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TRANSMUTATION STUDIES IN FRANCE, R&D PROGRAMME ON FUELS AND TARGETS M. Boidron 1 , N. Chauvin 1 , J.C. Garnier 1 , S Pillon 1 , G. Vambenepe 2 1 Direction des Réacteurs Nucléaires, CEA, Cadarache 13108 Saint Paul Lez Durance Cedex, France 2 EdF, 12-14 Av. Dutrievoz, 69628 Villeurbanne Cedex, France Abstract For the management of high level and long-lived radioactive waste, a large and continuous research and development effort is carried out in France, to provide a wide range of scientific and technical alternatives along three lines, partitioning and transmutation, disposal in deep geological formations and long term interim surface or subsurface storage. For the line one, and in close link with the partitioning studies, research is carried out to evaluate the transmutation potential of long-lived waste in appropriate reactors configurations (scenarios) relying on current technologies as well as innovative reactors. Performed to evaluate the theoretical feasibility of the Pu consumption and waste transmutation from the point of view of the reactor cores physics to reach the equilibrium of the material fluxes (i.e. consumption = production) and of the isotopic compositions of the fuels, these studies insure the “scientific” part of the transmutation feasibility. For the technological part of the feasibility of waste transmutation in reactors, a large programme on fuel development is underway. This includes solutions based on the advanced concepts for plutonium fuels in PWR and the development of specific fuels and targets for transmutation in fast reactors in the critical or sub-critical state. For the waste transmutation in fast reactors, an important programme has been launched to develop specific fuels and targets with experiments at various stages of preparation in different experimental reactors including Phénix. Composite fuels as well as particle fuels are considered. This programme is presented and recent results concerning the preparation of the experiments, the characterisation of the compounds properties, the thermal and mechanical modelling and the behaviour of U free fuels are given. 459
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Nuclear Development ACTINIDE AND FI
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FOREWORD The objective of the OECD/
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TABLE OF CONTENTS Foreword ........
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EXECUTIVE SUMMARY More than 160 par
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identified. In the fuel area, labor
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17:20-19:05 Session III: Partitioni
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Poster sessions Poster session: Par
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WELCOME ADDRESS Lucila Izquierdo Ge
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WELCOME ADDRESS Michel Hugon Co-ord
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WELCOME ADDRESS Philippe Savelli De
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developments. This will surely beco
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use of FBRs for transmutation toget
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view, i.e. better use of uranium an
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W. Forsberg proposes to reduce the
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1. From the open fuel cycle to the
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Figures 2 and 3 show the radiotoxic
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Denoting the transuranic (TRU) or m
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or, in terms of the fuel burn-up an
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quantities of LWR-MOX and FR-MOX wi
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view of the historic development, t
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Table 5. Assumptions for transmutat
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separating troublesome fission prod
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REFERENCES [1] L.H. Baetslé, Ch. D
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SESSION III Partitioning Chairs: J.
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OVERVIEW OF THE HYDROMETALLURGICAL
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2.1.3 Consequences Owing to the fac
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The extraction and separation mecha
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extractant was observed. As a conse
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2.3.2 Examples of strategies and
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3. Conclusions and perspectives 3.1
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SESSION IV Basic Physics, Materials
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TRANSMUTATION: A DECADE OF REVIVAL
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2.1 The IFR concept and the homogen
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2.3 Dedicated systems Making again
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compound “macro-dispersed” in M
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Figure 3. Sketch of ADS, liquid met
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3.3.2.1 The MEGAPIE project [40] ME
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3.3.2.2 The MUSE experiments The MU
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Figure 8. Comparison of the neutron
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Figure 9. Scenarios at equilibrium
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goals in this field. Since once-thr
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• The use of Thorium in PWRs alwa
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• Understanding of the role of AD
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[17] Y. Arai, T. Ogawa, Research on
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SESSION V Transmutation Systems and
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1. Introduction The term ADS compre
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• Safety should be “designed in
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3. Minor actinide and/or transurani
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Table 2. Values of Dj (neutron cons
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Table 4. Delayed neutron fraction I
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Figure 4. η (Neutrons released per
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Table 5. ADS Distinguishing feature
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While a favourable ADS safety featu
