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Figure 4.2.11 Samples and prominent primary and secondary sources on BePlBaP vs. Fa plot. Mixing curves are generated using nonnalized concentrations (A ppendix AJ) and isotopic values (Appendix A4) in the two component mixing model described in Appe ndix A7. The error bars represe nt the range <strong>of</strong>statistical variations in end-mem bers.
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POLYCYCLIC AROMATIC HYDROCARBONS IN
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composition. Portions ofthe lake th
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TABLE OF CONTENTS . ABSTRAcr._._ _
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6. CONCLUSIONS_._ _....._._._ _ ._
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FIGURE 3.104 CONfIGURATION OF ISOCH
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FIGURE 4 .2.12 SAMPLES AND PROMINEN
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fIGURE 5.3.1 DESCR1Pl1VE MODEL OF S
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APPENDIX B 3 _ T HEoerwt Of A PtUNC
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Ip » Ideno(l,2.3 cd)pyrene NIST =
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Figure L 1.1 The 16 parental polycy
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After release by the primary source
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decomposition processes (O'Malley e
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Figure 2.1.1 The Great Lakes draina
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;: Duluth Chicago 1 J Lake Superior
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are the Black River, the Cuyaho ga
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Figure 1.1.5 The pattern of permane
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sedimentary basins, Western. Centra
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Figure 2. 1.8 Summer (July) air and
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Natural Resources: The lower Great
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American waters under the current U
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continuously overflowed com bined s
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3.1 EXPERIMENTAL 3. METHODS 3.1.1 S
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Table 3,1.1 Locations and types ofs
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Figure 3.12 Extraction and purifica
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hexane. 2) the unsaturated aliphati
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this problem. Ratios ofthe two stab
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Figure 3. 1.4 Configuration ofIsoch
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3.2.1 UNl- AND BIVAJUATE METHODS Th
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f igure 3.2. 1 Mean and range (± s
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utilized the same instrument (Isoch
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Selecting lIt1J'iahlu: It was demon
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w- _ 71
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seven variables with fewer missing
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analysis also employed a greate r n
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description. The second cluster ana
Page 104 and 105: elationships between different site
Page 107: Figure 4.1.3 Regression ofthree fir
Page 112: Figure 4.[.5 Isotopic composition (
Page 116: Figure 4.1.6 Weights ofvariables (c
Page 120: Figure 4.1.8 Distri bution ofsample
Page 123 and 124: those at the majority ofstations. S
Page 126 and 127: Ion, 969, 971, 357, 358). In additi
Page 129: Figure 4.2.3 Samples and prominent
Page 132 and 133: analysis supported some ofthc previ
Page 135 and 136: , ", Is , , >\ ryr " II ,- - , I ,
Page 137 and 138: 11'
Page 139: sources (Fi g. 4.2 .5c). This compo
Page 143: Figure 4.2.7 The relative contribut
Page 146 and 147: ".1.1.2 Miring CllrIIU (isotopic co
Page 149: Figure 42.9 Samples and promin ent
Page 159: Figure 4.2. 14 Samples and prominen
Page 167 and 168: towards light values ofBePlBaP in a
Page 169 and 170: info nnation sec Section 3.2..2}. A
Page 171 and 172: -s: Cl 5 4 3 .a; ;0 2 .2: '" -.!l1
Page 174 and 175: Another 10.5% ofvariance is explain
Page 176 and 177: Table 5.1.1 Three clusters identifi
Page 179 and 180: mo re pervasive background signatur
Page 182: figure S.U Zones (clusters) in the
Page 186 and 187: is diverted in litis direction (Fig
Page 189: Figure 5.1.6 Station locations and
Page 192 and 193: the Detroit river (969, 358, 351) t
Page 196 and 197: (Fig. 4.1 .8a, 5. tA) can also be a
Page 199: Figure 5.1.9 Statio n locations and
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Figure 5.1.10 Surface drifter track
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f igure 5.1.12 Drift card trajector
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Figure 5. t .13 Driftobject tracks
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In conclus ion. fluvial input of PA
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Figure 5.2. 1 Cloud ofsamples andpr
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increased amount oflight eas ily pe
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Figure 5.2.2 Cloud ofsamples and pr
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Figure 5.:!.3 Six clusters identifi
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mass balance calculations show that
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The processes ofdegradation might p
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Although less intensive than at Det
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The processes ofweathering do not s
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subzones ofinfluence was suggested.
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possesses similar isotopic composit
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fallout office soots as indicated b
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confined to the northern part ofthe
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Section 5.1); may still be affected
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their relative position with respec
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5.3 A MODEL OF SOURCES, PATHWAYS. T
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originate from the Maumee River at
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6. CONCLUSIONS The major conclusion
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7. REFERENCES Abrajano T. A. Jr.•
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Einsenreich S. J. and Strachan W. M
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Lee R. F. and Takahashi M. ( 1977)
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Sherrill T. W. and Saylor G. S. (19
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8. APPENDICES 242
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l' Appendix AS. Characteristic PAil
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Appeodil: A1. The hyperbolic equati
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... '"
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Appeadil. 82. 1bc output of a princ
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Appendix 84. The output o r a princ
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Appendix C3 . The results ora local
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