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Annual Report 2009/2010 - JUWEL - Forschungszentrum Jülich

Annual Report 2009/2010 - JUWEL - Forschungszentrum Jülich

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In the drum, 4 ‘hot spots’ for Cs-137 and 1 ‘hot spot’ for Co-60 were identified. Two Cs-137-<br />

‘hot spots’ are positioned at a drum height of about 76 cm with the same radial position (13<br />

cm) but different angular positions (210° and 300°). The two other Cs-137-‘hot spots’ and<br />

the Co-60-‘hot spot’ are positioned at a drum height of about 60 cm with different radial and<br />

angular positions: (7 cm, 210°) and (11cm, 120°) for Cs-137 and (13 cm, 300°) for Co-60. It<br />

may be noted that the maximum of the count rate for a ‘hot spot’ occurred at a drum rotation<br />

angle - , which corresponds to the closest distance between the ‘hot spot’ and the<br />

detector during drum rotation. A second maximum may be observed at - <br />

depending on the ‘hot spot’ activity and position, the -ray energy and the attenuation<br />

properties of the matrix. The radioactive sources with an activity lower than 1 MBq are not<br />

detected because of the lead shielding structures. The mean thickness of the lead shielding<br />

in the drum segments containing the ‘hot spots’ was found to be 4 cm. The resulting activities<br />

of Cs-137 and Co-60 in the segments of the drum are shown in Fig. 92. They reflect well the<br />

axial distribution of the isotopes within the drums.<br />

Drum Segment<br />

1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20<br />

10 11 Drum Height [cm]<br />

10 10<br />

Cs-137<br />

Co-60<br />

10 9<br />

10 8<br />

Activity [Bq]<br />

10 7<br />

10 6<br />

10 5<br />

10 4<br />

10 3<br />

10 2<br />

4 8 12 16 20 24 28 32 36 40 44 48 52 56 60 64 68 70 74 78<br />

Fig. 92: Activity of Cs-137 and Co-60 in the segments of the drum with an apparent waste<br />

density of 2.63 g/cm 3 . The activity is calculated for a non uniform distribution of the<br />

isotopes and a heterogeneous sample matrix (see Fig. 3).<br />

The results obtained with the improved method compared to the true activity and to the<br />

activity calculated by the conventional method which assumes a homogeneous distribution of<br />

activity and matrix inside the drum segments are summarized for Cs-137 in Tab. 23. The<br />

mean ratio of calculated to true activity is shown for the different methods applied in Fig. 93.<br />

126

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