Nuclear Reactions in Stars & in the Laboratory
Nuclear Reactions in Stars & in the Laboratory
Nuclear Reactions in Stars & in the Laboratory
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<strong>Nuclear</strong> <strong>Reactions</strong> <strong>in</strong> <strong>Stars</strong> & <strong>in</strong> <strong>the</strong> <strong>Laboratory</strong><br />
Experimental techniques and formalism to simulate<br />
stellar burn<strong>in</strong>g processes <strong>in</strong> <strong>the</strong> laboratory and derive<br />
stellar reaction rates for nuclear reaction processes.
Reaction Rate Def<strong>in</strong>ition<br />
For a given relative velocity v with projectile number density n p<br />
λ<br />
=<br />
σ<br />
⋅<br />
n<br />
p<br />
⋅<br />
v<br />
[ ] s<br />
−1<br />
reaction/target particle<br />
energy/temperature dependent decay constant λ<br />
R<br />
=<br />
σ<br />
⋅<br />
n<br />
p<br />
⋅<br />
v<br />
⋅<br />
n<br />
T<br />
⋅V<br />
[ ] s<br />
−1<br />
reaction rate <strong>in</strong> volume V
Reaction Rate <strong>in</strong> Stellar Environment<br />
reaction rate per second and cm 3 :<br />
r<br />
= n ⋅n<br />
⋅σ<br />
⋅<br />
p<br />
T<br />
v<br />
Reaction rate for particles with velocity distribution Φ(v)<br />
r<br />
1<br />
= n ⋅ n ⋅∫σ<br />
⋅v<br />
⋅Φ(<br />
v)<br />
⋅ dv<br />
p T<br />
1+<br />
δ<br />
pT<br />
Account<strong>in</strong>g for reactions<br />
Between identical particles
Maxwell Boltzmann Distribution<br />
In stellar material of temperature T particles follow ideal gas law<br />
Φ(<br />
v)<br />
4<br />
=<br />
3/<br />
2<br />
2<br />
m v<br />
⎛ m ⎞ −<br />
2<br />
⎜ ⎟<br />
∫<br />
2kT<br />
π v e ( v dv =<br />
with<br />
4<br />
⎜<br />
2 kT<br />
⎟<br />
⎝ π ⎠<br />
Φ ) 1<br />
arbitrary units<br />
3<br />
2<br />
1<br />
max at<br />
E=kT<br />
example: <strong>in</strong> terms<br />
of energy<br />
E=1/2 m v 2<br />
0<br />
0 20 40 60 80<br />
energy (keV)
Temperature <strong>in</strong> <strong>Stars</strong>
Stellar reaction rates<br />
r<br />
1<br />
= YT<br />
Ypρ<br />
2 2<br />
NA<br />
< σv<br />
1+<br />
δ<br />
pT<br />
><br />
reactions per s and cm 3<br />
1<br />
λ = Y p<br />
ρ NA<br />
< σv<br />
1+<br />
δ<br />
pT<br />
><br />
reactions per s &<br />
Target nucleus<br />
this is usually referred to<br />
as <strong>the</strong> stellar reaction rate<br />
units of stellar reaction rate N A<br />
: usually cm 3 /s/mole<br />
n<br />
T<br />
X<br />
T<br />
= ρ ⋅ N<br />
A<br />
⋅ = ρ ⋅<br />
AT<br />
N<br />
A<br />
⋅Y<br />
T<br />
X T ; mass fraction<br />
Y T : abundance
Gamow-Range & Reaction Rate<br />
Stellar Energy Range -- Gamow W<strong>in</strong>dow<br />
-- Resonance Width<br />
∝ exp ( - E / kT )<br />
GAMOW PEAK<br />
σ ∝ exp ( - b / √E )<br />
∝ exp ( - E / kT )<br />
RESONANCE<br />
σ ∝<br />
Γ 2<br />
( E - E ) 2 + (Γ/ 2) 2<br />
Nonresonant Reaction Contributions<br />
N < σ v > ∝ T<br />
A<br />
-3/2<br />
∫<br />
σ E exp ( - E / kT ) d E<br />
σ: cross section<br />
N<br />
Resonant Reaction Rate<br />
-3/2<br />
A < σv > ∝ T ωγ<br />
exp ( - E / kT )<br />
R<br />
ωγ: res. strength<br />
E R : res. energy
The Gamow Range of Stellar Burn<strong>in</strong>g<br />
