Heterogeneously Catalyzed Oxidation Reactions Using ... - CHEC

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4.6 References CHAPTER 4 [1] J.M. Thomas, R. Raja, Chem. Commun. (2001) 675. [2] J.M. Bregeault, Dalton Trans. (2003) 3289. [3] T. Punniyamurthy, S. Velusamy, J. Iqbal, Chem. Rev. 105 (2005) 2329. [4] A.K. Suresh, M.M. Sharma, T. Sridhar, Ind. Eng. Chem. Res. 39 (2000) 3958. [5] F. Ullmann, "Ullmann's encyclopedia of industrial chemistry", 6 th edition, Wiley‐VCH, Weinheim, 2003. [6] H.J. Rozie, M.L.C. Dsinter, J.B. Dakka, A. Zoran, Y. Sasson, PCT Int. Appl., 9,520,560 (1995). [7] M.L. Kantam, B.M. Choudary, P. Sreekanth, K.K. Rao, K. Naik, T.P. Kumar, A.A. Khan, Eur. Pat. Appl., 1,088,810 (2001). [8] S. Park, J.S. Yoo, K. Jun, D.B. Raju, Y. Kim, U.S. Patent, 6,476,257 (2002). [9] W. Partenheimer, Catal. Today 23 (1995) 69. [10] V. Kumar, P.D. Grover, Ind. Eng. Chem. Res. 30 (1991) 1139. [11] G. Busca, J. Chem. Soc. Faraday 89 (1993) 753. [12] J.S. Yoo, J.A. Donohue, M.S. Kleefisch, P.S. Lin, S.D. Elfline, Appl. Catal. A 105 (1993) 83. [13] P.A. Hamley, T. Ilkenhans, J.M. Webster, E. Garcia‐Verdugo, E. Venardou, M.J. Clarke, R. Auerbach, W.B. Thomas, K. Whiston, M. Poliakoff, Green Chem. 4 (2002) 235. [14] T. Seki, M. Baiker, Chem. Rev. 109 (2009) 2409. [15] H.V. Borgaonkar, S.R. Raverkar, S.B. Chandalia, Ind. Eng. Chem. Prod. Res. Dev. 23 (1984) 455. [16] M. Hronec, Z. Hrabe, Ind. Eng. Chem. Prod. Res. Dev. 25 (1986) 257. [17] M. Ilyas, M. Sadiq, Catal. Lett. 128 (2009) 337. [18] B. Chou, J. Tsai, S. Cheng, Microporous Mesporous Mater. 48 (2001) 309. [19] F. Wang, J. Xu, X. Li, J. Gao, L. Zhou, R. Ohnishi, Adv. Synth. Catal. 347 (2005) 1987. [20] R. Raja, J.M. Thomas, V. Dreyer, Catal. Lett. 110 (2006) 179. [21] R. Raja, J.M. Thomas, Solid State Sci. 8 (2006) 326. [22] M.J. Beier, T.W. Hansen, J.‐D. Grunwaldt, J. Catal. 266 (2009) 320. [23] R. Strobel, A. Baiker, S.E. Pratsinis, Adv. Powder Technol. 17 (2006) 457. [24] R. Kydd, W.Y. Teoh, K. Wong, Y. Wang, J. Scott, Q. Zeng, A. Yu, J. Zou, R. Amal, Adv. Funct. Mater. 19 (2009) 369. [25] S. Hannemann, J.‐D. Grunwaldt, P. Lienemann, D. Guenther, F. Krumeich, S.E. Pratsinis, A. Baiker, Appl. Catal. A 316 (2007) 226. [26] H. Schulz, L. Mädler, R. Strobel, R. Jossen, S.E. Pratsinis, T. Johannessen, J. Mater. Res. 20 (2005) 2568. [27] J. Yuan, X. Liao, H. Wang, G. Yang, M. Tang, J. Phys. Chem. B. 113 (2009) 1418. [28] T. Ressler, J. Synchrotron Radiat. 5 (1998) 118. 122
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TECHNICAL UNIVERSITY OF DENMARK (DT
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Preface The present dissertation su
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the carboxylic acid, ceria inhibite
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Resume Denne afhandling giver indle
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hvorimod mængden af katalysator ku
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2.3.8 Oxidation of sulfides .......
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5.3.5 Macroscopic mass transport in
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Chapter 1 Introduction With its gre
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1. Introduction Scheme 1‐1: High
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1. Introduction Figure 1‐2: Phase
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1. Introduction [28] S. Bawaked, N.
