon energy<br />

(E) and physical density (p) by Z E p.<br />

Charlie Chong/ Fion Zhang<br />

http://radiopaedia.org/articles/pair-production


The electron and positron, once liberated within the medium are dissipated<br />

through successive interactions within the medium. The electron is quickly<br />

absorbed, however the fate <strong>of</strong> the positron is not so straight forward. As it<br />

comes to a rest, it combines with a neighbouring electron and the two<br />

particles neutralise each other in a phenomenon known as annihilation<br />

radiation. Here, the two particles are converted back into two photons <strong>of</strong><br />

electromagnetic radiation, each <strong>of</strong> 0.511 MeV energy travelling at 180<br />

degrees to each other (a concept utilised in positron emission tomography -<br />

PET). These photons are then absorbed or scattered within the medium.<br />

Pair production in reality does not become the dominant process in water<br />

below about 30 MeV (due to its dependence on the 'Z' <strong>of</strong> absorber) and is<br />

therefore <strong>of</strong> less importance in the low atomic number s<strong>of</strong>t tissue elements. In<br />

industrial radiography where high atomic number elements are irradiated, pair<br />

production can become the major attenuation process assuming the incident<br />

radiation energy exceeds 1.022 MeV.<br />

Charlie Chong/ Fion Zhang<br />

http://radiopaedia.org/articles/pair-production


Pair Production<br />

Charlie Chong/ Fion Zhang


Summary <strong>of</strong> different mechanisms that cause<br />

attenuation <strong>of</strong> an incident x-ray beam<br />

Photoelectric (PE) absorption <strong>of</strong> x-rays occurs when the x-ray photon is<br />

(totally) absorbed, resulting in the ejection <strong>of</strong> electrons from the outer shell <strong>of</strong><br />

the atom, and hence the ionization <strong>of</strong> the atom. Subsequently, the ionized<br />

atom returns to the neutral state with the emission <strong>of</strong> an x-ray characteristic <strong>of</strong><br />

the atom. This subsequent emission <strong>of</strong> lower energy photons is generally<br />

absorbed and does not contribute to (or hinder) the image making process.<br />

Photoelectron absorption is the dominant process for x-ray absorption up to<br />

energies <strong>of</strong> about 500 KeV (


Photoelectric (PE) absorption<br />

Photoelectric (PE) absorption <strong>of</strong> x-rays<br />

occurs when the x-ray photon is (totally)<br />

absorbed, resulting in the ejection <strong>of</strong><br />

electrons from the outer shell <strong>of</strong> the<br />

atom.<br />

Charlie Chong/ Fion Zhang


Effect <strong>of</strong> Photon Energy on Attenuation<br />

Absorption characteristics will increase or decrease as the energy <strong>of</strong> the x-<br />

ray is increased or decreased. Since attenuation characteristics <strong>of</strong> materials<br />

are important in the development <strong>of</strong> contrast in a radiograph, an<br />

understanding <strong>of</strong> the relationship between material thickness, absorption<br />

properties, and photon energy is fundamental to producing a quality<br />

radiograph. A radiograph with higher contrast will provide greater probability<br />

<strong>of</strong> detection <strong>of</strong> a given discontinuity. An understanding <strong>of</strong> absorption is also<br />

necessary when designing x-ray and gamma ray shielding, cabinets, or<br />

exposure vaults.<br />

The applet below can be used to investigate the effect that photon energy has<br />

on the type <strong>of</strong> interaction that the photon is likely to have with a particle <strong>of</strong> the<br />

material (shown in gray). Various materials and material thicknesses may be<br />

selected and the x-ray energy can be set to produce a range from 1 to 199<br />

KeV. Notice as various experiments are run with the applets that low energy<br />

radiation produces predominately photoelectric events and higher energy x-<br />

rays produce predominately Compton scattering events. Also notice that if the<br />

energy is too low, none <strong>of</strong> the radiation penetrates the material.<br />

Charlie Chong/ Fion Zhang


This second applet is similar to the one above except that the voltage (KVp)<br />

for a typical generic x-ray tube source can be selected. The applet displays<br />

the spectrum <strong>of</strong> photon energies (without any filtering) that the x-ray source<br />

produces at the selected voltage. Pressing the "Emit X-ray" button will show<br />

the interaction that will occur from one photon with an energy within the<br />

spectrum. Pressing the "Auto" button will show the interactions from a large<br />

number <strong>of</strong> photos with energies within the spectrum.<br />

Charlie Chong/ Fion Zhang


More <strong>Reading</strong> on: Photoelectric effect<br />

The photoelectric effect is the emission <strong>of</strong> electrons from matter upon the<br />

absorption <strong>of</strong> electromagnetic radiation, such as ultraviolet radiation or x-rays.<br />

Upon exposing a metallic surface to electromagnetic radiation that is above<br />

the threshold frequency or threshold wavelength (absorption edge?) (which is<br />

specific to the type <strong>of</strong> surface and material), the photons are absorbed and<br />

current is produced.<br />

No electrons are emitted for radiation with a frequency below that <strong>of</strong> the<br />

threshold, as the electrons are unable to gain sufficient energy to overcome<br />

the electrostatic barrier presented by the termination <strong>of</strong> the crystalline surface.<br />

By conservation <strong>of</strong> energy, the energy <strong>of</strong> the photon is absorbed by the<br />

electron and, if sufficient, the electron can escape from the material with a<br />

finite kinetic energy.<br />

A single photon can only eject a single electron, as the energy <strong>of</strong> one photon<br />

may only be absorbed by one electron.<br />

The electrons that are emitted are <strong>of</strong>ten termed photoelectrons.<br />

Charlie Chong/ Fion Zhang<br />

https://www.sciencedaily.com/terms/photoelectric_effect.htm


Photoelectric effect, or photoelectric absorption (PEA)<br />

is a form <strong>of</strong> interaction <strong>of</strong> X-ray or gamma photon with the matter. A low<br />

energy photon interacts with the electron in the atom and removes it from its<br />

shell.<br />

The probability <strong>of</strong> this effect is maximum when:<br />

• the energy <strong>of</strong> the incident photon is equal to or just greater than the<br />

binding energy <strong>of</strong> the electron in its shell ('absorption edge') and<br />

• the electron is tightly bound (as in K shell) (?)<br />

Charlie Chong/ Fion Zhang<br />

http://radiopaedia.org/articles/photoelectric-effect


The electron that is removed is then called a photoelectron. The incident<br />

photon is completely absorbed in the process. Hence it forms one <strong>of</strong> the<br />

reason for attenuation <strong>of</strong> X-ray beam as it passes through the matter.<br />

PEA is related to the atomic number <strong>of</strong> the attenuating medium (Z), the<br />

energy <strong>of</strong> the incident photon (E) and the physical density <strong>of</strong> the attenuating<br />

medium (ρ) by:<br />

PEA ∝ Z³ ·ρ / E³.<br />

Therefore, if Z doubles, PEA will increase by a factor <strong>of</strong> 8 (because 2³ is 8)<br />

and if E doubles, PEA will reduce by 8. As small changes in Z can have quite<br />

pr<strong>of</strong>ound changes in PEA this has practical implications in the field <strong>of</strong><br />

radiation protection and is why materials with a high Z such as lead (Z = 82)<br />

are useful shielding materials.<br />

Charlie Chong/ Fion Zhang<br />

http://radiopaedia.org/articles/photoelectric-effect


First principle mechanism <strong>of</strong> ionization<br />

The photoelectric effect <strong>of</strong> ionization involves the complete absorption <strong>of</strong> the<br />

photon energy during the process <strong>of</strong> knocking an electron out <strong>of</strong> orbit. This<br />

process primarily occurs with low energy photons ranging in energy between<br />

10 Kev and less than 500 Kev. (0.01~0.5MeV)<br />

Notice in the above illustration that an ion pair is created in the interaction<br />

between the radiation photon and the atom. During this process, when the<br />

photon liberates the electron, all <strong>of</strong> the photon s energy is transferred to create<br />

the ion pair and total absorption has occurred. Remember, there is a binding<br />

force that the holds the electron in its orbital shell. The amount <strong>of</strong> energy<br />

required to create the ion pair must be at least equal to this binding force.<br />

Charlie Chong/ Fion Zhang<br />

https://www.nde-ed.org/EducationResources/HighSchool/<strong>Radiography</strong>/photoelectric_popup.htm


If during the ionization process, only part <strong>of</strong> the photons energy is needed to<br />

liberate the electron, the rest <strong>of</strong> the energy is transferred to the electron in the<br />

form <strong>of</strong> speed (velocity). Now that all <strong>of</strong> the photon's energy is accounted for,<br />

the photon ceases to exist and total absorption has occurred. Remember that<br />

a photon is not a particle, but acts like one. When the energy <strong>of</strong> the photon is<br />

used, there is nothing left to cause further ionization.<br />

Keep in mind that electrons orbit in various shells <strong>of</strong> the atom and not all<br />

electrons have the same binding energy. This binding energy is dependent<br />

upon the elements (Z) number and the position <strong>of</strong> the electron in the atom.<br />

Those electrons nearer the nucleus possess greater binding energy and will<br />

require greater photon energy to remove them than will electrons in the outer<br />

shells.<br />

Charlie Chong/ Fion Zhang<br />

https://www.nde-ed.org/EducationResources/HighSchool/<strong>Radiography</strong>/photoelectric_popup.htm


Photoelectron Spectroscopy<br />

Charlie Chong/ Fion Zhang<br />

http://jahschem.wikispaces.com/Photoelectron+Spectroscopy


Photoelectron Spectroscopy<br />

Charlie Chong/ Fion Zhang<br />

http://www.met.reading.ac.uk/pplato2/h-flap/phys8_3.html


Photoelectron Spectroscopy<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikibooks.org/wiki/Basic_Physics_<strong>of</strong>_Digital_<strong>Radiography</strong>/The_Source


Photodisintegration (PD) is the process by which the x-ray photon is<br />

captured by the nucleus <strong>of</strong> the atom with the ejection <strong>of</strong> a particle from the<br />

nucleus when all the energy <strong>of</strong> the x-ray is given to the nucleus. Because <strong>of</strong><br />

the enormously high energies involved, this process may be neglected for the<br />

energies <strong>of</strong> x-rays used in radiography. (this photodisintegration to be<br />

distinguishes from photo annihilation <strong>of</strong> positron/electron pair)<br />

Charlie Chong/ Fion Zhang<br />

https://www.nde-ed.org/EducationResources/CommunityCollege/<strong>Radiography</strong>/Physics/attenuation.htm


Thomson scattering (R), also known as Rayleigh, coherent, or classical<br />

scattering, occurs when the x-ray photon interacts with the whole atom so<br />

that the photon is scattered with no change in internal energy to the scattering<br />

atom, nor to the x-ray photon. Thomson scattering is never more than a minor<br />

contributor to the absorption coefficient. The scattering occurs without the<br />

loss <strong>of</strong> energy. Scattering is mainly in the forward direction.<br />

Charlie Chong/ Fion Zhang<br />

https://www.nde-ed.org/EducationResources/CommunityCollege/<strong>Radiography</strong>/Physics/attenuation.htm


FIGURE 3. Pulse size as function <strong>of</strong> voltage in gas ion chamber.<br />

