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MOLTEN SALTS AS POSSIBLE FUEL FLUIDS FOR TRU FUELLED SYSTEMS: ISTC #1606 APPROACH Victor Ignatiev 1 , Raul Zakirov 1 , Konstantin Grebenkine 2 RRC-Kurchatov Institute, 123182, Moscow, Russian Federation 2 VNIITF, 456770, Snezinsk, Russian Federation 1 Abstract The principle attraction of the molten salt reactor (MSR) technology is the use of fuel/fertile material flexibility (easy of fuel preparation and processing) for gaining additional profits as compared with solid materials. This approach presents important departures from traditional philosophy, applied in current nuclear power plants, and to some extent contradicts the straightforward interpretation of the defence-in-depth principal. Nevertheless we understand there may be potential to use MSR technology to support back end fuel cycle technologies in future commercial environment. The paper aims at reviewing results of the work performed in Russia, relevant to the problems of MSR technology development. Also this contribution aims at evaluation of remaining uncertainties for molten salt burner concept implementation. Fuel properties & behaviour, container materials, and clean-up of fuels with emphasis on experiments will be of priority. Recommendations are made regarding the types of experimental studies needed on a way to implement molten salt technology to the back-end of the fuel cycle. To better understand the potential and limitations of the molten salts as a fuel for reactor of incinerator type, Russian Institutes have submitted to the ISTC the Task #1606 Experimental Study of Molten Salt Technology for Safe and Low Waste Treatment of Plutonium and Minor Actinides in Accelerator Driven and Critical Systems. The project goals, technical approach and expected specific results are discussed. 841
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Nuclear Development ACTINIDE AND FI
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FOREWORD The objective of the OECD/
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TABLE OF CONTENTS Foreword ........
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EXECUTIVE SUMMARY More than 160 par
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identified. In the fuel area, labor
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17:20-19:05 Session III: Partitioni
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Poster sessions Poster session: Par
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WELCOME ADDRESS Lucila Izquierdo Ge
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WELCOME ADDRESS Michel Hugon Co-ord
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WELCOME ADDRESS Philippe Savelli De
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developments. This will surely beco
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use of FBRs for transmutation toget
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view, i.e. better use of uranium an
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W. Forsberg proposes to reduce the
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1. From the open fuel cycle to the
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Figures 2 and 3 show the radiotoxic
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Denoting the transuranic (TRU) or m
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or, in terms of the fuel burn-up an
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quantities of LWR-MOX and FR-MOX wi
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view of the historic development, t
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Table 5. Assumptions for transmutat
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separating troublesome fission prod
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REFERENCES [1] L.H. Baetslé, Ch. D
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SESSION III Partitioning Chairs: J.
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OVERVIEW OF THE HYDROMETALLURGICAL
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2.1.3 Consequences Owing to the fac
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The extraction and separation mecha
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extractant was observed. As a conse
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2.3.2 Examples of strategies and
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3. Conclusions and perspectives 3.1
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SESSION IV Basic Physics, Materials
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TRANSMUTATION: A DECADE OF REVIVAL
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2.1 The IFR concept and the homogen
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2.3 Dedicated systems Making again
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compound “macro-dispersed” in M
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Figure 3. Sketch of ADS, liquid met
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3.3.2.1 The MEGAPIE project [40] ME
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3.3.2.2 The MUSE experiments The MU
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Figure 8. Comparison of the neutron
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Figure 9. Scenarios at equilibrium
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goals in this field. Since once-thr
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• The use of Thorium in PWRs alwa
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• Understanding of the role of AD
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[17] Y. Arai, T. Ogawa, Research on
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SESSION V Transmutation Systems and
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1. Introduction The term ADS compre
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• Safety should be “designed in
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3. Minor actinide and/or transurani
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Table 2. Values of Dj (neutron cons
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Table 4. Delayed neutron fraction I
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Figure 4. η (Neutrons released per
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Table 5. ADS Distinguishing feature
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While a favourable ADS safety featu
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Optimised mixes of MA and Pu can be
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Moreover, the fuel is where neutron
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REFERENCES [1] L. Van den Durpel et
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[19] D.C. Wade and E. Fujita, Trend
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POSTER SESSION Basic Physics: Nucle
