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• The need for consensus on figures of merit for P&T, etc. P&T has made various advances in the past ten years. It has been shown that separation of the minor actinides is a feasible process, exhibiting high separation factors at the laboratory level; figures of merit are needed in the future. Indications are that all separation processes, hydro-reprocessing as well as pyro-reprocessing, are becoming so complex that simplicity and thus cost-reductions should become prime criteria for future development. A large variety of transmutation concepts have been proposed in response to which partitioning has been continuously adapted (increasing recovery yields). As further development in partitioning and in transmutation becomes more expensive, choices on performance and specific objectives (i.e. criteria and indicators) for P&T will be needed. Future reprocessing processes are closely linked to fuel-fabrication aspects (fissile content of fuel, type of fuel). Pyro-processes will most probably be on a batch basis with low throughput because of the limiting transfer capacity between process steps. Continuous pyro-processes may be envisaged in a few decades time. The specific question of whether to include curium in a transmutation scheme influences the partitioning processes to be developed to a pre-industrial stage. The discussions indicated that no common view exists in that respect. Whereas fuel fabricators indicated a receptiveness to separate the curium and to store it in order to decay to plutonium for recycling after about 100 years; others indicated that this (concentrated) storage would involve difficult problems such as criticality, heat removal, doses. The discussion also covered the question of why P&T might be needed and the objectives involved. P&T may be justified in order to increase the utilisation of the natural uranium resources while minimising the possible impact of the long-lived radionuclides on the biosphere. Different strategies could be envisaged. Multiple recycling has to be considered both in “double strata” strategies and in standard critical reactors to consistently reduce the final potential radiotoxicity of waste (by factors up to 200-300). “Once-through” strategies would only allow lesser reductions (factors 30-40). It was pointed out that, to obtain significant P&T effectiveness in reducing the potential radiotoxicity of waste in a deep geological repository, process losses in the fuel cycle as low as 0.1% for all transuranics are required. Another option which might improve the disposal strategy would be to adopt partitioning and conditioning (P&C) in which specific conditioning of the minor actinides (MAs) and some of the long-lived fission products (LLFPs) is applied. Even before deploying P&T in a fuel cycle, questions arise about the role of plutonium in a truly sustainable nuclear option. Sustainable development may depend on a plutonium economy in order to extend the time span over which the natural resources are available to generate electricity. In this context, one should mention that the thorium option also involves specific problems that will require substantial developments in the area of fuel cycle. One may not forget that the time scales for implementation of P&T and of geological disposal are very different. While P&T could indeed reduce the mass and radioactivity of long-lived waste, for example by a factor of 100, achieving this reduction would take several decades to equilibrium and a few centuries to achieve the potential impact on the final waste disposal. This means an institutional decision to act on P&T early and for several decades in order to reduce potential very long-term impacts. Currently, the time period from decision to implementation of geological disposal is only about 40-50 years. There has been growing interest and activity in basic science supporting P&T. This is particularly the case in the high power proton accelerator field where a synergy can be envisaged between transmutation and other applications of intense neutron sources using these accelerators. In the nuclear physics field, nuclear data measurements have experienced a revival as deficiencies in data are 8
identified. In the fuel area, laboratories for MA-handling are being built in which, over the next decade, options should be experimentally proven. A difficulty however has been identified, i.e. the reduced number of fuel irradiation facilities. Other crucial elements in the development of fuel and materials relate to corrosion and irradiation resistance; these are supported in well-structured R&D programmes. New technologies emerging from other fields of science and technology could also play an interesting role in the R&D for P&T (hollow fibres, nano-materials, other uses of Pb-Bi). The panel discussion indicated that streamlining and prioritisation of R&D is needed in the future as P&T-related R&D starts to demand more resources and, as mentioned above, would benefit of a convergence of ideas and consensus on the selection of desirable fuel cycles schemes. Choices will need to be made in the coming years. Criteria and indicators will therefore need to be identified for future guidance of work. Basic science developments (materials, nuclear data and simulation, chemistry, etc.) will be very important and this will demand an international collaborative effort. The link with waste management was considered as a priority for future work by international programmes. Finally, simplicity in P&T should be sought. The closing session ended with the statement that “the P&T community will have to make up its mind!” in the near future in order to keep the R&D well supported and well focused on the ultimate objective. This issue will be the focus of the 7 th Information Exchange Meeting which is tentatively planned to be held at the end of the year 2002 and will be hosted by the Republic of Korea. 9
Page 1 and 2: Nuclear Development ACTINIDE AND FI
Page 3 and 4: FOREWORD The objective of the OECD/
Page 5 and 6: TABLE OF CONTENTS Foreword ........
