A&A 456, 565–580 (2006)DOI: 10.1051/0004-6361:20065260c○ ESO 2006Astronomy&AstrophysicsLow sulfur dep<strong>le</strong>tion in the Horsehead PDR ⋆,⋆⋆J. R. Goicoechea 1 ,J.Pety 1,2 , M. Gerin 1 , D. Teyssier 3 , E. Roueff 4 , P. Hily-Blant 2 , and S. Baek 11 LERMA–LRA, UMR 8112 CNRS, Observatoire de Paris and Éco<strong>le</strong> Norma<strong>le</strong> Supérieure, 24 Rue Lhomond,75231 Paris Cedex 05, Francee-mail: [javier;gerin]@lra.ens.fr2 IRAM, 300 rue de la Piscine, 38406 Grenob<strong>le</strong> Cedex, Francee-mail: [pety;hilyblan]@iram.fr3 European Space Astronomy Centre, Urb. Villafranca del Castillo, PO Box 50727, Madrid 28080, Spaine-mail: dteyssier@sciops.esa.int4 LUTH UMR 8102, CNRS and Observatoire de Paris, Place J. Janssen, 92195 Meudon Cedex, Francee-mail: evelyne.roueff@obspm.frReceived 23 March 2006 / Accepted 9 June 2006<strong>tel</strong>-<strong>00726959</strong>, version 1 - 31 Aug 2012ABSTRACTAims. We present 3.65 ′′ × 3.34 ′′ angular-resolution IRAM Plateau de Bure Interferometer (PdBI) observations of the CS J = 2–1 linetoward the Horsehead Photodissociation Region (PDR), comp<strong>le</strong>mented with IRAM-30m sing<strong>le</strong>-dish observations of several rotationallines of CS, C 34 SandHCS + . We analyse the CS and HCS + photochemistry, excitation and radiative transfer to obtain their abundancesand the physical conditions prevailing in the cloud edge. Since the CS abundance sca<strong>le</strong>s to that of sulfur, we determine the gas phasesulfur abundance in the PDR, an interesting intermediate medium between translucent clouds (where sulfur remains in the gas phase)and dark clouds (where large dep<strong>le</strong>tions have been invoked).Methods. A nonlocal non-LTE radiative transfer code including dust and cosmic background illumination adapted to the Horseheadgeometry has been developed to carefuly analyse the CS, C 34 S, HCS + and C 18 O rotational line emission. We use this model toconsistently link the line observations with photochemical models to determine the CS/HCS + /S/S + structure of the PDR.Results. Densities of n(H 2 ) ≃ (0.5−1.0) × 10 5 cm −3 are required to reproduce the CS and C 34 S J = 2–1 and 3–2 line emission.CS J = 5–4 lines show narrower line widths than the CS low-J lines and require higher density gas components not resolved by the∼10 ′′ IRAM-30m beam. These values are larger than previous estimates based in CO observations. We found χ(CS) = (7 ± 3) ×10 −9 and χ(HCS + ) = (4 ± 2) × 10 −11 as the averaged abundances in the PDR. According to photochemical models, the gas phasesulfur abundance required to reproduce these values is S/H = (3.5 ± 1.5) × 10 −6 , only a factor < ∼ 4 <strong>le</strong>ss abundant than the solar sulfure<strong>le</strong>mental abundance. Since only lower limits to the gas temperature are constrained, even lower sulfur dep<strong>le</strong>tion values are possib<strong>le</strong>if the gas is significantly warmer.Conclusions. The combination of CS, C 34 SandHCS + observations together with the inclusion of the most recent CS collisional andchemical rates in our models implies that sulfur dep<strong>le</strong>tion invoked to account for CS and HCS + abundances is much smal<strong>le</strong>r than inprevious studies.Key words. astrochemistry – ISM: clouds – ISM: mo<strong>le</strong>cu<strong>le</strong>s – ISM: individual objects: Horsehead nebula – radio lines: ISM –radiative transfer1. IntroductionSulfur is an abundant e<strong>le</strong>ment (the solar photosphere abundanceis S/H = 1.38 × 10 −5 ; Asplund et al. 2005), which remains undep<strong>le</strong>tedin diffuse inters<strong>tel</strong>lar gas (e.g. Howk et al. 2006) andHII regions (e.g. Martín-Hernández et al. 2002; García-Rojaset al. 2006, and references therein) but it is historically assumedto dep<strong>le</strong>te on grains in higher density mo<strong>le</strong>cular clouds by factorsas large as ∼10 3 (Tieftrunk et al. 1994). This conclusionis simply reached by adding up the observed gas phase abundancesof S-bearing mo<strong>le</strong>cu<strong>le</strong>s in well known dark clouds suchas TMC1 (e.g. Irvine et al. 1985; Ohishi & Kaifu 1998). As⋆ Based on observations obtained with the IRAM Plateau de Bureinterferometer and 30 m <strong>tel</strong>escope. IRAM is supported by INSU/CNRS(France), MPG (Germany), and IGN (Spain).