Charlie Chong/ Fion Zhang


Ion current chambers have a response magnitude proportional to<br />

the absorbed energy and are therefore widely used for making dose<br />

measurements.<br />

When (1) recombination is negligible, (2) gas amplification does not occur<br />

and (3) all other charges are efficiently collected, then the steady state current<br />

produced is an accurate measurement <strong>of</strong> the rate at which ion pairs are<br />

formed within the gas.<br />

Measurement <strong>of</strong> this ionization current is the principle behind the direct<br />

current ion chamber. Ion chambers may be constructed <strong>of</strong> several different<br />

materials and, because radiation must penetrate the wall <strong>of</strong> the chamber to<br />

ionize the gas volume, chambers are chosen for the specific radiation energy<br />

being evaluated. When considering a particular instrument the energy<br />

response curve should always be consulted (Fig. 4). Some instruments may<br />

also have an angular dependence (more sensitivity in some directions), which<br />

should also be considered when making measurements. Radio frequency<br />

shielded ionization chambers are available for measurements made near high<br />

level radio frequency sources.<br />

Charlie Chong/ Fion Zhang


FIGURE 3. Pulse size as function <strong>of</strong> voltage in gas ion chamber.<br />

Charlie Chong/ Fion Zhang


FIGURE 4. Energy and directional response <strong>of</strong> typical ion chamber survey<br />

meters: (a) example <strong>of</strong> response curve; (b) comparison <strong>of</strong> several response<br />

curves.<br />

Charlie Chong/ Fion Zhang


FIGURE 4. Energy and directional response <strong>of</strong> typical ion chamber survey<br />

meters: (a) example <strong>of</strong> response curve; (b) comparison <strong>of</strong> several response<br />

curves.<br />

Legend<br />

Charlie Chong/ Fion Zhang


Ionization Chambers<br />

Charlie Chong/ Fion Zhang


Ionization Chambers<br />

Charlie Chong/ Fion Zhang


Compton scattering (C) (incoherent scattering)<br />

occurs when the incident x-ray photon is deflected from its original path by an<br />

interaction with an electron. The electron gains energy and is ejected from its<br />

orbital position. The x-ray photon loses energy due to the interaction but<br />

continues to travel through the material along an altered path. Since the<br />

scattered x-ray photon has less energy, it, therefore, has a longer wavelength<br />

than the incident photon. The event is also known as incoherent scattering<br />

because the photon energy change resulting from an interaction is not always<br />

orderly and consistent. The energy shift depends on the angle <strong>of</strong> scattering<br />

and not on the nature <strong>of</strong> the scattering medium<br />

Charlie Chong/ Fion Zhang<br />

https://www.nde-ed.org/EducationResources/CommunityCollege/<strong>Radiography</strong>/Physics/attenuation.htm


Pair production (PP) can occur when the x-ray photon energy is greater than<br />

1.02 MeV, but really only becomes significant at energies around 10 MeV.<br />

Pair production occurs when an electron and positron are created with the<br />

annihilation <strong>of</strong> the x-ray photon. Positrons are very short lived and disappear<br />

(positron annihilation) with the formation <strong>of</strong> two photons <strong>of</strong> 0.51 MeV energy.<br />

Pair production is <strong>of</strong> particular importance when high-energy photons pass<br />

through materials <strong>of</strong> a high atomic number. (single photon for single pair<br />

production or single high energy photon for multiple pair production?)<br />

Charlie Chong/ Fion Zhang<br />

https://www.nde-ed.org/EducationResources/CommunityCollege/<strong>Radiography</strong>/Physics/attenuation.htm


Output Current Measurements<br />

The ionization current collected in the ion chamber flows through an external<br />

circuit for measurement. Although in principle an ammeter could be placed in<br />

the external circuit to read the ion current, in practice the ammeter is not<br />

placed there, for the current is very small.<br />

A 440 cm 3 (27 in. 3 ) ion chamber typically produces about 4 × 10 –15 A·μSv –1<br />

(4 × 10 –14 A·mR –1 ) at standard temperature and pressure.<br />

A high valued load resistor (on the order <strong>of</strong> 10 10 Ω) is placed in the circuit and<br />

the voltage drop across the resistor is measured with a sensitive electrometer.<br />

A metal oxide silicon field effect transistor (MOSFET) is used in some<br />

electrometers. The metal oxide silicon field effect transistor produces an input<br />

impedance on the order <strong>of</strong> 10 15 Ω to amplify the collected current (Fig. 5).<br />

Charlie Chong/ Fion Zhang


FIGURE 5. Operational configuration <strong>of</strong> current amplifier.<br />

Charlie Chong/ Fion Zhang


Vibrating Reed Electrometers<br />

An alternative approach to ion current measurement is to convert the signal<br />

from direct current to alternating current at an early stage. This allows a more<br />

stable amplification <strong>of</strong> the alternating current signal in subsequent operations.<br />

The conversion is accomplished in a dynamic capacitor or vibrating reed<br />

electrometer, by collecting the ion current across a resistive capacitive circuit.<br />

The capacitance is then changed rapidly, compared to the time constant <strong>of</strong><br />

the circuit. The induced alternating current voltage is proportional to the<br />

ionization current (Fig. 6).<br />

Charlie Chong/ Fion Zhang


FIGURE 6. Principle <strong>of</strong> vibrating reed electrometer; oscillations <strong>of</strong><br />

capacitance induce alternating current voltage proportional to steady state<br />

signal current.<br />

Charlie Chong/ Fion Zhang


Vibrating Reed Electrometers<br />

Cary Vibrating Reed Electrometer with Ionization Chamber ( late 1950s)<br />

Charlie Chong/ Fion Zhang<br />

https://www.orau.org/PTP/collection/ionchamber/vibratingreedion.htm


Cary Vibrating Reed Electrometer with Ionization Chamber ( late 1950s)<br />

The spherical ion chamber,<br />

electrometer head, and amplifier were<br />

made by Applied Physics Corporation<br />

<strong>of</strong> Pasadena, California. The Model 31,<br />

which replaced the Model 30, was<br />

introduced in 1957/1958 and seems to<br />

have been superceded by the Model 32<br />

in 1959 This system would have been<br />

used to measure the activity <strong>of</strong><br />

chemically unreactive gases such as<br />

krypton, xenon, CO2 and HT. Either the<br />

gas being analyzed would flow through<br />

the chamber or be held inside the<br />

chamber for the duration <strong>of</strong> the<br />

measurement.<br />

Charlie Chong/ Fion Zhang<br />

https://www.orau.org/PTP/collection/ionchamber/vibratingreedion.htm


The weak current generated in the chamber (less than 10 -12 amperes) was<br />

converted into an alternating current by the vibrating reed in the electrometer<br />

head. The AC current was then amplified and fed to a strip chart recorder.<br />

The electrometer readout employed multiple scales and measured up to 30<br />

volts.<br />

The spherical ion chamber, shown to the right, is connected directly to the<br />

electrometer head. Made <strong>of</strong> stainless steel, it is approximately 3" in diameter<br />

and has a 250 ml volume. The original version <strong>of</strong> the chamber was made <strong>of</strong><br />

Pyrex. The reed, a thin metal plate, was vibrated by an electromagnet at<br />

frequency <strong>of</strong> 450 cycles per second. The reed also formed part <strong>of</strong> a capacitor<br />

onto which the current from the chamber was sent. The cyclical movement <strong>of</strong><br />

the reed resulted in a fluctuating capacitance and the generation <strong>of</strong> an<br />

alternating current. The advantage the AC signal had over the original DC<br />

signal was that the former could be amplified much more reliably.<br />

Charlie Chong/ Fion Zhang<br />

https://www.orau.org/PTP/collection/ionchamber/vibratingreedion.htm


An electrometer is an electrical instrument for measuring electric<br />

charge or electrical potential difference. There are many different types,<br />

ranging from historical handmade mechanical instruments to high-precision<br />

electronic devices. Modern electrometers based on vacuum tube or solidstate<br />

technology can be used to make voltage and charge measurements<br />

with very low leakage currents, down to 1 femtoampere. A simpler but related<br />

instrument, the electroscope, works on similar principles but only indicates<br />

the relative magnitudes <strong>of</strong> voltages or charges.<br />

Charlie Chong/ Fion Zhang


Older electrometers<br />

Gold-leaf electroscope<br />

The gold-leaf electroscope was one <strong>of</strong> the first sensitive instruments used to<br />

indicate electric charge. It is still used for science demonstrations but has<br />

been superseded in most applications by electronic measuring instruments.<br />

The instrument consists <strong>of</strong> two thin leaves <strong>of</strong> gold foil suspended from an<br />

electrode. When the electrode is charged by induction or by contact, the<br />

leaves acquire similar electric charges and repel each other due to the<br />

Coulomb force. Their separation is a direct indication <strong>of</strong> the net charge stored<br />

on them. On the glass opposite the leaves, pieces <strong>of</strong> tin foil may be pasted,<br />

so that when the leaves diverge fully they may discharge into the ground. The<br />

leaves may be enclosed in a glass envelope to protect them from drafts, and<br />

the envelope may be evacuated to minimize charge leakage.<br />

A further cause <strong>of</strong> charge leakage is ionizing radiation, so to prevent this, the<br />

electrometer must be surrounded by lead shielding. This principle has been<br />

used to detect ionizing radiation, as seen in the quartz fibre electrometer and<br />

Kearny fallout meter.<br />

Charlie Chong/ Fion Zhang


This type <strong>of</strong> electroscope usually acts as an indicator and not a measuring<br />

device, although it can be calibrated. The Braun[dubious electroscope<br />

replaced [when?] the gold-leaf electroscope for more accurate measurements.<br />

The instrument was developed in the 18th century by several researchers,<br />

among them Abraham Bennet and Alessandro Volta.<br />

Charlie Chong/ Fion Zhang


Charlie Chong/ Fion Zhang<br />

Volta Electrometers


Kolbe electrometer, precision form <strong>of</strong> goldleaf<br />

instrument. This has a light pivoted<br />

aluminum vane hanging next to a vertical<br />

metal plate. When charged the vane is<br />

repelled by the plate and hangs at an angle.<br />

Charlie Chong/ Fion Zhang


Gold-leaf electroscope<br />

Charlie Chong/ Fion Zhang


Modern electrometers<br />

A modern electrometer is a highly sensitive electronic voltmeter whose input<br />

impedance is so high that the current flowing into it can be considered, for<br />

most practical purposes, to be zero. The actual value <strong>of</strong> input resistance for<br />

modern electronic electrometers is around 10 14 Ω, compared to around 10 10 Ω<br />

for nanovoltmeters. Owing to the extremely high input impedance, special<br />

design considerations must be applied to avoid leakage current such as<br />

driven shields and special insulation materials.<br />

Among other applications, electrometers are used in nuclear physics<br />

experiments as they are able to measure the tiny charges left in matter by the<br />

passage <strong>of</strong> ionizing radiation. The most common use for modern<br />

electrometers is the measurement <strong>of</strong> radiation with ionization chambers, in<br />

instruments such as Geiger counters.<br />

Charlie Chong/ Fion Zhang


Vibrating reed electrometers<br />

Vibrating reed electrometers use a variable capacitor formed between a<br />

moving electrode (in the form <strong>of</strong> a vibrating reed) and a fixed input electrode.<br />

