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Figure 5. Core mass balance for 0.50% and 100% 238 U in the fertile material input for Vfertile/Vfissile = 2 1 000 000 Loaded mass in reactor (kg) 100 000 10 000 1 000 100 10 1 TH 32 PA 33 U2 33 U2 34 U2 35 U2 36 U2 38 PU 38 PU 39 PU 40 PU 41 PU 42 AM 41 AM 43 100%Th 50% Th 50% U 100% U NP 37 CM 42 CM 43 CM 44 CM 45 5. A major safety asset: core drainage The salt is at its maximum reactivity in the graphite. A safe fallback position can thus be obtained by draining the core. As the fuel is liquid, it can be extracted from the core at any moment. For this, we adopted a concept proposed by EdF and the CEA, which consists in placing a drain tank under the core, which is permanently connected to it. Salt is confined within the core by a helium back-pressure (Figure 6). One therefore need simply interrupt the electric power supply to the He compressor for gravity drainage of the core. This feature, allied with the considerable thermal inertia of the reactor and the difficulty of rapidly inserting reactivity, should make the reactor particularly safe. Figure 6. Core drainage principle Thermal detector Reactor Salt Compressor He 264
6. R&D needed to validate the AMSTER concept To make the transition from concept to technology, much research and experimentation is required. Among the subjects covered will be: • Salt chemistry, structural corrosion by salt. • Processing chemistry, containment of transuranium elements in the salt. • Reactor dynamics. • Safety. It should be recalled that major R&D work was already carried out in the 60s/70s and a prototype functioned remarkably well (MSRE). A detailed preliminary project for a breeder reactor (MSBR) was conducted. The AMSTER concept is similar to these two reactors and the experience acquired would be directly applicable to it. 7. Fertile and fissile material utilisation The AMSTER concept should allow the production of energy with very reduced quantities of transuranium element waste (a few g per TWhe), and with no transportation of highly radiotoxic substances. AMSTER with a mixed thorium-uranium support with a peripheral fertile zone, breeding its own uranium, should further improve this performance. This reactor should in fact offer incinerating performance identical to that of the thorium AMSTER supplied with 235 U, while eliminating the need for uranium enrichment and making the reactor non-proliferating. Furthermore, this self-breeding reactor would consume only 50 kg of thorium and 50 kg of 238 U per TWhe, which in the light of estimated resources (1 to 4 million tonnes of thorium and 1 to 3 million tonnes of uranium), would allow the production of 20 to 70 million TWhe (the world’s annual electricity consumption from all sources together is about 15 000 TWhe); The depleted uranium stored in France (200 000 t), together with 200 000 t of thorium, could produce 4 million TWhe (annual production is 400 TWhe). Figure 7 compares the mass balance entering and leaving the reactor for a standard open-cycle PWR and a self-generating AMSTER with a support of 50% U and 50% Th. The inputs are natural or depleted uranium and thorium. The outputs comprise: • Transuranium element losses, U and Th vitrified with the FP. • Depleted uranium produced at enrichment of the support. This theoretical study shows that: • AMSTER would be far “cleaner” than a PWR (4 decades reduction of transuranium element waste). 265
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Nuclear Development ACTINIDE AND FI
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FOREWORD The objective of the OECD/
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TABLE OF CONTENTS Foreword ........
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EXECUTIVE SUMMARY More than 160 par
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identified. In the fuel area, labor
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17:20-19:05 Session III: Partitioni
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Poster sessions Poster session: Par
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WELCOME ADDRESS Lucila Izquierdo Ge
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WELCOME ADDRESS Michel Hugon Co-ord
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WELCOME ADDRESS Philippe Savelli De
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developments. This will surely beco
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use of FBRs for transmutation toget
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view, i.e. better use of uranium an
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W. Forsberg proposes to reduce the
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1. From the open fuel cycle to the
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Figures 2 and 3 show the radiotoxic
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Denoting the transuranic (TRU) or m
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or, in terms of the fuel burn-up an
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quantities of LWR-MOX and FR-MOX wi
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view of the historic development, t
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Table 5. Assumptions for transmutat
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separating troublesome fission prod
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REFERENCES [1] L.H. Baetslé, Ch. D
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SESSION III Partitioning Chairs: J.