The Gamow w<strong>in</strong>dow or <strong>the</strong> range of relevant cross section<br />
for “non-resonant” processes is calculated:<br />
Check derivation <strong>in</strong> book<br />
3/ 2<br />
⎛ bkT ⎞<br />
E0 = ⎜ ⎟ = 0.122⋅<br />
1 2<br />
T<br />
⎝ 2 ⎠<br />
(<br />
2 2<br />
)<br />
1/3 2/3<br />
Z Z A MeV<br />
9<br />
ΔE<br />
=<br />
4 6<br />
E0kT<br />
= 0.2368⋅<br />
1 2<br />
T9<br />
3<br />
(<br />
2 2<br />
)<br />
1/ 6 5/<br />
Z Z A MeV<br />
with A “reduced mass number” and T 9<br />
<strong>the</strong> temperature <strong>in</strong> GK
The Gamow peak for 12 C(p,γ) 13<br />
13 N<br />
Note:<br />
kT=2.5 keV !
Examples of Gamow w<strong>in</strong>dow energies<br />
EG amow [M eV]<br />
10.00<br />
1.00<br />
0.10<br />
0.01<br />
0.0 0.1 1.0 10.0<br />
temperature [GK]<br />
p+p<br />
12C+p<br />
12C+a<br />
12C+12C<br />
strong dependence<br />
on Z & temperature
Change <strong>in</strong> Abundance<br />
A + a ⇒ B<br />
A reaction is a random process with a reaction probability<br />
(reaction rate) and follows <strong>the</strong> laws of radioactive decay:<br />
Depletion of isotope A<br />
Formation of isotope B<br />
dn<br />
dt<br />
dn<br />
dt<br />
A<br />
B<br />
= −n<br />
λ = −n<br />
Y ρ NA<br />
= + n<br />
A<br />
A<br />
λ<br />
A<br />
a<br />
< σ v<br />
><br />
consequently:<br />
n<br />
A<br />
( t)<br />
=<br />
n<br />
0 A<br />
e<br />
−λ<br />
t<br />
n<br />
B<br />
( t)<br />
=<br />
n<br />
0 A<br />
(1 −<br />
e<br />
−λ<br />
t<br />
)
0.007<br />
Stellar lifetime of nuclei<br />
abundance<br />
0.006<br />
0.005<br />
0.004<br />
0.003<br />
0.002<br />
0.001<br />
Y A (t)<br />
τ<br />
Y B<br />
(t)<br />
same<br />
abundance<br />
level Y A<br />
(t=0)<br />
0<br />
10 -2 10 -1 10 0 10 1 10 2 10 3 10 4 10 5<br />
time<br />
Y<br />
Y<br />
A<br />
B<br />
( t)<br />
( t)<br />
=<br />
=<br />
Y<br />
Y<br />
0 A<br />
0 A<br />
e<br />
−λ<br />
t<br />
(1 −<br />
e<br />
−λ<br />
t<br />
)<br />
τ =<br />
1<br />
=<br />
λ<br />
1<br />
Y a<br />
ρ < σ v<br />
N A<br />
>
Energy production<br />
Reaction Q-value: Q<br />
Energy generated (if Q>0) by a s<strong>in</strong>gle reaction<br />
Q<br />
⎛<br />
2<br />
= c ⎜<br />
∑ m − ∑<br />
i<br />
m j<br />
⎝ <strong>in</strong>itial nuclei i f<strong>in</strong>al nuclei j<br />
⎞<br />
⎟<br />
⎠<br />
Difference between masses <strong>in</strong> entrance and exit channel<br />
Energy generation: Energy generated per g and sec by a reaction:<br />
ε<br />
r ⋅Q<br />
1<br />
= = Q ⋅ Y ⋅Y<br />
⋅ ρ ⋅ N<br />
2<br />
< σ v<br />
A a<br />
ρ 1+<br />
δ<br />
A<br />
aA<br />
>
Reaction Flow<br />
Reaction flow is def<strong>in</strong>ed as <strong>the</strong> net # of nuclei converted<br />
<strong>in</strong> time T from species A to B via a specific reaction<br />
F<br />
=<br />
T<br />
dY<br />
⎛ ⎞<br />
∫ ⎜<br />
A<br />
⎟ dt = ∫<br />
⎝ dt ⎠<br />
0<br />
via specific reaction<br />
T<br />
0<br />
λ( t)<br />
Y<br />
A<br />
( t)<br />
dt<br />
Reaction path is usually def<strong>in</strong>ed as <strong>the</strong> sequence of reactions<br />
with maximum reaction flow <strong>in</strong> a certa<strong>in</strong> stellar environment!
