My PhD thesis - Condensed Matter Theory - Imperial College London
My PhD thesis - Condensed Matter Theory - Imperial College London
My PhD thesis - Condensed Matter Theory - Imperial College London
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CHAPTER 8. APPLYING THE PLASMON NORMAL MODE THEORY TO<br />
SLAB SYSTEMS<br />
the interface:<br />
⎧<br />
⎪⎨ ik<br />
K<br />
ρ s = ɛ<br />
m<br />
(−E 1 + E 2 ) − ik<br />
K v<br />
E 3 at z = 0<br />
0<br />
⎪ ( ⎩ − ik<br />
K v<br />
E 0 e −Kvs − ik −E1<br />
K m<br />
e −Kms + E 2 e Kms) at z = s.<br />
(8.44)<br />
The dependence on x and t is exactly as for the E-field. Using equations (8.34),<br />
(8.36) and (8.38), the various field amplitudes may be related to each other and thus<br />
eliminated (except for one):<br />
E 0 = ±e Kvs E 3<br />
E 1 = 1 − R E 3<br />
2<br />
E 2 = 1 + R E 3 .<br />
2<br />
(8.45a)<br />
(8.45b)<br />
(8.45c)<br />
The surface charge density is then<br />
ρ s = ± ɛ 0ik<br />
K v<br />
ω 2 p<br />
E<br />
ω 2 − ωp<br />
2 3 . (8.46)<br />
The positive sign always applies at z = 0. For symmetric oscillation, it is also taken<br />
at z = s: the surface charge density variations on the two interfaces are then in<br />
phase. The negative sign applies at z = s in the case of antisymmetric oscillation,<br />
so that the two surface charge densities are in antiphase. The lower branch of the<br />
dispersion graph corresponds to symmetric oscillation.<br />
The electric field created by the surface charge is given by the solution of equation<br />
(8.1), with a charge density of<br />
ρ(x, z, t) = ρ 0 (ω) ( δ(z) ± δ(z − s) ) e i(ωt−kx) . (8.47)<br />
This longitudinal (electrostatic) field may be expressed as the gradient of a scalar<br />
potential, φ. Assuming a solution of the form<br />
φ(x, z, t) = φ z (z)e i(ωt−kx) (8.48)<br />
means that the scalar potential must satisfy the equation<br />
)<br />
(−k 2 + d2<br />
φ<br />
dz 2 z (z) = − ρ 0<br />
(δ(z) ± δ(z − s)) . (8.49)<br />
ɛ 0<br />
129