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To conclude, this poster session in
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Five other papers related to ADS co
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SESSION I OVERVIEW OF NATIONAL AND
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1. Current activities for radioacti
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3.2 Results to date and analyses of
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3.2.5.2 JNC JNC is considering the
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4.6 Short-term increase in radiatio
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Annex 1 R&D scheme for partitioning
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Annex 3 Members of the Advisory Com
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plutonium can be recycled in pressu
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choices and the implementation of m
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1. Introduction Since the 5th Infor
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strata” approach which would invo
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IAEA ACTIVITIES IN THE AREA OF EMER
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actually started to do so) because
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establishment of an international R
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The accelerator driven transmutatio
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substantiate this recommendation, s
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current, advanced and innovative nu
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ACCELERATOR DRIVEN SUB-CRITICAL SYS
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demonstration of feasibility of a E
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An extended “skeleton” for ADS
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• Fertile support (uranium) is no
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7. Conclusions The TWG under the ch
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1. Introduction The priorities for
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In the EURATOM Fourth Framework Pro
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Table 2. Cluster on transmutation-t
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6. Community research for the perio
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REFERENCES [1] “Council Decision
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1. Introduction Back in 1989, the O
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would need the continuation of tech
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individual isotopes as a function o
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Therefore, while there is continuin
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[9] OECD/NEA, Overview of Physics A
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RECENT TOPICS IN R&D FOR THE OMEGA
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Figure 1. Partitioning and transmut
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The present 4-GPP necessitates a pr
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5. Concluding remarks In 1999, the
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REFERENCES [1] T. Mukaiyama, T. Tak
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1. Introduction CIEMAT is actively
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adiotoxicity to be managed could al
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Figure 3. Mass composition of the d
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Figure 6. Fuel cycle assumed in the
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the 4 batches scheme, allowing to a
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Figure 11. Transmutation efficiency
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1. Introduction Spent fuels of mode
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Figure 3. A change in radiotoxicity
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These dependencies are shown on Fig
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When increasing the moderator fract
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Even greater power increases are ob
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The effect of a moderator volume fr
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Table 11. Different isotopes contri
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Thus the transmutation of such FPs
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ASSESSMENT OF NUCLEAR POWER SCENARI
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elease probabilities. The time dist
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Table 2. Annual heavy nuclide contr
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Figure 3. Reduction of potential ra
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DISPOSAL OF PARTITIONING-TRANSMUTAT
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Figure 2. Decay heat from SNF 2000
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Figure 3. Shorter-lived HHR reposit
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4. Management of low-heat, long-liv
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isotope from other caesium isotopes
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THE AMSTER CONCEPT J. Vergnes 1 , D
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Figure 1. Layout diagram of the mol
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Table 1. Definition of configuratio
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We therefore adopted a partial purg
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conceivable. Thus by increasing the
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6. R&D needed to validate the AMSTE
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SESSION III PARTITIONING J.P. Glatz
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PARTITIONING-SEPARATION OF METAL IO
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The terpyridyl reagent (ligand L 1
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Figure 2. The synthesis of ADTPTZ a
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2.4 Implications for partitioning T
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SEPARATION OF MINOR ACTINIDES FROM
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installed in a hot cell. The feed w
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the concentrations of U, Pu and Np
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Table 2 shows the recovery in the r
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PARTITIONING ANIONIC AGENTS BASED O
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which of these, the Co 3+ , Fe 3+ a