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OVERVIEW OF THE HYDROMETALLURGICAL
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2.1.3 Consequences Owing to the fac
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The extraction and separation mecha
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extractant was observed. As a conse
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2.3.2 Examples of strategies and
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3. Conclusions and perspectives 3.1
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SESSION IV Basic Physics, Materials
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TRANSMUTATION: A DECADE OF REVIVAL
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2.1 The IFR concept and the homogen
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2.3 Dedicated systems Making again
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compound “macro-dispersed” in M
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Figure 3. Sketch of ADS, liquid met
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3.3.2.1 The MEGAPIE project [40] ME
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3.3.2.2 The MUSE experiments The MU
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Figure 8. Comparison of the neutron
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Figure 9. Scenarios at equilibrium
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goals in this field. Since once-thr
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• The use of Thorium in PWRs alwa
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• Understanding of the role of AD
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[17] Y. Arai, T. Ogawa, Research on
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SESSION V Transmutation Systems and
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1. Introduction The term ADS compre
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• Safety should be “designed in
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3. Minor actinide and/or transurani
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Table 2. Values of Dj (neutron cons
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Table 4. Delayed neutron fraction I
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Figure 4. η (Neutrons released per
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Table 5. ADS Distinguishing feature
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While a favourable ADS safety featu
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Optimised mixes of MA and Pu can be
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Moreover, the fuel is where neutron
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REFERENCES [1] L. Van den Durpel et
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[19] D.C. Wade and E. Fujita, Trend
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POSTER SESSION Basic Physics: Nucle
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To conclude, this poster session in
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Five other papers related to ADS co
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SESSION I OVERVIEW OF NATIONAL AND
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1. Current activities for radioacti
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3.2 Results to date and analyses of
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3.2.5.2 JNC JNC is considering the
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4.6 Short-term increase in radiatio
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Annex 1 R&D scheme for partitioning
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Annex 3 Members of the Advisory Com
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plutonium can be recycled in pressu
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choices and the implementation of m
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1. Introduction Since the 5th Infor
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strata” approach which would invo
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IAEA ACTIVITIES IN THE AREA OF EMER
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actually started to do so) because
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establishment of an international R
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The accelerator driven transmutatio
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substantiate this recommendation, s
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current, advanced and innovative nu
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ACCELERATOR DRIVEN SUB-CRITICAL SYS
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demonstration of feasibility of a E
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An extended “skeleton” for ADS
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• Fertile support (uranium) is no
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7. Conclusions The TWG under the ch
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1. Introduction The priorities for
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In the EURATOM Fourth Framework Pro
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Table 2. Cluster on transmutation-t
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6. Community research for the perio
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REFERENCES [1] “Council Decision
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1. Introduction Back in 1989, the O
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would need the continuation of tech
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individual isotopes as a function o
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Therefore, while there is continuin
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[9] OECD/NEA, Overview of Physics A
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RECENT TOPICS IN R&D FOR THE OMEGA
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Figure 1. Partitioning and transmut
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The present 4-GPP necessitates a pr
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5. Concluding remarks In 1999, the
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REFERENCES [1] T. Mukaiyama, T. Tak
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1. Introduction CIEMAT is actively
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adiotoxicity to be managed could al
