Ph.D. thesis (pdf) - dirac

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190 BIBLIOGRAPHY Sekula, M., Pawlus, S., Hensel-bielowka, S., Ziolo, J., Paluch, M. and Roland, C. M. [2004]. Structural and secondary relaxations in supercooled di-n-butyl phthalate and diisobutyl phthalate at elevated pressure, J. Phys. Chem. B 108: 4997–5003. Sidebottom, D. L. and Sorensen, C. M. [1989]. Light-scattering study of the glasstransition in salol, Phys. Rev. B 40: 461–466. Sokolov, A. P., Calemczuk, R., Salce, B., Kisliuk, A., Quitmann, D. and Duval, E. [1997]. Low-temperature anomalies in strong and fragile glass formers, Phys. Rev. Lett. 78: 2405–2408. Sokolov, A. P., Rössler, E., Kisliuk, A. and Quitmann, D. [1993]. Dynamics of strong and fragile glass formers - differences and correlation with low-temperature properties, Phys. Rev. Lett. 71: 2062–2065. Squires [1978]. Introduction to the theory of thermal neutron scattering, Dover. Srivastava, S. and Das, S. P. [2001]. Fragility and Boson peak formation in a supercooled liquid, Phys. Lett. A 286: 76–79. Starr, F. W., Sastry, S., Douglas, J. F. and Glotzer, S. C. [2002]. What do we learn from the local geometry of glass-forming liquids?, Phys. Rev. Lett. 89: 125501. Sugai, S. and Onodera, A. [1996]. Medium-range order in permanently densified SiO 2 and GeO 2 class, Phys. Rev. Lett. 77: 4210–4213. Tarjus, G., Kivelson, D., Mossa, S. and Alba-Simionesco, C. [2004 a]. Disentangling density and temperature effects in the viscous slowing down of glassforming liquids, J. Chem. Phys. 120: 6135–6141. Tarjus, G., Mossa, S. and Alba-simionesco, C. [2004 b]. Response to: ”Comment on ’Disentangling density and temperature effects in the viscous slowing down of glassforming liquids’ ” [J. Chem. Phys. 121, 11503 (2004)], J. Chem. Phys. 121: 11505–11506. Tölle, A. [2001]. Neutron scattering studies of the model glass former orthoterphenyl, Rep. Prog. Phys. 64: 1473–1532. Tölle, A., Schober, H., Wuttke, J., Randl, O. G. and Fujara, F. [1998]. Fast relaxation in a fragile liquid under pressure, Phys. Rev. Lett. 80: 2374–2377. Vogel, H. [1921]. Das temperatureabhägigkeitsgesestz der visocosität von flüssigkeiten, Phys. Z. 22: 645–646.
BIBLIOGRAPHY 191 Wang, L. M., Velikov, V. and Angell, C. A. [2002]. Direct determination of kinetic fragility indices of glassforming liquids by differential scanning calorimetry: Kinetic versus thermodynamic fragilities, J. Chem. Phys. 117: 10184–10192. Wilson, L. C., Wilson, H. L., Wilding, W. V. and Wilson, G. M. [1996]. Critical point measurements for fourteen compounds by a static method and a flow method, J. Chem. Eng. Data 41: 1252–1254. Würflinger, A. [n.d.]. data. private communication. Yamaguchi, M., Nakayama, T. and Yagi, T. [1999]. Effects of high pressure on the Bose peak in a-GeS 2 studied by light scattering, Physica B 263: 258–260. Yannopoulos, S. N., Andrikopoulos, K. S. and Ruocco, G. [2006 a]. On the analysis of the vibrational boson peak and low-energy excitations in glasses, J. Non-Cryst. Solids 352: 4541–4551. Yannopoulos, S. N. and Johari, G. P. [2006]. Glass behaviour - Poisson’s ratio and liquid’s fragility, Nature 442: E7–E8 AUG 3 2006. Yannopoulos, S. N. and Papatheodorou, G. N. [2000]. Critical experimental facts pertaining to models and associated universalities for low-frequency Raman scattering in inorganic glass formers, Phys. Rev. B 62: 3728–3734.