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This dianionic species must be extr
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Figure 6 Ph 2 P acetone PPh 2 H2 O
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Figure 9 H 3 C RO(CH 2 )n CH 3 (CH
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[7] J. Rais and P. Selucky, Nucleon
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PYROCHEMICAL PROCESSING OF IRRADIAT
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The metallic cadmium product of the
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Figure 2. Schematic flow-sheet for
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R&D OF PYROCHEMICAL PARTITIONING IN
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(first of all pumps) for fluoride m
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4. Research on material and equipme
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REFERENCES [1] Uhlir J., Pyrochemic
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1. Introduction The increasing inte
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Figure 2. Stainless steel box with
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Figure 4. U deposit on solid cathod
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Figure 7. Schematic flow of the cou
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actinide elements from spent (metal
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DEVELOPMENT OF PLUTONIUM RECOVERY P
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uranium dendrite and that uranium c
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Table 1. Conditions and results of
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Cathode potential went down to -1.6
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Figure 6. Change of LCC potential i
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Figure 9. Relation between Pu conce
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consideration described in the prec
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[13] Y. Arai, S. Fukushima, K. Shio
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SESSION IV BASIC PHYSICS, MATERIALS
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1. Introduction The reduction of th
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agrees ours within limits of errors
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Figure 1. Thermal neutron capture c
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[18] A.P. Baerg, R.M. Bartholomew,
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1. Introduction Nowadays it is well
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In order to describe the inter-nucl
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kind of measurements allow to chara
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Figure 6. Two-dimensional cluster p
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Figure 8. Excitation functions for
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REFERENCES [1] D. Ridikas, thesis,
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1. Introduction Since 1991, the Com
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Experimental reactivity control tec
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Table 2. Neutron intensities Target
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experimental channels (horizontal a
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376
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Table 3. Planned experimental progr
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1. Introduction and benchmark speci
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neutrons. Since the neutron flux is
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Figure 2. Microscopic capture cross
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Figure 4. k eff variation in the st
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2.4 Neutron flux distribution One r
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etween the highest and the lowest v
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The isotope specific β eff values
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SESSION IV BASIC PHYSICS, MATERIALS
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1. Introduction Due to its excellen
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Figure 2. Tests scheme 0 340 h. 1 0
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Figure 4. Auger depth profile conce
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Figure 8. Auger depth profile conce
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deposited at the cold zone, and the
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inner layer grows inward from the o
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[8] V.M. Fedirko, O.I. Eliseeva, V.
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1. Introduction One of the main par
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3. Tantalum target irradiation The
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At 10-MeV neutron irradiation, radi
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1. Introduction HYPER (HYbrid Power
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this study, we used an orthogonal c
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Figure 5. Temperature distribution
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Figure 7. Thermal stress distributi
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FUEL/TARGET CONCEPTS FOR TRANSMUTAT
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(U 0.55 Pu 0.4 Np 0.05 )O 2 fuels w
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Figure 3. Left: Ceramograph of a (Z
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Figure 6. Left: ceramograph of a(Zr
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AMERICIUM TARGETS IN FAST REACTORS
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The reference case for all comparis
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It should be underlined that this c
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Cases Table 3. Heterogeneous recycl
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• A later step could be to add Cm
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RESEARCH ON NITRIDE FUEL AND PYROCH
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temperature for (Cm,Pu)N followed t
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Figure 1. Temperature dependence of
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The difference of two fuel pins exi
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In addition to the voltammetric stu
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2 wt% of Pu at 773 K. For the momen
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[13] M. Akabori, M. Takano, A. Itoh
