Heterogeneously Catalyzed Oxidation Reactions Using ... - CHEC

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TECHNICAL UNIVERSITY OF DENMARK (DT
Page 3 and 4:
Preface The present dissertation su
Page 5 and 6:
the carboxylic acid, ceria inhibite
Page 7 and 8:
Resume Denne afhandling giver indle
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hvorimod mængden af katalysator ku
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2.3.8 Oxidation of sulfides .......
Page 13 and 14:
5.3.5 Macroscopic mass transport in
Page 15 and 16:
Chapter 1 Introduction With its gre
Page 17 and 18:
1. Introduction Scheme 1‐1: High
Page 19 and 20:
1. Introduction Figure 1‐2: Phase
Page 21 and 22:
1. Introduction [28] S. Bawaked, N.
Page 23 and 24:
2.1 Introduction 2.1 Introduction E
Page 25 and 26:
2.2.1 Synthesis of gold catalysts 2
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2.2 Catalyst synthesis for oxidatio
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2.2 Catalyst synthesis for oxidatio
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2.3 Selective liquid‐phase oxidat
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Table 2-1: Overview over alcohol ox
Page 35 and 36:
2.3 Selective liquid‐phase oxidat
Page 37 and 38: 2.3 Selective liquid‐phase oxidat
Page 45 and 46: Ph O O Ph (4) (5) 2.3 Selective liq
Page 51 and 52: Table 2-4: Side-chain oxidation of
Page 53 and 54: 2.3.4 Oxidation of cyclohexane 2.3
Page 55 and 56: Table 2-5: Oxidatin of cyclohexane.
Page 59 and 60: Table 2-6: Ring hydroxylation of ar
Page 63 and 64: Table 2-7: Aerobic oxidation of ami
Page 65 and 66: Table 2-8: Oxidation of hydroquinon
Page 69 and 70: Table 2-9: Oxidation of silanes wit
Page 71 and 72: Table 2-10: Oxidation reactions cat
Page 73 and 74: 2.4 Strengths and opportunities of
Page 81 and 82: 2.6 References 2.6 References [1] M
Page 83 and 84: 2.6 References [56] H. Tumma, N. Na
Page 85 and 86: 2.6 References [113] C. Keresszegi,
Page 87: 2.6 References [169] Q. Zhu, Y. Lia
Page 91 and 92: Chapter 3 Selective Liquid-Phase Ox
Page 93 and 94: 3.2 Experimental 3.2.1 Catalyst pre
Page 95 and 96: 3.3 Results Scattering amplitudes a
Page 97 and 98: Absorption (a.u.) 1.2 1.0 0.8 0.6 0
Page 99 and 100: Conversion (%) 100 90 80 70 60 50 4
Page 101 and 102: 3.3 Results Figure 3‐5: In situ X
Page 103 and 104: 3.3 Results Table 3‐2: Conversion
Page 105 and 106: 3.3 Results In order to gain insigh
Page 107 and 108: 3.3 Results the cost of selectivity
Page 109 and 110: 3.4 Discussion synergetic interacti
Page 111 and 112: 3.5 Conclusions to corroborate the
Page 113 and 114: 3.6 References [29] T. Mitsudome, Y
Page 115 and 116: Chapter 4 Selective Side-Chain Oxid
Page 117 and 118: 4.2 Experimental single‐step flam
Page 119 and 120: 4.2 Experimental alcohol (Aldrich,
Page 121 and 122: 4.3 Results Scheme 4‐1: Oxidation
Page 123 and 124: 4.3 Results Figure 4‐2: Formation
Page 125 and 126: 4.3 Results oxidation by either 2,6
Page 127 and 128: Absorption (a.u.) Absorption (a.u.)
Page 129 and 130: 4.3 Results atomic mixing of Ag and
Page 131 and 132: 4.3 Results Figure 4‐7: Influence
Page 133 and 134: 4.4 Discussion and mechanistic cons
Page 135 and 136: 4.5 Conclusions heterogeneous radic
Page 137 and 138: 4.6 References [29] S.I. Zabinsky,
Page 139 and 140:
Chapter 5 Experimental Determinatio
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5.2 Experimental The most important
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5.2 Experimental Eurotherm 2216e te
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Figure 5-1: Schematic view of the e
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(Eq. 5‐5) AB i j ε AB i j β 5.2
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(a) (b) (c) (d) (e) (f) (g) (h) (i)
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5.3 Results two association sites o
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Pressure (bar) 150 145 140 135 5.3
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5.3 Results Figure 5‐7: Oxidation
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Weight (g) 5.3 Results Figure 5‐8
Page 159 and 160:
5.4 Discussion catalytic reactions
Page 161 and 162:
5.4 Discussion corresponding CO2‐
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5.5 Conclusions 5.5 Conclusions The
Page 165 and 166:
5.6 References [29] I. Tsivintzelis
Page 167 and 168:
6.1 Introduction 6.1 Introduction A
Page 169 and 170:
6.2 Experimental [38]. In a typical
Page 171 and 172:
6.3 Results out in 1 mm quartz tube
Page 173 and 174:
6.3 Results Figure 6‐2: Structure
Page 175 and 176:
6.3 Results Figure 6‐4: Epoxidati
Page 177 and 178:
6.3 Results Figure 6‐6: Compariso
Page 179 and 180:
6.3 Results Figure 6‐8: Influence
Page 181 and 182:
6.3 Results investigated the epoxid
Page 183 and 184:
6.3 Results Figure 6‐10: Co‐epo
Page 185 and 186:
6.3 Results Figure 6‐11: EXAFS an
Page 187 and 188:
6.4 Discussion would need to be for
Page 189 and 190:
6.5 Conclusions Formation of the ep
Page 191 and 192:
6.6 References [28] J. Perles, N. S
Page 193 and 194:
Chapter 7 Concluding Remarks 7.1 Co
Page 195 and 196:
7.2 Final remarks and outlook speci
Page 197 and 198:
Acknowledgements Acknowledgements T
Page 199:
Curriculum Vitae Matthias Josef Bei
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