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Optimised mixes of MA and Pu can be
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Moreover, the fuel is where neutron
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REFERENCES [1] L. Van den Durpel et
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[19] D.C. Wade and E. Fujita, Trend
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POSTER SESSION Basic Physics: Nucle
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To conclude, this poster session in
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Five other papers related to ADS co
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SESSION I OVERVIEW OF NATIONAL AND
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1. Current activities for radioacti
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3.2 Results to date and analyses of
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3.2.5.2 JNC JNC is considering the
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4.6 Short-term increase in radiatio
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Annex 1 R&D scheme for partitioning
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Annex 3 Members of the Advisory Com
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plutonium can be recycled in pressu
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choices and the implementation of m
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1. Introduction Since the 5th Infor
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strata” approach which would invo
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IAEA ACTIVITIES IN THE AREA OF EMER
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actually started to do so) because
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establishment of an international R
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The accelerator driven transmutatio
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substantiate this recommendation, s
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current, advanced and innovative nu
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ACCELERATOR DRIVEN SUB-CRITICAL SYS
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demonstration of feasibility of a E
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An extended “skeleton” for ADS
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• Fertile support (uranium) is no
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7. Conclusions The TWG under the ch
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1. Introduction The priorities for
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In the EURATOM Fourth Framework Pro
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Table 2. Cluster on transmutation-t
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6. Community research for the perio
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REFERENCES [1] “Council Decision
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1. Introduction Back in 1989, the O
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would need the continuation of tech
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individual isotopes as a function o
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Therefore, while there is continuin
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[9] OECD/NEA, Overview of Physics A
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RECENT TOPICS IN R&D FOR THE OMEGA
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Figure 1. Partitioning and transmut
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The present 4-GPP necessitates a pr
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5. Concluding remarks In 1999, the
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REFERENCES [1] T. Mukaiyama, T. Tak
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1. Introduction CIEMAT is actively
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adiotoxicity to be managed could al
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Figure 3. Mass composition of the d
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Figure 6. Fuel cycle assumed in the
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the 4 batches scheme, allowing to a
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Figure 11. Transmutation efficiency
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1. Introduction Spent fuels of mode
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Figure 3. A change in radiotoxicity
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These dependencies are shown on Fig
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When increasing the moderator fract
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Even greater power increases are ob
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The effect of a moderator volume fr
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Table 11. Different isotopes contri
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Thus the transmutation of such FPs
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ASSESSMENT OF NUCLEAR POWER SCENARI
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elease probabilities. The time dist
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Table 2. Annual heavy nuclide contr
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Figure 3. Reduction of potential ra
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DISPOSAL OF PARTITIONING-TRANSMUTAT
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Figure 2. Decay heat from SNF 2000
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Figure 3. Shorter-lived HHR reposit
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4. Management of low-heat, long-liv
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isotope from other caesium isotopes
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THE AMSTER CONCEPT J. Vergnes 1 , D
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Figure 1. Layout diagram of the mol
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Table 1. Definition of configuratio
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We therefore adopted a partial purg
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conceivable. Thus by increasing the
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6. R&D needed to validate the AMSTE
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SESSION III PARTITIONING J.P. Glatz
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PARTITIONING-SEPARATION OF METAL IO
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The terpyridyl reagent (ligand L 1
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Figure 2. The synthesis of ADTPTZ a
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2.4 Implications for partitioning T
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SEPARATION OF MINOR ACTINIDES FROM