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Figure 3. Mass composition of the d
Page 214 and 215: Figure 6. Fuel cycle assumed in the
Page 216 and 217: the 4 batches scheme, allowing to a
Page 218 and 219: Figure 11. Transmutation efficiency
Page 220 and 221: 1. Introduction Spent fuels of mode
Page 222 and 223: Figure 3. A change in radiotoxicity
Page 224 and 225: These dependencies are shown on Fig
Page 226 and 227: When increasing the moderator fract
Page 228 and 229: Even greater power increases are ob
Page 230 and 231: The effect of a moderator volume fr
Page 232 and 233: Table 11. Different isotopes contri
Page 234 and 235: Thus the transmutation of such FPs
Page 237 and 238: ASSESSMENT OF NUCLEAR POWER SCENARI
Page 239 and 240: elease probabilities. The time dist
Page 241 and 242: Table 2. Annual heavy nuclide contr
Page 243 and 244: Figure 3. Reduction of potential ra
Page 245 and 246: DISPOSAL OF PARTITIONING-TRANSMUTAT
Page 247 and 248: Figure 2. Decay heat from SNF 2000
Page 249 and 250: Figure 3. Shorter-lived HHR reposit
Page 251 and 252: 4. Management of low-heat, long-liv
Page 253 and 254: isotope from other caesium isotopes
Page 255 and 256: THE AMSTER CONCEPT J. Vergnes 1 , D
Page 257 and 258: Figure 1. Layout diagram of the mol
Page 259 and 260: Table 1. Definition of configuratio
Page 261 and 262: We therefore adopted a partial purg
Page 263: conceivable. Thus by increasing the
Page 267: SESSION III PARTITIONING J.P. Glatz
Page 271 and 272: PARTITIONING-SEPARATION OF METAL IO
Page 273 and 274: The terpyridyl reagent (ligand L 1
Page 275 and 276: Figure 2. The synthesis of ADTPTZ a
Page 277 and 278: 2.4 Implications for partitioning T
Page 279 and 280: SEPARATION OF MINOR ACTINIDES FROM
Page 281 and 282: installed in a hot cell. The feed w
Page 283 and 284: the concentrations of U, Pu and Np
Page 285 and 286: Table 2 shows the recovery in the r
Page 287 and 288: PARTITIONING ANIONIC AGENTS BASED O
Page 289 and 290: which of these, the Co 3+ , Fe 3+ a
Page 291 and 292: This dianionic species must be extr
Page 293 and 294: Figure 6 Ph 2 P acetone PPh 2 H2 O
Page 295 and 296: Figure 9 H 3 C RO(CH 2 )n CH 3 (CH
Page 297: [7] J. Rais and P. Selucky, Nucleon
Page 301 and 302: PYROCHEMICAL PROCESSING OF IRRADIAT
Page 303 and 304: The metallic cadmium product of the
Page 305 and 306: Figure 2. Schematic flow-sheet for
Page 307 and 308: R&D OF PYROCHEMICAL PARTITIONING IN
Page 309 and 310: (first of all pumps) for fluoride m
Page 311 and 312: 4. Research on material and equipme
Page 313: REFERENCES [1] Uhlir J., Pyrochemic
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1. Introduction The increasing inte
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Figure 2. Stainless steel box with
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Figure 4. U deposit on solid cathod
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Figure 7. Schematic flow of the cou
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actinide elements from spent (metal
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DEVELOPMENT OF PLUTONIUM RECOVERY P
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uranium dendrite and that uranium c
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Table 1. Conditions and results of
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Cathode potential went down to -1.6
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Figure 6. Change of LCC potential i
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Figure 9. Relation between Pu conce
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consideration described in the prec
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[13] Y. Arai, S. Fukushima, K. Shio
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SESSION IV BASIC PHYSICS, MATERIALS
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1. Introduction The reduction of th
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agrees ours within limits of errors
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Figure 1. Thermal neutron capture c
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[18] A.P. Baerg, R.M. Bartholomew,
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1. Introduction Nowadays it is well
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In order to describe the inter-nucl
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kind of measurements allow to chara
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Figure 6. Two-dimensional cluster p
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Figure 8. Excitation functions for
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REFERENCES [1] D. Ridikas, thesis,
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1. Introduction Since 1991, the Com
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Experimental reactivity control tec
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Table 2. Neutron intensities Target
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experimental channels (horizontal a
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376
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Table 3. Planned experimental progr
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1. Introduction and benchmark speci
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neutrons. Since the neutron flux is
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Figure 2. Microscopic capture cross
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Figure 4. k eff variation in the st
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2.4 Neutron flux distribution One r
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etween the highest and the lowest v
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The isotope specific β eff values
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SESSION IV BASIC PHYSICS, MATERIALS
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1. Introduction Due to its excellen
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Figure 2. Tests scheme 0 340 h. 1 0
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Figure 4. Auger depth profile conce
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Figure 8. Auger depth profile conce
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deposited at the cold zone, and the
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inner layer grows inward from the o
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[8] V.M. Fedirko, O.I. Eliseeva, V.
