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6.6 References CHAPTER 6 [1] F. Ullmann, "Ullmann's encyclopedia of industrial chemistry", 6 th edition, Wiley‐VCH, Weinheim, 2003. [2] M. McCoy, M.S. Reisch, A.H. Tullo, J. Tremblay, M. Voith, Chem. Eng. News 87 (2009) 51. [3] M. Dusi, T. Mallat, A. Baiker, Catal. Rev. Sci. Eng. 42 (2000) 213. [4] R. Murugavel, H.W. Roesky, Angew. Chem. Int. Edit. 36 (1997) 477. [5] A. Corma, H. Garcia, Chem. Rev. 102 (2002) 3837. [6] M.D. Hughes, Y.J. Xu, P. Jenkins, P. McMorn, P. Landon, D.I. Enache, A.F. Carley, G.A. Attard, G.J. Hutchings, F. King, E.H. Stitt, P. Johnston, K. Griffin, C.J. Kiely, Nature 437 (2005) 1132. [7] M. Turner, V.B. Golovko, O.P.H. Vaughan, P. Abdulkin, A. Berenguer‐Murcia, M.S. Tikhov, B.F.G. Johnson, R.M. Lambert, Nature 454 (2008) 981. [8] P. Lignier, S. Mangematin, F. Morfin, J. Rousset, V. Caps, Catal. Today 138 (2008) 50. [9] C. Aprile, A. Corma, M.E. Domine, H. Garcia, C. Mitchell, J. Catal. 264 (2009) 44. [10] F. Loeker, W. Leitner, Chem. Eur. J. 6 (2000) 2011. [11] D. Dhar, Y. Koltypin, A. Gedanken, S. Chandrasekaran, Catal. Lett. 86 (2003) 197. [12] E. Angelescu, R. Ionescu, O.D. Pavel, R. Zavoianu, R. Birjega, C.R. Luculescu, M. Florea, R. Olar, J. Mol. Catal. A 315 (2010) 178. [13] Q.H. Tang, Y. Wang, J. Liang, P. Wang, Q.H. Zhang, H.L. Wan, Chem. Commun. (2004) 440. [14] M. Salavati‐Niasari, S. Abdolmohammadi, M. Oftadeh, J. Coord. Chem. 61 (2008) 2837. [15] M.V. Patil, M.K. Yadav, R.V. Jasra, J. Mol. Catal. A 277 (2007) 72. [16] M.L. Kantam, B.P.C. Rao, R.S. Reddy, N.S. Sekhar, B. Sreedhar, B.M. Choudary, J. Mol. Catal. A 272 (2007) 1. [17] X. Zhang, C. Zeng, L. Zhang, N. Xu, Kinet. Catal. 50 (2009) 199. [18] X. Lu, Q. Xia, S. Fang, B. Xie, B. Qi, Z. Tang, Catal. Lett. 131 (2009) 517. [19] Q.H. Tang, Q.H. Zhang, H.L. Wu, Y. Wang, J. Catal. 230 (2005) 384. [20] J. Jiang, R. Li, H. Wang, Y. Zheng, H. Chen, J. Ma, Catal. Lett. 120 (2008) 221. [21] K.M. Jinka, J. Sebastian, R.V. Jasra, J. Mol. Catal. A 274 (2007) 33. [22] X. Quek, Q. Tang, S. Hu, Y. Yang, Appl. Catal. A 361 (2009) 130. [23] Z. Opre, T. Mallat, A. Baiker, J. Catal. 245 (2007) 482. [24] J. Lee, O.K. Farha, J. Roberts, K.A. Scheidt, S.T. Nguyen, J.T. Hupp, Chem. Soc. Rev. 38 (2009) 1450. [25] A.U. Czaja, N. Trukhan, U. Mueller, Chem. Soc. Rev. 38 (2009) 1284. [26] F.X. Llabres i Xamena, A. Abad, A. Corma, H. Garcia, J. Catal. 250 (2007) 294. [27] K. Brown, S. Zolezzi, P. Aguirre, D. Venegas‐Yazigi, V. Paredes‐Garcia, R. Baggio, M.A. Novak, E. Spodine, Dalton Trans. (2009) 1422. 176
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TECHNICAL UNIVERSITY OF DENMARK (DT
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Preface The present dissertation su
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the carboxylic acid, ceria inhibite
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Resume Denne afhandling giver indle
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hvorimod mængden af katalysator ku
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2.3.8 Oxidation of sulfides .......
