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COMPLETE DOCUMENT (1862 kb) - OECD Nuclear Energy Agency

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Table II.22 Masses in wastes (kg/TWhe) *<br />

ISOTOPE OPEN MIX 1 MIX 2 FAST<br />

237 Np 1.67 0.0300 0.0318 0.00806<br />

238 Pu<br />

239 Pu<br />

240 Pu<br />

241 Pu<br />

242 Pu<br />

1.12<br />

14.1<br />

6.44<br />

3.44<br />

2.54<br />

0.00684<br />

0.0329<br />

0.0462<br />

0.00903<br />

0.0139<br />

0.00656<br />

0.0159<br />

0.0372<br />

0.00706<br />

0.0140<br />

0.00299<br />

0.0857<br />

0.0573<br />

0.00713<br />

0.00536<br />

Total Pu 27.7 0.109 0.0807 0.159<br />

241 Am<br />

242m Am<br />

243 Am<br />

1.09<br />

0.00271<br />

0.550<br />

0.0508<br />

6.0×10 -4<br />

0.0553<br />

0.0520<br />

0.00285<br />

0.0588<br />

0.0330<br />

0.00188<br />

0.0158<br />

Total Am 1.65 0.107 0.114 0.0507<br />

242 Cm<br />

243 Cm<br />

244 Cm<br />

245 Cm<br />

2.63×10 -5<br />

0.00325<br />

0.220<br />

0.0198<br />

2.89×10 -5<br />

0.00220<br />

0.0557<br />

0.00282<br />

2.39×10 -5<br />

0.00174<br />

0.0535<br />

0.00271<br />

1.85×10 -5<br />

0.00159<br />

0.0236<br />

0.00128<br />

Total Cm 0.243 0.0608 0.0580 0.0264<br />

Total actinides 31 0.31 0.29 0.24<br />

Total actinides without<br />

Cm recycling<br />

31 6.3 6.0 2.9<br />

* 1 GWe-year = 8.76 TWh<br />

4.3.1.6 Conclusions<br />

Assuming industrial and economic feasibility, it would theoretically be possible to reduce<br />

substantially the output of radiotoxic heavy nuclei associated with the supply electricity from a mixed<br />

reactor park composed of LWR-UO 2 , LWR-MOX and FRs.<br />

This can be done by separating the heavy nuclei from the wastes during spent fuel<br />

reprocessing and recycling all of them (reprocessed U, Pu and MAs) to the reactor. Equilibrium between<br />

production and consumption of TRUs would theoretically require a period corresponding to at least<br />

5 complete fuel cycles. Such a scenario requires the gradual build-up of a FR generating capacity of at<br />

least 20% i.e. 20 GWe, the equivalent of about 14 EFRs of 1 450 GWe each, in a 100 GWe reactor<br />

park.<br />

The only “wastes” to be stored definitively would be the fission products and the residues due<br />

to losses in reprocessing and fuel fabrication operations. However, analyses of multi-recycling MAs<br />

show that they do not all offer the same potential for reducing the radiotoxic inventory:<br />

• Neptunium is in fact easily separable and neptunium fuels would raise no fabrication<br />

problems in homogeneous mode. However, the irradiation of neptunium leads to the<br />

formation of Pu-238 which is detrimental to reprocessing. Moreover, no significant<br />

205

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