Page 7: EXECUTIVE SUMMARY More than 160 par
Page 12 and 13: 17:20-19:05 Session III: Partitioni
Page 14 and 15: Poster sessions Poster session: Par
Page 17 and 18: WELCOME ADDRESS Lucila Izquierdo Ge
Page 19 and 20: WELCOME ADDRESS Michel Hugon Co-ord
Page 21 and 22: WELCOME ADDRESS Philippe Savelli De
Page 23: developments. This will surely beco
Page 26 and 27: use of FBRs for transmutation toget
Page 28 and 29: view, i.e. better use of uranium an
Page 30 and 31: W. Forsberg proposes to reduce the
Page 32 and 33: 1. From the open fuel cycle to the
Page 34 and 35: Figures 2 and 3 show the radiotoxic
Page 36 and 37: Denoting the transuranic (TRU) or m
Page 38 and 39: or, in terms of the fuel burn-up an
Page 40 and 41: quantities of LWR-MOX and FR-MOX wi
Page 42 and 43: view of the historic development, t
Page 44 and 45: Table 5. Assumptions for transmutat
Page 46 and 47: separating troublesome fission prod
Page 48 and 49: REFERENCES [1] L.H. Baetslé, Ch. D
Page 51 and 52: SESSION III Partitioning Chairs: J.
Page 53 and 54: OVERVIEW OF THE HYDROMETALLURGICAL
Page 55 and 56: 2.1.3 Consequences Owing to the fac
Page 57 and 58: The extraction and separation mecha
Page 59 and 60:
extractant was observed. As a conse
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2.3.2 Examples of strategies and
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3. Conclusions and perspectives 3.1
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SESSION IV Basic Physics, Materials
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TRANSMUTATION: A DECADE OF REVIVAL
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2.1 The IFR concept and the homogen
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2.3 Dedicated systems Making again
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compound “macro-dispersed” in M
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Figure 3. Sketch of ADS, liquid met
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3.3.2.1 The MEGAPIE project [40] ME
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3.3.2.2 The MUSE experiments The MU
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Figure 8. Comparison of the neutron
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Figure 9. Scenarios at equilibrium
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goals in this field. Since once-thr
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• The use of Thorium in PWRs alwa
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• Understanding of the role of AD
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[17] Y. Arai, T. Ogawa, Research on
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SESSION V Transmutation Systems and
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1. Introduction The term ADS compre
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• Safety should be “designed in
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3. Minor actinide and/or transurani
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Table 2. Values of Dj (neutron cons
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Table 4. Delayed neutron fraction I
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Figure 4. η (Neutrons released per
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Table 5. ADS Distinguishing feature
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While a favourable ADS safety featu
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Optimised mixes of MA and Pu can be
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Moreover, the fuel is where neutron
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REFERENCES [1] L. Van den Durpel et
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[19] D.C. Wade and E. Fujita, Trend
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POSTER SESSION Basic Physics: Nucle
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To conclude, this poster session in
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Five other papers related to ADS co
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SESSION I OVERVIEW OF NATIONAL AND
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1. Current activities for radioacti
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3.2 Results to date and analyses of
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3.2.5.2 JNC JNC is considering the
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4.6 Short-term increase in radiatio
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Annex 1 R&D scheme for partitioning
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Annex 3 Members of the Advisory Com
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plutonium can be recycled in pressu
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choices and the implementation of m
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1. Introduction Since the 5th Infor
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strata” approach which would invo
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IAEA ACTIVITIES IN THE AREA OF EMER
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actually started to do so) because
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establishment of an international R
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The accelerator driven transmutatio
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substantiate this recommendation, s
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current, advanced and innovative nu
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ACCELERATOR DRIVEN SUB-CRITICAL SYS
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demonstration of feasibility of a E
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An extended “skeleton” for ADS
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• Fertile support (uranium) is no
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7. Conclusions The TWG under the ch
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1. Introduction The priorities for
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In the EURATOM Fourth Framework Pro
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Table 2. Cluster on transmutation-t
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6. Community research for the perio
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REFERENCES [1] “Council Decision
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1. Introduction Back in 1989, the O
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would need the continuation of tech
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individual isotopes as a function o
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Therefore, while there is continuin
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[9] OECD/NEA, Overview of Physics A
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RECENT TOPICS IN R&D FOR THE OMEGA
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Figure 1. Partitioning and transmut
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The present 4-GPP necessitates a pr
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5. Concluding remarks In 1999, the
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REFERENCES [1] T. Mukaiyama, T. Tak
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1. Introduction CIEMAT is actively
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adiotoxicity to be managed could al
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Figure 3. Mass composition of the d
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Figure 6. Fuel cycle assumed in the
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the 4 batches scheme, allowing to a
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Figure 11. Transmutation efficiency
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1. Introduction Spent fuels of mode
