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True Coincidence Summing Correction in Gamma Spectroscopy

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For the radionuclide under consideration, the total effect with respect to γ-l<strong>in</strong>e g can<br />

be described by a co<strong>in</strong>cidence correction factor COI g<br />

COIg = (1 - Lg).(1 + Sg)<br />

(3.1)<br />

From the observed peak area, the corrected peak area (N’ p.g ), can be computed<br />

us<strong>in</strong>g the equation:<br />

p,g<br />

N<br />

p,g<br />

COI<br />

g<br />

N' = (3.2)<br />

In case of simple decay schemes, the problem of co<strong>in</strong>cidence correction is well<br />

understood for the po<strong>in</strong>t sources as can be seen <strong>in</strong> the section 2.10 (mathematical<br />

summ<strong>in</strong>g correction) while general formulae for complex decay schemes have been<br />

given by ANDREAV et al (1972, 1973) 11,12 . However, for a more general case such<br />

as volum<strong>in</strong>ous sources e.g. Mar<strong>in</strong>elli beakers and bottles, the correction for<br />

co<strong>in</strong>cidence summ<strong>in</strong>g is more complicated due to the complexity of self-absorption<br />

and the subsequent cascade summ<strong>in</strong>g with partial peak energies, and the formulae<br />

given <strong>in</strong> section 2.10 are no longer valid.<br />

3.2 Estimation of <strong>True</strong> <strong>Co<strong>in</strong>cidence</strong> <strong>Correction</strong>s for Volum<strong>in</strong>ous<br />

Sources<br />

The co<strong>in</strong>cidence summ<strong>in</strong>g depends on the position with<strong>in</strong> the source volume. To<br />

calculate summ<strong>in</strong>g correction for volum<strong>in</strong>ous sources the quantities ε and ε t (def<strong>in</strong>ed<br />

for the whole source) become useless due to the contribution of the <strong>in</strong>dividual source<br />

volume elements to the peak areas. The summ<strong>in</strong>g effects should therefore be<br />

calculated for each volume element dV from the full-energy peak efficiency ε(r) and<br />

the total efficiency ε t (r) for the specific position r of dV. So equation (2.3) is replaced<br />

by<br />

1<br />

1<br />

Similarly, ε t1 <strong>in</strong> eq. (2.5) is replaced by<br />

/ C1 = 1 ε<br />

t<br />

ε ( r)<br />

dV.<br />

(3.3)<br />

− ∫ 1(<br />

r)<br />

ε<br />

2<br />

( r)<br />

dV / ∫<br />

37

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