As the distance between the two electrodes varies, the capacitance also<br />

varies and electric charge is forced in and out <strong>of</strong> the capacitor. The alternating<br />

current signal produced by the flow <strong>of</strong> this charge is amplified and used as an<br />

analogue for the DC voltage applied to the capacitor. The DC input resistance<br />

<strong>of</strong> the electrometer is determined solely by the leakage resistance <strong>of</strong> the<br />

capacitor, and is typically extremely high, (although its AC input impedance is<br />

lower).<br />

For convenience <strong>of</strong> use, the vibrating reed assembly is <strong>of</strong>ten attached by a<br />

cable to the rest <strong>of</strong> the electrometer. This allows for a relatively small unit to<br />

be located near the charge to be measured while the much larger reed-driver<br />

and amplifier unit can be located wherever it is convenient for the operator.<br />

Charlie Chong/ Fion Zhang


Integrating Instruments<br />

The instruments described above (Fig. 7) are generally rate meters; that is,<br />

they indicate the radiation at the time <strong>of</strong> exposure and, depending on its time<br />

constant, will return to background levels as the source is removed. Some<br />

instruments may have an integration switch that introduces a capacitor to the<br />

circuit to accumulate the charge. Leaving such an instrument at an operator’s<br />

location will indicate the total amount <strong>of</strong> ionizing radiation that area has<br />

received, from the time the instrument is engaged.<br />

Charlie Chong/ Fion Zhang


FIGURE 7. <strong>Exam</strong>ples <strong>of</strong> ionization chambers located externally on survey<br />

instruments. Protective caps are removed, showing thin windows for low<br />

energy X-ray or beta detection.<br />

Charlie Chong/ Fion Zhang


Personnel Monitoring Instruments<br />

Pocket Chambers<br />

Personnel monitoring instruments, some the size <strong>of</strong> a ball point pen, are<br />

usually the integrating type and contain an ionization chamber. One version,<br />

the pocket chamber, requires the application <strong>of</strong> an initial charge <strong>of</strong> 150 to 200<br />

V by an external instrument. Zero dose is then indicated on a scale contained<br />

in the charging unit. Exposure <strong>of</strong> the chamber to ionization decreases the<br />

initial charge. When the chamber is reconnected to the charging unit the<br />

reduced charge is translated to the level <strong>of</strong> exposure (Fig. 8).<br />

Charlie Chong/ Fion Zhang


FIGURE 8. Cross section <strong>of</strong> quartz fiber pocket dosimeter.<br />

Legend<br />

1. Low atomic number wall<br />

2. Graphite coated paper shell<br />

3. Aluminum terminal head<br />

4. Aluminum terminal sleeve<br />

5. Polystyrene support bushing<br />

6. Central electrode, graphite coated<br />

7. Polyethylene insulating washer<br />

8. Polystyrene fixed bushing<br />

9. Electrode contact<br />

10. Retaining ring<br />

11. Aluminum base cap<br />

12. Polyethylene friction bushing<br />

Charlie Chong/ Fion Zhang


Quartz Fiber Pocket Dosimeter.<br />

Charlie Chong/ Fion Zhang


Quartz Fiber Pocket Dosimeter.<br />

Charlie Chong/ Fion Zhang<br />

https://www.nde-ed.org/EducationResources/CommunityCollege/RadiationSafety/Graphics/DOSE.gif


Quartz Fiber Pocket Dosimeter.<br />

Charlie Chong/ Fion Zhang


Quartz Fiber Pocket Dosimeter.<br />

Charlie Chong/ Fion Zhang


Pocket Chambers and Pocket Dosimeters<br />

Paul Frame, Oak Ridge Associated Universities<br />

Pocket chambers and pocket dosimeters are small ionization chambers that,<br />

as the name implies, are usually worn in the pocket. While they were<br />

designed to measure x-rays and gamma ray exposures, they would also<br />

respond to betas above 1 MeV. <strong>Neutron</strong>-sensitive versions were also<br />

available. The terms pocket chamber and pocket dosimeter are <strong>of</strong>ten used<br />

interchangeably. The original distinction between the two terms, used here, is<br />

rarely made anymore. In part, this is due to the fact that the devices that I call<br />

pocket chambers are rarely used any more.<br />

Note:<br />

pocket dosimeter is an ion chamber type.<br />

Charlie Chong/ Fion Zhang<br />

http://www.orau.org/ptp/collection/dosimeters/pocketchamdos.htm


Quartz Fiber Pocket Dosimeter.<br />

Charlie Chong/ Fion Zhang<br />

http://www.orau.org/ptp/collection/dosimeters/pocketchamdos.htm


1. Pocket Chambers<br />

Pocket chambers go by a variety <strong>of</strong> names: indirect-reading dosimeters, nonself-reading<br />

dosimeters and condenser-type pocket dosimeters. Prior to WW<br />

II, they were only used to a limited extent, primarily in medical facilities and<br />

around accelerators. The Manhattan Project however created a huge demand<br />

and they were worn by almost everyone who might be exposed to radiation.<br />

A pocket chamber acts as an air-filled condenser (capacitor) much like the<br />

thimble chambers used in radiology. Prior to being worn, it is given a charge<br />

with a charger-reader, e.g., the Victoreen Minometer. Any subsequent<br />

exposure to radiation ionizes the air inside the chamber and this reduces the<br />

stored charge. In order to quantify the exposure, the charge is measured and<br />

the decrease is related to the exposure.<br />

Charlie Chong/ Fion Zhang<br />

http://www.orau.org/ptp/collection/dosimeters/pocketchamdos.htm


Manhattan Project<br />

Charlie Chong/ Fion Zhang<br />

http://www.orau.org/ptp/collection/dosimeters/pocketchamdos.htm


Manhattan Project<br />

Charlie Chong/ Fion Zhang


Manhattan Project<br />

Charlie Chong/ Fion Zhang


Manhattan Project<br />

Charlie Chong/ Fion Zhang


Charlie Chong/ Fion Zhang


Manhattan Project<br />

Charlie Chong/ Fion Zhang


Manhattan Project<br />

Charlie Chong/ Fion Zhang


Manhattan Project Director<br />

J Robert Oppenheimer<br />

Charlie Chong/ Fion Zhang


WWII<br />

Charlie Chong/ Fion Zhang


Ion Chamber Charger<br />

& Reader<br />

PP-630(A)/PD Dosimeter Charger<br />

(ca. 1954-1961)<br />

The PP-630 (A)/PD Dosimeter<br />

Charger is the military equivalent <strong>of</strong><br />

the Keleket Model 430A chargerreader<br />

which was advertised as<br />

early as 1954. Since this PP-630(A)<br />

has "August 29 1961" stamped on it,<br />

I assume that it probably dates from<br />

1954 to 1961. Unfortunately I have<br />

not been able to locate any specific<br />

references to the PP-630A/PD.<br />

Charlie Chong/ Fion Zhang<br />

http://www.orau.org/ptp/collection/radiac/PP630.htm


Ion Chamber Charger & Reader<br />

Radiac Computer-Indicator CP-95A/PD is designed as a portable radiac computer-indicator, for computing & indicating the total amount <strong>of</strong> X and gamma radiation to which Radiac Detector<br />

DT-60()/PD has been exposed (and thus revealing the X and gamma radiation to which the wearer <strong>of</strong> the DT-60()/PD had been exposed). The CP-95A/PD operates in conjunction with<br />

Radiac Detector DT-60()/PD (not supplied) which contains a specially compounded silver-actuated phosphor glass. When the total radiation dosage <strong>of</strong> a DT-60()/PD is to be measured, the<br />

DT-60()/D is placed in Radiac Computer-Indicator C-95A/PD and exposed to a source <strong>of</strong> ultraviolet light. The ultraviolet light causes the silver-activated glass to emit an orange<br />

luminescence, the intensity <strong>of</strong> which is proportional to the total amount <strong>of</strong> radiation the glass has received. The intensity <strong>of</strong> the orange luminescence is measured by a photomultiplier tube<br />

which is fitted with a filter to prohibit the passage <strong>of</strong> blue and green light. The photomultiplier tube employs the principle <strong>of</strong> secondary emission to amplify the initial electron emission caused<br />

by the filtered orange illumination <strong>of</strong> the light-sensitive cathode. The output <strong>of</strong> the photomultiplier tube is applied to an indicating circuit to indicate the total amount <strong>of</strong> radiation to which the<br />

wearer <strong>of</strong> the DT60()/PD has been exposed.<br />

Charlie Chong/ Fion Zhang<br />

http://www.orau.org/ptp/collection/radiac/CP95APD.htm


Pocket chambers were approximately 4 - 5" long and 0.5" in diameter. An<br />

aluminum rod (ca. 0.0625” in diameter) running along the chamber axis<br />

served as one electrode, while the outer wall <strong>of</strong> the chamber served as the<br />

other electrode. The central electrode was suspended at each end with a<br />

polystyrene insulator and at one end it penetrated the insulator to serve as<br />

the charging contact. One problem with the early models involved the<br />

threaded caps that were used to protect the charging contact - they would<br />

wear and the metal fragments would get on the insulator. The graphite<br />

coating on the inside <strong>of</strong> the chamber wall caused a similar type <strong>of</strong> problem<br />

with some <strong>of</strong> the early models because it would sometimes flake <strong>of</strong>f and short<br />

out the chamber. The early models were also susceptible to discharge as a<br />

result <strong>of</strong> mechanical shock because the central electrode would flex and<br />

contact the chamber wall. To solve this problem, later versions used a thicker<br />

central electrode and/or positioned a small insulating disk in the center <strong>of</strong> the<br />

electrode. Because <strong>of</strong> these problems, it was usual for a worker to wear two<br />

dosimeters and the lower <strong>of</strong> the two readings was considered the most<br />

accurate.<br />

Charlie Chong/ Fion Zhang<br />

http://www.orau.org/ptp/collection/dosimeters/pocketchamdos.htm


Quartz Fiber Pocket Dosimeter.<br />

Charlie Chong/ Fion Zhang<br />

http://www.orau.org/ptp/collection/dosimeters/pocketchamdos.htm


2. Pocket Dosimeters (quartz fiber electroscopes)<br />

Like pocket chambers, pocket dosimeters are known by a number <strong>of</strong> other<br />

names, e.g., direct-reading dosimeters, self-reading pocket dosimeters and<br />

pocket electroscopes. They are actually quartz fiber electroscopes the<br />

sensing element <strong>of</strong> which is a movable bow-shaped quartz fiber that is<br />

attached at each end to a fixed post. The latter is also shaped like a bow (or<br />

horseshoe). The dose is determined by looking through the eyepiece on one<br />

end <strong>of</strong> the dosimeter, pointing the other end towards a light source, and<br />

noting the position <strong>of</strong> the fiber on a scale. Until 1950 or so, the vast majority <strong>of</strong><br />

pocket dosimeters had a range up to 200 mR, although a few high range<br />

versions were available for emergency situations. Higher range versions<br />

became more readily available in the 1950s for military and civil defense<br />

purposes.<br />

Charlie Chong/ Fion Zhang<br />

http://www.orau.org/ptp/collection/dosimeters/pocketchamdos.htm


Pocket dosimeters tended to be slightly larger than pocket chambers. Their<br />

walls might be made <strong>of</strong> aluminum, bakelite, or some other type <strong>of</strong> plastic. If<br />

