List of <strong>Abstracts</strong> 183P-Observations 2.36 ID:4310 10:30MAX-DOAS Monitoring Network Observations of NO2 and Aerosols over Japan, China, Korea, andRussiaYugo Kanaya 1 , Hitoshi Irie 1 , Hisahiro Takashima 1 , Hironobu Iwabuchi 1 , Hajime Akimoto 2 , KengoSudo 3 , Young-Joon Kim 4 , Pinhua Xie 5 , Evgeny Grechko 6 , Mikhail Panchenko 7 , Myojeong Gu 4 , JihyoChong 4 , Hanlim Lee 4 , Ang Li 5 , Fuqi Si 5 , Jin Xu 5 , Wenqing Liu 5 , Anatly Dzhola 6 , Mikhail Sviridenkov 6 ,Svetlana Terpugpva 71 Japan Agency for Marine-Earth Science and Technology (JAMSTEC), Yokohama, Japan2 Acid Deposition and Oxidant Research Center, Niigata, Japan3 Nagoya University, Nagoya, Japan4 Gwangju Institute of Science and Technology (GIST), Gwangju, Korea5 Anhui Institute of Optics and Fine Mechanics (AIOFM), CAS, Hefei, China6 A.M. Obukhov Institute of Atmospheric Physics (IAP), RAS, Moscow, Russia7 V.E. Zuev Institute of Atmospheric Optics (IAO), RAS-SB, Tomsk, RussiaContact: yugo@jamstec.go.jpAir quality change in Asia and surrounding regions is paid attention because of the rapid and substantialincrease in the human activity in this region. We have established a long-term MAX-DOAS (Multi-AxisDifferential Optical Absorption Spectroscopy) monitoring network over the region to provide verticallyresolved(or integrated) NO2 densities suitable for the validation of satellite data and chemical transportmodels. Standardized instruments were deployed at 6 stations: Cape Hedo (26.87N, 128.25E, starting inMarch 2007), Yokosuka, Japan (35.32N, 139.65E, April 2007), Gwangju, Korea (35.23N, 126.84E,February 2008), Hefei, China (31.91N, 117.16E, March 2008), Zvenigorod (55.70N, 36.78E, October 2008),and Tomsk, Russia (56.48N, 85.05E, January 2009). Scattered sunlight at 6 elevation angles (3, 5, 10, 20, 30,and 90 (sometimes 70) degrees) is received sequentially by a rotating mirror and then delivered to atemperature-regulated spectrometer by a bundle of optical fibers. A set of measurements at the 6 angles took30 minutes. A single algorithm comprising of DOAS spectral fitting and inversion to yield vertical columndensities (VCD) from slant columns was applied for all of the spectra and thus provided a systematic dataset. Observations of an O4 band at 476 nm provided optical path information (and thus aerosol extinction)together with NO2 (460-490nm). A wide range of the observed tropospheric NO2 VCD ((0.5-60)x10**15molecules cm-2) benefited the satellite data validation. Clear summertime minimum was found for the 3-year observations at Cape Hedo and Yokosuka. Generally-found daytime decreases were attributable to thephotolysis, oxidation by OH, and strong emissions in the morning. However, daytime increases were foundin winter in Yokosuka, suggesting transport from other polluted regions. The levels on Sundays werelowered for Yokosuka and Gwangju where transportation sector emission is dominant, while they were notfor Hefei, suggesting that dominant sources and/or weekly emission patterns are different.P-Observations 2.37 ID:4156 10:30Optical properties of aerosols during dry and wet season over AmazoniaKenia T. Wiedemann 1 , Paulo Artaxo 1 , Steven C. Wofsy 2 , Meinrat O. Andreae 3 , Christoph Gerbig 41 University of Sao Paulo, Sao Paulo, Brazil2 Harvard University, Cambridge, USA3 Max-Planck-Institute for Chemistry, Mainz, Germany4 Max-Planck-Institute for Biogeochemistry, Jena, GermanyContact: kenia@if.usp.brThe biogeochemical cycles, among many critical processes in land-atmosphere interactions, are offundamental importance in the global radiative balance. In particular, aerosol particles change the solarradiation balance and atmospheric temperature profile, affects cloud microphysics, and has other importantiCACGP-<strong>IGAC</strong> 2010 14 July, 2010