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Figure 3. A change in radiotoxicity
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These dependencies are shown on Fig
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When increasing the moderator fract
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Even greater power increases are ob
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The effect of a moderator volume fr
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Table 11. Different isotopes contri
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Thus the transmutation of such FPs
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ASSESSMENT OF NUCLEAR POWER SCENARI
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elease probabilities. The time dist
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Table 2. Annual heavy nuclide contr
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Figure 3. Reduction of potential ra
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DISPOSAL OF PARTITIONING-TRANSMUTAT
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Figure 2. Decay heat from SNF 2000
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Figure 3. Shorter-lived HHR reposit
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4. Management of low-heat, long-liv
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isotope from other caesium isotopes
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THE AMSTER CONCEPT J. Vergnes 1 , D
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Figure 1. Layout diagram of the mol
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Table 1. Definition of configuratio
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We therefore adopted a partial purg
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conceivable. Thus by increasing the
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6. R&D needed to validate the AMSTE
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SESSION III PARTITIONING J.P. Glatz
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PARTITIONING-SEPARATION OF METAL IO
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The terpyridyl reagent (ligand L 1
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Figure 2. The synthesis of ADTPTZ a
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2.4 Implications for partitioning T
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SEPARATION OF MINOR ACTINIDES FROM
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installed in a hot cell. The feed w
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the concentrations of U, Pu and Np
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Table 2 shows the recovery in the r
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PARTITIONING ANIONIC AGENTS BASED O
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which of these, the Co 3+ , Fe 3+ a
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This dianionic species must be extr
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Figure 6 Ph 2 P acetone PPh 2 H2 O
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Figure 9 H 3 C RO(CH 2 )n CH 3 (CH
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[7] J. Rais and P. Selucky, Nucleon
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PYROCHEMICAL PROCESSING OF IRRADIAT
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The metallic cadmium product of the
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Figure 2. Schematic flow-sheet for
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R&D OF PYROCHEMICAL PARTITIONING IN
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(first of all pumps) for fluoride m
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4. Research on material and equipme
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REFERENCES [1] Uhlir J., Pyrochemic
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1. Introduction The increasing inte
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Figure 2. Stainless steel box with
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Figure 4. U deposit on solid cathod
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Figure 7. Schematic flow of the cou
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actinide elements from spent (metal
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DEVELOPMENT OF PLUTONIUM RECOVERY P
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uranium dendrite and that uranium c
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Table 1. Conditions and results of
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Cathode potential went down to -1.6
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Figure 6. Change of LCC potential i
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Figure 9. Relation between Pu conce
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consideration described in the prec
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[13] Y. Arai, S. Fukushima, K. Shio
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SESSION IV BASIC PHYSICS, MATERIALS
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1. Introduction The reduction of th
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agrees ours within limits of errors
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Figure 1. Thermal neutron capture c
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[18] A.P. Baerg, R.M. Bartholomew,
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1. Introduction Nowadays it is well
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In order to describe the inter-nucl
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kind of measurements allow to chara
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Figure 6. Two-dimensional cluster p
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Figure 8. Excitation functions for
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REFERENCES [1] D. Ridikas, thesis,
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1. Introduction Since 1991, the Com
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Experimental reactivity control tec
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Table 2. Neutron intensities Target
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experimental channels (horizontal a
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376
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Table 3. Planned experimental progr
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1. Introduction and benchmark speci
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neutrons. Since the neutron flux is
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Figure 2. Microscopic capture cross
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Figure 4. k eff variation in the st
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2.4 Neutron flux distribution One r
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etween the highest and the lowest v
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The isotope specific β eff values
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SESSION IV BASIC PHYSICS, MATERIALS
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1. Introduction Due to its excellen
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Figure 2. Tests scheme 0 340 h. 1 0
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Figure 4. Auger depth profile conce
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Figure 8. Auger depth profile conce
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deposited at the cold zone, and the
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inner layer grows inward from the o
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[8] V.M. Fedirko, O.I. Eliseeva, V.
