Heterogeneously Catalyzed Oxidation Reactions Using ... - CHEC

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5.6 References CHAPTER 5 [1] M. Besson, P. Gallezot, Catal. Today 57 (2000) 127. [2] J.H.J. Kluytmans, A.P. Markusse, B.F.M. Kuster, G.B. Marin, J.C. Schouten, Catal. Today 57 (2000) 143. [3] T. Mallat, A. Baiker, Chem. Rev. 104 (2004) 3037. [4] A.M. Steele, J. Zhu, S.C. Tsang, Catal. Lett. 73 (2001) 9. [5] Z. Hou, N. Theyssen, W. Leitner, DGMK Tagungsber. 2005‐2 (2005) 61. [6] M. Caravati, J.‐D. Grunwaldt, A. Baiker, Catal. Today 91‐2 (2004) 1. [7] M. Caravati, J.‐D. Grunwaldt, A. Baiker, Phys. Chem. Chem. Phys. 7 (2005) 278. [8] M. Caravati, D.M. Meier, J.‐D. Grunwaldt, A. Baiker, J. Catal. 240 (2006) 126. [9] G. Jenzer, M.S. Schneider, R. Wandeler, T. Mallat, A. Baiker, J. Catal. 199 (2001) 141. [10] M. Caravati, J.‐D. Grunwaldt, A. Baiker, Catal. Today 126 (2007) 27. [11] X. Wang, H. Kawanami, S.E. Dapurkar, N.S. Venkataramanan, M. Chatterjee, T. Yokoyama, Y. Ikushima, Appl. Catal. A 349 (2008) 86. [12] B. Kimmerle, J.‐D. Grunwaldt, A. Baiker, Top. Catal. 44 (2007) 285. [13] G. Musie, M. Wei, B. Subramaniam, D.H. Busch, Coord. Chem. Rev. 219 (2001) 789. [14] J.‐D. Grunwaldt, R. Wandeler, A. Baiker, Catal. Rev. Sci. Eng. 45 (2003) 1. [15] T. Seki, M. Baiker, Chem. Rev. 109 (2009) 2409. [16] G. Jenzer, T. Mallat, A. Baiker, Catal. Lett. 73 (2001) 5. [17] R. Glaser, R. Jos, J. Williardt, Top. Catal. 22 (2003) 31. [18] A. Baiker, Chem. Rev. 99 (1999) 453. [19] I.G. Economou, Ind. Eng. Chem. Res. 41 (2002) 953. [20] C. Panayiotou, I.C. Sanchez, Macromolecules 24 (1991) 6231. [21] G.M. Kontogeorgis, E.C. Voutsas, I.V. Yakoumis, D.P. Tassios, Ind. Eng. Chem. Res. 35 (1996) 4310. [22] G.M. Kontogeorgis, M.L. Michelsen, G.K. Folas, S. Derawi, N. von Solms, E.H. Stenby, Ind. Eng. Chem. Res. 45 (2006) 4855. [23] G.M. Kontogeorgis, M.L. Michelsen, G.K. Folas, S. Derawi, N. von Solms, E.H. Stenby, Ind. Eng. Chem. Res. 45 (2006) 4869. [24] C. Crampon, G. Charbit, E. Neau, J. Supercrit. Fluid. 16 (1999) 11. [25] R. Wandeler, N. Kunzle, M.S. Schneider, T. Mallat, A. Baiker, J. Catal. 200 (2001) 377. [26] NIST Standard Reference Database, available at http://www.nist.org/news.php, last accessed 12/2010. [27] S.H. Huang, M. Radosz, Ind. Eng. Chem. Res. 29 (1990) 2284. [28] M. Chiu, S. Chen, H. Hsu, C. Lee, T. Chiu, J. Chin. Inst. Chem. Eng. 3 (1972) 113. 150
5.6 References [29] I. Tsivintzelis, M.J. Beier, J.‐D. Grunwaldt, A. Baiker, G.M. Kontogeorgis, Fluid Phase Equilib., available at DOI: 10.1016/j.fluid.2010.10.001. [30] DIPPR DIADEM‐ The DIPPR Information and Data Evaluation Manager for the Design Institute for Physical Properties. 2006, Version1.1.0. (Computer Program). [31] J. Chen, M. Lee, Fluid Phase Equilib. 130 (1997) 231. [32] A. Fredenslund, G.A. Sather, J. Chem. Eng. Data 15 (1970) 17. [33] A. Bamberger, G. Sieder, G. Maurer, J. Supercrit. Fluid. 17 (2000) 97. [34] J.A. Nighswander, N. Kalogerakis, A.K. Mehrotra, J. Chem. Eng. Data 34 (1989) 355. [35] J. Kiepe, S. Horstmann, K. Fischer, J. Gmehling, Ind. Eng. Chem. Res. 41 (2002) 4393. [36] H.N. Sólimo, M.B. Gramajo de Doz, Fluid Phase Equilib. 107 (1995) 213. [37] R.M. Stephenson, J. Chem. Eng. Data 38 (1993) 630. [38] P.S. Pavlova, D.M. Popov, V.M. Olevskii, Tr. Gos. Nauch. Issled. Proekt. Inst. Azotn. Prom. Prod. Org. Sin. No. 15 (1972) 89. [39] D. Walther, G. Maurer, Phys. Chem. Chem. Phys. 96 (1992) 981. [40] D. Walther, G. Maurer, J. Chem. Eng. Data 38 (1993) 247. [41] J.