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sites in humic substances: Testing the BEST7 program with a weak-acid mixture", Analytica Chimica Acta, vol.5445, p. 86-98 DEINES Peter, 1980, "The carbon isotopic composition of diamonds: relationship to diamond shape, color, occurrence and vaport composition", Geochimica et Cosmochimica Acta, vol.44, p. 943-961 DEL CASTILLO Carlos E., COBLE Paula G., MORELL Julio M., LOPEZ José M., CORREDOR Jorge E., 1999, "Analysis of the optical properties of the Orinoco River plume by absorption and fluorescence spectroscopy", Marine Chemistry, vol.66, p.35-51 DEL CASTILLO Carlos E., COBLE Paula G., 2000, "Seasonal variability of the colored dissolved organic matter during the 1994-95 NE and SW Monsoons in the Arabian Sea", Deep-Sea Research II, vol.47, p. 1563-1579 DEL VECCHIO Rossana, BLOUGH Neil V., 2002, "Photobleaching of chromophoric dissolved organic matter in natural waters: kinetics and modeling", Marine Chemistry, vol.78, p. 231-253 DEL VECCHIO Rossana, BLOUGH Neil V., 2004, "Spatial and seasonal distribution of chromophoric dissolved organic matter and dissolved organic carbon in the Middle Alantic Bight", Marine Chemistry, vol.89, p. 169-187 DIGNAC Marie-France, SCRIBE Pierre (directeur de thèse), 1998, "Caractérisation chimique de la matière organique au cours du traitement des eaux usées par boues actives – Chemical characterization of organic matter during the treatment of wastewater by activated sludge process", Thèse, Université de Paris 6. DONARD O.F.X., LAMOTTE M., BELIN C., EWALD M., 1989, "High-Sensitivity Fluorescence Spectroscopy of Mediterranean Waters Using a Conventional or a Pulsed Laser Excitation Source", Marine Chemistry, vol.27, p. 117-136 DUAN Zicheng, FIELD Robert W., YAMAKITA Nami, TSUCHIYA Soji, 2006, "Differential temperature laser induced fluorescence spectroscopy", Chemical Physics, vol.324, p. 709-720 DUDAL Y., HOLGADO R., MAESTRI G., GUILLON E., DUPONT L., 2006, "Rapid screening of DOM’s metal-binding ability using a fluorescence-based microplate assay", Science of the Total Environment, vol. 354, p. 286– 291 DUDLEY R.L., FYFE C.A., 1982, "Evaluation of the quantitative reliability of the 13C CP/MAS technique for the analysis of coals and related materials", Fuel A., vol.61, p. 651–657 ELKINS Kelly M., NELSON Donald J., 2001, "Fluorescence and FT-IR spectroscopy studies of Suwannee river fulvic acid complexation with aluminum, terbium and calcium", Journal of Inorganic Biochemistry, vol.87, p. 81-96 ESTEVES DA SILVA Joaquim C.G., MACHADO Adélio A.S.C., 1995, "Evolving factor analysis of synchronous fluorescence spectra of humic substances in the presence of Cu(II)", Chemometrics and Intelligent Laboratory Systems, vol.27, p. 115-128 ESTEVES DA SILVA Joaquim C.G., MACHADO Adélio A.S.C., 1996, "Characterization of the binding sites for Al(III) and Be(II) in a sample of marine fulvic acids", Marine Chemistry, vol.54, p. 135
293-302 ESTEVES DA SILVA Joaquim C.G., MACHADO Adélio A.S.C., SILVA Carla S.P.C.O., 1996, "Simultaneous use of evolving factor analysis of fluorescence spectral data and analysis of pH titration data for comparison of the acid-base properties of fulvic acids", Analytica Chimica Acta, vol. 318, p. 365-372 ESTEVES DA SILVA Joaquim C.G., MACHADO Adélio A.S.C., OLIVEIRA César J.S., PINTO Marta S.S.D.S., 1998, "Fluorescence quenching of anthropogenic fulvic acids by Cu(II), Fe(III) and UO2 2+ ", Talanta, vol.45, p. 1155-1165 ESTEVES DA SILVA Joaquim C.G., TAVARES Maria J.C.G., TAULER Romá, 2006, "Multivariate curve resolution of multidimensional excitation-emission quenching matrices of a Laurentian soil fulvic acid", Chemosphere, vol.64, p. 1939-1948 FERNÁNDEZ-CALVIÑO D., SOLER-ROVIRA P., POLO A., ARIAS-ESTÉVEZ M., PLAZA C., 2010, "Influence of humified organic matter on copper behavior in acid polluted soils", Environmental Pollution, vol.158, p. 3634-3641 FERRARI G.M., MINGAZZINI M., 1995, "Synchronous fluorescence spectra of dissolved organic matter (DOM) of algal origin in marine coastal waters", Marine Ecology Progress Series A., vol.125, p. 305-315 FILELLA Montserrat, TOWN Raewyn, 2000, "Determination of metal ion binding parameters for humic substances Part 1. Application of a simple calculation method for extraction of meaningful parameters from reverse pulse polarograms", Journal of Electroanalytical Chemistry, vol.485, p. 21-33 FLORENCE T.M., BATLEY G.E., 1980, "Chemical Speciation in Natural Waters", Analytical Chemistry, vol.9, p. 1962 FUENTES Marta, GONZÁLEZ-GAITANO Gustavo, GARCÍA-MINA José M., 2006, "The usefulness of UV-visible and fluorescence spectroscopies to study the chemical nature of humic substances from soils and composts", Organic Geochemistry, vol.37, p. 1949-1959 FUKUSHIMA M., TANAKA S., NAKAYASU K., 1997, "Investigation of copper(II)-binding behavior of fulvic acids by three-dimensional fluorescence spectrometry", Analytical sciences A., vol.13, p. 1011-1015 GALAPATE Ritchelita P., BAES Aloysius U., ITO Kazuaki, MUKAI Tetsuo, SHOTO Eiji, OKADA Mitsumasa, 1998, "Detection of Domestic Wastes in Kurose River Using Synchronous Fluorescence Spectroscopy", Water Research, vol.32, p. 2232-2239 GARCIA-MINA Jose M., 2006, "Stability, solubility and maximum metal binding capacity in metal–humic complexes involving humic substances extracted from peat and organic compost", Organic Geochemistry, vol.37, p. 1960-1972 GARNIER Cédric, Thèse, 2004, "Modélisation et évaluation des équilibres de complexation entre la matière organique naturelle, les métaux traces et le proton : applications aux eaux naturelles", Université du Sud Toulon - Var, 200 pages 136
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Ecole Doctorale SCIENCES DE L’ENV
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~~至爸爸妈妈~~ A papa et maman
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Remerciements : Approchant de la fi
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i Table des matières INTRODUCTION