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1. Introduction For the management
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The scientific feasibility of pluto
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Another option using a basis of sta
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6.2.1 Inert matrices 6.2.1.1 MgAl 2
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eached respectively 38.5% and 70% F
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Figure 4. Experiments for MA transm
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Figure 5a. Ecrix B rig Figure 5b. E
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A CEA/Minatom work programme is und
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9.3 Programme for dedicated fuels F
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[14] R.J.M. Konings et al., The EFT
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1. Introduction An accelerator driv
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corresponding Pb-Bi velocity is 1.1
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the fission product target. The rod
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fuel rods are at the TRU assembly t
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SESSION V TRANSMUTATION SYSTEMS AND
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1. Introduction Since the 50s, nitr
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A three dimensional model of a sub-
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Figure 4. Change in k-eigenvalue fo
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[4] Y. Arai et al., Experimental Re
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Nomenclature ADS: ATW: GT-MHR: LOF:
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Regarding switching off the beam, o
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Figure 3. Beam blocking 10 min (200
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Figure 7. A possible scenario for n
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[15] Greenspan E. et al., The Encap
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1. Introduction In the EADF design
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Equation (6) can be improved by con
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where L is obtained by a summation
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Figure 1. The natural convection im
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Figure 4 shows the temperature tren
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[12] P.H. Wakker, Thermal Hydraulic
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1. Introduction Research and develo
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Table 2. Core design parameters for
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2.2 Representation of MA transmutat
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Figure 1(b) shows the cases for the
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It is found that the higher MA tran
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REFERENCES [1] T. Ikegami, H. Hayas
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1. Introduction The management of t
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Table 1. Core performance of MA and
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Figure 3. Nuclear electricity capac
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Table 3. Experimental items at PEF
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REFERENCES [1] Takano H., Akie H.,
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1. Introduction and background The
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neutron source, the reactor can mai
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atoms. For fuel region Rf = 2.5 cm,
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Figure 3. Neutron flux spectra for
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A possible way to maintain the k ef
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higher than 99% of 239 Pu, and high
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TRANSMUTATION OF NUCLEAR WASTES WIT
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Figure 1. PBT conceptual view Table
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very tight holders for fission frag
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5. Cooling system A preliminary des
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spectral densities [10,11] and can
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MYRRHA, A MULTI-PURPOSE ADS FOR R&D
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hexagonal assemblies of 122 mm plat
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to achieve the requested performanc
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3 MYRRHA associated R&D programme F
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collaboration with Forschungszentru
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• Industrial partners, in particu
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1. Introduction The transmutation o
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Existing accelerators have been des
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suggested to look for an innovative
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Table 1. Main lead-bismuth eutectic
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4.3 The core The basic fuel sub-ass
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Figure 1. Experimental accelerator
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HELIUM-COOLED REACTOR TECHNOLOGIES
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of its potential use in nuclear wea
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Figure 2. Neutron flux distribution
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atio. Given this rate of destructio
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Figure 5. Irradiated TRISO particle
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in ceramic-coated microspheres of t
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(LOCA) event. The effect on this fe
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Figure 13. Elevation AD-FMHR The fa
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Deep burn-up of 239 Pu and fissiona
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POSTER SESSION PARTITIONING M.J. Hu
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1. Introduction The study of the be
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Plutonium was simulated with the no
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The influence of uranium and pluton
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The influence of uranium and pluton
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REFERENCES [1] I.I. Nazarenko, A.M.
