Thesis for the Degree of Doctor of Philosophy - DTU Orbit

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Liu, Y., Gunten, H.R., 1988. Migration chemistry and behaviour of iodine relevant to geological disposal of radioactive wastes, A literature review with a compilation of sorption data, PSI-16, Paul Scherrer Institute, Switzerland. Moore RM., Zafiriou, OC. 1994. Photochemical production of methyl iodide in seawater. J. Geophys. Res. 99, 16415-16420 Reifenhäuser C & Heumann KG. 1990. Development of a definitive method for iodine speciation in aquatic systems. Fresenius J. Anal. Chem., 336: 559-563. Reithmeier H, Lazarev V, Ruhm W, Nolte E. 2007. 129I measurements in lake water for an estimate of regional 129I depositions. Science of the total environment. 376, 285-293. Schwehr KA. 2003. 129I and 127I in the environment. Ph.D. Dissertation, Department of Oceanography, Texas A&M Universtity, College Station, TX, 2003. Stevenson, F.J., 1994. Humic Chemistry: Genesis, Composition, Reactions, 2nd ed. Wiley, New York. Wong, G. T. F. 1991. The marine geochemistry of iodine. Rev. Aquat. Sci., 4 (1), 45-73. Wong G.T.F. and Cheng X.H. (2001).The formation of iodide in inshore waters from the photochemical decomposition of dissolved organic iodine.Mar. Chem. 74, 53-64. Wong, G.T.F., Zhang, L.S., 2003. The geochemical dynamics of iodine in marginal seas: the southern East China Sea. Deep-Sea Reasearch (II), 50, 1147-1162. Zic V & Branica M. 2006. The distributions of iodate and iodide in Rogoznica Lake (East Adriatic Coast). Estuarine, Coastal and Shelf Science 66, 55-66 12
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Chemical Speciation Analysis and En
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Thesis for the Degree of Doctor of
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Abstract This thesis deals with che
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environment since they reflect the
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organiske jodformer. Adsorption af
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None of this would have been possib
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Abbreviations and acronyms b+ - pos
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3.1 Analytical Development………
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Table 1 Some properties of iodine P
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In soils/sediments iodine occurs as
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Table 2 Nuclear properties of iodin
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Liquid scintillation counting (LSC)
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The bioavailability of radioactive
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data (Englund et al., 2010; Hou et
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2. Analytical procedures used in th
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2.3 Quantification of total iodine
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Fig. 5 Quantification of total iodi
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iodate were measured by counting 12
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Fig. 6 Sequential extraction proced
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a Fig. 8 Calibration curve for (a)
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experiment was subjected to combust
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Table 7 Adsorption of iodine specie
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numbers 11-14), which is about the
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marine environment from nuclear fue
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127 I - (ppb) 127 IO3 - (ppb) a b 1
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Although the oxygen concentration d
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129 I TBq 2,00E+00 1,80E+00 1,60E+0
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• Adsorption of iodine species on
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Reference Aldahan A, Kekli A, Possn
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Fuge R& Johnson C. 1986. The geoche
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Lo´pez-Gutie´rrez JM, Garcı ´a-
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Shinohara K. 2004. Measurement and
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http://www.irsn.fr/EN/news/Document
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Review Analytica Chimica Acta 632 (
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Table 1 Nuclear properties and prod
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Fig. 2. Liquid discharges of 129 I
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Fig. 5. Schematic diagram and pictu
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129 I in iodide and iodate is then
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Fig. 8. Diagram of air sampler for
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Fig. 10. Iodine L3-edge (a) and K-e
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analysis of 129 I in water sample a
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Yi P, Aldahan A, Hansen V, Possnert
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FIGURE 1. Sampling sites (the red s
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FIGURE 3. Horizontal distribution o
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FIGURE 5. Time series data of 129 I
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Environmental Science & Technology
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prepared using KI and KIO3. No diff
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of their contribution to the Baltic
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Fig. S-1 Sampling sites (the red so
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Fig. S-3 Vertical distribution of I
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Fig. S-5 Marine discharges function
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Fig.S-7 Relationship between I-129
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Table S-1 Results of I-129 and I-12
Page 107 and 108: S17
Page 109 and 110: Paper III Hansen,V., Yi, P., Hou, X
Page 111 and 112: conversion process between iodide a
Page 113 and 114: Table 1 Analytical results of 129 I
Page 115 and 116: August April I-129 iodide ( 10 8 at
Page 117 and 118: References Aldahan A, Kekli A, Poss
Page 119 and 120: Partition of iodine ( 129 I and 127
Page 121 and 122: Norway (Table 1). CTD-casts with ox
Page 123 and 124: 5. Discussion 5.1. Separation of hu
Page 125 and 126: In the present study 40e60% of 129
Page 127 and 128: Hutta, M., Gora, R., 2003. Novel st
Page 129 and 130: Analysis of 129 I and 127 I in arch
Page 131 and 132: et al., 2002). Due to the fact that
Page 133 and 134: espectively. The iodine was leached
Page 135 and 136: salinities in the same area. Apart
Page 137 and 138: North Sea. 129 I/ 127 I ratios in w
Page 139 and 140: Table 2 Analytical results of 129-I
Page 141 and 142: 129 I/ 127 I 1,40E-07 1,20E-07 1,00
Page 143 and 144: References Aldahan A, Englund E, Po
Page 145 and 146: O’Dowd, C.; Jimenez, J. L.; Bahre
Page 147 and 148: Iodine ( 129 I and 127 I) speciatio
Page 149 and 150: water in winter by molecular oxygen
Page 151 and 152: 0.2 M KNO3. The effluent and the wa
Page 153 and 154: maximum values is at 0.03-0.06×10
Page 155 and 156: into the English Channel from the L
Page 157: References Aldahan A, Kekli A, Poss
Page 161: Risø DTU is the National Laborator
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Thesis for the Degree of Doctor of Philosophy - DTU Orbit

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