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Etude de la combustion de gaz de synthèse issus d'un processus de ...

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Introduction<br />

proves to have higher efficiency. In fact, gasification is seen as one of the most<br />

promising ways to produce energy from biomass (Knoef, 2003).<br />

Table 1.1 - Thermo-chemical processes efficiency (Bridgwater, 2003)<br />

Process Liquid Coal Gas<br />

Pyrolysis 75% 12% 13%<br />

Gasification 5% 10% 85%<br />

The main attraction of this technology is the production of a fuel gas, elsewhere called<br />

produced gas or syngas, which can be used into an engine or turbine for power<br />

production. Besi<strong>de</strong>s, the low heating value of syngas its advantages over conventional<br />

<strong>combustion</strong> in terms of pollutants emissions, particu<strong>la</strong>rly of nitrous oxi<strong>de</strong>s (NO x ) and<br />

soot are <strong>de</strong>terminant for its use.<br />

tel-00623090, version 1 - 13 Sep 2011<br />

1.1 Motivation and objective<br />

Syngas obtained from gasification of biomass is consi<strong>de</strong>red to be an attractive new<br />

fuel, especially for stationary power generation. The research in this field has been<br />

focused upstream the syngas production, and therefore there is a <strong>la</strong>ck of knowledge at<br />

the downstream level of the syngas production manly as far as <strong>combustion</strong><br />

characteristics is concerned.<br />

The consi<strong>de</strong>rable variation of syngas composition is a challenge in <strong>de</strong>signing efficient<br />

end use applications such as burners and <strong>combustion</strong> chambers to suit changes in fuel<br />

composition. Designing such <strong>combustion</strong> appliances needs fundamental un<strong>de</strong>rstanding<br />

of the implications of variation of different constituents of syngas fuel for its <strong>combustion</strong><br />

characteristics, such as the burning velocity.<br />

Burning velocity values for single component fuels such as methane and hydrogen are<br />

abundantly avai<strong>la</strong>ble in the literature for various operating conditions. Some studies on<br />

burning velocities are also avai<strong>la</strong>ble for binary fuel mixtures such as H 2 –CH 4 (Halter et<br />

al., 2005; Coppens et al., 2007), and H 2 –CO (Vagelopoulos and Egolfopoulos, 1994;<br />

McLean et al., 1994; Brown et al., 1996; Sun et al., 2007).<br />

Natarajan et al., (2007) test an equally weighted, 50:50 H 2 -CO, fuel mixture with 0 and<br />

20% CO 2 dilution. Prathap et al. (2008) study the effect of N 2 dilution on <strong>la</strong>minar<br />

burning velocity and f<strong>la</strong>me structure for H 2 –CO (50% H 2 –50% CO by volume) fuel<br />

mixtures. All these studies use unreal syngas compositions. Therefore, there is <strong>la</strong>ck of<br />

knowledge in the fundamental <strong>combustion</strong> characteristics of actual syngas<br />

compositions where there is a combined effect of N 2 and CO 2 dilution in the H 2 -CO-CH 4<br />

fuel gases that composes the actual syngas fuel. This motivated the present work to<br />

14

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