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2.1. TROPOSPHERIC RESEARCH GROUP 25<br />

2.1.8 Long-Path-DOAS Measurements with new fibre optic set-up<br />

André Merten (Jens Tschritter)<br />

Abstract For the first time during a field campaign a new fibre optics set up was used to couple the<br />

light source in the telescope and to receive the light from the reflector. This set-up provides a higher<br />

stability of the alignment and improves the spectral characteristics of the light source.<br />

Figure 2.9: schematic view of the new fibre optic set-up for DOAS devices<br />

Background Long-Path-Telescopes are commonly<br />

used for atmospheric trace gas measurement,<br />

especially in combination with the DOAS<br />

(Differential Optical Absorption Spectroscopy)<br />

analysis technique. Such an instrument combines<br />

the emitting and receiving telescope in one device<br />

with a double-Newton-style set up and a Xe-high<br />

pressure lamp as light source and has a typical size<br />

from 1..2m. Therefore this instrument requires a<br />

high effort in planning and executing of field measurements<br />

and has also a limited signal-to-noise<br />

ratio. The signal-to-noise ratio is limited due to<br />

the inadequate characterization of the spectrum of<br />

the light source. The used Xenon-high pressures<br />

arc lamps are showing strong variation of spectral<br />

structures across the arc. When using a ’shortcut<br />

optics’ to obtain the lamp emission spectrum is<br />

not guaranteed that the same area of the arc is<br />

imaged used in the measurement. This can cause<br />

strong residual structures, which can be misinterpreted<br />

as optical densities. Another problem is<br />

the complicated alignment of the Long-Path telescope,<br />

since all optical elements must be adjusted<br />

exactly to obtain good light throughput, which is<br />

only possible at night and limits it use as an automatic<br />

running air quality monitor. The dimensions<br />

and the weight of the lamp house require<br />

also a certain size and stability of the whole telescope.<br />

A smaller and easier to handle, and more<br />

reliable telescope would extend the range of the<br />

application for DOAS instruments.<br />

Methods and results Transmitting the light<br />

of the lamp by an optical fibre placed in the focus<br />

of the main mirror, instead of the first plane<br />

mirror, was already tested successfully. The lamp<br />

must not be connected mechanically with the tele-<br />

scope anymore and the same area of the arc is imaged<br />

in measurement and short cut regime. Since<br />

the retroreflector is imaged again to its origin<br />

(with a small displacement) emitting and receiving<br />

fibres were combined together in a bundle.<br />

Now as son as the telescope catches the reflector,<br />

the reflected light hits also to the receiving<br />

fibre (Figure 2.9). The system is now much easier<br />

to align and due to the fewer degrees of freedom<br />

much more stable. And in addition, it is also more<br />

efficient. For the quality of the short cut system a<br />

uniform illumination of the receiving fibre is important.<br />

Different reflecting materials were tested<br />

and the best results were reached with a quartz<br />

stray disc that is placed with a small motor directly<br />

in front of the fibre bundle. This set-up was<br />

tested successfully with a telescope with 1,5m focal<br />

length in the visible and near UV ranges and<br />

then used successfully in the MCMA-2006 (Mexico<br />

City Metropolitan Area) campaign in march<br />

2006 measure NO2, HCHO, Glyoxal and other<br />

species. For three weeks no manual realignment<br />

of the telescope was necessary, except for the illumination<br />

of the fibre by the lamp, which is not<br />

automated yet but can be done very simple when<br />

running the short cut optics.<br />

Outlook/Future work The optimal fibre optic<br />

configuration is now a topic of diploma thesis<br />

that should lead to the complete understanding<br />

of the optical behaviour and therefore to a new<br />

generation of DOAS telescopes [see report from<br />

Tschritter, 2.1.13]. The use of fibre optics offers<br />

the possibility to work with other light sources<br />

like LED or SLD and a fast switch between these<br />

sources.

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