Inorganic Microporous Membranes for Gas Separation in Fossil Fuel ...

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Curriculum Vitae – George van der Donk George van der Donk was born in Nijmegen at 1978. He started his study chemical engineering at the University of Twente in 1997. His traineeship on solid oxide fuels cells was performed at Risø National Laboratory in Denmark. George graduated, as a member of the Inorganic Materials Science research group, from the University of Twente. His thesis: “Oxygen coulometric titration of mixed conducting perovskites”. After university he went to Forschungszentrum Jülich GmbH (Germany) to start his Ph.D. For the Institute for materials and processes in energy systems, in cooperation with the Ruhr University of Bochum, he wrote this Ph.D thesis and other publications. Currently he is working as a Design Engineer at Sensata Technologies Holland B.V. in Almelo (the Netherlands), where he develops electrochemical sensors for the automotive industry.
Acknowledgement First of all, I would like to thank my Doktorvater Professor Stöver for giving me the opportunity to do this PhD. I am grateful to Buchkremer for his enthousiasm for this topic about inorganic membranes and for his efforts to setup the membrane group in Jülich. I would also thank Robert Vassen and his Thermal barrier layer group for their support. The person who answered most of my scientific and social questions is my supervisor Willi Meulenberg. With his motivation, we were able to create, on short notice, a wellaccepted inorganic membrane group. Besides he also formed a bridge between the German work culture and my Dutch culture. The inorganic membrane group including Vicente, Martin Bram, Kampel, Hansch, Wiener, Betz, Willi, Tim, Oli and Jose are gratefully acknowledged. Many of the experiments and characterisations could not have been done without the help of e.g. Sebold, Fischer, Lersch, Coenen, Pracht, Werner, Kicky, Mai, Hannelore, Vicky and Kappertz from our institute and Wim Pyckhout-Hinzten, Michulitz, Esser, Peica, Besmehn and Breuer from the other institutes of the Forschungszentrum Jülich. Professor Gies, Bernd-“ich bin mahl gespannt”-Marler and Somsen from the Ruhr Universität Bochum are thanked respectively for scientific zeolite discussions, cooking together D1H and SEM/TEM analysis. Mieke is thanked for introducing me in to the world of ceramic manufacturing. Rob Delhez is gratefully acknowledged for the discussions on crystallinity. My joy in inorganic membrane science was enhanced by the chats with Miquel Menendez, Joe Da Costa, Frederic, Marcel den Exter and Rune Bredesen. The high quality of the article containing the permeance of titania-zirconia membranes is mainly due to the effort of Nieck Benes and Marcus van Schilt from the University of Eindhoven. Most of the permeance measurements were performed by Marcus. Due to the personalities of Nati and Jozef as well, our office quickly changed to the most popular gossip and coffee room. Both roommates contributed to the positive work atmosphere. Jürgen and Dirk, my carpool-mates, transported me daily to Jülich and back. Thanks for that. It was an honour to defend several times the running-cup for the fastest FZJ institute. This could not have been achieved without the frequent trainings with Xabier, JB, Alexandra, Daniel and Ettler. Special thanks are addressed to Henny Bouwmeester from the University of Twente. He was constantly interested in my progress and in our project. This resulted finally in a corporation between the University of Twente and FZJ. Many improvements to this thesis are a result of scientific discussions with Henny. It was a great pleasure to write two papers with Jose Manuel Serra Alfaro. His work mentality and scientific thoroughness trigged me constantly.
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Mitglied der Helmholtz-Gemeinschaft
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Forschungszentrum Jülich GmbH Inst
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List of Abbreviations Ac Acetyl Ace
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Summary CO2 capture and storage mig
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Zusammenfassung Die Abtrennung und
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Content Content CONTENT............
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1 Introduction and aims 1 Introduct
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1 Introduction and aims Candidate m
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2 Theoretical background 2 Theoreti
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2 Theoretical background Despite th
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2 Theoretical background Table 2 Ox
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2 Theoretical background 2.1.2 Micr
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2 Theoretical background Poly-cryst
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2 Theoretical background membranes
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2 Theoretical background Dry or wet
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2 Theoretical background the materi
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2 Theoretical background Figure 9 D
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2 Theoretical background Figure 11
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2 Theoretical background due to its
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2 Theoretical background 2.3.3.2 Mi
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2 Theoretical background 2.4 Microp
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2 Theoretical background Figure 15
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2 Theoretical background wall inter
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3 Experimental 3 Experimental The m
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3 Experimental vacuum sample holder
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3 Experimental o of as-made DOH cry
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3 Experimental Another solution was
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3 Experimental 3.4 Characterisation
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3 Experimental Element analysis The
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3 Experimental Additionally, the hy
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4 Results and discussion Abundance
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4 Results and discussion 4.2 Zeolit
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4 Results and discussion Table 14 D
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4 Results and discussion hours usin
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4 Results and discussion Intensity
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4 Results and discussion The carbon
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4 Results and discussion DOH crysta
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4 Results and discussion 900 [ºC]
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4 Results and discussion characteri
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4 Results and discussion without a
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Page 84 and 85: 4 Results and discussion Solid Cont
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Page 94 and 95: 4 Results and discussion Vads / cm
Page 96 and 97: 4 Results and discussion The increa
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Page 100 and 101: 4 Results and discussion V micro /V
Page 102 and 103: 4 Results and discussion In pure Ti
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Page 106 and 107: 4 Results and discussion Intensity
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Page 112 and 113: 4 Results and discussion Raman Inte
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Page 116 and 117: 4 Results and discussion Mol% Carbo
Page 118 and 119: 4 Results and discussion Permeance
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Page 122 and 123: 5 Conclusions and recommendations m
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Page 126 and 127: 6 References 22. Shao, Z., Dong, H.
Page 128 and 129: 6 References 65. Van den Berg, A. W
Page 130 and 131: 6 References 108. Wen, T. L., Heber
Page 134: Last but not least, I would like to
Page 137: Band | Volume 8 ISBN 978-3-89336-52
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Inorganic Microporous Membranes for Gas Separation in Fossil Fuel ...

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