Ph.D. thesis (pdf) - dirac

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208 Data compilations Polystyrene m P = 77, 133 [Huang et al., 2002], [Plazek and Ngai, 1991] m ρ = 55 [Huang et al., 2002] β = 0.35 [Plazek and Ngai, 1991] Polymethylmethacrylate m P = 102, 102, 122 [Huang et al., 2002], [Plazek and Ngai, 1991], [Roland et al., 2004] m ρ = 80, 94 [Huang et al., 2002], [Roland et al., 2004] β = 0.41 [Plazek and Ngai, 1991] 1,4 Polybutadiene m P = 60, 77, 107 [Scopigno et al., 2003],[Alba-Simionesco et al., 2004],[Huang and McKenna, 2001] m ρ = 64 [Alba-Simionesco et al., 2004] x = 1.8 [Alba-Simionesco et al., 2004] α = 0.4, f Q (T g ) = 0.71 [Scopigno et al., 2003],[Fioretto et al., 1999] The ∗ indicates that the value is not given in the corresponding reference but is calculated from the data therein. The molecular weight of polymers are not always given in the references. However, for PIB and PS data are for this high molecular samples.
Appendix C Dielectric setup Figure C.1: The experimental setup for dielectric spectroscopy under pressure at Orsay. The Teflon parts shown in grey to distinguish from the metal. The length of the autoclave is ∼ 30 cm, the Teflon cell is 5 cm. 209
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THÈSE présentée par Kristine NIS
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Acknowledgement First of all I woul
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Contents Abstract iii Acknowledgeme
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CONTENTS ix 9 Summarizing discussio
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2 Introduction fragility with other
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Résumé du chapitre 2 De manière
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8 Slow and fast dynamics glass. The
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10 Slow and fast dynamics energy in
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12 Slow and fast dynamics increasin
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14 Slow and fast dynamics (linear)
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16 Slow and fast dynamics The dynam
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18 Slow and fast dynamics T > T 2
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20 Slow and fast dynamics as theore
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22 Slow and fast dynamics and sugge
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24 Slow and fast dynamics The boson
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26 Slow and fast dynamics modulus 3
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Chapter 3 What we learn from pressu
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3.2. Empirical scaling law and some
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3.3. Correlations with fragility 37
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3.4. Temperature dependences 39 mea
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3.5. Summary 41 assumption that the
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Chapter 4 Experimental techniques a
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4.2. Dielectric spectroscopy 47 4.1
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4.2. Dielectric spectroscopy 49 fie
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4.3. Inelastic Scattering Experimen
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Résumé du chapitre 5 La relaxatio
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72 Alpha Relaxation the dielectric
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74 Alpha Relaxation Measuring the c
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76 Alpha Relaxation 4 2 0 This work
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78 Alpha Relaxation for the 1 s iso
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80 Alpha Relaxation log10(τ α ) 2
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82 Alpha Relaxation 2 1 0 216.4K th
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84 Alpha Relaxation function has a
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86 Alpha Relaxation 2.5 2.5 2 2 log
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88 Alpha Relaxation 0.4 log 10 Im(
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90 Alpha Relaxation keeping the rel
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92 Alpha Relaxation correlation bet
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Chapter 6 High Q collective modes I
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6.1. Inelastic X-ray scattering 97
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6.2. Sound speed and attenuation 99
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6.3. Nonergodicity factor 105 where
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6.3. Nonergodicity factor 107 1 0.9
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6.3. Nonergodicity factor 109 high
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6.4. Nonergodicity factor and fragi
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6.5. Summary 117 d log (e(ρ))/ d l
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Résumé du chapitre 7 Dans ce chap
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122 Mean squared displacement colle
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124 Mean squared displacement 1.5 I
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126 Mean squared displacement 1.4 1
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128 Mean squared displacement a cen
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130 Mean squared displacement cumen
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132 Mean squared displacement / a
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134 Mean squared displacement I P i
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136 Mean squared displacement as be
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Résumé du chapitre 8 Le pic de bo
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142 Boson Peak The FEC-model sugges
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144 Boson Peak the Qout Q in factor
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146 Boson Peak We are mainly intere
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148 Boson Peak 1.5 x 10−3 ω [meV
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150 Boson Peak comparison of the ev
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152 Boson Peak In figure 8.6 we sho
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154 Boson Peak Predictions/explanat
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156 Boson Peak meaning that the Deb
Page 168 and 169: 158 Boson Peak g(ω)/ω 2 [arb. uni
Page 170 and 171: 160 Boson Peak are equivalent becau
Page 172 and 173: 162 Boson Peak m P /m ρ 2 1.8 1.6
Page 174 and 175: 164 Boson Peak S(ω) [arb.unit] S(
Page 176 and 177: 166 Boson Peak 3 2.5 S(ω) [arb. un
Page 178 and 179: 168 Boson Peak perature effect on t
Page 181 and 182: Chapter 9 Summarizing discussion Wh
Page 183 and 184: 173 temperature in the harmonic app
Page 185: Chapter 10 Perspectives In this wor
Page 188 and 189: 178 BIBLIOGRAPHY Angell, C. A. [199
Page 190 and 191: 180 BIBLIOGRAPHY Casalini, R. and R
Page 192 and 193: 182 BIBLIOGRAPHY Farago, B., Arbe,
Page 194 and 195: 184 BIBLIOGRAPHY Inamura, Y., Arai,
Page 196 and 197: 186 BIBLIOGRAPHY Monaco, A., Chumak
Page 198 and 199: 188 BIBLIOGRAPHY Patkowski, A., Gap
Page 200 and 201: 190 BIBLIOGRAPHY Sekula, M., Pawlus
Page 203 and 204: Appendix A Details on the samples T
Page 205 and 206: A.1. Cumene 195 the value found fro
Page 207 and 208: A.2. PIB 197 The temperature depend
Page 209 and 210: A.4. DBP 199 peak differently at di
Page 211 and 212: A.6. Other samples 201 NH 2 tempera
Page 213 and 214: Appendix B Data compilations B.1 Da
Page 215 and 216: B.1. Data compilation 205 DHIQ = De
Page 217: B.1. Data compilation 207 Triphenyl
Page 222: Abstract The degree of departure fr
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