Page 1:
THÈSE présentée par Kristine NIS
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Acknowledgement First of all I woul
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Contents Abstract iii Acknowledgeme
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CONTENTS ix 9 Summarizing discussio
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2 Introduction fragility with other
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Résumé du chapitre 2 De manière
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8 Slow and fast dynamics glass. The
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10 Slow and fast dynamics energy in
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12 Slow and fast dynamics increasin
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14 Slow and fast dynamics (linear)
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16 Slow and fast dynamics The dynam
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18 Slow and fast dynamics T > T 2
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20 Slow and fast dynamics as theore
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22 Slow and fast dynamics and sugge
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24 Slow and fast dynamics The boson
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26 Slow and fast dynamics modulus 3
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Chapter 3 What we learn from pressu
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3.2. Empirical scaling law and some
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Page 45 and 46:
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3.3. Correlations with fragility 37
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3.4. Temperature dependences 39 mea
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3.5. Summary 41 assumption that the
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Chapter 4 Experimental techniques a
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4.2. Dielectric spectroscopy 47 4.1
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4.2. Dielectric spectroscopy 49 fie
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4.3. Inelastic Scattering Experimen
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Page 79:
Résumé du chapitre 5 La relaxatio
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72 Alpha Relaxation the dielectric
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74 Alpha Relaxation Measuring the c
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76 Alpha Relaxation 4 2 0 This work
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78 Alpha Relaxation for the 1 s iso
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80 Alpha Relaxation log10(τ α ) 2
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82 Alpha Relaxation 2 1 0 216.4K th
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84 Alpha Relaxation function has a
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86 Alpha Relaxation 2.5 2.5 2 2 log
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88 Alpha Relaxation 0.4 log 10 Im(
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90 Alpha Relaxation keeping the rel
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92 Alpha Relaxation correlation bet
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Chapter 6 High Q collective modes I
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6.1. Inelastic X-ray scattering 97
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6.2. Sound speed and attenuation 99
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6.3. Nonergodicity factor 105 where
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6.3. Nonergodicity factor 107 1 0.9
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6.3. Nonergodicity factor 109 high
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6.4. Nonergodicity factor and fragi
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6.5. Summary 117 d log (e(ρ))/ d l
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Résumé du chapitre 7 Dans ce chap
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122 Mean squared displacement colle
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124 Mean squared displacement 1.5 I
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126 Mean squared displacement 1.4 1
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128 Mean squared displacement a cen
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130 Mean squared displacement cumen
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132 Mean squared displacement / a
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134 Mean squared displacement I P i
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136 Mean squared displacement as be
Page 149: Résumé du chapitre 8 Le pic de bo
Page 152 and 153: 142 Boson Peak The FEC-model sugges
Page 154 and 155: 144 Boson Peak the Qout Q in factor
Page 156 and 157: 146 Boson Peak We are mainly intere
Page 158 and 159: 148 Boson Peak 1.5 x 10−3 ω [meV
Page 160 and 161: 150 Boson Peak comparison of the ev
Page 162 and 163: 152 Boson Peak In figure 8.6 we sho
Page 164 and 165: 154 Boson Peak Predictions/explanat
Page 166 and 167: 156 Boson Peak meaning that the Deb
Page 168 and 169: 158 Boson Peak g(ω)/ω 2 [arb. uni
Page 170 and 171: 160 Boson Peak are equivalent becau
Page 172 and 173: 162 Boson Peak m P /m ρ 2 1.8 1.6
Page 174 and 175: 164 Boson Peak S(ω) [arb.unit] S(
Page 176 and 177: 166 Boson Peak 3 2.5 S(ω) [arb. un
Page 178 and 179: 168 Boson Peak perature effect on t
Page 181 and 182: Chapter 9 Summarizing discussion Wh
Page 183 and 184: 173 temperature in the harmonic app
Page 185: Chapter 10 Perspectives In this wor
Page 188 and 189: 178 BIBLIOGRAPHY Angell, C. A. [199
Page 190 and 191: 180 BIBLIOGRAPHY Casalini, R. and R
Page 192 and 193: 182 BIBLIOGRAPHY Farago, B., Arbe,
Page 194 and 195: 184 BIBLIOGRAPHY Inamura, Y., Arai,
Page 196 and 197: 186 BIBLIOGRAPHY Monaco, A., Chumak
Page 198 and 199: 188 BIBLIOGRAPHY Patkowski, A., Gap
Page 203 and 204: Appendix A Details on the samples T
Page 205 and 206: A.1. Cumene 195 the value found fro
Page 207 and 208: A.2. PIB 197 The temperature depend
Page 209 and 210: A.4. DBP 199 peak differently at di
Page 211 and 212: A.6. Other samples 201 NH 2 tempera
Page 213 and 214: Appendix B Data compilations B.1 Da
Page 215 and 216: B.1. Data compilation 205 DHIQ = De
Page 217 and 218: B.1. Data compilation 207 Triphenyl
Page 219 and 220: Appendix C Dielectric setup Figure
Page 222: Abstract The degree of departure fr
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