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optical characterisation of rare-earth doped fluoride and phosphate ...

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107detuning can be written as a function <strong>of</strong> the input pump intensity, x x0 2= + KI inc jc j 2 ; (4.9)¡xwhere K is a constant dening the amount <strong>of</strong> spatial overlap between the perturbation<strong>and</strong> the energy distribution <strong>of</strong> the mode. This equation produces the black line inthe gure which scans across jc j 2 with increasing values <strong>of</strong> incident pump I inc . Theintersection points between the line <strong>and</strong> jc j 2 are solutions to the cubic equation inEqn. 4.7. The cubic equation in Eqn. 4.7 produces a response similar to that shownin Fig. 4.11(b). In reality, these intersections describe the positioning <strong>of</strong> the cavityresonance relative to the pump frequency (c.f. the movie linked in Fig. 4.11). In caseswhere the line intersects at three points for increasing I inc , the most stable positionis that with minimum detuning. Alternatively, for decreasing I inc , the most stableposition is that with maximum detuning. There are no stable solutions where the lineintersects two points. The internal microsphere intensity amplitude is jc j 2 E 2 o whereI inc / E 2 o. A theoretical bistable plot <strong>of</strong> the internal sphere eld is plotted in Fig.4.11(c) <strong>and</strong> clearly mimics the results in Fig. 4.6.Comparison <strong>of</strong> the bistability plots for IR lasing in Fig. 4.5 <strong>and</strong> uorescence in Fig.4.6 indicates somewhat unusual behaviour around the switch-low position. The IRlasing suddenly peaks at 10 mW launched power before switching to the lower state.All spheres have demonstrated this behaviour to a greater or lesser degree. Despitethis, the uorescence never shows a sudden jump before switching to the lower state.In particular, a sudden increase in absorption (as determined from the ratio <strong>of</strong> thetwo green emissions discussed in Section 4.3.3) in the sphere at this point, is neverobserved. There seems to be no similar eect observed in Fabry-Perot cavities <strong>and</strong>other resonators, which might have shed some insight onto the problem. A possible

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