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1. Introduction The long-term radio
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Ce Ce 3+ Cl - Cl 2 The voltammogram
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Figure 3. Chronopotentiograms for t
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Figure 4. Potentiometric titrations
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Experimental solubilization tests w
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[13] H. Flood T. Förland and K. Mo
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1. Introduction The separation of l
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Figure 4. Synthesis of amides 11-15
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1. Introduction Over the recent yea
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2.3.2 Set-up We set up a single HFM
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lower flow rates, Am(III) would be
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THE POTENTIAL OF NANO- AND MICROPAR
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efficiently and stable. This can be
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Figure 1a. Zetapotential of NTA-mod
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Scheme 7. Magnetic silica particles
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[13] L.H. Delmau, N. Simon, M.J. Sc
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1. Introduction 137 90 Extraction p
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Figure 3. Schematic drawing of the
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(24), 8-PhPO(OH)-O-COSAN (25), and
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REFERENCES [1] Kyrš M., +H PiQHN S
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1. Introduction A heavy-water CANDU
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These data show that fuel lifetime
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RECENT PROGRESSES ON PARTITIONING S
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hot tests (See Table2) was enough f
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trace amount of Am and Eu. The HBTM
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6. Conclusion Declassification of t
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POSTER SESSION BASIC PHYSICS: NUCLE
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1. Introduction Among the large num
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The simulation of the spallation pr
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Table 1. Parameters of the two coll
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Figure 4. Radial distribution of th
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6. The neutron escape line The comm
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Figure 7. Neutron background at the
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RECENT CAPTURE CROSS-SECTIONS VALID
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Figure 1. The GENEPI accelerator an
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2.3.3 Neutron flux measurements •
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Figure 6. Time spectrum of 3 He gas
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4. Analysis 4.1 Background subtract
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Figure 11. ENDF/B-VI, JEF2.2 and JE
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DOUBLE DIFFERENTIAL CROSS-SECTION F
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3. Conclusion Double differential c
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Figure 3. Preliminary results of do
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MEASUREMENTS OF PARTICULE EMISSION
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2. Experimental set-up The experime
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4. Results Figure 3 presents neutro
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1. Introduction Intermediate-energy
Page 724 and 725:
Table 1. Relative neutron-induced c
Page 726 and 727:
elow about 70 MeV [24] , where σ n
Page 728 and 729:
Since for sub-actinides Γ f /Γ n
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[10] V.P. Eismont, A.V. Prokofiev,
Page 733 and 734:
NUCLEON-INDUCED FISSION CROSS-SECTI
Page 735 and 736:
Figure 1. Scheme of the new code Z
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Figure 3. Neutron-induced fission c
Page 739:
REFERENCES [1] J. Raynal, Proceedin
Page 742 and 743:
1. Introduction During the past few
Page 744 and 745:
(same surface and 0.5 mm thickness)
Page 746 and 747:
Figure 2. Dependence of the total a
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Figure 3. Neutron radiative capture
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[8] MCNP, A General Monte Carlo Cod
Page 752 and 753:
1. Introduction New reactors using
Page 754 and 755:
Figure 1. Excited states of 209 Bi
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Figure 3. The fission probability o
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MEASUREMENT OF DOUBLE DIFFERENTIAL
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Figure 1. Global view of the experi
Page 763 and 764:
To get the proton (deuteron) energy