the material was not conductive, the inner surface <strong>of</strong> the chamber was coated<br />

with Aquadag (graphite). The central electrode was usually a phosphor<br />

bronze rod. This made pocket dosimeters more energy dependent than<br />

pocket chambers whose central electrodes were usually aluminum. Some<br />

dosimeters (e.g., Keleket Model K-145) employed boron-lined chambers<br />

which made them sensitive to thermal neutrons.<br />

Pocket dosimeters must be charged (ca. 150 ~ 200 volts) with some sort <strong>of</strong><br />

charger, but they do not require another device to read them. This allows the<br />

worker to determine his or her exposure at any time, an important advantage<br />

when working in high radiation fields.<br />

The first direct reading pocket dosimeters were built by Charlie Lauritsen at<br />

the California Institute <strong>of</strong> Technology.<br />

Charlie Chong/ Fion Zhang<br />

http://www.orau.org/ptp/collection/dosimeters/pocketchamdos.htm


3. Pocket Chambers (indirect-reading) vs Pocket Dosimeters (direct<br />

reading)<br />

1. Pocket chambers were far less expensive (ca. $5 vs $40 in 1950)<br />

2. Pocket chambers, despite their problems, were more reliable.<br />

3. Pocket chambers did not permit the wearer to know their exposure, for<br />

military purposes, this was sometimes desirable.<br />

4. Pocket dosimeters allowed the worker to check their exposure during a<br />

particular task and to take corrective actions when appropriate.<br />

5. Pocket dosimeters did not have to be recharged every time they were read.<br />

6. Pocket dosimeters could use very small chargers, small enough to easily<br />

fit into a pocket.<br />

Charlie Chong/ Fion Zhang<br />

http://www.orau.org/ptp/collection/dosimeters/pocketchamdos.htm


Quartz Fiber Pocket Dosimeter.<br />

CDV-750 Dosimeter Charger and THREE (3) CDV-742 Dosimeters<br />

$260.00 The direct-reading pocket dosimeter is a portable instrument designed to measure the total dose <strong>of</strong> moderate and<br />

high levels <strong>of</strong> gamma radiation. The instruments make use <strong>of</strong> a small quartz fiber electroscope as an exposure detector and<br />

indicator. An image <strong>of</strong> the fiber is projected onto a film scale and viewed through the eyepiece lens. The scale is calibrated in<br />

roentgens (R) and may be read by looking through the eyepiece toward a lamp or other source <strong>of</strong> light. A CDV-750 dosimeter<br />

charger must be used in conjunction with the dosimeter to set the instrument to zero. The charger may also be used to read the<br />

scale or you can hold the dosimeter up to any light source and look through it.<br />

NOTE: the CDV-750 uses 1 D cell Battery (not included). The CDV-742 Dosimeter is an 'electroscope' it is electro statically<br />

charged by the CDV-750 charger. The Dosimeter does NOT use a battery. No battery to replace, no battery to go bad, EVER!<br />

Charlie Chong/ Fion Zhang<br />

http://josephdanielassociates.us/index.php?main_page=product_info&products_id=356


Charlie Chong/ Fion Zhang<br />

http://www.orau.org/ptp/collection/dosimeters/pocketchamdos.htm


Charlie Chong/ Fion Zhang


Ion Chamber Charger & Reader<br />

Charlie Chong/ Fion Zhang<br />

http://www.orau.org/ptp/collection/dosimeters/pocketchamdos.htm


Ion Chamber Charger & Reader<br />

Charlie Chong/ Fion Zhang<br />

http://www.orau.org/ptp/collection/dosimeters/pocketchamdos.htm


Quartz Fiber Pocket Dosimeter.<br />

Charlie Chong/ Fion Zhang<br />

http://www.orau.org/ptp/collection/dosimeters/pocketchamdos.htm


WWII Heroes<br />

Charlie Chong/ Fion Zhang


Direct <strong>Reading</strong> DosimetersThe direct reading dosimeter operates on the<br />

principle <strong>of</strong> the gold leaf electroscope (Fig. 9). A quartz fiber is displaced<br />

electrostatically by charging it to a potential <strong>of</strong> about 200 V. An image <strong>of</strong> the<br />

fiber is focused on a scale and viewedthrough a lens at one end <strong>of</strong> the<br />

instrument. Radiationexposure <strong>of</strong> the dosimeter discharges the fiber,<br />

allowing itto return to its original position.Personnel dosimeters may have a<br />

full scale reading <strong>of</strong> 1 to 50 mSv (100 mR to 5 R) (0.1R ~ 5R) and may have<br />

other scales according to applicable regulations. Chambers are available with<br />

thin walls for sensitivity to beta radiation over 1 MeV and may be coated on<br />

the inside with boron for neutron sensitivity. Figure 10 demonstrates the<br />

energy response <strong>of</strong> self- reading pocket dosimeters. Table 2 lists<br />

performance specifications <strong>of</strong> dosimeters in general.<br />

Keypoints:<br />

■ Chambers are available with thin walls for sensitivity to beta radiation<br />

1 MeV<br />

■ may be coated on the inside with boron for neutron sensitivity.<br />

Charlie Chong/ Fion Zhang


FIGURE 8. Cross section <strong>of</strong> quartz fiber pocket dosimeter.<br />

Charlie Chong/ Fion Zhang


FIGURE 9. Cross section <strong>of</strong> pocket (direct reading) ionization chamber.<br />

Charlie Chong/ Fion Zhang


FIGURE 10. Energy dependence <strong>of</strong> response <strong>of</strong> different commercial selfreading<br />

dosimeters.<br />

Charlie Chong/ Fion Zhang


TABLE 2. General performance specifications for dosimeters.<br />

Charlie Chong/ Fion Zhang


Proportional Counters<br />

If the electric field in an ion chamber is raised above the ionization potential<br />

but below saturation potential, enough energy is imparted to the ions for<br />

production <strong>of</strong> secondary electrons by collision and gas amplification.<br />

Operation at this electric potential overcomes the difficulty <strong>of</strong> the small<br />

currents in the ionization region yet takes advantage <strong>of</strong> pulse size<br />

dependence for separating various ionizing energies.<br />

When an ionization chamber is operated in this region it is called a<br />

proportional counter.<br />

The size <strong>of</strong> the output pulse is determined by, and proportional to, the number<br />

<strong>of</strong> electrons collected at the anode (n) and the voltage applied (V) at the<br />

detector (Output∝n·V) . By careful selection <strong>of</strong> gases and voltages, a<br />

properly designed proportional counter can detect alphas in the presence <strong>of</strong><br />

betas, or higher energy beta and gamma radiation in the presence <strong>of</strong> lower<br />

energies. Proportional counters are <strong>of</strong>ten used in X-ray diffraction<br />

applications.<br />

Charlie Chong/ Fion Zhang


REM (Roentgen equivalent man) – Dose Equivalent<br />

One <strong>of</strong> the two standard units used to measure the dose equivalent (or<br />

effective dose), which combines the amount <strong>of</strong> energy (from any type <strong>of</strong><br />

ionizing radiation that is deposited in human tissue), along with the medical<br />

effects <strong>of</strong> the given type <strong>of</strong> radiation. For beta and gamma radiation, the dose<br />

equivalent is the same as the absorbed dose. By contrast, the dose<br />

equivalent is larger than the absorbed dose for alpha and neutron radiation,<br />

because these types <strong>of</strong> radiation are more damaging to the human body.<br />

Thus, the dose equivalent (in rems) is equal to the absorbed dose (in rads)<br />

multiplied by the quality factor <strong>of</strong> the type <strong>of</strong> radiation [see Title 10, Section<br />

20.1004, <strong>of</strong> the Code <strong>of</strong> Federal Regulations (10 CFR 20.1004), "Units <strong>of</strong><br />

Radiation Dose"]. The related international system unit is the sievert (Sv),<br />

where 100 rem is equivalent to 1 Sv. For additional information, see Doses in<br />

Our Daily Lives and Measuring Radiation.<br />

先 有 rad 才 有 rem / 先 有 Gray 才 有 Sievert<br />

Charlie Chong/ Fion Zhang<br />

http://www.nrc.gov/reading-rm/basic-ref/glossary/rem-roentgen-equivalent-man.html


Townsend Discharges (Avalanches)<br />

The Townsend discharge or Townsend avalanche is a gas ionisation process<br />

where free electrons are accelerated by an electric field, collide with gas<br />

molecules, and consequently free additional electrons. Those electrons are in<br />

turn accelerated and free additional electrons. The result is an avalanche<br />

multiplication that permits electrical conduction through the gas. The<br />

discharge requires a source <strong>of</strong> free electrons and a significant electric field;<br />

without both, the phenomenon does not occur.<br />

The Townsend discharge is named after John Sealy Townsend, who<br />

discovered the fundamental ionisation mechanism by his work between 1897<br />

and 1901.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Townsend_avalanche


Sir John Sealy Townsend<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Townsend_avalanche


General description <strong>of</strong> the phenomenon<br />

The avalanche occurs in a gaseous medium that can be ionised (such as air).<br />

The electric field and the mean free path <strong>of</strong> the electron must allow free<br />

electrons to acquire an energy level (velocity) that can cause impact<br />

ionisation. If the electric field is too small, then the electrons do not acquire<br />

enough energy. If the mean free path is too short, the electron gives up its<br />

acquired energy in a series <strong>of</strong> non-ionising collisions. If the mean free path is<br />

too long, then the electron reaches the anode before colliding with another<br />

molecule.<br />

A positive charge q is placed in a uniform<br />

electric field E set up between two charged<br />

parallel plates. If the particle is at a<br />

distance s from the negative plate, its<br />

electrical potential energy is qEs joules<br />

(C·N·C-1·m = N.m)<br />

http://www.physchem.co.za/OB11-ele/charge3.htm<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Townsend_avalanche


Note:<br />

• If the electric field is too small, then the electrons do not acquire enough<br />

energy.<br />

• If the mean free path is too small, then the electrons do not acquire<br />

enough kinetic energy.<br />

• If the mean free path is too short, the electron collides too early with low<br />

energy, gives up its acquired energy in a series <strong>of</strong> non-ionising collisions.<br />

• If the mean free path is too long, then the electron reaches the anode<br />

before colliding with another molecule.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Townsend_avalanche


The avalanche mechanism is shown in the accompanying diagram. The<br />

electric field is applied across a gaseous medium; initial ions are created with<br />

ionising radiation (for example, cosmic rays, X radiation and gamma ray). An<br />

original ionisation event produces an ion pair; the positive ion accelerates<br />

towards the cathode while the free electron accelerates towards the anode. If<br />

the electric field is strong enough, the free electron can gain sufficient velocity<br />

(energy) (qEs) to liberate another electron when it next collides with a<br />

molecule.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Townsend_avalanche


The two free electrons then travel towards the anode and gain sufficient<br />

energy from the electric field to cause further impact ionisations, and so on.<br />

This process is effectively a chain reaction that generates free electrons.<br />

The total number <strong>of</strong> electrons reaching the anode is equal to the number <strong>of</strong><br />

collisions, plus the single initiating free electron. (n+1) Initially, the number <strong>of</strong><br />

collisions grows exponentially. (?) The limit to the multiplication in an electron<br />

avalanche is known as the Raether limit.<br />

The Townsend avalanche can have a large range <strong>of</strong> current densities. In<br />

common gas-filled tubes, such as those used as gaseous ionisation detectors,<br />

magnitudes <strong>of</strong> currents flowing during this process can range from about<br />

