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William Angerer - Department of Physics and Astronomy - University ...

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76<br />

<strong>of</strong> :UN is deposited on the Ah03 substrate prior to deposition <strong>of</strong> GaN. The Al~ film<br />

serves as a buffer layer <strong>and</strong> facilitates nucleation <strong>of</strong> GaN on the substrate. All <strong>of</strong> our<br />

calculations <strong>of</strong> linear <strong>and</strong> nonlinear optical transmission <strong>and</strong> reflection approximate<br />

the GaN/AIN/Ah03 sample as a GaN/AI 2 0 3 sample. Using the reported values for<br />

the index <strong>of</strong> refraction <strong>of</strong> AIN [54] <strong>and</strong> the nonlinear susceptibility <strong>of</strong> AIN [55], we<br />

calculated that this simplified two film model introduces an error <strong>of</strong> less than l.-1o/c<br />

(6%) in the linear (nonlinear) transmission measurements as compared with the three<br />

slab model. Therefore, we are justified in ignoring the contribution <strong>of</strong> the thin .-\1,:\<br />

buffer layer in our calculations, <strong>and</strong> adopt the simpler model.<br />

4.1 Linear Measurement <strong>of</strong> Film Thicknesses<br />

Because linear spectroscopic measurements inherently encompass multiple interference.<br />

knowledge <strong>of</strong> the thin film thickness is required to determine the optical constants.<br />

In this section, I describe the theory <strong>and</strong> experimental techniques we used to<br />

determine the thickness <strong>of</strong> thin films grown on transparent substrates.<br />

4.1.1 Experimental Techniques<br />

The experimental apparatus used to measure thin film thickness is displayed in<br />

Fig. 4.1. The experiment consisted <strong>of</strong> measuring the reflection coefficient as a function<br />

<strong>of</strong> the angle between the GaN / Al 2 0 3 surface normal <strong>and</strong> the incident beam. The<br />

Reproduced with permission <strong>of</strong> the copyright owner. Further reproduction prohibited without permission.

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