Global Change Abstracts The Swiss Contribution - SCNAT
Global Change Abstracts The Swiss Contribution - SCNAT
Global Change Abstracts The Swiss Contribution - SCNAT
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<strong>Global</strong> <strong>Change</strong> <strong>Abstracts</strong> – <strong>The</strong> <strong>Swiss</strong> <strong>Contribution</strong> | Atmosphere 63<br />
08.1-70<br />
Aerosols in polar regions: A historical overview<br />
based on optical depth and in situ observations<br />
Tomasi C, Vitale V, Lupi A, Di Carmine C, Campanelli<br />
M, Herber A, Treffeisen R, Stone R S, Andrews<br />
E, Sharma S, Radionov V, von Hoyningen Huene<br />
W, Stebel K, Hansen G H, Myhre C L, Wehrli C,<br />
Aaltonen V, Lihavainen H, Virkkula A, Hillamo R,<br />
Stroem J, Toledano C, Cachorro V E, Ortiz P, de Frutos<br />
A M, Blindheim S, Frioud M, Gausa M, Zielinski<br />
T, Petelski T, Yamanouchi T<br />
Italy, Germany, USA, Canada, Russia, Norway, Switzerland,<br />
Finland, Sweden, Spain, Poland, Japan<br />
Meteorology & Atmospheric Sciences , Modelling<br />
Large sets of filtered actinometer, filtered pyrheliometer<br />
and Sun photometer measurements have<br />
been carried out over the past 30 years by various<br />
groups at different Arctic and Antarctic sites and<br />
for different time periods. <strong>The</strong>y were examined<br />
to estimate ensemble average, long-term trends<br />
of the summer background aerosol optical depth<br />
AOD(500 nm) in the polar regions (omitting the<br />
data influenced by Arctic haze and volcanic eruptions).<br />
<strong>The</strong> trend for the Arctic was estimated to<br />
be between -1.6% and -2.0% per year over 30 years,<br />
depending on location. No significant trend was<br />
observed for Antarctica. <strong>The</strong> time patterns of<br />
AOD(500 nm) and angstrom ngstrom’s parameters<br />
a and beta measured with Sun photometers during<br />
the last 20 years at various Arctic and Antarctic<br />
sites are also presented. <strong>The</strong>y give a measure<br />
of the large variations of these parameters due to<br />
El Chichon, Pinatubo, and Cerro Hudson volcanic<br />
particles, Arctic haze episodes most frequent in<br />
winter and spring, and the transport of Asian dust<br />
and boreal smokes to the Arctic region. Evidence<br />
is also shown of marked differences between the<br />
aerosol optical parameters measured at coastal<br />
and high-altitude sites in Antarctica. In situ optical<br />
and chemical composition parameters of aerosol<br />
particles measured at Arctic and Antarctic<br />
sites are also examined to achieve more complete<br />
information on the multimodal size distribution<br />
shape parameters and their radiative properties.<br />
A characterization of aerosol radiative parameters<br />
is also defined by plotting the daily mean values<br />
of a as a function of AOD(500 nm), separately for<br />
the two polar regions, allowing the identification<br />
of different clusters related to fifteen aerosol<br />
classes, for which the spectral values of complex<br />
refractive index and single scattering albedo were<br />
evaluated.<br />
Journal of Geophysical Research Atmospheres,<br />
2007, V112, ND16, AUG 21 ARTN: D16205.<br />
08.1-71<br />
Aerosol partitioning between the interstitial<br />
and the condensed phase in mixed-phase<br />
clouds<br />
Verheggen B, Cozic J, Weingartner E, Bower K,<br />
Mertes S, Connolly P, Gallagher M W, Flynn M,<br />
Choularton T, Baltensperger U<br />
Germany, England, Switzerland<br />
Meteorology & Atmospheric Sciences<br />
(1) <strong>The</strong> partitioning of aerosol particles between<br />
the cloud and the interstitial phase (i.e., unactivated<br />
aerosol) has been investigated during several<br />
Cloud and Aerosol Characterization Experiments<br />
(CLACE-3, CLACE-3 1/2 and CLACE-4) conducted in<br />
winter and summer 2004 and winter 2005 at the<br />
high alpine research station Jungfraujoch (3580<br />
m altitude, Switzerland). Ambient air was sampled<br />
using different inlets in order to determine<br />
the activated fraction of aerosol particles, F-N, defined<br />
as the fraction of the total aerosol number<br />
concentration (with particle diameter d(p) > 100<br />
nm) that has been incorporated into cloud particles.<br />
<strong>The</strong> liquid and ice water content of mixedphase<br />
clouds were characterized by analyzing<br />
multiple cloud probes. <strong>The</strong> dependence of the activated<br />
fraction on several environmental factors<br />
is discussed on the basis of more than 900 h of incloud<br />
observations and parameterizations for key<br />
variables are given. FN is found to increase with<br />
increasing liquid water content and to decrease<br />
with increasing particle number concentration in<br />
liquid clouds. FN also decreases with increasing<br />
cloud ice mass fraction and with decreasing temperature<br />
from 0 to -25 degrees C. <strong>The</strong> Wegener-<br />
Bergeron-Findeisen process probably contributed<br />
to this trend, since the presence of ice crystals<br />
causes liquid droplets to evaporate, thus releasing<br />
the formerly activated particles back into the<br />
interstitial phase. Ice nucleation could also have<br />
prevented additional cloud condensation nuclei<br />
from activating. <strong>The</strong> observed activation behavior<br />
has significant implications for our understanding<br />
of the indirect effect of aerosols on climate.<br />
Journal of Geophysical Research Atmospheres,<br />
2007, V112, ND23, DEC 13 ARTN: D23202.<br />
08.1-72<br />
Alpha-Pinene oxidation in the presence of<br />
seed aerosol: Estimates of nucleation rates,<br />
growth rates, and yield<br />
Verheggen B, Mozurkewich M, Caffrey P, Frick G,<br />
Hoppel W, Sullivan W<br />
Canada, Switzerland, USA<br />
Meteorology & Atmospheric Sciences , Modelling<br />
A recently developed inverse-modeling procedure<br />
has been applied to a case study of particle nucle-