‐D. Grunwaldt, M. Caravati, M. Ramin, A. Baiker, Catal. Lett. 90 (2003) 221. [42] J.‐D. Grunwaldt, M. Caravati, A. Baiker, J. Phys. Chem. B 110 (2006) 25586. [43] Y. Xie, Z. Zhang, S. Hu, J. Song, W. Li, B. Han, Green Chem. 10 (2008) 278. [44] C. Keresszegi, T. Burgi, T. Mallat, A. Baiker, J. Catal. 211 (2002) 244. [45] C. Keresszegi, J.‐D. Grunwaldt, T. Mallat, A. Baiker, J. Catal. 222 (2004) 268. [46] J.‐D. Grunwaldt, C. Keresszegi, T. Mallat, A. Baiker, J. Catal. 213 (2003) 291. [47] C. Keresszegi, D. Ferri, T. Mallat, A. Baiker, J. Phys. Chem. B 109 (2005) 958. 151
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TECHNICAL UNIVERSITY OF DENMARK (DT
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Preface The present dissertation su
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the carboxylic acid, ceria inhibite
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Resume Denne afhandling giver indle
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hvorimod mængden af katalysator ku
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2.3.8 Oxidation of sulfides .......
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5.3.5 Macroscopic mass transport in
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Chapter 1 Introduction With its gre
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1. Introduction Scheme 1‐1: High
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1. Introduction Figure 1‐2: Phase
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1. Introduction [28] S. Bawaked, N.
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2.1 Introduction 2.1 Introduction E
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2.2.1 Synthesis of gold catalysts 2
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2.2 Catalyst synthesis for oxidatio
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2.2 Catalyst synthesis for oxidatio
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2.3 Selective liquid‐phase oxidat
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Table 2-1: Overview over alcohol ox
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Ph O O Ph (4) (5) 2.3 Selective liq
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Table 2-4: Side-chain oxidation of
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2.3.4 Oxidation of cyclohexane 2.3
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Table 2-5: Oxidatin of cyclohexane.
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Table 2-6: Ring hydroxylation of ar
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Table 2-7: Aerobic oxidation of ami
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Table 2-8: Oxidation of hydroquinon
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Table 2-9: Oxidation of silanes wit
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Table 2-10: Oxidation reactions cat
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2.4 Strengths and opportunities of
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2.6 References 2.6 References [1] M
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2.6 References [56] H. Tumma, N. Na
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2.6 References [113] C. Keresszegi,
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2.6 References [169] Q. Zhu, Y. Lia
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2.6 References [223] M. Fetizon, M.
