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188 BIBLIOGRAPHY Patkowski, A., Gapinski, J. and Meier, G. [2004]. Dynamics of supercooled van der Waals liquid under pressure. A dynamic light scattering study, Coll. Polym. Sci. 282: 874–881. Plazek, D. J. and Ngai, K. L. [1991]. Correlation of polymer segmental chain dynamics with temperature-dependent time-scale shifts, Macromolecules 24: 1222–1224. Qin, Q. and McKenna, G. B. [2006]. Correlation between dynamic fragility and glass transition temperature for different classes of glass forming liquids, J. Non-Cryst. Solids 352: 2977–2985. Quitmann, D. and Soltwisch, M. [1998]. Intermediate-range order and the liquid - glass transformation, Phil. Mag. B 77: 287–296. Reiser, A., Kasper, G. and Hunklinger, S. [2005]. Pressure-induced isothermal glass transition of small organic molecules, Phys. Rev. B 72: 094204. Richert, R. [2002]. Heterogeneous dynamics in liquids: fluctuations in space and time, J. Phys-condens Mat. 14: R703–R738. Richert, R., Duvvuri, K. and Duong, L. T. [2003]. Dynamics of glass-forming liquids. VII. Dielectric relaxation of supercooled tris-naphthylbenzene, squalane, and decahydroisoquinoline, J. Chem. Phys. 118: 1828. Roland, C. M. and Casalini, R. [2003a]. Temperature and volume effects on local segmental relaxation in poly(vinyl acetate), Macromolecules 36: 1361–1367. Roland, C. M. and Casalini, R. [2003b]. Temperature dependence of local segmental motion in polystyrene and its variation with molecular weight, J. Chem. Phys. 119: 1838–1842. Roland, C. M. and Casalini, R. [2004]. Comment on: ”Disentangling density and temperature effects in the viscous slowing down of glass forming liquids” [J. Chem. Phys. 120, 6135 (2004)], J. Chem. Phys. 121: 11503–11504. Roland, C. M., Hensel-Bielowka, S., Paluch, M. and Casalini, R. [2005]. Supercooled dynamics of glass-forming liquids and polymers under hydrostatic pressure, Rep. Prog. Phys. 68: 1405–1478. Roland, C. M., Paluch, M., Pakula, T. and Casalini, R. [2004]. Volume and temperature as control parameters for the dielectric α relaxation of polymers and molecular glass formers, Phil. Mag. 84: 1573–1581.
BIBLIOGRAPHY 189 Rössler, E. and Sokolov, A. P. [1996]. The dynamics of strong and fragile glass formers, Chemical Geology 128: 143–153. Ruffle, B., Foret, M., Courtens, E., Vacher, R. and Monaco, G. [2003]. Observation of the onset of strong scattering on high frequency acoustic phonons in densified silica glass, Phys. Rev. Lett. 90: 095502. Ruffle, B., Guimbretiere, G., Courtens, E., Vacher, R. and Monaco, G. [2006]. Glass-specific behavior in the damping of acousticlike vibrations, Phys. Rev. Lett. 96: 045502. Ruocco, G., Sciortino, F., Zamponi, F., Michele, C. D. and Scopigno, T. [2004]. Landscapes and fragilities, J. Chem. Phys. 120: 10666–10680. Ruocco, G. and Sette, F. [2001]. High-frequency vibrational dynamics in glasses, J. Phys-Condens. Mat. 13: 9141–9164. Ruocco, G., Sette, F., leonardo, R. D., Monaco, G., Sampoli, M., Scopigno, T. and Viliani, G. [2000]. Relaxation processes in harmonic glasses?, Phys. Rev. Lett. 84: 5788–5791. Sanchez, I. C. and Cho, J. [1995]. A universal equation of state for polymer liquids, Polymer 36: 2929–2939. Schiener, B., Chamberlin, R. V., Diezemann, G. and Böhmer, R. [1997]. Nonresonant dielectric hole burning spectroscopy of supercooled liquids, J. Chem. Phys. 107: 7746–7761. Schiener, B., Loidl, A., Chamberlin, R. V. and Böhmer, R. [1996]. Dielectric study of supercooled triphenylphosphite and butyronitrile: Comparison with a mesoscopic model, J. Mol. Liq. 69: 243–251. Schroeder, J., Wu, W. M., Apkarian, J. L., Lee, M., Hwa, L. G. and Moynihan, C. T. [2004]. Raman scattering and Boson peaks in glasses: temperature and pressure effects, J. Non-Cryst. Solids 349: 88–97. Scopigno, T. [2007]. et. al. to be published. Scopigno, T., Ruocco, G., Sette, F. and Monaco, G. [2003]. Is the fragility of a liquid embedded in the properties of its glass?, Science 302: 849–852. Scopigno, T., Suck, J. B., Angelini, R., Albergamo, F. and Ruocco, G. [2006]. Highfrequency dynamics in metallic glasses, Phys. Rev. Lett. 96: 135501.