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installed in a hot cell. The feed w
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the concentrations of U, Pu and Np
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Table 2 shows the recovery in the r
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PARTITIONING ANIONIC AGENTS BASED O
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which of these, the Co 3+ , Fe 3+ a
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This dianionic species must be extr
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Figure 6 Ph 2 P acetone PPh 2 H2 O
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Figure 9 H 3 C RO(CH 2 )n CH 3 (CH
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[7] J. Rais and P. Selucky, Nucleon
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PYROCHEMICAL PROCESSING OF IRRADIAT
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The metallic cadmium product of the
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Figure 2. Schematic flow-sheet for
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R&D OF PYROCHEMICAL PARTITIONING IN
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(first of all pumps) for fluoride m
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4. Research on material and equipme
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REFERENCES [1] Uhlir J., Pyrochemic
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1. Introduction The increasing inte
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Figure 2. Stainless steel box with
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Figure 4. U deposit on solid cathod
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Figure 7. Schematic flow of the cou
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actinide elements from spent (metal
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DEVELOPMENT OF PLUTONIUM RECOVERY P
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uranium dendrite and that uranium c
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Table 1. Conditions and results of
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Cathode potential went down to -1.6
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Figure 6. Change of LCC potential i
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Figure 9. Relation between Pu conce
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consideration described in the prec
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[13] Y. Arai, S. Fukushima, K. Shio
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SESSION IV BASIC PHYSICS, MATERIALS
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1. Introduction The reduction of th
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agrees ours within limits of errors
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Figure 1. Thermal neutron capture c
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[18] A.P. Baerg, R.M. Bartholomew,
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1. Introduction Nowadays it is well
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In order to describe the inter-nucl
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kind of measurements allow to chara
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Figure 6. Two-dimensional cluster p
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Figure 8. Excitation functions for
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REFERENCES [1] D. Ridikas, thesis,
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1. Introduction Since 1991, the Com
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Experimental reactivity control tec
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Table 2. Neutron intensities Target
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experimental channels (horizontal a
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376
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Table 3. Planned experimental progr
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1. Introduction and benchmark speci
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neutrons. Since the neutron flux is
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Figure 2. Microscopic capture cross
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Figure 4. k eff variation in the st
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2.4 Neutron flux distribution One r
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etween the highest and the lowest v
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The isotope specific β eff values
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SESSION IV BASIC PHYSICS, MATERIALS
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1. Introduction Due to its excellen
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Figure 2. Tests scheme 0 340 h. 1 0
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Figure 4. Auger depth profile conce
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Figure 8. Auger depth profile conce
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deposited at the cold zone, and the
Page 408 and 409: inner layer grows inward from the o
Page 410 and 411: [8] V.M. Fedirko, O.I. Eliseeva, V.
Page 412 and 413: 1. Introduction One of the main par
Page 414 and 415: 3. Tantalum target irradiation The
Page 416 and 417: At 10-MeV neutron irradiation, radi
Page 418 and 419: 1. Introduction HYPER (HYbrid Power
Page 420 and 421: this study, we used an orthogonal c
Page 422 and 423: Figure 5. Temperature distribution
Page 424 and 425: Figure 7. Thermal stress distributi
Page 427 and 428: FUEL/TARGET CONCEPTS FOR TRANSMUTAT
Page 429 and 430: (U 0.55 Pu 0.4 Np 0.05 )O 2 fuels w
Page 431 and 432: Figure 3. Left: Ceramograph of a (Z
Page 433 and 434: Figure 6. Left: ceramograph of a(Zr
Page 435 and 436: AMERICIUM TARGETS IN FAST REACTORS
Page 437 and 438: The reference case for all comparis
Page 439 and 440: It should be underlined that this c
Page 441 and 442: Cases Table 3. Heterogeneous recycl
Page 443 and 444: • A later step could be to add Cm
Page 445 and 446: RESEARCH ON NITRIDE FUEL AND PYROCH
Page 447 and 448: temperature for (Cm,Pu)N followed t
Page 449 and 450: Figure 1. Temperature dependence of
Page 451 and 452: The difference of two fuel pins exi
Page 453 and 454: In addition to the voltammetric stu
Page 455 and 456: 2 wt% of Pu at 773 K. For the momen
Page 457: [13] M. Akabori, M. Takano, A. Itoh
Page 461 and 462: concepts for plutonium consumption
Page 463 and 464: Table 2. Objectives for transmutati
Page 465 and 466: eing adjusted to take into account
Page 467 and 468: 6.2.1.4 ZrO 2 Due to its low heat c
Page 469 and 470: Figure 3a. 3D idealised meshing of
Page 471 and 472: of 5% [24]. The target irradiation
