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scostep 2010 (stp12) - Leibniz-Institut für Atmosphärenphysik an der ...

scostep 2010 (stp12) - Leibniz-Institut für Atmosphärenphysik an der ...

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STP12 Abstracts<br />

Berlin, 12 - 16 July <strong>2010</strong><br />

SCOSTEP Symposium <strong>2010</strong><br />

Microphysics of electrified aerosols <strong>an</strong>d cloud droplets: Laboratory experiments<br />

Rzes<strong>an</strong>ke D<strong>an</strong>iel 1 , Leisner Thomas 2<br />

1 Karlsruhe <strong>Institut</strong>e of Technology (KIT), IMK-AAF, 2 KIT <strong>an</strong>d IUP Heidelberg<br />

The global electric circuit is one of the c<strong>an</strong>didates for a coupling of terrestrial climate with<br />

solar activity [1]. It has been suggested that the vertical electric currents in the atmosphere,<br />

which are carried by ions, ionic clusters <strong>an</strong>d electrified aerosol particles c<strong>an</strong> modify the cloud<br />

microphysics <strong>an</strong>d thereby c<strong>an</strong> link the atmospheric layers [2]. In the framework of the DFG<br />

priority program CAWSES we conduct laboratory experiments which qu<strong>an</strong>tify the interaction<br />

between electrified aerosol particles <strong>an</strong>d cloud droplets in or<strong>der</strong> to assess the atmospheric<br />

relev<strong>an</strong>ce of this link between the higher <strong>an</strong>d lower atmosphere.<br />

More specific, we qu<strong>an</strong>tify the influence of charges, electrical fields <strong>an</strong>d ionizing radiation on<br />

the heterogeneous <strong>an</strong>d homogeneous freezing nucleation in cloud droplets, their evaporation<br />

behaviour <strong>an</strong>d their scavenging efficiency for aerosol particles. The latter are relev<strong>an</strong>t for<br />

contact freezing rates in clouds <strong>an</strong>d therefore cloud development <strong>an</strong>d lifetime. The<br />

experiments are carried out un<strong>der</strong> realistic atmospheric conditions on individual particles in<br />

electrodynamic levitation within a miniaturized climate chamber [3, 4]. The main methods of<br />

investigations are microscopy, microspectroscopy <strong>an</strong>d light scattering <strong>an</strong>alysis [5].<br />

In our contribution, we present <strong>an</strong> overview of the effects <strong>an</strong>alyzed so far, demonstrate charge<br />

dependent evaporation <strong>an</strong>d scattering efficiencies <strong>an</strong>d estimate their atmospheric relev<strong>an</strong>ce.<br />

References:<br />

[1] - E. Friis-Christensen, "Solar variability <strong>an</strong>d climate", Space Science Review 94,<br />

2000<br />

[2] - B. Tinsley, "Influence of solar wind on the global electric circuit, <strong>an</strong>d inferred<br />

effects on cloud microphysics, temperature, <strong>an</strong>d dynamics in the troposphere", Space<br />

Science Review 94, 2000<br />

[3] - E. J. Davis, "A history of single aerosol particle levitation", Aerosol Science <strong>an</strong>d<br />

Technology 26, 1997<br />

[4] - D. Duft, et al., "Shape oscilliations <strong>an</strong>d stability of charged microdroplets",<br />

Physical Review Letters 89 (8), 2002<br />

[5] - D. Duft <strong>an</strong>d T. Leisner, "The index of refraction of supercooled solutions<br />

determined by the <strong>an</strong>alysis of optical rainbow scattering from levitated droplets",<br />

International Journal of Mass Spectrometry 233 (1-3), 2004

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