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Figure 4.1.4 Distri bution ofsamp les along (a) 1st PC, (b) 2nd PC and (c) 3rd PC identified by PeA utilizing concentrations of 7 selected compounds (Ae, Fl. Fa. BbF. Per. DBA. BP). Three first PCs explained 95.8% oftotal variance in samples.
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POLYCYCLIC AROMATIC HYDROCARBONS IN
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composition. Portions ofthe lake th
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TABLE OF CONTENTS . ABSTRAcr._._ _
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6. CONCLUSIONS_._ _....._._._ _ ._
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FIGURE 3.104 CONfIGURATION OF ISOCH
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FIGURE 4 .2.12 SAMPLES AND PROMINEN
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fIGURE 5.3.1 DESCR1Pl1VE MODEL OF S
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APPENDIX B 3 _ T HEoerwt Of A PtUNC
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Ip » Ideno(l,2.3 cd)pyrene NIST =
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Figure L 1.1 The 16 parental polycy
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After release by the primary source
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decomposition processes (O'Malley e
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Figure 2.1.1 The Great Lakes draina
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;: Duluth Chicago 1 J Lake Superior
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are the Black River, the Cuyaho ga
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Figure 1.1.5 The pattern of permane
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sedimentary basins, Western. Centra
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Figure 2. 1.8 Summer (July) air and
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Natural Resources: The lower Great
Page 57 and 58: American waters under the current U
Page 60 and 61: continuously overflowed com bined s
Page 63 and 64: 3.1 EXPERIMENTAL 3. METHODS 3.1.1 S
Page 66 and 67: Table 3,1.1 Locations and types ofs
Page 68: Figure 3.12 Extraction and purifica
Page 72 and 73: hexane. 2) the unsaturated aliphati
Page 75: this problem. Ratios ofthe two stab
Page 78: Figure 3. 1.4 Configuration ofIsoch
Page 82 and 83: 3.2.1 UNl- AND BIVAJUATE METHODS Th
Page 84: f igure 3.2. 1 Mean and range (± s
Page 87 and 88: utilized the same instrument (Isoch
Page 90 and 91: Selecting lIt1J'iahlu: It was demon
Page 92 and 93: w- _ 71
Page 95 and 96: seven variables with fewer missing
Page 97 and 98: analysis also employed a greate r n
Page 99: description. The second cluster ana
Page 104 and 105: elationships between different site
Page 107: Figure 4.1.3 Regression ofthree fir
Page 115 and 116: The western zone is characterized b
Page 118: Figure 4.1.7. Regress ion ofthree f
Page 122 and 123: that at Cbeland. Conversely, Detroi
Page 124: Figure 42 .1 Ratios ofselected 4-,
Page 127: Figure 4.2.2 Samp les and prominent
Page 131 and 132: implies that compounds there either
Page 133: Figure 4.1.4 Weights ofvariables (c
Page 136 and 137: Figure 4.1.5 Distribution orsamples
Page 138 and 139: The third PC is responsible for 11.
Page 142 and 143: sources on the graphs for Pa, Fa. B
Page 145 and 146: These sources contribute as much as
Page 147: Figure 4.2.8 Samples and prominent
Page 151: Figure 4.2. 10 Samples andprominent
Page 155: Figure 4.2.12 Samples and prominent
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Figure 4.2. 14 Samples and prominen
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Figure 4.2.16 Samples and prominent
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towards light values ofBePlBaP in a
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info nnation sec Section 3.2..2}. A
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-s: Cl 5 4 3 .a; ;0 2 .2: '" -.!l1
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Another 10.5% ofvariance is explain
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Table 5.1.1 Three clusters identifi
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mo re pervasive background signatur
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figure S.U Zones (clusters) in the
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is diverted in litis direction (Fig
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Figure 5.1.6 Station locations and
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the Detroit river (969, 358, 351) t
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(Fig. 4.1 .8a, 5. tA) can also be a
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Figure 5.1.9 Statio n locations and
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Figure 5.1.10 Surface drifter track
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f igure 5.1.12 Drift card trajector
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Figure 5. t .13 Driftobject tracks
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In conclus ion. fluvial input of PA
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Figure 5.2. 1 Cloud ofsamples andpr
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increased amount oflight eas ily pe
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Figure 5.2.2 Cloud ofsamples and pr
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Figure 5.:!.3 Six clusters identifi
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mass balance calculations show that
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The processes ofdegradation might p
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Although less intensive than at Det
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The processes ofweathering do not s
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subzones ofinfluence was suggested.
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possesses similar isotopic composit
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fallout office soots as indicated b
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confined to the northern part ofthe
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Section 5.1); may still be affected
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their relative position with respec
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5.3 A MODEL OF SOURCES, PATHWAYS. T
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originate from the Maumee River at
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6. CONCLUSIONS The major conclusion
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7. REFERENCES Abrajano T. A. Jr.•
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Einsenreich S. J. and Strachan W. M
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Lee R. F. and Takahashi M. ( 1977)
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Sherrill T. W. and Saylor G. S. (19
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8. APPENDICES 242
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l' Appendix AS. Characteristic PAil
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Appeodil: A1. The hyperbolic equati
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... '"
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Appeadil. 82. 1bc output of a princ
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Appendix 84. The output o r a princ
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Appendix C3 . The results ora local
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