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Figure 42 .1 Ratios ofselected 4-, S· ring compounds compared to characteristic ratios of prominent primarysources (combustion vs. pctrolewn. and anthropogenic vs. natural diagenetic ). btios of primary sources are those identified by O' Malley (1994) for an urbanized area in eastern CanWa (see Appendix AS).
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POLYCYCLIC AROMATIC HYDROCARBONS IN
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composition. Portions ofthe lake th
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TABLE OF CONTENTS . ABSTRAcr._._ _
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6. CONCLUSIONS_._ _....._._._ _ ._
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FIGURE 3.104 CONfIGURATION OF ISOCH
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FIGURE 4 .2.12 SAMPLES AND PROMINEN
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fIGURE 5.3.1 DESCR1Pl1VE MODEL OF S
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APPENDIX B 3 _ T HEoerwt Of A PtUNC
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Ip » Ideno(l,2.3 cd)pyrene NIST =
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Figure L 1.1 The 16 parental polycy
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After release by the primary source
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decomposition processes (O'Malley e
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Figure 2.1.1 The Great Lakes draina
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;: Duluth Chicago 1 J Lake Superior
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are the Black River, the Cuyaho ga
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Figure 1.1.5 The pattern of permane
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sedimentary basins, Western. Centra
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Figure 2. 1.8 Summer (July) air and
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Natural Resources: The lower Great
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American waters under the current U
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continuously overflowed com bined s
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3.1 EXPERIMENTAL 3. METHODS 3.1.1 S
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Table 3,1.1 Locations and types ofs
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Figure 3.12 Extraction and purifica
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hexane. 2) the unsaturated aliphati
Page 75: this problem. Ratios ofthe two stab
Page 78: Figure 3. 1.4 Configuration ofIsoch
Page 82 and 83: 3.2.1 UNl- AND BIVAJUATE METHODS Th
Page 84: f igure 3.2. 1 Mean and range (± s
Page 87 and 88: utilized the same instrument (Isoch
Page 90 and 91: Selecting lIt1J'iahlu: It was demon
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Page 95 and 96: seven variables with fewer missing
Page 97 and 98: analysis also employed a greate r n
Page 99: description. The second cluster ana
Page 104 and 105: elationships between different site
Page 107: Figure 4.1.3 Regression ofthree fir
Page 112: Figure 4.[.5 Isotopic composition (
Page 116: Figure 4.1.6 Weights ofvariables (c
Page 120: Figure 4.1.8 Distri bution ofsample
Page 123: those at the majority ofstations. S
Page 127: Figure 4.2.2 Samp les and prominent
Page 131 and 132: implies that compounds there either
Page 133: Figure 4.1.4 Weights ofvariables (c
Page 136 and 137: Figure 4.1.5 Distribution orsamples
Page 138 and 139: The third PC is responsible for 11.
Page 142 and 143: sources on the graphs for Pa, Fa. B
Page 145 and 146: These sources contribute as much as
Page 147: Figure 4.2.8 Samples and prominent
Page 151: Figure 4.2. 10 Samples andprominent
Page 159: Figure 4.2. 14 Samples and prominen
Page 167 and 168: towards light values ofBePlBaP in a
Page 169 and 170: info nnation sec Section 3.2..2}. A
Page 171 and 172: -s: Cl 5 4 3 .a; ;0 2 .2: '" -.!l1
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Another 10.5% ofvariance is explain
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Table 5.1.1 Three clusters identifi
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mo re pervasive background signatur
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figure S.U Zones (clusters) in the
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is diverted in litis direction (Fig
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Figure 5.1.6 Station locations and
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the Detroit river (969, 358, 351) t
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(Fig. 4.1 .8a, 5. tA) can also be a
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Figure 5.1.9 Statio n locations and
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Figure 5.1.10 Surface drifter track
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f igure 5.1.12 Drift card trajector
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Figure 5. t .13 Driftobject tracks
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In conclus ion. fluvial input of PA
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Figure 5.2. 1 Cloud ofsamples andpr
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increased amount oflight eas ily pe
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Figure 5.2.2 Cloud ofsamples and pr
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Figure 5.:!.3 Six clusters identifi
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mass balance calculations show that
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The processes ofdegradation might p
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Although less intensive than at Det
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The processes ofweathering do not s
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subzones ofinfluence was suggested.
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possesses similar isotopic composit
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fallout office soots as indicated b
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confined to the northern part ofthe
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Section 5.1); may still be affected
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their relative position with respec
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5.3 A MODEL OF SOURCES, PATHWAYS. T
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originate from the Maumee River at
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6. CONCLUSIONS The major conclusion
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7. REFERENCES Abrajano T. A. Jr.•
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Einsenreich S. J. and Strachan W. M
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Lee R. F. and Takahashi M. ( 1977)
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Sherrill T. W. and Saylor G. S. (19
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8. APPENDICES 242
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l' Appendix AS. Characteristic PAil
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Appeodil: A1. The hyperbolic equati
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... '"
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Appeadil. 82. 1bc output of a princ
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Appendix 84. The output o r a princ
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Appendix C3 . The results ora local
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