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Thesis High-Resolution Photoemission Study of Kondo Insulators ...

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6.3. Results and Discussion 89<br />

<strong>of</strong> EF . Under this normalization, the DOS at − 50 meV and − 80 meV are almost<br />

identical and both decrease slightly on cooling for all samples.<br />

DOS(T) / DOS(300 K)<br />

0<br />

- 0 meV<br />

- 20 meV<br />

- 50 meV<br />

- 80 meV<br />

100<br />

T (K)<br />

Yb 1-x Lu x B 12<br />

200<br />

x = 0.00<br />

x = 0.25<br />

x = 0.50<br />

x = 0.75<br />

x = 1.00<br />

Figure 6.10: Temperature-dependent DOS <strong>of</strong> Yb1−xLuxB12 at various energies. We<br />

have re-normalized the DOS to the values at 300 K.<br />

We subtracted the DOS at 7 K from those at 300 K for each x in Fig. 6.11. As<br />

is visible in Fig. 6.9, the depressed DOS is always positive under the normalization<br />

in Fig. 6.9. At − 80 meV, the depressed DOS decreases as Yb content increases corresponding<br />

to the evolution <strong>of</strong> the broad peak. The x dependence at − 50 meV is<br />

substantially the same as that at − 80 meV. The depression is much stronger at − 20<br />

meV but its response against x resembles that at − 50 meV and − 80 meV. However,<br />

the x dependence at EF is qualitatively different from those below − 20 meV: The<br />

depression at EF is identical to that at − 20 meV for x ≥ 0.5 but the depression at<br />

EF is remarkably enhanced for x ≤ 0.25. This indicates that the sharp (pseudo)gap,<br />

which opens less than 20 meV from EF and governs the low-temperature transport and<br />

thermodynamic properties <strong>of</strong> YbB12, disappears between x = 0.25 and 0.50. Such a<br />

nonlinear response at EF against x would suggest that the effect beyond the single-site<br />

mechanism plays an important role in the low-energy electronic properties in YbB12<br />

300

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