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5.3.5 Macroscopic mass transport in
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Chapter 1 Introduction With its gre
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1. Introduction Scheme 1‐1: High
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1. Introduction Figure 1‐2: Phase
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1. Introduction [28] S. Bawaked, N.
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2.1 Introduction 2.1 Introduction E
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2.2.1 Synthesis of gold catalysts 2
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2.2 Catalyst synthesis for oxidatio
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2.2 Catalyst synthesis for oxidatio
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2.3 Selective liquid‐phase oxidat
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Table 2-1: Overview over alcohol ox
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Ph O O Ph (4) (5) 2.3 Selective liq
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Table 2-4: Side-chain oxidation of
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2.3.4 Oxidation of cyclohexane 2.3
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Table 2-5: Oxidatin of cyclohexane.
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Table 2-6: Ring hydroxylation of ar
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Table 2-7: Aerobic oxidation of ami
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Table 2-8: Oxidation of hydroquinon
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Table 2-9: Oxidation of silanes wit
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Table 2-10: Oxidation reactions cat
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2.4 Strengths and opportunities of
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2.6 References 2.6 References [1] M
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2.6 References [56] H. Tumma, N. Na
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2.6 References [113] C. Keresszegi,
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2.6 References [169] Q. Zhu, Y. Lia
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2.6 References [223] M. Fetizon, M.
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Chapter 3 Selective Liquid-Phase Ox
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3.2 Experimental 3.2.1 Catalyst pre
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3.3 Results Scattering amplitudes a
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Absorption (a.u.) 1.2 1.0 0.8 0.6 0
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Conversion (%) 100 90 80 70 60 50 4
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3.3 Results Figure 3‐5: In situ X
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3.3 Results Table 3‐2: Conversion
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3.3 Results In order to gain insigh
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3.3 Results the cost of selectivity
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3.4 Discussion synergetic interacti
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3.5 Conclusions to corroborate the
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3.6 References [29] T. Mitsudome, Y
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Chapter 4 Selective Side-Chain Oxid
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4.2 Experimental single‐step flam
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4.2 Experimental alcohol (Aldrich,
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4.3 Results Scheme 4‐1: Oxidation
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4.3 Results Figure 4‐2: Formation
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4.3 Results oxidation by either 2,6
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Absorption (a.u.) Absorption (a.u.)
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4.3 Results atomic mixing of Ag and
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4.3 Results Figure 4‐7: Influence
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4.4 Discussion and mechanistic cons
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4.5 Conclusions heterogeneous radic
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4.6 References [29] S.I. Zabinsky,
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Page 147 and 148: (Eq. 5‐5) AB i j ε AB i j β 5.2
Page 149 and 150: (a) (b) (c) (d) (e) (f) (g) (h) (i)
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Page 153 and 154: Pressure (bar) 150 145 140 135 5.3
Page 155 and 156: 5.3 Results Figure 5‐7: Oxidation
Page 157 and 158: Weight (g) 5.3 Results Figure 5‐8
Page 159 and 160: 5.4 Discussion catalytic reactions
Page 161 and 162: 5.4 Discussion corresponding CO2‐
Page 163 and 164: 5.5 Conclusions 5.5 Conclusions The
Page 165 and 166: 5.6 References [29] I. Tsivintzelis
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Page 169 and 170: 6.2 Experimental [38]. In a typical
Page 171 and 172: 6.3 Results out in 1 mm quartz tube
Page 173 and 174: 6.3 Results Figure 6‐2: Structure
Page 175 and 176: 6.3 Results Figure 6‐4: Epoxidati
Page 177 and 178: 6.3 Results Figure 6‐6: Compariso
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Page 181 and 182: 6.3 Results investigated the epoxid
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Page 185 and 186: 6.3 Results Figure 6‐11: EXAFS an
Page 187 and 188: 6.4 Discussion would need to be for
Page 189: 6.5 Conclusions Formation of the ep
Page 193 and 194: Chapter 7 Concluding Remarks 7.1 Co
Page 195 and 196: 7.2 Final remarks and outlook speci
Page 197 and 198: Acknowledgements Acknowledgements T
Page 199: Curriculum Vitae Matthias Josef Bei
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