10 −18 amperes to about 10 −5 amperes.<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Townsend_avalanche


Visualization <strong>of</strong> Proportional Counter Gas Magnification Event<br />

Single gas<br />

avalanche near<br />

the anode?<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Townsend_avalanche


Visualization <strong>of</strong> Proportional Counter Gas Magnification Event<br />

Single gas<br />

avalanche near<br />

the anode?<br />

Charlie Chong/ Fion Zhang<br />

https://en.wikipedia.org/wiki/Townsend_avalanche


Multiple Gas Amplification due to multiple ionization<br />

Single gas<br />

avalanche near<br />

the anode<br />

Charlie Chong/ Fion Zhang


dose equivalent (in rems) is equal to the absorbed dose (in rads)<br />

multiplied by the quality factor <strong>of</strong> the type <strong>of</strong> radiation<br />

rems<br />

rads<br />

Charlie Chong/ Fion Zhang<br />

http://www.nrc.gov/reading-rm/basic-ref/glossary/rem-roentgen-equivalent-man.html


PART 3. Geiger-Müller Counters<br />

Operating Voltage Level<br />

Increasing voltage beyond the proportional region (Fig. 3) will eventually<br />

cause the gas avalanche to extend along the entire length <strong>of</strong> the anode wire.<br />

When this happens, the end <strong>of</strong> the proportionalregion is reached and the<br />

geiger-müller region begins. An instrument operating in this voltage range,<br />

using a sealed gas filled detector, is referred to as a geiger-müller counter, a<br />

GM counter or simply a geiger tube. This instrument was introduced in 1928<br />

and its simplicity and low cost have made it the most popular radiation<br />

detector since then. Geiger-müller counters complement the ion chamber and<br />

proportional counter and comprise the third category <strong>of</strong> gas filled<br />

detectors based on ionization.<br />

Charlie Chong/ Fion Zhang


Operating Voltage Level<br />

Charlie Chong/ Fion Zhang


Visualization <strong>of</strong> Geiger Muller Gas Magnification Event- Townsend<br />

Avalanches<br />

Multiple gas<br />

avalanche<br />

Charlie Chong/ Fion Zhang


Visualization <strong>of</strong> Geiger Muller Gas Magnification Event- Townsend<br />

Avalanches<br />

Visualization <strong>of</strong> the spread <strong>of</strong><br />

Townsend avalanches by means<br />

<strong>of</strong> UV photons. This mechanism<br />

allows a single ionising event to<br />

ionise all the gas surrounding the<br />

anode by triggering multiple<br />

avalanches.<br />

Charlie Chong/ Fion Zhang


Properties<br />

Extension <strong>of</strong> the gas avalanche increases the gas amplification factors so that<br />

10 9 to 10 10 ion pairs are formed in the discharge. This results in an output<br />

pulse large enough (0.25 to 10 V) to require no sophisticated electronic<br />

amplification circuitry for readout. At this voltage, the size <strong>of</strong> all pulses,<br />

regardless <strong>of</strong> the nature <strong>of</strong> the ionization, is the same.<br />

When operated in the geiger-müller region, a counter cannot distinguish<br />

among the several types <strong>of</strong> radiation and therefore is not useful for<br />

spectroscopy or for the detection <strong>of</strong> one energy event in the presence <strong>of</strong><br />

another. An external shield is <strong>of</strong>ten used to filter out alpha and beta particles<br />

in the presence <strong>of</strong> gamma energies.<br />

Note:<br />

The amplification factor: 10 9 to 10 10 ion pairs are formed in the discharge for<br />

single ionization <strong>of</strong> multiple events avalanches<br />

Charlie Chong/ Fion Zhang


Resolving Time<br />

As an ionizing event occurs in the counter, the avalanche <strong>of</strong> ions paralyzes<br />

the counter. The counter is then incapable <strong>of</strong> responding to another event<br />

until the discharge dissipates and proper potential is established.<br />

The time it takes to reestablish the electric field intensity is referred to as the<br />

resolving time.<br />

Average resolving time for a geiger-müller counter is about 100 ms, which<br />

must be corrected at high level readings. Resolving time τ <strong>of</strong> a counter may<br />

be determined by counting two sources independently (R 1 and R 2 ), then<br />

together (R 1 , R 2 ). The background count is R b .<br />

Charlie Chong/ Fion Zhang


Correct counting rate R can be calculated from observed counting rate R o<br />

andresolving time τ in the following equation for nonparalyzable systems:<br />

Charlie Chong/ Fion Zhang


Dead Time<br />

The relationship <strong>of</strong> resolving time to dead time and recovery is illustrated in<br />

Fig. 11.Resolving time may be a function <strong>of</strong> the detector alone or <strong>of</strong> the<br />

detector and its signal processing electronics. Its effect on the real counting<br />

rate depends on whether the system design is paralyzableor nonparalyzable.<br />

Charlie Chong/ Fion Zhang


FIGURE 11. Resolving time, dead time and recovery time for geiger-müller<br />

system.<br />

Charlie Chong/ Fion Zhang


Nonparalyzable Systems<br />

In Fig. 12, a time scale is shown indicating six randomly spaced events in the<br />

detector. At the bottom <strong>of</strong> the illustration is the corresponding dead time<br />

behavior <strong>of</strong> a detector assumed to be nonparalyzable. A fixed time τ follows<br />

each event that occurs during the live period <strong>of</strong> the detector. Events occurring<br />

during the dead time have no effect on the detector, which would record four<br />

counts from the six interactions.<br />

Charlie Chong/ Fion Zhang


FIGURE 12. Processing <strong>of</strong> detector interactions in paralyzable<br />

and nonparalyzable systems.<br />

Charlie Chong/ Fion Zhang


Paralyzable Systems The top line <strong>of</strong> Fig. 12 illustrates a paralyzable system.<br />

Resolving time τ follows each interaction, whether it is recorded or not.<br />

Events that occur during resolving time τ are not recorded and further extend<br />

the dead time by another period τ. The chart indicates only three recorded<br />

events from the six interactions. In this case, τ increases with increased<br />

number <strong>of</strong> interactions. It can be demonstrated that with a paralyzable system<br />

(at increasingly higher interaction rates), the observed counting rates can<br />

actually decrease with an increased number <strong>of</strong> events. When using a<br />

counting system that may be paralyzable, extreme caution must be taken to<br />

ensure that low observed counting rates correspond to low interaction rates,<br />

rather than very high interaction rates with accompanying, long dead time. It<br />

is possible for a paralyzable system to record the first interaction and then be<br />

paralyzed, recording zero counts in high radiation fields.<br />

Charlie Chong/ Fion Zhang


Quenching<br />

As positive ions are collected after a pulse, they give up their kinetic energy<br />

by striking the wall <strong>of</strong> the tube; Ultraviolet photons and/or electrons are<br />

liberated, producing spurious counts. Prevention <strong>of</strong> such counts is called<br />

quenching. Quenching may be accomplished electronically (by lowering the<br />

anode voltage after a pulse) or chemically (by using a self-quenching gas).<br />

■ Electronic Quenching (by lowering the anode voltage after a pulse)<br />

Electronic quenching is accomplished by introducing a high value <strong>of</strong><br />

resistance into the voltage circuit. This will drop the anode potential until all<br />

the positive ions have been collected.<br />

Charlie Chong/ Fion Zhang


■ Self-Quenching Gas (absorb ultraviolet (UV) photons)<br />

A self-quenching gas is one that can absorb ultraviolet (UV) photons without<br />

becoming ionized. One way to use this characteristic is to introduce a small<br />

amount <strong>of</strong> organic vapor, such as alcohol or ether, into the tube. The energy<br />

from the ultraviolet photons is then dissipated by dissociating the gas<br />

molecule. Such a tube is useful only as long as it has a sufficient number <strong>of</strong><br />

organic molecules to dissociate, generally about 10 8 counts.<br />

To avoid the problem <strong>of</strong> limited lifetime, some tubes use halogens (chlorine or<br />

bromine) as the quench gas. The halogen molecules also dissociate in the<br />

quenching process but they are replenished by spontaneous recombination at<br />

a later time. Halogen quench tubes have an infinite lifetime and are preferred<br />

for extended applications.<br />

Reaction products <strong>of</strong> the discharge <strong>of</strong>ten produce contamination <strong>of</strong> the gas or<br />

deposition on the anode surface and generally limit the lifetimes <strong>of</strong> geigermüller<br />

tubes.<br />

Charlie Chong/ Fion Zhang


FIGURE 13. Assortment <strong>of</strong> geiger-müller counters demonstrating availability<br />

<strong>of</strong> sizes and shapes. Smallest counter shown isabout 30 mm (1 in.) long.<br />

Charlie Chong/ Fion Zhang


Geiger Muller<br />

Charlie Chong/ Fion Zhang<br />

http://solderpad.com/solderpad/mightyohm-geiger-counter/board/embed


Geiger Muller<br />

Charlie Chong/ Fion Zhang<br />

http://www.jonshobbies.com/civil-defense-lionel-cd-v-700-model-6b-geiger-counter.html


Geiger Muller<br />

Charlie Chong/ Fion Zhang<br />

http://www.jonshobbies.com/civil-defense-lionel-cd-v-700-model-6b-geiger-counter.html


Geiger Muller<br />

Charlie Chong/ Fion Zhang<br />

http://www.jonshobbies.com/civil-defense-lionel-cd-v-700-model-6b-geiger-counter.html


Geiger Muller<br />

Charlie Chong/ Fion Zhang<br />

http://www.jonshobbies.com/civil-defense-lionel-cd-v-700-model-6b-geiger-counter.html


Geiger Muller<br />

Charlie Chong/ Fion Zhang<br />

http://www.jonshobbies.com/civil-defense-lionel-cd-v-700-model-6b-geiger-counter.html


Geiger Muller<br />

Charlie Chong/ Fion Zhang<br />

http://www.jonshobbies.com/civil-defense-lionel-cd-v-700-model-6b-geiger-counter.html


Geiger Muller<br />

Charlie Chong/ Fion Zhang<br />

http://www.jonshobbies.com/civil-defense-lionel-cd-v-700-model-6b-geiger-counter.html


Smart Geiger Counter<br />

Charlie Chong/ Fion Zhang<br />

http://akihabaranews.com/2015/10/05/article-en/app-enabled-geiger-counter-smartphones-113561601


Design Variations<br />

Geiger-müller counters (Fig. 13) are available in various shapes and sizes.<br />

