CHAPTER 4 – SOUTH AMERICAThe National Commission for the Environment (CONAMA, now Ministry for theEnvironment) has over the years driven various campaigns to assess the composition of particles[e.g., Artaxo et al., 1999; Didyk et al., 2000; Kavouras et al., 1999; Gramsch et al., 2009] and toaddress speciation of volatile organic compounds and photochemical products [e.g., Rappenglücket al., 2000; Rubio et al., 2004; Rappenglück et al., 2005]. Other studies have been developedwithin a pure academic framework addressing, again, particles and photochemistry [e.g., Sienra etal., 2005; Sienra and Rosazza, 2006; Rubio et al., 2006; Richter et al., 2007; Morata et al., 2008;Elshorbany et al., 2009a; 2009b; Seguel et al., 2009].In addition to air quality stations, a meteorological network was put in place in 1997. Itconsisted of 22 stations and it was designed to capture mesoscale meteorological featuresinduced by complex topography in the area. Today, only 10 stations are operational. Verticalsoundings have been sporadic, and only since 2007, a ceilometer located in downtown Santiago isproviding a record of daytime mixed layer for cloud free days [Muñoz and Undurraga, 2010]. In2010, a backscatter LIDAR was installed by the Chilean Weather Office that is expected to provideunprecedented information about atmospheric stability and aerosol properties.Regarding impacts of air pollution, health issues have received the greatest attention,particularly the association between particulate matter and morbidity and mortality statistics [e.g.,Adonis and Gil, 1993; Ostro et al., 1996; Ostro et al., 1999; Ilabaca et al., 1999; Cifuentes et al.,2001a; 2001b]. A few studies have approached health issues within the framework of climatechange scenarios and mitigation measures [e.g., Cifuentes et al., 2001a; 2001b]. Less attentionhas been paid to effects on vegetation [e.g., García-Huidobro et al., 2001]. Only recently, thepotential impacts of air pollution on the stratus deck downwind from Santiago are beginning to bestudied [e.g., Mena et al., 2009; Spak et al., 2010; Saide et al., 2012; Heinrichs et al., 2012].Since the implementation of the attainment plan for Santiago, CONAMA has supportedformulation of emission inventories for base years 1997, 2000, and 2005, and a projection for 2010[CENMA, 1997; CENMA, 2000; DICTUC, 2007]. Unfortunately, over time this endeavour has beencontracted under consultancies of different organizations giving room for differences betweenmethodologies and even lack of transparency in some results.Mobile emissions were estimated in the CENMA inventories (1997, 2000) according to abottom-up methodology [Corvalán et al., 2002] considering official traffic modelling results,comprehensive traffic counts, analysis of databases for vehicle technology distribution andemission factors from COPERT III model [Ntziachristos and Samaras, 2000] and localmeasurements. Later, subsequent contractors have modified this methodology but it is unclearwhat the modifications are. Industrial and biogenic emissions are estimated following USEPAmethodologies.In the first version of the attainment plan (1997), curbing measures considered theintroduction of natural gas in the industrial sector, a reduction in sulphur content in diesel (from5000 ppm in 1989 to 1000 ppm in 1997, and 300 ppm in 2001), introducing emission controls forvehicles and phasing out 3000 old buses, etc. These measures explain the relatively fast reductionin PM 10 and SO 2 between 1997 and 2000. A second revision of the attainment plan in 2004emphasized emission control for vehicles, including a reduction in diesel sulphur content to 50 ppm,and the introduction of an ambitious public transportation system called Transantiago(http://www.transantiagoinforma.cl/). Transantiago intended to completely overhaul the existingtransportation system with new EURO III diesel buses, and reducing the total amount of busesfrom more than 8000 to ~4000. Soon after its implementation in early 2006, the collapse of thesystem due to increased demand required that 2500 old buses (which had been removed fromcirculation) to be reintroduced, bringing the current total to 6500 units. The contracts required thatthese old buses would use retrofitted particulate filters, as their emissions are roughly 10 timeshigher than the new Euro III buses. To date these buses continue to circulate without particulatefilters, making the success of Transantiago’s emission reductions less apparent.158