Page 473 and 474: for the Cochix irradiation (optimis
Page 475 and 476: • Their high minor actinides (Np,
Page 477 and 478: REFERENCES [1] P. Bernard, B. Barr
Page 479 and 480: FISSION PRODUCT TARGET DESIGN FOR H
Page 481 and 482: 2. General description of the core
Page 483 and 484: 3. Basic characteristics of FP tran
Page 485 and 486: Figure 6. FP target configuration a
Page 487: Figure 7. Neutron energy spectrum f
Page 491 and 492: SAFETY ANALYSIS OF NITRIDE FUELS IN
Page 493 and 494: worth was calculated by removing al
Page 495 and 496: component increases with pin pitch,
Page 497 and 498: 4. Conclusions Having calculated th
Page 499 and 500: ASPECTS OF SEVERE ACCIDENTS IN TRAN
Page 501 and 502: direct cycle gas-cooled fast spectr
Page 503 and 504: If an inlet blockage occurred in an
Page 505 and 506: Another innovative approach is part
Page 507 and 508: REFERENCES [1] US DOE, Generation I
Page 509 and 510:
A SIMPLE MODEL TO EVALUATE THE NATU
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That in steady state conditions bec
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Moreover, the a leg of the assumed
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2.4 The gravitational pull calculat
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Figure 2. The natural convection im
Page 519 and 520:
REFERENCES [1] C. Rubbia et al., Co
Page 521 and 522:
COMPARATIVE STUDY FOR MINOR ACTINID
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nitride fuel, reflection effect of
Page 525 and 526:
Table 3. Core design parameters for
Page 527 and 528:
2.4 Comparison of neutron spectra T
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The vertical and horizontal axes re
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and adjoint flux. Relatively large
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STUDY ON A LEAD-BISMUTH COOLED ACCE
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Proton beam-trip analysis: In an AD
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Figure 2. Temperature change in pri
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4. Lead-bismuth technology Lead-bis
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Figure 4. Schematic cross-section o
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TRANSURANICS ELIMINATION IN AN OPTI
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Figure 2. Main actinides radiotoxic
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Table 1. Fuel composition Isotope D
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Table 3. Average microscopic cross-
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Table 4. Residual fractions of the
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number of C nuclei is near 2 400 ti
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[12] Salvatores M., Spiro M., The I
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1. Introduction Accelerator driven
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• The sub-critical nuclear core,
Page 562 and 563:
Figure 3. TRU elimination vs. irrad
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Table 4. General characteristics of
Page 566 and 567:
[9] Rugama Y., Muñoz-Cobo J.L., Va
Page 568 and 569:
1. Introduction SCK•CEN, the Belg
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to 40 to 70 MeV and a booster furth
Page 572 and 573:
2.4 Confinement building Parallel t
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3.2 Spallation source The choice of
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• Ente per le Nuove tecnologie, l
Page 579 and 580:
ADS: STATUS OF THE STUDIES PERFORME
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There is no specific need at the fi
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3.4 The primary coolant and the rea
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these fluids and the insurance of n
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• A solid fuel for the transmutat
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its extended use will not become a
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Figure 2. Experimental accelerator
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1. Introduction Nuclear waste can b
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Figure 1. Impact of removing & tran
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epository due to corrosion of the c
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Figure 4. Burn-up of plutonium usin
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accelerator-driven sub-critical mod
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characteristics of this direct (Bra
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The plutonium and minor actinides a
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investigated. Most of the fuel in t
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POSTER SESSIONS 611
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STUDIES ON BEHAVIOUR OF SELENIUM AN
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2.2 Chemical speciation The oxidati
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Figure 2. Isothermal equilibrium cu
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Table 2. Influence of aqueous acid
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Figure 7. Influence of HNO 3 concen
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SOLUBILIZATION STUDIES OF RARE EART
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2. Experiment details Cyclic voltam
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Figure 2 (b). Comparison between th
Page 631 and 632:
Activity coefficients of MeCl 3 in
Page 633 and 634:
Table 2. Solubility products, pk s
Page 635 and 636:
the interactions Me-substrate and M
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CALIX[6]ARENES FUNCTIONALISED WITH
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These compounds were reacted with a
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ACTINIDE(III)/LANTHANIDE(III) PARTI
Page 643 and 644:
2. Experimental 2.1 Synthesis and c
Page 645 and 646:
Figure 3. Americium(III) extraction
Page 647:
REFERENCES [1] OECD Nuclear Energy
Page 650 and 651:
1. Introduction Nano- and micropart
Page 652 and 653:
3. Selective removal of histidine-t
Page 654 and 655:
Scheme 6. Formation of the macrocyc
Page 656 and 657:
REFERENCES [1] M.D. Kaminski, and L
Page 659 and 660:
NEW EXTRACTANTS FOR PARTITIONING OF
Page 661 and 662:
of COSAN derivatives allowed for us
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On the other hand, all the above an
Page 665 and 666:
All compounds presented above were
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INFLUENCE OF INTERMEDIATE CHEMICAL
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3. Natural or slightly enriched ura
Page 671:
enrichment 1%, the burn-up grows 1.