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1. Introduction One of the main par
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3. Tantalum target irradiation The
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At 10-MeV neutron irradiation, radi
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1. Introduction HYPER (HYbrid Power
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this study, we used an orthogonal c
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Figure 5. Temperature distribution
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Figure 7. Thermal stress distributi
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FUEL/TARGET CONCEPTS FOR TRANSMUTAT
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(U 0.55 Pu 0.4 Np 0.05 )O 2 fuels w
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Figure 3. Left: Ceramograph of a (Z
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Figure 6. Left: ceramograph of a(Zr
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AMERICIUM TARGETS IN FAST REACTORS
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The reference case for all comparis
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It should be underlined that this c
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Cases Table 3. Heterogeneous recycl
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• A later step could be to add Cm
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RESEARCH ON NITRIDE FUEL AND PYROCH
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temperature for (Cm,Pu)N followed t
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Figure 1. Temperature dependence of
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The difference of two fuel pins exi
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In addition to the voltammetric stu
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2 wt% of Pu at 773 K. For the momen
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[13] M. Akabori, M. Takano, A. Itoh
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1. Introduction For the management
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The scientific feasibility of pluto
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Another option using a basis of sta
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6.2.1 Inert matrices 6.2.1.1 MgAl 2
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eached respectively 38.5% and 70% F
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Figure 4. Experiments for MA transm
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Figure 5a. Ecrix B rig Figure 5b. E
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A CEA/Minatom work programme is und
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9.3 Programme for dedicated fuels F
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[14] R.J.M. Konings et al., The EFT
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1. Introduction An accelerator driv
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corresponding Pb-Bi velocity is 1.1
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the fission product target. The rod
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fuel rods are at the TRU assembly t
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SESSION V TRANSMUTATION SYSTEMS AND
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1. Introduction Since the 50s, nitr
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A three dimensional model of a sub-
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Figure 4. Change in k-eigenvalue fo
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[4] Y. Arai et al., Experimental Re
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Nomenclature ADS: ATW: GT-MHR: LOF:
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Regarding switching off the beam, o
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Figure 3. Beam blocking 10 min (200
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Figure 7. A possible scenario for n
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[15] Greenspan E. et al., The Encap
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1. Introduction In the EADF design
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Equation (6) can be improved by con
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where L is obtained by a summation
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Figure 1. The natural convection im
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Figure 4 shows the temperature tren
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[12] P.H. Wakker, Thermal Hydraulic
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1. Introduction Research and develo
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Table 2. Core design parameters for
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2.2 Representation of MA transmutat
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Figure 1(b) shows the cases for the
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It is found that the higher MA tran
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REFERENCES [1] T. Ikegami, H. Hayas
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1. Introduction The management of t
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Table 1. Core performance of MA and
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Figure 3. Nuclear electricity capac
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Table 3. Experimental items at PEF
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REFERENCES [1] Takano H., Akie H.,
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1. Introduction and background The
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neutron source, the reactor can mai
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atoms. For fuel region Rf = 2.5 cm,
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Figure 3. Neutron flux spectra for
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A possible way to maintain the k ef
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higher than 99% of 239 Pu, and high
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TRANSMUTATION OF NUCLEAR WASTES WIT
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Figure 1. PBT conceptual view Table
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very tight holders for fission frag
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5. Cooling system A preliminary des
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spectral densities [10,11] and can
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MYRRHA, A MULTI-PURPOSE ADS FOR R&D
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hexagonal assemblies of 122 mm plat
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to achieve the requested performanc
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3 MYRRHA associated R&D programme F
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collaboration with Forschungszentru
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• Industrial partners, in particu
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1. Introduction The transmutation o
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Existing accelerators have been des
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suggested to look for an innovative
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Table 1. Main lead-bismuth eutectic
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4.3 The core The basic fuel sub-ass
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Figure 1. Experimental accelerator
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HELIUM-COOLED REACTOR TECHNOLOGIES
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of its potential use in nuclear wea
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Figure 2. Neutron flux distribution
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atio. Given this rate of destructio
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Figure 5. Irradiated TRISO particle
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in ceramic-coated microspheres of t
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(LOCA) event. The effect on this fe
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Figure 13. Elevation AD-FMHR The fa
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Deep burn-up of 239 Pu and fissiona
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POSTER SESSION PARTITIONING M.J. Hu
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1. Introduction The study of the be
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Plutonium was simulated with the no
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The influence of uranium and pluton
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The influence of uranium and pluton
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REFERENCES [1] I.I. Nazarenko, A.M.