CHAPTER 4 – SOUTH AMERICABetween 2000 and 2006, a toll based urban highway was built, which allowed sprawlingsuburbs to connect with the city in substantially less time. The combination of a slow publictransportation system with an efficient highway system may have led previous users of the publictransportation system to buy cars and motorcycles. From 2000 to 2008, the number of cars inSantiago grew by 42% to 1.2 million. This growth in private transportation probably accounts forthe lack of substantial reductions in pollutant levels despite the improvements in fuel and vehicletechnology over the same period. In addition, after 2004, imports of natural gas from Argentinawere restricted forcing industry to reconvert to other liquid fuels, such as petroleum products ordiesel. This caused increased SO 2 and NO X emissions, ultimately leading to increased PM 2.5 yearlymeans for 2007 and 2008. It is hoped that the recent installation of a Liquefied Natural Gasterminal will allow natural gas use to be re-established in Chile. The latest revision of the air qualitypollution prevention programme (2009) includes retrofitting particulate filters in new and old busesand trucks, a scrapping programme for older gasoline and diesel vehicles, introducing a morestringent emission standard for wood burning heaters, banning agricultural burns, and a cap andtrade system for SO 2 and NO X emissions from industry.According to Fuenzalida et al. [2006] who provided the first set of regional present andfuture climate scenarios using dynamical downscaling, the central part of Chile, where Santiago islocated, will see a 40% decline in precipitation, an increase in surface temperatures, and asouthward expansion of the subtropical high. These changes may in turn affect stability andventilation but these aspects were not addressed in this study. One can only speculate that theprobable southward expansion of the arid regime could intensify the radiatively driven circulation inthe Santiago basin, generating more summer like conditions, which are very favourable forphotochemical pollution. If the degree of centralization persists, the expected demographicscombined with a warmer climate may result in increased vulnerability [e.g., Bell et al., 2008].Santiago’s air quality has been subject to multiple studies since, at least, the early 1980’s.Over the years, the amount and the complexity of such studies have increased notoriously. Like inmany other cities in the world, research and management initiatives in Santiago were triggered byacute air pollution problems, in this case very high concentrations of inhalable particles (800 mg/m 3hourly averages in the late 1980’s) and associated respiratory problems that followed fromuncontrolled traffic and urban growth in the mid 70’s [e.g., Romero et al., 1999]. Therefore, theaccent of these initiatives has focused first on reducing extreme pollution events that areresponsible for acute effects and short-term air quality standards. Measures have focused on largeemitters: industries, non-catalytic cars, buses and trucks [e.g., Emmelin et al., 2007; Morales et al.,2006]. Such curbing measures could be identified based on relatively imprecise emissioninventories for criteria pollutants and simple receptor modelling approaches. However, as theattainment objectives become more ambitious (e.g., long-term air quality standards for dealing withaccumulative effects), the need of determining more subtle cost-effective measures and moreprecise tools increases. This, in turn, requires coordinated efforts to provide more of a systemicapproach [e.g., Molina and Molina, 2004].The number of active, highly qualified (PhD) researchers that can contribute to address airquality and climate issues is increasing but it is still insufficient. For instance, according to theChilean Academy of Science, in 2005 there were around 50 active scientists in the area ofanalytical and environmental chemistry, twice as many as in 1997 [Allende et al., 2005]. InAtmospheric Science, there are less than 20 active researchers at PhD level, and this number hasprobably tripled over the last decade. Up to now, the connection between policy making andresearch has been made based on short-term consultancies, which by construction hampers theestablishment of necessary synergies and the study of more complex issues. Hence, it appearsnecessary to create a research consortium able to convey scientists from different disciplines,combining natural and social science, which, in addition to scientific knowledge, is able to provideindependent opinions to environmental authorities. Such consortium could provide a platform forinternational collaboration and capacity building.159
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