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2.1 Introduction 2.1 Introduction E
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2.2.1 Synthesis of gold catalysts 2
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2.2 Catalyst synthesis for oxidatio
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2.2 Catalyst synthesis for oxidatio
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2.3 Selective liquid‐phase oxidat
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Table 2-1: Overview over alcohol ox
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Ph O O Ph (4) (5) 2.3 Selective liq
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Table 2-4: Side-chain oxidation of
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2.3.4 Oxidation of cyclohexane 2.3
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Table 2-5: Oxidatin of cyclohexane.
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Table 2-6: Ring hydroxylation of ar
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Table 2-7: Aerobic oxidation of ami
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Table 2-8: Oxidation of hydroquinon
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Table 2-9: Oxidation of silanes wit
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Table 2-10: Oxidation reactions cat
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2.4 Strengths and opportunities of
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2.6 References 2.6 References [1] M
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2.6 References [56] H. Tumma, N. Na
Page 85 and 86: 2.6 References [113] C. Keresszegi,
Page 87 and 88: 2.6 References [169] Q. Zhu, Y. Lia
Page 89 and 90: 2.6 References [223] M. Fetizon, M.
Page 91 and 92: Chapter 3 Selective Liquid-Phase Ox
Page 93 and 94: 3.2 Experimental 3.2.1 Catalyst pre
Page 95 and 96: 3.3 Results Scattering amplitudes a
Page 97 and 98: Absorption (a.u.) 1.2 1.0 0.8 0.6 0
Page 99 and 100: Conversion (%) 100 90 80 70 60 50 4
Page 101 and 102: 3.3 Results Figure 3‐5: In situ X
Page 103 and 104: 3.3 Results Table 3‐2: Conversion
Page 105 and 106: 3.3 Results In order to gain insigh
Page 107 and 108: 3.3 Results the cost of selectivity
Page 109 and 110: 3.4 Discussion synergetic interacti
Page 111 and 112: 3.5 Conclusions to corroborate the
Page 113 and 114: 3.6 References [29] T. Mitsudome, Y
Page 115 and 116: Chapter 4 Selective Side-Chain Oxid
Page 117 and 118: 4.2 Experimental single‐step flam
Page 119 and 120: 4.2 Experimental alcohol (Aldrich,
Page 121 and 122: 4.3 Results Scheme 4‐1: Oxidation
Page 123 and 124: 4.3 Results Figure 4‐2: Formation
Page 125 and 126: 4.3 Results oxidation by either 2,6
Page 127 and 128: Absorption (a.u.) Absorption (a.u.)
Page 129 and 130: 4.3 Results atomic mixing of Ag and
Page 131 and 132: 4.3 Results Figure 4‐7: Influence
Page 133 and 134: 4.4 Discussion and mechanistic cons
Page 135: 4.5 Conclusions heterogeneous radic
Page 139 and 140: Chapter 5 Experimental Determinatio
Page 141 and 142: 5.2 Experimental The most important
Page 143 and 144: 5.2 Experimental Eurotherm 2216e te
Page 145 and 146: Figure 5-1: Schematic view of the e
Page 147 and 148: (Eq. 5‐5) AB i j ε AB i j β 5.2
Page 149 and 150: (a) (b) (c) (d) (e) (f) (g) (h) (i)
Page 151 and 152: 5.3 Results two association sites o
Page 153 and 154: Pressure (bar) 150 145 140 135 5.3
Page 155 and 156: 5.3 Results Figure 5‐7: Oxidation
Page 157 and 158: Weight (g) 5.3 Results Figure 5‐8
Page 159 and 160: 5.4 Discussion catalytic reactions
Page 161 and 162: 5.4 Discussion corresponding CO2‐
Page 163 and 164: 5.5 Conclusions 5.5 Conclusions The
Page 165 and 166: 5.6 References [29] I. Tsivintzelis
Page 167 and 168: 6.1 Introduction 6.1 Introduction A
Page 169 and 170: 6.2 Experimental [38]. In a typical
Page 171 and 172: 6.3 Results out in 1 mm quartz tube
Page 173 and 174: 6.3 Results Figure 6‐2: Structure
Page 175 and 176: 6.3 Results Figure 6‐4: Epoxidati
Page 177 and 178: 6.3 Results Figure 6‐6: Compariso
Page 179 and 180: 6.3 Results Figure 6‐8: Influence
Page 181 and 182: 6.3 Results investigated the epoxid
Page 183 and 184: 6.3 Results Figure 6‐10: Co‐epo
Page 185 and 186: 6.3 Results Figure 6‐11: EXAFS an
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6.4 Discussion would need to be for
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6.5 Conclusions Formation of the ep
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6.6 References [28] J. Perles, N. S
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Chapter 7 Concluding Remarks 7.1 Co
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7.2 Final remarks and outlook speci
Page 197 and 198:
Acknowledgements Acknowledgements T
Page 199:
Curriculum Vitae Matthias Josef Bei
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