Thermal properties in mesoscopics: physics and ... - ResearchGate
Thermal properties in mesoscopics: physics and ... - ResearchGate
Thermal properties in mesoscopics: physics and ... - ResearchGate
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two superconduct<strong>in</strong>g contacts <strong>and</strong> δG is a positive temperature<br />
<strong>and</strong> voltage-dependent correction to the conductance.<br />
Its magnitude for typical geometries is at maximum<br />
some 0.1GN. The proximity-<strong>in</strong>duced conductance<br />
correction is widely studied <strong>in</strong> the literature <strong>and</strong> we refer<br />
to (Belzig et al., 1999; Lambert <strong>and</strong> Raimondi, 1998) for<br />
a more detailed list of references on this topic.<br />
The thermal conductance of Andreev <strong>in</strong>terferometers<br />
has been studied very recently. The formulation of the<br />
problem is very similar as for the conductance correction.<br />
For E ≪ ∆, there is no energy current <strong>in</strong>to the superconductors.<br />
Therefore, it is enough to solve for the energy<br />
current jL = DL∂xf L <strong>in</strong> the wires 1, 2 <strong>and</strong> 5. This yields<br />
˙Q = GN /e 2<br />
<br />
dEEDL(E)(f L eq(E; T2) − f L eq(E; T1)),<br />
where f L eq(E; T ) = tanh[E/(2kBT )] <strong>and</strong> the thermal<br />
conductance correction is obta<strong>in</strong>ed from DL(E) =<br />
( L dx<br />
0 DL(x;E) /L)−1 . Here the spatial <strong>in</strong>tegral runs along<br />
the wire between the two normal-metal reservoirs. In<br />
the general case, DL has to be calculated numerically.<br />
The thermal conductance correction has been analyzed<br />
by Bezuglyi <strong>and</strong> V<strong>in</strong>okur (2003) <strong>and</strong> Jiang <strong>and</strong> Ch<strong>and</strong>rasekhar<br />
(2005b). They found that it can be strongly<br />
modulated with the phase φ: <strong>in</strong> the short-junction limit<br />
where ET ≫ ∆, for φ = 0, DL almost vanishes, whereas<br />
for φ = π, DL approaches unity <strong>and</strong> thus the thermal<br />
conductance approaches its normal-state value. For a<br />
long junction with ET ∆, the effect becomes smaller,<br />
but still clearly observable. The first measurements<br />
(Jiang <strong>and</strong> Ch<strong>and</strong>rasekhar, 2005a) of the proximity<strong>in</strong>duced<br />
correction to the thermal conductance show the<br />
predicted tendency of the phase-dependent decrease of κ<br />
compared to the normal-state (Wiedemann-Franz) value.<br />
Prior to the experiments on heat conductance <strong>in</strong> proximity<br />
structures, the thermoelectric power α was experimentally<br />
studied <strong>in</strong> Andreev <strong>in</strong>terferometers (Dik<strong>in</strong><br />
et al., 2002a,b; Eom et al., 1998; Jiang <strong>and</strong> Ch<strong>and</strong>rasekhar,<br />
2004; Parsons et al., 2003a,b). The observed<br />
thermopower was surpris<strong>in</strong>gly large, of the order of 100<br />
neV/K — at least one to two orders of magnitude larger<br />
than the thermopower <strong>in</strong> normal-metal samples. Also<br />
contrary to the Mott relation (c.f., below Eqs. (39)),<br />
this value depends nonmonotonically on the temperature<br />
(Eom et al., 1998) at the temperatures of the order of a<br />
few hundred mK, <strong>and</strong> even a sign change could be found<br />
(Parsons et al., 2003b). Moreover, the thermopower was<br />
found to oscillate as a function of the phase φ. The symmetry<br />
of the oscillations has <strong>in</strong> most cases been found to<br />
be antisymmetric with respect to φ = 0, i.e., α vanishes<br />
for φ = 0. However, <strong>in</strong> some measurements, the Ch<strong>and</strong>rasekhar’s<br />
group (Eom et al., 1998; Jiang <strong>and</strong> Ch<strong>and</strong>rasekhar,<br />
2004) have found symmetric oscillations, i.e.,<br />
α had the same phase as the conductance.<br />
The observed behavior of the thermopower is not completely<br />