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1. Introduction One of the main par
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3. Tantalum target irradiation The
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At 10-MeV neutron irradiation, radi
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1. Introduction HYPER (HYbrid Power
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this study, we used an orthogonal c
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Figure 5. Temperature distribution
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Figure 7. Thermal stress distributi
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FUEL/TARGET CONCEPTS FOR TRANSMUTAT
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(U 0.55 Pu 0.4 Np 0.05 )O 2 fuels w
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Figure 3. Left: Ceramograph of a (Z
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Figure 6. Left: ceramograph of a(Zr
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AMERICIUM TARGETS IN FAST REACTORS
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The reference case for all comparis
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It should be underlined that this c
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Cases Table 3. Heterogeneous recycl
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• A later step could be to add Cm
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RESEARCH ON NITRIDE FUEL AND PYROCH
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temperature for (Cm,Pu)N followed t
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Figure 1. Temperature dependence of
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The difference of two fuel pins exi
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In addition to the voltammetric stu
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2 wt% of Pu at 773 K. For the momen
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[13] M. Akabori, M. Takano, A. Itoh
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1. Introduction For the management
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The scientific feasibility of pluto
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Another option using a basis of sta
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6.2.1 Inert matrices 6.2.1.1 MgAl 2
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eached respectively 38.5% and 70% F
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Figure 4. Experiments for MA transm
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Figure 5a. Ecrix B rig Figure 5b. E
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A CEA/Minatom work programme is und
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9.3 Programme for dedicated fuels F
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[14] R.J.M. Konings et al., The EFT
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1. Introduction An accelerator driv
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corresponding Pb-Bi velocity is 1.1
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the fission product target. The rod
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fuel rods are at the TRU assembly t
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SESSION V TRANSMUTATION SYSTEMS AND
Page 492 and 493:
1. Introduction Since the 50s, nitr
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A three dimensional model of a sub-
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Figure 4. Change in k-eigenvalue fo
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[4] Y. Arai et al., Experimental Re
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Nomenclature ADS: ATW: GT-MHR: LOF:
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Regarding switching off the beam, o
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Figure 3. Beam blocking 10 min (200
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Figure 7. A possible scenario for n
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[15] Greenspan E. et al., The Encap
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1. Introduction In the EADF design
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Equation (6) can be improved by con
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where L is obtained by a summation
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Figure 1. The natural convection im
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Figure 4 shows the temperature tren
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[12] P.H. Wakker, Thermal Hydraulic
Page 522 and 523:
1. Introduction Research and develo
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Table 2. Core design parameters for
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2.2 Representation of MA transmutat
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Figure 1(b) shows the cases for the
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It is found that the higher MA tran
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REFERENCES [1] T. Ikegami, H. Hayas
Page 534 and 535:
1. Introduction The management of t
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Table 1. Core performance of MA and
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Figure 3. Nuclear electricity capac
Page 540 and 541:
Table 3. Experimental items at PEF
Page 542 and 543:
REFERENCES [1] Takano H., Akie H.,
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1. Introduction and background The
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neutron source, the reactor can mai
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atoms. For fuel region Rf = 2.5 cm,
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Figure 3. Neutron flux spectra for
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A possible way to maintain the k ef
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higher than 99% of 239 Pu, and high
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TRANSMUTATION OF NUCLEAR WASTES WIT
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Figure 1. PBT conceptual view Table
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very tight holders for fission frag
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5. Cooling system A preliminary des
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spectral densities [10,11] and can
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MYRRHA, A MULTI-PURPOSE ADS FOR R&D
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hexagonal assemblies of 122 mm plat
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to achieve the requested performanc
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3 MYRRHA associated R&D programme F
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collaboration with Forschungszentru
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• Industrial partners, in particu
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1. Introduction The transmutation o
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Existing accelerators have been des
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suggested to look for an innovative
Page 586 and 587:
Table 1. Main lead-bismuth eutectic
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4.3 The core The basic fuel sub-ass
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Figure 1. Experimental accelerator
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HELIUM-COOLED REACTOR TECHNOLOGIES
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of its potential use in nuclear wea
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Figure 2. Neutron flux distribution
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atio. Given this rate of destructio
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Figure 5. Irradiated TRISO particle
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in ceramic-coated microspheres of t
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(LOCA) event. The effect on this fe
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Figure 13. Elevation AD-FMHR The fa
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Deep burn-up of 239 Pu and fissiona
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POSTER SESSION PARTITIONING M.J. Hu
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1. Introduction The study of the be
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Plutonium was simulated with the no
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The influence of uranium and pluton
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The influence of uranium and pluton
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REFERENCES [1] I.I. Nazarenko, A.M.
