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Activity Report 2010 - CNRS

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HIGHLIGHT : NANOPHOTONICS<br />

CONTACTS<br />

julien.claudon@cea.fr<br />

FURTHER READING<br />

J. Claudon et al. Nature Photonics, 4,<br />

p174, (<strong>2010</strong>)<br />

J. Bleuse et al, Phys. Rev. Lett, 106,<br />

103601 (2011)<br />

5<br />

A BRIGHT SINGLE-<br />

PHOTON SOURCE<br />

BASED ON A PHOTONIC<br />

NANOWIRE<br />

The realization of an efficient, on-demand<br />

single-photon source (SPS) is an<br />

important goal for the development of<br />

quantum cryptography and photonic<br />

quantum information processing. In this<br />

context, semiconductor quantum dots<br />

(QD) are very attractive: at low<br />

temperature, they offer a stable singlephoton<br />

emission with a nearly perfect<br />

radiative yield. However, they are<br />

generally embedded in a high index<br />

semiconductor matrix that prevents the<br />

efficient collection of light in the far field.<br />

Within the “Strongchip” young scientist<br />

project supported by the Nanoscience<br />

Foundation, we have overcome this<br />

limitation and demonstrated a very bright<br />

SPS by inserting the QD inside a novel,<br />

well controlled electromagnetic<br />

environment: a photonic nanowire.<br />

A photonic wire is a monomode optical<br />

waveguide that is made of a high index<br />

dielectric material. Specifically, we<br />

consider here a structure defined in III-<br />

As semiconductors and shown in Fig. 1:<br />

the wire is made of GaAs (n=3.5) and is<br />

surrounded by air (n=1). It contains an<br />

InAs QD whose fundamental optical<br />

transition emits single photons at a free<br />

space wavelength around 920 nm. The<br />

high refractive index contrast between<br />

the wire and the air cladding has two<br />

important consequences. First, the<br />

guided mode is confined very tightly<br />

inside a wire having a 200 nm diameter,<br />

which guarantees a good coupling to the<br />

emitter. In addition, the coupling to the<br />

continuum of non-guided modes is<br />

strongly inhibited, thanks to a<br />

pronounced dielectric screening effect. As<br />

a consequence, the spontaneous<br />

emission of the QD is nearly completely<br />

funneled into the guided mode. Next, one<br />

has to collect efficiently the guided<br />

photons with a microscope objective<br />

located above the wire. For this goal, the<br />

two ends of the wire are carefully<br />

engineered. The photons emitted<br />

downward are reflected back into the<br />

guided mode with an integrated mirror,<br />

made of gold and silica. The upper wire<br />

end features a conical tip, designed to<br />

deconfine progressively the guided mode<br />

into the air cladding, in order to obtain a<br />

more directive far-field emission pattern.<br />

The fabrication process of such devices<br />

starts from a planar structure grown by<br />

molecular beam epitaxy. After deposition<br />

of the SiO 2 -Au mirror and a flip-chip step,<br />

the photonic nanowires are obtained with<br />

a dry plasma etching. Because it defines<br />

the nanowire geometry, this last step is<br />

critical and was carefully optimized.<br />

The sample was then mounted in a<br />

micro-photoluminescence setup and<br />

cooled down to liquid helium<br />

temperature. The injection of electronhole<br />

pairs to excite the QD luminescence<br />

was provided by a pulsed laser. The<br />

source efficiency, defined as the<br />

probability to emit a photon into the<br />

collecting cone of the microscope<br />

objective after an excitation pulse,<br />

reaches a maximum when the emitter is<br />

saturated. In these conditions, a record<br />

value of 0.72 photon per pulse was<br />

obtained. Simultaneously, intensity<br />

correlation measurements have provided<br />

the unambiguous signature of a very<br />

pure single-photon emission (g (2)

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