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3.1 Corrections Several corrections
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Figure 11. Active target fraction (
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d 2 σ Figure 14. Proton for n + Pb
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HIGH AND INTERMEDIATE ENERGY NUCLEA
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eactions, since the pre-equilibrium
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calculate the very short-lived radi
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cross-sections; the secondary react
Page 779 and 780:
All possible nuclear reactions will
Page 781 and 782:
A STUDY ON BURNABLE ABSORBER FOR A
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2. Burnable absorber for HYPER 2.1
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Table 2. One-group effective cross-
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of the core, is directly determined
Page 789 and 790: Figure 4. Required proton beam curr
Page 791 and 792: Figure 8. 10 B depletion in HYPER-H
Page 793: POSTER SESSION TRANSMUTATION SYSTEM
Page 796 and 797: 1. Introduction In the framework of
Page 798 and 799: Φ >1 MeV = 1.0 10 13 to 1.0 x 10 1
Page 800 and 801: 3. Irradiation targets and irradiat
Page 802 and 803: e transmuted in BR2 hence remain va
Page 804 and 805: Table 6. Atom percent concentration
Page 806 and 807: advantage, with respect to FRs, of
Page 809 and 810: ENHANCEMENT OF ACTINIDE INCINERATIO
Page 811 and 812: Here Σ fC , ( E) are the fission a
Page 813 and 814: pellet and the steel cladding. In o
Page 815 and 816: Table 3.Neutronics parameters of hy
Page 817 and 818: Figure 3. Neutron spectra averaged
Page 819 and 820: containing FA with B 4 C cladding i
Page 821: REFERENCES [1] ANSALDO Technical Re
Page 824 and 825: 1. Introduction At present, there a
Page 826 and 827: target means a change in k and the
Page 828 and 829: Following the normal procedure for
Page 830 and 831: Acknowledgements This study has bee
Page 832 and 833: 1. ADS description A conceptual des
Page 834 and 835: Substitution of (9) into (8), and u
Page 836 and 837: With the coupling LAHET + MCNP-DSP,
Page 838 and 839: Figure 3. Comparison for 1 and 5 pu
Page 842 and 843: 1. Introduction Last years importan
Page 844 and 845: eaches about 0.5% mole at a tempera
Page 846 and 847: 3.2 Precipitation of oxides Althoug
Page 848 and 849: potentials that must be maintained
Page 850 and 851: Based on experimental data received
Page 853 and 854: COMPARATIVE ASSESSMENT OF THE TRANS
Page 855 and 856: 3.1 Reference configuration As in t
Page 857 and 858: if they are distributed exactly as
Page 859 and 860: From the perspective of the whole d
Page 861 and 862: Figure 5. Radial distribution of th
Page 863: Table 10. Transmutation rates (kg/T
Page 866 and 867: 1. Introduction The concept of a hi
Page 868 and 869: underground, the radiation field ge
Page 870 and 871: REFERENCES [1] T. Iwamura et al., R
Page 872 and 873: Figure 2. Layout of deep undergroun
Page 874 and 875: 1. Introduction The problem of the
Page 876 and 877: The data presented show that the ra
Page 878 and 879: 1. Introduction The problem of the
Page 880 and 881: Table 3. Decay heat power of actini
Page 882 and 883: 1. Scientific activity on ADS in wo
Page 884 and 885: 4. Possible technical tasks on crea
Page 887 and 888: ON NECESSITY OF CREATION OF ACCELER
Page 889 and 890: Table 2. Transmutation of 99 Tc wit
Page 891:
Another important problem concernin
Page 894 and 895:
1. Introduction During the last yea
Page 896 and 897:
Other original proposal of the indi
Page 898 and 899:
Other original offer about sectiona
Page 900 and 901:
concentration of lead in heavy wate
Page 902 and 903:
[5] Kolesov V.P., Gughovski B.Ya.,
Page 905 and 906:
CONDITIONS OF PLUTONIUM, AMERICIUM
Page 907 and 908:
The further increase after 500 days
Page 909 and 910:
decrease. Total actinide amount muc
Page 911 and 912:
DEMONSTRATION ACCELERATOR DRIVEN CO
Page 913 and 914:
Thus, stable nuclides will be forme
Page 915:
Table 4. Characteristics of linac w
Page 918 and 919:
1. Introduction Nuclear waste radio
Page 920 and 921:
Figure 1. Lengthwise section view o
Page 922 and 923:
Scenario S0. This is our reference
Page 924 and 925:
Scenario 3 shows that mixing of was
Page 926 and 927:
REFERENCES [1] International GT-MHR
Page 929 and 930:
THE USE OF PB-BI EUTECTIC AS THE CO
Page 931 and 932:
P d T = 6.0E+07, time at reactor fu
Page 933 and 934:
The partial differential equations
Page 935 and 936:
Figure 5. Core and heat exchanger p
Page 937 and 938:
with the STAR-CD results is still t
Page 939 and 940:
ONE WAY TO CREATE PROLIFERATION-PRO
Page 941 and 942:
By supposing that FA manufacturing
Page 943 and 944:
exponentially reduces with rather l
Page 945 and 946:
Thus, 232 U generation by only one
Page 947 and 948:
TRANSMUTATION OF LONG-LIVED NUCLIDE
Page 949 and 950:
In the existing open fuel cycle, in
Page 951 and 952:
then include 31% of Np, 66% of Am a
Page 953 and 954:
Let us discuss the radiation balanc
Page 955 and 956:
Higher requirements for the cleanin
Page 957 and 958:
RW disposal is multibarrier configu
Page 960 and 961:
ALSO AVAILABLE ECONOMIC AND TECHNIC
Page 962:
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