List of <strong>Abstracts</strong> 184effects. The Amazon Basin, as a huge ecosystem, is of particular interest because of its influence in the localand global climate. Aerosol particles have a strong connection with the carbon uptake in this area, throughchange in diffuse to direct radiation. As part of the LBA/BARCA experiment, an airborne campaign wasperformed for large scale measurements of the physical properties of the aerosol particles over the AmazonBasin. The campaign occurred during November/December-2008 (Phase-A) and May-2009 (Phase-B),covering a large part of the Amazon region. A non-pressurized turbo-prop Brazilian EMBRAER Bandeiranteairplane was used, and more than 150 vertical profiles were obtained, up to 4000m, including over thetropical Atlantic Ocean. The aircraft was equipped for optical scattering measurements (TSI-Nephelometer),absorption (Thermo-MAAP5012), particle size distribution (TSI-SMPS), optical particle size distribution(OPC Lasair II), total particle concentration (TSI-CPC3010), and for trace gases measurements, includingO3, CO, CO2, CH4, and N2O. Measurements of the aerosol vertical profile show a very well mixedatmosphere, with a weak signal from the top of the boundary layer, in particular during the wet season(Phase-B). Light scattering was about 2-6 Mm-1, at the boundary layer, going down to 1 Mm-1 at 3500m,and absorption coefficients was bellow 1 Mm-1, which is close to the detection limit of the MAAPinstrument. The obtained data are being analysed in conjunction to greenhouse gases, and in terms of opticalproperties.P-Observations 2.38 ID:4167 10:30Spatio-temporal variability of light-absorbing carbon concentration in a residential area impacted bywoodsmokePatricia Krecl 1 , Christer Johansson 2 , Johan Ström 31 Universidade Estadual de Londrina2 Stockholm University3 Norwegian Polar InstituteContact: patricia.krecl@lycos.comResidential wood combustion (RWC) is responsible for 33% of the total carbon mass emitted in Europe.With the new European targets to increase the use of renewable energy, there is a growing concern that thepopulation exposure to woodsmoke will also increase. This study investigates observed and simulated lightabsorbingcarbon mass (MLAC) concentrations in a residential neighborhood (Lycksele, Sweden) whereRWC is a major air pollution source during winter. The measurements analysis included descriptivestatistics, correlation coefficient, coefficient of divergence, linear regression, concentration roses, diurnalpattern, and weekend versus weekday concentration ratios. Hourly RWC and road traffic contributions toMLAC were simulated with a Gaussian dispersion model to assess whether the model was able to mimic theobservations. Hourly mean and standard deviation concentrations measured at six sites ranged from 0.58 to0.74 µg m-3 and from 0.59 to 0.79 µg m-3, respectively. Both the temporal and spatial variability decreasedwith increasing averaging time. Low-wind periods with relatively high MLAC concentrations correlatedmore strongly than high-wind periods with low concentrations. On average, the model overestimated theobservations by 3-5 fold and explained less than 10% of the measured hourly variability at all sites. Largeresidual concentrations were associated with weak winds and relatively high MLAC loadings. Theexplanation of the observed variability increased to 31-45% when daily mean concentrations were compared.When the contribution from the boilers within the neighborhood was excluded from the simulations, themodel overestimation decreased to 16-71%. When assessing the exposure to light-absorbing carbon particlesusing this type of model, we suggest employing a longer averaging period (i.e., daily concentrations) in alarger area with an updated and very detailed emission inventory.iCACGP-<strong>IGAC</strong> 2010 14 July, 2010
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List of Authors 237Beck, Veronica .
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