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True Coincidence Summing Correction in Gamma Spectroscopy

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close to the detector, often <strong>in</strong> Mar<strong>in</strong>elli beakers. The extent to which TCS is ignored is<br />

best illustrated <strong>in</strong> Figure 2.7, which shows the results of an <strong>in</strong>tercomparison arranged<br />

by the National Physics Laboratory <strong>in</strong> UK (NPL) <strong>in</strong> 1989 for the measurements of<br />

various radionuclides, <strong>in</strong>clud<strong>in</strong>g Cs-134, at environmental levels. Out of 58 Cs-134<br />

results reported, only four were with<strong>in</strong> the range expected by the NPL (i.e. with<strong>in</strong> the<br />

shaded band <strong>in</strong> the Figure-2.7.) and <strong>in</strong> only 11 cases, the true results lied with<strong>in</strong> the<br />

68% confidence limit reported by the laboratory. It is obvious that the majority of the<br />

results were low; 64% of results reported were more than 5% below the expected<br />

value. The most likely reason for this is that TCS had not been taken <strong>in</strong>to account by<br />

the laboratories report<strong>in</strong>g these results.<br />

Figure 2.7 Summarized Cs-134 results from the 1989 NPL environmental radioactivity<br />

<strong>in</strong>tercomparison exercise.[8]<br />

To achieve accurate results, the true co<strong>in</strong>cidence summ<strong>in</strong>g must be taken <strong>in</strong>to<br />

account. In fact, further NPL <strong>in</strong>tercomparison exercises <strong>in</strong> 1990 and 1992 showed<br />

similar biases <strong>in</strong> the Cs-134 results, although slightly smaller on average. Inspite of<br />

the grow<strong>in</strong>g awareness of TCS, many labroratories do not take it <strong>in</strong>to account.<br />

2.8 Achiev<strong>in</strong>g Valid Close Geometry Efficiency<br />

Calibrations<br />

A valid efficiency calibration curve can only be measured for close geometry<br />

conditions by us<strong>in</strong>g radionuclides which do not suffer from TCS. Table-2.2 lists<br />

several nuclides which emit only a s<strong>in</strong>gle gamma-ray and therefore cannot<br />

25

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