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1. Introduction The long-term radio
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Ce Ce 3+ Cl - Cl 2 The voltammogram
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Figure 3. Chronopotentiograms for t
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Figure 4. Potentiometric titrations
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Experimental solubilization tests w
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[13] H. Flood T. Förland and K. Mo
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1. Introduction The separation of l
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Figure 4. Synthesis of amides 11-15
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1. Introduction Over the recent yea
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2.3.2 Set-up We set up a single HFM
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lower flow rates, Am(III) would be
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THE POTENTIAL OF NANO- AND MICROPAR
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efficiently and stable. This can be
Page 653 and 654:
Figure 1a. Zetapotential of NTA-mod
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Scheme 7. Magnetic silica particles
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[13] L.H. Delmau, N. Simon, M.J. Sc
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1. Introduction 137 90 Extraction p
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Figure 3. Schematic drawing of the
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(24), 8-PhPO(OH)-O-COSAN (25), and
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REFERENCES [1] Kyrš M., +H PiQHN S
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1. Introduction A heavy-water CANDU
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These data show that fuel lifetime
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RECENT PROGRESSES ON PARTITIONING S
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hot tests (See Table2) was enough f
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trace amount of Am and Eu. The HBTM
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6. Conclusion Declassification of t
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POSTER SESSION BASIC PHYSICS: NUCLE
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1. Introduction Among the large num
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The simulation of the spallation pr
Page 688 and 689:
Table 1. Parameters of the two coll
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Figure 4. Radial distribution of th
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6. The neutron escape line The comm
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Figure 7. Neutron background at the
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RECENT CAPTURE CROSS-SECTIONS VALID
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Figure 1. The GENEPI accelerator an
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2.3.3 Neutron flux measurements •
Page 703 and 704:
Figure 6. Time spectrum of 3 He gas
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4. Analysis 4.1 Background subtract
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Figure 11. ENDF/B-VI, JEF2.2 and JE
Page 709 and 710:
DOUBLE DIFFERENTIAL CROSS-SECTION F
Page 711 and 712:
3. Conclusion Double differential c
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Figure 3. Preliminary results of do
Page 715 and 716:
MEASUREMENTS OF PARTICULE EMISSION
Page 717 and 718:
2. Experimental set-up The experime
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4. Results Figure 3 presents neutro
Page 722 and 723:
1. Introduction Intermediate-energy
Page 724 and 725:
Table 1. Relative neutron-induced c
Page 726 and 727:
elow about 70 MeV [24] , where σ n
Page 728 and 729:
Since for sub-actinides Γ f /Γ n
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[10] V.P. Eismont, A.V. Prokofiev,
Page 733 and 734:
NUCLEON-INDUCED FISSION CROSS-SECTI
Page 735 and 736:
Figure 1. Scheme of the new code Z
Page 737 and 738:
Figure 3. Neutron-induced fission c
Page 739:
REFERENCES [1] J. Raynal, Proceedin
Page 742 and 743:
1. Introduction During the past few
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(same surface and 0.5 mm thickness)
Page 746 and 747:
Figure 2. Dependence of the total a
Page 748 and 749:
Figure 3. Neutron radiative capture
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[8] MCNP, A General Monte Carlo Cod
Page 752 and 753:
1. Introduction New reactors using
Page 754 and 755:
Figure 1. Excited states of 209 Bi
Page 756 and 757:
Figure 3. The fission probability o
Page 759 and 760:
MEASUREMENT OF DOUBLE DIFFERENTIAL
Page 761 and 762:
Figure 1. Global view of the experi
Page 763 and 764:
To get the proton (deuteron) energy
Page 765 and 766:
3.1 Corrections Several corrections
Page 767 and 768:
Figure 11. Active target fraction (
Page 769 and 770:
d 2 σ Figure 14. Proton for n + Pb
Page 771 and 772:
HIGH AND INTERMEDIATE ENERGY NUCLEA
Page 773 and 774:
eactions, since the pre-equilibrium
Page 775 and 776:
calculate the very short-lived radi
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cross-sections; the secondary react
Page 779 and 780:
All possible nuclear reactions will
Page 781 and 782:
A STUDY ON BURNABLE ABSORBER FOR A
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2. Burnable absorber for HYPER 2.1
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Table 2. One-group effective cross-