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Chapter 3 Selective Liquid-Phase Ox
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3.2 Experimental 3.2.1 Catalyst pre
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3.3 Results Scattering amplitudes a
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Absorption (a.u.) 1.2 1.0 0.8 0.6 0
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Conversion (%) 100 90 80 70 60 50 4
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3.3 Results Figure 3‐5: In situ X
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3.3 Results Table 3‐2: Conversion
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3.3 Results In order to gain insigh
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3.3 Results the cost of selectivity
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3.4 Discussion synergetic interacti
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3.5 Conclusions to corroborate the
Page 113 and 114: 3.6 References [29] T. Mitsudome, Y
Page 115 and 116: Chapter 4 Selective Side-Chain Oxid
Page 117 and 118: 4.2 Experimental single‐step flam
Page 119 and 120: 4.2 Experimental alcohol (Aldrich,
Page 121 and 122: 4.3 Results Scheme 4‐1: Oxidation
Page 123 and 124: 4.3 Results Figure 4‐2: Formation
Page 125 and 126: 4.3 Results oxidation by either 2,6
Page 127 and 128: Absorption (a.u.) Absorption (a.u.)
Page 129 and 130: 4.3 Results atomic mixing of Ag and
Page 131 and 132: 4.3 Results Figure 4‐7: Influence
Page 133 and 134: 4.4 Discussion and mechanistic cons
Page 135 and 136: 4.5 Conclusions heterogeneous radic
Page 137 and 138: 4.6 References [29] S.I. Zabinsky,
Page 139 and 140: Chapter 5 Experimental Determinatio
Page 141 and 142: 5.2 Experimental The most important
Page 143 and 144: 5.2 Experimental Eurotherm 2216e te
Page 145 and 146: Figure 5-1: Schematic view of the e
Page 147 and 148: (Eq. 5‐5) AB i j ε AB i j β 5.2
Page 149 and 150: (a) (b) (c) (d) (e) (f) (g) (h) (i)
Page 151 and 152: 5.3 Results two association sites o
Page 153 and 154: Pressure (bar) 150 145 140 135 5.3
Page 155 and 156: 5.3 Results Figure 5‐7: Oxidation
Page 157 and 158: Weight (g) 5.3 Results Figure 5‐8
Page 159 and 160: 5.4 Discussion catalytic reactions
Page 161 and 162: 5.4 Discussion corresponding CO2‐
Page 163: 5.5 Conclusions 5.5 Conclusions The
Page 167 and 168: 6.1 Introduction 6.1 Introduction A
Page 169 and 170: 6.2 Experimental [38]. In a typical
Page 171 and 172: 6.3 Results out in 1 mm quartz tube
Page 173 and 174: 6.3 Results Figure 6‐2: Structure
Page 175 and 176: 6.3 Results Figure 6‐4: Epoxidati
Page 177 and 178: 6.3 Results Figure 6‐6: Compariso
Page 179 and 180: 6.3 Results Figure 6‐8: Influence
Page 181 and 182: 6.3 Results investigated the epoxid
Page 183 and 184: 6.3 Results Figure 6‐10: Co‐epo
Page 185 and 186: 6.3 Results Figure 6‐11: EXAFS an
Page 187 and 188: 6.4 Discussion would need to be for
Page 189 and 190: 6.5 Conclusions Formation of the ep
Page 191 and 192: 6.6 References [28] J. Perles, N. S
Page 193 and 194: Chapter 7 Concluding Remarks 7.1 Co
Page 195 and 196: 7.2 Final remarks and outlook speci
Page 197 and 198: Acknowledgements Acknowledgements T
Page 199: Curriculum Vitae Matthias Josef Bei
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