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1. Introduction The long-term radio
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Ce Ce 3+ Cl - Cl 2 The voltammogram
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Figure 3. Chronopotentiograms for t
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Figure 4. Potentiometric titrations
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Experimental solubilization tests w
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[13] H. Flood T. Förland and K. Mo
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1. Introduction The separation of l
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Figure 4. Synthesis of amides 11-15
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1. Introduction Over the recent yea
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2.3.2 Set-up We set up a single HFM
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lower flow rates, Am(III) would be
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THE POTENTIAL OF NANO- AND MICROPAR
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efficiently and stable. This can be
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Figure 1a. Zetapotential of NTA-mod
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Scheme 7. Magnetic silica particles
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[13] L.H. Delmau, N. Simon, M.J. Sc
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1. Introduction 137 90 Extraction p
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Figure 3. Schematic drawing of the
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(24), 8-PhPO(OH)-O-COSAN (25), and
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REFERENCES [1] Kyrš M., +H PiQHN S
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1. Introduction A heavy-water CANDU
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These data show that fuel lifetime
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RECENT PROGRESSES ON PARTITIONING S
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hot tests (See Table2) was enough f
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trace amount of Am and Eu. The HBTM
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6. Conclusion Declassification of t
Page 681:
POSTER SESSION BASIC PHYSICS: NUCLE
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1. Introduction Among the large num
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The simulation of the spallation pr
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Table 1. Parameters of the two coll
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Figure 4. Radial distribution of th
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6. The neutron escape line The comm
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Figure 7. Neutron background at the
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RECENT CAPTURE CROSS-SECTIONS VALID
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Figure 1. The GENEPI accelerator an
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2.3.3 Neutron flux measurements •
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Figure 6. Time spectrum of 3 He gas
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4. Analysis 4.1 Background subtract
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Figure 11. ENDF/B-VI, JEF2.2 and JE
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DOUBLE DIFFERENTIAL CROSS-SECTION F
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3. Conclusion Double differential c
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Figure 3. Preliminary results of do
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MEASUREMENTS OF PARTICULE EMISSION
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2. Experimental set-up The experime
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4. Results Figure 3 presents neutro
Page 722 and 723:
1. Introduction Intermediate-energy
Page 724 and 725:
Table 1. Relative neutron-induced c
Page 726 and 727:
elow about 70 MeV [24] , where σ n
Page 728 and 729:
Since for sub-actinides Γ f /Γ n
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[10] V.P. Eismont, A.V. Prokofiev,
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NUCLEON-INDUCED FISSION CROSS-SECTI
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Figure 1. Scheme of the new code Z
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Figure 3. Neutron-induced fission c
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REFERENCES [1] J. Raynal, Proceedin
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1. Introduction During the past few
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(same surface and 0.5 mm thickness)
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Figure 2. Dependence of the total a
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Figure 3. Neutron radiative capture
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[8] MCNP, A General Monte Carlo Cod
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1. Introduction New reactors using
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Figure 1. Excited states of 209 Bi
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Figure 3. The fission probability o
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MEASUREMENT OF DOUBLE DIFFERENTIAL
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Figure 1. Global view of the experi
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To get the proton (deuteron) energy
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3.1 Corrections Several corrections
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Figure 11. Active target fraction (
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d 2 σ Figure 14. Proton for n + Pb
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HIGH AND INTERMEDIATE ENERGY NUCLEA
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eactions, since the pre-equilibrium
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calculate the very short-lived radi
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cross-sections; the secondary react