⋆⋆ Appendix A is only availab<strong>le</strong> in e<strong>le</strong>ctronic form athttp://www.edpsciences.orgsulfur is easily ionized (ionization potential ∼10.36 eV), sulfurions are probably the dominant gas-phase sulfur species intranslucent gas. Ruff<strong>le</strong> et al. (1999) proposed that if dust grainsare typically negatively charged, S + may freeze-out onto dustgrains during cloud collapse more efficiently than neutral speciessuch as oxygen. However, the nature of sulphur on dust grains(either in mant<strong>le</strong>s or cores) is not obvious. Van der Tak et al.(2003) observed large abundances of gas phase OCS, ∼10 −8 ,instar forming regions, and suggested that together with the detectionof solid OCS (with an abundance of ∼10 −7 ; Palumboet al. 1997), it implies that OCS is a major sulfur carrier in dustgrains. However, the ∼4.9 µm ice feature attributed to OCS isbest reproduced when OCS is mixed with methanol. In fact, theband is b<strong>le</strong>nded with a methanol overtone whose contributionhas not been studied in detail (Dartois 2005). In any case, the absenceof strong IR features due to S-bearing ices in many ISO’smid-IR spectra (e.g. Boogert et al. 2000; Gibb et al. 2004) andArtic<strong>le</strong> published by EDP Sciences and availab<strong>le</strong> at http://www.edpsciences.org/aa or http://dx.doi.org/10.1051/0004-6361:20065260
566 J. R. Goicoechea et al.: Low sulfur dep<strong>le</strong>tion in the Horsehead PDRTab<strong>le</strong> 1. Observation parameters.Phase centerNumber of fieldsMosaic 1 α 2000 = 05 h 40 m 54.27 s δ 2000 = −02 ◦ 28 ′ 00 ′′ 7Mosaic 2 α 2000 = 05 h 40 m 53.00 s δ 2000 = −02 ◦ 28 ′ 00 ′′ 4Mo<strong>le</strong>cu<strong>le</strong> & Line Frequency Beam PA Noise a Obs. date(GHz) (arcsec) ( ◦ ) (Kkms −1 )Mosaic 1CS J = 2–1 97.981 3.65 × 3.34 48 1.2 × 10 −1 Aug. & Oct. 2004 and Mar. 2005C 18 O J = 2–1 219.560 6.54 × 4.31 65 9.8 × 10 −2 Mar. 2003Mosaic 2CO J = 1–0 115.271 5.95 × 5.00 65 1.2 × 10 −1 Nov. 199912 CO J = 2–1 230.538 2.97 × 2.47 66 1.7 × 10 −1 Nov. 1999a The noise values quoted here are the noises at the mosaic center (Mosaic noise is inhomogeneous due to primary beam correction; it steeplyincreases at the mosaic edges). Those noise values have been computed in 1 km s −1 velocity bin.<strong>tel</strong>-<strong>00726959</strong>, version 1 - 31 Aug 2012the presence of S ii recombination lines in dark clouds such asRho Ophiuchi (Pankonin & Walms<strong>le</strong>y 1978) all argue againsta large dep<strong>le</strong>tion of sulfur from the gas phase. In this case, theabundance of species such as CS may indicate that somethingimportant is lacking from chemical models or that an abundantsulfur-bearing carrier has been missed. Therefore, the abundancesof sulfur species remain interesting puzz<strong>le</strong>s for inters<strong>tel</strong>larchemistry. In the case of dense clouds, standard chemicalmodels predict that most of the gas phase sulfur is shared betweenS, SO and CS (Millar & Herbst 1990), whi<strong>le</strong> H 2 Sisalsoabundant in the Orion Bar PDR (Jansen et al. 1995). In all thesecases, a large sulfur dep<strong>le</strong>tion, ∼10 2 , was required in the modelsto explain the observed abundances.PDRs offer an ideal intermediate medium between diffuseand dark cloud gas to investigate the sulfur dep<strong>le</strong>tion prob<strong>le</strong>m.In this work we have tried to determine the CS abundancein the Horsehead PDR as a tool for estimating the sulfur gasphase abundance. However, CS chemistry is an open issue itselfin different environments, from hot cores (e.g. Wakelam et al.2004) to extragalactic sources (e.g. Martín et al. 2005). Recentlaboratory experiments on dissociative recombination of HCS +and OCS + (Montaigne