Reaction Network Simulations<br />
Reaction Network Simulations<br />
Change of istopic abundances:<br />
d Y<br />
d t i<br />
+<br />
i<br />
j,k,l<br />
of Stellar Nucleosyn<strong>the</strong>sis<br />
= Σ N λ Y + N ρ N < j,k ><br />
j<br />
2 2<br />
A j k l<br />
Σ N ρ N < j,k,l > Y Y Y<br />
j,k,l<br />
i<br />
j<br />
j<br />
(p,γ)<br />
(γ,p)<br />
j<br />
Σ j,k<br />
+<br />
(β ν)<br />
i<br />
j,k A j k<br />
(α,γ)<br />
Reaction flux = net number of reactions:<br />
Y Y +<br />
Coupled system of nonl<strong>in</strong>ear<br />
differential equations
A+p<br />
capture<br />
Resonance<br />
Cross-Section and S<br />
Cross section and reaction rate<br />
Section and S-Factor<br />
B<br />
energy<br />
cross section often expressed as S-factor<br />
A+p<br />
A+p<br />
Resonance<br />
B<br />
direct<br />
capture<br />
B<br />
cross section<br />
S(E) = σ(E) E exp(2πη)<br />
direct<br />
capture<br />
uncerta<strong>in</strong>ties at low energies<br />
due to deviations from<br />
Resonance<br />
l=0 Coulomb penetrability<br />
and due to threshold contributions<br />
energy<br />
cross section often expressed as S-factor<br />
S-factor<br />
direct<br />
capture<br />
energy<br />
Resonance<br />
S-factor to correct for Coulomb barrier: S(E) = σ(E) E e 2πη<br />
S(E) = σ(E) E exp(2πη)<br />
-factor<br />
direct<br />
capture
Example: 12 C(p,γ) cross section<br />
need cross section<br />
here !<br />
2π<br />
⋅η<br />
=<br />
2π<br />
⋅ Z<br />
h<br />
2<br />
1<br />
⋅ Z<br />
2⋅<br />
E<br />
μ<br />
2<br />
2<br />
cm<br />
⋅e<br />
2<br />
S(E) = σ ⋅E<br />
⋅e<br />
= 31.38⋅<br />
Z<br />
2<br />
1<br />
E<br />
⋅ Z<br />
cm<br />
2π<br />
⋅η<br />
2<br />
2<br />
⋅<br />
μ<br />
[ MeV ]
S-factor Conversion<br />
S≈1.3·10 -3 MeV-b<br />
From <strong>the</strong> NACRE compilation of charged particle <strong>in</strong>duced reaction rates on<br />
stable nuclei from H to Si (see C. Angulo et al. Nucl. Phys. A 656, 3 (1999);<br />
or: http://pntpm3.ulb.ac.be/Nacre/barre_database.htm)
Reaction rate from S-factorS<br />
If S-factor ~ constant over <strong>the</strong> Gamow range<br />
<strong>the</strong> rate is calculated <strong>in</strong> terms of <strong>the</strong> S-factor<br />
S(E)=S(E 0 )<br />
N<br />
A<br />
< σv<br />
>=<br />
7.83⋅10<br />
9<br />
⎛<br />
⎜<br />
⎝<br />
Z1Z<br />
μT<br />
9<br />
2<br />
⎞<br />
⎟<br />
⎠<br />
1/3<br />
S(<br />
E<br />
0<br />
)[MeV barn]<br />
e<br />
⎛<br />
−4.2487⎜<br />
⎝<br />
2<br />
1<br />
Z Z<br />
T<br />
9<br />
2<br />
2<br />
μ ⎞<br />
⎟<br />
⎠<br />
1/ 3<br />
O<strong>the</strong>rwise energy dependence needs to be approximated!
