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U natural<br />

18 424<br />

Enrichment<br />

2434<br />

Depleted U<br />

15 990<br />

Uranium<br />

oxide<br />

fabrication<br />

Storage: two years<br />

Uranium oxide<br />

irradiation<br />

in LWR<br />

Losses (%)<br />

U 100<br />

Pu 100<br />

MA 100<br />

FP 100<br />

All mass flow in kg/TW·h(e)<br />

Losses:<br />

U 2276.01<br />

Pu 29.21<br />

MA 3.59<br />

High level waste<br />

TRU = 32.82 HM = 2308.83<br />

FIG. 5. The once through fuel cycle. FP: fission products.<br />

4.1.2. Plutonium recycling in light water reactor MOX<br />

Since natural uranium contains only 0.72% of the fissile 235 U isotope, the<br />

recycling of uranium and plutonium from spent fuel through the RFC scenario<br />

(Fig. 6) has been from the beginning of the nuclear era the standard scenario of<br />

nuclear energy production. There has, however, been reduced support for this<br />

approach in many States in recent years, owing to economic factors and particularly<br />

to proliferation concerns.<br />

By processing according to this RFC scenario, the major fraction<br />

(~99.9%) of the uranium and plutonium streams is extracted and only a very<br />

minor fraction of the major actinides is transferred to the HLLW (and consequently<br />

to the vitrified HLW) and eventually to the geologic repository.<br />

However, if public and/or political acceptance of very long term disposal<br />

of HLW cannot be obtained, the removal of MAs from high active residua or<br />

HLLW would be a technical solution that might reduce the residual radiotoxicity<br />

of the HLW. Moreover, with increasing burnup, the generation of MAs<br />

becomes more and more important. The addition of an MA partitioning<br />

37

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