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During casting, a partial vacuum (10-25 torr) was drawn above the melt for<br />

approximately twenty minutes. From data on evaporation rates of tungsten under<br />

increased pressure, it was estimated that the evaporation rate of americium could be<br />

reduced two hundred times by casting under a pressure of about 800 torr.<br />

Furthermore, based on experience with U-Zr injection casting, the vacuum level in<br />

the molds could be as high as 150 torr and the molds would still fill. (The filling<br />

technique starts at partial vacuum in the space above the melt and then pressurizes<br />

it, drawing the melt up into the glass tubes.) A judicious choice of casting<br />

parameters combined with feed stocks free of volatile impurities should make<br />

fabrication of minor actinide containing fuels quite viable.<br />

The minor-actinide-containing test pin (U-20Pu-1.3Np-1.2Am) was irradiated in<br />

EBR-II to 6% burnup, but this test too was prematurely terminated when EBR-II<br />

was shut down in 1994. The post-irradiation examinations showed very satisfactory<br />

irradiation performance. The micrograph shown in Figure 6-7 does not exhibit any<br />

features not seen in other fuels. The radial distribution of the fuel constituents is<br />

also shown in Figure 6-7. The uranium, plutonium, and zirconium distribution is<br />

very similar to that in the standard U-Pu-Zr fuel. Neptunium does not migrate; it<br />

stays put. Americium generally follows zirconium, precipitates in pores, and tends<br />

to migrate more in porous fuel. Although this was a limited test, the information it<br />

gave was positive, indicating that recycle in IFR all-actinide fuel should raise no<br />

new difficulties from spent fuel with only the major isotopes in it.<br />

(a)<br />

(b)<br />

U<br />

Pu<br />

Zr<br />

Am<br />

Np<br />

1 mm<br />

0 1<br />

2<br />

Fuel radius from center (mm)<br />

Figure 6-7. Post irradiation examinations for minor-actinide-containing fuel<br />

at 6% burnup (U-20Pu-1.3Np-1.2Am)<br />

6.10 Other Characteristics<br />

Metal fuel greatly eases the requirements placed on the non-reactor portion of<br />

the fuel cycle. Fabrication is simple, easy and cheap, processing is done in only a<br />

133

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