The most common form is that <strong>of</strong> a cylinder with a central anode wire. If low<br />

energy beta or alpha particles are to be counted, a unit with a thin entrance<br />

window (1 to 4 mg·cm –2 ) should be selected. For surveying large surfaces,<br />

pancake or large window counters are available.<br />

High count rate instruments, greater than 0.14 mSv·s –1 (50 mR·h –1 ), generally<br />

contain a small tube to minimize resolving time <strong>of</strong> the system; large volume<br />

detectors may require significant correction.<br />

Note: small volume minimize resolving time<br />

A geiger-müller counter response to gamma rays occurs by way <strong>of</strong> gamma<br />

ray interaction with the solid wall <strong>of</strong> the tube. The incident gamma ray<br />

interacts with the wall and produces a secondary electron that subsequently<br />

reaches the gas. The probability <strong>of</strong> gamma ray interaction generally increases<br />

with higher density wall material.<br />

Charlie Chong/ Fion Zhang


A geiger-müller counter response to gamma rays occurs by way <strong>of</strong> gamma<br />

ray interaction with the solid wall <strong>of</strong> the tube. The incident gamma ray<br />

interacts with the wall and produces a secondary electron that subsequently<br />

reaches the gas. The probability <strong>of</strong> gamma ray interaction generally increases<br />

with higher density wall material.<br />

Note:<br />

■ Smaller chamber volume, minimize resolving time<br />

■ Gamma ray interact with the chamber wall<br />

■ Higher the density higher the probability <strong>of</strong> interaction<br />

■ Higher the atomic number higher the interaction<br />

Charlie Chong/ Fion Zhang


FIGURE 14. Dose rate ratio versus effective energy for<br />

personnel radiation monitor.<br />

Charlie Chong/ Fion Zhang


FIGURE 14. Dose rate ratio versus effective energy for<br />

personnel radiation monitor.<br />

Ir-192<br />

Charlie Chong/ Fion Zhang


TABLE 1. Characteristics <strong>of</strong> three isotope sources commonly used for<br />

radiography.<br />

Charlie Chong/ Fion Zhang


Alarming Rate Meters (Personnel Monitors)<br />

Small geiger-müller tubes are used in pocket-sized units for personnel<br />

monitoring. They generally emit a high frequency chirp at a rate proportional<br />

to the subjected dose rate. United States regulations specify an alarm<br />

threshold <strong>of</strong> 500 mSv·h –1 (500 mR·h –1 ) (500 μR·h–1) for field gamma<br />

radiography. The energy dependence curve for one such instrument is shown<br />

in Fig. 14.<br />

Charlie Chong/ Fion Zhang


Mini Geiger Muller Alarm Meter<br />

Charlie Chong/ Fion Zhang


Mini Geiger Muller Alarm Meter<br />

Charlie Chong/ Fion Zhang


Mini Geiger Muller Alarm Meter<br />

Charlie Chong/ Fion Zhang


Smart Geiger Counter<br />

Charlie Chong/ Fion Zhang<br />

http://xronosclock.com/home/?p=4238


Charlie Chong/ Fion Zhang


Charlie Chong/ Fion Zhang


Charlie Chong/ Fion Zhang


Applications<br />

Geiger-müller counters are the most widely used, general purpose radiation<br />

survey instruments. It must be remembered that geiger-müller counters,<br />

unlike current ionization chambers, read pulses (regardless <strong>of</strong> their energy or<br />

ionizing potential) and register in counts per minute. Some instruments have<br />

a scale calibrated in milliroentgens per hour (mR·h –1 ); however, this is an<br />

arbitrary scale calibrated on the radiation from radium-226, cesium-137 or<br />

some other energy (Fig. 15). Another scale is microsieverts per second<br />

(μSv·s –1 ). A sensitivity versus energy table should always be consulted<br />

before making measurements with a geiger-müller instrument.<br />

Charlie Chong/ Fion Zhang


FIGURE 15. Typical energy response curves for geiger-müller counters<br />

(a) shielded versus unshielded;<br />

(b) radiation incident on side versus front;<br />

(c) exposure ratio close to ideal with radiation incident normal to long axis <strong>of</strong><br />

probe;<br />

(d) radiation incident normal to long axis <strong>of</strong> probe.<br />

Charlie Chong/ Fion Zhang


(a) shielded versus unshielded;<br />

Charlie Chong/ Fion Zhang


(b) radiation incident on side versus front;<br />

Charlie Chong/ Fion Zhang


(c) exposure ratio close to ideal with radiation incident normal to long axis <strong>of</strong><br />

probe;<br />

Charlie Chong/ Fion Zhang


(d) radiation incident normal to long axis <strong>of</strong> probe.<br />

Charlie Chong/ Fion Zhang


PART 4. Scintillation Detectors<br />

Soon after the discovery <strong>of</strong> X-rays and radioactivity, it was observed that<br />

certain materials emit visible light photons after interacting with ionizing<br />

radiation. These light photons appear to flash or sparkle and the materials are<br />

said to scintillate. Scintillators commonly used with radiation survey<br />

instruments are solid materials. Being denser than gases, these scintillators<br />

have greater detection efficiencies and are useful for low level measurements.<br />

For gamma photons, scintillators have detection efficiencies 10 6 times greater<br />

than typical gas ionization chambers. Detection <strong>of</strong> alpha and beta particles,<br />

neutrons and gamma photons is possible with various scintillator systems<br />

(Table 3).<br />

Charlie Chong/ Fion Zhang


TABLE 3. Common scintillators.<br />

Charlie Chong/ Fion Zhang


Scintillation Process<br />

Radiation interactions with matter produce excitation as well as irrigation.<br />

Ionization refers to the removal <strong>of</strong> an electron from an atom and excitation<br />

refers to the elevation <strong>of</strong> an electron’s energy state. The return <strong>of</strong> excited<br />

electrons to their normal, lower energy state is called deexcitation.<br />

Scintillators excited by ionizing radiation return to lower energy states quickly<br />

and emit visible light during the deexcitation process. Radiation detection is<br />

possible by measuring the scintillator’s light output (Fig. 16).<br />

Charlie Chong/ Fion Zhang


FIGURE 16. Energy diagram <strong>of</strong> scintillation process.<br />

Charlie Chong/ Fion Zhang


Materials and Characteristics<br />

Scintillation materials come in gaseous, liquid and solid forms. Organic liquids<br />

and solids, as well as inorganic gases and solids, are common scintillators.<br />

Organic, solid scintillators are available as crystals, plastics and gels.<br />

Inorganic solid scintillators are usually alkali halide crystals.<br />

The scintillation process in inorganic materials requires the presence <strong>of</strong> small<br />

amounts <strong>of</strong> an impurity, or activator. Inorganic solid scintillators are commonly<br />

used with radiation survey instruments and are listed in Table 3.<br />

Charlie Chong/ Fion Zhang


Desirable Scintillator Characteristics<br />

A useful and practical scintillator needs to have most <strong>of</strong> the characteristics<br />

listed below. Not all <strong>of</strong> these characteristics are ideally satisfied by each<br />

scintillator and <strong>of</strong>ten a compromise is acceptable.<br />

1. The scintillator should be <strong>of</strong> high density and large enough to ensure<br />

adequate interaction with the ionizing radiation.<br />

2. Efficient conversion <strong>of</strong> the electron’s kinetic energy into visible light is<br />

required and the light yield should be linearly related to the deposited<br />

electron kinetic energy.<br />

3. The scintillator should be <strong>of</strong> good optical quality, transparent to its emitted<br />

light and free <strong>of</strong> hydroscopic effects, and should have an index <strong>of</strong><br />

refraction close to that <strong>of</strong> glass.<br />

4. The wavelength <strong>of</strong> the emitted light should be appropriate for matching to<br />

a photomultiplier tube.<br />

Charlie Chong/ Fion Zhang


Photomultiplier Tubes<br />

Before the advent <strong>of</strong> photomultiplier tubes (PMTs), scintillation light photons<br />

had to be visually counted. This limited the use and development <strong>of</strong><br />

scintillators. In the 1940s, the photomultiplier tube was developed and<br />

dramatically increased the use <strong>of</strong> scintillators, to the point where scintillators<br />

are preferred over other radiation detectors for many survey applications. The<br />

photomultiplier tube’s function is to convert the scintillator’s light output into a<br />

electrical pulse. The photomultiplier tube is composed <strong>of</strong> a photosensitive<br />

layer, called the photocathode, and a number <strong>of</strong> electron multiplication<br />

structures called dynodes. Conversion <strong>of</strong> the scintillation light into<br />

photoelectrons is accomplished by the photocathodes through the<br />

photoelectric effect. To maximize the information contained in the scintillation<br />

light, the photomultiplier tube photocathode should be matched to the<br />

scintillator; the scintillator and photomultiplier tube should be optically coupled<br />

to minimize light losses.<br />

Charlie Chong/ Fion Zhang


Electron multiplication, or gain, is accomplished by positively charging the<br />

dynodes in successive stages, so that the total voltage applied to the<br />

photomultiplier tube is around 1000 V. Electrons emitted by the photocathode<br />

are focused toward the first dynode; more electrons are emitted than were<br />

initially incident on the dynode. This is repeated at each dynode stage. The<br />

photocathode and dynodes are positioned in a glass enclosed vacuum so<br />

that air molecules will not interfere with the collection <strong>of</strong> electrons. The net<br />

result <strong>of</strong> the photomultiplier tube may be an electron gain up to 10 10 per<br />

emitted photoelectron. Figure 17 illustrates the structure <strong>of</strong> a photomultiplier<br />

tube.<br />

Charlie Chong/ Fion Zhang


FIGURE 17. Cutaway drawing <strong>of</strong> photomultiplier tube, showing crystal,<br />

photocathode, collecting dynodes and voltage divider network.<br />

Charlie Chong/ Fion Zhang


PMT<br />

Charlie Chong/ Fion Zhang


PMT<br />

Charlie Chong/ Fion Zhang


PMT<br />

Charlie Chong/ Fion Zhang


PMT - Photomultiplier tubes lining the walls <strong>of</strong> the Daya Bay neutrino detector.<br />

The tubes are designed to amplify and record the faint flashes <strong>of</strong> light that<br />

signify an antineutrino interaction. This experiment aims to measure the final<br />

unknown mixing angle that describes how neutrinos oscillate — another<br />

chapter in Brookhaven National Laboratory's long history <strong>of</strong> neutrino research<br />

over the last several decades.<br />

Charlie Chong/ Fion Zhang<br />

https://www.bnl.gov/newsroom/news.php?a=24055


System Electronics<br />

Once the output pulse from a photomultiplier tube is generated, it is amplified<br />

and analyzed. The pulse height, or amplitude, is proportional to the amount <strong>of</strong><br />

energy deposited within the scintillator and can be correlated to a count rate<br />

or scale <strong>of</strong> microsievert per second (μSv·s –1 ) or milliroentgen per hour<br />

(mR·h –1 ) when calibrated against a known energy source. (See Fig. 18.)<br />

Charlie Chong/ Fion Zhang


FIGURE 18. Comparison <strong>of</strong> sodium iodide (thallium activated) and<br />

germanium detectors for gamma spectroscopy.<br />

Charlie Chong/ Fion Zhang<br />

Energy (MeV)


PART 5. Luminescent Dosimetry<br />

Thermoluminescent Dosimetry<br />

Thermoluminescence is the emission <strong>of</strong> light from previously irradiated<br />

materials after gentle heating. The radiation effect in thermoluminescent (TL)<br />

materials is similar to that observed in scintillators, except that light photon<br />

emission does not occur in thermoluminescent materials until some heat<br />

energy is supplied (Fig. 19). Measurement <strong>of</strong> the light photons emitted after<br />

heating permits correlation to the amount <strong>of</strong> ionizing radiation energy that was<br />

absorbed in the thermoluminescent material.<br />

Thermoluminescent dosimetry (TLD) is possible for beta, gamma and neutron<br />

(alpha?) radiations, if the appropriate thermoluminescent material is used.<br />

