VUV Spectroscopy of Atoms, Molecules and Surfaces

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Contents Preface iii 1 VUV light generation: possibilities and limitations 1 1.1 Introduction . . . . . . . . . . . . . . . . . . . . . . . . . . . . 1 1.2 Frequency mixing . . . . . . . . . . . . . . . . . . . . . . . . . 4 1.3 High-harmonic generation . . . . . . . . . . . . . . . . . . . . 6 1.4Comparison with other methods of VUV light- and X-ray generation . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 13 2 Negative ions 23 2.1 Introduction . . . . . . . . . . . . . . . . . . . . . . . . . . . . 23 2.2 Negative-ionstructure ...................... 24 2.3 Status on negative-ion knowledge . . . . . . . . . . . . . . . . 26 2.4Theoretical approaches to negative-ion structure . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 29 2.4.1 Computational methods . . . . . . . . . . . . . . . . . 29 2.4.2 The hyperspherical-coordinate approach . . . . . . . . 32 3 High-resolution VUV spectroscopy of H − 43 3.1 Introduction . . . . . . . . . . . . . . . . . . . . . . . . . . . . 4 3 3.2 Experimental approach. . . . . . . . . . . . . . . . . . . . . . 4 6 3.3 Resultsanddiscussion ...................... 50 3.4 Conclusion . . . . . . . . . . . . . . . . . . . . . . . . . . . . 56 4 4 4 Lifetimes of molecular negative ions 61 .1 Introduction . . . . . . . . . . . . . . . . . . . . . . . . . . . . 61 4.2 Notation and molecular quantum numbers . . . . . . . . . . . 63 .3 Experimental setup . . . . . . . . . . . . . . . . . . . . . . . . 64 4.4 N − 2 . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 65 68 4.5 CO − 2
Page 1: VUV Spectroscopy of Atoms, Molecule
Page 5 and 6: Preface The present thesis, submitt
Page 7 and 8: Acknowledgements In the course of m
Page 9 and 10: List of publications The thesis is
Page 11 and 12: Chapter 1 VUV light generation: pos
Page 13 and 14: 1.1 Introduction 3 The studies pres
Page 15 and 16: 1.2 Frequency mixing 5 the frequenc
Page 17 and 18: 1.3 High-harmonic generation 7 Inte
Page 19 and 20: 1.3 High-harmonic generation 9 can
Page 21 and 22: 1.3 High-harmonic generation 11 To
Page 23 and 24: 1.4 Comparison with other methods .
Page 25 and 26: 1.4 Comparison with other methods .
Page 27 and 28: References [1] H. Stapelfeldt et al
Page 29 and 30: REFERENCES 19 [33] K. J. Schafer et
Page 31 and 32: REFERENCES 21 [80] P. M. Paul et al
Page 33 and 34: Chapter 2 Negative ions 2.1 Introdu
Page 35 and 36: 2.2 Negative-ion structure 25 state
Page 37 and 38: 2.3 Status on negative-ion knowledg
Page 39 and 40: 2.4 Theoretical approaches to negat
Page 47 and 48: References [1] L.H.Andersenet al.,
Page 49 and 50: REFERENCES 39 [38] W. P. Wijesunder
Page 51 and 52: REFERENCES 41 [86] A. R. P. Rau, Re
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Chapter 3 High-resolution VUV spect
Page 55 and 56:
3.1 Introduction 45 Cross section (
Page 57 and 58:
3.2 Experimental approach 47 INJECT
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3.2 Experimental approach 49 Electr
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3.3 Results and discussion 51 Mean
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3.3 Results and discussion 53 Cross
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3.3 Results and discussion 55 Table
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3.4 Conclusion 57 Cross section (Mb
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References [1] A.R.P.Rau,J.Astrophy
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Chapter 4 Lifetimes of molecular ne
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4.2 Notation and molecular quantum
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4.4 N − 2 method. The upper limit
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4.4 N − 2 NEUTRAL YIELD 5 C-120-4
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4.5 CO − 2 linear CO2 molecules r
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4.5 CO − 2 the lowest-lying CO
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4.5 CO − 2 by sputtering, the sit
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References [1] C. Blondel, Physica
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REFERENCES 77 [41] A. Dreuw and L.
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Chapter 5 Femtosecond VUV core-leve
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5.1 Introduction 81 difference in o
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5.2 Laser-induced desorption 83 abi
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5.2 Laser-induced desorption 85 Fig
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5.2 Laser-induced desorption 87 the
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5.3 The technique of core-level spe
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5.3 The technique of core-level spe
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5.4 Core-level spectroscopic tests
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5.5 The VUV light source of high-or
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5.6 Future prospects 113 5.6 Future
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5.6 Future prospects 115 LEED Sputt
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5.6 Future prospects 117 core-ioniz
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References [1] G.A.Somorjoi,Introdu
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REFERENCES 121 [40] T. A. Germer et
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REFERENCES 123 [82] K. Siegbahn et
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REFERENCES 125 [128] T. Sasaki and
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Chapter 6 Two-colour pump-probe exp
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6.1 Introduction 129 lower levels a
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6.2 Experimental approach 131 with
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6.2 Experimental approach 133 Delay
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6.3 Results and discussion 135 Ion
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6.4 Conclusion 141 Ion signal (arb.
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References [1] A. Dalgarno and S. L
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REFERENCES 145 [37] J. Larsson et a
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Summary For an atom or molecule in
Page 159:
149 from the surface. A source of f
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VUV Spectroscopy of Atoms, Molecules and Surfaces

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