Page 1:
THÈSE présentée par Kristine NIS
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Acknowledgement First of all I woul
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Contents Abstract iii Acknowledgeme
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CONTENTS ix 9 Summarizing discussio
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2 Introduction fragility with other
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Résumé du chapitre 2 De manière
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8 Slow and fast dynamics glass. The
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10 Slow and fast dynamics energy in
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12 Slow and fast dynamics increasin
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14 Slow and fast dynamics (linear)
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16 Slow and fast dynamics The dynam
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18 Slow and fast dynamics T > T 2
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20 Slow and fast dynamics as theore
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22 Slow and fast dynamics and sugge
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24 Slow and fast dynamics The boson
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26 Slow and fast dynamics modulus 3
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Chapter 3 What we learn from pressu
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3.2. Empirical scaling law and some
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Page 45 and 46:
Page 47 and 48:
3.3. Correlations with fragility 37
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3.4. Temperature dependences 39 mea
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3.5. Summary 41 assumption that the
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Chapter 4 Experimental techniques a
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4.2. Dielectric spectroscopy 47 4.1
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4.2. Dielectric spectroscopy 49 fie
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4.3. Inelastic Scattering Experimen
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Page 77 and 78:
Page 79:
Résumé du chapitre 5 La relaxatio
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72 Alpha Relaxation the dielectric
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74 Alpha Relaxation Measuring the c
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76 Alpha Relaxation 4 2 0 This work
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78 Alpha Relaxation for the 1 s iso
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80 Alpha Relaxation log10(τ α ) 2
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82 Alpha Relaxation 2 1 0 216.4K th
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84 Alpha Relaxation function has a
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86 Alpha Relaxation 2.5 2.5 2 2 log
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88 Alpha Relaxation 0.4 log 10 Im(
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90 Alpha Relaxation keeping the rel
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92 Alpha Relaxation correlation bet
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Chapter 6 High Q collective modes I
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6.1. Inelastic X-ray scattering 97
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6.2. Sound speed and attenuation 99
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6.3. Nonergodicity factor 105 where
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6.3. Nonergodicity factor 107 1 0.9
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6.3. Nonergodicity factor 109 high
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6.4. Nonergodicity factor and fragi
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Page 125 and 126:
Page 127 and 128:
6.5. Summary 117 d log (e(ρ))/ d l
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Résumé du chapitre 7 Dans ce chap
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122 Mean squared displacement colle
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124 Mean squared displacement 1.5 I
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126 Mean squared displacement 1.4 1
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128 Mean squared displacement a cen
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130 Mean squared displacement cumen
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132 Mean squared displacement / a
Page 144 and 145:
134 Mean squared displacement I P i
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136 Mean squared displacement as be
Page 149: Résumé du chapitre 8 Le pic de bo
Page 152 and 153: 142 Boson Peak The FEC-model sugges
Page 154 and 155: 144 Boson Peak the Qout Q in factor
Page 156 and 157: 146 Boson Peak We are mainly intere
Page 158 and 159: 148 Boson Peak 1.5 x 10−3 ω [meV
Page 160 and 161: 150 Boson Peak comparison of the ev
Page 162 and 163: 152 Boson Peak In figure 8.6 we sho
Page 164 and 165: 154 Boson Peak Predictions/explanat
Page 166 and 167: 156 Boson Peak meaning that the Deb
Page 168 and 169: 158 Boson Peak g(ω)/ω 2 [arb. uni
Page 170 and 171: 160 Boson Peak are equivalent becau
Page 172 and 173: 162 Boson Peak m P /m ρ 2 1.8 1.6
Page 174 and 175: 164 Boson Peak S(ω) [arb.unit] S(
Page 176 and 177: 166 Boson Peak 3 2.5 S(ω) [arb. un
Page 178 and 179: 168 Boson Peak perature effect on t
Page 181 and 182: Chapter 9 Summarizing discussion Wh
Page 183 and 184: 173 temperature in the harmonic app
Page 185: Chapter 10 Perspectives In this wor
Page 188 and 189: 178 BIBLIOGRAPHY Angell, C. A. [199
Page 190 and 191: 180 BIBLIOGRAPHY Casalini, R. and R
Page 192 and 193: 182 BIBLIOGRAPHY Farago, B., Arbe,
Page 194 and 195: 184 BIBLIOGRAPHY Inamura, Y., Arai,
Page 196 and 197: 186 BIBLIOGRAPHY Monaco, A., Chumak
Page 200 and 201: 190 BIBLIOGRAPHY Sekula, M., Pawlus
Page 203 and 204: Appendix A Details on the samples T
Page 205 and 206: A.1. Cumene 195 the value found fro
Page 207 and 208: A.2. PIB 197 The temperature depend
Page 209 and 210: A.4. DBP 199 peak differently at di
Page 211 and 212: A.6. Other samples 201 NH 2 tempera
Page 213 and 214: Appendix B Data compilations B.1 Da
Page 215 and 216: B.1. Data compilation 205 DHIQ = De
Page 217 and 218: B.1. Data compilation 207 Triphenyl
Page 219 and 220: Appendix C Dielectric setup Figure
Page 222: Abstract The degree of departure fr
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