Charlie Chong/ Fion Zhang


Thermoluminescence<br />

Charlie Chong/ Fion Zhang


Thermoluminescence<br />

Charlie Chong/ Fion Zhang


Lithium Fluoride Properties<br />

The most common thermoluminescent phosphor used in gamma and neutron<br />

personnel dosimetry is lithium fluoride ( 6 3LiF for neutron detection)) .<br />

Other thermoluminescent phosphors are available for personnel dosimetry<br />

but, for various reasons, are not as well suited as lithium fluoride. The<br />

advantages <strong>of</strong> lithium fluoride include its:<br />

1. usefulness over a wide dose range,<br />

2. linear dose response,<br />

3. near dose rate independence,<br />

4. reusability,<br />

5. stability,<br />

6. short readout time and<br />

7. near tissue equivalence.<br />

Charlie Chong/ Fion Zhang


Disadvantages include the loss <strong>of</strong> information after readout and lack <strong>of</strong><br />

information about the incident radiation energy.<br />

Both gamma photons and neutrons produce ionization indirectly. Gamma<br />

photons interact with matter, releasing electrons that in turn cause ionization.<br />

Lithium fluoride undergoes interactions with gamma photons and is therefore<br />

used in gamma dosimetry.<br />

Slow neutrons require the presence <strong>of</strong> the lithium fluoride enriched with<br />

lithium-6 for detection <strong>of</strong> the (n, α) nuclear reaction.<br />

6<br />

3 Li + n → 4 2 He + 2 1 D + γ<br />

Charlie Chong/ Fion Zhang


Fast neutron detection with lithium fluoride would only be possible if the fast<br />

neutrons were slowed down to thermal energies before reaching the lithium<br />

fluoride thermoluminescent dosimeter. Nearly complete elimination <strong>of</strong> neutron<br />

response in lithium fluoride is possible with lithium fluoride enriched with<br />

lithium-7. In a mixed gamma and slow neutron field, distinction <strong>of</strong> gamma and<br />

neutron doses is possible by comparing the readings <strong>of</strong> two lithium fluoride<br />

thermoluminescent dosimeters with different lithium-6 contents.<br />

Keywords:<br />

• Nearly complete elimination <strong>of</strong> neutron response in lithium fluoride is<br />

possible with lithium fluoride enriched with lithium-7.<br />

• In a mixed gamma and slow neutron field, distinction <strong>of</strong> gamma and<br />

neutron doses is possible by comparing the readings <strong>of</strong> two lithium<br />

fluoride thermoluminescent dosimeters with different lithium-6 contents.<br />

Charlie Chong/ Fion Zhang


Thermoluminescent Dosimetric Readout Systems<br />

Thermoluminescent dosimetric readout systems are commonly made up <strong>of</strong> a<br />

sample holder, heating system, photomultiplier tube (light detector), high<br />

voltage supply, signal amplifier and a recording instrument. The<br />

thermoluminescent dosimetric sample is heated indirectly, using electrical<br />

resistance heat applied to a pan or planchette. The photomultiplier tube<br />

converts the light output into an electronic pulse that is then amplified before<br />

recording. The recording instrument may be a plotter or any other instrument<br />

that can measure the amplified photomultiplier tube output signal. A plot <strong>of</strong><br />

the output signal versus time is equivalent to emitted light intensity versus<br />

heat and results in a glow curve.<br />

The area under the glow curve is proportional to the absorbed dose (Fig. 20).<br />

Uses <strong>of</strong> thermoluminescent measurement <strong>of</strong> radiation include personnel<br />

dosimetry, medical dosimetry, environmental monitoring and archeological<br />

and geological dating.<br />

Charlie Chong/ Fion Zhang


FIGURE 19. Thermoluminescence process.5<br />

Charlie Chong/ Fion Zhang


FIGURE 20. Typical glow curve. Integrated area under curve is measure <strong>of</strong><br />

radiation exposure.<br />

Charlie Chong/ Fion Zhang


Optically Stimulated Luminescence Dosimetry<br />

Optically stimulated luminescence dosimeters typically have aluminum oxide<br />

detectors and are available in plastic holders, or body badges, that are worn<br />

at collar level to measure full body dose. They can measure gamma ray and<br />

X-ray doses from 10μSv to 10Sv (1 mrem to 1 krem).<br />

Charlie Chong/ Fion Zhang


TDL<br />

Charlie Chong/ Fion Zhang<br />

http://www.rpe.org.in/article.asp?issn=0972-0464;year=2011;volume=34;issue=1;spage=6;epage=16;aulast=Bhatt;type=3


TDL<br />

Charlie Chong/ Fion Zhang<br />

http://www.rpe.org.in/article.asp?issn=0972-0464;year=2011;volume=34;issue=1;spage=6;epage=16;aulast=Bhatt;type=3


TDL<br />

Charlie Chong/ Fion Zhang<br />

http://www.rpe.org.in/article.asp?issn=0972-0464;year=2011;volume=34;issue=1;spage=6;epage=16;aulast=Bhatt;type=3


TDL<br />

Charlie Chong/ Fion Zhang<br />

http://www.rpe.org.in/article.asp?issn=0972-0464;year=2011;volume=34;issue=1;spage=6;epage=16;aulast=Bhatt;type=3


PART 6. <strong>Neutron</strong> Detection<br />

Characteristics<br />

The neutron is a part <strong>of</strong> the nucleus, has no charge and is somewhat larger in<br />

mass than the proton. It is similar to the photon in that it has no charge and<br />

produces ionization indirectly; it is different from the photon because it is a<br />

nuclear particle and not a unit <strong>of</strong> electromagnetic energy. Because the<br />

neutron is an uncharged particle, its interactions with matter are different from<br />

those <strong>of</strong> charged particles or photons. Ionization by neutrons is indirect: as a<br />

result <strong>of</strong> neutron interactions with matter, recoil nuclei, photons or charged<br />

particles are produced and then interact with matter by various mechanisms<br />

that cause ionization.<br />

Charlie Chong/ Fion Zhang


<strong>Neutron</strong> Sources<br />

<strong>Neutron</strong>s are classified according to their energies as shown in Table 4.<br />

Some radionuclides (such as californium-252) may decay by<br />

spontaneousfission and emit neutrons with fission fragments, photons and<br />

electrons.<br />

Induced fission reactions, such as those occurring in a nuclear reactor with<br />

uranium, emit about 2.5 neutrons per fission. Fission neutrons range in<br />

energy from 0.025 eV to about 16 MeV.<br />

Other neutron sources are the result <strong>of</strong> various nuclear reactions and produce<br />

either a spectrum <strong>of</strong> neutron energies or monoenergetic neutrons. Common<br />

neutron producing nuclear reactions are the (γ, n), (α, n), (p, n), (d, n) and (α,<br />

2n) reactions and may use radionuclide emissions or accelerated particles to<br />

initiate the reaction. <strong>Neutron</strong> radiography usually uses radionuclides that emit<br />

alpha or gamma photons and produce neutrons by (α, n) and (γ, n) reactions<br />

with various target materials.<br />

Charlie Chong/ Fion Zhang


TABLE 4. <strong>Neutron</strong> classification.<br />

Class<br />

Thermal<br />

Epithermal<br />

Slow<br />

Intermediate<br />

Fast<br />

Relativistic greater than<br />

Energy<br />

< 0.3 meV<br />

>1 eV<br />

0 meV to 100 eV<br />

100 eV to 10 keV<br />

10 keV to 10 MeV<br />

10 MeV<br />

Charlie Chong/ Fion Zhang


<strong>Neutron</strong> Detectors<br />

There are several mechanisms and devices used to detect neutrons <strong>of</strong><br />

various energies. Ionization chambers, proportional counters, scintillators,<br />

activation foils, track etch detectors, film emulsions, nuclear emulsions and<br />

thermoluminescent phosphors are some <strong>of</strong> the many devices used to detect<br />

neutrons. The main mechanisms used to detect neutrons in these devices are<br />

the (n, α), (n, p), (n, d), (n, f) and (n, γ) nuclear reactions.<br />

(n, f ) f= fragments<br />

Proportional <strong>Neutron</strong> Detectors Many fast and slow neutron counters use<br />

proportional counting chambers filled with boron trifluoride (BF 3 ) gas, <strong>of</strong>ten<br />

enriched in boron-10. The interaction <strong>of</strong> thermal (slow) neutrons with boron<br />

gas releases an alpha particle <strong>of</strong> several mega electron volts that is easily<br />

detected in the proportional mode. Fast neutrons are detected by a similar<br />

counter, in which thermal neutrons are absorbed in an external cadmium<br />

shield; the fast neutrons that pass through the shield are thermalized in<br />

hydrogen rich material and counted in the proportional chambers.<br />

10<br />

5 B + n → 4 2 He2+ + 7 3 Li + γ<br />

Charlie Chong/ Fion Zhang


Scintillation<br />

Scintillators containing lithium-6, boron-10 and hydrogenous plastics have<br />

been used as neutron detectors. Lithium-6 is used as lithium iodide (europium<br />

activated) and in lithium glasses to detect slow and fast neutrons. Scintillators<br />

loaded with boron-10 are used for slow neutron detection. Plastic scintillators<br />

with high hydrogen content are used in fast neutron detection and<br />

spectroscopy by measuring the energy deposited by recoil protons.<br />

Activation Foils Introducing certain materials to an incident neutron flux will<br />

result in these materials becoming radioactive. The process is called<br />

activation and gaining information about the incident neutron flux and energy<br />

is possible by analyzing the radiations emitted from the activated foil.<br />

Activation foils rely on (n, γ), (n, p), (n, α), (n, f ) and other nuclear reactions<br />

to cause the activation. Selection <strong>of</strong> the proper activation foil can give a rough<br />

estimate <strong>of</strong> the neutron energy spectrum. In high neutron flux fields, where<br />

instruments would fail, activation foils are used as integrating detectors.<br />

Charlie Chong/ Fion Zhang


Miscellaneous <strong>Neutron</strong> Detectors Track etch detectors, nuclear<br />

emulsions and film have all been used to detect neutrons. Various neutron<br />

interactions with the detector material or foils in intimate contact with the<br />

detectors allow these systems to operate as integrating dosimeters.<br />

Charlie Chong/ Fion Zhang


TABLE 6. Properties <strong>of</strong> Some Thermal <strong>Neutron</strong> <strong>Radiography</strong> Conversion Materials<br />