Example: 12 C(p,γ) 13<br />
13<br />
N<br />
Calculate <strong>the</strong> reaction rate as function of temperature!
Calculate life time of 12 C<br />
Determ<strong>in</strong>e 12 C life time <strong>in</strong> <strong>the</strong> sun T=0.015 GK!<br />
τ≈6 10 13 s = 2 10 6 y
Resonant Reaction Rate<br />
N<br />
A<br />
σv<br />
=<br />
.54⋅10<br />
⋅ωγ<br />
[ MeV ]<br />
⎛ 1<br />
⋅<br />
⎜<br />
⎝ μ ⋅T<br />
⎞<br />
⎟<br />
⎠<br />
3/ 2<br />
⋅e<br />
⎛ 11.605⋅E<br />
−<br />
⎜<br />
⎝ T<br />
R<br />
1<br />
11<br />
9<br />
9<br />
[ MeV ]<br />
⎞<br />
⎟<br />
⎠<br />
ωγ =<br />
2<br />
( J + 1)<br />
Γ<br />
⋅Γ<br />
<strong>in</strong> out<br />
⋅<br />
Γ =<br />
( ) ( )<br />
∑ tot<br />
Γ<br />
i i<br />
j + 1 ⋅2<br />
j + 1 Γ<br />
p<br />
2<br />
T<br />
tot<br />
Γ<br />
<strong>in</strong><br />
Θ<br />
p,<br />
α<br />
at low energy astrophysical conditions: Γ <strong>in</strong>
12 C(<br />
13 N<br />
Example: Calculate <strong>the</strong> 12 C(p, p,γ) 13<br />
resonance rate<br />
Resonance strength:<br />
Resonance energy:<br />
ωγ= 0.65 eV= 6.5 10 -7 MeV<br />
Experimental value: E<br />
cm<br />
r =0.45 MeV<br />
Assumed value: E<br />
cm<br />
r =0.05 MeV<br />
Significantly higher<br />
impact at lower energies!
Comparison between resonant and<br />
non-resonant contributions!<br />
Low energy resonances limit <strong>the</strong><br />
impact of non-resonant components!
Impact of effective life-time of isotope<br />
Fictitious low energy resonance reduces <strong>the</strong> life-time<br />
of solar 12 C from ~2 Million years to ~1 year only !
Reaction rates for <strong>in</strong>verse Processes<br />
Detailed balance between<br />
forward & <strong>in</strong>verse reaction.<br />
A(a,b)B<br />
The reaction rate ratio<br />
between <strong>the</strong> forward &<br />
<strong>the</strong> <strong>in</strong>verse reaction<br />
depends on <strong>the</strong> Q-value<br />
and <strong>the</strong> temperature T!<br />
kT=T[GK]/11.605<br />
μ=m 1·m 2<br />
/(m 1<br />
+m 2<br />
)
Photodis<strong>in</strong>tegrations Processes<br />
Equilibrium between forward<br />
and <strong>in</strong>verse processes<br />
Saha equation<br />
In units [1/s]