Ph.D. thesis (pdf) - dirac

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204 Data compilations Propylen carbonate m P = 90, 93, 104 [Paluch et al., 2001], [Richert et al., 2003], [Qin and McKenna, 2006] m ρ = 57, 65 ∗ [Casalini and Roland, 2005 b], [Reiser et al., 2005] R = 1.1 (this work) β = 0.73 [Paluch et al., 2001] BMPC = 1,1’-bis(p-methoxyphenyl)cyclohexane m P = 70, 90 [Casalini and Roland, 2005 c], [Patkowski et al., 2004] m ρ = 26 [Casalini and Roland, 2005 c] β = 0.6 [Hensel-Bielowka et al., 2002 b] BMMPC = 1,1’-di(4-methoxy-5-methylphenyl)cyclohexane m P = 58, 59 [Casalini and Roland, 2005 b], [Gapinski et al., 2002] m ρ = 25 [Casalini and Roland, 2005 b] β = 0.55 [Casalini et al., 2003] DEP A = diglycidylether of bisphenol A m P = 95 [Roland et al., 2004] m ρ = 57 [Roland et al., 2004] β = 0.38 [Paluch et al., 2003 b] KDE = cresolphtalein-dimethyl-ether m P = 64, 68, 73 [Casalini and Roland, 2005 b], [Roland and Casalini, 2003b], [Paluch et al., 2001] m ρ = 34 [Casalini and Roland, 2005 b] β = 0.75 [Paluch et al., 2001]
B.1. Data compilation 205 DHIQ = Decahydroisoquinoline m P = 158, 163 [Richert et al., 2003], [Casalini et al., 2006] m ρ = 117 [Casalini et al., 2006] R = 1.3 (this work) β = 0.36 [Richert et al., 2003] ∣ = 5 (this work) P ∂ log〈u 2 〉 ∂ log T Cumene m P = 90 ∗ [Barlow et al., 1966] m ρ = 57 ∗ [Barlow et al., 1966; Bridgman, 1949] x = 4.85 8 [Barlow et al., 1966; Bridgman, 1949] R = 0.95 (this work) β = 0.66 (this work) ∣ = 4.1 (this work) P ∂ log〈u 2 〉 ∂ log T α = 0.44, f Q (T g ) = 0.6 (this work) Salol m P = 63, 68, 73 [Laughlin and Uhlmann, 1972], [Roland et al., 2005],[Paluch et al., 2001] m ρ = 36 [Roland et al., 2005] R = 0.85, 0.95 [Sokolov et al., 1993], (this work) β = 0.53, 0.6 [Böhmer et al., 1993], [Sidebottom and Sorensen, 1989] α = 0.64 [Scopigno et al., 2003] x = 5.2 [Roland et al., 2005]
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THÈSE présentée par Kristine NIS
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Acknowledgement First of all I woul
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Contents Abstract iii Acknowledgeme
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CONTENTS ix 9 Summarizing discussio
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2 Introduction fragility with other
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Résumé du chapitre 2 De manière
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8 Slow and fast dynamics glass. The
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10 Slow and fast dynamics energy in
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12 Slow and fast dynamics increasin
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14 Slow and fast dynamics (linear)
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16 Slow and fast dynamics The dynam
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18 Slow and fast dynamics T > T 2
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20 Slow and fast dynamics as theore
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22 Slow and fast dynamics and sugge
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24 Slow and fast dynamics The boson
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26 Slow and fast dynamics modulus 3
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Chapter 3 What we learn from pressu
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3.2. Empirical scaling law and some
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3.3. Correlations with fragility 37
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3.4. Temperature dependences 39 mea
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3.5. Summary 41 assumption that the
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Chapter 4 Experimental techniques a
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4.2. Dielectric spectroscopy 47 4.1
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4.2. Dielectric spectroscopy 49 fie
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4.3. Inelastic Scattering Experimen
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Page 79:
Résumé du chapitre 5 La relaxatio
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72 Alpha Relaxation the dielectric
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74 Alpha Relaxation Measuring the c
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76 Alpha Relaxation 4 2 0 This work
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78 Alpha Relaxation for the 1 s iso
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80 Alpha Relaxation log10(τ α ) 2
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82 Alpha Relaxation 2 1 0 216.4K th
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84 Alpha Relaxation function has a
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86 Alpha Relaxation 2.5 2.5 2 2 log
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88 Alpha Relaxation 0.4 log 10 Im(
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90 Alpha Relaxation keeping the rel
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92 Alpha Relaxation correlation bet
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Chapter 6 High Q collective modes I
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6.1. Inelastic X-ray scattering 97
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6.2. Sound speed and attenuation 99
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6.3. Nonergodicity factor 105 where
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6.3. Nonergodicity factor 107 1 0.9
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6.3. Nonergodicity factor 109 high
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6.4. Nonergodicity factor and fragi
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6.5. Summary 117 d log (e(ρ))/ d l
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Résumé du chapitre 7 Dans ce chap
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122 Mean squared displacement colle
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124 Mean squared displacement 1.5 I
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126 Mean squared displacement 1.4 1
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128 Mean squared displacement a cen
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130 Mean squared displacement cumen
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132 Mean squared displacement / a
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134 Mean squared displacement I P i
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136 Mean squared displacement as be
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Résumé du chapitre 8 Le pic de bo
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142 Boson Peak The FEC-model sugges
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144 Boson Peak the Qout Q in factor
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146 Boson Peak We are mainly intere
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148 Boson Peak 1.5 x 10−3 ω [meV
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150 Boson Peak comparison of the ev
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152 Boson Peak In figure 8.6 we sho
Page 164 and 165: 154 Boson Peak Predictions/explanat
Page 166 and 167: 156 Boson Peak meaning that the Deb
Page 168 and 169: 158 Boson Peak g(ω)/ω 2 [arb. uni
Page 170 and 171: 160 Boson Peak are equivalent becau
Page 172 and 173: 162 Boson Peak m P /m ρ 2 1.8 1.6
Page 174 and 175: 164 Boson Peak S(ω) [arb.unit] S(
Page 176 and 177: 166 Boson Peak 3 2.5 S(ω) [arb. un
Page 178 and 179: 168 Boson Peak perature effect on t
Page 181 and 182: Chapter 9 Summarizing discussion Wh
Page 183 and 184: 173 temperature in the harmonic app
Page 185: Chapter 10 Perspectives In this wor
Page 188 and 189: 178 BIBLIOGRAPHY Angell, C. A. [199
Page 190 and 191: 180 BIBLIOGRAPHY Casalini, R. and R
Page 192 and 193: 182 BIBLIOGRAPHY Farago, B., Arbe,
Page 194 and 195: 184 BIBLIOGRAPHY Inamura, Y., Arai,
Page 196 and 197: 186 BIBLIOGRAPHY Monaco, A., Chumak
Page 198 and 199: 188 BIBLIOGRAPHY Patkowski, A., Gap
Page 200 and 201: 190 BIBLIOGRAPHY Sekula, M., Pawlus
Page 203 and 204: Appendix A Details on the samples T
Page 205 and 206: A.1. Cumene 195 the value found fro
Page 207 and 208: A.2. PIB 197 The temperature depend
Page 209 and 210: A.4. DBP 199 peak differently at di
Page 211 and 212: A.6. Other samples 201 NH 2 tempera
Page 213: Appendix B Data compilations B.1 Da
Page 217 and 218: B.1. Data compilation 207 Triphenyl
Page 219 and 220: Appendix C Dielectric setup Figure
Page 222: Abstract The degree of departure fr
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