Page 779 and 780:
All possible nuclear reactions will
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A STUDY ON BURNABLE ABSORBER FOR A
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2. Burnable absorber for HYPER 2.1
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Table 2. One-group effective cross-
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of the core, is directly determined
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Figure 4. Required proton beam curr
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Figure 8. 10 B depletion in HYPER-H
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POSTER SESSION TRANSMUTATION SYSTEM
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1. Introduction In the framework of
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Φ >1 MeV = 1.0 10 13 to 1.0 x 10 1
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3. Irradiation targets and irradiat
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e transmuted in BR2 hence remain va
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Table 6. Atom percent concentration
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advantage, with respect to FRs, of
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ENHANCEMENT OF ACTINIDE INCINERATIO
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Here Σ fC , ( E) are the fission a
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pellet and the steel cladding. In o
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Table 3.Neutronics parameters of hy
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Figure 3. Neutron spectra averaged
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containing FA with B 4 C cladding i
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REFERENCES [1] ANSALDO Technical Re
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1. Introduction At present, there a
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target means a change in k and the
Page 828 and 829:
Following the normal procedure for
Page 830 and 831:
Acknowledgements This study has bee
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1. ADS description A conceptual des
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Substitution of (9) into (8), and u
Page 836 and 837:
With the coupling LAHET + MCNP-DSP,
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Figure 3. Comparison for 1 and 5 pu
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MOLTEN SALTS AS POSSIBLE FUEL FLUID
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2. The fuel salt for MSB concept Ma
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and minor actinides must be removed
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4. Container material studies 4.1 F
Page 849 and 850:
management. The major developments
Page 851:
REFERENCES [1] H.J. MacPherson, Dev
Page 854 and 855:
1. Introduction The Energy Amplifie
Page 856 and 857:
Table 1. Main parameters of the EAD
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Table 5. Neutron balance in the who
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Table 7. Neutron flux distributions
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Table 8. Displacement rates DPA/yea
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DEEP UNDERGROUND TRANSMUTOR (PASSIV
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passive state. By operating at a hi
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I have proposed using an accelerato
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Figure 1. Layout of deep undergroun
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RADIATION CHARACTERISTICS OF PWR MO
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Table 1. Radiotoxicity of actinides
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RADIATION CHARACTERISTICS OF URANIU
Page 879 and 880:
Table 1. Radiotoxicity of actinides
Page 881 and 882:
INTERNATIONAL CO-OPERATION ON CREAT
Page 883 and 884:
an international base to combine ef
Page 885:
• Second topic: interaction of pr
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1. Introduction The role of acceler
Page 890 and 891:
MEPI within the framework of Projec
Page 893 and 894:
NEW ORIGINAL IDEAS ON ACCELERATOR D
Page 895 and 896:
During conceptual investigations of
Page 897 and 898:
delay, interface and computer. The
Page 899 and 900:
2. Channel-vessel design of ADS bla
Page 901 and 902:
Table 1. Characteristics of the ful
Page 903:
[14] Karavaev G.N., Kiselev G.V., M
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1. Introduction The problem of nucl
Page 908 and 909:
Table 3. Radiotoxicity in americium
Page 910 and 911:
Table 5. Characteristics of station
Page 912 and 913:
1. Introduction The atomic power en
Page 914 and 915:
of lead-bismuth target are given in
Page 917 and 918:
CRITICAL AND SUB-CRITICAL GT-MHRs F
Page 919 and 920:
Table 1. Basic GT-MHR reactor param
Page 921 and 922:
Figure 2. Typical change of the ave
Page 923 and 924:
Scenario S4. This case is actually
Page 925 and 926:
Figure 3. A change in radiotoxicity
Page 927:
[13] P. Goberis, Modelling of Innov
Page 930 and 931:
1. Introduction The Nuclear Enginee
Page 932 and 933:
Some simplifications have been made
Page 934 and 935:
Figure 3. Velocity vectors Some of
Page 936 and 937:
Figure 6. Temperature evolution at
Page 938 and 939:
• Two main reasons can explain th
Page 940 and 941:
1. Introduction Actually, we notice
Page 942 and 943:
This problem can be solved by using
Page 944 and 945:
The evaluations obtained in [2] hav
Page 946 and 947:
REFERENCES [1] Management and Dispo
Page 948 and 949:
1. Background Radiation background
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the long-term hazard of spent fuel,
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In a transmutation fuel cycle inclu
Page 954 and 955:
Figure 4. Potential biological haza
Page 956 and 957:
cooling prior to SF reprocessing an
Page 958:
REFERENCES [1] White Book of Nuclea
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ORDER FORM OECD Nuclear Energy Agen
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