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1. Introduction The final disposal
Page 676 and 677:
Table 3. Calculated and experimenta
Page 678 and 679:
Figure 2. General flow-sheet of Tot
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[10] J. Wang, B. Liu, J. Chen, C. S
Page 683 and 684:
DESIGN AND CHARACTERISTICS OF THE n
Page 685 and 686:
The realisation of the present desi
Page 687 and 688:
In the upper right corner of Figure
Page 689 and 690:
Figure 3. Top view of the area wher
Page 691 and 692:
y neutron reactions. The level reac
Page 693 and 694:
The geometry of the beam dump propo
Page 695:
REFERENCES [1] S. Abramovich et al.
Page 698 and 699:
1. Introduction At the dawn of XXI
Page 700 and 701:
The K parameter value, function of
Page 702 and 703:
3. Experimental results The detecto
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Figure 7: Experimental (full line)
Page 706 and 707:
Figure 9. ENDF/B-VI and JEF2.2 simu
Page 708 and 709:
5. Conclusion The neutron capture c
Page 710 and 711:
1. Experimental set-up The charged
Page 712 and 713:
Figure 2. Preliminary results of do
Page 714 and 715:
REFERENCES [1] Alford W.P. and Spic
Page 716 and 717:
1. Introduction For many accelerato
Page 718 and 719:
eam dump. We observe that the major
Page 721 and 722:
INTERMEDIATE ENERGY NEUTRON-INDUCED
Page 723 and 724:
2. Up-to-date status of the (n,f) c
Page 725 and 726:
Figure 2. The 181 Ta(n,f), nat W(n,
Page 727 and 728:
obtained more recently. It is seen
Page 729 and 730:
REFERENCES [1] C. Rubbia, The Energ
Page 731:
[20] P. Staples, P.W. Lisowski, and
Page 734 and 735:
1. Introduction Nuclear fission of
Page 736 and 737:
3. Results and perspectives On the
Page 738 and 739:
Figure 4. Yields of U isotopes in t
Page 741 and 742:
NEUTRON RADIATIVE CAPTURE CROSS-SEC
Page 743 and 744:
15 µA. At the end of the proton be
Page 745 and 746:
conditions with the minimum thermal
Page 747 and 748:
only assumption of the code is that
Page 749 and 750:
4. Conclusions The values of the ne
Page 751 and 752:
DETERMINATION OF THE NEUTRON FISSIO
Page 753 and 754:
Therefore, the neutron induced fiss
Page 755 and 756:
Figure 2. Singles protons and deute
Page 757:
Following the procedure proposed by
Page 760 and 761:
1. Introduction The renewal interes
Page 762 and 763:
Figure 3. Schematic view of a teles
Page 764 and 765:
Figure 6. Calibration curves used f
Page 766 and 767:
Figure 9. Proton spectrum before an
Page 768 and 769:
this energy and the deuteron data o
Page 770 and 771:
absolute values of proton spectra.