understood, but the major features can be expla<strong>in</strong>ed.<br />
The first theoretical predictions were given by<br />
α SN,2 ( µV/K)<br />
4<br />
3<br />
2<br />
1<br />
T0 , V= 0 T0 , V= 0<br />
φ S S φ<br />
3<br />
5<br />
4<br />
2<br />
2<br />
1 2<br />
N N<br />
T1, V1<br />
T2, V2 0<br />
0 5 10<br />
k T / E<br />
B 2 T<br />
15<br />
14<br />
FIG. 7 Supercurrent-<strong>in</strong>duced N-S thermopower αNS for the<br />
system depicted <strong>in</strong> the <strong>in</strong>set. Solid l<strong>in</strong>e: αNS at T1 ≈ T2. Dotted<br />
l<strong>in</strong>e: approximation (47). The correction (48) accounts<br />
for most of the difference. Dashed l<strong>in</strong>e: αNS at kBT1 = 3.6ET<br />
with vary<strong>in</strong>g T2. Dash-dotted l<strong>in</strong>e: the correspond<strong>in</strong>g approximation.<br />
Inset: Andreev <strong>in</strong>terferometer where thermoelectric<br />
effects are studied. Two superconduct<strong>in</strong>g reservoirs with<br />
phase difference φ are connected to two normal-metal reservoirs<br />
through diffusive normal-metal wires. Adapted from<br />
(Virtanen <strong>and</strong> Heikkilä, 2004b).<br />
Claughton <strong>and</strong> Lambert (1996), who constructed a scatter<strong>in</strong>g<br />
theory to describe the effect of Andreev reflection<br />
on the thermoelectric <strong>properties</strong> of proximity systems.<br />
Based on their work, it was shown (Heikkilä et al., 2000)<br />
that the presence of Andreev reflection can lead to a violation<br />
of the Mott relation. This means that a f<strong>in</strong>ite<br />
thermopower can arise even <strong>in</strong> the presence of electronhole<br />
symmetry. Seviour <strong>and</strong> Volkov (2000b), Kogan et al.<br />
(2002), <strong>and</strong> Virtanen <strong>and</strong> Heikkilä (2004a,b) showed that<br />
<strong>in</strong> Andreev <strong>in</strong>terferometers carry<strong>in</strong>g a supercurrent, a<br />
large voltage can be <strong>in</strong>duced by the temperature gradient<br />
both between the normal-metal reservoirs <strong>and</strong> between<br />
the normal metals <strong>and</strong> the superconduct<strong>in</strong>g contacts.<br />
Virtanen <strong>and</strong> Heikkilä (2004b) showed that <strong>in</strong> long<br />
junctions, the <strong>in</strong>duced voltages between the two normalmetal<br />
reservoirs <strong>and</strong> the superconductors can be related<br />
to the temperature dependent equilibrium supercurrent<br />
IS(T ) flow<strong>in</strong>g between the two superconductors via<br />
V 0<br />
1/2<br />
= 1<br />
2<br />
R5(2R4/3 + R5)R3/4 [IS(T1) − IS(T2)]<br />
. (47)<br />
RNNNRSNS<br />
Here RNNN = R1 + R2 + R5, RSNS = R3 + R4 + R5<br />
<strong>and</strong> Rk are the resistances of the five wires def<strong>in</strong>ed <strong>in</strong><br />
the <strong>in</strong>set of Fig. 7. This is <strong>in</strong> most situations the dom<strong>in</strong>ant<br />
term <strong>and</strong> it can be also phenomenologically argued<br />
based on the temperature dependence of the supercurrent<br />
<strong>and</strong> the conservation of total current (supercurrent<br />
plus quasiparticle current) <strong>in</strong> the circuit (Virtanen <strong>and</strong><br />
Heikkilä, 2004b). A similar result can also be obta<strong>in</strong>ed<br />
<strong>in</strong> the quasiequilibrium limit for the l<strong>in</strong>ear-response thermopower<br />
(Virtanen <strong>and</strong> Heikkilä, 2004a). In addition to<br />
this term, the ma<strong>in</strong> correction <strong>in</strong> the long-junction limit<br />
comes from the anomalous coefficient T an ,<br />
eV 1<br />
1/2 = ∓R1/2 〈T<br />
RNNN<br />
an<br />
1/2 〉 ∓ R3/4R5 〈T<br />
RNNNRSNS<br />
an<br />
5 〉. (48)<br />
Lk<br />
0 dx ∞<br />
0<br />
Here 〈T an<br />
1<br />
an<br />
k 〉 ≡ dET Lk<br />
k (E)[f L eq(E, T1) −<br />
f L eq(E, T2)] <strong>and</strong> Lk is the length of wire k. One f<strong>in</strong>ds