Material<br />

Useful Reactions<br />

Cross Section for<br />

Life<br />

Thermal <strong>Neutron</strong>s (barns)<br />

Lithium<br />

6 Li(n,α) 3 H<br />

910<br />

prompt<br />

Boron<br />

10 B(n,α) 7 Li<br />

3,830<br />

prompt<br />

Rhodium<br />

103 Rh(n) 104m Rh<br />

11<br />

45 min<br />

103<br />

Rh(n) 104 Rh<br />

139<br />

42 s<br />

Silver<br />

107 Ag(n) 108 Ag<br />

35<br />

2.3 min<br />

109 Ag (n) 110 Ag<br />

91<br />

24 s<br />

Cadmium<br />

113 Cd((n,γ) 114 Cd<br />

20,000<br />

prompt<br />

Indium<br />

115 In(n) 116 n<br />

157<br />

54 min<br />

115<br />

In(n) 116m ln<br />

42<br />

14 s<br />

Samarium<br />

149 Sm(n,γ) 150 Sm<br />

41,000<br />

prompt<br />

I52<br />

Sm(n) 153 Sm<br />

210<br />

47 h<br />

Europium<br />

151 Eu(n) 152 Eu<br />

3,000<br />

9.2 h<br />

Gadolinium<br />

155<br />

Gd(n,γ) I56 Gd<br />

61,000<br />

prompt<br />

157<br />

Gd(n.γ) 158 Gd<br />

254,000<br />

prompt<br />

Dyprosium<br />

164<br />

Dy(n) 165 mDy<br />

2,200<br />

1.25 min<br />

164<br />

Dy(n) 165 Dy<br />

800<br />

140 min<br />

Gold<br />

197 Au(n) 198 Au<br />

99<br />

2.7 days<br />

Charlie Chong/ Fion Zhang


PART 7. Semiconductors<br />

Certain semiconductor crystals, when exposed to ionizing radiation, become<br />

conductors and may be used as radiation detectors. Semiconductors are<br />

most <strong>of</strong>ten used for low level spectroscopic measurements <strong>of</strong> alpha particles,<br />

beta particles and gamma rays in laboratory settings and in X-ray diffraction<br />

equipment (Table 5). The most widely used semiconductor devices are<br />

diffused p-n junction, surface barrier and lithium drifted detectors.<br />

Semiconductor detectors have found their broadest application in the field <strong>of</strong><br />

spectroscopy, although lithium drifted detectors are also being used for<br />

gamma ray detection.<br />

Charlie Chong/ Fion Zhang


Detector<br />

The diffused p-n junction detector (Fig. 21a) gets its name from its<br />

manufacturing process. A slice <strong>of</strong> p type (electron depleted) silicon or<br />

germanium crystal, with a layer <strong>of</strong> n type (electron rich) impurity (usually<br />

phosphorus) deposited on the surface, is heated to form a p-n junction just<br />

below the surface. The phosphorus may also be painted onto the silicon and<br />

made to diffuse into it by applying heat. Because the n type material has an<br />

excess <strong>of</strong> electrons and the p type has an excess <strong>of</strong> holes (holes may be<br />

thought <strong>of</strong> as unit positive charges), the natural action <strong>of</strong> the combined<br />

materials tends to align the electrons on one side <strong>of</strong> the junction and the<br />

holes on the other. Thus a difference <strong>of</strong> potential is built up across the<br />

junction. By applying an external voltage to the crystal <strong>of</strong> such polarity as to<br />

oppose the natural movement <strong>of</strong> electrons and holes (reverse bias), the<br />

potential barrier across the junction is increased and a depletion region is<br />

produced.<br />

Charlie Chong/ Fion Zhang


This depletion region is the sensitive part <strong>of</strong> the detector and is analogous to<br />

the gas volume in a gas ionization detector. Charged particles, on entering<br />

the depletion region, produce electron hole pairs analogous to the ion pairs<br />

produced in gas ionization chambers. Because an electric field exists in this<br />

region, the charge produced by the ionizing particle is collected, producing a<br />

pulse <strong>of</strong> current. The size <strong>of</strong> the pulse is proportional to the energy expended<br />

by the particle.<br />

Charlie Chong/ Fion Zhang


Surface Barrier Detectors<br />

The operation <strong>of</strong> surface barrier and lithium drifted detectors is the same as<br />

for the p-n junction: a depletion region is produced, in which there exists an<br />

electric field. The means <strong>of</strong> producing the depletion region (as well as its<br />

dimension and location within the crystal) vary from one type <strong>of</strong> detector to<br />

another. The operation <strong>of</strong> a surface barrier detector (Fig. 21b) depends on the<br />

surface conditions <strong>of</strong> the silicon or germanium. At the surface <strong>of</strong> a piece <strong>of</strong><br />

pure crystal, an electric field exists such that both holes and electrons are<br />

excluded from a thin region near the surface. For n type crystals, the field<br />

repels free electrons. If a metal is joined to the crystal, the free electrons are<br />

still repelled but a concentration <strong>of</strong> holes is produced directly under the<br />

surface. If a reverse bias is then applied, a depletion region is produced.<br />

Surface barrier detectors give better resolution for particle spectroscopy than<br />

p-n junctions but wider depletion regions are possible with the latter. (The<br />

wider the depletion region, the higher the energy <strong>of</strong> particles can be analyzed<br />

because a particle must expend all its energy in a depletion region.)<br />

Charlie Chong/ Fion Zhang


Lithium Drifted Detectors<br />

The lithium drifted detector (Fig. 22) is produced by diffusing lithium into low<br />

resistivity p-type silicon or germanium. When heated under reverse bias, the<br />

lithium ions serve as an n type donor. These ions drift into the silicon or<br />

germanium in such a way that a wide layer <strong>of</strong> the p type material is<br />

compensated by the lithium, yielding an effective resistivity comparable to that<br />

<strong>of</strong> the intrinsic material. Wider depletion regions can be obtained with the<br />

lithium drift process than by any other means. Consequently, lithium drifted<br />

detectors are most useful in gamma spectroscopy work. Silicon detectors can<br />

be operated at room temperatures but exhibit low efficiency for gamma rays.<br />

Germanium detectors have higher gamma efficiencies but must be operated<br />

at liquid nitrogen temperatures. For these reasons, coupled with the small<br />

sensitive volumes obtainable to date, semiconductor detectors have not<br />

received widespread application in radiation survey instruments.<br />

Charlie Chong/ Fion Zhang


TABLE 5. Radiation detector types.<br />

Charlie Chong/ Fion Zhang


FIGURE 21. Cross sections: (a) diffused p-n junction detector;<br />

(b) surface barrier detector.<br />

Charlie Chong/ Fion Zhang


FIGURE 21. Cross sections: (a) diffused p-n junction detector;<br />

(b) surface barrier detector.<br />

Charlie Chong/ Fion Zhang


FIGURE 22. Cross section <strong>of</strong> lithium drifted detector.<br />

Charlie Chong/ Fion Zhang


PART 8. Film Badges<br />

One <strong>of</strong> the most important uses <strong>of</strong> radiographic film as a means <strong>of</strong> measuring<br />

radiation is in film badges. Individuals who work with isotope radiation<br />

sources and X-ray machines are required by codes to wear badges indicating<br />

cumulative exposure to ionizing radiation. Film badges are discussed in this<br />

volume’s chapter on radiation safety and elsewhere<br />

Charlie Chong/ Fion Zhang


Latent Image Formation<br />

Latent image formation is a very subtle change in the silver halide grain <strong>of</strong> film.<br />

The process may involve the absorption <strong>of</strong> only one or, at most, a few<br />

photons <strong>of</strong> radiation and this may affect only a few atoms out <strong>of</strong> some 10 9 or<br />

10 10 atoms in a typical photographic grain. Formation <strong>of</strong> the latent image,<br />

therefore, cannot be detected by direct physical or analytical chemical means.<br />

The process that made an exposed photographic grain capable <strong>of</strong><br />

transformation into metallic silver (by the mild reducing action <strong>of</strong> a developer)<br />

involved a concentration <strong>of</strong> silver atoms at one or more discrete sites on the<br />

photographic grain. In industrial radiography, the image forming effects <strong>of</strong> X-<br />

rays and gamma rays, rather than those <strong>of</strong> light, are <strong>of</strong> primary interest.<br />

The agent that actually exposes a film grain (a silver bromide crystal in the<br />

emulsion) is not the X-ray photon itself but rather the electrons (photoelectric<br />

and compton) resulting from an absorption event.<br />

The most striking difference between X-ray and visible light exposures arises<br />

from the difference in the amounts <strong>of</strong> energy involved.<br />

Charlie Chong/ Fion Zhang


The absorption <strong>of</strong> a single photon <strong>of</strong> light transfers a very small amount <strong>of</strong><br />

energy to the crystal — only enough energy to free a single electron from a<br />

bromide (Br – ) ion. Several successive light photons are required to make a<br />

single grain developable (to produce within it, or on it, a stable latent image).<br />

The passage <strong>of</strong> an electron through a grain can transmit hundreds <strong>of</strong> times<br />

more energy than the absorption <strong>of</strong> a light photon. Even though this energy is<br />

used inefficiently the amount is enough to make the grain developable. In fact,<br />

a photoelectron or compton electron can have a fairly long path through a film<br />

emulsion and can render many grains developable. The number <strong>of</strong> grains<br />

exposed per photon interaction varies from one (for X-radiation <strong>of</strong> about 10<br />

keV) to 50 or more (for a 1 MeV photon). Because a grain is completely<br />

exposed by the passage <strong>of</strong> an energetic electron, all X-ray exposures are, as<br />

far as the individual grain is concerned, extremely short. The actual time that<br />

an electron is within a grain depends on the electron velocity, the grain<br />

dimensions and the squareness <strong>of</strong> the hit. A time on the order <strong>of</strong> 10 –13 s is<br />

representative. (In the case <strong>of</strong> light, the exposure time for a single grain is the<br />

interval between the arrival <strong>of</strong> the first photon and the arrival <strong>of</strong> the last<br />

photon required to produce a stable latent image.)<br />

Charlie Chong/ Fion Zhang


Development<br />

Many materials discolor with exposure to light (some kinds <strong>of</strong> wood and<br />

human skin are examples) and could be used to record images. Most <strong>of</strong> these<br />

materials react to light exposure on a 1:1 basis — one photon <strong>of</strong> light alters<br />

one molecule or atom. In the silver halide system <strong>of</strong> radiography, however, a<br />

few atoms <strong>of</strong> photolytically deposited silver can, by development, be made to<br />

trigger the subsequent chemical deposition <strong>of</strong> some 10 9 or 10 10 additional<br />

silver atoms, resulting in an amplification factor on the order <strong>of</strong> 10 9 or greater.<br />

This amplification process can be uniform and reproducible enough for<br />

quantitative radiation measurements. Development is essentially a chemical<br />

reduction in which silver halide is converted to metallic silver. To retain the<br />

photographic image, however, the reaction must be limited largely to those<br />

grains that contain a latent image; that is, to those grains that have received<br />

more than a prescribed minimum radiation exposure.<br />

Charlie Chong/ Fion Zhang


Compounds that can be used as photographic developing agents are those in<br />

which the reduction <strong>of</strong> silver halide to metallic silver is catalyzed (speeded up)<br />

by the presence <strong>of</strong> metallic silver in the latent image. Those compounds that<br />

reduce silver halide, in the absence <strong>of</strong> a catalytic effect by the latent image,<br />

are not suitable developing agents because they produce a uniform overall<br />

density on the processed film.<br />

Charlie Chong/ Fion Zhang


Closing<br />

More information on the radiographic latent image, its formation and<br />

processing are available elsewhere. The correct use <strong>of</strong> film badges is<br />

especially important for safety in the conduct <strong>of</strong> radiographic testing programs<br />

and is discussed in this book’s chapter on radiation safety and elsewhere.<br />

Charlie Chong/ Fion Zhang


Charlie Chong/ Fion Zhang


Charlie Chong/ Fion Zhang


Charlie Chong/ Fion Zhang


Good Luck!<br />

Charlie Chong/ Fion Zhang

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