Page 772 and 773:
1. Introduction The HINDAS project
Page 774 and 775:
calculated. Moreover, the optical p
Page 776 and 777:
Figure 2. The Berlin ball detector
Page 778 and 779:
Finally, a new experimental techniq
Page 780 and 781:
REFERENCES [1] S. Benck, I. Slypen,
Page 782 and 783:
1. Introduction In Korea, an accele
Page 784 and 785:
Figure 1. Configuration of the Pb-B
Page 786 and 787:
3. Numerical results The performanc
Page 788 and 789:
operation), respectively. This is b
Page 790 and 791:
790 Figure 6. Normalised radial pow
Page 792 and 793:
REFERENCES [1] W.S. Part et al., HY
Page 795 and 796:
MA AND LLFP TRANSMUTATION IN MTRs A
Page 797 and 798:
70 MW. The beryllium matrix has 79
Page 799 and 800:
Table 1. Neutronic design parameter
Page 801 and 802:
Table 3. Target-volume-averaged dir
Page 803 and 804:
Only the fission process allows com
Page 805 and 806:
amounts of MAs. In addition, one sh
Page 807:
[9] E. Malambu, Progress Report on
Page 810 and 811:
1. Introduction In the last years t
Page 812 and 813:
4. Core with zirconium hydride in f
Page 814 and 815:
Figure1. Reference reactor core Fig
Page 816 and 817:
Table 4. Comparison of burn-up para
Page 818 and 819:
8. Power distribution in the refere
Page 820 and 821:
where P r is the reactor power, I p
Page 823 and 824:
REMARKS ON KINETICS PARAMETERS OF A
Page 825 and 826:
2. Sub-critical multiplication The
Page 827 and 828:
Figure 2. Radial flux distribution
Page 829 and 830:
Using such a traditional expression
Page 831 and 832:
NOISE METHOD FOR MONITORING THE SUB
Page 833 and 834:
And the descriptor used in noise an
Page 835 and 836:
Figure 1. Amplitude versus frequenc
Page 837 and 838:
As suggested by Uhrig [6], a method
Page 839:
observed that the precision of the
Page 842 and 843:
1. Introduction Last years importan
Page 844 and 845:
eaches about 0.5% mole at a tempera
Page 846 and 847:
3.2 Precipitation of oxides Althoug
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potentials that must be maintained
Page 850 and 851:
Based on experimental data received
Page 853 and 854:
COMPARATIVE ASSESSMENT OF THE TRANS
Page 855 and 856:
3.1 Reference configuration As in t
Page 857 and 858:
if they are distributed exactly as
Page 859 and 860:
From the perspective of the whole d
Page 861 and 862:
Figure 5. Radial distribution of th
Page 863:
Table 10. Transmutation rates (kg/T
Page 866 and 867:
1. Introduction The concept of a hi
Page 868 and 869:
underground, the radiation field ge
Page 870 and 871:
REFERENCES [1] T. Iwamura et al., R
Page 872 and 873:
Figure 2. Layout of deep undergroun
Page 874 and 875:
1. Introduction The problem of the
Page 876 and 877:
The data presented show that the ra
Page 878 and 879:
1. Introduction The problem of the
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Table 3. Decay heat power of actini
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1. Scientific activity on ADS in wo
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4. Possible technical tasks on crea
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ON NECESSITY OF CREATION OF ACCELER
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Table 2. Transmutation of 99 Tc wit
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Another important problem concernin
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1. Introduction During the last yea
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Other original proposal of the indi
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Other original offer about sectiona
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concentration of lead in heavy wate
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[5] Kolesov V.P., Gughovski B.Ya.,
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CONDITIONS OF PLUTONIUM, AMERICIUM
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The further increase after 500 days
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decrease. Total actinide amount muc
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DEMONSTRATION ACCELERATOR DRIVEN CO
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Thus, stable nuclides will be forme
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Table 4. Characteristics of linac w
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1. Introduction Nuclear waste radio
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Figure 1. Lengthwise section view o
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Scenario S0. This is our reference
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Scenario 3 shows that mixing of was
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REFERENCES [1] International GT-MHR
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THE USE OF PB-BI EUTECTIC AS THE CO
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P d T = 6.0E+07, time at reactor fu
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The partial differential equations
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Figure 5. Core and heat exchanger p
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with the STAR-CD results is still t
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ONE WAY TO CREATE PROLIFERATION-PRO
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By supposing that FA manufacturing
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exponentially reduces with rather l
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Thus, 232 U generation by only one
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TRANSMUTATION OF LONG-LIVED NUCLIDE
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In the existing open fuel cycle, in
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then include 31% of Np, 66% of Am a
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Let us discuss the radiation balanc
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Higher requirements for the cleanin
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RW disposal is multibarrier configu
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ALSO AVAILABLE ECONOMIC AND TECHNIC
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