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iii IV.F.6 Milieu des eaux intersti
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La science restera toujours la sati
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FACtor analysis » (PARAFAC). A l
Page 16 and 17:
Le bon sens surtout vaut mieux que
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4 Condensation Acides humiques (AH)
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insolubles dans l’eau quelque soi
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matière organique, des propriété
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phénoliques (φ-OH) ou hydroxyles
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12 I.D.1.b Fonctions et structures
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Kogut, 2001 ;Louis et al., 2008), p
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La science doit être tirée de la
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L’absorption d’un photon ne dur
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Un exemple de l’utilisation de ce
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20 I F lc ( ) −2, 303ε ( λ ) (
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PM. Le gain du tube PM dépend donc
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24 jusqu'à la mer des Sargasses A
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elaxation de la fluorescence qui es
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On définit le temps de vie τ de f
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optiques de ce dernier. Les électr
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Chapitre III. MOD et spectroscopie
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La spectroscopie de fluorescence es
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Figure 18: Exemple de l’image MEE
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l’environnement (Stedmon, Markage
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III.C.2.b Effets d’écran Puisque
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normés γn des N composants et de
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L’équation 43 permet de modélis
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Chapitre IV. Fluo 3D : ubiquité ou
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L’objectif de cette étude est un
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Les eaux de sol (ES) sont prélevé
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Figure 25: Site des prélèvements
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Figure 28: Plan des sites de prél
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IV.A.7 Bosnie (ED) Les prélèvemen
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IV.B Paramètres d’acquisition de
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Ensuite, les couples de MEEF sont a
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A: B: Une fois le traitement achev
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λex λex 450 400 350 300 450 400 3
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λex 450 400 350 300 250 300 400 λ
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λex 450 400 350 300 250 300 400 λ
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pics fluorescents considérés des
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C4 entre les contributions des acid
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Figure 51: Composants obtenus par P
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Figure 54: Composants obtenus par P
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Comme dans l’interprétation pré
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λex souvent considéré comme fais
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λex Figure 64: Composants globaux
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Nom de milieu Nom de mission N° de
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IV.F Application de PARAFAC aux mis
Page 105 and 106: Le composant 2 (λEX/λEM = 295nm/3
Page 107 and 108: Finalement, pour les eaux de mer, l
Page 109 and 110: Nom de milieu Eaux douces Nom de mi
Page 111 and 112: Ainsi, il ne suffit pas d'avoir un
Page 113 and 114: l'analyse globale est très proche
Page 115 and 116: A) B) T) présents dans les eaux c
Page 117 and 118: Nom de milieu Résumé des fluoroph
Page 119 and 120: Les lignes A, B, C et T représente
Page 121 and 122: A: distingue 3 zones pour des longu
Page 123 and 124: A : respectrivement) possède globa
Page 125 and 126: A: λex B: C: D: λex 450 400 350 3
Page 127 and 128: Chapitre V. Phénomènes de complex
Page 129 and 130: L’interaction entre la MON dissou
Page 131 and 132: Un exemple célèbre de Buffle (198
Page 133 and 134: des intensités des ligands libres
Page 135 and 136: 2009) ; ou encore la MON dissoute (
Page 137: fluorescence en envisageant une vis
Page 140 and 141: 115 VI.A Couplage PARAFAC - PROSECE
Page 143 and 144: Conclusion et perspectives
Page 145 and 146: La matière organique naturelle (MO
Page 147: Dans ce travail, l’échantillon
Page 150 and 151: La science du passé est d’un gra
Page 152 and 153: BAKER Andy, 2001, "Fluorescence Exc
Page 154 and 155: 1526-1528 CABANISS Stephen E., 1992
Page 158 and 159: GHEORGHIU C., SMITH D.S., AL-REASI
Page 160 and 161: HOLLAS J. Michael, 1998, "Spectroph
Page 162 and 163: LLOYD J.B.F., 1971, "Synchronized e
Page 164 and 165: vol.181, p. 28-32 MIANO T.M., SENES
Page 166 and 167: OHNO Tsutomu, GRIFFIN Timothy S., L
Page 168 and 169: acid", Journal of Photochemistry an
Page 170 and 171: STOBER Q.J., JONES R.D., SCHEIDT D.
Page 172 and 173: organisms as inferred from their or
Page 174 and 175: Articles d’avertissement CHAN Win
Page 176 and 177: 155 Figure 35: Composants obtenus p
Page 178 and 179: Annexe 2 - Liste des Tableaux 157 T
Page 180 and 181: PARAFAC : 159 Auteur Année Baghoth
Page 182 and 183: 161
Page 184 and 185: 163
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