et al. 2005) imply a substantial modificationof previous reaction rate coefficients, dissociative channelsand branching ratios used in chemical models. The latest availab<strong>le</strong>reaction rates and collisional coefficients have been used inour photochemical and radiative transfer models.1.1. The Horsehead nebulaThe Horsehead nebula, appears as a dark patch of ∼5 ′ diameteragainst the bright HII region IC 434. Emission from gas anddust associated with this globu<strong>le</strong> has been detected from IR tomillimeter wave<strong>le</strong>ngths (Abergel et al. 2002, 2003; Pound et al.2003; Teyssier et al. 2004, Habart et al. 2005; Pety et al. 2005a),although the first astronomical plates were taken ∼120 yr ago. Inparticular, the Horsehead western edge is a PDR viewed nearlyedge-on and illuminated by the O9.5V star σOri at a projecteddistance of ∼3.5 pc (Anthony-Twarog 1982). The intensity ofthe incident FUV radiation field is χ ≃ 60 relative to the inters<strong>tel</strong>larradiation field (ISRF) in Draine’s units (Draine 1978).According to the evolutionary view of Reipurth & Bouchet(1984), the Horsehead nebula was a quiescent and dense cloudcore embedded in a more diffuse cloud (L1630). The erosiveaction of the UV radiation from σOri on the ambient gas <strong>le</strong>dto the apparent emergence of the core cloud, as in the earlieststages of Bok globu<strong>le</strong>s still attached to their parental cloud.However, the observed morphology together with the velocitygradients of the cloud, require a more involved description includinga pre-existing rotating velocity field as well as densityinhomogeneities in the initial structures (Pound et al. 2003;Hily-Blant et al. 2005). The erosive effect of the ionizing anddissociating radiation field together with these initial conditionsexplain the peculiar shaping of the Horsehead nebula. In particular,the densest regions of the initial inhomogeneities are nowbelieved to be the East-West filamentary material connecting itto the parental cloud, and the PDR. In this work we have studiedthe PDR through CS, C 34 SandHCS + observations.2. Observations and data reduction2.1. Observations2.1.1. Pico Ve<strong>le</strong>ta sing<strong>le</strong>-dishThe sing<strong>le</strong>-dish data presented in this paper have been gatheredbetween February and October 2004 at the IRAM 30-m <strong>tel</strong>escope.The Horsehead nebula PDR was mapped in the CS J =2–1 and 5–4 lines in order to provide the short-spacings for theinterferometric observations presented thereafter. The final mapconsists of 5 on-the-fly coverages performed along perpendicularscanning directions, and combined with the PLAIT algorithmintroduced by Emerson & Gräve (1888), allowing to efficientlyreduce the stripes over the map. The noise <strong>le</strong>vels (1σ rms) perregridded pixel and resolution channel of 80 kHz are of the orderof 0.15 K at 3 mm, and 0.64 K at 1.3 mm. The latter valuewas not low enough to provide any useful mapping informationat 1.3 mm since the CS J = 5–4 line peak is < ∼ 1K.In comp<strong>le</strong>ment to these data, dedicated positions wereprobed over a larger set of species and transitions. The frequencyswitching mode was used to observe CS J = 2–1, 3–2and 5–4 lines, as well as C 34 S J = 2–1, 3–2, and HCS + J =2–1 lines. Tab<strong>le</strong> 2 summarizes the corresponding observing parameters.Longer integrations allowed to reach, in a resolutionchannel of 40 kHz, rms noise <strong>le</strong>vels of 25, 42 and 36 mK at 3,2, and 1.3 mm respectively. All CS and C 34 S lines were detectedwith a S/N ratio better than 10. Figures 4 and 8 show some spectracol<strong>le</strong>cted at positions inside and across the PDR.The data were first calibrated to the TA ∗ sca<strong>le</strong> using the socal<strong>le</strong>dchopper wheel method (Penzias & Burrus 1973), andfinally converted to main beam temperatures using efficiencies(B eff /F eff ) of 0.81, 0.74 and 0.50 at 3, 2 and 1.3 mmrespectively.
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