08.12.2012 Views

Global Change Abstracts The Swiss Contribution - SCNAT

Global Change Abstracts The Swiss Contribution - SCNAT

Global Change Abstracts The Swiss Contribution - SCNAT

SHOW MORE
SHOW LESS

Create successful ePaper yourself

Turn your PDF publications into a flip-book with our unique Google optimized e-Paper software.

<strong>Global</strong> <strong>Change</strong> <strong>Abstracts</strong> – <strong>The</strong> <strong>Swiss</strong> <strong>Contribution</strong> | Atmosphere 63<br />

08.1-70<br />

Aerosols in polar regions: A historical overview<br />

based on optical depth and in situ observations<br />

Tomasi C, Vitale V, Lupi A, Di Carmine C, Campanelli<br />

M, Herber A, Treffeisen R, Stone R S, Andrews<br />

E, Sharma S, Radionov V, von Hoyningen Huene<br />

W, Stebel K, Hansen G H, Myhre C L, Wehrli C,<br />

Aaltonen V, Lihavainen H, Virkkula A, Hillamo R,<br />

Stroem J, Toledano C, Cachorro V E, Ortiz P, de Frutos<br />

A M, Blindheim S, Frioud M, Gausa M, Zielinski<br />

T, Petelski T, Yamanouchi T<br />

Italy, Germany, USA, Canada, Russia, Norway, Switzerland,<br />

Finland, Sweden, Spain, Poland, Japan<br />

Meteorology & Atmospheric Sciences , Modelling<br />

Large sets of filtered actinometer, filtered pyrheliometer<br />

and Sun photometer measurements have<br />

been carried out over the past 30 years by various<br />

groups at different Arctic and Antarctic sites and<br />

for different time periods. <strong>The</strong>y were examined<br />

to estimate ensemble average, long-term trends<br />

of the summer background aerosol optical depth<br />

AOD(500 nm) in the polar regions (omitting the<br />

data influenced by Arctic haze and volcanic eruptions).<br />

<strong>The</strong> trend for the Arctic was estimated to<br />

be between -1.6% and -2.0% per year over 30 years,<br />

depending on location. No significant trend was<br />

observed for Antarctica. <strong>The</strong> time patterns of<br />

AOD(500 nm) and angstrom ngstrom’s parameters<br />

a and beta measured with Sun photometers during<br />

the last 20 years at various Arctic and Antarctic<br />

sites are also presented. <strong>The</strong>y give a measure<br />

of the large variations of these parameters due to<br />

El Chichon, Pinatubo, and Cerro Hudson volcanic<br />

particles, Arctic haze episodes most frequent in<br />

winter and spring, and the transport of Asian dust<br />

and boreal smokes to the Arctic region. Evidence<br />

is also shown of marked differences between the<br />

aerosol optical parameters measured at coastal<br />

and high-altitude sites in Antarctica. In situ optical<br />

and chemical composition parameters of aerosol<br />

particles measured at Arctic and Antarctic<br />

sites are also examined to achieve more complete<br />

information on the multimodal size distribution<br />

shape parameters and their radiative properties.<br />

A characterization of aerosol radiative parameters<br />

is also defined by plotting the daily mean values<br />

of a as a function of AOD(500 nm), separately for<br />

the two polar regions, allowing the identification<br />

of different clusters related to fifteen aerosol<br />

classes, for which the spectral values of complex<br />

refractive index and single scattering albedo were<br />

evaluated.<br />

Journal of Geophysical Research Atmospheres,<br />

2007, V112, ND16, AUG 21 ARTN: D16205.<br />

08.1-71<br />

Aerosol partitioning between the interstitial<br />

and the condensed phase in mixed-phase<br />

clouds<br />

Verheggen B, Cozic J, Weingartner E, Bower K,<br />

Mertes S, Connolly P, Gallagher M W, Flynn M,<br />

Choularton T, Baltensperger U<br />

Germany, England, Switzerland<br />

Meteorology & Atmospheric Sciences<br />

(1) <strong>The</strong> partitioning of aerosol particles between<br />

the cloud and the interstitial phase (i.e., unactivated<br />

aerosol) has been investigated during several<br />

Cloud and Aerosol Characterization Experiments<br />

(CLACE-3, CLACE-3 1/2 and CLACE-4) conducted in<br />

winter and summer 2004 and winter 2005 at the<br />

high alpine research station Jungfraujoch (3580<br />

m altitude, Switzerland). Ambient air was sampled<br />

using different inlets in order to determine<br />

the activated fraction of aerosol particles, F-N, defined<br />

as the fraction of the total aerosol number<br />

concentration (with particle diameter d(p) > 100<br />

nm) that has been incorporated into cloud particles.<br />

<strong>The</strong> liquid and ice water content of mixedphase<br />

clouds were characterized by analyzing<br />

multiple cloud probes. <strong>The</strong> dependence of the activated<br />

fraction on several environmental factors<br />

is discussed on the basis of more than 900 h of incloud<br />

observations and parameterizations for key<br />

variables are given. FN is found to increase with<br />

increasing liquid water content and to decrease<br />

with increasing particle number concentration in<br />

liquid clouds. FN also decreases with increasing<br />

cloud ice mass fraction and with decreasing temperature<br />

from 0 to -25 degrees C. <strong>The</strong> Wegener-<br />

Bergeron-Findeisen process probably contributed<br />

to this trend, since the presence of ice crystals<br />

causes liquid droplets to evaporate, thus releasing<br />

the formerly activated particles back into the<br />

interstitial phase. Ice nucleation could also have<br />

prevented additional cloud condensation nuclei<br />

from activating. <strong>The</strong> observed activation behavior<br />

has significant implications for our understanding<br />

of the indirect effect of aerosols on climate.<br />

Journal of Geophysical Research Atmospheres,<br />

2007, V112, ND23, DEC 13 ARTN: D23202.<br />

08.1-72<br />

Alpha-Pinene oxidation in the presence of<br />

seed aerosol: Estimates of nucleation rates,<br />

growth rates, and yield<br />

Verheggen B, Mozurkewich M, Caffrey P, Frick G,<br />

Hoppel W, Sullivan W<br />

Canada, Switzerland, USA<br />

Meteorology & Atmospheric Sciences , Modelling<br />

A recently developed inverse-modeling procedure<br />

has been applied to a case study of particle nucle-

Hooray! Your file is uploaded and ready to be published.

Saved successfully!

Ooh no, something went wrong!