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of the core, is directly determined
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Figure 4. Required proton beam curr
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Figure 8. 10 B depletion in HYPER-H
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POSTER SESSION TRANSMUTATION SYSTEM
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1. Introduction In the framework of
Page 798 and 799:
Φ >1 MeV = 1.0 10 13 to 1.0 x 10 1
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3. Irradiation targets and irradiat
Page 802 and 803:
e transmuted in BR2 hence remain va
Page 804 and 805:
Table 6. Atom percent concentration
Page 806 and 807:
advantage, with respect to FRs, of
Page 809 and 810:
ENHANCEMENT OF ACTINIDE INCINERATIO
Page 811 and 812:
Here Σ fC , ( E) are the fission a
Page 813 and 814:
pellet and the steel cladding. In o
Page 815 and 816:
Table 3.Neutronics parameters of hy
Page 817 and 818:
Figure 3. Neutron spectra averaged
Page 819 and 820:
containing FA with B 4 C cladding i
Page 821:
REFERENCES [1] ANSALDO Technical Re
Page 824 and 825:
1. Introduction At present, there a
Page 826 and 827:
target means a change in k and the
Page 828 and 829:
Following the normal procedure for
Page 830 and 831:
Acknowledgements This study has bee
Page 832 and 833:
1. ADS description A conceptual des
Page 834 and 835:
Substitution of (9) into (8), and u
Page 836 and 837:
With the coupling LAHET + MCNP-DSP,
Page 838 and 839:
Figure 3. Comparison for 1 and 5 pu
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MOLTEN SALTS AS POSSIBLE FUEL FLUID
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2. The fuel salt for MSB concept Ma
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and minor actinides must be removed
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4. Container material studies 4.1 F
Page 849 and 850:
management. The major developments
Page 851:
REFERENCES [1] H.J. MacPherson, Dev
Page 854 and 855:
1. Introduction The Energy Amplifie
Page 856 and 857:
Table 1. Main parameters of the EAD
Page 858 and 859:
Table 5. Neutron balance in the who
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Table 7. Neutron flux distributions
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Table 8. Displacement rates DPA/yea
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DEEP UNDERGROUND TRANSMUTOR (PASSIV
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passive state. By operating at a hi
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I have proposed using an accelerato
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Figure 1. Layout of deep undergroun
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RADIATION CHARACTERISTICS OF PWR MO
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Table 1. Radiotoxicity of actinides
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RADIATION CHARACTERISTICS OF URANIU
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Table 1. Radiotoxicity of actinides
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INTERNATIONAL CO-OPERATION ON CREAT
Page 883 and 884:
an international base to combine ef
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• Second topic: interaction of pr
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1. Introduction The role of acceler
Page 890 and 891:
MEPI within the framework of Projec
Page 893 and 894:
NEW ORIGINAL IDEAS ON ACCELERATOR D
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During conceptual investigations of
Page 897 and 898:
delay, interface and computer. The
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2. Channel-vessel design of ADS bla
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Table 1. Characteristics of the ful
Page 903:
[14] Karavaev G.N., Kiselev G.V., M
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1. Introduction The problem of nucl
Page 908 and 909:
Table 3. Radiotoxicity in americium
Page 910 and 911:
Table 5. Characteristics of station
Page 912 and 913:
1. Introduction The atomic power en
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of lead-bismuth target are given in
Page 917 and 918:
CRITICAL AND SUB-CRITICAL GT-MHRs F
Page 919 and 920:
Table 1. Basic GT-MHR reactor param
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Figure 2. Typical change of the ave
Page 923 and 924:
Scenario S4. This case is actually
Page 925 and 926:
Figure 3. A change in radiotoxicity
Page 927:
[13] P. Goberis, Modelling of Innov
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1. Introduction The Nuclear Enginee
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Some simplifications have been made
Page 934 and 935:
Figure 3. Velocity vectors Some of
Page 936 and 937:
Figure 6. Temperature evolution at
Page 938 and 939:
• Two main reasons can explain th
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1. Introduction Actually, we notice
Page 942 and 943:
This problem can be solved by using
Page 944 and 945:
The evaluations obtained in [2] hav
Page 946 and 947:
REFERENCES [1] Management and Dispo
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1. Background Radiation background
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the long-term hazard of spent fuel,
Page 952 and 953:
In a transmutation fuel cycle inclu
Page 954 and 955:
Figure 4. Potential biological haza
Page 956 and 957:
cooling prior to SF reprocessing an
Page 958:
REFERENCES [1] White Book of Nuclea
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ORDER FORM OECD Nuclear Energy Agen
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